Showing 1–50 of 311 results for author: Xu, M

Nonreciprocity reversal of magnetoacoustic attenuation in NiFe alloy thin films

Authors: Mingran Xu, Kei Yamamoto, Kouta Kondou, Zheng Zhu, Liyang Liao, Kiyohiro Adachi, Tomoka Kikitsu, Daisuke Hashizume, Dirk Grundler, Sadamichi Maekawa, Yoshichika Otani

Abstract: Nonreciprocity, the asymmetry of transport, underlies technologies from the diode to the microwave isolator. In a ferromagnet, a surface acoustic wave generates an elliptical effective field with propagation-locked handedness, breaking the reciprocity of its propagation. Despite decades of study on this phenomenon, a method for controlling the sign of the nonreciprocity has remained elusive. Here… ▽ More Nonreciprocity, the asymmetry of transport, underlies technologies from the diode to the microwave isolator. In a ferromagnet, a surface acoustic wave generates an elliptical effective field with propagation-locked handedness, breaking the reciprocity of its propagation. Despite decades of study on this phenomenon, a method for controlling the sign of the nonreciprocity has remained elusive. Here we observe a sign reversal in Ni$_x$Fe$_{100-x}$ films. A 0.8 at.% change across Permalloy's zero-magnetostriction composition, where the magnetoelastic coefficient $b$ changes sign, reverses the handedness of the elliptical effective field and thereby the nonreciprocity, from 78.6% to -61.8%. Angle-dependent measurements and spin-wave-ellipticity modelling show that reversing the sign of $b$ reverses the handedness of the elliptically polarized effective field. Aided by cubic frequency scaling, we resolve the sign of $b$ down to -0.05 MPa in a 10-nm film, establishing nonreciprocity as a nanoscale probe of magnetoelastic coupling. △ Less

Submitted 6 August, 2026; originally announced August 2026.

Comments: 13 pages, 4 figures

Spectral Topology and Non-Bloch Band Theory for Domain-Wall Systems

Authors: Mingtao Xu, Rui Wang, Tian-Shu Deng, Wei Yi

Abstract: We study the spectral topology of one-dimensional non-Hermitian models in a domain-wall configuration, where different domains are arranged in a ring geometry. While eigenstates can localize near an interface under the non-Hermitian skin effect, we show that the localization of an eigenstate originates from the difference in the spectral winding numbers, with respect to the corresponding eigenener… ▽ More We study the spectral topology of one-dimensional non-Hermitian models in a domain-wall configuration, where different domains are arranged in a ring geometry. While eigenstates can localize near an interface under the non-Hermitian skin effect, we show that the localization of an eigenstate originates from the difference in the spectral winding numbers, with respect to the corresponding eigenenergy, between the two adjacent domains. We then obtain the conditions for the generalized Brillouin zone (GBZ) in the complex momentum space, by extending the Ronkin-function formalism to the domain-wall configuration. In addition to the conventional skin modes that correspond to standing waves on individual domains under the open boundary condition, a unique type of traveling-wave-like skin modes emerges, whose construction involves all domains. Besides their difference in the spatial profiles, these two types of modes obey distinct GBZ conditions, making them differentiable on the GBZ. Interestingly, the traveling-wave-like modes further carry a finite flux spectral winding number, indicating their boundary sensitivity. △ Less

Submitted 24 July, 2026; originally announced July 2026.

Comments: 27 pages, 6 figures

Levitated nano-trampoline resonators for magnetic field sensing

Authors: Xianfeng Chen, Nirmala Raj, Matthew R. Chua, Yi Fan Chen, Chenyue Gu, Minxing Xu, Young-Wook Cho, Syed M. Assad, Lu Ding, Ping Koy Lam

Abstract: Levitated systems and high-$Q$ membrane nanomechanical resonators have achieved exceptional sensitivity in precision sensing, but functionalizing such resonators for practical applications without degrading their low dissipation remains challenging. Here, we combine diamagnetic levitation with a high-$Q$ nanomechanical resonator to realize a high-precision magnetometer for sensing weak oscillating… ▽ More Levitated systems and high-$Q$ membrane nanomechanical resonators have achieved exceptional sensitivity in precision sensing, but functionalizing such resonators for practical applications without degrading their low dissipation remains challenging. Here, we combine diamagnetic levitation with a high-$Q$ nanomechanical resonator to realize a high-precision magnetometer for sensing weak oscillating magnetic fields. A macroscopic diamagnetically levitated graphite plate acts as a free-floating proof mass that couples strongly to magnetic fields, converting them into mechanical motion that is resonantly amplified by a low-dissipation nano-trampoline resonator. Operating at room temperature and without magnetic shielding, we achieve a peak magnetic-field sensitivity of $4.5\, \mathrm{pT}/\sqrt{\mathrm{Hz}}$ using a resonator with a mechanical quality factor of $Q=6\times10^{6}$ at $443\, \mathrm{kHz}$. The system sensitivity is limited by thermomechanical noise. With further improvements in mechanical $Q$, this hybrid levitated platform offers a pathway toward femtotesla-level AC magnetic-field sensing, establishing diamagnetically levitated nanomechanical resonators as a new class of high-sensitivity magnetometers at room temperature. △ Less

Submitted 24 July, 2026; originally announced July 2026.

Comments: 16 pages, 13 figures

Strong Quantum Mpemba Effect from Exact Slow-Mode Selection in Constrained Rydberg Chains

Authors: Mingdi Xu, Kaixiang Lu, Zijun Wei, Xiang-Ping Jiang, Haiping Hu, Lei Pan

Abstract: CStrong quantum Mpemba acceleration requires suppressing the slowest visible Liouvillian relaxation channel, but a robust many-body mechanism for enforcing such suppression remains challenging. We identify such a mechanism in locally dephased constrained Rydberg chains through exact slow-mode selection. For constrained single-spin-flip Hamiltonians, local dephasing turns the Hamiltonian itself int… ▽ More CStrong quantum Mpemba acceleration requires suppressing the slowest visible Liouvillian relaxation channel, but a robust many-body mechanism for enforcing such suppression remains challenging. We identify such a mechanism in locally dephased constrained Rydberg chains through exact slow-mode selection. For constrained single-spin-flip Hamiltonians, local dephasing turns the Hamiltonian itself into an exact left Liouvillian eigenmode, $\mathcal L^\dagger(H)=-γH$. A finite-temperature reference state generically overlaps with this $H$-like slow mode, whereas translationally invariant states with $\mathrm{Tr}(Hρ_0)=0$ remove it and are confined to the $Q=0$ operator sector. When the next visible $Q=0$ mode decays faster, these selected states exhibit a strong quantum Mpemba effect. We demonstrate this mechanism in the PXP chain for a zero-energy scar eigenstate, the all-zero product state, and a translation-invariant $Z_2$ cat state, and show that it persists in the $(2,3)$ model and the longer-range blockade family. Our results identify Liouvillian mode visibility, rather than special scar wave functions, as the organizing principle for anomalously fast relaxation in constrained open quantum systems. △ Less

Submitted 4 August, 2026; v1 submitted 20 July, 2026; originally announced July 2026.

Comments: 8+13 pages, 4 figures, comments are welcome

Phase-shifted multicomponent spin-charge nematicity in an altermagnet

Authors: Christopher Candelora, Siyu Cheng, Muxian Xu, Keyu Zeng, Hengxin Tan, Younghun Hwang, Binghai Yan, Federico Mazzola, Ziqiang Wang, Ilija Zeljkovic

Abstract: Altermagnets host spin-split Fermi surfaces without net magnetization. This intrinsically multicomponent electronic setting raises the possibility that familiar correlated electron phases acquire unconventional spin-charge structure. Here we report the discovery of altermagnetic nematicity in Co0.25NbSe2. Using spectroscopic-imaging scanning tunneling microscopy and spin-polarized scanning tunneli… ▽ More Altermagnets host spin-split Fermi surfaces without net magnetization. This intrinsically multicomponent electronic setting raises the possibility that familiar correlated electron phases acquire unconventional spin-charge structure. Here we report the discovery of altermagnetic nematicity in Co0.25NbSe2. Using spectroscopic-imaging scanning tunneling microscopy and spin-polarized scanning tunneling microscopy, we find that the three nominally C3-related directions lose rotational equivalence in the zero-field state, in both charge and spin-sensitive tunneling channels. Strikingly, the dominant spin-sensitive component is shifted by one C3 sector relative to the dominant charge component, revealing a phase-shifted spin-charge nematic response. A phenomenological theory shows that altermagnetic order favors a finite relative phase between the charge and spin-sensitive nematic components -- C3 lattice pinning frustrates this preferred offset and selects the observed phase locking. These results establish altermagnetic nematicity as a new form of multicomponent electronic liquid-crystal order and point to a potentially generic route by which altermagnets can transform conventional correlated phases into symmetry-engineered spin-charge orders. △ Less

Submitted 14 July, 2026; originally announced July 2026.

Comments: submitted version June 1, 2026

Analytical and numerical solutions to the non-diffusive Stefan problem

Authors: Matthew Van Ham, Minghan Xu, Samuel Huberman

Abstract: In this work, the Maxwell--Cattaneo--Vernotte (MCV) equation is used to model the one-dimensional hyperbolic Stefan problem in the limit of a small Stefan number (Ste $\ll$ 1). The solutions are approximated with perturbation series expansions using a reformulation in which time is expressed as a function of the solid-liquid interface position. The first proposed solution is derived in a framework… ▽ More In this work, the Maxwell--Cattaneo--Vernotte (MCV) equation is used to model the one-dimensional hyperbolic Stefan problem in the limit of a small Stefan number (Ste $\ll$ 1). The solutions are approximated with perturbation series expansions using a reformulation in which time is expressed as a function of the solid-liquid interface position. The first proposed solution is derived in a framework that considers diffusive heat transfer at the phase change interface, for analytic tractability. Two rectification strategies are proposed to address the asymptotic divergence present in this formulation: a rescaled inner solution which is then combined with the outer solution to yield a composite solution, and size-dependent thermo-physical system parameters for better capture of hyperbolic effects at the phase change interface. The resulting interface profiles exhibit a characteristic parabolic-like shape, consistent with diffusive Stefan problem findings, with pronounced early-time hyperbolic effects at larger thermal relaxation times. Parametric studies are done over three pertinent variables in the dimensionless system: the Stefan number ($\mathrm{Ste}$), the dimensionless thermal relaxation time ($\widetilde τ$), and the thermal diffusivity ($α$). The studies suggest that model error scales with the Stefan number in accordance with the theoretical truncation error of the perturbation expansion. Additionally, larger values of $\widetilde τ$ amplify early-time hyperbolic effects, thereby increasing model error, while larger $α$ extends the relative temporal domain over which these hyperbolic effects remain significant, also corresponding to an increase in model error. △ Less

Submitted 13 July, 2026; originally announced July 2026.

Comments: 35 pages, 12 figures

MSC Class: 80A22; 41A60

Notes on remanent magnetization measurements in superconductors and hard ferromagnets

Authors: Sergey L. Bud'ko, Mingyu Xu, Weiwei Xie, Chaowei Hu, Ni Ni, Paul C. Canfield

Abstract: Data on zero applied field measurements of remanent magnetization and magnetic relaxation in a BCS superconductor LuNi2B2C and several hard ferromagnets are presented and compared. Apparent similarities and differences, in particular in Thermoremanent Magnetization (TRM) - like, Isothermal Remanent Magnetization (IRM) - like, and remanent magnetization measurements with zigzag temperature sweep me… ▽ More Data on zero applied field measurements of remanent magnetization and magnetic relaxation in a BCS superconductor LuNi2B2C and several hard ferromagnets are presented and compared. Apparent similarities and differences, in particular in Thermoremanent Magnetization (TRM) - like, Isothermal Remanent Magnetization (IRM) - like, and remanent magnetization measurements with zigzag temperature sweep measurements are outlined. It is discussed how these results could be relevant for the magnetization measurements in diamond anvil cells. △ Less

Submitted 21 June, 2026; originally announced June 2026.

Physics-governed executable modelling of triboelectric nanogenerators

Authors: Hongfa Zhao, Baiqiao Wang, Tiancong Zhao, Chun Jin, Hanlin Zhou, Mingrui Shu, Minyi Xu, Liwei Lin, Wenbo Ding, Zhong Lin Wang

Abstract: Predictive modelling of triboelectric nanogenerators (TENGs) remains fragmented across analytical theories, finite-geometry solvers and disconnected simulation workflows. These disparate approaches must be unified into an executable framework to advance quantitative TENG research.Here we introduce a charge-defined modelling framework and implement it as TENG-CLAW, a physics-governed platform for t… ▽ More Predictive modelling of triboelectric nanogenerators (TENGs) remains fragmented across analytical theories, finite-geometry solvers and disconnected simulation workflows. These disparate approaches must be unified into an executable framework to advance quantitative TENG research.Here we introduce a charge-defined modelling framework and implement it as TENG-CLAW, a physics-governed platform for traceable TENG simulation. The framework establishes a self-consistent electrostatic hierarchy in which triboelectric charges, pre-charging charges and compensating electrode charges serve as defining state variables.This hierarchy connects the infinite plate analytical limit for near-uniform fields with finite-geometry numerical formulations required for edge-dominated devices. Built on this basis, TENG-CLAW converts user-defined research requests into physically admissible simulation tasks, so that generated outputs are tied to explicit charge states, boundary conditions, solver routes and reusable artifacts across spatial, temporal, field-level, comparative and reporting workflows. This work establishes a rigorous computational basis for interpreting TENG mechanisms and provides reproducible research infrastructure for simulation and physics-guided device design. △ Less

Submitted 22 June, 2026; originally announced June 2026.

The FAST Framework: Developing a Data-Efficient Machine Learning Potential to Decode Superionic Transition-Induced Thermophysical and Kinetic Anomalies in UO2 under Extreme Conditions

Authors: Fengnian Zhuang, Gaosheng Yan, Hong Chen, Yi Zhang, Wenshan Yu, Minglong Xu, Shengping Shen

Abstract: Uranium dioxide ($UO_2$) serves as the predominant nuclear fuel globally. Despite its widespread application, evaluating its mechanical, thermophysical, and species transport behaviors under extreme accident scenarios remains a formidable challenge for conventional experimental and computational methods. To address this, we develop a versatile machine learning interatomic potential (MLIP) for… ▽ More Uranium dioxide ($UO_2$) serves as the predominant nuclear fuel globally. Despite its widespread application, evaluating its mechanical, thermophysical, and species transport behaviors under extreme accident scenarios remains a formidable challenge for conventional experimental and computational methods. To address this, we develop a versatile machine learning interatomic potential (MLIP) for $UO_2$ by proposing an efficient training strategy, termed the "FAST" (Fine-tuning via Active-learning and Superionic-Targeting) framework. Our "FAST" framework integrates superionic transition-targeted sampling with active learning-enhanced exploration to efficiently construct a highly compact dataset comprising only 500 configurations for fine-tuning a foundation model. By rigorously accounting for the strong correlation of uranium 5f electrons and antiferromagnetic (AFM) ground state during DFT labeling, we train a robust DFT-level neuroevolution potential (NEP) for $UO_2$. We demonstrate that this NEP exhibits superior predictive capability for various physical properties, encompassing mechanical, defect, thermophysical, and ionic diffusion over an extensive temperature range. Moreover, this NEP accurately captures the anomalous thermophysical and kinetic behaviors triggered by superionic transition. Specifically, it reproduces both the $λ$-peak in linear thermal expansion coefficient (LTEC) and "non-Arrhenius" anionic diffusion. Crucially, NEP-based simulations elucidate the microscopic origins underlying these anomalies: the pre-melting of oxygen sublattice and resultant kinetic decoupling between U and O ions. △ Less

Submitted 19 June, 2026; originally announced June 2026.

Comments: 51 pages,14 figures

Site Preferences and "Coloring Problem" in Cu-doped BiMn$_7$O$_{12}$ Quadruple Perovskite

Authors: Cheng Peng, Mingyu Xu, Yang Zhang, Ismail El Baggari, Jie Li, Weiwei Xie

Abstract: Lightly Cu-doped BiMn$_7$O$_{12}$ (x = 0.05, 0.10, and 0.15) was investigated using high-pressure synthesis, single-crystal X-ray diffraction, pair distribution function (PDF) analysis, STEM, magnetic measurements, and first-principles calculations. All compositions retain an average monoclinic $I$2/$m$ structure, while Cu substitution progressively suppresses the monoclinic distortion and drives… ▽ More Lightly Cu-doped BiMn$_7$O$_{12}$ (x = 0.05, 0.10, and 0.15) was investigated using high-pressure synthesis, single-crystal X-ray diffraction, pair distribution function (PDF) analysis, STEM, magnetic measurements, and first-principles calculations. All compositions retain an average monoclinic $I$2/$m$ structure, while Cu substitution progressively suppresses the monoclinic distortion and drives the lattice toward a pseudo-cubic metric symmetry. PDF analysis reveals increasing local structural disorder and reduced medium-range coherence with increasing Cu concentration, despite preservation of the overall quadruple-perovskite framework. Single-crystal refinements indicate enhanced electron density at the octahedral Mn B sites, suggesting preferential Cu occupation within the MnO$_6$ network rather than the conventional square-planar sites expected for Cu$^{2+}$. Magnetic measurements reveal two characteristic anomalies near $T_1$ ~ 100-120 K and $T_2$ ~ 50-60 K, together with pronounced magnetic irreversibility, field-dependent hysteresis, and unsaturated magnetization. Increasing Cu concentration progressively suppresses the low-temperature magnetic state and weakens the field-induced moment. First-principles calculations favor Cu occupation at the square-planar sites, contrasting with the experimental refinements and highlighting strong competitions among local bonding, short-range disorder, and metastability in this highly frustrated quadruple perovskite system. △ Less

Submitted 10 June, 2026; originally announced June 2026.

Comments: 24+3 pages, 6+4 figures

Superconductivity in the high-pressure tetragonal phase of UTe2

Authors: Yuhang Deng, Gabriel Mee, Tyler Wannamaker, Keke Feng, Mingyu Xu, Weiwei Xie, M. Brian Maple

Abstract: Electrical transport and magnetic measurements have been made on UTe2 under pressure P up to approximately 16 GPa to determine the superconducting transition temperature Tc vs P phase diagram in the high-pressure tetragonal phase. Superconductivity emerges near 5 GPa, coincident with the orthorhombic to tetragonal phase transition; in the tetragonal phase, Tc reaches a maximum value of approximate… ▽ More Electrical transport and magnetic measurements have been made on UTe2 under pressure P up to approximately 16 GPa to determine the superconducting transition temperature Tc vs P phase diagram in the high-pressure tetragonal phase. Superconductivity emerges near 5 GPa, coincident with the orthorhombic to tetragonal phase transition; in the tetragonal phase, Tc reaches a maximum value of approximately 4 K at 6 GPa and then decreases with P and appears to vanish near 18 GPa. Tetragonal UTe2 has a relatively small upper critical field Hc2(0) $\approx$ 1.2 T at 5.3 GPa, smaller than the Pauli paramagnetic limit, and is orbitally limited with a coherence length $ξ$tetra $\approx$ 16.5 nm. This small value of Hc2(0) favors more conventional superconductivity; in contrast, the large values of Hc2(T) for orthorhombic UTe2 exceed the Pauli paramagnetic limit in all three crystallographic directions and have been attributed to unconventional superconductivity, widely believed to involve spin-triplet pairing. The temperature-pressure phase diagram of UTe2 shows a striking dichotomy: a narrow, fragile, unconventional superconducting region in the orthorhombic phase vs a broad, robust, and more conventional superconducting dome in the tetragonal phase. This dichotomy is consistent with the proposal that U-dimers, present (absent) in the orthorhombic (tetragonal) phase, may play a role in spin-triplet superconductivity of orthorhombic UTe2. In the tetragonal phase, the normal-state electrical resistivity $ρ$(T) exhibits metallic behavior with a knee between 200 and 240 K that depends weakly on P and most likely marks the onset of a transition to a magnetically ordered phase that coexists with superconductivity. △ Less

Submitted 5 June, 2026; originally announced June 2026.

Unconventional crystallization pathway bypassing the intermediate cubic phase in phase-change superlattices

Authors: Bai-Qian Wang, Nian-Ke Chen, Yao-Jie Wang, Jia Sun, Yu-Ting Huang, Ming Xu, Shengbai Zhang, Xian-Bin Li

Abstract: The Ge-Sb-Te (GST) superlattice phase-change material is a promising candidate for overcoming the high power-consumption of phase-change memory (PCM). However, the working mechanism of the superlattice PCM remains controversial. Partial amorphization, which is currently considered the most plausible mechanism, remains hotly debated: how does the partially amorphized GST recrystallize into its supe… ▽ More The Ge-Sb-Te (GST) superlattice phase-change material is a promising candidate for overcoming the high power-consumption of phase-change memory (PCM). However, the working mechanism of the superlattice PCM remains controversial. Partial amorphization, which is currently considered the most plausible mechanism, remains hotly debated: how does the partially amorphized GST recrystallize into its superlattice phase instead of the conventionally expected cubic phase? Here, we address this issue using large-scale molecular dynamics simulations enabled by a machine-learning interatomic potential. Starting from a partially melted GST superlattice, we demonstrate that the residual crystalline regions serve as nuclei, enabling the amorphous GST to recrystallize directly into the superlattice phase without passing through the intermediate cubic phase. Moreover, the recrystallized phase is not an ideal superlattice, but rather a structurally ordered and chemically disordered defective superlattice characterized by anti-site defects and stacking faults. The defective superlattice region is also more susceptible to melting than the defect-free superlattice, and thereby can act as the active region of the PCM device. These results help to clarify the longstanding debates concerning the mechanism of superlattice-based PCM. △ Less

Submitted 2 June, 2026; originally announced June 2026.

Comments: 13 pages, 6 figures

Suppression of p-Wave Altermagnetism by Localized 4f Electrons in CeNiAsO

Authors: Jiuxiang Zhang, Yueyang Sun, Honglin Zhou, Jumin Shi, Di Wu, Hongze Gu, Wenjin Mao, Hengrui Dong, Yu Xu, Yinghao Li, Ziling Cao, Taimin Miao, Bo Liang, Neng Cai, Wenpei Zhu, Mingkai Xu, Jiaqi Chen, Chunhong Deng, Bo Liu, Xun Ma, Zhengtai Liu, Mao Ye, Shenjin Zhang, Zhimin Wang, Fengfeng Zhang , et al. (10 additional authors not shown)

Abstract: Altermagnetism, characterized by momentum-dependent spin splitting and zero net magnetization, has so far been explored mainly in weakly or moderately correlated d-electron systems. How symmetry-allowed altermagnetic band splitting manifests in heavy-fermion materials, where magnetic exchange competes with Kondo correlations, remains unclear. Here we use high-resolution angle-resolved photoemissio… ▽ More Altermagnetism, characterized by momentum-dependent spin splitting and zero net magnetization, has so far been explored mainly in weakly or moderately correlated d-electron systems. How symmetry-allowed altermagnetic band splitting manifests in heavy-fermion materials, where magnetic exchange competes with Kondo correlations, remains unclear. Here we use high-resolution angle-resolved photoemission spectroscopy (ARPES) to investigate CeNiAsO, a Kondo-lattice system that was predicted to be a candidate for p-wave altermagnetism. Fermi surface mapping and polarization-dependent ARPES show that the experimentally observed itinerant bands are mainly derived from Ni 3d orbitals, while resonant photoemission reveals that the Ce 4f states remain predominantly localized with residual c-f hybridization. Ultra-low-temperature measurements reveal no resolvable near-Fermi-level p-wave-like exchange splitting on the Ni 3d-derived conduction bands across the successive antiferromagnetic transitions. These experimental observations cannot be captured by an itinerant-4f band-structure description, which predicts a sizable p-wave splitting in the itinerant bands. When the localized Ce 4f character is incorporated, our band structure calculations indicate that the itinerant Ce 4f band weight is shifted away from the Fermi level and the p-wave-like splitting on the Ni 3d-derived bands is reduced to the few-meV scale. These results establish CeNiAsO as a strongly correlated f-electron setting in which the magnetic symmetry allows p-wave-like band splitting, but localized 4f electrons strongly suppress its observable itinerant single-particle signature. △ Less

Submitted 17 June, 2026; v1 submitted 1 June, 2026; originally announced June 2026.

Comments: 22 pages, 4 figures; Revised version corresponding to the journal-submitted manuscript; expanded ARPES analysis and revised discussion

Defect engineering of ultrathin gallium nitride via electric fields for advanced electronic, magnetic, and gas sensing applications

Authors: Yujia Tian, Devesh R. Kripalani, Ming Xue, Kun Zhou

Abstract: Scaling wide-band-gap semiconductors to the ultrathin limit offers a transformative pathway for power electronics, with gallium nitride (GaN) representing a cornerstone material in this class. However, the operational resilience and functional tunability of its two-dimensional form (g-GaN) remain underexplored. This work shifts the focus from idealized systems to the complex materials behavior und… ▽ More Scaling wide-band-gap semiconductors to the ultrathin limit offers a transformative pathway for power electronics, with gallium nitride (GaN) representing a cornerstone material in this class. However, the operational resilience and functional tunability of its two-dimensional form (g-GaN) remain underexplored. This work shifts the focus from idealized systems to the complex materials behavior under realistic conditions, investigating how the synergistic effects of point vacancy defects, strain, and external electric fields govern its electronic, magnetic, and sensing landscapes. We demonstrate that these factors are not merely perturbations but are fundamental to modulating the material response. Our first-principles calculations suggest g-GaN maintains electronic stability under intense electric fields; notably, gallium vacancies are predicted to further extend the theoretical stability limit. While in-plane tension preserves the band gap evolution under an electric field, in-plane compression facilitates low-field metallization. Using nitrogen monoxide (NO) adsorption as a prototype, we find that the interaction is defect-modulated and potentially tunable by electric fields. Analysis of adsorption energetics and diffusion barriers suggests the gallium vacancy may act as a thermodynamic trap for NO. Targeted hybrid-functional (HSE06) validation confirms the reliability of observed adsorption trends and theoretical metallization thresholds, while revealing that precise electronic-exchange treatment is critical for capturing the magnetic ground state of nitrogen vacancies. By systematically examining the geometry, energetics, band structure, density of states, magnetic response, and charge transfer, this study clarifies the interplay between defects and external electric fields, providing insights into theoretical upper bounds for property tuning and semiconductor device engineering. △ Less

Submitted 26 May, 2026; originally announced May 2026.

Comments: 8 figures

Journal ref: ACS Nano (2026) 20, 14378-14391

Symmetry-Induced Relaxation Comb and Strong Quantum Mpemba Effect in Long-Range XXZ Spin Chains

Authors: Zijun Wei, Mingdi Xu, Yefeng Song, Xiang-Ping Jiang, Yangqian Yan, Lei Pan

Abstract: We uncover a symmetry-filtered mechanism for anomalous dissipative relaxation in a long-range XXZ spin chain subject to local dephasing. At the isotropic point, the coherent Hamiltonian has global $SU(2)$ symmetry, whereas the full Liouvillian retains only the $U(1)$ symmetry associated with total magnetization. This structure pins a family of spatially uniform zero-$U(1)$-charge left eigenoperato… ▽ More We uncover a symmetry-filtered mechanism for anomalous dissipative relaxation in a long-range XXZ spin chain subject to local dephasing. At the isotropic point, the coherent Hamiltonian has global $SU(2)$ symmetry, whereas the full Liouvillian retains only the $U(1)$ symmetry associated with total magnetization. This structure pins a family of spatially uniform zero-$U(1)$-charge left eigenoperators with exact eigenvalues $λ=-2q$, forming a Liouvillian relaxation comb. For the ferromagnetic Dicke ground state, the overlap envelope on this comb is known exactly at finite size and becomes Gaussian in the large-$S$ limit. Since higher-$q$ components decay rapidly, the $q=1$ comb tooth controls the long-time dynamics and yields universal $D(t)\sim e^{-2t}$ relaxation independent of system size and interaction range. This mode-accessibility filtering realizes a spectral strong quantum Mpemba effect: an initially farther state relaxes faster than closer thermal states because slow non-steady Liouvillian modes are inaccessible. Weak breaking of the Hamiltonian $SU(2)$ symmetry restores slow-mode overlap and suppresses this acceleration. △ Less

Submitted 28 July, 2026; v1 submitted 20 May, 2026; originally announced May 2026.

Defect Control via Cu Enrichment Enhances Multifunctional Properties in the Polar Semiconductor Cu1+xMn1-ySiTe3

Authors: Subrata Ghosh, Yu Liu, Saugata Sarker, Boyang Zheng, Sreekant Anil, Soumi Mondal, Yuxi Zhang, Sai Venkata Gayathri Ayyagari, Mingyu Xu, Yingdong Guan, Tsung-Han Yang, Xiaoping Wang, Vincent H. Crespi, Nasim Alem, Weiwei Xie, Venkatraman Gopalan, Qiang Zhang, Zhiqiang Mao

Abstract: Polar materials have recently attracted significant interest due to their rich multifunctional properties. The chalcogenide polar semiconductor Cu1-xMn1+ySiTe3 (Cu-deficient) is an emerging multiferroic system in which electric polarization is coupled to magnetization. However, its macroscopic ferroelectric polarization is strongly suppressed due to the presence of a high density of stacking fault… ▽ More Polar materials have recently attracted significant interest due to their rich multifunctional properties. The chalcogenide polar semiconductor Cu1-xMn1+ySiTe3 (Cu-deficient) is an emerging multiferroic system in which electric polarization is coupled to magnetization. However, its macroscopic ferroelectric polarization is strongly suppressed due to the presence of a high density of stacking faults. In this work, we demonstrate that these crystal defects, likely originating from non-stoichiometry, can be substantially reduced by increasing the Cu content. Cu-enriched samples, Cu1+xMn1-ySiTe3, crystallize in a noncentrosymmetric monoclinic structure (space group Pm) as the Cu-deficient counterpart but show a nearly stacking-fault-free phase, which is attributed to the emergence of an interstitial site. Consequently, the Cu-enriched samples show a pronounced enhancement of the second-harmonic generation (SHG) response compared to Cu-deficient compositions. Magnetically, the Cu-enriched crystals retain long-range antiferromagnetic order with a Neel temperature of TN ~ 33 K without a glassy state but manifest a distinct spin-flop transition along the polar b-axis that is absent in the Cu-deficient compositions. Furthermore, the electronic ground state evolves from insulating to doped semiconducting behavior upon Cu enrichment. Together, these results establish this material system as a unique and versatile platform for elucidating the interplay among composition, crystal defects, and multifunctional properties, offering a route to design magnetic polar systems with tunable quantum functionalities. △ Less

Submitted 18 May, 2026; originally announced May 2026.

Comments: 23 pages

Experimental investigation of altermagnetic order in Cr-doped FeSb2

Authors: A K M Ashiquzzaman Shawon, Eoghan Downey, Shane Smolenski, Thomas J. Hicken, Tatenda Kanyowa, Amir Henderson, Si Athena Chen, Mingyu Xu, Trisha Musall, Rafael Lopes Sabainsk, Zachary J. Morgan, Wei Tian, Yuan Zhu, Weiwei Xie, Elena Gati, Lu Li, Zurab Guguchia, Huibo Cao, Na Hyun Jo

Abstract: Altermagnets are a class of materials with compensated magnetic moments, in which spin sublattices are related by specific rotational symmetries other than inversion or translation. This allows time-reversal symmetry to be broken without a net magnetization. Cr-doped FeSb2 has been theoretically proposed as a candidate d-wave altermagnetic system, yet its magnetic ground state has remained unresol… ▽ More Altermagnets are a class of materials with compensated magnetic moments, in which spin sublattices are related by specific rotational symmetries other than inversion or translation. This allows time-reversal symmetry to be broken without a net magnetization. Cr-doped FeSb2 has been theoretically proposed as a candidate d-wave altermagnetic system, yet its magnetic ground state has remained unresolved. Here, we synthesize single crystals of Fe1-xCrxSb2 and investigate their electrical transport and magnetic properties, with a focus on Fe0.85Cr0.15Sb2. Magnetization measurements suggest spin-compensated ordering below ~3.5 K, where magnetic moments align along the crystallographic b-direction. Transport measurements reveal a crossover from large positive to negative magnetoresistance, while an anomalous Hall response emerges below 5 K, indicating time-reversal symmetry breaking. Muon spin relaxation measurements confirm that the magnetic ordering below 3.5 K is bulk in nature. The absence of coherent oscillations in zero-field μSR spectra and of magnetic Bragg intensity in single-crystal neutron diffraction establishes that the magnetically ordered state is short-range or disordered, rather than collinear altermagnetic order. These results demonstrate that Cr-doping alone breaks time-reversal symmetry without stabilizing long-range altermagnetic order in FeSb2. △ Less

Submitted 7 July, 2026; v1 submitted 1 May, 2026; originally announced May 2026.

Chirality Transfer to the Magnetic Sublattice in the Hybrid Perovskite (R)-/(S)-3-Fluoropyrrolidinium Copper(II) Chloride

Authors: Zheng Zhang, Mingyu Xu, Jose L. Gonzalez Jimenez, Stephen Zhang, Weiwei Xie, Xianghan Xu, Daniel B. Straus

Abstract: Incorporating chiral organic cations into organic-inorganic hybrid materials has been shown to enable the inorganic sublattice to display chiroptical properties. We report a new two-dimensional magnetic ($S=1/2$) chiral metal halide perovskite, (R)- and (S)-$(C_4H_9FN)_2CuCl_4$ (where $(C_4H_9FN)^+$ is 3-fluoropyrrolidinium), which consists of Cu-Cl inorganic layers separated by $(C_4H_9FN)^+$ org… ▽ More Incorporating chiral organic cations into organic-inorganic hybrid materials has been shown to enable the inorganic sublattice to display chiroptical properties. We report a new two-dimensional magnetic ($S=1/2$) chiral metal halide perovskite, (R)- and (S)-$(C_4H_9FN)_2CuCl_4$ (where $(C_4H_9FN)^+$ is 3-fluoropyrrolidinium), which consists of Cu-Cl inorganic layers separated by $(C_4H_9FN)^+$ organic cations. The presence of the chiral $(C_4H_9FN)^+$ organic cation induces formation of chiral magnetic order, even though the inorganic sublattice itself is nearly structurally centrosymmetric. We also report the racemic variant, containing an equal amount of (R)- and (S)- cations, which shows no evidence of chiral magnetic order. When the magnetic susceptibility is measured perpendicular to inorganic Cu-Cl layer propagation direction, an antiferromagnetic phase transition at Néel temperature $T_N = 2.23~K$ is observed in both the chiral and racemic materials, and the existence of the magnetic phase transition is supported by specific heat capacity measurements. Field-induced magnetic chirality is observed through the existence of a second-order magnetoelectric effect in the chiral variant, while no magnetoelectric signal is observed for the racemic material, indicating the absence of magnetic chirality. Our findings demonstrate that materials exhibiting chiral magnetic order can be created through the incorporation of a chiral cation into an organic-inorganic hybrid magnetic material, potentially allowing for the design of tailored materials that combine chiral magnetism with other desirable optical and electronic properties that come from structural chirality. △ Less

Submitted 14 August, 2026; v1 submitted 24 April, 2026; originally announced April 2026.

Comments: Version of record. Main text is 10 pages containing 7 figures. The Supporting Information is an additional 13 pages with 11 supplementary figures. Crystallographic data can be obtained from via the joint Cambridge Crystallographic Data Centre (CCDC) and Fachinformationszentrum Karlsruhe Access Structures service at https://ccdc.cam.ac.uk/structures under Deposition Numbers 2543946-2543948

Journal ref: J. Am. Chem. Soc. 148 (2026) 33895-33904

Experimental Quantification of Nonlinear Mode Coupling in Nanomechanical Resonators using Multi-tone Excitation

Authors: Chris F. D. Wattjes, Zichao Li, Minxing Xu, Richard A. Norte, Peter G. Steeneken, Farbod Alijani

Abstract: Nonlinear modal interactions in resonant systems govern a wide range of phenomena, with broad relevance across modern physics and engineering. Yet, experimentally determining the strength of nonlinear coupling in multimode resonators remains highly challenging. Here, we introduce a multi-tone spectroscopy method for identifying nonlinear coupling coefficients directly from experimental data. Our a… ▽ More Nonlinear modal interactions in resonant systems govern a wide range of phenomena, with broad relevance across modern physics and engineering. Yet, experimentally determining the strength of nonlinear coupling in multimode resonators remains highly challenging. Here, we introduce a multi-tone spectroscopy method for identifying nonlinear coupling coefficients directly from experimental data. Our approach employs dual-tone excitation near selected resonances which, in combination with additional probing tones at higher-order modes, generates sideband responses associated with specific modal couplings. These spectral signatures are analyzed using an inverse reconstruction procedure to quantitatively determine the corresponding nonlinear coupling strengths in the frequency domain. Using this method, we determine ten pairwise nonlinear coupling parameters across five modes of highly tensioned nanostrings, enabling the reconstruction of fully experimental, device-specific nonlinear reduced-order models. Our experimentally derived models show excellent agreement with values obtained numerically using finite element based nonlinear reduced-order models. Our method is generic and can be used for the characterization of diverse modal and intermodal couplings in mechanical and hybrid resonant systems. △ Less

Submitted 15 April, 2026; originally announced April 2026.

Anion Ordering and Phase Stability Govern Optical Band Gaps in BaZr(S,Se)3

Authors: Erik Fransson, Michael Xu, Prakriti Kayastha, Kevin Ye, Ida Sadeghi, Rafael Jaramillo, James M. LeBeau, Lucy Whalley, Paul Erhart

Abstract: Chalcogenide perovskites have emerged as promising lead free materials for photovoltaic and thermoelectric applications. Among them, BaZrS3 has attracted particular attention due to its thermal and chemical stability, favorable optoelectronic properties, and low thermal conductivity. Here, we combine molecular dynamics and Monte Carlo simulations based on machine learned interatomic potentials wit… ▽ More Chalcogenide perovskites have emerged as promising lead free materials for photovoltaic and thermoelectric applications. Among them, BaZrS3 has attracted particular attention due to its thermal and chemical stability, favorable optoelectronic properties, and low thermal conductivity. Here, we combine molecular dynamics and Monte Carlo simulations based on machine learned interatomic potentials with scanning transmission electron microscopy to investigate mixing thermodynamics and phase stability in the BaZr(S,Se)3 system. We identify an unusual ordered structure that persists at room temperature, most prominently at 33% S, where S and Se atoms form alternating layers within the crystal. Free energy calculations yield the temperature composition phase diagram, including a nonperovskite delta phase in the Se rich limit and a perovskite phase in the S rich limit, separated by a broad two phase region. Analysis of the dielectric function and the absorption coefficient demonstrates that composition, crystal structure, and anion ordering jointly control the optical band gap. Selenium alloying enables tuning between approximately 1.6 and 1.9eV, while anion ordering within a given composition reduces the gap by about 0.12eV. Lastly, variations between structural polymorphs give rise to band gap differences of up to 0.4eV. △ Less

Submitted 15 April, 2026; originally announced April 2026.

Mott-Derived Local Moments and Kondo Hybridization in a d-electron Kagome lattice

Authors: Xing Zhang, Xintong Li, Boqin Song, Yuyang Xie, Qinghong Wang, Taimin Miao, Shusen Ye, Junhao Liu, Bo Liang, Neng Cai, Hao Chen, Wenpei Zhu, Mingkai Xu, Wei-Jian Li, Shun-Li Yu, Shenjin Zhang, Fengfeng Zhang, Feng Yang, Zhimin Wang, Qinjun Peng, Hanqing Mao, Zhihai Zhu, Guodong Liu, Zuyan Xu, Yi-feng Yang , et al. (3 additional authors not shown)

Abstract: Unlike canonical Kondo lattices in f-electron systems, where localized f orbitalsnaturally provide local moments, d-electron Kondo lattices require a distinct mechanism for local-moment formation. However, the study of d-electron Kondo lattices in bulk materials remains far from settled, particularly with regard to the microscopic origin of the local moments. Here, we report a microscopic mechanis… ▽ More Unlike canonical Kondo lattices in f-electron systems, where localized f orbitalsnaturally provide local moments, d-electron Kondo lattices require a distinct mechanism for local-moment formation. However, the study of d-electron Kondo lattices in bulk materials remains far from settled, particularly with regard to the microscopic origin of the local moments. Here, we report a microscopic mechanism for this process in the bilayer kagome metal CsCr6Sb6, where strong correlations drive a Mott splitting of the kagome flat band to supply the requisite local moments. By combining STM/STS and ARPES, we resolve a spectroscopic hierarchy between high-energy correlation effects and low temperature hybridization. Low-temperature STS reveals a robust asymmetric suppression of the density of states near EF that is well captured phenomenologically by a Fano-type lineshape, while ARPES detects a sharp quasiparticlepeak near EF. These low-energy signatures evolveon the same temperature scale and disappear upon warming, consistent with the onset of Kondo hybridization. At the same time, STS resolves symmetric humps at approximately +-50 mV and ARPES identifies a weakly dispersive feature around 50 meV below EF; unlike the near-EF hybridization signatures, these features persist to substantially higher temperatures. This separation of energy and temperature scales supports a two-stage picture in which a kagome flat band first undergoes correlation-driven splitting into lower and upper Hubbard bands, and the occupied lower Hubbard band supplies the local moments that later hybridize with itinerant electrons at lower temperature. Our results therefore move beyond the phenomenology of a kagome Kondo lattice candidate and instead provide a microscopic spectroscopic picture linking Mottness to Kondo hybridization in a frustrated d-electron system. △ Less

Submitted 3 April, 2026; originally announced April 2026.

Journal ref: Science China-Physics, Mechanics and Astronomy 69, 297413 (2026)

Measuring impurity-induced shifts in Coulomb crystallization

Authors: Mingyao Xu, Aaron A. Smith, Leonid Prokhorov, Vera Guarrera, Giovanni Barontini

Abstract: We report a laboratory measurement of how impurities shift Coulomb crystallization in a strongly interacting ionic system. This is achieved by using laser cooled Ca$^+$ crystals doped with a controlled number of Xe$^{12+}$ highly charged ions. We find that the crystallization threshold is unchanged at low impurity concentration, but shows a clear crossover once the impurity content becomes suffici… ▽ More We report a laboratory measurement of how impurities shift Coulomb crystallization in a strongly interacting ionic system. This is achieved by using laser cooled Ca$^+$ crystals doped with a controlled number of Xe$^{12+}$ highly charged ions. We find that the crystallization threshold is unchanged at low impurity concentration, but shows a clear crossover once the impurity content becomes sufficiently large, after which the shift grows approximately linearly. Complementary measurements reveal that this global effect originates from a local pinning of the crystal around the impurities. We further show how the measured shift could impact standard models of crystallization in white dwarfs and neutron stars. Our results provide an experimental route to incorporating impurity effects into models of multicomponent Coulomb matter, relevant to stellar crystallization and strongly coupled plasmas. △ Less

Submitted 16 March, 2026; originally announced March 2026.

Pressure-Induced Chemical Bonding Effects on Lattice and Magnetic Instabilities in Antiferromagnetic Insulating CaMn$_2$Sb$_2$

Authors: Matt Boswell, Antonio M. dos Santos, Mingyu Xu, Madalynn Marshall, Su-Yang Xu, Weiwei Xie

Abstract: Exotic quantum phenomena often emerge near an electronic delocalization transition (EDT) from an antiferromagnetic insulating phase to a strongly correlated metallic state under pressure. We report the pressure-induced structural and magnetic evolution of the antiferromagnetic insulator CaMn$_2$Sb$_2$. Single-crystal X-ray diffraction reveals a first-order phase transition near 5.4 GPa from a trig… ▽ More Exotic quantum phenomena often emerge near an electronic delocalization transition (EDT) from an antiferromagnetic insulating phase to a strongly correlated metallic state under pressure. We report the pressure-induced structural and magnetic evolution of the antiferromagnetic insulator CaMn$_2$Sb$_2$. Single-crystal X-ray diffraction reveals a first-order phase transition near 5.4 GPa from a trigonal P-3m1 structure to a monoclinic P2$_1$/m phase, accompanied by a ~7% volume collapse. Residual electron density analysis at intermediate pressures reveals charge localization along Mn-Sb chains, signaling electronic instability preceding the structural transition. Bonding analysis indicates anisotropic Mn-Sb orbital reconfiguration under pressure, driving a distorted square-pyramidal geometry. Neutron scattering confirms the transition and identifies a pressure-induced incommensurate magnetic order, distinct from the ambient antiferromagnetic state. In the monoclinic phase, zigzag Mn chains exhibit antiferromagnetic coupling along the ac-plane, enabled by enhanced orbital overlap. These results establish CaMn$_2$Sb$_2$ as a model system for studying the coupling of structural distortion, charge redistribution, and magnetic order in layered Mn pnictides under pressure. △ Less

Submitted 12 March, 2026; originally announced March 2026.

Comments: 28 pages, 6+3 figures

Observation of Iso-Symmetric Structural and Lifshitz Transitions in Quasi-one-dimensional CrNbSe$_5$

Authors: Mingyu Xu, Peng Cheng, Shuyuan Huyan, Wenli Bi, Su-Yang Xu, Sergey L. Bud'ko, Paul C. Canfield, Weiwei Xie

Abstract: Chalcogenides-rich transition metal compounds host a rich landscape of emergent quantum phenomena that are intimately governed by their quasi-one-dimensional chemical-bonding frameworks and their response to external perturbations such as pressure. Here, we report a pressure-induced iso-symmetric structural transition in the quasi-one-dimensional compound CrNbSe$_5$, in which the electronic ground… ▽ More Chalcogenides-rich transition metal compounds host a rich landscape of emergent quantum phenomena that are intimately governed by their quasi-one-dimensional chemical-bonding frameworks and their response to external perturbations such as pressure. Here, we report a pressure-induced iso-symmetric structural transition in the quasi-one-dimensional compound CrNbSe$_5$, in which the electronic ground state is controlled not by symmetry breaking but by a continuous reorganization of local bonding interactions. Applied pressure reversibly tunes CrNbSe$_5$ between semiconducting and semimetallic states, enabling access to low- and high-carrier electronic regimes through direct modulation of metal-chalcogen bonding. High-pressure single-crystal X-ray diffraction directly resolves the evolution of Cr-Se and Nb-Se bond distances, coordination polyhedra, and connectivity, revealing a fully reversible semimetal-semiconductor-semimetal transition driven by gradual yet cooperative bond rearrangements within a preserved crystallographic symmetry. In contrast to chemical substitution, which irreversibly alters composition and introduces disorder, pressure acts as a clean, continuous control parameter that reshapes the bonding landscape without disrupting structural symmetry. These results establish CrNbSe$_5$ as a model system for electronically driven phase switching via tunable chemical bonding, highlighting iso-symmetric bond reorganization as a powerful design principle for pressure-controlled electronic and spintronic functionalities. △ Less

Submitted 12 March, 2026; originally announced March 2026.

Comments: 29 pages, 5+6 figures

Materials Acceleration Platform for Electrochemistry: a Platform for Autonomous Electrochemistry

Authors: Daniel Persaud, Mike Werezak, Mark Xu, Melyne Zhou, Frank Benkel, Xin Pang, Vahid Attari, Brian DeCost, Ashley Dale, Nicholas Senior, Gabriel Birsan, Jason Hattrick-Simpers

Abstract: Corrosion testing is slow, labor-intensive, and sensitive to operator technique, limiting the generation of large, high-quality datasets for data-driven materials discovery. The Materials Acceleration Platform for Electrochemistry (MAP-E) is an autonomous, high-throughput system, capable of performing parallel electrochemical experiments. It integrates robotic liquid handling, sample transfer with… ▽ More Corrosion testing is slow, labor-intensive, and sensitive to operator technique, limiting the generation of large, high-quality datasets for data-driven materials discovery. The Materials Acceleration Platform for Electrochemistry (MAP-E) is an autonomous, high-throughput system, capable of performing parallel electrochemical experiments. It integrates robotic liquid handling, sample transfer with a multi-channel potentiostatic control to extract corrosion metrics without human intervention. Validation against an ASTM G61-analog benchmark demonstrates good reproducibility, with a standard deviation of 75 mV in pitting potential across 32 automated measurements. The platform was then employed to autonomously construct pH-chloride stability diagrams for 304 stainless steel using an uncertainty-driven sampling strategy on a Gaussian process surrogate model. This approach reduces operator involvement and accelerates the exploration of environmental spaces. The MAP-E establishes a framework for autonomous electrochemical experimentation, enabling generation of corrosion datasets that inform materials discovery, alloy design, and durability assessment in service environments. △ Less

Submitted 26 May, 2026; v1 submitted 10 March, 2026; originally announced March 2026.

Comments: 22 pages, 6 figures

Pressure-Induced Structural and Magnetic Evolution in Layered Antiferromagnet YbMn$_2$Sb$_2$

Authors: Mingyu Xu, Matt Boswell, Aya Rutherford, Cheng Peng, Ying Zhou, Shuyang Wang, Zhaorong Yang, Antonio M. dos Santos, Haidong Zhou, Weiwei Xie

Abstract: Electronic states under pressure exhibit unconventional spin and charge dynamics that provide a powerful route to uncover exotic phases in quantum materials. Here, we present the structural, magnetic, and electronic evolution of YbMn$_2$Sb$_2$ under pressure. Single-crystal X-ray diffraction reveals a pressure-induced structural transition from the space group trigonal $P\bar{3}m1$ to the monoclin… ▽ More Electronic states under pressure exhibit unconventional spin and charge dynamics that provide a powerful route to uncover exotic phases in quantum materials. Here, we present the structural, magnetic, and electronic evolution of YbMn$_2$Sb$_2$ under pressure. Single-crystal X-ray diffraction reveals a pressure-induced structural transition from the space group trigonal $P\bar{3}m1$ to the monoclinic $P2_1$/$m$ phase near 3.5 GPa, which remains stable up to 10 GPa. Magnetization measurements display an anomalously weak net magnetic moment and the absence of Curie-Weiss behavior up to 400 K, suggesting the formation of short-range Mn moment pairs that cancel macroscopically and subsequently evolve into long-range order upon cooling. Temperature-dependent resistivity shows semiconducting behavior with a transition at ~119 K at ambient pressure, while pressure induces a dramatic suppression of resistance and the emergence of metallic-like temperature dependence, stabilized beyond 5 GPa. This pressure-driven semiconductor-metal transition is consistent with our density functional theory calculations, confirming the closing of the band gap under compression. Neutron diffraction under pressure identifies an incommensurate magnetic structure with antiparallel correlations between paired spins. Together, these results demonstrate how pressure-driven structural tuning and competing exchange interactions stabilize unconventional magnetic states in this low-dimensional magnetic semiconductor. △ Less

Submitted 10 March, 2026; originally announced March 2026.

Comments: 36 pages 10+6 figures

Journal ref: Advanced Electronic Materials, 2026

Pressure-Stabilized MnSb$_2$ with Complex Incommensurate Magnetic Order

Authors: Mingyu Xu, Matt Boswell, Qing-Ping Ding, Cheng Peng, Aashish Sapkota, Qiang Zhang, Danielle Yahne, Sergey. L. Bud'ko, Yuji Furukawa, Paul. C. Canfield, Raquel A. Ribeiro, Weiwei Xie

Abstract: Marcasite-type compounds have been proposed as promising hosts of exotic magnetic quantum states, yet experimental realizations in stoichiometric, disorder-free systems remain limited. Here, we report the high-pressure stabilization and magnetic characterization of MnSb$_2$, a marcasite-type compound that is thermodynamically metastable under ambient pressure. Single crystals were synthesized usin… ▽ More Marcasite-type compounds have been proposed as promising hosts of exotic magnetic quantum states, yet experimental realizations in stoichiometric, disorder-free systems remain limited. Here, we report the high-pressure stabilization and magnetic characterization of MnSb$_2$, a marcasite-type compound that is thermodynamically metastable under ambient pressure. Single crystals were synthesized using a cubic multi-anvil press, and powder and single-crystal X-ray diffraction confirm the orthorhombic $Pnnm$ structure. These crystals are stable at ambient pressure for a long time up to between 450-500 K. Heat-capacity measurements reveal phase transitions at approximately 220 K and 118 K. Neutron diffraction uncovers an unconventional magnetic ground state below 220 K. Magnetic powder neutron diffraction refinements reveal possible multiple magnetic configurations that provide comparably acceptable fits to the experimental data. While most solutions are consistent with a spin-density-wave (SDW) description, helical models systematically yield inferior agreement factors. Across a broad range of models, the Mn ordered moment reaches a maximum value of approximately 2 $μ_B$ and remains predominantly collinear, with minimal canting along the $c$-axis. At 200 K, the magnetic propagation vector is $q$ = (0, 0.3975, 0.3783); upon cooling, the $b$ component increases toward 0.5, reflecting a temperature-dependent evolution of the modulation. The need for modification of the magnetic model between high and low temperatures further highlights the complex and strongly temperature-dependent nature of the magnetic order in this system. These results establish MnSb$_2$ as a pressure-stabilized marcasite magnet with a highly tunable, complex magnetic ground state and a compelling stoichiometric platform for exploring unconventional magnetic behavior, including potential altermagnetism. △ Less

Submitted 2 July, 2026; v1 submitted 10 March, 2026; originally announced March 2026.

Comments: 34 pages,5+7figures

Emergent quantum phenomena via phase-coherence engineering in infinite-layer nickelate superconductors

Authors: Haoran Ji, Zheyuan Xie, Xiaofang Fu, Zihan Cui, Minghui Xu, Guang-Ming Zhang, Yi-feng Yang, Haiwen Liu, Yi Liu, Liang Qiao, Jian Wang

Abstract: Dimensionality of a physical system, conventionally an invariant geometric characteristic, fundamentally governs the universality class of phase transitions and the landscape of emergent collective phenomena. In low-dimensional or layered high-temperature superconductors, the macroscopic phase coherence of superconducting orders is typically confined in two dimensions, underscoring the critical ro… ▽ More Dimensionality of a physical system, conventionally an invariant geometric characteristic, fundamentally governs the universality class of phase transitions and the landscape of emergent collective phenomena. In low-dimensional or layered high-temperature superconductors, the macroscopic phase coherence of superconducting orders is typically confined in two dimensions, underscoring the critical role of phase fluctuations in determining the overall phase diagrams. Here, we strategically enhance the phase fluctuations by fabricating periodically arranged nano-holes in the infinite-layer nickelate superconducting films, effectively constructing Josephson junction arrays. In the nano-patterned films, the weakening of macroscopic phase coherence drives a two-stage superconducting transition towards an anomalous metallic ground state with saturated resistance. The emergence of charge-2e quantum oscillations manifests the coherence across the array, while an anomalous zero-field magnetoresistance peak signifies the extreme quantum phase fluctuations persisting to ultralow temperatures. Remarkably, with quantum fluctuations enhanced synergistically by nano-patterning and magnetic fields, an anomalous reversal of superconducting anisotropy is observed in Nd-nickelates, where in-plane critical fields fall below out-of-plane values. The evolution of anisotropy may unmask an internal exchange-Zeeman field coupled to the collective electronic states. Our results unveil how superconductivity evolves in response to phase fluctuations, establishing nano-patterning as a powerful paradigm to uncover hidden intertwined orders in strongly correlated systems. △ Less

Submitted 28 February, 2026; originally announced March 2026.

Dissipative charging of tight-binding quantum batteries

Authors: Mingdi Xu, Yiming Liu, Yefeng Song, Xiang-Ping Jiang, Lei Pan

Abstract: We investigate autonomous dissipative charging mechanisms for lattice quantum batteries within the framework of open quantum systems. Focusing on engineered Markovian dissipation, we show that appropriately designed Lindblad jump operators can drive tight-binding systems into highly excited band-edge states, resulting in steady states with large ergotropy. We illustrate this mechanism in a one-dim… ▽ More We investigate autonomous dissipative charging mechanisms for lattice quantum batteries within the framework of open quantum systems. Focusing on engineered Markovian dissipation, we show that appropriately designed Lindblad jump operators can drive tight-binding systems into highly excited band-edge states, resulting in steady states with large ergotropy. We illustrate this mechanism in a one-dimensional tight-binding chain and in a two-dimensional graphene lattice. We find that disorder enhances the charging power, indicating that dissipation-assisted localization effects can be beneficial for energy storage. Moreover, the dissipative charging process remains robust against additional local dephasing noise. Our results establish bond dissipation as an effective and physically transparent mechanism for charging lattice quantum batteries in realistic open-system settings. △ Less

Submitted 24 March, 2026; v1 submitted 19 February, 2026; originally announced February 2026.

Comments: 10 pages, 5 figures, comments are welcome

Quantum Pontus--Mpemba Effect in Dissipative Quasiperiodic Chains

Authors: Yefeng Song, Junxiao Chen, Xiangyu Yang, Mingdi Xu, Xiang-Ping Jiang, Lei Pan

Abstract: We investigate how quasiperiodic spatial structure enables protocol-induced acceleration in open quantum systems by analyzing the Pontus-Mpemba effect in one-dimensional chains subject to Markovian dephasing. The dynamics are governed by a Lindblad superoperator that drives all initial states toward a maximally mixed infinite-temperature steady state, isolating dynamical mechanisms from static equ… ▽ More We investigate how quasiperiodic spatial structure enables protocol-induced acceleration in open quantum systems by analyzing the Pontus-Mpemba effect in one-dimensional chains subject to Markovian dephasing. The dynamics are governed by a Lindblad superoperator that drives all initial states toward a maximally mixed infinite-temperature steady state, isolating dynamical mechanisms from static equilibrium properties. Considering two representative quasiperiodic models, namely a tight-binding chain with a mosaic potential and its extension with power-law long-range hopping, we show that a properly engineered two-step protocol, in which the system is first steered to a finite temperature intermediate state, yields a strictly shorter overall relaxation time than direct evolution from the same initial configuration. This protocol-induced acceleration persists for both initially localized and extended eigenstates and remains robust in the presence of long-range hopping. A Liouvillian spectral analysis reveals that the mechanism originates from a redistribution of spectral weight that suppresses overlap with the slowest decay modes, rather than from any modification of the decay spectrum itself. Our results establish quasiperiodic chains as a controlled setting for engineering relaxation pathways through Liouvillian spectral structure. △ Less

Submitted 17 February, 2026; originally announced February 2026.

Comments: All comments are welcome!

A scalable non-superconducting tunnel junction technology

Authors: Juho Luomahaara, Kristupas Razas, Omid Sharifi Sedeh, Renan P. Loreto, Janne S. Lehtinen, Mingchi Xu, Armel A. Cotten, Aldo Tarascio, Peter Müller, Nikolai Yurttagül, Lassi Lehtisyrjä, Leif Grönberg, Christian P. Scheller, Jonathan R. Prance, Michael D. Thompson, Richard P. Haley, Mika Prunnila, Dominik M. Zumbühl

Abstract: Tunnel junctions are one of the key elements of chip-scale microsystems serving various technologies from classical microelectronics to quantum information. Aluminium and its oxide (AlOx) have dominated cryogenic tunnel junction technology for decades due to the high quality of AlOx barriers and Al superconducting properties below 1.2 K. However, many applications require non-superconducting junct… ▽ More Tunnel junctions are one of the key elements of chip-scale microsystems serving various technologies from classical microelectronics to quantum information. Aluminium and its oxide (AlOx) have dominated cryogenic tunnel junction technology for decades due to the high quality of AlOx barriers and Al superconducting properties below 1.2 K. However, many applications require non-superconducting junctions, either standalone or in combination with superconducting technology, motivating efforts to suppress Al superconductivity through magnetic fields, doping, or proximity effects -- approaches that so far suffered from integration compatibility and scalability issues. Here, we present a CMOS-compatible normal-metal tunnel junction technology based on TiW alloy and AlOx barriers. We demonstrate wafer-scale fabrication of TiW/Al-AlOx/TiW junctions and validate their performance in Coulomb blockade thermometers operating down to 20 mK, confirming robust normal-state behavior. This TiW-based architecture offers a scalable solution for non-superconducting tunnel junctions across a broad temperature range, enabling integration into advanced cryogenic, quantum and nanoelectronic chip-level systems. △ Less

Submitted 16 February, 2026; originally announced February 2026.

Comments: 9 pages, 6 figures; equal contribution of J.L., K.R., O.S.S, and R.P.L

Coexistence of Antiferromagnetic Spin Fluctuations and Superconductivity in La2SmNi2O7 Thin Films

Authors: Minhui Xu, Yibo Wang, Jia Liu, Long Cheng, Shuyin Li, Shuaishuai Yin, Xu Zheng, Lixin Yu, Aidi Zhao, Xiaolong Li, Jiandi Zhang, Xiaofang Zhai

Abstract: The interplay between magnetic fluctuations and superconductivity is fundamental for understanding unconventional high-temperature superconductors. In the recently discovered Ruddlesden-Popper phase nickelates-which achieve superconducting transition temperatures up to ~100 K-this connection has been theoretically predicted but experimentally unverified. Using compressively strained La2SmNi2O7 thi… ▽ More The interplay between magnetic fluctuations and superconductivity is fundamental for understanding unconventional high-temperature superconductors. In the recently discovered Ruddlesden-Popper phase nickelates-which achieve superconducting transition temperatures up to ~100 K-this connection has been theoretically predicted but experimentally unverified. Using compressively strained La2SmNi2O7 thin films, we report direct evidence for this interplay. We observe a characteristic 'Mexican hat'-shaped magnetoresistance, a signature of superconductivity coexisting with emergent antiferromagnetic (AFM) fluctuations. This distinctive feature arises from a competition between the magnetic field's suppression of AFM fluctuation-driven scattering and its suppression of superconducting fluctuations. We quantify these AFM fluctuations by a crossover field, B*, whose magnitude decreases with increasing temperature and vanishes near the superconducting onset-behavior contrasting sharply with that in high-Tc cuprates. Our results establish not merely coexistence, but also a direct and novel correlation between AFM instability and superconductivity in nickelates, offering crucial insight into their pairing mechanism. △ Less

Submitted 8 February, 2026; originally announced February 2026.

Electronic Structure and Superconducting Gap of HgBa$_2$Ca$_2$Cu$_3$O$_{8+δ}$ Revealed by Laser-Based Angle-Resolved Photoemission Spectroscopy

Authors: Taimin Miao, Wenshan Hong, Qinghong Wang, Shanshan Zhang, Bo Liang, Wenpei Zhu, Neng Cai, Mingkai Xu, Shenjin Zhang, Fengfeng Zhang, Feng Yang, Zhimin Wang, Qinjun Peng, Zuyan Xu, Hanqing Mao, Zhihai Zhu, Xintong Li, Guodong Liu, Lin Zhao, Yuan Li, X. J. Zhou

Abstract: The spatially-resolved laser-based high resolution angle resolved photoemission spectroscopy (ARPES) measurements have been performed on the optimally-doped HgBa$_2$Ca$_2$Cu$_3$O$_{8+δ}$ (Hg1223) superconductor with a $T_c$ at 133 K. Two distinct regions are identified on the cleaved surface: the single Fermi surface region where only one Fermi surface is observed, and the double Fermi surface reg… ▽ More The spatially-resolved laser-based high resolution angle resolved photoemission spectroscopy (ARPES) measurements have been performed on the optimally-doped HgBa$_2$Ca$_2$Cu$_3$O$_{8+δ}$ (Hg1223) superconductor with a $T_c$ at 133 K. Two distinct regions are identified on the cleaved surface: the single Fermi surface region where only one Fermi surface is observed, and the double Fermi surface region where two Fermi surface sheets are resolved coming from both the inner (IP) and outer (OP) CuO$_2$ planes. The electronic structure and superconducting gap are measured on both of these two regions. In both cases, the observed electronic states are mainly concentrated near the nodal region. The momentum dependence of superconducting gap deviates from the standard d-wave form. These results indicate that the surface electronic structure of Hg1223 behaves more like that of underdoped cuprates. △ Less

Submitted 5 February, 2026; originally announced February 2026.

Comments: 14 pages, 5 figures

Journal ref: Chinese Physics B 35, 027402 (2026)

Higher-order Liouvillian exceptional points in the dissipative dynamics of quadratic fermions

Authors: Mingtao Xu, Wei Yi

Abstract: We propose a general class of open fermionic models where quadratic Liouvillians governing the dissipative dynamics feature analytically characterized higher-order exceptional points (EPs). Invoking the formalism of third quantization, we show that, among the multiple EPs of Liouvillian, an EP with its order approaching the system size arises as the dominant modes of the system at long times, lead… ▽ More We propose a general class of open fermionic models where quadratic Liouvillians governing the dissipative dynamics feature analytically characterized higher-order exceptional points (EPs). Invoking the formalism of third quantization, we show that, among the multiple EPs of Liouvillian, an EP with its order approaching the system size arises as the dominant modes of the system at long times, leading to a gapless Liouvillian spectrum. By introducing perturbations, in the form of many-body quantum-jump processes, these higher-order EPs break down, leading to finite Liouvillian gaps with fractional power-law scalings. While the power-law scaling is a signature of the higher-order EP, its explicit form is sensitively dependent on the many-body perturbation. Finally, we discuss the long-time dynamics which can serve as detectable signals for the higher-order Liouvillian EPs. △ Less

Submitted 18 July, 2026; v1 submitted 30 January, 2026; originally announced February 2026.

Comments: 12 pages, 3 figures

Journal ref: Phys. Rev. A 113, 062455(2026)

Electronic Origin of Density Wave Orders in a Trilayer Nickelate

Authors: Jiangang Yang, Jun Zhan, Taimin Miao, Mengwu Huo, Qichen Xu, Yinghao Li, Yuyang Xie, Bo Liang, Neng Cai, Hao Chen, Wenpei Zhu, Mingkai Xu, Shenjin Zhang, Fengfeng Zhang, Feng Yang, Zhimin Wang, Qinjun Peng, Hanqing Mao, Xintong Li, Zhihai Zhu, Guodong Liu, Zuyan Xu, Jiangping Hu, Xianxin Wu, Meng Wang , et al. (2 additional authors not shown)

Abstract: The discovery of superconductivity in Ruddlesden-Popper nickelates has established a new frontier in the study of high-temperature superconductors. However, the underlying pairing mechanism and its relationship to the material's electronic and magnetic ground states remain elusive. Since unconventional superconductivity often emerges from a complex interplay of magnetic correlations, elucidating t… ▽ More The discovery of superconductivity in Ruddlesden-Popper nickelates has established a new frontier in the study of high-temperature superconductors. However, the underlying pairing mechanism and its relationship to the material's electronic and magnetic ground states remain elusive. Since unconventional superconductivity often emerges from a complex interplay of magnetic correlations, elucidating the magnetic ground state of the nickelates at ambient pressure is crucial for understanding the emergence of superconductivity under high pressure. Here, we combine high-resolution angle-resolved photoemission spectroscopy with tight-binding model simulation to investigate the electronic structure of the representative trilayer Ruddlesden-Popper nickelate La$_4$Ni$_3$O$_{10}$. We provide the first experimental evidence of band splitting induced by interlayer coupling and further resolve the momentum-dependent density wave gap structures along all the Fermi surfaces. Our findings identify the mirror-selective Fermi surface nesting as the origin of the interlayer antiferromagnetic spin density wave and demonstrate the dominant role of Ni-3d$_{z^2}$ orbitals in the low-energy physics of La$_4$Ni$_3$O$_{10}$. These results provide a fundamental framework for understanding the magnetic interactions and high-temperature superconductivity mechanism in the Ruddlesden-Popper nickelate family. △ Less

Submitted 30 January, 2026; originally announced January 2026.

Comments: 22 pages, 5 figures

Synthesis of Monolayer Ice on a Hydrophobic Metal Surface

Authors: Qiaoxiao Zhao, Meiling Xu, Dong Li, Zhicheng Gao, Yudian Zhou, Wenbo Liu, Jingyan Chen, Peng Cheng, Sheng Meng, Kehui Wu, Yanchao Wang, Lan Chen, Baojie Feng

Abstract: Understanding water-metal interactions is central to disciplines spanning catalysis, electrochemistry, and atmospheric science. Monolayer ice phases are well established on hydrophilic surfaces, where strong water-substrate interactions stabilize ordered hydrogen-bond networks. In contrast, their formation on hydrophobic metals has been deemed ther-modynamically unfavourable, with water typically… ▽ More Understanding water-metal interactions is central to disciplines spanning catalysis, electrochemistry, and atmospheric science. Monolayer ice phases are well established on hydrophilic surfaces, where strong water-substrate interactions stabilize ordered hydrogen-bond networks. In contrast, their formation on hydrophobic metals has been deemed ther-modynamically unfavourable, with water typically assembling into amorphous films, three-dimensional crystallites, or interlocked bilayer ice. Here, we demonstrate the synthesis of a monolayer ice phase on the hydrophobic Au(111) surface using a low-energy-electron-assisted growth method. Combined experimental characterizations including low-energy electron diffraction, angle-resolved photoemission spectroscopy, and X-ray photoelectron spectroscopy, complemented by first-principles calculations, prove that the monolayer ice phase composes of intact water molecules. This approach provides a generalizable strategy for stabilizing ordered two-dimensional ice on inert substrates and offers new insight into the interplay between water and low-energy electrons at hydrophobic interfaces. △ Less

Submitted 29 January, 2026; originally announced January 2026.

Journal ref: J. Am. Chem. Soc. (2026)

Unusual Dual Flat Bands and two-dimensional Dirac-node Arc State in Kagome Metal Ni3In2S2

Authors: Bo Liang, Yichen Liu, Jie Pang, Hanbin Deng, Taimin Miao, Wenpei Zhu, Neng Cai, Tiantian Zhang, Jiayu Liu, Zhicheng Jiang, Zhanfeng Liu, Hongen Zhu, Yuliang Li, Tongrui Li, Mingkai Xu, Hao Chen, Xiaolin Ren, Chaohui Yin, Yingjie Shu, Yiwen Chen, Yu-Tian Zhang, Zhengtai Liu, Dawei Shen, Mao Ye, Fengfeng Zhang , et al. (14 additional authors not shown)

Abstract: Kagome materials are at the frontier of condensed matter physics. An ideal kagome lattice features only one geometrically frustrated flat band spanning the entire momentum space and a single Dirac cone at the Brillouin-zone corners. However, for the first time, here we observe unusual flat-band and Dirac physics in the newly discovered "322" kagome material Ni3In2S2 by combining high-resolution sy… ▽ More Kagome materials are at the frontier of condensed matter physics. An ideal kagome lattice features only one geometrically frustrated flat band spanning the entire momentum space and a single Dirac cone at the Brillouin-zone corners. However, for the first time, here we observe unusual flat-band and Dirac physics in the newly discovered "322" kagome material Ni3In2S2 by combining high-resolution synchrotron- and laser-based angle-resolved photoemission spectroscopy with a micro-focused beam, scanning tunneling microscopy, and first-principles calculations. We resolve two distinct electronic flat-band states located in close proximity to the Fermi level: a robust Topological Surface Flat Band at ~40 meV below the Fermi level on the Sulfur-terminated surface, originating from weak topological insulator states, and a kagome lattice-derived flat band at ~100 meV binding energy with an ultranarrow bandwidth (~5 meV). Instead of the single Dirac cone, the Indium-terminated surface hosts a rare two-dimensional Dirac-node arc state, where the gapless Dirac nodes extend along an open one-dimensional line crossing the Brillouin-zone boundary, exhibiting sharp linear dispersion, exceptionally high Fermi velocity, and pronounced circular dichroism. These findings establish Ni3In2S2 as a unique topological kagome metal in which multiple flat-band states of different physical origin coexist with an unusual Dirac-node arc, opening an avenue for discovering flat-band--driven and topology-enabled quantum phenomena. △ Less

Submitted 26 January, 2026; originally announced January 2026.

Comments: 26 pages, 4 figures

Direct observation of vortex liquid droplets in the iron pnictide superconductor CaKAs$_4$Fe$_4$ at $0.5T$_c$

Authors: Oscar Bou Marqués, Jose A. Moreno, Pablo García Talavera, Mingyu Xu, Juan Schmidt, Sergey L. Bud'ko, Paul C. Canfield, Isabel Guillamón, Edwin Herrera, Hermann Suderow

Abstract: Type-II superconductors under magnetic fields are in a quantum coherent non-dissipative state as long as vortices remain pinned. Dissipation appears when vortices depin, eventually driven by thermal fluctuations. This can be associated to a melting transition between a vortex solid and a vortex liquid. This transition is almost always observed very close to T$_c$ when probed by macroscopic experim… ▽ More Type-II superconductors under magnetic fields are in a quantum coherent non-dissipative state as long as vortices remain pinned. Dissipation appears when vortices depin, eventually driven by thermal fluctuations. This can be associated to a melting transition between a vortex solid and a vortex liquid. This transition is almost always observed very close to T$_c$ when probed by macroscopic experiments. However, it remains unclear how the vortex solid responds to thermal fluctuations at the scale of individual vortices far from the melting transition. Here we use scanning tunneling microscopy (STM) to visualize vortices in CaKAs$_4$Fe$_4$ (T$_c \approx$ 35 K). We find vortex liquid droplets-localized regions in space where vortices strongly fluctuate due to thermal exctiation-at temperatures as low as 0.5\,T$_c$. Our results show that the onset of dissipation at the local scale occurs at temperatures considerably below T$_c$ in type-II superconductors. △ Less

Submitted 26 January, 2026; originally announced January 2026.

Correlation between superfluid density and transition temperature in infinite-layer nickelate superconductor $Nd_{1-x}Sr_xNiO_2$

Authors: Z. J. Li, R . Z. Zhang, M. H. Xu, K. Y. Liang, Y. Zhao, Q. S. He, Q. Z. Zhou, B. R. Chen, P. H. Zhang, K. Z. Yao, H. X. Yao, L. Qiao, Y. H. Wang

Abstract: A strong correlation between zero-temperature superfluid density ($ρ_{s0}$) and transition temperature ($T_c$) is considered as a hallmark of unconventional superconductivity. However, their relationship has yet to be unveiled in nickelates due to sample inhomogeneity. Here we perform local susceptometry on an infinite-layer nickelate superconductor $Nd_{0.8}Sr_{0.2}NiO_2$. The sample shows inhomo… ▽ More A strong correlation between zero-temperature superfluid density ($ρ_{s0}$) and transition temperature ($T_c$) is considered as a hallmark of unconventional superconductivity. However, their relationship has yet to be unveiled in nickelates due to sample inhomogeneity. Here we perform local susceptometry on an infinite-layer nickelate superconductor $Nd_{0.8}Sr_{0.2}NiO_2$. The sample shows inhomogeneous superfluid density and $T_c$ on micron-scale. The spatial statistics for different scan areas reveal a linear dependence of local $T_c$ on $ρ_{s0}$ for $T_c$>8 K and a sub-linear one for $T_c$<8 K. Remarkably, the overall relationship is reminiscent of that reported in overdoped cuprate superconductors, hinting at a close connection between them. △ Less

Submitted 18 January, 2026; originally announced January 2026.

Supercritical Snapping and Controlled Launching via Dual Latch Gels

Authors: Xiaona M. Xu, Nolan A. Miller, Gregory M. Grason, Alfred J. Crosby

Abstract: Natural organisms have evolved integrated Latch-Mediated Spring Actuation systems (LaMSA) that consist of multiple latches and springs to enhance power output and adapt to diverse environmental conditions. Similar designs are appealing yet largely unexplored in engineered materials due to the complexity of integrating multiple components into a single material platform. Here, we report a dual-latc… ▽ More Natural organisms have evolved integrated Latch-Mediated Spring Actuation systems (LaMSA) that consist of multiple latches and springs to enhance power output and adapt to diverse environmental conditions. Similar designs are appealing yet largely unexplored in engineered materials due to the complexity of integrating multiple components into a single material platform. Here, we report a dual-latched magneto-elastic shell device capable of selectively activating the latches to regulate snapping pathways and energy output based on specific actuation requirements. Differential deswelling across the thickness acts as the motor to load the elastic energy into the shell, which is then released via the snap-through instability once the loading reaches the critical threshold, constituting an intrinsic mechanical latch. Activation of the external magnetic latch delays snapping onset beyond the threshold of the intrinsic latch, leading to a power-amplified supercritical snap-through instability as well as a bifurcation instability. The combined function of both latches allows for flexible control over energy storage and release. Additionally, this integrated LaMSA system possesses an untethered anchoring mechanism, enabling the device to launch in arbitrary directions from the substrate, driven by the energy released during snapping. We envision that the design principles of dual-latched LaMSA systems will create opportunities for power-dense actuation in engineered materials and robotic devices. △ Less

Submitted 15 January, 2026; originally announced January 2026.

Frustrated Magnetism in FeGe$_3$O$_4$ with a Chiral Trillium Network

Authors: Matt Boswell, Mingyu Xu, Haozhe Wang, Mouyang Cheng, N. Li, X. F. Sun, Haidong Zhou, Huibo Cao, Mingda Li, Weiwei Xie

Abstract: The discovery of new magnetic ground states in geometrically frustrated lattices remains a central challenge in materials science. Here, we report the synthesis, structural characterization, and frustrated magnetic properties of FeGe$_3$O$_4$, a newly identified compound that crystallizes in the noncentrosymmetric cubic space group $P2_13$. In this structure, Fe atoms form an intricate double-tril… ▽ More The discovery of new magnetic ground states in geometrically frustrated lattices remains a central challenge in materials science. Here, we report the synthesis, structural characterization, and frustrated magnetic properties of FeGe$_3$O$_4$, a newly identified compound that crystallizes in the noncentrosymmetric cubic space group $P2_13$. In this structure, Fe atoms form an intricate double-trillium lattice with nearest-neighbor Fe--Fe distances of $\sim$4.2~Å, while Ge$^{2+}$ ions mediate magnetic interactions through Fe-Ge-Fe pathways. Field-dependent magnetization at 2~K shows a pronounced nonlinearity, reaching a maximum moment of 2.55(3)~$μ_\mathrm{B}$/Fe$^{2+}$ at 70~kOe without evidence of saturation. Magnetic susceptibility, heat capacity, and neutron scattering collectively reveal the onset of short-range magnetic interactions near 5~K, with no long-range ordering detected down to 0.06~K. Specific heat measurements demonstrate strong frustration: only $\sim$34\% of the expected magnetic entropy is recovered at 2.4~K. Taken together, these results establish FeGe$_3$O$_4$ as a rare example of a geometrically frustrated trillium-lattice magnet, offering a promising platform for exploring exotic quantum magnetic phenomena. △ Less

Submitted 13 January, 2026; originally announced January 2026.

Comments: 26 pages, 4+6 figures

Simulating Non-Markovian Dynamics in Open Quantum Systems

Authors: Meng Xu, Vasilii Vadimov, J. T. Stockburger, J. Ankerhold

Abstract: Recent advances in quantum technologies and related experiments have created a need for highly accurate, versatile, and computationally efficient simulation techniques for the dynamics of open quantum systems. Long-lived correlation effects (non-Markovianity), system-environment hybridization, and the necessity for accuracy beyond the Born-Markov approximation form particular challenges. Approache… ▽ More Recent advances in quantum technologies and related experiments have created a need for highly accurate, versatile, and computationally efficient simulation techniques for the dynamics of open quantum systems. Long-lived correlation effects (non-Markovianity), system-environment hybridization, and the necessity for accuracy beyond the Born-Markov approximation form particular challenges. Approaches to meet these challenges have been introduced, originating from different fields, such as hierarchical equations of motion, Lindblad-pseudomode formulas, chain-mapping approaches, quantum Brownian motion master equations, stochastic unravelings, and refined quantum master equations. This diversity, while indicative of the field's relevance, has inadvertently led to a fragmentation that hinders cohesive advances and their effective cross-community application to current problems for complex systems. How are different approaches related to each other? What are their strengths and limitations? Here we give a systematic overview and concise discussion addressing these questions. We make use of a unified framework which very conveniently allows to link different schemes and, this way, may also catalyze further progress. In line with the state of the art, this framework is formulated not in a fully reduced space of the system but in an extended state space which in a minimal fashion includes effective reservoir modes. This in turn offers a comprehensive understanding of existing methods, elucidating their physical interpretations, interconnections, and applicability. △ Less

Submitted 7 January, 2026; v1 submitted 5 January, 2026; originally announced January 2026.

Comments: 28 pages, 3 figures; Rev. Mod. Phys

Detection of MEMS Acoustics via Scanning Tunneling Microscopy

Authors: R. J. G. Elbertse, M. Xu, A. Keşkekler, S. Otte, R. A. Norte

Abstract: Scanning tunneling microscopy (STM) and micro-electromechanical systems (MEMS) have traditionally addressed vastly different length scales - one resolving atoms, the other engineering macroscopic motion. Here we unite these two fields to perform minimally invasive-measurements of high aspect-ratio MEMS resonators using the STM tip as both actuator and detector. Operating at cryogenic temperatures,… ▽ More Scanning tunneling microscopy (STM) and micro-electromechanical systems (MEMS) have traditionally addressed vastly different length scales - one resolving atoms, the other engineering macroscopic motion. Here we unite these two fields to perform minimally invasive-measurements of high aspect-ratio MEMS resonators using the STM tip as both actuator and detector. Operating at cryogenic temperatures, we resolve acoustic modes of millimeter-scale, high-Q membranes with picometer spatial precision, without making use of lasers or capacitive coupling. The tunneling junction introduces negligible back-action or heating, enabling direct access to the intrinsic dynamics of microgram-mass oscillators. In this work we explore three different measurement modalities, each offering unique advantages. Combined, they provide a pathway to quantum-level readout and exquisite high-precision measurements of forces, displacements, and pressures at cryogenic conditions. This technique provides a general platform for minimally-perturbative detection across a wide range of nanomechanical and quantum devices. △ Less

Submitted 7 January, 2026; v1 submitted 3 January, 2026; originally announced January 2026.

Comments: Main and Supplementary

Coulomb crystallization of xenon highly charged ions in a laser-cooled Ca+ matrix

Authors: Leonid Prokhorov, Aaron A. Smith, Mingyao Xu, Kostas Georgiou, Vera Guarrera, Lakshmi P. Kozhiparambil Sajith, Elwin A. Dijck, Christian Warnecke, Malte Wehrheim, Alexander Wilzewski, Laura Blackburn, Matthias Keller, Vincent Boyer, Thomas Pfeifer, Ullrich Schwanke, Cigdem Issever, Steven Worm, Piet O. Schmidt, José R. Crespo Lopez-Urrutia, Giovanni Barontini

Abstract: We report on the sympathetic cooling and Coulomb crystallization of xenon highly charged ions (HCIs) with laser-cooled Ca$^+$ ions. The HCIs are produced in a compact electron beam ion trap, then charge selected, decelerated, and finally injected into a cryogenic linear Paul trap. There, they are captured into $^{40}$Ca$^+$ Coulomb crystals, and co-crystallized within them, causing dark voids in t… ▽ More We report on the sympathetic cooling and Coulomb crystallization of xenon highly charged ions (HCIs) with laser-cooled Ca$^+$ ions. The HCIs are produced in a compact electron beam ion trap, then charge selected, decelerated, and finally injected into a cryogenic linear Paul trap. There, they are captured into $^{40}$Ca$^+$ Coulomb crystals, and co-crystallized within them, causing dark voids in their fluorescence images. Fine control over the number of trapped ions and HCIs allows us to realize mixed-species crystals with arbitrary ordering patterns. By investigating Xe$^{q+}$--Ca$^+$ strings, we confirm the HCI charge states, measure their lifetime and characterize the mixed-species motional modes. Our system effectively combines the established quantum control toolbox for Ca$^+$ with the rich set of atomic properties of Xe highly charged ions, providing a resourceful platform for optical frequency metrology, searches for signatures of new physics, and quantum information science. △ Less

Submitted 11 June, 2026; v1 submitted 13 December, 2025; originally announced December 2025.

Journal ref: Phys. Rev. A 113, L041102 (2026)

Pervasive electronic nematicity as the parent state of kagome superconductors

Authors: Muxian Xu, Siyu Cheng, Andrea Capa Salinas, Ganesh Pokharel, Alexander LaFleur, Hong Li, Hengxin Tan, Brenden R. Ortiz, Qinwen Deng, Binghai Yan, Ziqiang Wang, Stephen D. Wilson, Ilija Zeljkovic

Abstract: Kagome superconductors $A$V$_3$Sb$_5$ ($A$ = Cs, K, Rb) have developed into an exciting playground for realizing and exploring exotic solid state phenomena. Abundant experimental evidence suggests that electronic structure breaks rotational symmetry of the lattice, but whether this may be a simple consequence of the symmetry of the underlying 2 $\times$ 2 charge density wave phase or an entirely d… ▽ More Kagome superconductors $A$V$_3$Sb$_5$ ($A$ = Cs, K, Rb) have developed into an exciting playground for realizing and exploring exotic solid state phenomena. Abundant experimental evidence suggests that electronic structure breaks rotational symmetry of the lattice, but whether this may be a simple consequence of the symmetry of the underlying 2 $\times$ 2 charge density wave phase or an entirely different mechanism remains intensely debated. We use spectroscopic imaging scanning tunneling microscopy to explore the phase diagram of the prototypical kagome superconductor CsV$_3$Sb$_5$ as a function of doping. We intentionally suppress the charge density wave phase with chemical substitutions selectively introduced at two distinct lattice sites, and investigate the resulting system. We discover that rotational symmetry breaking of the electronic structure -- now present in short-range nanoscale regions -- persists in all samples, in a wide doping range long after all charge density waves have been suppressed. As such, our experiments uncover ubiquitous electronic nematicity across the $A$V$_3$Sb$_5$ phase diagram, unrelated to the 2 $\times$ 2 charge density wave. This further points towards electronic nematicity as the intrinsic nature of the parent state of kagome superconductors, under which other exotic low-temperature phenomena subsequently emerge. △ Less

Submitted 26 November, 2025; originally announced November 2025.

Expansion of Momentum Space and Full 2$π$ Solid Angle Photoelectron Collection in Laser-Based Angle-Resolved Photoemission Spectroscopy by Applying Sample Bias

Authors: Taimin Miao, Yu Xu, Bo Liang, Wenpei Zhu, Neng Cai, Mingkai Xu, Di Wu, Hongze Gu, Wenjin Mao, Shenjin Zhang, Fengfeng Zhang, Feng Yang, Zhimin Wang, Qinjun Peng, Zuyan Xu, Zhihai Zhu, Xintong Li, Hanqing Mao, Lin Zhao, Guodong Liu, X. J. Zhou

Abstract: Angle-resolved photoemission spectroscopy (ARPES) directly probes the energy and momentum of electrons in quantum materials, but conventional setups capture only a small fraction of the full 2$π$ solid angle. This limitation is acute in laser-based ARPES, where the low photon energy restricts momentum space despite ultrahigh resolution. Here we present systematic studies of bias ARPES, where apply… ▽ More Angle-resolved photoemission spectroscopy (ARPES) directly probes the energy and momentum of electrons in quantum materials, but conventional setups capture only a small fraction of the full 2$π$ solid angle. This limitation is acute in laser-based ARPES, where the low photon energy restricts momentum space despite ultrahigh resolution. Here we present systematic studies of bias ARPES, where applying a sample bias expands the accessible momentum range and enables full 2$π$ solid angle collection in two dimension using our 6.994 eV laser source. An analytical conversion relation is established and validated to accurately map the detector angle to the emission angle and the electron momentum in two dimensions. A precise approach is developed to determine the sample work function which is critical in the angle-momentum conversion of the bias ARPES experiments. Energy and angular resolutions are preserved under biases up to 100 V, and minimizing beam size is shown to be crucial. The technique is effective both near normal and off-normal geometries, allowing flexible Brillouin zone access with lower biases. Bias ARPES thus elevates laser ARPES to a new level, extending momentum coverage while retaining high resolution, and is applicable across a broad photon-energy range. △ Less

Submitted 25 March, 2026; v1 submitted 24 November, 2025; originally announced November 2025.

Comments: 57 pages, 17 figures

Journal ref: Review of Scientific Instruments 97, 033908 (2026)

Interface-engineered voltage-driven magnetic tunnel junctions with ultra-low-energy magnetization switching

Authors: Yu Zhang, Meng Xu, Bowei Zhou, Carter Eckel, Supriya Ghosh, Hwanhui Yun, Ali Habiboglu, Deyuan Lyu, Daniel B Gopman, Jian-Ping Wang, K. Andre Mkhoyan, Weigang Wang

Abstract: Electric-field control of spin states offers a promising route to ultra-low-power, ultra-fast magnetization switching in spintronic devices such as magnetic tunnel junctions (MTJs). Recent progress in modulating spin-orbit interactions at the interfaces between 3d transition-metal ferromagnets and dielectric layers has underscored the role of atomic-scale heavy-metal doping in optimizing device pe… ▽ More Electric-field control of spin states offers a promising route to ultra-low-power, ultra-fast magnetization switching in spintronic devices such as magnetic tunnel junctions (MTJs). Recent progress in modulating spin-orbit interactions at the interfaces between 3d transition-metal ferromagnets and dielectric layers has underscored the role of atomic-scale heavy-metal doping in optimizing device performance. Here, we experimentally demonstrate highly energy-efficient, voltage-driven magnetization switching in MTJs exhibiting large tunnel magnetoresistance (TMR), enabled by a remote doping technique that precisely controls the iridium (Ir) concentration near the MgO-CoFeB interface in the free layer. Our devices achieve a switching energy of only 3.5 fJ per bit for nanoscale MTJs operating in the sub-nanosecond regime, while maintaining a TMR ratio up to 160 percent after 400 C post-annealing. These findings establish a viable pathway toward scalable, ultra-low-power nonvolatile memory, positioning voltage-driven MTJs as strong contenders for next-generation magnetoresistive random-access memory (MRAM) and other emerging spintronic applications. △ Less

Submitted 22 November, 2025; originally announced November 2025.

Design boosters: from constant-time quantum chaos to $\infty$-designs and beyond

Authors: Soumik Ghosh, Arjun Mirani, Yihui Quek, Michelle Xu

Abstract: We study a counterintuitive property of 'conditioning' on the result of measuring a subsystem of a quantum state: such conditioning can boost design quality, at the cost of increased system size. We work in the setting of deep thermalization from many-body physics: starting from a bipartite state on a global system $(A,B)$ drawn from a $k$-design, we measure system $B$ in the computational basis,… ▽ More We study a counterintuitive property of 'conditioning' on the result of measuring a subsystem of a quantum state: such conditioning can boost design quality, at the cost of increased system size. We work in the setting of deep thermalization from many-body physics: starting from a bipartite state on a global system $(A,B)$ drawn from a $k$-design, we measure system $B$ in the computational basis, keep the outcome and examine the state that remains in system $A$, approximating the overall ensemble (the 'projected ensemble') by a $k'$-design. We ask: how does the design quality change due to this procedure, or how does $k'$ compare to $k$? We give the first rigorous example of unitary dynamics generating a state such that, projection at very early (constant) times can boost design randomness. These dynamics are those of quantum chaos, modeled by the evolution of a Hamiltonian drawn from the Gaussian Unitary Ensemble (GUE). We show that, even though a state generated by such dynamics at constant time only forms a $k=\mathcal{O}(1)$ design, the projected ensemble is Haar-random (or a $k'=\infty$ design) in the thermodynamic limit (i.e. when $N_B=\infty$). This phenomenon persists even with weaker and more physically realistic assumptions; our results can be appropriately applied to non-GUE Hamiltonians that nevertheless show likely chaotic signatures in their eigenbases. Moreover, we show that with no assumption on how the global state was generated, a $k$-design experiences a degradation in design quality to $k' = \lfloor k/2 \rfloor$. This improves upon best prior results on the deep thermalization of designs. Together, our contributions argue for design boosting as a result of chaos and showcase a novel mechanism to generate good designs. △ Less

Submitted 11 November, 2025; originally announced November 2025.

Comments: 41 pages, 2 figures

Intrinsic Non-linearity of Josephson Junctions as an Alternative Origin of the Missing First Shapiro Step

Authors: Lei Xu, Shuhang Mai, Manzhang Xu, Xue Yang, Lihong Hu, Xinyi Zheng, Sicheng Zhou, Siyuan Zhou, Bingbing Tong, Xiaohui Song, Jie Shen, Zhaozheng Lyu, Ziwei Dou, Xiunian Jing, Fanming Qu, Peiling Li, Guangtong Liu, Li Lu

Abstract: The missing first Shapiro step in microwave-irradiated Josephson junctions has been widely interpreted as a hallmark of Majorana bound states. However, conventional mechanisms like junction underdamping or Joule heating can produce similar signatures. Here, we demonstrate that the intrinsic non-linear current-voltage characteristic of low-to-moderate transparency junctions can also suppress the fi… ▽ More The missing first Shapiro step in microwave-irradiated Josephson junctions has been widely interpreted as a hallmark of Majorana bound states. However, conventional mechanisms like junction underdamping or Joule heating can produce similar signatures. Here, we demonstrate that the intrinsic non-linear current-voltage characteristic of low-to-moderate transparency junctions can also suppress the first step, accompanied by distinctive zigzag boundaries between the zeroth and first step at intermediate driving frequencies. Microwave measurements on Al/WTe2 junctions and numerical simulations of a non-linear resistively and capacitively shunted junction model reveal the first step collapse induced by switching jumps of current, together with zigzag features absent in scenarios solely driven by finite \b{eta} or Joule heating. This zigzag signature therefore provides a crucial diagnostic tool, emphasizing the necessity of comprehensive analysis of microwave spectra before attributing the absence of the first Shapiro step to Majorana physics. △ Less

Submitted 22 October, 2025; originally announced October 2025.

Comments: 18 pages, 4 figures

Superconductivity suppression and bilayer decoupling in Pr substituted YBa$_2$Cu$_3$O$_{7-δ}$

Authors: Jinming Yang, Zheting Jin, Siqi Wang, Camilla Moir, Mingyu Xu, Brandon Gunn, Xian Du, Zhibo Kang, Keke Feng, Makoto Hashimoto, Donghui Lu, Jessica McChesney, Martin Sundermann, Hlynur Gretarsson, Shize Yang, Wei-Wei Xie, Alex Frano, Sohrab Ismail-Beigi, M. Brian Maple, Yu He

Abstract: The mechanism behind superconductivity suppression induced by Pr substitutions in YBa$_2$Cu$_3$O$_{7-δ}$ (YBCO) has been a mystery since its discovery: in spite of being isovalent to Y$^{3+}$ with a small magnetic moment, it is the only rare-earth element that has a dramatic impact on YBCO's superconducting properties. Using angle-resolved photoemission spectroscopy (ARPES) and DFT+$U$ calculation… ▽ More The mechanism behind superconductivity suppression induced by Pr substitutions in YBa$_2$Cu$_3$O$_{7-δ}$ (YBCO) has been a mystery since its discovery: in spite of being isovalent to Y$^{3+}$ with a small magnetic moment, it is the only rare-earth element that has a dramatic impact on YBCO's superconducting properties. Using angle-resolved photoemission spectroscopy (ARPES) and DFT+$U$ calculations, we uncover how Pr substitution modifies the low-energy electronic structure of YBCO. Contrary to the prevailing Fehrenbacher-Rice (FR) and Liechtenstein-Mazin (LM) models, the low energy electronic structure contains no signature of any $f$-electron hybridization or new states. Yet, strong electron doping is observed primarily on the antibonding Fermi surface. Meanwhile, we reveal major electronic structure modifications to Cu-derived states with increasing Pr substitution: a pronounced CuO$_2$ bilayer decoupling and an enhanced CuO chain hopping, implying indirect electron-release pathways beyond simple 4$f$ state ionization. Our results challenge the long-standing FR/LM mechanism and establish Pr substituted YBCO as a potential platform for exploring correlation-driven phenomena in coupled 1D-2D systems. △ Less

Submitted 19 December, 2025; v1 submitted 16 October, 2025; originally announced October 2025.