Showing 1–50 of 150 results for author: Kudo, K

Zero-field superconducting diode effect induced by magnetic flux in a van der Waals superconductor trigonal PtBi$_2$

Authors: Nan Jiang, Masaki Maeda, Yuhi Yamaguchi, Mori Watanabe, Masashi Tokuda, Kensuke Takaki, Sebun Masaki, Takumi Ikushima, Takayoshi Koyanagi, Masakazu Matsubara, Kazutaka Kudo, Yasuhiro Niim

Abstract: The superconducting diode effect is one of the nonreciprocal transport phenomena, where the critical current depends on the current direction. This effect is typically realized in superconductors with broken spatial-inversion and time-reversal symmetry. To break the time-reversal symmetry, external magnetic fields are commonly used. Here, we demonstrate a sign-controllable superconducting diode ef… ▽ More The superconducting diode effect is one of the nonreciprocal transport phenomena, where the critical current depends on the current direction. This effect is typically realized in superconductors with broken spatial-inversion and time-reversal symmetry. To break the time-reversal symmetry, external magnetic fields are commonly used. Here, we demonstrate a sign-controllable superconducting diode effect under zero external magnetic field in a van der Waals superconductor trigonal PtBi$_2$. The sign of the zero-field superconducting diode effect is controlled by the poling magnetic field, that is a large magnetic field applied prior to measurements. This result indicates that trapped magnetic flux are responsible for breaking the time-reversal symmetry. Our findings highlight the crucial role of trapped magnetic flux in generating the superconducting diode effect and provide a general pathway for realizing a zero-field superconducting diode effect. △ Less

Submitted 5 December, 2025; originally announced December 2025.

Comments: 14 pages, 14 figures

Repulsive-Interaction-Driven Topological Superconductivity in a Landau Level Coupled to an $s$-Wave Superconductor

Authors: Koji Kudo, Ryota Nakai, Hiroki Isobe, J. K. Jain, Kentaro Nomura

Abstract: A two-dimensional topologically nontrivial state of noninteracting electrons, such as the surface state of a three-dimensional topological insulator, is predicted to realize a topological superconductor when proximity-coupled to an ordinary $s$-wave superconductor. In contrast, noninteracting electrons partially occupying a Landau level, with Rashba spin-orbit coupling that lifts the spin degenera… ▽ More A two-dimensional topologically nontrivial state of noninteracting electrons, such as the surface state of a three-dimensional topological insulator, is predicted to realize a topological superconductor when proximity-coupled to an ordinary $s$-wave superconductor. In contrast, noninteracting electrons partially occupying a Landau level, with Rashba spin-orbit coupling that lifts the spin degeneracy, fail to develop topological superconductivity under similar proximity coupling in the presence of the conventional Abrikosov vortex lattice. We demonstrate through exact diagonalization that, at half-filled Landau level, introducing a repulsive interaction between electrons induces topological superconductivity for a range of parameters. This appears rather surprising because a repulsive interaction is expected to inhibit, not promote, pairing, but suggests an appealing principle for realizing topological superconductivity: proximity-coupling a composite Fermi liquid to an ordinary $s$-wave superconductor. △ Less

Submitted 6 October, 2025; originally announced October 2025.

Comments: 16 pages, 9 figures

Performance of the Extended Ising Machine for the Quadratic Knapsack Problem

Authors: Haruka Akishima, Hirotaka Tamura, Kazue Kudo

Abstract: The extended Ising machine (EIM) enhances conventional Ising models, which handle only binary quadratic forms by allowing constraints through real-valued dependent variables. We address the quadratic knapsack problem (QKP), hard to solve using Ising machines when formulated as a quadratic unconstrained binary optimization (QUBO). We demonstrated the EIM's superiority by comparing it with the conve… ▽ More The extended Ising machine (EIM) enhances conventional Ising models, which handle only binary quadratic forms by allowing constraints through real-valued dependent variables. We address the quadratic knapsack problem (QKP), hard to solve using Ising machines when formulated as a quadratic unconstrained binary optimization (QUBO). We demonstrated the EIM's superiority by comparing it with the conventional Ising model-based approach, a commercial exact solver, and a state-of-the-art heuristic solver for QKP. △ Less

Submitted 9 August, 2025; originally announced August 2025.

Comments: 6 pages

Journal ref: J. Phys. Soc. Jpn. 94, 095002 (2025)

Stoichiometry control and epitaxial growth of AgCrSe2 thin films by pulsed-laser deposition

Authors: Yusuke Tajima, Kenshin Inamura, Sebun Masaki, Takumi Yamazaki, Takeshi Seki, Kazutaka Kudo, Jobu Matsuno, Junichi Shiogai

Abstract: We report on epitaxial growth in thin-film synthesis of a polar magnetic semiconductor AgCrSe2 on lattice-matched yttria-stabilized zirconia (111) substrate by pulsed-layer deposition (PLD). By using Ag-rich PLD target to compensate for Ag deficiency in thin films, the nucleation of impurity phases is suppressed, resulting in the c-axis-oriented and single-phase AgCrSe2 thin film. Structural analy… ▽ More We report on epitaxial growth in thin-film synthesis of a polar magnetic semiconductor AgCrSe2 on lattice-matched yttria-stabilized zirconia (111) substrate by pulsed-layer deposition (PLD). By using Ag-rich PLD target to compensate for Ag deficiency in thin films, the nucleation of impurity phases is suppressed, resulting in the c-axis-oriented and single-phase AgCrSe2 thin film. Structural analysis using x-ray diffraction and cross-sectional scanning transmission electron microscopy reveals epitaxial growth with the presence of both twisted and polar domains. Optical absorbance spectrum and magnetization measurements show absorption edge at around 0.84 eV and magnetic transition temperature at 41 K, respectively. These values are consistent with the reported values of direct bandgap and Néel temperature of bulk AgCrSe2, reflecting a single-phase and stoichiometric feature of the obtained film. Our demonstration of epitaxial thin-film growth of AgCrSe2 serves as a bedrock for exploration of its potential thermoelectric and spintronic functionalities at surface or heterointerfaces. △ Less

Submitted 27 May, 2025; originally announced May 2025.

Comments: Accepted in APL Materials

Odd-parity magnetism by quantum geometry

Authors: Kanta Kudo, Youichi Yanase

Abstract: We study the effects of quantum geometry on parity-violating magnetism that is classified as odd-parity multipole magnetism. By comparing the spin susceptibility and odd-parity multipole susceptibility in the multisublattice model, we find that the ferroic multipole fluctuation is induced by the quantum geometry of Bloch electrons over a wide range of parameters. Due to the Hubbard interaction, th… ▽ More We study the effects of quantum geometry on parity-violating magnetism that is classified as odd-parity multipole magnetism. By comparing the spin susceptibility and odd-parity multipole susceptibility in the multisublattice model, we find that the ferroic multipole fluctuation is induced by the quantum geometry of Bloch electrons over a wide range of parameters. Due to the Hubbard interaction, the quantum-geometric multipole fluctuations condense into the multipole order. We predict complex magnetic correlations, which are a signature of quantum-geometric multipole magnetism, and propose experimental verification. △ Less

Submitted 27 May, 2025; originally announced May 2025.

Chirality-selective proximity effect between chiral $p$-wave superconductors and quantum Hall insulators

Authors: Ryota Nakai, Koji Kudo, Hiroki Isobe, Kentaro Nomura

Abstract: Heterostructures of superconductors and quantum-Hall insulators are promising platforms of topological quantum computation. However, these two systems are incompatible in some aspects such as a strong magnetic field, the Meissner effect, and chirality. In this work, we address the condition that the superconducting proximity effect works in the bulk of quantum Hall states, and identify an essentia… ▽ More Heterostructures of superconductors and quantum-Hall insulators are promising platforms of topological quantum computation. However, these two systems are incompatible in some aspects such as a strong magnetic field, the Meissner effect, and chirality. In this work, we address the condition that the superconducting proximity effect works in the bulk of quantum Hall states, and identify an essential role played by the vortex lattice regardless of pairing symmetry. We extend this finding to a heterostructure of a chiral $p$-wave superconductor in the mixed state and an integer quantum Hall insulator. The proximity effect works selectively in the lowest Landau level depending on relative chiralities. If the chiralities align, a topological phase transition to a topological superconductor occurs. △ Less

Submitted 14 November, 2025; v1 submitted 2 May, 2025; originally announced May 2025.

Comments: 12 pages, 5 figures

Journal ref: Phys. Rev. B 112, 094520 (2025)

Engineered substrates for domain control in CrSe thin-film growth: Single-domain formation on lattice-matched YSZ(111) substrate

Authors: Yusuke Tajima, Junichi Shiogai, Masayuki Ochi, Kazutaka Kudo, Jobu Matsuno

Abstract: Epitaxial thin-film growth is a versatile and powerful technique for achieving a precise control of composition, stabilizing non-equilibrium phases, tailoring growth orientation, as well as forming heterointerfaces of various quantum materials. For synthesis of highly crystalline thin films, in-depth understanding of epitaxial relationship between the desired thin film and the single-crystalline s… ▽ More Epitaxial thin-film growth is a versatile and powerful technique for achieving a precise control of composition, stabilizing non-equilibrium phases, tailoring growth orientation, as well as forming heterointerfaces of various quantum materials. For synthesis of highly crystalline thin films, in-depth understanding of epitaxial relationship between the desired thin film and the single-crystalline substrates is necessary. In this study, we investigate epitaxial relationship in thin-film growth of triangular-lattice antiferromagnet CrSe on the (001) plane of Al2O3 and the lattice-matched (111) plane of yttria-stabilized zirconia (YSZ) substrates. Structural characterization using out-of-plane and in-plane x-ray diffraction shows that the presence of 19.1o-twisted domains of CrSe significantly dominates the aligned domain on the Al2O3 substrate while it reveals a single-domain formation on the YSZ substrate. The stability of the 19.1o-twisted domain rather than the aligned domain can be explained by rotational commensurate epitaxy, which is well reproduced by density functional theory calculations. The single-domain CrSe thin film on the YSZ substrate exhibits a superior metallic conductivity compared to the twisted-domain thin film on the Al2O3 substrate, implying contribution of the grain boundary scattering mechanism to electrical transport. △ Less

Submitted 12 March, 2025; originally announced March 2025.

Comments: 24 pages, 4 figures

Collaborative filtering based on nonnegative/binary matrix factorization

Authors: Yukino Terui, Yuka Inoue, Yohei Hamakawa, Kosuke Tatsumura, Kazue Kudo

Abstract: Collaborative filtering generates recommendations by exploiting user-item similarities based on rating data, which often contains numerous unrated items. To predict scores for unrated items, matrix factorization techniques such as nonnegative matrix factorization (NMF) are often employed. Nonnegative/binary matrix factorization (NBMF), which is an extension of NMF, approximates a nonnegative matri… ▽ More Collaborative filtering generates recommendations by exploiting user-item similarities based on rating data, which often contains numerous unrated items. To predict scores for unrated items, matrix factorization techniques such as nonnegative matrix factorization (NMF) are often employed. Nonnegative/binary matrix factorization (NBMF), which is an extension of NMF, approximates a nonnegative matrix as the product of nonnegative and binary matrices. While previous studies have applied NBMF primarily to dense data such as images, this paper proposes a modified NBMF algorithm tailored for collaborative filtering with sparse data. In the modified method, unrated entries in the rating matrix are masked, enhancing prediction accuracy. Furthermore, utilizing a low-latency Ising machine in NBMF is advantageous in terms of the computation time, making the proposed method beneficial. △ Less

Submitted 29 July, 2025; v1 submitted 14 October, 2024; originally announced October 2024.

Comments: 12 pages, 8 figures

Journal ref: Front. Big Data 8, 1599704 (2025)

Spontaneous magnetic field and disorder effects in BaPtAs_1-x_Sb_x_ with honeycomb network

Authors: T. Adachi, T. Ogawa, Y. Komiyama, T. Sumura, Y. Saito-Tsuboi, T. Takeuchi, K. Mano, K. Manabe, K. Kawabata, T. Imazu, A. Koda, W. Higemoto, H. Okabe, J. G. Nakamura, T. U. Ito, R. Kadono, C. Baines, I. Watanabe, T. Kida, M. Hagiwara, Y. Imai, J. Goryo, M. Nohara, K. Kudo

Abstract: Chiral superconductivity exhibits the formation of novel electron pairs that breaks the time-reversal symmetry and has been actively studied in various quantum materials in recent years. However, despite its potential to provide definitive information, effects of disorder in the crystal structure on the chiral superconductivity has not yet been clarified, and therefore the investigation using a so… ▽ More Chiral superconductivity exhibits the formation of novel electron pairs that breaks the time-reversal symmetry and has been actively studied in various quantum materials in recent years. However, despite its potential to provide definitive information, effects of disorder in the crystal structure on the chiral superconductivity has not yet been clarified, and therefore the investigation using a solid-solution system is desirable. We report muon-spin-relaxation (muSR) results of layered pnictide BaPtAs_1-x_Sb_x_ with a honeycomb network composed of Pt and (As, Sb). We observed an increase of the zero-field muon-spin relaxation rate in the superconducting (SC) state at the Sb end of x=1.0, suggesting the occurrence of spontaneous magnetic field due to the time-reversal symmetry breaking in the SC state. On the other hand, spontaneous magnetic field was almost and completely suppressed for the As-Sb mixed samples of x=0.9 and 0.2, respectively, suggesting that the time-reversal symmetry breaking SC state in x=1.0 is sensitive to disorder. The magnetic penetration depth estimated from transverse-field muSR measurements at x=1.0 and 0.2 behaved like weak-coupling s-wave superconductivity. These seemingly incompatible zero-field and transverse-field muSR results of BaPtAs_1-x_Sb_x_ with x=1.0 could be understood in terms of chiral d-wave superconductivity with point nodes on the three-dimensional Fermi surface. △ Less

Submitted 17 March, 2025; v1 submitted 8 September, 2024; originally announced September 2024.

Comments: 7 pages, 3 figures, 1 table, Phys. Rev. B Letter (in press)

Journal ref: Phys. Rev. B 111, L100508 (2025)

Annealing-based approach to solving partial differential equations

Authors: Kazue Kudo

Abstract: Solving partial differential equations (PDEs) using an annealing-based approach involves solving generalized eigenvalue problems. Discretizing a PDE yields a system of linear equations (SLE). Solving an SLE can be formulated as a general eigenvalue problem, which can be transformed into an optimization problem with an objective function given by a generalized Rayleigh quotient. The proposed algori… ▽ More Solving partial differential equations (PDEs) using an annealing-based approach involves solving generalized eigenvalue problems. Discretizing a PDE yields a system of linear equations (SLE). Solving an SLE can be formulated as a general eigenvalue problem, which can be transformed into an optimization problem with an objective function given by a generalized Rayleigh quotient. The proposed algorithm requires iterative computations. However, it enables efficient annealing-based computation of eigenvectors to arbitrary precision without increasing the number of variables. Investigations using simulated annealing demonstrate how the number of iterations scales with system size and annealing time. Computational performance depends on system size, annealing time, and problem characteristics. △ Less

Submitted 23 December, 2025; v1 submitted 25 June, 2024; originally announced June 2024.

Comments: 6 pages, 4 figures

Quantum anomalous, spin, and valley Hall effects in pentalayer rhombohedral graphene moiré superlattices

Authors: Koji Kudo, Ryota Nakai, Kentaro Nomura

Abstract: Recent experiments on pentalayer rhombohedral graphene moiré superlattices have observed the quantum anomalous Hall effect at moiré filling factor of $ν= 1$ and various fractional values. These phenomena are attributed to a flat Chern band induced by electron-electron interactions. In this study, we demonstrate that at $ν= 2$, many-body effects can lead to the emergence of quantum spin Hall and qu… ▽ More Recent experiments on pentalayer rhombohedral graphene moiré superlattices have observed the quantum anomalous Hall effect at moiré filling factor of $ν= 1$ and various fractional values. These phenomena are attributed to a flat Chern band induced by electron-electron interactions. In this study, we demonstrate that at $ν= 2$, many-body effects can lead to the emergence of quantum spin Hall and quantum valley Hall states, in addition to the quantum anomalous Hall state, even in the absence of spin-orbit coupling or valley-dependent potentials. These three topological states can be selectively induced by the application and manipulation of a magnetic field. Furthermore, we show that at $ν= 3$ and $4$, the ground state can be a combination of topologically trivial and nontrivial states, unlike the cases of $ν=1$ and 2. This contrasts with the conventional quantum Hall effect in graphene where the ground state at filling factor $ν$ is given as the particle-hole counterpart at $4-ν$. △ Less

Submitted 25 December, 2024; v1 submitted 20 June, 2024; originally announced June 2024.

Comments: 11 pages, 7 figures

Journal ref: Phys. Rev. B 110, 245135 (2024)

Observation of two-level critical-state in a van-der-Waals superconductor Pt(Bi$_{1-x}$Se$_x$)$_2$

Authors: Y. Samukawa, M. Maeda, N. Jiang, R. Nakamura, M. Watanabe, K. Takaki, Y. Moriyasu, K. Kudo, Y. Niimi

Abstract: Trigonal PtBi$_2$ is one of the attractive van-der-Waals materials because of the enhancement of its superconducting transition temperature $T_{\rm{c}}$ by doping chalcogen elements such as Se and Te. Recently, it has been reported that $T_{\rm{c}}$ of Pt(Bi$_{1-x}$Se$_x$)$_2$ is enhanced by a factor of 4, compared to the pristine PtBi$_2$, together with the polar-nonpolar structural phase transit… ▽ More Trigonal PtBi$_2$ is one of the attractive van-der-Waals materials because of the enhancement of its superconducting transition temperature $T_{\rm{c}}$ by doping chalcogen elements such as Se and Te. Recently, it has been reported that $T_{\rm{c}}$ of Pt(Bi$_{1-x}$Se$_x$)$_2$ is enhanced by a factor of 4, compared to the pristine PtBi$_2$, together with the polar-nonpolar structural phase transition. Thus, it is desirable to study electrical transport properties for this new superconducting compound. Here, we have performed magnetotransport measurements for Pt(Bi$_{1-x}$Se$_x$)$_2$ ($x$ = 0.06 and 0.08) thin-film devices and have observed a peculiar magnetoresistance where a finite hysteresis appears when the superconducting state is broken. By measuring the magnetoresistance systematically, we have attributed this magnetoresistance to the two-level critical-state where fluxons pinned in Pt(Bi$_{1-x}$Se$_x$)$_2$ play an important role. △ Less

Submitted 30 April, 2024; originally announced April 2024.

Comments: 7 pages, 5 figures

Non-coplanar spin structure in a metallic thin film of triangular lattice antiferromagnet CrSe

Authors: Yusuke Tajima, Junichi Shiogai, Kohei Ueda, Hirotake Suzaki, Kensuke Takaki, Takeshi Seki, Kazutaka Kudo, Jobu Matsuno

Abstract: An antiferromagnetic metal with two-dimensional triangular network offers a unique playground of intriguing magneto-transport properties and functionalities stemming from interplay between conducting electrons and intricate magnetic phases. A NiAs-type CrSe is one of the candidates owing to alternate stackings of Cr and Se triangular atomic networks in its crystal structure. While fabrication of C… ▽ More An antiferromagnetic metal with two-dimensional triangular network offers a unique playground of intriguing magneto-transport properties and functionalities stemming from interplay between conducting electrons and intricate magnetic phases. A NiAs-type CrSe is one of the candidates owing to alternate stackings of Cr and Se triangular atomic networks in its crystal structure. While fabrication of CrSe thin films is indispensable to develop functional devices, studies on its thin-film properties have been limited to date due to the lack of metallic samples. Here, we report on realization of metallic conductivities of CrSe thin films, which allows to investigate their intrinsic magneto-transport properties. The metallic sample exhibits co-occurrence of a weak ferromagnetism with perpendicular magnetic anisotropy and the antiferromagnetic behavior, indicating the presence of non-coplanar spin structures. In addition, control of polarity and tilting angle of the non-coplanar spin structure is accomplished by a sign of cooling magnetic fields. The observed non-coplanar spin structure, which can be a source of emergent magnetic field acting on the conducting electrons, highlights a high potential of the triangular lattice antiferromagnet and provide unique platform for functional thin-film devices composed of NiAs-type derivative Cr chalcogenides and pnictides. △ Less

Submitted 26 March, 2024; originally announced March 2024.

Comments: The following article has been accepted by APL Materials

Crossover from Integer to Fractional Quantum Hall Effect

Authors: Koji Kudo, Jonathan Schirmer, Jainendra K. Jain

Abstract: The parton theory constructs candidate fractional quantum Hall states by decomposing the physical particles into unphysical partons, placing the partons in integer quantum Hall states, and then gluing the partons back into the physical particles. Field theoretical formulations execute the gluing process through the device of emergent gauge fields. Here we study numerically the process of going fro… ▽ More The parton theory constructs candidate fractional quantum Hall states by decomposing the physical particles into unphysical partons, placing the partons in integer quantum Hall states, and then gluing the partons back into the physical particles. Field theoretical formulations execute the gluing process through the device of emergent gauge fields. Here we study numerically the process of going from the integer quantum Hall effect of two species of fermionic partons to the fractional quantum Hall effect of bosons by introducing an attractive interaction between the fermions of different species and continuously increasing its strength to glue them into bosons. To properly capture the physics in the bulk, we implement this process in a lattice version of the spherical geometry, which allows us to keep the full Hilbert space. Even though the two end-point states are topologically distinct, we find that, for the small system sizes accessible to our study, the energy gap remains open, indicating a crossover between these two states. △ Less

Submitted 26 May, 2024; v1 submitted 12 January, 2024; originally announced January 2024.

Comments: 11 pages, 8 figures

Disorder-induced topological superconductivity in a spherical quantum-Hall--superconductor hybrid

Authors: Koji Kudo, Ryota Nakai, Kentaro Nomura

Abstract: Quantum-Hall--Superconductor hybrids have been predicted to exhibit various types of topological order, providing possible platforms for intrinsically fault-tolerant quantum computing. In this paper, we develop a formulation to construct this hybrid system on a sphere, a useful geometry for identifying topologically ordered states due to its compact and contractible nature. As a preliminary step u… ▽ More Quantum-Hall--Superconductor hybrids have been predicted to exhibit various types of topological order, providing possible platforms for intrinsically fault-tolerant quantum computing. In this paper, we develop a formulation to construct this hybrid system on a sphere, a useful geometry for identifying topologically ordered states due to its compact and contractible nature. As a preliminary step using this framework, we investigate disorder effects on the Rashba-coupled quantum Hall system combined with the type-II superconductor. By diagonalizing the BdG Hamiltonian projected into a Rashba-coupled Landau level, we demonstrate the emergence of a topological superconducting phase resulting from disorders and proximity-induced pairing. Distinctive gapless modes appear in the real-space entanglement spectrum, which is consistent with topological superconductivity. △ Less

Submitted 9 January, 2024; originally announced January 2024.

Comments: 11 pages, 6 figures

Phase separation and phase transitions in undoped and Rh3+ doped iron pnictide CaFe2As2: a Raman scattering study

Authors: V. P. Gnezdilov, A. Yu. Glamazda, P. Lemmens, K. Kudo, M. Nohara

Abstract: Iron-pnictides Ca(Fe1-xRhx)2As2 (x = 0, 0.035, and 0.19) were studied across the tetragonal-orthorhombic and uncollapsed to collapsed tetragonal phase transitions using Raman spectroscopy. The effect of the phase separation was observed in the high-temperature phase for the first time. Two phases with the low-spin and high-spin states of the Fe2+ ions coexist in the undoped (x = 0) and doped (x =… ▽ More Iron-pnictides Ca(Fe1-xRhx)2As2 (x = 0, 0.035, and 0.19) were studied across the tetragonal-orthorhombic and uncollapsed to collapsed tetragonal phase transitions using Raman spectroscopy. The effect of the phase separation was observed in the high-temperature phase for the first time. Two phases with the low-spin and high-spin states of the Fe2+ ions coexist in the undoped (x = 0) and doped (x = 0.035) samples at ambient conditions. These two phases are present on a larger length scale and they are not limited to the local distortions. Both phases in the undoped sample successfully undergo tetra-to-ortho phase transitions approximately at the same temperature T0 = 160 K. In doped samples, a cascade of phase transitions is observed at temperatures T* = 100 K and Tc = 72 K with cooling for the first time. A complex type of the re-entrant magnetic structure is realized in the x = 0.035 sample at temperatures below Tc, which is distinct from the usual orthorhombic twofold one. The overdoped sample (x = 0.19) also shows phase separation at temperatures 7 - 295 K in Raman spectra similar to these of the remnant phase. △ Less

Submitted 16 August, 2023; originally announced August 2023.

Comments: 18 pages, 8 figures

Candidate local parent Hamiltonian for 3/7 fractional quantum Hall effect

Authors: Koji Kudo, A. Sharma, G. J. Sreejith, J. K. Jain

Abstract: While a parent Hamiltonian for Laughlin $1/3$ wave function has been long known in terms of the Haldane pseudopotentials, no parent Hamiltonians are known for the lowest-Landau-level projected wave functions of the composite fermion theory at $n/(2n+1)$ with $n\geq2$. If one takes the two lowest Landau levels to be degenerate, the Trugman-Kivelson interaction produces the unprojected 2/5 wave func… ▽ More While a parent Hamiltonian for Laughlin $1/3$ wave function has been long known in terms of the Haldane pseudopotentials, no parent Hamiltonians are known for the lowest-Landau-level projected wave functions of the composite fermion theory at $n/(2n+1)$ with $n\geq2$. If one takes the two lowest Landau levels to be degenerate, the Trugman-Kivelson interaction produces the unprojected 2/5 wave function as the unique zero energy solution. If the lowest three Landau levels are assumed to be degenerate, the Trugman-Kivelson interaction produces a large number of zero energy states at $ν=3/7$. We propose that adding an appropriately constructed three-body interaction yields the unprojected $3/7$ wave function as the unique zero energy solution, and report extensive exact diagonalization studies that provide strong support to this proposal. △ Less

Submitted 3 September, 2023; v1 submitted 21 May, 2023; originally announced May 2023.

Comments: 11 pages, 2 figures

Observation of Localization Using a Noisy Quantum Computer

Authors: Kazue Kudo

Abstract: Quantum dynamics in a strongly disordered quantum many-body system show localization properties. The initial state memory is maintained owing to slow relaxation when the system is in the localized regime. This work demonstrates how localization can be observed using a noisy quantum computer by evaluating the magnetization and twist overlap in a quantum spin chain after short-time evolution. The qu… ▽ More Quantum dynamics in a strongly disordered quantum many-body system show localization properties. The initial state memory is maintained owing to slow relaxation when the system is in the localized regime. This work demonstrates how localization can be observed using a noisy quantum computer by evaluating the magnetization and twist overlap in a quantum spin chain after short-time evolution. The quantities obtained from quantum-circuit simulation and real-device computation show their apparent dependence on disorder strength, although real-device computation suffers from noise-induced errors significantly. Using the exact diagonalization of the Hamiltonian, we analyze how noise-induced errors affect those quantities. The analysis also suggests how the twist overlap can reflect the information on the eigenstates of the Hamiltonian. △ Less

Submitted 11 January, 2024; v1 submitted 22 March, 2023; originally announced March 2023.

Comments: 8 pages, 4 figures

Journal ref: J. Phys. Soc. Jpn. 93, 024002 (2024)

Superconductivity in a system of interacting spinful semions

Authors: Koji Kudo, Jonathan Schirmer

Abstract: Non-interacting particles obeying certain fractional statistics have been predicted to exhibit superconductivity. We discuss the issue in an attractively interacting system of spinful semions on a lattice by numerically investigating the presence of off-diagonal long-range order at zero temperature. For this purpose, we construct a Hubbard model wherein two semions with opposite spin can virtually… ▽ More Non-interacting particles obeying certain fractional statistics have been predicted to exhibit superconductivity. We discuss the issue in an attractively interacting system of spinful semions on a lattice by numerically investigating the presence of off-diagonal long-range order at zero temperature. For this purpose, we construct a Hubbard model wherein two semions with opposite spin can virtually coincide while maintaining consistency with the fractional braiding statistics. Clear off-diagonal long range order is seen in the strong coupling limit, consistent with the expectation that a pair of semions obeys Bose statistics. We find that the semion system behaves similarly to a system of fermions with the same attractive Hubbard $U$ interaction for a wide range of $U$, suggesting that semions also undergo a BCS to BEC crossover as a function of $U$. △ Less

Submitted 28 December, 2022; v1 submitted 7 October, 2022; originally announced October 2022.

Comments: 11 pages, 10 figures

Localization detection based on quantum dynamics

Authors: Kazue Kudo

Abstract: Detecting many-body localization (MBL) typically requires the calculation of high-energy eigenstates using numerical approaches. This study investigates methods that assume the use of a quantum device to detect disorder-induced localization. Numerical simulations for small systems demonstrate how the magnetization and twist overlap, which can be easily obtained from the measurement of qubits in a… ▽ More Detecting many-body localization (MBL) typically requires the calculation of high-energy eigenstates using numerical approaches. This study investigates methods that assume the use of a quantum device to detect disorder-induced localization. Numerical simulations for small systems demonstrate how the magnetization and twist overlap, which can be easily obtained from the measurement of qubits in a quantum device, change from the thermal phase to the localized phase. The twist overlap evaluated using the wave function at the end of the time evolution behaves similarly to the one evaluated with eigenstates in the middle of the energy spectrum under a specific condition. The twist overlap evaluated using the wave function after time evolution for many disorder realizations is a promising probe for detecting MBL in quantum computing approaches. △ Less

Submitted 28 October, 2022; v1 submitted 18 June, 2022; originally announced June 2022.

Comments: 9 pages, 4 figures

Journal ref: Entropy 24, 1085 (2022)

Exactly Solvable Hamiltonian for Non-Abelian Quasiparticles

Authors: Koji Kudo, A. Sharma, G. J. Sreejith, J. K. Jain

Abstract: Particles obeying non-Abelian braid statistics have been predicted to emerge in the fractional quantum Hall effect. In particular, a model Hamiltonian with short-range three-body interaction ($\hat{V}^\text{Pf}_3$) between electrons confined to the lowest Landau level provides exact solutions for quasiholes, and thereby allows a proof of principle for the existence of quasiholes obeying non-Abelia… ▽ More Particles obeying non-Abelian braid statistics have been predicted to emerge in the fractional quantum Hall effect. In particular, a model Hamiltonian with short-range three-body interaction ($\hat{V}^\text{Pf}_3$) between electrons confined to the lowest Landau level provides exact solutions for quasiholes, and thereby allows a proof of principle for the existence of quasiholes obeying non-Abelian braid statistics. We construct, in terms of two- and three- body Haldane pseudopotentials, a model Hamiltonian that can be solved exactly for both quasiholes and quasiparticles, and provide evidence of non-Abelian statistics for the latter as well. The structure of the quasiparticle states of this model is in agreement with that predicted by the bipartite composite-fermion model of quasiparticles with exact lowest Landau level projection. We further demonstrate adiabatic continuity for the ground state, the ordinary neutral excitation, and the topological exciton as we deform our model Hamiltonian continuously into the lowest Landau-level $\hat{V}^\text{Pf}_3$ Hamiltonian. △ Less

Submitted 21 July, 2022; v1 submitted 15 June, 2022; originally announced June 2022.

Comments: 15 pages, 10 figures

Revisiting excitation gaps in the fractional quantum Hall effect

Authors: Tongzhou Zhao, Koji Kudo, W. N. Faugno, Ajit C. Balram, J. K. Jain

Abstract: Recent systematic measurements of the quantum well width dependence of the excitation gaps of fractional quantum Hall states in high mobility samples [Villegas Rosales {\it et al.}, Phys. Rev. Lett. {\bf 127}, 056801 (2021)] open the possibility of a better quantitative understanding of this important issue. We present what we believe to be accurate theoretical gaps including the effects of finite… ▽ More Recent systematic measurements of the quantum well width dependence of the excitation gaps of fractional quantum Hall states in high mobility samples [Villegas Rosales {\it et al.}, Phys. Rev. Lett. {\bf 127}, 056801 (2021)] open the possibility of a better quantitative understanding of this important issue. We present what we believe to be accurate theoretical gaps including the effects of finite width and Landau level (LL) mixing. While theory captures the width dependence, there still remains a deviation between the calculated and the measured gaps, presumably caused by disorder. It is customary to model the experimental gaps of the $n/(2n\pm 1)$ states as $Δ_{n/(2n\pm 1)} = Ce^2/[(2n\pm 1)\varepsilon l]-Γ$, where $\varepsilon$ is the dielectric constant of the background semiconductor and $l$ is the magnetic length; the first term is interpreted as the cyclotron energy of composite fermions and $Γ$ as a disorder-induced broadening of composite-fermion LLs. Fitting the gaps for various fractional quantum Hall states, we find that $Γ$ can be nonzero even in the absence of disorder. △ Less

Submitted 31 May, 2022; originally announced May 2022.

Comments: 6 pages, 7 figures, includes supplemental material

Journal ref: Phys. Rev. B 105, 205147 (2022)

Procedure to Reveal the Mechanism of Pattern Formation Process by Topological Data Analysis

Authors: Yoh-ichi Mototake, Masaichiro Mizumaki, Kazue Kudo, Kenji Fukumizu

Abstract: Topological data analysis (TDA) is a versatile tool that can be used to extract scientific knowledge from complex pattern formation processes. However, the physics correspondence between the features obtained from TDA and pattern dynamics does not agree one-to-one, and the physical interpretation of the TDA features needs to be set appropriately according to the phenomenon to be analyzed. In this… ▽ More Topological data analysis (TDA) is a versatile tool that can be used to extract scientific knowledge from complex pattern formation processes. However, the physics correspondence between the features obtained from TDA and pattern dynamics does not agree one-to-one, and the physical interpretation of the TDA features needs to be set appropriately according to the phenomenon to be analyzed. In this study, we propose an analytical procedure to physically interpret pattern dynamics through TDA and machine learning techniques. The proposed procedure was applied to the process of magnetic domain pattern formation to quantify non-trivial domain pattern classifications and reveal the nature of the underlying dynamics. On the basis of these findings, we also propose a candidate reduction model to understand the nature of magnetic domain formation. △ Less

Submitted 8 July, 2024; v1 submitted 26 April, 2022; originally announced April 2022.

Comments: 54 pages, 19 figures

Adiabatic Continuity of the Spinful Quantum Hall States

Authors: Koji Kudo, Yasuhiro Hatsugai

Abstract: By using the extended Hubbard model of anyons, we numerically demonstrate the adiabatic deformation of the spinful quantum Hall (QH) states by transmutation of statistical fluxes. While the ground state is always spin-polarized in a series of $ν=1$ integer QH system, the adiabatic continuity between the singlet QH states at $ν=2$ and $ν=2/5$ is confirmed. These results are consistent with the comp… ▽ More By using the extended Hubbard model of anyons, we numerically demonstrate the adiabatic deformation of the spinful quantum Hall (QH) states by transmutation of statistical fluxes. While the ground state is always spin-polarized in a series of $ν=1$ integer QH system, the adiabatic continuity between the singlet QH states at $ν=2$ and $ν=2/5$ is confirmed. These results are consistent with the composite fermion theory with spin. The many-body Chern number of the ground state multiplet works as an adiabatic invariant and also explains the wild change of the topological degeneracy during the evolution. The generalized Streda formula of spinful systems is justified. △ Less

Submitted 19 January, 2022; originally announced January 2022.

Comments: 8 pages, 5 figures

Domain dependent Fermi arcs observed in a striped phase dichalcogenide

Authors: T. Mizokawa, A. Barinov, V. Kandyba, A. Giampietri, R. Matsumoto, Y. Okamoto, K. Takubo, K. Miyamoto, T. Okuda, S. Pyon, H. Ishii, K. Kudo, M. Nohara, N. L. Saini

Abstract: Angle-resolved photoemission spectromicroscopy on IrTe2 reveals evolution of mesoscopic striped domains across its first order phase transition at about 280 K. The striped texture of the domains is characterized by a herringbone arrangement of the electronic anisotropy axes. Under further cooling down to 47 K, the striped domains evolve into trijunction domains with the electronic anisotropy in th… ▽ More Angle-resolved photoemission spectromicroscopy on IrTe2 reveals evolution of mesoscopic striped domains across its first order phase transition at about 280 K. The striped texture of the domains is characterized by a herringbone arrangement of the electronic anisotropy axes. Under further cooling down to 47 K, the striped domains evolve into trijunction domains with the electronic anisotropy in three directions. Each domain harbors quasi one-dimensional surface bands forming Fermi arcs with peculiar spin polarization. The Fermi arc corresponds to an edge state of the two-dimensional bulk electronic states truncated at the surface, indicating an interesting interplay between the symmetry breaking and the surface electronic states. △ Less

Submitted 11 December, 2021; originally announced December 2021.

Comments: 11 pages + 5 figures

$^{139}$La-NMR study of spin-dynamics coupled with hole mobility in $T$*-type La$_{0.86}$Eu$_{0.86}$Sr$_{0.28}$CuO$_{4-δ}$

Authors: Takanori Taniguchi, Shunsaku Kitagawa, Kenji Ishida, Shun Asano, Kota Kudo, Motofumi Takahama, Peiao Xie, Takashi Noji, Masaki Fujita

Abstract: In $T$*-type cuprate oxides with five oxygen coordination, little is known about the relationship between the spin correlations and dope carriers. We performed $^{139}$La-nuclear magnetic resonance (NMR) and electrical resistivity measurements on an as-sintered (AS) and oxidation annealed (OA) polycrystalline $T$*-type La$_{0.86}$Eu$_{0.86}$S$_{0.28}$CuO$_4$ (LESCO) to investigate its magnetic and… ▽ More In $T$*-type cuprate oxides with five oxygen coordination, little is known about the relationship between the spin correlations and dope carriers. We performed $^{139}$La-nuclear magnetic resonance (NMR) and electrical resistivity measurements on an as-sintered (AS) and oxidation annealed (OA) polycrystalline $T$*-type La$_{0.86}$Eu$_{0.86}$S$_{0.28}$CuO$_4$ (LESCO) to investigate its magnetic and superconducting (SC) properties. Upon cooling, the NMR spectrum of AS LESCO broadened below 3 K, at which the nuclear spin-lattice relaxation rate $1/T_1$ against the temperature exhibited a maximum, thereby indicating the appearance of static magnetism. The temperature dependence of $1/T_1$ between 3 K and 20 K was similar to that of the resistivity displaying the semiconducting behavior. Furthermore, the energy scale of the transport gap and spin-dynamics estimated was found to be comparable. These results suggest a close connection between the mobility of the doped carriers and low-energy spin-dynamics, as reported for lightly doped $T$-type La$_{2-x}$Sr$_x$CuO$_4$. In the OA SC sample, we confirmed the absence of a magnetic order and the Korringa relation above 10 K. Therefore, in the $T$*-type LESCO with $x$ = 0.28, the magnetic state coupled with holes drastically turns to the weakly correlated metallic state by oxidation annealing. △ Less

Submitted 23 October, 2021; originally announced October 2021.

Comments: 6 pages, 6 figures

Bulk-edge Correspondence in the Adiabatic Heuristic Principle

Authors: Koji Kudo, Yoshihito Kuno, Yasuhiro Hatsugai

Abstract: Using the Laughlin's argument on a torus with two pin-holes, we numerically demonstrate that the discontinuities of the center-of-mass work well as an invariant of the pumping phenomena during the process of the flux-attachment, trading the magnetic flux for the statistical one. This is consistent with the bulk-edge correspondence of the fractional quantum Hall effect of anyons. We also confirm th… ▽ More Using the Laughlin's argument on a torus with two pin-holes, we numerically demonstrate that the discontinuities of the center-of-mass work well as an invariant of the pumping phenomena during the process of the flux-attachment, trading the magnetic flux for the statistical one. This is consistent with the bulk-edge correspondence of the fractional quantum Hall effect of anyons. We also confirm that the general feature of the edge states remains unchanged during the process while the topological degeneracy is discretely changed. This supports the stability of the quantum Hall edge states in the adiabatic heuristic principle. △ Less

Submitted 19 January, 2022; v1 submitted 19 June, 2021; originally announced June 2021.

Comments: 7 pages, 5 figures

Higher-Order Topological Mott Insulator on the Pyrochlore Lattice

Authors: Yuichi Otsuka, Tsuneya Yoshida, Koji Kudo, Seiji Yunoki, Yasuhiro Hatsugai

Abstract: We provide the first unbiased evidence for a higher-order topological Mott insulator in three dimensions by numerically exact quantum Monte Carlo simulations. This insulating phase is adiabatically connected to a third-order topological insulator in the noninteracting limit, which features gapless modes around the corners of the pyrochlore lattice and is characterized by a $\mathbb{Z}_{4}$ spin-Be… ▽ More We provide the first unbiased evidence for a higher-order topological Mott insulator in three dimensions by numerically exact quantum Monte Carlo simulations. This insulating phase is adiabatically connected to a third-order topological insulator in the noninteracting limit, which features gapless modes around the corners of the pyrochlore lattice and is characterized by a $\mathbb{Z}_{4}$ spin-Berry phase. The difference between the correlated and non-correlated topological phases is that in the former phase the gapless corner modes emerge only in spin excitations being Mott-like. We also show that the topological phase transition from the third-order topological Mott insulator to the usual Mott insulator occurs when the bulk spin gap solely closes. △ Less

Submitted 25 October, 2021; v1 submitted 20 May, 2021; originally announced May 2021.

Comments: 10 pages, 9 figures

Journal ref: Scientific Reports 11, 20270 (2021)

Pattern Formation Simulated by an Ising Machine

Authors: Kanon Mukai, Kazue Kudo

Abstract: In a ferromagnetic Ising system, domain pattern formation, i.e., phase-ordering, occurs after a sudden quench. We propose the method to simulate the pattern formation dynamics by an Ising machine. We demonstrate that the method reproduces domain patterns similar to those simulated by the Monte Carlo method. Moreover, the same domain growth law is observed in the proposed method and the Monte Carlo… ▽ More In a ferromagnetic Ising system, domain pattern formation, i.e., phase-ordering, occurs after a sudden quench. We propose the method to simulate the pattern formation dynamics by an Ising machine. We demonstrate that the method reproduces domain patterns similar to those simulated by the Monte Carlo method. Moreover, the same domain growth law is observed in the proposed method and the Monte Carlo method. △ Less

Submitted 28 January, 2021; originally announced January 2021.

Comments: 3 pages, 2 figures

Journal ref: J. Phys. Soc. Jpn. 90, 025004 (2021)

Fermi-liquid state in $T$*-type La$_{1-x/2}$Eu$_{1-x/2}$Sr$_x$CuO$_4$ revealed via element substitution effects on magnetism

Authors: Takanori Taniguchi, Kota Kudo, Shun Asano, Motofumi Takahama, Isao Watanabe, Akihiro Koda, Masaki Fujita

Abstract: Despite its unique structural features, the magnetism of single-layered cuprate with five oxygen coordination ($T$*-type structure) has not been investigated thus far. Here, we report the results of muon spin relaxation and magnetic susceptibility measurements to elucidate the magnetism of $T$*-type La$_{1-x/2}$Eu$_{1-x/2}$Sr$_x$CuO$_4$ (LESCO) via magnetic Fe- and non-magnetic Zn-substitution. We… ▽ More Despite its unique structural features, the magnetism of single-layered cuprate with five oxygen coordination ($T$*-type structure) has not been investigated thus far. Here, we report the results of muon spin relaxation and magnetic susceptibility measurements to elucidate the magnetism of $T$*-type La$_{1-x/2}$Eu$_{1-x/2}$Sr$_x$CuO$_4$ (LESCO) via magnetic Fe- and non-magnetic Zn-substitution. We clarified the inducement of the spin-glass (SG)-like magnetically ordered state in La$_{1-x/2}$Eu$_{1-x/2}$Sr$_x$Cu$_y$Fe$_{1-y}$O$_4$ with $x = 0.24 + y$, and the non-magnetic state in La$_{1-x/2}$Eu$_{1-x/2}$Sr$_x$Cu$_y$Zn$_{1-y}$O$_4$ with $x$ = 0.24 after the suppression of superconductivity for $y$ $\geq$ 0.025. The SG state lies below $\sim$7 K in a wide Sr concentration range between 0.19 and 0.34 in 5$\%$ Fe-substituted LESCO. The short-range SG state is consistent with that originating from the Ruderman-Kittel-Kasuya-Yosida interaction in a metallic state. Thus, the results provide the first evidence for Fermi liquid (FL) state in the pristine $T$*-type LESCO. Taking into account the results of an oxygen $K$-edge X-ray absorption spectroscopy measurement $[$J. Phys. Soc. Jpn. 89, 075002 (2020)$]$ reporting the actual hole concentrations in LESCO, our results demonstrate the existence of the FL state in a lower hole-concentration region, compared to that in $T$-type La$_{2-x}$Sr$_x$CuO$_4$. The emergence of the FL state in a lower hole-concentration region is possibly associated with a smaller charge transfer gap energy in the parent material with five oxygen coordination. △ Less

Submitted 7 August, 2024; v1 submitted 7 December, 2020; originally announced December 2020.

Comments: 8 pages, 6 figures, accepted for publication in Phys. Rev. B

Image Analysis Based on Nonnegative/Binary Matrix Factorization

Authors: Hinako Asaoka, Kazue Kudo

Abstract: Using nonnegative/binary matrix factorization (NBMF), a matrix can be decomposed into a nonnegative matrix and a binary matrix. Our analysis of facial images, based on NBMF and using the Fujitsu Digital Annealer, leads to successful image reconstruction and image classification. The NBMF algorithm converges in fewer iterations than those required for the convergence of nonnegative matrix factoriza… ▽ More Using nonnegative/binary matrix factorization (NBMF), a matrix can be decomposed into a nonnegative matrix and a binary matrix. Our analysis of facial images, based on NBMF and using the Fujitsu Digital Annealer, leads to successful image reconstruction and image classification. The NBMF algorithm converges in fewer iterations than those required for the convergence of nonnegative matrix factorization (NMF), although both techniques perform comparably in image classification. △ Less

Submitted 2 July, 2020; originally announced July 2020.

Comments: 3 pages, 1 figure

Journal ref: J. Phys. Soc. Jpn. 89, 085001 (2020)

Fate of fractional quantum Hall states in open quantum systems: characterization of correlated topological states for the full Liouvillian

Authors: Tsuneya Yoshida, Koji Kudo, Hosho Katsura, Yasuhiro Hatsugai

Abstract: Despite previous extensive analysis of open quantum systems described by the Lindblad equation, it is unclear whether correlated topological states, such as fractional quantum Hall states, are maintained even in the presence of the jump term. In this paper, we introduce the pseudo-spin Chern number of the Liouvillian which is computed by twisting the boundary conditions only for one of the subspac… ▽ More Despite previous extensive analysis of open quantum systems described by the Lindblad equation, it is unclear whether correlated topological states, such as fractional quantum Hall states, are maintained even in the presence of the jump term. In this paper, we introduce the pseudo-spin Chern number of the Liouvillian which is computed by twisting the boundary conditions only for one of the subspaces of the doubled Hilbert space. The existence of such a topological invariant elucidates that the topological properties remain unchanged even in the presence of the jump term which does not close the gap of the effective non-Hermitian Hamiltonian (obtained by neglecting the jump term). In other words, the topological properties are encoded into an effective non-Hermitian Hamiltonian rather than the full Liouvillian. This is particularly useful when the jump term can be written as a strictly block-upper (-lower) triangular matrix in the doubled Hilbert space, in which case the presence or absence of the jump term does not affect the spectrum of the Liouvillian. With the pseudo-spin Chern number, we address the characterization of fractional quantum Hall states with two-body loss but without gain, elucidating that the topology of the non-Hermitian fractional quantum Hall states is preserved even in the presence of the jump term. This numerical result also supports the use of the non-Hermitian Hamiltonian which significantly reduces the numerical cost. Similar topological invariants can be extended to treat correlated topological states for other spatial dimensions and symmetry (e.g., one-dimensional open quantum systems with inversion symmetry), indicating the high versatility of our approach. △ Less

Submitted 8 September, 2020; v1 submitted 26 May, 2020; originally announced May 2020.

Comments: 16 pages, 4figures, (to appear in Phys. Rev. Research)

Journal ref: Phys. Rev. Research 2, 033428 (2020)

Distinct variation of electronic states due to annealing in La$_{1.8}$Eu$_{0.2}$CuO$_4$ and Nd$_{2}$CuO$_4$

Authors: Shun Asano, Kenji Ishii, Daiju Matsumura, Takuya Tsuji, Kota Kudo, Takanori Taniguchi, Shin Saito, Toshiki Sunohara, Takayuki Kawamata, Yoji Koike, Masaki Fujita

Abstract: We performed Cu {\it K}-edge X-ray absorption fine structure measurements on T'-type La$_{1.8}$Eu$_{0.2}$CuO$_4$ (LECO) and Nd$_2$CuO$_4$ (NCO) to investigate the variation in the electronic state associated with the emergence of superconductivity due to annealing. The X-ray absorption near-edge structure spectra of as-sintered (AS) LECO are quite similar to those of AS NCO, indicating that the gr… ▽ More We performed Cu {\it K}-edge X-ray absorption fine structure measurements on T'-type La$_{1.8}$Eu$_{0.2}$CuO$_4$ (LECO) and Nd$_2$CuO$_4$ (NCO) to investigate the variation in the electronic state associated with the emergence of superconductivity due to annealing. The X-ray absorption near-edge structure spectra of as-sintered (AS) LECO are quite similar to those of AS NCO, indicating that the ground state of AS T'-type LECO is a Mott insulator. We found a significant variation of the electronic state at the Cu sites in LECO due to annealing. The electron density after annealing ($n_{\rm AN}$) was evaluated for both superconducting LECO and non-superconducting NCO and found to be 0.40 and 0.05 electrons per Cu, respectively. In LECO but not in NCO, extended X-ray absorption fine structure analysis revealed a softening in the strength of the Cu-O bond in the CuO$_2$ plane due to annealing, which is consistent with the screening effect on phonons in the metallic state. Since the amounts of oxygen loss due to annealing ($δ$) for LECO and NCO are comparable with each other, these results suggest distinct electron-doping processes in the two compounds. That electron-doping in NCO approximately follows the relation $n_{\rm AN}=2δ$ can be understood if electrons are doped through oxygen deficiency, but the anneal-induced metallic nature and large $n_{\rm AN}$ of LECO suggest a variation of the electronic band structure causes self-doping of carriers. The origin of the difference in doping processes due to annealing is discussed in connection with the size of the charge transfer gap. △ Less

Submitted 21 May, 2020; originally announced May 2020.

Comments: 6 pages, 4 figures, 1 table

Adiabatic Heuristic Principle on a Torus and Generalized Streda Formula

Authors: Koji Kudo, Yasuhiro Hatsugai

Abstract: Although the adiabatic heuristic argument of the fractional quantum Hall states has been successful, continuous modification of the flux/statistics of anyons is strictly prohibited due to algebraic constrains of the braid group on a torus. We have numerically shown that the adiabatic heuristic principle for anyons is still valid even though the Hamiltonians cannot be modified continuously. The Che… ▽ More Although the adiabatic heuristic argument of the fractional quantum Hall states has been successful, continuous modification of the flux/statistics of anyons is strictly prohibited due to algebraic constrains of the braid group on a torus. We have numerically shown that the adiabatic heuristic principle for anyons is still valid even though the Hamiltonians cannot be modified continuously. The Chern number of the ground state multiplet is the adiabatic invariant, while the number of the topological degeneracy behaves wildly. A generalized Streda formula is proposed that explains the degeneracy pattern. Nambu-Goldston modes associated with the anyon superconductivity are also suggested numerically. △ Less

Submitted 10 September, 2020; v1 submitted 2 April, 2020; originally announced April 2020.

Comments: 7 pages

Journal ref: Phys. Rev. B 102, 125108 (2020)

Thermal Conductivity and Magnetic Phase Diagram of CuB2O4

Authors: T. Kawamata, N. Sugawara, S. M. Haidar, T. Adachi, T. Noji, K. Kudo, N. Kobayashi, Y. Fujii, H. Kikuchi, M. Chiba, G. A. Petrakovskii, M. A. Popov, L. N. Bezmaternykh, Y. Koike

Abstract: We have measured temperature and magnetic field dependences of the thermal conductivity along the c-axis, kc, and that along the [110] direction, k110, of CuB2O4 single crystals in zero field and magnetic fields along the c-axis and along the [110] direction. It has been found that the thermal conductivity is nearly isotropic and very large in zero field and that the thermal conductivity due to ph… ▽ More We have measured temperature and magnetic field dependences of the thermal conductivity along the c-axis, kc, and that along the [110] direction, k110, of CuB2O4 single crystals in zero field and magnetic fields along the c-axis and along the [110] direction. It has been found that the thermal conductivity is nearly isotropic and very large in zero field and that the thermal conductivity due to phonons is dominant in CuB2O4. The temperature and field dependences of kc and k110 have markedly changed at phase boundaries in the magnetic phase diagram, which has been understood to be due to the change of the mean free path of phonons caused by the change of the phonon-spin scattering rate at the phase boundaries. It has been concluded that thermal conductivity measurements are very effective for detecting magnetic phase boundaries. △ Less

Submitted 30 September, 2019; originally announced October 2019.

Comments: 18 pages, 6 figures

Scale-invariant relaxation dynamics in two-component Bose-Einstein condensates with large particle-number imbalance

Authors: Kazuya Fujimoto, Kazunori Haneda, Kazue Kudo, Yuki Kawaguchi

Abstract: We theoretically study the scale-invariant relaxation dynamics in segregating two-component Bose-Einstein condensates with large particle-number imbalance, and uncover that random walk of droplet for the minor component plays a fundamental role in the relaxation process. Our numerical simulations based on the binary Gross-Pitaevskii model reveal the emergence of the dynamical scaling during the re… ▽ More We theoretically study the scale-invariant relaxation dynamics in segregating two-component Bose-Einstein condensates with large particle-number imbalance, and uncover that random walk of droplet for the minor component plays a fundamental role in the relaxation process. Our numerical simulations based on the binary Gross-Pitaevskii model reveal the emergence of the dynamical scaling during the relaxation, which is a hallmark of scale-invariant dynamics, in a correlation function for the minor condensate. Tracking exponents characterizing the dynamical scaling in time, we find out a crossover phenomenon that features the change in power exponents of the correlation length. To understand the fundamental mechanism inherent in the scale-invariant relaxation dynamics, we construct a random walk model for droplets. Employing the model, we analytically derive the $1/3$ and $1/2$ power laws and predict the crossover of the scaling. These exponents are in reasonable agreement with the values obtained in the numerical calculations. We also discuss a possible experimental setup for observing the scale-invariant dynamics. △ Less

Submitted 19 January, 2020; v1 submitted 30 July, 2019; originally announced July 2019.

Comments: 16 pages, 10 figures

Journal ref: Phys. Rev. A 101, 023608 (2020)

Non-Hermitian fractional quantum Hall states

Authors: Tsuneya Yoshida, Koji Kudo, Yasuhiro Hatsugai

Abstract: We demonstrate the emergence of a topological ordered phase for non-Hermitian systems. Specifically, we elucidate that systems with non-Hermitian two-body interactions show a fractional quantum Hall (FQH) state. The non-Hermitian Hamiltonian is considered to be relevant to cold atoms with dissipation. We conclude the emergence of the non-Hermitian FQH state by the presence of the topological degen… ▽ More We demonstrate the emergence of a topological ordered phase for non-Hermitian systems. Specifically, we elucidate that systems with non-Hermitian two-body interactions show a fractional quantum Hall (FQH) state. The non-Hermitian Hamiltonian is considered to be relevant to cold atoms with dissipation. We conclude the emergence of the non-Hermitian FQH state by the presence of the topological degeneracy and by the many-body Chern number for the ground state multiplet showing $C_{\mathrm{tot}}=1$. The robust topological degeneracy against non-Hermiticity arises from the many-body translational symmetry. Furthermore, we discover that the FQH state emerges without any repulsive interactions, which is attributed to a phenomenon reminiscent of the continuous quantum Zeno effect. △ Less

Submitted 22 July, 2019; v1 submitted 17 July, 2019; originally announced July 2019.

Comments: 8 pages, 5 figures, typos were corrected

Journal ref: Scientific Reports 9, 16895 (2019)

Higher-order Topological Mott Insulators

Authors: Koji Kudo, Tsuneya Yoshida, Yasuhiro Hatsugai

Abstract: We propose a new correlated topological state which we call a higher-order topological Mott insulator (HOTMI). This state exhibits a striking bulk-boundary correspondence due to electron correlations. Namely, the topological properties in the bulk, characterized by the Z3 spin-Berry phase, result in gapless corner modes emerging only in spin excitations (i.e., the single-particle excitations remai… ▽ More We propose a new correlated topological state which we call a higher-order topological Mott insulator (HOTMI). This state exhibits a striking bulk-boundary correspondence due to electron correlations. Namely, the topological properties in the bulk, characterized by the Z3 spin-Berry phase, result in gapless corner modes emerging only in spin excitations (i.e., the single-particle excitations remain gapped around the corner). We demonstrate the emergence of the HOTMI in a Hubbard model on the kagome lattice, and elucidate how strong correlations change gapless corner modes at the noninteracting case. △ Less

Submitted 12 November, 2019; v1 submitted 9 May, 2019; originally announced May 2019.

Journal ref: Phys. Rev. Lett. 123, 196402 (2019)

Oxidation annealing effects on the spin-glass-like magnetism and appearance of superconductivity in T*-type La$_{1-x/2}$Eu$_{1-x/2}$Sr$_x$CuO$_4$ (0.14 $\leq x \leq$ 0.28)

Authors: Shun Asano, Kensuke M. Suzuki, Kota Kudo, Isao Watanabe, Akihiro Koda, Ryosuke Kadono, Takashi Noji, Yoji Koike, Takanori Taniguchi, Shunsaku Kitagawa, Kenji Ishida, Masaki Fujita

Abstract: We investigated the magnetism and superconductivity in as-sintered (AS) and oxidation annealed (OA) T*-type La$_{1-x/2}$Eu$_{1-x/2}$Sr$_x$CuO$_4$ (LESCO) with 0.14 $\leq x \leq$ 0.28 by the first comprehensive muon spin rotation/relaxation ($μ$SR), magnetic susceptibility, and electrical resistivity measurements. In OA superconducting samples, no evidence of magnetic order was observed, whereas AS… ▽ More We investigated the magnetism and superconductivity in as-sintered (AS) and oxidation annealed (OA) T*-type La$_{1-x/2}$Eu$_{1-x/2}$Sr$_x$CuO$_4$ (LESCO) with 0.14 $\leq x \leq$ 0.28 by the first comprehensive muon spin rotation/relaxation ($μ$SR), magnetic susceptibility, and electrical resistivity measurements. In OA superconducting samples, no evidence of magnetic order was observed, whereas AS semiconducting samples exhibited evidence of a disordered magnetic state in the measured temperature range between $\sim$4 K and $\sim$8 K. Therefore, the ground state in LESCO drastically varies with oxidation annealing and the magnetic phase competitively exists with the superconducting (SC) phase. The magnetic phase in the AS LESCO is quite robust against Sr doping, while the SC phase degrades with increasing $x$. A monotonous decrease of the SC transition temperature from 24.5 K in $x$ = 0.14 to 9.0 K in $x$ = 0.28 suggests the disappearance of the SC phase at $x$ $\sim$ 0.34. Furthermore, we clarified the simultaneous development of (quasi) static magnetism and the electrical resistivity at a low temperature in AS samples, suggesting the inducement of magnetism by the suppression of carrier mobility. The variation in magnetism due to annealing is discussed from a viewpoint of structural defects, which was previously reported from neutron diffraction measurements. △ Less

Submitted 12 June, 2019; v1 submitted 16 April, 2019; originally announced April 2019.

Journal ref: J. Phys. Soc. Jpn. 88, 084709 (2019)

Localization in the constrained quantum annealing of graph coloring

Authors: Kazue Kudo

Abstract: Constrained quantum annealing (CQA) is a quantum annealing approach that is designed so that constraints are satisfied without penalty terms. There is an analogy between the model for the CQA of graph coloring and a set of disordered spin chains. In the model for the CQA of graph coloring, disorder corresponds to the fluctuation of effective local fields that increase in a CQA process. Numerical s… ▽ More Constrained quantum annealing (CQA) is a quantum annealing approach that is designed so that constraints are satisfied without penalty terms. There is an analogy between the model for the CQA of graph coloring and a set of disordered spin chains. In the model for the CQA of graph coloring, disorder corresponds to the fluctuation of effective local fields that increase in a CQA process. Numerical simulations of effective fields and entanglement demonstrate how localization appears in the CQA. Some notable features appear in the concurrence, which is a measure of entanglement, plotted as a function of the fluctuation of effective fields. △ Less

Submitted 1 March, 2020; v1 submitted 21 February, 2019; originally announced February 2019.

Comments: 7 pages, 7 figures

Journal ref: J. Phys. Soc. Jpn. 89, 064001 (2020)

Temperature-dependent local structure of superconducting BaPd$_2$As$_2$ and SrPd$_2$As$_2$

Authors: K. Terashima, E. Paris, L. Simonelli, E. Salas-Colera, A. Puri, T. Wakita, Y. Yamada, S. Nakano, H. Idei, K. Kudo, M. Nohara, Y. Muraoka, T. Mizokawa, T. Yokoya, N. L. Saini

Abstract: The local structures of 122-type paradium arsenides, namely BaPd$_2$As$_2$ and SrPd$_2$As$_2$, are examined by As K-edge extended x-ray absorption fine structure measurements to find a possible correlation between the variation of their superconducting transition temperature and the local structure. The local atomic distances are found to be consistent with average distances measured by diffractio… ▽ More The local structures of 122-type paradium arsenides, namely BaPd$_2$As$_2$ and SrPd$_2$As$_2$, are examined by As K-edge extended x-ray absorption fine structure measurements to find a possible correlation between the variation of their superconducting transition temperature and the local structure. The local atomic distances are found to be consistent with average distances measured by diffraction techniques. The temperature dependence of mean square relative displacements reveal that, while BaPd$_2$As$_2$ is characterized by a local As-Pd soft mode, albeit with larger atomic disorder, SrPd$_2$As$_2$ shows anomalous As-Pd correlations with a kink at $\sim$160 K due to hardening by raising temperature. We have discussed implications of these results and possible mechanism of differing superconducting transition temperature in relation with the structural instability. △ Less

Submitted 1 October, 2018; originally announced October 2018.

Comments: Main text: 5 pages, 4 figures, Supplemental information: 2 pages, 1 figure, 1 table

Journal ref: Phys. Rev. B 98, 094525 (2018)

Composition-induced structural instability and strong-coupling superconductivity in Au1-xPdxTe2

Authors: Kazutaka Kudo, Hiroyuki Ishii, Minoru Nohara

Abstract: The physical properties and structural evolution of the MX$_2$-type solid solution Au$_{1-x}$Pd$_x$Te$_2$ are reported. The end member AuTe$_2$ is a normal metal with a monoclinic distorted CdI$_2$-type structure with preformed Te-Te dimers. A monoclinic--trigonal structural phase transition at a finite temperature occurs upon Pd substitution and is suppressed to zero temperature near $x$ = 0.55,… ▽ More The physical properties and structural evolution of the MX$_2$-type solid solution Au$_{1-x}$Pd$_x$Te$_2$ are reported. The end member AuTe$_2$ is a normal metal with a monoclinic distorted CdI$_2$-type structure with preformed Te-Te dimers. A monoclinic--trigonal structural phase transition at a finite temperature occurs upon Pd substitution and is suppressed to zero temperature near $x$ = 0.55, and a superconducting phase with a maximum $T_{\rm c}$ = 4.65 K emerges. A clear indication of strong coupling superconductivity is observed near the composition of the structural instability. The competitive relationship between Te-Te dimers and superconductivity is proposed. △ Less

Submitted 4 September, 2018; originally announced September 2018.

Comments: 6 pages, 8 figures

Journal ref: Phys. Rev. B 93, 140505(R) (2016)

Superconductivity in BaPtSb with an Ordered Honeycomb Network

Authors: Kazutaka Kudo, Yuki Saito, Takaaki Takeuchi, Shin-ya Ayukawa, Takayuki Kawamata, Shinichiro Nakamura, Yoji Koike, Minoru Nohara

Abstract: Superconductivity in BaPtSb with the SrPtSb-type structure (space group $P\bar{6}m2$, $D_{3h}^1$, No. 187) is reported. The structure consists of a PtSb ordered honeycomb network that stacks along the $c$-axis so that spatial inversion symmetry is broken globally. Electrical resistivity and specific-heat measurements revealed that the compound exhibited superconductivity at 1.64 K. The noncentrosy… ▽ More Superconductivity in BaPtSb with the SrPtSb-type structure (space group $P\bar{6}m2$, $D_{3h}^1$, No. 187) is reported. The structure consists of a PtSb ordered honeycomb network that stacks along the $c$-axis so that spatial inversion symmetry is broken globally. Electrical resistivity and specific-heat measurements revealed that the compound exhibited superconductivity at 1.64 K. The noncentrosymmetric structure and the strong spin-orbit coupling of Pt and Sb make BaPtSb an attractive compound for studying the exotic superconductivity predicted for a honeycomb network. △ Less

Submitted 3 September, 2018; originally announced September 2018.

Comments: 3 pages, 2 figures

Journal ref: J. Phys. Soc. Jpn. 87, 063702 (2018)

Superconductivity in Hexagonal BaPtAs: SrPtSb- and YPtAs-type Structures with Ordered Honeycomb Network

Authors: Kazutaka Kudo, Takaaki Takeuchi, Hiromi Ota, Yuki Saito, Shin-ya Ayukawa, Kazunori Fujimura, Minoru Nohara

Abstract: The crystal structure and superconductivity of hexagonal BaPtAs are reported. Single-crystal X-ray diffraction, magnetization, electrical resistivity, and specific heat measurements were performed in this study. Two hexagonal structures with different PtAs honeycomb network stacking sequences, namely, SrPtSb- (space group $P\bar{6}m2$, $D_{3h}^1$, No. 187) and YPtAs-type ($P6_3/mmc$, $D_{6h}^4$, N… ▽ More The crystal structure and superconductivity of hexagonal BaPtAs are reported. Single-crystal X-ray diffraction, magnetization, electrical resistivity, and specific heat measurements were performed in this study. Two hexagonal structures with different PtAs honeycomb network stacking sequences, namely, SrPtSb- (space group $P\bar{6}m2$, $D_{3h}^1$, No. 187) and YPtAs-type ($P6_3/mmc$, $D_{6h}^4$, No. 194) structures, were identified and found to exhibit superconductivity at 2.8 and 2.1-3.0 K, respectively. In contrast, the cubic LaIrSi-type structure ($P2_13$, $T^4$, No. 198) did not exhibit superconductivity above 0.1 K. BaPtAs provides a unique opportunity to study superconductivity with broken and preserved spatial inversion symmetry. △ Less

Submitted 3 September, 2018; originally announced September 2018.

Comments: 8 pages, 7 figures, 2 tables

Journal ref: J. Phys. Soc. Jpn. 87, 073708 (2018)

Many-body Chern number without integration

Authors: Koji Kudo, Haruki Watanabe, Toshikaze Kariyado, Yasuhiro Hatsugai

Abstract: The celebrated work of Niu, Thouless, and Wu demonstrated the quantization of Hall conductance in the presence of many-body interactions by revealing the many-body counterpart of the Chern number. The generalized Chern number is formulated in terms of the twisted angles of the boundary condition, instead of the single particle momentum, and involves an integration over all possible twisted angles.… ▽ More The celebrated work of Niu, Thouless, and Wu demonstrated the quantization of Hall conductance in the presence of many-body interactions by revealing the many-body counterpart of the Chern number. The generalized Chern number is formulated in terms of the twisted angles of the boundary condition, instead of the single particle momentum, and involves an integration over all possible twisted angles. However, this formulation is physically unnatural, since topological invariants directly related to observables should be defined for each Hamiltonian under a fixed boundary condition. In this work, we show via numerical calculations that the integration is indeed unnecessary - the integrand itself is effectively quantized and the error decays exponentially with the system size. This implies that the numerical cost in computing the many-body Chern number could, in principle, be significantly reduced as it suffices to compute the Berry connection for a single value of the twisted boundary condition if the system size is sufficiently large. △ Less

Submitted 10 April, 2019; v1 submitted 30 August, 2018; originally announced August 2018.

Journal ref: Phys. Rev. Lett. 122, 146601 (2019)

Constrained quantum annealing of graph coloring

Authors: Kazue Kudo

Abstract: We investigate a quantum annealing approach based on real-time quantum dynamics for graph coloring. In this approach, a driving Hamiltonian is chosen so that constraints are naturally satisfied without penalty terms, and the dimension of the Hilbert space is considerably reduced. The total Hamiltonian, which consists of driving and problem Hamiltonians, resembles a disordered quantum spin chain. T… ▽ More We investigate a quantum annealing approach based on real-time quantum dynamics for graph coloring. In this approach, a driving Hamiltonian is chosen so that constraints are naturally satisfied without penalty terms, and the dimension of the Hilbert space is considerably reduced. The total Hamiltonian, which consists of driving and problem Hamiltonians, resembles a disordered quantum spin chain. The ground state of the problem Hamiltonian for graph coloring is degenerate. This degeneracy is advantageous and is characteristic of this approach. Real-time quantum simulations in a small system demonstrate interesting results and provide some insight into quantum annealing. △ Less

Submitted 17 July, 2018; v1 submitted 14 June, 2018; originally announced June 2018.

Comments: 6 pages, 8 figures

Journal ref: Phys. Rev. A 98, 022301 (2018)

Commensurate vs incommensurate charge ordering near the superconducting dome in Ir$_{1-x}$Pt$_x$Te$_2$ revealed by resonant x-ray scattering

Authors: K. Takubo, K. Yamamoto, Y. Hirata, H. Wadati, T. Mizokawa, R. Sutarto, F. He, K. Ishii, Y. Yamasaki, H. Nakao, Y. Murakami, G. Matsuo, H. Ishii, M. Kobayashi, K. Kudo, M. Nohara

Abstract: The electronic-structural modulations of Ir$_{1-x}$Pt$_x$Te$_2$ (0 $\leqq x\leqq$ 0.12) have been examined by resonant elastic x-ray scattering (REXS) and resonant inelastic x-ray scattering (RIXS) techniques at both the Ir and Te edges. Charge-density-wave-like superstructure with wave vectors of $\mathbf{Q}$=(1/5 0 $-$1/5), (1/8 0 $-$1/8), and (1/6 0 $-$1/6) are observed on the same sample of Ir… ▽ More The electronic-structural modulations of Ir$_{1-x}$Pt$_x$Te$_2$ (0 $\leqq x\leqq$ 0.12) have been examined by resonant elastic x-ray scattering (REXS) and resonant inelastic x-ray scattering (RIXS) techniques at both the Ir and Te edges. Charge-density-wave-like superstructure with wave vectors of $\mathbf{Q}$=(1/5 0 $-$1/5), (1/8 0 $-$1/8), and (1/6 0 $-$1/6) are observed on the same sample of IrTe$_2$ at the lowest temperature, the patterns of which are controlled by the cooling speeds. In contrast, superstructures around $\mathbf{Q}$=(1/5 0 $-$1/5) are observed for doped samples (0.02 $\leqq x\leqq$ 0.05). The superstructure reflections persist to higher Pt substitution than previously assumed, demonstrating that a charge density wave (CDW) can coexists with superconductivity. The analysis of the energy-dependent REXS and RIXS lineshape reveals the importance of the Te 5$p$ state rather than the Ir 5$d$ states in the formation of the spatial modulation of these systems. The phase diagram re-examined in this work suggests that the CDW incommensurability may correlate the emergence of superconducting states as-like Cu$_x$TiSe$_2$ and Li$_x$TaS$_2$. △ Less

Submitted 14 May, 2018; originally announced May 2018.

Comments: 10 pages ,9 figures

Fractional Quantum Hall Effect in n=0 Landau Band of Graphene with Chern Number Matrix

Authors: Koji Kudo, Yasuhiro Hatsugai

Abstract: Fully taking into account of the honeycomb lattice structure, fractional quantum Hall states of graphene are considered by a pseudopotential projected into the n = 0 Landau band. By using a chirality as an internal degree of freedom, the Chern number matrices are defined and evaluated numerically. Quantum phase transition induced by changing a range of the interaction is demonstrated which is asso… ▽ More Fully taking into account of the honeycomb lattice structure, fractional quantum Hall states of graphene are considered by a pseudopotential projected into the n = 0 Landau band. By using a chirality as an internal degree of freedom, the Chern number matrices are defined and evaluated numerically. Quantum phase transition induced by changing a range of the interaction is demonstrated which is associated with chirality ferromagnetism. The chirality-unpolarized ground state is consistent with the Halperin 331 state of the bilayer quantum Hall system. △ Less

Submitted 15 May, 2018; v1 submitted 27 March, 2018; originally announced March 2018.

Comments: 4 pages, 2 figures

Journal ref: J. Phys. Soc. Jpn. 87, 063701 (2018)

Finite-size scaling with respect to interaction and disorder strength at the many-body localization transition

Authors: Kazue Kudo, Tetsuo Deguchi

Abstract: We present a finite-size scaling for both interaction and disorder strengths in the critical regime of the many-body localization (MBL) transition for a spin-1/2 XXZ spin chain with a random field by studying level statistics. We show how the dynamical transition from the thermal to MBL phase depends on interaction together with disorder by evaluating the ratio of adjacent level spacings, and thus… ▽ More We present a finite-size scaling for both interaction and disorder strengths in the critical regime of the many-body localization (MBL) transition for a spin-1/2 XXZ spin chain with a random field by studying level statistics. We show how the dynamical transition from the thermal to MBL phase depends on interaction together with disorder by evaluating the ratio of adjacent level spacings, and thus, extend previous studies in which interaction coupling is fixed. We introduce an extra critical exponent in order to describe the nontrivial interaction dependence of the MBL transition. It is characterized by the ratio of the disorder strength to the power of the interaction coupling with respect to the extra critical exponent and not by the simple ratio between them. △ Less

Submitted 6 June, 2018; v1 submitted 17 March, 2018; originally announced March 2018.

Comments: 5 pages, 3 figures

Journal ref: Phys. Rev. B 97, 220201 (2018)

Direct Observation of the Quantum Phase Transition of SrCu$_{2}$(BO$_{3}$)$_{2}$ by High-Pressure and Terahertz Electron Spin Resonance

Authors: Takahiro Sakurai, Yuki Hirao, Keigo Hijii, Susumu Okubo, Hitoshi Ohta, Yoshiya Uwatoko, Kazutaka Kudo, Yoji Koike

Abstract: High-pressure and high-field electron spin resonance (ESR) measurements have been performed on a single crystal of the orthogonal-dimer spin system SrCu$_{2}$(BO$_{3}$)$_{2}$. With frequencies below 1 THz, ESR signals associated with transitions from the singlet ground state to the one-triplet excited states and the two-triplet bound state were observed at pressures up to 2.1 GPa. We obtained dire… ▽ More High-pressure and high-field electron spin resonance (ESR) measurements have been performed on a single crystal of the orthogonal-dimer spin system SrCu$_{2}$(BO$_{3}$)$_{2}$. With frequencies below 1 THz, ESR signals associated with transitions from the singlet ground state to the one-triplet excited states and the two-triplet bound state were observed at pressures up to 2.1 GPa. We obtained directly the pressure dependence of the gap energies, finding a clear first-order phase transition at $P_{c}=1.85\pm0.05$ GPa. By comparing this pressure dependence with the calculated excitation energies obtained from an exact diagonalization, we determined the precise pressure dependence for inter- ($J'$) and intra-dimer ($J$) exchange interactions considering the Dzyaloshinski-Moriya interaction. Thus this system undergoes a first-order quantum phase transition from the dimer singlet phase to a plaquette singlet phase above the ratio $(J'/J)_{c}=0.660\pm0.003$. △ Less

Submitted 24 January, 2018; originally announced January 2018.

Journal ref: J. Phys. Soc. Jpn. 87 (2018) 033701/1-4