Showing 1–50 of 75 results for author: Xiang, L

Dissipationless Photovoltaic Spin Hall Effect from Spin-current Vorticity

Authors: Longjun Xiang, Jian Wang

Abstract: Spin-current vorticity (SCV) can generate the linear magnetic spin Hall effect [\href{https://doi.org/10.1038/s41586-018-0853-0}{Nature \textbf{565}, 627 (2019)}], yet its role in nonlinear spin Hall transport has been much less explored. Here, we show that, under a dc electric field, SCV can deflect optically excited electrons to drive a dissipationless photovoltaic spin Hall effect (PSHE), in wh… ▽ More Spin-current vorticity (SCV) can generate the linear magnetic spin Hall effect [\href{https://doi.org/10.1038/s41586-018-0853-0}{Nature \textbf{565}, 627 (2019)}], yet its role in nonlinear spin Hall transport has been much less explored. Here, we show that, under a dc electric field, SCV can deflect optically excited electrons to drive a dissipationless photovoltaic spin Hall effect (PSHE), in which optical excitation by circularly and linearly polarized light is governed by the Berry curvature and quantum metric, respectively. Because the Berry curvature is $\mathcal{T}$-odd whereas the quantum metric is $\mathcal{T}$-even, their respective combinations with the $\mathcal{T}$-odd SCV give rise to $\mathcal{T}$-even and $\mathcal{T}$-odd PSHEs, where $\mathcal{T}$ denotes time-reversal symmetry. Remarkably, we find that the spin current of the $\mathcal{T}$-even PSHE can be reversed by switching the light helicity, as illustrated in monolayer WTe$_2$. By contrast, the $\mathcal{T}$-odd PSHE in altermagnets changes sign upon Néel-vector reversal, as demonstrated in a $d$-wave altermagnetic model. Beyond the PSHE, we show that the SCV dipole governs both the Drude and intrinsic nonlinear spin Hall effects proposed recently. Our results reveal two switchable spin Hall mechanisms and establish SCV as a unifying concept for understanding dissipationless nonlinear spin Hall transport. △ Less

Submitted 13 August, 2026; originally announced August 2026.

Comments: Three figures

Hyperuniform charge distributions and phase transitions in a generalized Aubry-André model

Authors: Lujia Xiang, Junmo Jeon, Shiro Sakai

Abstract: We show the existence of distinct inhomogeneous charge distributions and a phase transition between them in aperiodic fermion systems. Using a generalized Aubry-André model as an example, we obtain various types of charge distributions, which we classify by means of hyperuniformity, a general mean to quantify and classify the global uniformity of spatial distributions. Examining various cases of f… ▽ More We show the existence of distinct inhomogeneous charge distributions and a phase transition between them in aperiodic fermion systems. Using a generalized Aubry-André model as an example, we obtain various types of charge distributions, which we classify by means of hyperuniformity, a general mean to quantify and classify the global uniformity of spatial distributions. Examining various cases of filling fraction and potential strength and shape, we find that the many-body charge distribution in this model is always hyperuniform, i.e., showing an anomalously suppressed long-range fluctuation, while its hyperuniformity class depends on the localization properties of the states around the Fermi energy, irrespective of those of high-energy states. Namely, the change in the localization properties of these single-particle states leaves a signature in the hyperuniformity class of many-body charge distribution. We further show a change of the hyperuniformity class corresponds to a phase transition between inhomogeneous many-body states, and that it is of the third order. △ Less

Submitted 16 June, 2026; originally announced June 2026.

Comments: 12 pages, 9 figures

Third-order intrinsic anomalous Hall effect as a transport fingerprint of altermagnets

Authors: Longjun Xiang, Hao Jin, Jian Wang

Abstract: The intrinsic anomalous Hall effect (IAHE) provides a powerful transport fingerprint of quantum magnets, with its linear and second-order responses distinguishing ferromagnets and $\mathcal{P}\mathcal{T}$-symmetric antiferromagnets, respectively. Altermagnets, as an emergent class of quantum magnets, have recently been shown to host a third-order extrinsic anomalous Hall effect, raising a question… ▽ More The intrinsic anomalous Hall effect (IAHE) provides a powerful transport fingerprint of quantum magnets, with its linear and second-order responses distinguishing ferromagnets and $\mathcal{P}\mathcal{T}$-symmetric antiferromagnets, respectively. Altermagnets, as an emergent class of quantum magnets, have recently been shown to host a third-order extrinsic anomalous Hall effect, raising a question of whether an \textit{intrinsic} counterpart can serve as a diagnostic of altermagnetic order. Based on spin-group symmetry analysis, we demonstrate that the third-order IAHE is generically allowed in the ten spin Laue groups relevant to altermagnets when spin-orbit coupling (SOC) is taken into account. By combining these symmetry constraints with the anomalous velocity induced by the second-order Berry curvature, we uncover a resonant third-order IAHE arising near the altermagnetic band crossings at generic momenta in both the Lieb-lattice altermagnet and the experimentally realized altermagnet V$_2$Se$_2$O. Notably, we identify the Berry curvature quadrupole, encoded in the second-order Berry curvature and activated by finite SOC, as the microscopic quantum geometric origin of this resonance. Our results establish the third-order IAHE as an intrinsic quantum geometric transport fingerprint of altermagnets and extend the hierarchy of IAHE across collinear quantum magnets. △ Less

Submitted 29 April, 2026; originally announced April 2026.

Comments: Four figures

Dual Quantum Geometric Tensors and Local Topological Invariant

Authors: Rongjie Cui, Longjun Xiang, Fuming Xu, Jian Wang

Abstract: The conventional quantum geometric tensor (QGT) is Hermitian, with a real symmetric quantum metric and an imaginary antisymmetric Berry curvature. We show that the Zeeman QGT is generically non-Hermitian and admits a natural decomposition into normal and anomalous metric-curvature sectors. The normal sector reduces to the conventional Hermitian structure, whereas the anomalous sector contains an i… ▽ More The conventional quantum geometric tensor (QGT) is Hermitian, with a real symmetric quantum metric and an imaginary antisymmetric Berry curvature. We show that the Zeeman QGT is generically non-Hermitian and admits a natural decomposition into normal and anomalous metric-curvature sectors. The normal sector reduces to the conventional Hermitian structure, whereas the anomalous sector contains an imaginary symmetric metric-like tensor and a real antisymmetric curvature-like tensor with no counterpart in the standard QGT. In a two-dimensional Dirac system, the anomalous Zeeman curvature develops a radial flux singularity that is Hodge-dual to the tangential winding field of the Dirac node. This recasts the same local $π_1$ topology into a curvature-flux language, analogous to the flux representation of global $π_2$ topology by the conventional Berry curvature. At the level of linear response, the four symmetry-resolved components of the gyrotropic conductivity are in one-to-one correspondence with the four components of the Zeeman QGT, while their distinct low-frequency scalings provide an additional diagnostic for isolating the underlying geometric sector. The reciprocal kinetic magnetoelectric response offers a complementary experimental route to probe the same structure. These results establish a unified framework connecting non-Hermitian Zeeman quantum geometry, local Dirac-node topology, and measurable transport signatures. △ Less

Submitted 28 April, 2026; v1 submitted 9 April, 2026; originally announced April 2026.

Comments: revised manuscript

Granular Superconductivity in La$_{2}$PrNi$_{2}$O$_{7-δ}$ Thin Films

Authors: Ziao Han, Lifen Xiang, X. J. Zhou, Zhihai Zhu

Abstract: Superconductivity realized in bilayer nickelate thin films enables direct spectroscopic and transport studies at ambient pressure. However, a persistent two-step resistive transition remains a major barrier to achieving optimal superconducting properties. Here, we show that the two-step transition in La$_2$PrNi$_2$O$_{7-δ}$ thin films originates from the granular nature of superconductivity, speci… ▽ More Superconductivity realized in bilayer nickelate thin films enables direct spectroscopic and transport studies at ambient pressure. However, a persistent two-step resistive transition remains a major barrier to achieving optimal superconducting properties. Here, we show that the two-step transition in La$_2$PrNi$_2$O$_{7-δ}$ thin films originates from the granular nature of superconductivity, specifically, the coexistence of two distinct superconducting grain phases coupled by a Josephson junction network. A secondary, lower-temperature transition appears in the $R(T)$ curve, even when residual resistance becomes vanishingly small near 30 K. This two-step behavior significantly lowers the zero-resistance transition temperature, $T_{c, zero}$$\approx$ 10 K, and limits advanced spectroscopic studies. Our findings reveal the microscopic mechanism underlying the two-step transition in thin films and underscore the need for improved oxygen homogeneity to achieve bulk superconductivity in this system. △ Less

Submitted 9 April, 2026; originally announced April 2026.

Flat-Band Generation in InAs/GaSb Quantum Wells through Vertically Engineered Heterostructures

Authors: Zachery A. Enderson, Jiyuan Fang, Wei-Chen Wang, Li Xiang, Mykhaylo Ozerov, Dmitry Smirnov, Zhigang Jiang, Samuel D. Hawkins, Aaron J. Muhowski, John F. Klem, Wei Pan

Abstract: Quantum materials constitute a novel category of substances wherein quantum effects and electron-electron (e-e) interactions give rise to unforeseen phenomena on a macroscopic scale. Of particular interest within the realm of quantum materials are flat bands, which promote heavy conduction electrons and enhance e-e correlation effects. While the engineering of such flat bands has been demonstrated… ▽ More Quantum materials constitute a novel category of substances wherein quantum effects and electron-electron (e-e) interactions give rise to unforeseen phenomena on a macroscopic scale. Of particular interest within the realm of quantum materials are flat bands, which promote heavy conduction electrons and enhance e-e correlation effects. While the engineering of such flat bands has been demonstrated in graphene and two-dimensional transition metal dichalcogenides moiré superlattices and in lithography defined semiconductor moiré superlattices, conventional tear-and-stack fabrication methods face challenges due to inevitable twist-angle disorder, strain, and relaxation effects, leading to issues with reproducibility and scalability. Here, we explore the creation and modification of flat bands through vertically engineered III-V semiconductor heterostructures, without the need for twisting. These artificial quantum materials offer a reproducible and scalable means for producing high-quality flat-band materials via molecular beam epitaxy growth. Our investigation includes magnetotransport and infrared magneto-spectroscopy studies of quad-layer InAs/GaSb quantum wells, accompanied by k*p band structure calculations, which illustrate the flattening of bands in vertically designed heterostructures. △ Less

Submitted 26 March, 2026; v1 submitted 16 March, 2026; originally announced March 2026.

Comments: 12 pages, 6 figures

Quantum Geometric Entropy Production and Entropy Hall Effect

Authors: Longjun Xiang, Jinxiong Jia, Jian Wang

Abstract: Quantum geometry, encoded in the Berry curvature and quantum metric, has unified diverse anomalous transport phenomena in solids, yet a microscopic quantum-geometric theory of entropy transport for Bloch electrons is still lacking. We formulate an entropy continuity equation for noninteracting fermions driven by an electric field, starting from the von Neumann entropy, and obtain quantum-mechanica… ▽ More Quantum geometry, encoded in the Berry curvature and quantum metric, has unified diverse anomalous transport phenomena in solids, yet a microscopic quantum-geometric theory of entropy transport for Bloch electrons is still lacking. We formulate an entropy continuity equation for noninteracting fermions driven by an electric field, starting from the von Neumann entropy, and obtain quantum-mechanical expressions for the entropy current density and entropy production rate. Introducing relaxation through a relaxation-time dissipator, we identify the quantum metric as the origin of the leading entropy production, providing a direct microscopic diagnostic of dissipation in both the extrinsic Drude response and an intrinsic nonlinear Ohmic contribution controlled by quantum metric. We further predict an entropy Hall effect arising from the Berry curvature and show that it obeys an Onsager reciprocal relation with the anomalous Nernst effect under a temperature gradient. Finally, we establish universal relations connecting entropy and charge currents under DC and AC driving, offering experimentally accessible probes of quantum geometry through nonequilibrium entropy flow. △ Less

Submitted 2 February, 2026; originally announced February 2026.

Field-induced magnetic phase transition driven by a ground state level-crossing in CsErSe$_2$

Authors: Hope Whitelock, Allen O. Scheie, Marissa McMaster, Ian A. Leahy, Li Xiang, Mykhaylo Ozerov, Dmitry Smirnov, Eun Sang Choi, C. dela Cruz, M. O. Ajeesh, Eliana S. Krakovsky, Daniel A. Rehn, Jie Xing, Athena S. Sefat, Minhyea Lee

Abstract: We report a comprehensive study of the low-temperature magnetic properties of the insulating rare-earth triangular magnet CsErSe$_2$. We uncover a field-induced level crossing at the crystal electric field (CEF) ground state, which gives rise to a first order phase transition as well as to distinctive magnetic properties. This crossing is identified by the accurate determination of the single-ion… ▽ More We report a comprehensive study of the low-temperature magnetic properties of the insulating rare-earth triangular magnet CsErSe$_2$. We uncover a field-induced level crossing at the crystal electric field (CEF) ground state, which gives rise to a first order phase transition as well as to distinctive magnetic properties. This crossing is identified by the accurate determination of the single-ion Hamiltonian, the reliability of which is substantially enhanced by field-dependent optical spectroscopy that directly tracks the Zeeman splittings of Kramers doublets. We also observe spontaneous antiferromagnetic ordering in CsErSe$_2$ below $T_N \approx 110$ mK, and resolve the corresponding magnetic structure using elastic neutron scattering. We discuss how the rich magnetic behavior of CsErSe$_2$ arises from the interplay of non-trivial field-dependent single-ion physics and spontaneous ordering, and highlight the implications of these results for understanding magnetic phenomena across a wide range of insulating rare-earth magnets. △ Less

Submitted 6 August, 2026; v1 submitted 24 October, 2025; originally announced October 2025.

Comments: 12 pages, 7 figures, title and abstract updated. Major revision in the main text

Quantum geometric map of magnetotransport

Authors: Longjun Xiang, Jinxiong Jia, Fuming Xu, Jian Wang

Abstract: We propose a quantum geometric map for the magnetononlinear Hall effect (MNHE), the planar Hall effect (PHE), and the ordinary Hall effect (OHE). These magnetotransport phenomena originate from the bilinear charge current of Bloch electrons in electromagnetic fields, incorporating both spin Zeeman coupling and orbital minimal coupling to the applied magnetic field. Benchmarked against Onsager reci… ▽ More We propose a quantum geometric map for the magnetononlinear Hall effect (MNHE), the planar Hall effect (PHE), and the ordinary Hall effect (OHE). These magnetotransport phenomena originate from the bilinear charge current of Bloch electrons in electromagnetic fields, incorporating both spin Zeeman coupling and orbital minimal coupling to the applied magnetic field. Benchmarked against Onsager reciprocity, we demonstrate that the spin- and orbital-induced MNHEs are governed by the time-reversal-even Zeeman quantum metric dipole and conventional quantum metric quadrupole, respectively; the spin- and orbital-induced PHEs are dominated by the time-reversal-odd Zeeman Berry curvature dipole and conventional Berry curvature quadrupole, respectively. We further show that the OHE contains an interband contribution that is related to the quantum metric quadrupole, contrary to conventional wisdom. Navigated by this map, we study the previously unexplored spin-induced PHE in the surface Dirac cone of topological insulators, where we uncover a step-like PHE. Our work offers a unified quantum geometric framework for understanding magnetotransport experiments. △ Less

Submitted 16 April, 2026; v1 submitted 2 October, 2025; originally announced October 2025.

Comments: Compared to the old version, this updated version has undergone significant changes to more clearly state the key results. In addition, the Onsager reciprocal relation on EB current response is added

Journal ref: Phys. Rev. B 113, L201406 (2026)

Stabilizing and Tuning Superconductivity in La$_3$Ni$_2$O$_{7-δ}$ Films: Oxygen Recycling Protocol Reveals Hole-Doping Analogue

Authors: Lifen Xiang, Siyi Lei, Xiaolin Ren, Ziao Han, Zijian Xu, X. J. Zhou, Zhihai Zhu

Abstract: The recent achievement of superconductivity in La$_3$Ni$_2$O$_{7-δ}$ with transition temperatures exceeding 40 K in thin films under compressive strain and 80 K in bulk crystals under high pressure opens new avenues for research on high-temperature superconductivity. The realization of superconductivity in thin films requires delicate control of growth conditions, which presents significant challe… ▽ More The recent achievement of superconductivity in La$_3$Ni$_2$O$_{7-δ}$ with transition temperatures exceeding 40 K in thin films under compressive strain and 80 K in bulk crystals under high pressure opens new avenues for research on high-temperature superconductivity. The realization of superconductivity in thin films requires delicate control of growth conditions, which presents significant challenges in the synthesis process. Furthermore, the stability of superconducting La$_3$Ni$_2$O$_{7-δ}$ films is compromised by oxygen loss, which complicates their characterization. We introduce an effective recycling protocol that involves oxygen removal in a precursor phase followed by ozone-assisted annealing, which restores superconducting properties. By tuning the oxygen content, we construct an electronic phase diagram that highlights oxygen addition as a potential analogue to hole doping via La substitution with Sr, providing insights into the doping mechanism and guiding future material optimization. △ Less

Submitted 16 January, 2026; v1 submitted 15 August, 2025; originally announced August 2025.

Journal ref: Phys. Rev. B 113, 104522(2026)

Nonlinear Magnetoelectric Edelstein Effect

Authors: Jinxiong Jia, Longjun Xiang, Zhenhua Qiao, Jian Wang

Abstract: The linear Edelstein effect is a cornerstone phenomenon in spintronics that describes the generation of spin magnetization in response to an applied electric field. Recent theoretical advances have reignited interest in its nonlinear counterpart, the nonlinear Edelstein effect, in which spin magnetization is induced by a second-order electric field. However, the intrinsic contribution to both effe… ▽ More The linear Edelstein effect is a cornerstone phenomenon in spintronics that describes the generation of spin magnetization in response to an applied electric field. Recent theoretical advances have reignited interest in its nonlinear counterpart, the nonlinear Edelstein effect, in which spin magnetization is induced by a second-order electric field. However, the intrinsic contribution to both effects is generally forbidden in systems preserving time-reversal symmetry ($\mathcal{T}$) or composite symmetries such as $\mathcal{T}τ_{1/2}$, where $τ_{1/2}$ denotes a half-lattice translation. In such systems, spin magnetization typically emerges either from extrinsic mechanisms but limited to metals due to their Fermi-surface property, or from dynamical electric fields with a terahertz driving frequency. Here, we propose a new mechanism for spin magnetization, arising from the interplay of magnetic and electric fields, termed the nonlinear magnetoelectric Edelstein effect. Remarkably, its intrinsic component, determined purely by the material's band structure, can appear even in $\mathcal{T}$-invariant materials, but lacking inversion symmetry ($\mathcal{P}$), including insulators. On the other hand, we illustrate that its extrinsic component can serve as a sensitive indicator of the Néel vector reversal in $\mathcal{P}\mathcal{T}$-symmetric antiferromagnetic materials, offering a novel route for antiferromagnetic order detection. To validate our theory, we perform explicit calculations using a two-band Dirac model and a tight-binding model on a honeycomb lattice, finding that both effects yield sizable spin magnetization. Our findings establish the nonlinear magnetoelectric Edelstein effect as a versatile platform for both exploring nonlinear spin physics and enabling symmetry-based detection of antiferromagnetic order. △ Less

Submitted 31 July, 2025; originally announced July 2025.

Journal ref: Phys. Rev. Lett. 136, 226302 (2026)

Lithography defined semiconductor moires with anomalous in-gap quantum Hall states

Authors: Wei Pan, D. Bruce Burckel, Catalin D. Spataru, Keshab R. Sapkota, Aaron J. Muhowski, Samuel D. Hawkins, John F. Klem, Layla S. Smith, Doyle A. Temple, Zachery A. Enderson, Zhigang Jiang, Komalavalli Thirunavukkuarasu, Li Xiang, Mykhaylo Ozerov, Dmitry Smirnov, Chang Niu, Peide D. Ye, Praveen Pai, Fan Zhang

Abstract: Quantum materials and phenomena have attracted great interest for their potential applications in next-generation microelectronics and quantum-information technologies. In one especially interesting class of quantum materials, moire superlattices (MSL) formed by twisted bilayers of 2D materials, a wide range of novel phenomena are observed. However, there exist daunting challenges such as reproduc… ▽ More Quantum materials and phenomena have attracted great interest for their potential applications in next-generation microelectronics and quantum-information technologies. In one especially interesting class of quantum materials, moire superlattices (MSL) formed by twisted bilayers of 2D materials, a wide range of novel phenomena are observed. However, there exist daunting challenges such as reproducibility and scalability of utilizing 2D MSLs for microelectronics and quantum technologies due to their exfoliate-tear-stack method. Here, we propose lithography defined semiconductor moires superlattices, in which three fundamental parameters, electron-electron interaction, spin-orbit coupling, and band topology, are designable. We experimentally investigate quantum transport properties in a moire specimen made in an InAs quantum well. Strong anomalous in-gap states are observed within the same integer quantum Hall state. Our work opens up new horizons for studying 2D quantum-materials phenomena in semiconductors featuring superior industry-level quality and state-of-the-art technologies, and they may potentially enable new quantum information and microelectronics technologies. △ Less

Submitted 6 June, 2025; originally announced June 2025.

Comments: published by Nano Letters

Unconventional Hall Effect in Gapless Superconductors: Transverse Supercurrent Converted from Normal Current

Authors: Miaomiao Wei, Longjun Xiang, Fuming Xu, Bin Wang, Jian Wang

Abstract: A normal metallic system proximitized by a superconductor can exhibit a gapless superconducting state characterized by segmented Fermi surfaces, as confirmed experimentally. In such a state, quasiparticle states remain gapless along one direction, while a superconducting gap opens in the perpendicular direction. This anisotropy enables a novel Hall effect in gapless superconductors, termed the sup… ▽ More A normal metallic system proximitized by a superconductor can exhibit a gapless superconducting state characterized by segmented Fermi surfaces, as confirmed experimentally. In such a state, quasiparticle states remain gapless along one direction, while a superconducting gap opens in the perpendicular direction. This anisotropy enables a novel Hall effect in gapless superconductors, termed the superconducting Hall effect (ScHE), where a longitudinal normal current carried by quasiparticles is converted into a dissipationless transverse supercurrent. Employing both the thermodynamic approach for bulk systems and quantum transport theory for a four-probe setup, we demonstrate the existence of this effect and reveal its intrinsic origin as the quasiparticle Berry curvature. The predicted ScHE can be experimentally verified via the standard angular-dependent Hall measurements performed on gapless superconductors. △ Less

Submitted 29 May, 2025; originally announced May 2025.

Comments: 6 pages, 3 figures

Mechanical resonant sensing of spin texture dynamics in a two-dimensional antiferromagnet

Authors: S M Enamul Hoque Yousuf, Yunong Wang, Shreyas Ramachandran, John Koptur-Palenchar, Chiara Tarantini, Li Xiang, Stephen McGill, Dmitry Smirnov, Elton J. G. Santos, Philip X. -L. Feng, Xiao-Xiao Zhang

Abstract: The coupling between the spin degrees of freedom and macroscopic mechanical motions, including striction, shearing, and rotation, has attracted wide interest with applications in actuation, transduction, and information processing. Experiments so far have established the mechanical responses to the long-range ordered or isolated single spin states. However, it remains elusive whether mechanical mo… ▽ More The coupling between the spin degrees of freedom and macroscopic mechanical motions, including striction, shearing, and rotation, has attracted wide interest with applications in actuation, transduction, and information processing. Experiments so far have established the mechanical responses to the long-range ordered or isolated single spin states. However, it remains elusive whether mechanical motions can couple to a different type of magnetic structure, the non-collinear spin textures, which exhibit nanoscale spatial variations of spin (domain walls, skyrmions, etc.) and are promising candidates to realize high-speed computing devices. Here, we report the detection of collective spin texture dynamics with nanoelectromechanical resonators made of two-dimensional antiferromagnetic (AFM) MnPS3 with $10^{-9}$ strain sensitivity. By examining radio frequency mechanical oscillations under magnetic fields, new magnetic transitions were identified with sharp dips in resonant frequency. They are attributed to the collective AFM domain wall motions as supported by the analytical modeling of magnetostriction and large-scale spin-dynamics simulations. Additionally, an abnormally large modulation in the mechanical nonlinearity at the transition field infers a fluid-like response due to the ultrafast domain motion. Our work establishes a strong coupling between spin texture and mechanical dynamics, laying the foundation for electromechanical manipulation of spin texture and developing quantum hybrid devices. △ Less

Submitted 14 March, 2025; originally announced March 2025.

Light-induced thermal noise \textit{anomaly} governed by quantum metric

Authors: Longjun Xiang, Lei Zhang, Jun Chen, Fuming Xu, Yadong Wei, Jian Wang

Abstract: Traditionally, thermal noise in electric currents, arising from thermal agitation, is expected to increase with temperature $T$ and disappear as $T$ approaches zero. Contrary to this expectation, we discover that the resonant DC thermal noise (DTN) in photocurrents not only persists at $T=0$ but also exhibits a divergence proportional to $1/T$. This thermal noise \textit{anomaly} arises from the u… ▽ More Traditionally, thermal noise in electric currents, arising from thermal agitation, is expected to increase with temperature $T$ and disappear as $T$ approaches zero. Contrary to this expectation, we discover that the resonant DC thermal noise (DTN) in photocurrents not only persists at $T=0$ but also exhibits a divergence proportional to $1/T$. This thermal noise \textit{anomaly} arises from the unique electron-photon interactions near the Fermi surface, manifesting as the interplay between the inherent Fermi-surface property and the resonant optical selection rules of DTN, and thereby represents an unexplored noise regime. Notably, we reveal that this \textit{anomalous} DTN, especially in time-reversal-invariant systems, is intrinsically linked to the quantum metric. We illustrate this \textit{anomalous} DTN in massless Dirac materials, including two-dimensional graphene, the surfaces of three-dimensional topological insulators, and three-dimensional Weyl semimetals, where the quantum metric plays a pivotal role. Finally, we find that the total noise spectrum at low temperatures, which includes both the DC shot noise and the \textit{anomalous} DTN, will universally peak at $ω_p=2|μ|$ with $ω_p$ the frequency of light and $μ$ the chemical potential of the bulk crystals. △ Less

Submitted 17 December, 2024; originally announced December 2024.

Light-Induced Electron Pairing in a Bilayer Structure

Authors: Qiaochu Wan, Daniel Vaz, Li Xiang, Anshul Ramavath, Brandon Vargo, Juntong Ye, Jonathan Beaumariage, Kenji Watanabe, Takashi Taniguchi, Zheng Sun, Dmitry Smirnov, Nathan Youngblood, Igor V. Bondarev, David W. Snoke

Abstract: Previous experimental and theoretical work has given evidence of the existence of doubly charged exciton states in strongly screened bilayers of transition metal dichalcogenide (TMD) layers. These complexes are important because they are performed electron pairs that can, in principle, undergo Bose-Einstein condensation (BEC), in which case they would also form a new type of superconductor, consis… ▽ More Previous experimental and theoretical work has given evidence of the existence of doubly charged exciton states in strongly screened bilayers of transition metal dichalcogenide (TMD) layers. These complexes are important because they are performed electron pairs that can, in principle, undergo Bose-Einstein condensation (BEC), in which case they would also form a new type of superconductor, consisting of stable bosons with net charges. In this paper, we present key electrostatic and magnetic measurements that definitively confirm the existence of these charged bosons. These measurements include 1) continuous control of the doping density with both positive and negative carriers, showing the expected population dependencies on the free carrier density, and 2) measurement of the dependence on the magnetic field, showing that this new bound state is a spin triplet. These results imply that it is promising to look for BEC and superconductivity in this system. △ Less

Submitted 12 December, 2024; v1 submitted 9 December, 2024; originally announced December 2024.

Comments: 16 pages, 10 figures

Pseudo-Riemannian metric: a new perspective on the quantum realm

Authors: Miaomiao Wei, Longjun Xiang, Fuming Xu, Baigeng Wang, Jian Wang

Abstract: As a fundamental concept in condensed matter physics, quantum geometry within the Riemannian metric elucidates various exotic phenomena, including the Hall effects driven by Berry curvature and quantum metric. In this work, we propose novel quantum geometries within a pseudo-Riemannian framework to explore unique characteristic of quantum matter. By defining distinct distances on pseudo-Riemannian… ▽ More As a fundamental concept in condensed matter physics, quantum geometry within the Riemannian metric elucidates various exotic phenomena, including the Hall effects driven by Berry curvature and quantum metric. In this work, we propose novel quantum geometries within a pseudo-Riemannian framework to explore unique characteristic of quantum matter. By defining distinct distances on pseudo-Riemannian manifolds and incorporating spin degree of freedom, we introduce the Pauli quantum geometric tensor. The imaginary part of this tensor corresponds to the Pauli Berry curvature, leading to the discovery a novel quantum phase: Pauli semimetal in PT-symmetric systems. This phase, characterized by the topological Pauli Chern number, manifests as a two-dimensional Pauli Chern insulator with helical edge states. These topological phases, uniquely revealed by the Pauli-Riemannian metric, go beyond the familiar Riemannian metric, where Berry curvature vanishes due to PT-symmetry. Pauli Chern number can classify helical topological insulator with or without time reversal symmetry. Pseudo-Riemannian metrics offer new insights into quantum materials and extend the scope of quantum geometry. △ Less

Submitted 29 September, 2024; originally announced September 2024.

Quantum intrinsic ${\cal T}$-odd spin Hall effect in altermagnets

Authors: Miaomiao Wei, Longjun Xiang, Fuming Xu, Baigeng Wang, Jian Wang

Abstract: Drude weight, historically associated with the longitudinal Drude conductivity, can be generalized to describe the transverse or Hall component of the extrinsic conductivity tensor. In particular, transverse Drude weights, such as band geometric quantities Berry curvature dipole and spin vorticity, manifest themselves through the \textit{extrinsic} second-order nonlinear Hall effect and \textit{ex… ▽ More Drude weight, historically associated with the longitudinal Drude conductivity, can be generalized to describe the transverse or Hall component of the extrinsic conductivity tensor. In particular, transverse Drude weights, such as band geometric quantities Berry curvature dipole and spin vorticity, manifest themselves through the \textit{extrinsic} second-order nonlinear Hall effect and \textit{extrinsic} linear spin Hall effect (SHE) in diffusive transport, respectively. In this work, we uncover a new class of intrinsic Hall effects in quantum transport regime, termed as quantum intrinsic Hall effect (QIHE), which is the manifestation of system symmetry through intrinsic transport phenomena. For a given Hamiltonian, its transport characteristics can be revealed either intrinsically through QIHE in ballistic regime or extrinsically via the transverse Drude weight in diffusive transport, where both intrinsic and extrinsic effects share the same salient transport features governed by symmetry of the Hamiltonian. The physical origin of QIHE is attributed to quantum boundary scattering of the measurement setup that respects the system symmetry, as exemplified by the contact resistance of a two-terminal ballistic conductor. We demonstrate our finding by studying the quantum ${\cal T}$-odd ($\mathcal{T}$, time-reversal) SHE in altermagnets. Our work paves a way towards the quantum transport manifestation of band geometric characteristics. △ Less

Submitted 8 September, 2024; originally announced September 2024.

Quantum highway: Observation of minimal and maximal speed limits for few and many-body states

Authors: Zitian Zhu, Lei Gao, Zehang Bao, Liang Xiang, Zixuan Song, Shibo Xu, Ke Wang, Jiachen Chen, Feitong Jin, Xuhao Zhu, Yu Gao, Yaozu Wu, Chuanyu Zhang, Ning Wang, Yiren Zou, Ziqi Tan, Aosai Zhang, Zhengyi Cui, Fanhao Shen, Jiarun Zhong, Tingting Li, Jinfeng Deng, Xu Zhang, Hang Dong, Pengfei Zhang , et al. (8 additional authors not shown)

Abstract: Tracking the time evolution of a quantum state allows one to verify the thermalization rate or the propagation speed of correlations in generic quantum systems. Inspired by the energy-time uncertainty principle, bounds have been demonstrated on the maximal speed at which a quantum state can change, resulting in immediate and practical tasks. Based on a programmable superconducting quantum processo… ▽ More Tracking the time evolution of a quantum state allows one to verify the thermalization rate or the propagation speed of correlations in generic quantum systems. Inspired by the energy-time uncertainty principle, bounds have been demonstrated on the maximal speed at which a quantum state can change, resulting in immediate and practical tasks. Based on a programmable superconducting quantum processor, we test the dynamics of various emulated quantum mechanical systems encompassing single- and many-body states. We show that one can test the known quantum speed limits and that modifying a single Hamiltonian parameter allows the observation of the crossover of the different bounds on the dynamics. We also unveil the observation of minimal quantum speed limits in addition to more common maximal ones, i.e., the lowest rate of change of a unitarily evolved quantum state. Our results establish a comprehensive experimental characterization of quantum speed limits and pave the way for their subsequent study in engineered non-unitary conditions. △ Less

Submitted 21 August, 2024; originally announced August 2024.

Comments: 9 pages,4 figures + supplementary information

Spin transport revealed by the spin quantum geometry

Authors: Longjun Xiang, Hao Jin, Jian Wang

Abstract: We present the framework of \textit{spin quantum geometry}, which is fundamentally linked to the spin degree of freedom of Bloch electrons and incorporates both the spin quantum geometric tensor (QGT) and the recently introduced Zeeman QGT, to elucidate the spin transport. We show that the spin and Zeeman QGTs, respectively, provide a unified framework for revealing known spin currents, such as th… ▽ More We present the framework of \textit{spin quantum geometry}, which is fundamentally linked to the spin degree of freedom of Bloch electrons and incorporates both the spin quantum geometric tensor (QGT) and the recently introduced Zeeman QGT, to elucidate the spin transport. We show that the spin and Zeeman QGTs, respectively, provide a unified framework for revealing known spin currents, such as the intrinsic spin Hall effect, and spin magnetization, such as the Edelstein effect, of Bloch electrons under an electric field. In addition, we predict the linear displacement spin Hall effect, wherein an AC electric field induces a transverse spin current in insulating systems. Furthermore, we propose two novel nonlinear spin responses: the nonlinear Drude spin current (NDSC) and the nonlinear Drude spin magnetization (NDSM), both of which exhibit a quadratic dependence on the relaxation time, like the nonlinear Drude charge current, and are governed by the \textit{spin quantum geometry}. Finally, we evaluate the NDSC and NDSM with Dirac models of topological insulators and find that, in the moderately dirty regime, the NDSC and NDSM can exceed their respective nonlinear intrinsic counterparts, which have recently garnered significant interest in spintronics. △ Less

Submitted 4 August, 2025; v1 submitted 4 June, 2024; originally announced June 2024.

Comments: We rewrite the drfact with the concept of spin quantum geometry. Any comments are welcome

Equivalence of semiclassical and response theories for second-order nonlinear ac Hall effects

Authors: Jinxiong Jia, Longjun Xiang, Zhenhua Qiao, Jian Wang

Abstract: It has been known that the semiclassical theory and the response theory can equivalently give the Drude and the intrinsic anomalous Hall conductivities in the linear order of electric field. However, recent theoretical advances implied that the second-order nonlinear conductivities calculated with both approaches are no longer equivalent, which leads to various experimental explanations even in a… ▽ More It has been known that the semiclassical theory and the response theory can equivalently give the Drude and the intrinsic anomalous Hall conductivities in the linear order of electric field. However, recent theoretical advances implied that the second-order nonlinear conductivities calculated with both approaches are no longer equivalent, which leads to various experimental explanations even in a similar experimental setup conducted in \href{https://www.science.org/doi/10.1126/science.adf1506}{[\textit{Science \textbf{381}, 181 (2023)}]} and \href{https://www.nature.com/articles/s41586-023-06363-3}{[\textit{Nature \textbf{621}, 487 (2023)}]}, respectively. Herein, by extending the AC semiclassical theory up to the second order of electric field, we show that the semiclassical theory is still equivalent to the response theory in the second order of electric field when the relaxation is taken into account on the same footing. In particular, we show that the familiar second-order nonlinear current responses, including the nonlinear Drude current and the Berry curvature (quantum metric) dipole driven extrinsic (intrinsic) nonlinear Hall current, can be derived by both approaches. Further, we show that the quantum-corrected intrinsic nonlinear longitudinal current, as recently proposed by the response theory or in a similar manner, can also be reproduced by the semiclassical theory. Beyond those known second-order current responses, with both approaches, we uncover two previously overlooked nonlinear displacement currents unique to the AC electric field. As a consequence of this equivalence,... △ Less

Submitted 6 December, 2024; v1 submitted 25 April, 2024; originally announced April 2024.

Comments: published in Physical Review B

A predictive machine learning force field framework for liquid electrolyte development

Authors: Sheng Gong, Yumin Zhang, Zhenliang Mu, Zhichen Pu, Hongyi Wang, Zhiao Yu, Mengyi Chen, Tianze Zheng, Zhi Wang, Lifei Chen, Zhenze Yang, Xiaojie Wu, Shaochen Shi, Weihao Gao, Wen Yan, Liang Xiang

Abstract: Despite the widespread applications of machine learning force fields (MLFF) in solids and small molecules, there is a notable gap in applying MLFF to simulate liquid electrolyte, a critical component of the current commercial lithium-ion battery. In this work, we introduce BAMBOO (\textbf{B}yteDance \textbf{A}I \textbf{M}olecular Simulation \textbf{Boo}ster), a predictive framework for molecular d… ▽ More Despite the widespread applications of machine learning force fields (MLFF) in solids and small molecules, there is a notable gap in applying MLFF to simulate liquid electrolyte, a critical component of the current commercial lithium-ion battery. In this work, we introduce BAMBOO (\textbf{B}yteDance \textbf{A}I \textbf{M}olecular Simulation \textbf{Boo}ster), a predictive framework for molecular dynamics (MD) simulations, with a demonstration of its capability in the context of liquid electrolyte for lithium batteries. We design a physics-inspired graph equivariant transformer architecture as the backbone of BAMBOO to learn from quantum mechanical simulations. Additionally, we introduce an ensemble knowledge distillation approach and apply it to MLFFs to reduce the fluctuation of observations from MD simulations. Finally, we propose a density alignment algorithm to align BAMBOO with experimental measurements. BAMBOO demonstrates state-of-the-art accuracy in predicting key electrolyte properties such as density, viscosity, and ionic conductivity across various solvents and salt combinations. The current model, trained on more than 15 chemical species, achieves the average density error of 0.01 g/cm$^3$ on various compositions compared with experiment. △ Less

Submitted 1 April, 2025; v1 submitted 10 April, 2024; originally announced April 2024.

Comments: Figures provided as the tex source files

Exciton-activated effective phonon magnetic moment in monolayer MoS2

Authors: Chunli Tang, Gaihua Ye, Cynthia Nnokwe, Mengqi Fang, Li Xiang, Masoud Mahjouri-Samani, Dmitry Smirnov, Eui-Hyeok Yang, Tingting Wang, Lifa Zhang, Rui He, Wencan Jin

Abstract: Optical excitation of chiral phonons plays a vital role in studying the phonon-driven magnetic phenomena in solids. Transition metal dichalcogenides host chiral phonons at high symmetry points of the Brillouin zone, providing an ideal platform to explore the interplay between chiral phonons and valley degree of freedom. Here, we investigate the helicity-resolved magneto-Raman response of monolayer… ▽ More Optical excitation of chiral phonons plays a vital role in studying the phonon-driven magnetic phenomena in solids. Transition metal dichalcogenides host chiral phonons at high symmetry points of the Brillouin zone, providing an ideal platform to explore the interplay between chiral phonons and valley degree of freedom. Here, we investigate the helicity-resolved magneto-Raman response of monolayer MoS2 and identify a doubly degenerate Brillouin-zone-center chiral phonon mode at ~270 cm-1. Our wavelength- and temperature-dependent measurements show that this chiral phonon is activated through the resonant excitation of A exciton. Under an out-of-plane magnetic field, the chiral phonon exhibits giant Zeeman splitting, which corresponds to an effective magnetic moment of ~2.5mu_B. Moreover, we carry out theoretical calculations based on the morphic effects in nonmagnetic crystals, which reproduce the linear Zeeman splitting and Raman cross-section of the chiral phonon. Our study provides important insights into lifting the chiral phonon degeneracy in an achiral covalent material, paving a new route to excite and control chiral phonons. △ Less

Submitted 7 April, 2024; v1 submitted 22 March, 2024; originally announced March 2024.

Journal ref: Phys. Rev. B 109, 155426 (2024)

Comparative Raman Scattering Study of Crystal Field Excitations in Co-based Quantum Magnets

Authors: Banasree S. Mou, Xinshu Zhang, Li Xiang, Yuanyuan Xu, Ruidan Zhong, Robert J. Cava, Haidong Zhou, Zhigang Jiang, Dmitry Smirnov, Natalia Drichko, Stephen M. Winter

Abstract: Co-based materials have recently been explored due to potential to realise complex bond-dependent anisotropic magnetism. Prominent examples include Na$_2$Co$_2$TeO$_6$, BaCo$_2$(AsO$_4$)$_2$, Na$_2$BaCo(PO$_4$)$_2$, and CoX$_2$ (X = Cl, Br, I). In order to provide insight into the magnetic interactions in these compounds, we make a comparative analysis of their local crystal electric field excitat… ▽ More Co-based materials have recently been explored due to potential to realise complex bond-dependent anisotropic magnetism. Prominent examples include Na$_2$Co$_2$TeO$_6$, BaCo$_2$(AsO$_4$)$_2$, Na$_2$BaCo(PO$_4$)$_2$, and CoX$_2$ (X = Cl, Br, I). In order to provide insight into the magnetic interactions in these compounds, we make a comparative analysis of their local crystal electric field excitations spectra via Raman scattering measurements. Combining these measurements with theoretical analysis confirms the validity of $j_{\rm eff} = 1/2$ single-ion ground states for all compounds, and provides accurate experimental estimates of the local crystal distortions, which play a prominent role in the magnetic couplings between spin-orbital coupled Co moments. △ Less

Submitted 18 March, 2024; originally announced March 2024.

Comments: 11 pages, 7 figures

Enhanced quantum state transfer: Circumventing quantum chaotic behavior

Authors: Liang Xiang, Jiachen Chen, Zitian Zhu, Zixuan Song, Zehang Bao, Xuhao Zhu, Feitong Jin, Ke Wang, Shibo Xu, Yiren Zou, Hekang Li, Zhen Wang, Chao Song, Alexander Yue, Justine Partridge, Qiujiang Guo, Rubem Mondaini, H. Wang, Richard T. Scalettar

Abstract: The ability to realize high-fidelity quantum communication is one of the many facets required to build generic quantum computing devices. In addition to quantum processing, sensing, and storage, transferring the resulting quantum states demands a careful design that finds no parallel in classical communication. Existing experimental demonstrations of quantum information transfer in solid-state qua… ▽ More The ability to realize high-fidelity quantum communication is one of the many facets required to build generic quantum computing devices. In addition to quantum processing, sensing, and storage, transferring the resulting quantum states demands a careful design that finds no parallel in classical communication. Existing experimental demonstrations of quantum information transfer in solid-state quantum systems are largely confined to small chains with few qubits, often relying upon non-generic schemes. Here, by using a large-scale superconducting quantum circuit featuring thirty-six tunable qubits, accompanied by general optimization procedures deeply rooted in overcoming quantum chaotic behavior, we demonstrate a scalable protocol for transferring few-particle quantum states in a two-dimensional quantum network. These include single-qubit excitation and also two-qubit entangled states, and two excitations for which many-body effects are present. Our approach, combined with the quantum circuit's versatility, paves the way to short-distance quantum communication for connecting distributed quantum processors or registers, even if hampered by inherent imperfections in actual quantum devices. △ Less

Submitted 1 February, 2024; originally announced February 2024.

Comments: 10 pages, 4 figures (main text); 14 pages, 20 figures (supplementary materials)

Creating and controlling global Greenberger-Horne-Zeilinger entanglement on quantum processors

Authors: Zehang Bao, Shibo Xu, Zixuan Song, Ke Wang, Liang Xiang, Zitian Zhu, Jiachen Chen, Feitong Jin, Xuhao Zhu, Yu Gao, Yaozu Wu, Chuanyu Zhang, Ning Wang, Yiren Zou, Ziqi Tan, Aosai Zhang, Zhengyi Cui, Fanhao Shen, Jiarun Zhong, Tingting Li, Jinfeng Deng, Xu Zhang, Hang Dong, Pengfei Zhang, Yang-Ren Liu , et al. (8 additional authors not shown)

Abstract: Greenberger-Horne-Zeilinger (GHZ) states, also known as two-component Schrödinger cats, play vital roles in the foundation of quantum physics and, more attractively, in future quantum technologies such as fault-tolerant quantum computation. Enlargement in size and coherent control of GHZ states are both crucial for harnessing entanglement in advanced computational tasks with practical advantages,… ▽ More Greenberger-Horne-Zeilinger (GHZ) states, also known as two-component Schrödinger cats, play vital roles in the foundation of quantum physics and, more attractively, in future quantum technologies such as fault-tolerant quantum computation. Enlargement in size and coherent control of GHZ states are both crucial for harnessing entanglement in advanced computational tasks with practical advantages, which unfortunately pose tremendous challenges as GHZ states are vulnerable to noise. Here we propose a general strategy for creating, preserving, and manipulating large-scale GHZ entanglement, and demonstrate a series of experiments underlined by high-fidelity digital quantum circuits. For initialization, we employ a scalable protocol to create genuinely entangled GHZ states with up to 60 qubits, almost doubling the previous size record. For protection, we take a new perspective on discrete time crystals (DTCs), originally for exploring exotic nonequilibrium quantum matters, and embed a GHZ state into the eigenstates of a tailor-made cat scar DTC to extend its lifetime. For manipulation, we switch the DTC eigenstates with in-situ quantum gates to modify the effectiveness of the GHZ protection. Our findings establish a viable path towards coherent operations on large-scale entanglement, and further highlight superconducting processors as a promising platform to explore nonequilibrium quantum matters and emerging applications. △ Less

Submitted 13 October, 2024; v1 submitted 16 January, 2024; originally announced January 2024.

Comments: 7 pages, 4 figures + supplementary information

Journal ref: Nat. Commun. 15, 8823 (2024)

Long-lived topological time-crystalline order on a quantum processor

Authors: Liang Xiang, Wenjie Jiang, Zehang Bao, Zixuan Song, Shibo Xu, Ke Wang, Jiachen Chen, Feitong Jin, Xuhao Zhu, Zitian Zhu, Fanhao Shen, Ning Wang, Chuanyu Zhang, Yaozu Wu, Yiren Zou, Jiarun Zhong, Zhengyi Cui, Aosai Zhang, Ziqi Tan, Tingting Li, Yu Gao, Jinfeng Deng, Xu Zhang, Hang Dong, Pengfei Zhang , et al. (16 additional authors not shown)

Abstract: Topologically ordered phases of matter elude Landau's symmetry-breaking theory, featuring a variety of intriguing properties such as long-range entanglement and intrinsic robustness against local perturbations. Their extension to periodically driven systems gives rise to exotic new phenomena that are forbidden in thermal equilibrium. Here, we report the observation of signatures of such a phenomen… ▽ More Topologically ordered phases of matter elude Landau's symmetry-breaking theory, featuring a variety of intriguing properties such as long-range entanglement and intrinsic robustness against local perturbations. Their extension to periodically driven systems gives rise to exotic new phenomena that are forbidden in thermal equilibrium. Here, we report the observation of signatures of such a phenomenon -- a prethermal topologically ordered time crystal -- with programmable superconducting qubits arranged on a square lattice. By periodically driving the superconducting qubits with a surface-code Hamiltonian, we observe discrete time-translation symmetry breaking dynamics that is only manifested in the subharmonic temporal response of nonlocal logical operators. We further connect the observed dynamics to the underlying topological order by measuring a nonzero topological entanglement entropy and studying its subsequent dynamics. Our results demonstrate the potential to explore exotic topologically ordered nonequilibrium phases of matter with noisy intermediate-scale quantum processors. △ Less

Submitted 8 January, 2024; originally announced January 2024.

Comments: 8 pages (main text), 16 pages (supplementary information)

Intrinsic gyrotropic magnetic current from Zeeman quantum geometry

Authors: Longjun Xiang, Jinxiong Jia, Fuming Xu, Zhenhua Qiao, Jian Wang

Abstract: Quantum geometric tensor (QGT), which is usually obtained by evaluating the quantum distance between Bloch states parametrized by momentum, plays a key role in exploring the exotic responses of quantum materials. Herein, we revisit the concept of QGT by further taking into account the spin degree of freedom. Besides the conventional QGT relating to momentum translation, we uncover a new QGT (terme… ▽ More Quantum geometric tensor (QGT), which is usually obtained by evaluating the quantum distance between Bloch states parametrized by momentum, plays a key role in exploring the exotic responses of quantum materials. Herein, we revisit the concept of QGT by further taking into account the spin degree of freedom. Besides the conventional QGT relating to momentum translation, we uncover a new QGT (termed Zeeman QGT) relating to momentum translation as well as spin rotation, whose imaginary (real) part gives the Zeeman Berry curvature (quantum metric). Notably, we show that these novel quantum geometric quantities can drive an intrinsic gyrotropic magnetic current (IGMC) in spin-orbit coupled materials when the electron spin is steered by an oscillating magnetic field. With symmetry analysis, we show that a wide range of materials can support the IGMC, as illustrated by model calculations. Finally, we discuss the experimental aspects of detecting the IGMC driven by Zeeman QGT. △ Less

Submitted 7 January, 2025; v1 submitted 7 December, 2023; originally announced December 2023.

Comments: highlight the novel Zeeman quantum geometry!

Journal ref: Phys. Rev. Lett. 134, 116301 (2025)

Classification of spin Hall effect in two-dimensional systems

Authors: Longjun Xiang, Fuming Xu, Luyang Wang, Jian Wang

Abstract: Physical properties such as the conductivity are usually classified according to the symmetry of the underlying system using Neumann's principle, which gives an upper bound for the number of independent components of the corresponding property tensor. However, for a given Hamiltonian, this global approach usually can not give a definite answer on whether a physical effect such as spin Hall effect… ▽ More Physical properties such as the conductivity are usually classified according to the symmetry of the underlying system using Neumann's principle, which gives an upper bound for the number of independent components of the corresponding property tensor. However, for a given Hamiltonian, this global approach usually can not give a definite answer on whether a physical effect such as spin Hall effect (SHE) exists or not. It is found that the parity and types of spin-orbit interactions (SOIs) are good indicators that can further reduce the number of independent components of the spin Hall conductivity for a specific system. In terms of the parity as well as various Rashba-like and Dresselhaus-like SOIs, we propose a local approach to classify SHE in two-dimensional (2D) two-band models, where sufficient conditions for identifying the existence or absence of SHE in all 2D magnetic point groups are presented. △ Less

Submitted 11 November, 2023; originally announced November 2023.

Journal ref: Front. Phys. 19(3), 33205 (2024)

Gapless superconducting state and mirage gap in altermagnets

Authors: Miaomiao Wei, Longjun Xiang, Fuming Xu, Lei Zhang, Gaomin Tang, Jian Wang

Abstract: The interplay between spin-orbit interaction (SOI) and magnetism produces interesting phenomena in superconductors. When a two-dimensional (2D) system with strong SOI is coupled to an $s$-wave superconductor, an in-plane magnetic field can drive the system into a gapless superconducting state and induce a mirage gap at finite energies for an Ising superconductor. In this work, we demonstrate that… ▽ More The interplay between spin-orbit interaction (SOI) and magnetism produces interesting phenomena in superconductors. When a two-dimensional (2D) system with strong SOI is coupled to an $s$-wave superconductor, an in-plane magnetic field can drive the system into a gapless superconducting state and induce a mirage gap at finite energies for an Ising superconductor. In this work, we demonstrate that when an $s$-wave superconductor is proximitized to an altermagnet, the intrinsic anisotropic spin splitting of the altermagnet can result in a gapless superconducting state and a pair of mirage gaps at finite energy. The gapless superconductivity exhibits spin-polarized segmented Fermi surfaces, with coexisting spin-singlet and spin-triplet pairings that have a $d$-wave character. Importantly, the gapless superconducting and mirage gap features are quantified through quantum transport. Our results suggest that altermagnet is an ideal platform for studying gapless superconducting states and mirage gap physics. △ Less

Submitted 14 May, 2024; v1 submitted 31 July, 2023; originally announced August 2023.

Comments: This work has been accepted by PRB Letter

Linear displacement current solely driven by the quantum metric

Authors: Longjun Xiang, Bin Wang, Yadong Wei, Zhenhua Qiao, Jian Wang

Abstract: Quantum metric and Berry curvature are the real part and imaginary part of the quantum geometric tensor, respectively. The T-odd (T: time-reversal) nonlinear Hall effect driven by the quantum metric dipole, recently confirmed in Science 381, 181 (2023) and Nature 621, 487 (2023), established the geometric duality to the T-even nonlinear Hall effect that driven by the Berry curvature dipole. Intere… ▽ More Quantum metric and Berry curvature are the real part and imaginary part of the quantum geometric tensor, respectively. The T-odd (T: time-reversal) nonlinear Hall effect driven by the quantum metric dipole, recently confirmed in Science 381, 181 (2023) and Nature 621, 487 (2023), established the geometric duality to the T-even nonlinear Hall effect that driven by the Berry curvature dipole. Interestingly, a similar geometric duality between the quantum metric and the Berry curvature, particularly for the linear response of Bloch electrons, has not been established, although the T-odd linear intrinsic anomalous Hall effect (IAHE) solely driven by the Berry curvature has been known for a long time. Herein, we develop the quantum theory for displacement current under an AC electric field. Particularly, we show that the T-even component of the linear displacement current conductivity (LDCC) is solely determined by the quantum metric, by both the response theory and the semiclassical theory. Notably, with symmetry analysis we find that the T-even LDCC can contribute a Hall current in T-invariant systems but with low symmetry, while its longitudinal component is immune to symmetry. Furthermore, employing the Dirac Hamiltonian, we arrive at a $1/μ$ ($μ$: chemical potential) experimental observable enhancement of the displacement current owing to the divergent behavior of quantum metric near Dirac point, similar to the IAHE at Weyl point. Our work reveals the band geometric origin of the linear displacement current and establishes, together with the IAHE, the geometric duality for the linear response of Bloch electrons. Additionally, our work offers the very first intrinsic Hall effect in T-invariant materials, which can not be envisioned in DC transport in both linear and nonlinear regimes. △ Less

Submitted 6 February, 2024; v1 submitted 14 July, 2023; originally announced July 2023.

Comments: 3 figures

Disorder-enriched magnetic excitations in the Kitaev quantum spin liquid candidate Na$_2$Co$_2$TeO$_6$

Authors: Li Xiang, Ramesh Dhakal, Mykhaylo Ozerov, Yuxuan Jiang, Banasree S. Mou, Andrzej Ozarowski, Qing Huang, Haidong Zhou, Jiyuan Fang, Stephen M. Winter, Zhigang Jiang, Dmitry Smirnov

Abstract: Using optical magneto-spectroscopy, we investigate the magnetic excitations of Na$_2$Co$_2$TeO$_6$ in a broad magnetic field range ($0\ \rm{T}\leq B\leq 17.5\ \rm{T}$) at low temperature. Our measurements reveal rich spectra of in-plane magnetic excitations with a surprisingly large number of modes, even in the high-field spin-polarized state. Theoretical calculations find that the Na-occupation d… ▽ More Using optical magneto-spectroscopy, we investigate the magnetic excitations of Na$_2$Co$_2$TeO$_6$ in a broad magnetic field range ($0\ \rm{T}\leq B\leq 17.5\ \rm{T}$) at low temperature. Our measurements reveal rich spectra of in-plane magnetic excitations with a surprisingly large number of modes, even in the high-field spin-polarized state. Theoretical calculations find that the Na-occupation disorder in \NCTO plays a crucial role in generating these modes. Our work demonstrates the necessity to consider disorder in the spin environment in the search for Kitaev quantum spin liquid states in practicable materials. △ Less

Submitted 12 May, 2023; originally announced May 2023.

Quantifying the photocurrent fluctuation in quantum materials by shot noise

Authors: Longjun Xiang, Hao Jin, Jian Wang

Abstract: The DC photocurrent can detect the topology and geometry of quantum materials without inversion symmetry. Herein, we propose that the DC shot noise (DSN), as the fluctuation of photocurrent operator, can also be a diagnostic of quantum materials. Particularly, we develop the quantum theory for DSNs in gapped systems and identify the shift and injection DSNs by dividing the second-order photocurren… ▽ More The DC photocurrent can detect the topology and geometry of quantum materials without inversion symmetry. Herein, we propose that the DC shot noise (DSN), as the fluctuation of photocurrent operator, can also be a diagnostic of quantum materials. Particularly, we develop the quantum theory for DSNs in gapped systems and identify the shift and injection DSNs by dividing the second-order photocurrent operator into off-diagonal and diagonal contributions, respectively. Remarkably, we find that the DSNs can not be forbidden by inversion symmetry, while the constraint from time-reversal symmetry depends on the polarization of light. Furthermore, we show that the DSNs also encode the geometrical information of Bloch electrons, such as the Berry curvature and the quantum metric. Finally, guided by symmetry, we apply our theory to evaluate the DSNs in monolayer GeS and bilayer MoS$_2$ with and without inversion symmetry and find that the DSNs can be larger in centrosymmetric phase. △ Less

Submitted 14 May, 2024; v1 submitted 16 March, 2023; originally announced March 2023.

Comments: two figures

Infrared-induced ultrafast melting of nanostructured platinum films probed by an X-ray free-electron laser

Authors: Luca Gelisio, Young Yong Kim, Seon Woo Lim, Daewoong Nam, Intae Eom, Minseok Kim, Sangsoo Kim, Ruslan Khubbutdinov, Li Xiang, Hoyeol Lee, Moonhor Ree, Chae Un Kim, Ivan A. Vartanyants

Abstract: Understanding melting in metals is a hot topic of present research. This may be accomplished by pumping the system with infrared (IR) laser radiation, and probing it with hard X-rays produced by an X-ray Free-Electron Laser (XFEL). In this work we studied nanostructured polycrystalline thin films of platinum that were illuminated by IR radiation of increasing fluences. We characterized the structu… ▽ More Understanding melting in metals is a hot topic of present research. This may be accomplished by pumping the system with infrared (IR) laser radiation, and probing it with hard X-rays produced by an X-ray Free-Electron Laser (XFEL). In this work we studied nanostructured polycrystalline thin films of platinum that were illuminated by IR radiation of increasing fluences. We characterized the structural response as well as the nucleation and propagation of the liquid phase as a function of time delay between the IR pump and X-ray probe. We observed partial melting of the samples for IR fluences higher than 200 mJ$\cdot$cm$^{-2}$. To fit the contribution of the liquid phase to the scattering pattern in platinum we applied a model of liquid metal. The two-temperature model simulations were performed to understand the solid-state fraction of the sample heating process as a function of time delay and fluence. △ Less

Submitted 23 February, 2023; originally announced February 2023.

Quantum Fluctuation of the Quantum Geometric Tensor and its Manifestation as Intrinsic Hall Signatures in Time-Reversal Invariant Systems

Authors: Miaomiao Wei, Luyang Wang, Bin Wang, Longjun Xiang, Fuming Xu, Baigeng Wang, Jian Wang

Abstract: In time-reversal invariant systems, all charge Hall effects predicted so far are extrinsic effects due to the dependence on the relaxation time. We explore intrinsic Hall signatures by studying quantum noise spectrum of the Hall current in time-reversal invariant systems, and discover intrinsic thermal Hall noises in both linear and nonlinear regimes. As the band geometric characteristics, quantum… ▽ More In time-reversal invariant systems, all charge Hall effects predicted so far are extrinsic effects due to the dependence on the relaxation time. We explore intrinsic Hall signatures by studying quantum noise spectrum of the Hall current in time-reversal invariant systems, and discover intrinsic thermal Hall noises in both linear and nonlinear regimes. As the band geometric characteristics, quantum geometric tensor and Berry curvature play critical roles in various Hall effects, so are their quantum fluctuations. It is found that the thermal Hall noise in linear order of the electric field is purely intrinsic, and the second-order thermal Hall noise has both intrinsic and extrinsic contributions. In particular, the intrinsic part of the second-order thermal Hall noise is a manifestation of the quantum fluctuation of quantum geometric tensor, which widely exists as long as Berry curvature is nonzero. These intrinsic thermal Hall noises provide direct measurable means to band geometric information, including Berry curvature related quantities and quantum fluctuation of quantum geometric tensor. △ Less

Submitted 27 January, 2023; originally announced January 2023.

Journal ref: Physical Review Letters 130, 036202 (2023)

Effects of physical and chemical pressure on charge density wave transitions in LaAg1-xAuxSb2 single crystals

Authors: Li Xiang, Dominic H. Ryan, Paul C. Canfield, Sergey L. Bud'ko

Abstract: The structural characterization and electrical transport measurements at ambient and applied pressures of the compounds of the La(Ag1-xAux)Sb2 family are presented. Up to two charge density wave (CDW) transitions could be detected upon cooling from room temperature and an equivalence of the effects of chemical and physical pressure on the CDW ordering temperatures was observed with the unit cell v… ▽ More The structural characterization and electrical transport measurements at ambient and applied pressures of the compounds of the La(Ag1-xAux)Sb2 family are presented. Up to two charge density wave (CDW) transitions could be detected upon cooling from room temperature and an equivalence of the effects of chemical and physical pressure on the CDW ordering temperatures was observed with the unit cell volume being a salient structural parameter. As such La(Ag1-xAux)Sb2 is a rare example of a non-cubic system that exhibits good agreement between the effects of applied, physical, pressure and changes in unit cell volume from steric changes induced by isovalent substitution. Additionally, for La(Ag0.54Au0.46)Sb2 anomalies in low temperature electrical transport were observed in the pressure range where the lower charge density wave is completely suppressed. △ Less

Submitted 21 November, 2022; originally announced November 2022.

Journal ref: Crystals 12(12), 1693, 2022

Digital simulation of non-Abelian anyons with 68 programmable superconducting qubits

Authors: Shibo Xu, Zheng-Zhi Sun, Ke Wang, Liang Xiang, Zehang Bao, Zitian Zhu, Fanhao Shen, Zixuan Song, Pengfei Zhang, Wenhui Ren, Xu Zhang, Hang Dong, Jinfeng Deng, Jiachen Chen, Yaozu Wu, Ziqi Tan, Yu Gao, Feitong Jin, Xuhao Zhu, Chuanyu Zhang, Ning Wang, Yiren Zou, Jiarun Zhong, Aosai Zhang, Weikang Li , et al. (9 additional authors not shown)

Abstract: Non-Abelian anyons are exotic quasiparticle excitations hosted by certain topological phases of matter. They break the fermion-boson dichotomy and obey non-Abelian braiding statistics: their interchanges yield unitary operations, rather than merely a phase factor, in a space spanned by topologically degenerate wavefunctions. They are the building blocks of topological quantum computing. However, e… ▽ More Non-Abelian anyons are exotic quasiparticle excitations hosted by certain topological phases of matter. They break the fermion-boson dichotomy and obey non-Abelian braiding statistics: their interchanges yield unitary operations, rather than merely a phase factor, in a space spanned by topologically degenerate wavefunctions. They are the building blocks of topological quantum computing. However, experimental observation of non-Abelian anyons and their characterizing braiding statistics is notoriously challenging and has remained elusive hitherto, in spite of various theoretical proposals. Here, we report an experimental quantum digital simulation of projective non-Abelian anyons and their braiding statistics with up to 68 programmable superconducting qubits arranged on a two-dimensional lattice. By implementing the ground states of the toric-code model with twists through quantum circuits, we demonstrate that twists exchange electric and magnetic charges and behave as a particular type of non-Abelian anyons, i.e., the Ising anyons. In particular, we show experimentally that these twists follow the fusion rules and non-Abelian braiding statistics of the Ising type, and can be explored to encode topological logical qubits. Furthermore, we demonstrate how to implement both single- and two-qubit logic gates through applying a sequence of elementary Pauli gates on the underlying physical qubits. Our results demonstrate a versatile quantum digital approach for simulating non-Abelian anyons, offering a new lens into the study of such peculiar quasiparticles. △ Less

Submitted 11 May, 2023; v1 submitted 17 November, 2022; originally announced November 2022.

Journal ref: Chin. Phys. Lett. 40 060301 (2023)

Magnetism and $T-x$ phase diagrams of Na and Ag substituted EuCd$_2$As$_2$

Authors: Brinda Kuthanazhi, Kamal R. Joshi, Sunil Ghimire, Erik Timmons, Lin-Lin Wang, Elena Gati, Li Xiang, Ruslan Prozorov, Sergey L. Bud'ko, Paul C. Canfield

Abstract: EuCd$_2$As$_2$ is an antiferromagnetic semimetal, that can host non-trivial topological properties, depending upon its magnetic state and excitations. Here, we report the synthesis and characterization of Eu(Cd$_{1-x}$Ag$_x$)$_2$As$_2$ and Eu$_{1-y}$Na$_y$Cd$_2$As$_2$, and study the evolution and nature of magnetic order with doping. Temperature-substitution phase diagrams are constructed from the… ▽ More EuCd$_2$As$_2$ is an antiferromagnetic semimetal, that can host non-trivial topological properties, depending upon its magnetic state and excitations. Here, we report the synthesis and characterization of Eu(Cd$_{1-x}$Ag$_x$)$_2$As$_2$ and Eu$_{1-y}$Na$_y$Cd$_2$As$_2$, and study the evolution and nature of magnetic order with doping. Temperature-substitution phase diagrams are constructed from the electrical resistance and magnetic susceptibility data. We observe a splitting of the magnetic transition into two different transitions, and the gradual increase in one of the transition temperatures with Ag- and Na-substitution. The other transition remains more or less independent of doping. We further show that a magnetic state with a net ferromagnetic moment is stabilized by both Ag and Na doping and this can be explained by considering the changes in band filling due to substitution as suggested by density functional theory (DFT) calculations. We thus show that chemical substitution and the subsequent changes in band filling could be a pathway to tune the magnetic ground state and to stabilize a ferromagnetic phase in EuCd$_2$As$_2$. △ Less

Submitted 16 November, 2022; originally announced November 2022.

Observation of many-body Fock space dynamics in two dimensions

Authors: Yunyan Yao, Liang Xiang, Zexian Guo, Zehang Bao, Yong-Feng Yang, Zixuan Song, Haohai Shi, Xuhao Zhu, Feitong Jin, Jiachen Chen, Shibo Xu, Zitian Zhu, Fanhao Shen, Ning Wang, Chuanyu Zhang, Yaozu Wu, Yiren Zou, Pengfei Zhang, Hekang Li, Zhen Wang, Chao Song, Chen Cheng, Rubem Mondaini, H. Wang, J. Q. You , et al. (3 additional authors not shown)

Abstract: Quantum many-body simulation provides a straightforward way to understand fundamental physics and connect with quantum information applications. However, suffering from exponentially growing Hilbert space size, characterization in terms of few-body probes in real space is often insufficient to tackle challenging problems such as quantum critical behavior and many-body localization (MBL) in higher… ▽ More Quantum many-body simulation provides a straightforward way to understand fundamental physics and connect with quantum information applications. However, suffering from exponentially growing Hilbert space size, characterization in terms of few-body probes in real space is often insufficient to tackle challenging problems such as quantum critical behavior and many-body localization (MBL) in higher dimensions. Here, we experimentally employ a new paradigm on a superconducting quantum processor, exploring such elusive questions from a Fock space view: mapping the many-body system onto an unconventional Anderson model on a complex Fock space network of many-body states. By observing the wave packet propagating in Fock space and the emergence of a statistical ergodic ensemble, we reveal a fresh picture for characterizing representative many-body dynamics: thermalization, localization, and scarring. In addition, we observe a quantum critical regime of anomalously enhanced wave packet width and deduce a critical point from the maximum wave packet fluctuations, which lend support for the two-dimensional MBL transition in finite-sized systems. Our work unveils a new perspective of exploring many-body physics in Fock space, demonstrating its practical applications on contentious MBL aspects such as criticality and dimensionality. Moreover, the entire protocol is universal and scalable, paving the way to finally solve a broader range of controversial many-body problems on future larger quantum devices. △ Less

Submitted 10 November, 2022; originally announced November 2022.

Comments: 8 pages, 4 figures + supplementary information

Electronically phase separated nano-network in antiferromagnetic insulating LaMnO3/PrMnO3/CaMnO3 tricolor superlattice

Authors: Qiang Li, Tian Miao, Huimin Zhang, Weiyan Lin, Wenhao He, Yang Zhong, Lifen Xiang, Lina Deng, Biying Ye, Qian Shi, Yinyan Zhu, Hangwen Guo, Wenbin Wang, Changlin Zheng, Lifeng Yin, Xiaodong Zhou, Hongjun Xiang, Jian Shen

Abstract: Strongly correlated materials often exhibit an electronic phase separation (EPS) phenomena whose domain pattern is random in nature. The ability to control the spatial arrangement of the electronic phases at microscopic scales is highly desirable for tailoring their macroscopic properties and/or designing novel electronic devices. Here we report the formation of EPS nanoscale network in a mono-ato… ▽ More Strongly correlated materials often exhibit an electronic phase separation (EPS) phenomena whose domain pattern is random in nature. The ability to control the spatial arrangement of the electronic phases at microscopic scales is highly desirable for tailoring their macroscopic properties and/or designing novel electronic devices. Here we report the formation of EPS nanoscale network in a mono-atomically stacked LaMnO3/CaMnO3/PrMnO3 superlattice grown on SrTiO3 (STO) (001) substrate, which is known to have an antiferromagnetic (AFM) insulating ground state. The EPS nano-network is a consequence of an internal strain relaxation triggered by the structural domain formation of the underlying STO substrate at low temperatures. The same nanoscale network pattern can be reproduced upon temperature cycling allowing us to employ different local imaging techniques to directly compare the magnetic and transport state of a single EPS domain. Our results confirm the one-to-one correspondence between ferromagnetic (AFM) to metallic (insulating) state in manganite. It also represents a significant step in a paradigm shift from passively characterizing EPS in strongly correlated systems to actively engaging in its manipulation. △ Less

Submitted 3 November, 2022; originally announced November 2022.

Journal ref: Nat. Commun. 13, 6593 (2022)

Thickness and twist angle dependent interlayer excitons in metal monochalcogenide heterostructures

Authors: Wenkai Zheng, Li Xiang, Felipe de Quesada, Mathias Augustin, Zhengguang Lu, Matthew Wilson, Aditya Sood, Fengcheng Wu, Dmitry Shcherbakov, Shahriar Memaran, Ryan E. Baumbach, Gregory T. McCandless, Julia Y. Chan, Song Liu, James Edgar, Chun Ning Lau, Chun Hung Lui, Elton Santos, Aaron Lindenberg, Dmitry Smirnov, Luis Balicas

Abstract: Interlayer excitons, or bound electron-hole pairs whose constituent quasiparticles are located in distinct stacked semiconducting layers, are being intensively studied in heterobilayers of two dimensional semiconductors. They owe their existence to an intrinsic type-II band alignment between both layers that convert these into p-n junctions. Here, we unveil a pronounced interlayer exciton (IX) in… ▽ More Interlayer excitons, or bound electron-hole pairs whose constituent quasiparticles are located in distinct stacked semiconducting layers, are being intensively studied in heterobilayers of two dimensional semiconductors. They owe their existence to an intrinsic type-II band alignment between both layers that convert these into p-n junctions. Here, we unveil a pronounced interlayer exciton (IX) in heterobilayers of metal monochalcogenides, namely gamma-InSe on epsilon-GaSe, whose pronounced emission is adjustable just by varying their thicknesses given their number of layers dependent direct bandgaps. Time-dependent photoluminescense spectroscopy unveils considerably longer interlayer exciton lifetimes with respect to intralayer ones, thus confirming their nature. The linear Stark effect yields a bound electron-hole pair whose separation d is just (3.6 \pm 0.1) Å with d being very close to dSe = 3.4 Å which is the calculated interfacial Se separation. The envelope of IX is twist angle dependent and describable by superimposed emissions that are nearly equally spaced in energy, as if quantized due to localization induced by the small moiré periodicity. These heterostacks are characterized by extremely flat interfacial valence bands making them prime candidates for the observation of magnetism or other correlated electronic phases upon carrier doping. △ Less

Submitted 15 October, 2022; originally announced October 2022.

Comments: ACS Nano, in press 42 pages plus, 4 figures, plus supplementary information file, containing 21 supplementary figures

Third-order intrinsic anomalous Hall effect with generalized semiclassical theory

Authors: Longjun Xiang, Chao Zhang, Luyang Wang, Jian Wang

Abstract: The linear intrinsic anomalous Hall effect (IAHE) and second-order IAHE have been intensively investigated in time-reversal broken systems. However, as one of the important members of the nonlinear Hall family, the investigation of third-order IAHE remains absent due to the lack of an appropriate theoretical approach, although the third-order extrinsic AHE has been studied within the framework of… ▽ More The linear intrinsic anomalous Hall effect (IAHE) and second-order IAHE have been intensively investigated in time-reversal broken systems. However, as one of the important members of the nonlinear Hall family, the investigation of third-order IAHE remains absent due to the lack of an appropriate theoretical approach, although the third-order extrinsic AHE has been studied within the framework of first- and second-order semiclassical theory. Herein, we generalize the semiclassical theory for Bloch electrons under the uniform electric field up to the third-order using wavepacket method and based on which we predict that the third-order IAHE can also occur in time-reversal broken systems. Same as the second-order IAHE, we find the band geometric quantity, the second-order field-dependent Berry curvature arising from the second-order field-induced positional shift, plays a pivotal role to observe this effect. Moreover, with symmetry analysis, we find that the third-order IAHE, as the leading contribution, is supported by 15 time-reversal broken 3D magnetic point groups (MPGs), corresponding to a wide class of antiferromagnetic (AFM) materials. Guided by the symmetry arguments, a two-band model is chosen to demonstrate the generalized theory. Furthermore, the generalized third-order semiclassical theory depends only on the properties of Bloch bands, implying that it can also be employed to explore the IAHE in realistic AFM materials, by combining with first-principles calculations. △ Less

Submitted 27 January, 2023; v1 submitted 30 September, 2022; originally announced September 2022.

Comments: 1 figure

Pressure-temperature phase diagram of CaK(Fe$_{1-x}$Mn$_x$)$_4$As$_4$ for $x$=0.024

Authors: Li Xiang, Mingyu Xu, Sergey L. Bud'ko, Paul C. Canfield

Abstract: Resistance measurements on single crystals of CaK(Fe$_{1-x}$Mn$_x$)$_4$As$_4$ ($x$ = 0.024) were performed under hydrostatic pressure up to 5.15 GPa. The pressure dependence of the magnetic and superconducting transition temperatures and that of the superconducting upper critical field are reported. Our results show that upon increasing pressure, the magnetic transition temperature $T_{N}$ is supp… ▽ More Resistance measurements on single crystals of CaK(Fe$_{1-x}$Mn$_x$)$_4$As$_4$ ($x$ = 0.024) were performed under hydrostatic pressure up to 5.15 GPa. The pressure dependence of the magnetic and superconducting transition temperatures and that of the superconducting upper critical field are reported. Our results show that upon increasing pressure, the magnetic transition temperature $T_{N}$ is suppressed, whereas the superconducting transition temperature $T_{c}$ first increases and then decreases, exhibiting a maximum at a pressure $p_c$ corresponding to the intersection of the $T_{N}$($p$) and $T_{c}$($p$) lines. In addition, a minimum in the normalized slope of the superconducting upper critical field as well as a change in the pressure dependence of the inferred superconducting coherence length are observed at $p_c$, suggesting a difference in the Fermi surface of the paramagnetic and antiferromagnetic states. Finally, CaK(Fe$_{1-x}$Mn$_x$)$_4$As$_4$ ($x$ = 0.024) likely goes through a half-collapsed-tetragonal phase transition at $\sim$ 4.3 GPa, further demonstrating that the half-collapsed-tetragonal transition pressure in the CaKFe$_4$As$_4$ system is relatively insensitive to transition metal substitution. △ Less

Submitted 20 September, 2022; originally announced September 2022.

Comments: 6 figures

Intrinsic in-plane magnetononlinear Hall effect in tilted Weyl semimetals

Authors: Longjun Xiang, Jian Wang

Abstract: Armed with the extended semiclassical theory, we propose a Hall effect at $EB$ order, particularly in Weyl semimetals (WSMs). We dub this effect the in-plane magnetononlinear Hall effect (IMHE) since the Hall current and the driving electric and magnetic fields are confined in the same plane. Similar to the intrinsic anomalous Hall effect, the IMHE features an intrinsic nature because it arises fr… ▽ More Armed with the extended semiclassical theory, we propose a Hall effect at $EB$ order, particularly in Weyl semimetals (WSMs). We dub this effect the in-plane magnetononlinear Hall effect (IMHE) since the Hall current and the driving electric and magnetic fields are confined in the same plane. Similar to the intrinsic anomalous Hall effect, the IMHE features an intrinsic nature because it arises from the field-induced anomalous velocity $\vec{E} \times \vecΩ^B$, where $\vecΩ^B$ is the Berry curvature induced by the magnetic field through both minimal and Zeeman couplings. Employing the low-energy effective Hamiltonian of WSMs, we reveal that the tilt of the Weyl cone is the key to triggering this effect. Notably, we find that the IMHE can survive even when the \textit{chiral anomaly} disappears because $\vectΩ^B$ (as the correction of the conventional Berry curvature) does not contribute to the monopole charge. Furthermore, we elucidate the interplay between minimal and Zeeman couplings for this effect. Finally, the experimental strategy to detect the IMHE is discussed. △ Less

Submitted 16 February, 2024; v1 submitted 7 September, 2022; originally announced September 2022.

Comments: 3 figures

Quantum third-order nonlinear Hall effect of a four-terminal device with time-reversal symmetry

Authors: Miaomiao Wei, Longjun Xiang, Luyang Wang, Fuming Xu, Jian Wang

Abstract: The third-order nonlinear Hall effect induced by Berry-connection polarizability tensor has been observed in Weyl semimetals T$_d$-MoTe$_2$ as well as T$_d$-TaIrTe$_4$. The experiments were performed on bulk samples, and the results were interpreted with the semiclassical Boltzmann approach. Beyond the bulk limit, we develop a quantum nonlinear transport theory to investigate the third-order Hall… ▽ More The third-order nonlinear Hall effect induced by Berry-connection polarizability tensor has been observed in Weyl semimetals T$_d$-MoTe$_2$ as well as T$_d$-TaIrTe$_4$. The experiments were performed on bulk samples, and the results were interpreted with the semiclassical Boltzmann approach. Beyond the bulk limit, we develop a quantum nonlinear transport theory to investigate the third-order Hall response of a four-terminal setup with time-reversal symmetry in quantum regime. The quantum nonlinear theory is verified on a model system of monolayer MoTe$_2$, and numerical results on the angle-resolved Hall currents are qualitatively consistent with the experiment. More importantly, quantum signatures of the third-order Hall effect are revealed, which are independent of the system symmetry. The first quantum signature is quantum enhancement of the third-order Hall current, which is characterized by sharp current peaks whose magnitudes are three orders larger than the first-order Hall current. Such quantum enhancement originates from quantum interference in coherent transport, and it can be easily destroyed by dephasing effect. The second quantum signature is disorder-induced enhancement of the third-order Hall current for weak disorders. Our findings reveal quantum characteristics of the third-order Hall effect, and we propose feasible ways to enhance it in nanoscale systems. The quantum third-order theory developed in this work provides a general formalism for describing nonlinear coherent transport properties in multi-terminal devices, regardless of the system symmetry. △ Less

Submitted 22 July, 2022; originally announced July 2022.

Journal ref: Phys. Rev. B 106, 035307 (2022)

Superconductivity and phase diagrams of CaK(Fe$_{1-x}$Mn$_{x}$)$_{4}$As$_{4}$ single crystals

Authors: M. Xu, J. Schmidt, E. Gati, L. Xiang, W. R. Meier, V. G. Kogan, S. L. Bud'ko, P. C. Canfield

Abstract: Members of the CaK(Fe$_{1-x}$Mn$_{x}$)$_{4}$As$_{4}$ series have been synthesized in single crystalline form and characterized by elemental analysis, thermodynamic and transport measurements. These measurements show that the superconducting transition temperature decreases monotonically and is finally suppressed below 1.8 K. For $x$-values greater than 0.016, signatures of a magnetic transition ca… ▽ More Members of the CaK(Fe$_{1-x}$Mn$_{x}$)$_{4}$As$_{4}$ series have been synthesized in single crystalline form and characterized by elemental analysis, thermodynamic and transport measurements. These measurements show that the superconducting transition temperature decreases monotonically and is finally suppressed below 1.8 K. For $x$-values greater than 0.016, signatures of a magnetic transition can be detected in both thermodynamic and transport measurements in which kink-like features allow for the determination of the transition temperature, $T^*$, that increases as Mn substitution increases. A temperature-composition ($T$-$x$) phase diagram is constructed, revealing a half-dome of superconductivity with the magnetic transition temperature, $T^*$, appearing near 26 K for $x$ $\sim$ 0.017 and rising slowly up to 33 K for $x$ $\sim$ 0.036. Specific heat data are used to track the jump in specific heat at $T_c$; The CaK(Fe$_{1-x}$Mn$_x$)$_4$As$_4$ data does not follow the scaling of $Δ$$C_{p}$ with $T_{c}^3$ as many of the other Fe-based superconducting systems do. Elastoresistivity coefficients, $2m_{66}$ and $m_{11}-m_{12}$, as a function of temperature are also measured. $2m_{66}$ and $m_{11}-m_{12}$ are qualitatively similar to CaK(Fe$_{1-x}$Ni$_x$)$_4$As$_4$. This may indicate that the magnetic order in Mn substituted system may be still the same as CaK(Fe$_{1-x}$Ni$_x$)$_4$As$_4$. A clear change in $H^\prime_{c2}$($T$)/$T_c$, where $H^\prime_{c2}$($T$) is d$H_{c2}$($T$)/d$T$, at $x$ $\sim$ 0.015 is observed and probably is related to change of the Fermi surface due to magnetic order. Coherence lengths and the London penetration depths are also calculated based on $H_{c1}$ and $H_{c2}$ data. Coherence lengths as the function of $x$ also shows the changes near $x$ = 0.015. △ Less

Submitted 2 May, 2022; v1 submitted 22 April, 2022; originally announced April 2022.

Comments: Fig. 16 a and b were corrected

Journal ref: Phys. Rev. B 105, 214526 (2022)

Effects of external pressure on the narrow gap semiconductor Ce$_{3}$Cd$_{2}$As$_{6}$

Authors: M. M. Piva, L. Xiang, J. D. Thompson, S. L. Bud'ko, R. A. Ribeiro, P. C. Canfield, P. F. S. Rosa

Abstract: Here we report the magnetic and electronic properties of recently discovered Ce$_{3}$Cd$_{2}$As$_{6}$. At ambient pressure, Ce$_{3}$Cd$_{2}$As$_{6}$ presents a semiconducting behavior with an activation gap of 74(1)~meV. At 136~K, a sudden increase of the electrical resistivity and a peak in specific heat are consistent with a charge density wave transition. At low temperatures, antiferromagnetic… ▽ More Here we report the magnetic and electronic properties of recently discovered Ce$_{3}$Cd$_{2}$As$_{6}$. At ambient pressure, Ce$_{3}$Cd$_{2}$As$_{6}$ presents a semiconducting behavior with an activation gap of 74(1)~meV. At 136~K, a sudden increase of the electrical resistivity and a peak in specific heat are consistent with a charge density wave transition. At low temperatures, antiferromagnetic order of the Ce$^{3+}$ ions occurs below $T_{\rm N} = 4.0$~K with a magnetic hard axis along the $c$-axis and a $Γ_{6} = |\pm1/2\rangle$ doublet ground state. The application of external pressure strongly suppresses the charge density wave order, which is completely suppressed above 0.8(1)~GPa, and induces a metallic ground state. No evidence for superconductivity is detected above 2~K. Conversely, the antiferromagnetic state is favored by pressure, reaching a transition temperature of 5.3~K at 3.8(1)~GPa. Notably, the resistivity anomaly characterizing the antiferromagnetic order changes with increasing pressure, indicating that two different magnetic phases might be present in Ce$_{3}$Cd$_{2}$As$_{6}$ under pressure. This change in ordering appears to be associated to the crossing of the $T_{\rm CDW}$ and $T_{\rm N}$ lines. △ Less

Submitted 18 March, 2022; originally announced March 2022.

Small moment antiferromagnetic ordering in single crystalline La2Ni7

Authors: Raquel A. Ribeiro, Sergey L. Bud'ko, Li Xiang, Dominic H. Ryan, Paul C. Canfield

Abstract: Single crystals of La2Ni7 have been grown out of a binary, La-Ni melt. Temperature dependent, zero magnetic field, specific heat, electrical resistivity, and low field magnetization measurements indicate that there is a series of antiferromagnetic phase transitions at T1 = 61.0 \pm 0.2 K, T2 = 56.5 \pm 0.2 K and T3 = 42.2 \pm 0.2 K. The three specific heat anomalies found at these temperatures qua… ▽ More Single crystals of La2Ni7 have been grown out of a binary, La-Ni melt. Temperature dependent, zero magnetic field, specific heat, electrical resistivity, and low field magnetization measurements indicate that there is a series of antiferromagnetic phase transitions at T1 = 61.0 \pm 0.2 K, T2 = 56.5 \pm 0.2 K and T3 = 42.2 \pm 0.2 K. The three specific heat anomalies found at these temperatures qualitatively have very small entropy changes associated with them and the anisotropic M(H) data saturate at ~ 0.12 μB/Ni; both observations strongly suggesting the AFM order is associated with very small, itinerant, moments. Anisotropic, H||c and H{\perp}c, ρ(H) and M(H) isotherms as well as constant field, ρ(T) and M(T) sweeps manifest signatures of multiple phase lines and result in H-T phase diagrams that are clearly anisotropic. Analysis of M(T) and M(H) data allow for the identification of the two lower temperature magnetically ordered states as antiferromagnetically ordered, with the moments aligned along the crystallographic c-axis, and the higher temperature, T2 < T < T1, state as having a finite ferromagnetic component. In addition, the metamagnetic transition at low temperatures, for H applied along the crystallographic c-axis (H||c) appears to be a near classic example of a spin-flop transition, resulting in a field stabilized antiferromagnetic state with the moments ordered perpendicular to the c-axis. Although the small moment ordering, and existence of multiple phase transitions in field and temperature, suggesting an energetic proximity of these states, could foretell a degree of pressure sensitivity, our measurements of R(T) for applied pressures up to 2.0 GPa indicate that there is very little pressure dependence of T1, T2 and T3. △ Less

Submitted 12 October, 2021; originally announced October 2021.

Comments: 22 figures

Pressure-induced ferromagnetism in the topological semimetal EuCd$_2$As$_2$

Authors: Elena Gati, Sergey L. Bud'ko, Lin-Lin Wang, Adrian Valadkhani, Ritu Gupta, Brinda Kuthanazhi, Li Xiang, John M. Wilde, Aashish Sapkota, Zurab Guguchia, Rustem Khasanov, Roser Valenti, Paul C. Canfield

Abstract: The antiferromagnet and semimetal EuCd$_2$As$_2$ has recently attracted a lot of attention due to a wealth of topological phases arising from the interplay of topology and magnetism. In particular, the presence of a single pair of Weyl points is predicted for a ferromagnetic configuration of Eu spins along the $c$-axis in EuCd$_2$As$_2$. In the search for such phases, we investigate here the effec… ▽ More The antiferromagnet and semimetal EuCd$_2$As$_2$ has recently attracted a lot of attention due to a wealth of topological phases arising from the interplay of topology and magnetism. In particular, the presence of a single pair of Weyl points is predicted for a ferromagnetic configuration of Eu spins along the $c$-axis in EuCd$_2$As$_2$. In the search for such phases, we investigate here the effects of hydrostatic pressure in EuCd$_2$As$_2$. For that, we present specific heat, transport and $μ$SR measurements under hydrostatic pressure up to $\sim\,2.5\,$GPa, combined with {\it ab initio} density functional theory (DFT) calculations. Experimentally, we establish that the ground state of EuCd$_2$As$_2$ changes from in-plane antiferromagnetic (AFM$_{ab}$) to ferromagnetic at a critical pressure of $\,\approx\,$2\,GPa, which is likely characterized by the moments dominantly lying within the $ab$ plane (FM$_{ab}$). The AFM$_{ab}$-FM$_{ab}$ transition at such a relatively low pressure is supported by our DFT calculations. Furthermore, our experimental and theoretical results indicate that EuCd$_2$As$_2$ moves closer to the sought-for FM$_c$ state (moments $\parallel$ $c$) with increasing pressure further. We predict that a pressure of $\approx$\,23\,GPa will stabilize the FM$_c$ state, if Eu remains in a 2+ valence state. Thus, our work establishes hydrostatic pressure as a key tuning parameter that (i) allows for a continuous tuning between magnetic ground states in a single sample of EuCd$_2$As$_2$ and (ii) enables the exploration of the interplay between magnetism and topology and thereby motivates a series of future experiments on this magnetic Weyl semimetal. △ Less

Submitted 4 August, 2021; originally announced August 2021.

Comments: 8 figures in main text, 6 figures in Appendix; 14 pages total

Formation of short-range magnetic order and avoided ferromagnetic quantum criticality in pressurized LaCrGe$_3$

Authors: Elena Gati, John M. Wilde, Rustem Khasanov, Li Xiang, Sachith Dissanayake, Ritu Gupta, Masaaki Matsuda, Feng Ye, Bianca Haberl, Udhara Kaluarachchi, Robert J. McQueeney, Andreas Kreyssig, Sergey L. Bud'ko, Paul C. Canfield

Abstract: LaCrGe$_3$ has attracted attention as a paradigm example of the avoidance of ferromagnetic (FM) quantum criticality in an itinerant magnet. By combining thermodynamic, transport, x-ray and neutron scattering as well as $μ$SR measurements, we refined the temperature-pressure phase diagram of LaCrGe$_3$. We provide thermodynamic evidence (i) for the first-order character of the FM transition when it… ▽ More LaCrGe$_3$ has attracted attention as a paradigm example of the avoidance of ferromagnetic (FM) quantum criticality in an itinerant magnet. By combining thermodynamic, transport, x-ray and neutron scattering as well as $μ$SR measurements, we refined the temperature-pressure phase diagram of LaCrGe$_3$. We provide thermodynamic evidence (i) for the first-order character of the FM transition when it is suppressed to low temperatures and (ii) for the formation of new phases at high pressures. From our microscopic data, we infer that short-range FM ordered clusters exist in these high-pressure phases. These results suggest that LaCrGe$_3$ is a rare example, which fills the gap between the two extreme limits of avoided FM quantum criticality in clean and strongly disordered metals. △ Less

Submitted 9 November, 2020; originally announced November 2020.

Comments: 7 pages, 4 figures plus Supplemental Information

Journal ref: Phys. Rev. B 103, 075111 (2021)