Showing 1–50 of 215 results for author: Feng, D

Unconventional Pressure Evolution of Spin-Density-Wave State in La$_{3}$Ni$_{2}$O$_{7}$

Authors: Xiaoxiang Zhou, Shiyu Xie, Liangxin Qiao, Hengyuan Zhang, Jun Shu, Rui Liu, Mengwu Huo, Deyuan Hu, Hengjie Liu, Chuansheng Hu, Yilin Wang, Ge He, Zeming Qi, Meng Wang, Dong-Lai Feng, Zengyi Du

Abstract: The discovery of pressure-induced high temperature superconductivity in the bilayer nickelate La$_{3}$Ni$_{2}$O$_{7}$ has raised the question of how its spin-density-wave (SDW) state evolves toward the superconducting regime. Here, we report a systematic electronic Raman study of La$_{3}$Ni$_{2}$O$_{7}$ single crystals under hydrostatic pressures up to 16.51 GPa. Both the SDW gap energy and the tr… ▽ More The discovery of pressure-induced high temperature superconductivity in the bilayer nickelate La$_{3}$Ni$_{2}$O$_{7}$ has raised the question of how its spin-density-wave (SDW) state evolves toward the superconducting regime. Here, we report a systematic electronic Raman study of La$_{3}$Ni$_{2}$O$_{7}$ single crystals under hydrostatic pressures up to 16.51 GPa. Both the SDW gap energy and the transition temperature $T_{\mathrm{SDW}}$ show an overall increase with pressure, while the dimensionless coupling ratio 2$Δ_{\text{SDW}}/(k_{\text{B}}T_{\text{SDW}})$ remains constant around $\sim7.5$, indicating a robust strong-coupling character of SDW state. At the same time, the Raman SDW peak broadens as pressure is applied, indicating a gradual weakening of long-range SDW order. These results reveal an unusual pressure evolution in which the SDW energy scale is enhanced while the SDW state becomes progressively less coherent, providing spectroscopic constraints on the magnetic correlations relevant to superconductivity in bilayer nickelates. △ Less

Submitted 18 August, 2026; originally announced August 2026.

Dimensional crossover and local strain induced deflection of the spin spiral state in multiferroic NiI2

Authors: Tianxing Jiang, Lianchuang Li, Haiyan Zhu, Hongyu Wang, Junchao Tian, Wenzhao Wang, Weiyi Pan, Haitao Wang, Changlin Zheng, Hongjun Xiang, Changsong Xu, Donglai Feng, Tong Zhang

Abstract: Low-dimensional multiferroics hold great promise for integrated magnetoelectric devices. Spin spiral state has recently been shown to induce ferroelectricity in single-layer van der Waals (vdW) material NiI2. However, how this state evolves and can be tuned towards the two-dimensional limit remain unclear. Here, we combine spin-polarized scanning tunneling microscopy, layer-by-layer film growth, a… ▽ More Low-dimensional multiferroics hold great promise for integrated magnetoelectric devices. Spin spiral state has recently been shown to induce ferroelectricity in single-layer van der Waals (vdW) material NiI2. However, how this state evolves and can be tuned towards the two-dimensional limit remain unclear. Here, we combine spin-polarized scanning tunneling microscopy, layer-by-layer film growth, and multi-scale theoretical modeling to investigate the spin spirals in NiI2 thin films. As the film thickness increases from 1 to 7 monolayers, we observed a continuous increase of spin-spiral wavelength and a rotation of wavevector from near [110] to [1-10] direction, which evidences a dimensional crossover primarily driven by enhanced interlayer exchange energy. Moreover, we find that the film wrinkles can cause deflection of the spin spiral wavevector, which is caused by local curvature induced modification of exchange interactions. Our findings establish thickness and local strain as two tuning methods for engineering non-collinear helical magnetism and accompanied electric polarization in vdW multiferroics. △ Less

Submitted 12 August, 2026; originally announced August 2026.

Journal ref: Science Bulletin 2026

Marginal-Fermi-Liquid-like Behavior without Pseudogap in Infinite-Layer Nickelates

Authors: Yu Fan, Zhitong An, Xiang Ding, Xingtian Sun, Yutong Chen, Zhihui Chen, Shenglin Tang, Chihao Li, Jiahao Ye, Timur Kim, Haichao Xu, Rui Peng, Donglai Feng

Abstract: Pseudogap formation, strange-metal behavior and unconventional superconductivity are closely intertwined in hole-doped cuprates, yet their relationship remains unresolved. Infinite-layer nickelates offer a distinct 3d9-derived platform to address this question by combining a cuprate-like Ni dx2-y2 Fermi surface with multiband electronic degrees of freedom. Here we use angle-resolved photoemission… ▽ More Pseudogap formation, strange-metal behavior and unconventional superconductivity are closely intertwined in hole-doped cuprates, yet their relationship remains unresolved. Infinite-layer nickelates offer a distinct 3d9-derived platform to address this question by combining a cuprate-like Ni dx2-y2 Fermi surface with multiband electronic degrees of freedom. Here we use angle-resolved photoemission spectroscopy to resolve the low-energy spectral function of superconducting La0.8Ca0.2NiO2 and parent LaNiO2 thin films. In La0.8Ca0.2NiO2, the electronic self-energy Im Sigma(omega) is approximately linear in energy and its slope increases from (pi/2, pi/2) to (pi, 0), revealing momentum-dependent marginal-Fermi-liquid-like scattering. Both films show a progressive suppression of low-energy spectral weight from the diagonal direction toward (pi, 0), with stronger suppression in parent LaNiO2. However, finite Fermi-level spectral weight persists around the entire Fermi surface, with no leading-edge shift or back-bending indicative of pseudogap formation in either the electron pocket or the cuprate-like hole band. Our results demonstrate that momentum-selective correlations and marginal-Fermi-liquid-like scattering can occur without a detectable cuprate-like pseudogap, providing a benchmark for identifying the essential normal-state electronic ingredients of high-temperature superconductivity. △ Less

Submitted 18 July, 2026; originally announced July 2026.

Comments: 16 pages, 5 figures

A Disconnected Superconducting Regime at the Parent Limit of Infinite-Layer Nickelates

Authors: Chihao Li, Yutong Chen, Yaolong Bian, Yihao Zhang, Jiahao Ye, Zhitong An, Xingtian Sun, Yu Fan, Zhihui Chen, Zhanze Wang, Jinglei Zhang, Haichao Xu, Rui Peng, Donglai Feng

Abstract: Infinite-layer nickelates have been widely viewed as cuprate analogs in which superconductivity emerges and forms a superconducting dome centered around 10-20% cation substitution. Here we show that pristine and stoichiometric PrNiO2, without cation substitution, exhibits intrinsic superconductivity characterized by zero resistance and diamagnetism in uncapped films. Through heterostructure engine… ▽ More Infinite-layer nickelates have been widely viewed as cuprate analogs in which superconductivity emerges and forms a superconducting dome centered around 10-20% cation substitution. Here we show that pristine and stoichiometric PrNiO2, without cation substitution, exhibits intrinsic superconductivity characterized by zero resistance and diamagnetism in uncapped films. Through heterostructure engineering, we further exclude an interfacial origin of the superconductivity. Remarkably, zero-resistance superconductivity is consistently observed in trivalent-substituted PrNiO2, whereas it is rapidly suppressed by dilute divalent substitution. Combined with angle-resolved photoemission studies, these results indicate that such a new superconducting regime is confined to within 3% additional hole doping from pristine PrNiO2. Furthermore, this phase is separated from the previously established superconducting dome around ~ 20% divalent doping by a non-superconducting region in the phase diagram, and is further distinguished by a remarkably stronger upper-critical-field anisotropy. These findings establish a unique separated superconducting regime, suggesting that infinite-layer nickelates are not merely cuprate analogs but host distinct superconducting physics. △ Less

Submitted 18 July, 2026; originally announced July 2026.

Comments: 7 pages, 4 figures

MSC Class: 82D55

Direct observation of interfacial exchange coupling in a magnetic tunnel junction through spin-polarized quasiparticle interference

Authors: Xu Wang, Chenxi Wang, Ying Yang, Yining Hu, Qingle Zhang, Chen Chen, Donglai Feng, Tong Zhang

Abstract: Interfacial exchange coupling plays a critical role in enabling novel phenomena in magnetic heterostructures, such as spin triplet superconductivity, quantum anomalous Hall effect (QAHE), and advanced spintronic functionalities. While microscopic characterization of this coupling is essential for elucidating the underlying mechanism, it remains technically challenging. Here, using spin-polarized s… ▽ More Interfacial exchange coupling plays a critical role in enabling novel phenomena in magnetic heterostructures, such as spin triplet superconductivity, quantum anomalous Hall effect (QAHE), and advanced spintronic functionalities. While microscopic characterization of this coupling is essential for elucidating the underlying mechanism, it remains technically challenging. Here, using spin-polarized scanning tunneling microscopy (SP-STM) and quasiparticle interference, we directly observed interfacial exchange coupling in a magnetic tunnel junction formed by an Fe coated tip and a Cr(001) surface. We found the ferromagnetic tip induces significant energy shift (up to 10 meV) in the spin-polarized surface state of Cr(001). This shift is highly sensitive to the tip-surface distance and the spin-alignment between Fe tip and Cr surface, which can be switched by external magnetic field. Our results demonstrate that extended 2D surface states can mediate strong exchange coupling across a heterojunction, enabling local control of interfacial exchange interaction induced phenomena. △ Less

Submitted 26 June, 2026; originally announced June 2026.

Journal ref: Nano Lett. 2026, 26, 22, 7364

A first-principles approach for predicting infrared optical properties of solids

Authors: Sreerag Sundaram, Ziqi Guo, Dudong Feng, Karthik Sasihithlu, Xiulin Ruan

Abstract: We present a simplified formalism for predicting infrared optical constants from first-principles calculations. Addressing limitations of the widely used four-parameter semi-quantum Lorentz model, the proposed approach bridges the gap between the harmonic three-parameter model and full self-energy-based methods. By incorporating essential anharmonic effects including four-phonon scattering and pho… ▽ More We present a simplified formalism for predicting infrared optical constants from first-principles calculations. Addressing limitations of the widely used four-parameter semi-quantum Lorentz model, the proposed approach bridges the gap between the harmonic three-parameter model and full self-energy-based methods. By incorporating essential anharmonic effects including four-phonon scattering and phonon renormalisation, the model provides an efficient and accurate alternative while maintaining low computational cost. The frequency-dependent refractive indices of MgO and rutile TiO$_2$ are computed and compared with experimental data, demonstrating good quantitative agreement. The framework offers a practical approach for predicting optical properties of materials across a wide range of materials. △ Less

Submitted 11 June, 2026; originally announced June 2026.

Electronic Origin of Ferromagnetic Excitations in the Candidate Spin-Triplet Superconductor CeSb2

Authors: Xiaoxiao Wang, Xiaoyang Chen, Suppanut Sangphet, Yifei Fang, Yilin Wang, Chihao Li, Minyinan Lei, Nan Guo, Yuanhe Song, Rui Peng, Haichao Xu, Donglai Feng

Abstract: The origin of quasi-one-dimensional (q1D) ferromagnetic (FM) excitations in the candidate spin-triplet superconductor CeSb$_2$ has remained unclear. Here we report an electronic mechanism for emergent q1D magnetism in the quasi-two-dimensional lattice of CeSb$_2$, revealed by angle-resolved photoemission spectroscopy (ARPES). High-resolution ARPES resolves no spin-density-wave gap on the dispersiv… ▽ More The origin of quasi-one-dimensional (q1D) ferromagnetic (FM) excitations in the candidate spin-triplet superconductor CeSb$_2$ has remained unclear. Here we report an electronic mechanism for emergent q1D magnetism in the quasi-two-dimensional lattice of CeSb$_2$, revealed by angle-resolved photoemission spectroscopy (ARPES). High-resolution ARPES resolves no spin-density-wave gap on the dispersive Fermi pockets, disfavoring a nesting-driven mechanism for the q1D FM excitations. Instead, resonant ARPES reveals a pronounced selective enhancement of Ce 4$f$ spectral weight on the $C_2$-distributed Fermi pockets aligned with the Ce ladder. This observation signifies band-selective Kondo coupling that generates strongly anisotropic magnetic exchange interactions, which can naturally account for both the q1D ferromagnetic excitations and the competing magnetic orders. Our results identify a band-selective Kondo coupling mechanism for emergent low-dimensional magnetism in correlated $f$-electron systems. △ Less

Submitted 28 May, 2026; originally announced May 2026.

$3d_{z^2}$ orbital delocalization and magnetic collapse in superconducting (La,Pr)$_3$Ni$_2$O$_{7-δ}$ films

Authors: Xiaoyang Chen, Wenliang Zhang, Fei Peng, Ting Cui, Guangdi Zhou, Zezhong Li, Jaewon Choi, Lizhi Xu, Yiu-Fung Chiu, Stefano Agrestini, Sahil Tippireddy, Haoliang Huang, Heng Wang, Xianfeng Wu, Peng Li, Jin-Feng Jia, Mirian Garcia-Fernandez, Yi Lu, Er-Jia Guo, Qi-Kun Xue, Zhuoyu Chen, Donglai Feng, Ke-Jin Zhou

Abstract: The recent discovery of Ruddlesden--Popper (RP) nickelate thin-film superconductors has opened a new frontier in unconventional superconductivity. Its realization requires both compressive epitaxial strain and highly oxidative growth conditions, yet the microscopic pathway from the parent phase to the superconducting phase remains elusive. Here, X-ray absorption spectra and resonant inelastic X-ra… ▽ More The recent discovery of Ruddlesden--Popper (RP) nickelate thin-film superconductors has opened a new frontier in unconventional superconductivity. Its realization requires both compressive epitaxial strain and highly oxidative growth conditions, yet the microscopic pathway from the parent phase to the superconducting phase remains elusive. Here, X-ray absorption spectra and resonant inelastic X-ray scattering are employed to track this evolution by independently tuning strain and oxygen content in (La,Pr)$_3$Ni$_2$O$_{7-δ}$ thin films. We uncover a remarkable two-step narrative. First, signatures of delocalization emerge in the same way upon two independent tunings: Spectral weight transfers from a ''Upper Hubbard''-like peak to the hole-like peak associated with O $2p_z$ state, and in parallel, the initially localized Ni $3d_{z^2}$ orbital becomes more itinerant followed by the broadening and weakening of $dd$ orbital excitations. Second, as itinerancy increases, long-range spin-density-wave (SDW) order is suppressed in both intensity and correlation length, indicating direct competition with superconductivity. Yet, short-range magnons persist: they become damped but their bandwidth stays unchanged. Our results paint a coherent picture that both strain and oxygenation drive the RP bilayer nickelates towards the superconducting instability, where the O $2p_z$ and Ni $3d_{z^2}$ orbitals become delocalized. Concomitantly, the long-range magnetic order loses coherence and gets suppressed. These findings establish an orbital-selective route to RP nickelate superconductivity, in which the delocalization of the $2p_z$ and $3d_{z^2}$ orbitals and the robust short-range magnons upon the melting of SDW order are prerequisites, providing strong constraints for theory and the roadmap for designing nickelate superconductors. △ Less

Submitted 24 April, 2026; v1 submitted 23 April, 2026; originally announced April 2026.

Comments: 9 pages, 4 figures

Microscopic evidence of spin-driven multiferroicity and topological spin textures in monolayer NiI2

Authors: Haitao Wang, Tianxing Jiang, Weiyi Pan, Xu Wang, Hongyu Wang, Junchao Tian, Lianchuang Li, Dongming Zhao, Qingle Zhang, Chenxi Wang, Ying Yang, Hongjun Xiang, Changsong Xu, Donglai Feng, Tong Zhang

Abstract: In type II multiferroics, noncollinear spin textures are expected to induce electric polarization directly, leading to strong magnetoelectric coupling. Realizing such spin driven multiferroicity in two-dimensional systems, and elucidating the interplay between local spins and electric polarization, are of both fundamental and technological importance. Here, using vectorial spin polarized scanning… ▽ More In type II multiferroics, noncollinear spin textures are expected to induce electric polarization directly, leading to strong magnetoelectric coupling. Realizing such spin driven multiferroicity in two-dimensional systems, and elucidating the interplay between local spins and electric polarization, are of both fundamental and technological importance. Here, using vectorial spin polarized scanning tunneling microscopy, we investigated the spin-driven multiferroicity in monolayer NiI2 at atomic scale. We identify a canted spin-spiral state with fully determined spin rotation plane, accompanied by a 2Q charge modulation. At spin spiral domain walls, we discover topological spin textures that composed of meron/antimeron pairs. These textures are associated with distinct charge pattern and notable band shifts, indicating local bound charges induced by variations of ferroelectricity at domain wall. Our observations are well captured by a realistic spin model incorporating Kitaev interactions and generalized spin-current model of type II multiferroicity. The findings provide microscopic evidence of spin-driven multiferroicity in an extreme 2D system and establish a platform for low-dissipation, electric-field control of topological spin textures. △ Less

Submitted 8 April, 2026; originally announced April 2026.

Comments: 26 pages, 20 figures, supplementary materials included

Journal ref: Phys. Rev. Lett. 136, 026402 (2026)

Dissecting superconductivity in the Ruddlesden-Popper nickelates: The role of electron correlation and interlayer magnetic exchange

Authors: Xiaoyang Chen, Zezhong Li, Mei Xie, Deyuan Hu, Yiu-Fung Chiu, Stefano Agrestini, Wenliang Zhang, Yi Lu, Meng Wang, Mirian Garcia-Fernandez, Donglai Feng, Ke-Jin Zhou

Abstract: The discovery of superconductivity in the Ruddlesden-Popper (RP) nickelates has opened a new chapter in the search for high superconducting transition temperatures ($T_\mathrm{c}$) materials. A central and puzzling feature of this family is the wide variation in $T_\mathrm{c}$ despite their common NiO$_2$ building blocks, as highlighted by the recent observation of superconductivity at $\sim$ 30 K… ▽ More The discovery of superconductivity in the Ruddlesden-Popper (RP) nickelates has opened a new chapter in the search for high superconducting transition temperatures ($T_\mathrm{c}$) materials. A central and puzzling feature of this family is the wide variation in $T_\mathrm{c}$ despite their common NiO$_2$ building blocks, as highlighted by the recent observation of superconductivity at $\sim$ 30 K in trilayer $\mathrm{La_4Ni_3O_{10}}$, significantly lower than 80 K reported in bilayer $\mathrm{La_3Ni_2O_7}$. Understanding the factors that control $T_\mathrm{c}$ in this family is therefore of paramount importance. Here, we use resonant inelastic x-ray scattering (RIXS) to investigate the electronic and magnetic excitations of $\mathrm{La_4Ni_3O_{10}}$ in direct comparison with its bilayer counterpart. Our results reveal a markedly different landscape. $\mathrm{La_4Ni_3O_{10}}$ exhibits a more itinerant character, evidenced by broader Ni $dd$ orbital excitations and a strong Ni 3$d$ fluorescence continuum, suggesting weaker electronic correlations than in the bilayer. Despite this, well-defined collective spin excitations persist, including dispersive acoustic and optical magnon branches alongside an incommensurate spin density wave. Using linear spin wave theory, we extract the interlayer superexchange interaction ($J_z$) to be $\sim$ 22 meV, much smaller than that in $\mathrm{La_3Ni_2O_7}$. The weaker correlation and reduced interlayer exchange together provide a consistent explanation for the substantially lower $T_\mathrm{c}$ in the trilayer compound. Our findings establish interlayer magnetic coupling and electronic correlation as key parameters governing superconductivity in layered nickelates and offer critical constraints for understanding the pairing mechanism in this emerging family. △ Less

Submitted 2 April, 2026; originally announced April 2026.

Comments: 11 pages, 4 figures

Distinguishing impurity-induced bound states from Majorana-like zero-energy peaks in strained CsCa2Fe4As4F2 by scanning tunneling microscopy

Authors: Mingzhe Li, Jiashuo Gong, Huaxun Li, Jiakang Zhang, Yuanji Li, Ruotong Yin, Shiyuan Wang, Guanghan Cao, Dong-Lai Feng, Ya-Jun Yan

Abstract: Iron-based superconductors offer a versatile platform for exploring topological superconductivity and Majorana zero modes (MZMs), with experimental confirmations in Fe(Te,Se), (Li,Fe)OHFeSe and CaKFe4As4 at ambient pressure, as well as in LiFeAs under local strain. The related properties in other iron-based superconductors still need to be explored, especially under the application of local strain… ▽ More Iron-based superconductors offer a versatile platform for exploring topological superconductivity and Majorana zero modes (MZMs), with experimental confirmations in Fe(Te,Se), (Li,Fe)OHFeSe and CaKFe4As4 at ambient pressure, as well as in LiFeAs under local strain. The related properties in other iron-based superconductors still need to be explored, especially under the application of local strain. In this study, we conduct scanning tunneling microscopy/spectroscopy measurements on CsCa2Fe4As4F2 crystals under unidirectional local strain. A fully developed superconducting gap with multiple pairs of coherence peaks are observed, and the gap sizes can be significantly modulated by local strain. Spectroscopic measurements on various types of defects including the nonmagnetic Cs-site vacancies consistently reveal pair-breaking effects. These phenomena support a fully gapped multiband superconductivity scenario with sign-changing. Notably, a sharp zero-energy conductance peak (ZECP) is universally observed on a particular type of defects by using a metallic tip, resembling the MZMs observed at interstitial Fe atoms in Fe(Te,Se) [Nat. Phys. 11, 543 (2015)]. However, by using a superconducting tip to enhance energy resolution as well as by studying the ZECP evolution as functions of magnetic field and tunneling transmissivity, we demonstrate that the ZECP originates from nearly degenerate Yu-Shiba-Rusinov states rather than MZMs. Our study not only provides more insights into the superconducting pairing symmetry of CsCa2Fe4As4F2, but also establishes systematic experimental methods for identifying weak impurity state signals and discerning the physical origins of ZECPs. △ Less

Submitted 28 March, 2026; originally announced March 2026.

Comments: 19 pages, 8 figures

Scanning tunneling microscopy study of helimagnetic monolayer CrBr2 on s-wave superconductor NbSe2: a topologically trivial system due to weak interfacial coupling

Authors: Yuanji Li, Ruotong Yin, Mingzhe Li, Shiyuan Wang, Jiashuo Gong, Ziyuan Chen, Jiakang Zhang, Dong-Lai Feng, Ya-Jun Yan

Abstract: Hybrid magnet-superconductor heterostructures attract significant interest for their potential to host unconventional superconductivity, topological superconductivity, and Majorana physics. Transition metal dihalides (MX2, M = transition metal, X = Cl, Br, I) are compelling magnetic candidates due to their novel magnetic structures and possible ferroelectricity. Here, we employ low-temperature sca… ▽ More Hybrid magnet-superconductor heterostructures attract significant interest for their potential to host unconventional superconductivity, topological superconductivity, and Majorana physics. Transition metal dihalides (MX2, M = transition metal, X = Cl, Br, I) are compelling magnetic candidates due to their novel magnetic structures and possible ferroelectricity. Here, we employ low-temperature scanning tunneling microscopy/spectroscopy to investigate the interfaces fabricated by growing helimagnet candidate CrBr2 on s-wave superconductor NbSe2. Our results reveal that the monolayer CrBr2 is insulating, the measured low-energy electronic states on it derive entirely from the NbSe2 substrate. The superconducting properties of CrBr2/NbSe2 are nearly identical to the bare NbSe2, manifested by the superconducting gap spectra and their temperature and magnetic field dependence, as well as the spatial distribution and bound states of magnetic vortices. Furthermore, in-gap excitations appear only at the dirty edges of CrBr2 islands and are absent from clean edges, suggesting the lack of intrinsic edge states. Taken together, these findings establish the topologically trivial nature of the helimagnetic insulator/s-wave superconductor system CrBr2/NbSe2, attributable to the absence of interfacial superconducting proximity and weak magnetic coupling. △ Less

Submitted 28 March, 2026; originally announced March 2026.

Comments: 12 pages, 4 figures

Journal ref: Phys. Rev. B 113, 094519 (2026)

Magnetic-field-tunable commensurate multi-q charge orders on UTe2 (011) surface

Authors: Yuanji Li, Ruotong Yin, Jiashuo Gong, Dengpeng Yuan, Yuguang Wang, Shiyuan Wang, Mingzhe Li, Jiakang Zhang, Ziwei Xue, Zengyi Du, Shiyong Tan, Dong-Lai Feng, Ya-Jun Yan

Abstract: The heavy-fermion superconductor UTe2 has attracted intense interest as a candidate for spin-triplet pairing. Recent scanning tunneling microscopy (STM) studies have reported complex charge orders (COs) on its (011) surface, but their origin and relationship with superconductivity remain controversial. Here, by performing temperature-, magnetic field-, and sample-dependent STM measurements, we ide… ▽ More The heavy-fermion superconductor UTe2 has attracted intense interest as a candidate for spin-triplet pairing. Recent scanning tunneling microscopy (STM) studies have reported complex charge orders (COs) on its (011) surface, but their origin and relationship with superconductivity remain controversial. Here, by performing temperature-, magnetic field-, and sample-dependent STM measurements, we identify multiple new CO wave vectors beyond those previously reported. All these CO wave vectors are strictly locked to integer multiples of 1/14 and 1/4 of the reciprocal lattice vectors of the UTe2 (011) surface, and multiple of them coexist in real space, collectively revealing a family of field-tunable, commensurate multi-q COs. These COs exist within an energy range much larger than the superconducting energy scale, their emergence suppresses the density of states near EF, yet show negligible coupling to bulk superconductivity and magnetic vortices. Our findings strongly disfavor the Fermi surface nesting or primary pair-density-wave pictures, but are consistent with a surface parent spin order. △ Less

Submitted 28 March, 2026; originally announced March 2026.

Comments: 25 pages, 15 figures

Differentiable Maximum Likelihood Noise Estimation for Quantum Error Correction

Authors: Hanyan Cao, Dongyang Feng, Cheng Ye, Feng Pan

Abstract: Accurate noise estimation is essential for fault-tolerant quantum computing, as decoding performance depends critically on the fidelity of the circuit-level noise parameters. In this work, we introduce a differentiable Maximum Likelihood Estimation (dMLE) framework that enables exact, efficient, and fully differentiable computation of syndrome log-likelihoods, allowing circuit-level noise paramete… ▽ More Accurate noise estimation is essential for fault-tolerant quantum computing, as decoding performance depends critically on the fidelity of the circuit-level noise parameters. In this work, we introduce a differentiable Maximum Likelihood Estimation (dMLE) framework that enables exact, efficient, and fully differentiable computation of syndrome log-likelihoods, allowing circuit-level noise parameters to be optimized directly via gradient descent. Leveraging the exact Planar solver for repetition codes and a novel, simplified Tensor Network (TN) architecture combined with optimized contraction path finding for surface codes, our method achieves tractable and fully differentiable likelihood evaluation even for distance 5 surface codes with up to 25 rounds. Our method recovers the underlying error probabilities with near-exact precision in simulations and reduces logical error rates by up to 30.6(3)% for repetition codes and 8.1(2)% for surface codes on experimental data from Google's processor compared to previous state-of-the-art methods: correlation analysis and Reinforcement Learning (RL) methods. Our approach yields provably optimal, decoder-independent error priors by directly maximizing the syndrome likelihood, offering a powerful noise estimation and control tool for unlocking the full potential of current and future error-corrected quantum processors. △ Less

Submitted 23 February, 2026; originally announced February 2026.

Anisotropic Electronic Correlations in the Spin Density Wave State of La$_3$Ni$_2$O$_7$

Authors: Ge He, Jun Shen, Shiyu Xie, Haotian Zhang, Mengwu Huo, Jun Shu, Deyuan Hu, Xiaoxiang Zhou, Yanmin Zhang, Lei Qin, Liangxin Qiao, Hengjie Liu, Chuansheng Hu, Xijie Dong, Dengjing Wang, Jun Liu, Wei Hu, Jie Yuan, Yajun Yan, Zeming Qi, Kui Jin, Zengyi Du, Meng Wang, Donglai Feng

Abstract: The bilayer nickelate superconductor La$_3$Ni$_2$O$_7$ undergoes a density wave transition near 150 K that has attracted intensive scrutiny, yet its microscopic origin remains elusive. Here we report polarization-resolved electronic Raman scattering measurements on high-quality single crystals of La$_3$Ni$_2$O$_7$. Below 150\,K, we observe a pronounced, symmetry-dependent redistribution of spectra… ▽ More The bilayer nickelate superconductor La$_3$Ni$_2$O$_7$ undergoes a density wave transition near 150 K that has attracted intensive scrutiny, yet its microscopic origin remains elusive. Here we report polarization-resolved electronic Raman scattering measurements on high-quality single crystals of La$_3$Ni$_2$O$_7$. Below 150\,K, we observe a pronounced, symmetry-dependent redistribution of spectral weight in B$_{1g}$ and B$_{2g}$ channels, consistent with the formation of spin-density-wave (SDW) gaps. Quantitative analysis reveals momentum-selective SDW gap amplitudes, with intermediate-to-strong coupling near X/Y points of the Brillouin zone and weaker coupling along the diagonal direction, indicating an unconventional SDW driven by anisotropic electronic correlations. Our results establish the electronic character of the SDW in La$_3$Ni$_2$O$_7$, and provide a microscopic foundation for understanding the emergence of high-temperature superconductivity under pressure in nickelates. △ Less

Submitted 8 February, 2026; originally announced February 2026.

Comments: 10 pages, 4 figures

Contrasting Momentum-Selective Spin-Density-Wave Gaps in Bilayer and Trilayer Nickelates

Authors: Jun Shu, Jun Shen, Xiaoxiang Zhou, Yinghao Zhu, Qingsong Wang, Dengjing Wang, Weihong He, Jie Yuan, Kui Jin, Dawei Shen, Congcong Le, Jun Zhao, Zengyi Du, Ge He, Donglai Feng

Abstract: Resolving where the density-wave gap opens in momentum space is essential for identifying the microscopic origin of the instability in layered nickelates. Using polarization-resolved electronic Raman scattering, we map the momentum selectivity of the spin-density-wave (SDW) gap in trilayer La4Ni3O10. We observe a SDW-induced redistribution of spectral weight on both the $α$ pocket at the Brillouin… ▽ More Resolving where the density-wave gap opens in momentum space is essential for identifying the microscopic origin of the instability in layered nickelates. Using polarization-resolved electronic Raman scattering, we map the momentum selectivity of the spin-density-wave (SDW) gap in trilayer La4Ni3O10. We observe a SDW-induced redistribution of spectral weight on both the $α$ pocket at the Brillouin-zone centre and a portion of the $β$ pocket near the zone boundary, characterized by gap energies of approximately 55~meV. In contrast, no comparable spectral weight suppression is observed along the diagonal region of $β$ pockets, implying little or no gap opening. This gap topology contrasts sharply with that in La3Ni2O7, where anisotropic SDW gaps open solely on the $β$ pocket. Our results establish a distinct momentum-space gap topology between bilayer and trilayer nickelates, placing new constraints on the ordering wave vector and the mechanism of the density-wave instability relevant to superconductivity. △ Less

Submitted 2 February, 2026; originally announced February 2026.

Comments: 6 pages, 3 figures

Direct Observation of Unidirectional Density Wave and Band splitting in a Single-Domain Trilayer Nickelate Pr$_4$Ni$_3$O$_{10}$

Authors: Zhicheng Jiang, Enkang Zhang, Yuxin Wang, Zhengtai Liu, Jishan Liu, Runfeng Zhang, Xinnuo Zhang, Wenchuan Jing, Yu Huang, Qi Jiang, Mao Ye, Kun Jiang, Jun Zhao, Dawei Shen, Donglai Feng

Abstract: Unraveling the interplay between density-wave (DW) instabilities and multi-orbital physics is critical for understanding superconductivity in Ruddlesden-Popper nickelates, yet intrinsic electronic features have been persistently obscured by material inhomogeneity and thus the multi-domain averaging effect. Here, we employ micro-focused angle-resolved photoemission spectroscopy ($μ$-ARPES) on singl… ▽ More Unraveling the interplay between density-wave (DW) instabilities and multi-orbital physics is critical for understanding superconductivity in Ruddlesden-Popper nickelates, yet intrinsic electronic features have been persistently obscured by material inhomogeneity and thus the multi-domain averaging effect. Here, we employ micro-focused angle-resolved photoemission spectroscopy ($μ$-ARPES) on single-domain Pr$_4$Ni$_3$O$_{10}$ to disentangle the complex hierarchy of intrinsic and back-folded bands, explicitly identifying the electronic states driving the DW phase transition. We provide decisive spectroscopic evidence that the low-energy reconstruction is governed by inter-orbital nesting between the $α$ and $β$ bands. Specifically, we resolve a orbital-dependent gap of $\sim44$ meV on the $α$ pocket, a value quantitatively consistent with prior measurements, unifying previously conflicting experimental reports regarding the locus and magnitude of the DW gap. Furthermore, we reveal strong orbital-selective mass renormalization in the $d_{z^2}$ states and successfully resolve the long-sought intrinsic trilayer $β$-band splitting, establishing a critical lower bound for the outer-layer hopping. These results define a coherent microscopic fingerprint for the trilayer nickelates, identifying the specific nesting channels and correlation effects that underpin the phase diagram. △ Less

Submitted 2 February, 2026; originally announced February 2026.

Comments: 10 pages,5 figures

MicroEvoEval: A Systematic Evaluation Framework for Image-Based Microstructure Evolution Prediction

Authors: Qinyi Zhang, Duanyu Feng, Ronghui Han, Yangshuai Wang, Hao Wang

Abstract: Simulating microstructure evolution (MicroEvo) is vital for materials design but demands high numerical accuracy, efficiency, and physical fidelity. Although recent studies on deep learning (DL) offer a promising alternative to traditional solvers, the field lacks standardized benchmarks. Existing studies are flawed due to a lack of comparing specialized MicroEvo DL models with state-of-the-art sp… ▽ More Simulating microstructure evolution (MicroEvo) is vital for materials design but demands high numerical accuracy, efficiency, and physical fidelity. Although recent studies on deep learning (DL) offer a promising alternative to traditional solvers, the field lacks standardized benchmarks. Existing studies are flawed due to a lack of comparing specialized MicroEvo DL models with state-of-the-art spatio-temporal architectures, an overemphasis on numerical accuracy over physical fidelity, and a failure to analyze error propagation over time. To address these gaps, we introduce MicroEvoEval, the first comprehensive benchmark for image-based microstructure evolution prediction. We evaluate 14 models, encompassing both domain-specific and general-purpose architectures, across four representative MicroEvo tasks with datasets specifically structured for both short- and long-term assessment. Our multi-faceted evaluation framework goes beyond numerical accuracy and computational cost, incorporating a curated set of structure-preserving metrics to assess physical fidelity. Our extensive evaluations yield several key insights. Notably, we find that modern architectures (e.g., VMamba), not only achieve superior long-term stability and physical fidelity but also operate with an order-of-magnitude greater computational efficiency. The results highlight the necessity of holistic evaluation and identify these modern architectures as a highly promising direction for developing efficient and reliable surrogate models in data-driven materials science. △ Less

Submitted 18 November, 2025; v1 submitted 11 November, 2025; originally announced November 2025.

Comments: Accepted by AAAI 2026

A Review of AI-Driven Approaches for Nanoscale Heat Conduction and Radiation

Authors: Ziqi Guo, Daniel Carne, Krutarth Khot, Dudong Feng, Guang Lin, Xiulin Ruan

Abstract: Heat conduction and radiation are two of the three fundamental modes of heat transfer, playing a critical role in a wide range of scientific and engineering applications ranging from energy systems to materials science. However, traditional physics-based simulation methods for modeling these processes often suffer from prohibitive computational costs. In recent years, the rapid advancements in Art… ▽ More Heat conduction and radiation are two of the three fundamental modes of heat transfer, playing a critical role in a wide range of scientific and engineering applications ranging from energy systems to materials science. However, traditional physics-based simulation methods for modeling these processes often suffer from prohibitive computational costs. In recent years, the rapid advancements in Artificial Intelligence (AI) and machine learning (ML) have demonstrated remarkable potential in the modeling of nanoscale heat conduction and radiation. This review presents a comprehensive overview of recent AI-driven developments in modeling heat conduction and radiation at the nanoscale. We first discuss the ML techniques for predicting phonon properties, including phonon dispersion and scattering rates, which are foundational for determining material thermal properties. Next, we explore the role of machine-learning interatomic potentials (MLIPs) in molecular dynamics simulations and their applications to bulk materials, low-dimensional systems, and interfacial transport. We then review the ML approaches for solving radiative heat transfer problems, focusing on data-driven solutions to Maxwell's equations and the radiative transfer equation. We further discuss the ML-accelerated inverse design of radiative energy devices, including optimization-based and generative model-based methods. Finally, we discuss open challenges and future directions, including data availability, model generalization, uncertainty quantification, and interpretability. Through this survey, we aim to provide a foundational understanding of how AI techniques are reshaping thermal science and guiding future research in nanoscale heat transfer. △ Less

Submitted 29 October, 2025; originally announced October 2025.

Visible Imaging of Incoherent 1200-nm Light via Triplet--Triplet Annihilation Upconversion

Authors: Pournima Narayanan, Rabeeya Hamid, Linda Pucurimay, Ona Segura Lecina, Ben P. Carwithen, Jacob Schopp, Justin S. Edwards, Oluwaseun Noah Adeyeye, Demeng Feng, Diptarka Hait, Todd J. Martinez, Timothy W. Schmidt, Michael P. Nielsen, Murad J. Y. Tayebjee, Mikhail A. Kats, Daniel N. Congreve

Abstract: Upconversion of low-energy photons to higher-energy photons provides an opportunity to surpass traditional limitations in fields such as 3D printing, photovoltaics, and photocatalysis. Triplet--triplet annihilation upconversion (TTA-UC) is particularly appealing for such applications as it can efficiently upconvert low-intensity, incoherent light. However, previously demonstrated thin-film TTA sys… ▽ More Upconversion of low-energy photons to higher-energy photons provides an opportunity to surpass traditional limitations in fields such as 3D printing, photovoltaics, and photocatalysis. Triplet--triplet annihilation upconversion (TTA-UC) is particularly appealing for such applications as it can efficiently upconvert low-intensity, incoherent light. However, previously demonstrated thin-film TTA systems are simultaneously constrained by modest efficiencies and limited reach into the near infrared (NIR). Here, we design a single-layer thin-film bulk heterojunction that integrates PbS quantum dots (QDs) as tunable NIR absorbers within an organic semiconductor matrix of TES-ADT, achieving large anti-Stokes shifts up to 500 nm and high internal quantum efficiencies across the NIR-I and NIR-II windows (800-1200 nm). Through the incorporation of 5-tetracene carboxylic acid ligands on the PbS QD surface, the yield of sensitized triplets was boosted, as confirmed by transient absorption and time-resolved photoluminescence measurements. The resulting films demonstrated a 15-fold improvement in UC efficiency. Furthermore, we demonstrate visible imaging of incoherent 1200 nm light via thin-film TTA-UC at incident intensities at the imaging mask as low as 20 mWcm$^2$, marking a significant advance toward practical implementation of solid-state NIR-to-visible upconversion. △ Less

Submitted 17 June, 2026; v1 submitted 16 October, 2025; originally announced October 2025.

Thermoelectricity evidence for quantum criticality in clean infinite-layer nickelate films

Authors: Xu Zhang, Chihao Li, Mingwei Yang, Yan Zhao, Zhitong An, Danfeng Li, Liang Qiao, Haichao Xu, Rui Peng, Donglai Feng, Shiyan Li

Abstract: We investigate the Seebeck coefficient ($S$) in infinite-layer nickelate films with different disorder levels. The disordered NdNiO$_{2}$ film exhibits a flat $S/T$ curve, whereas cleaner samples display a logarithmic divergence with decreasing temperature, followed by a pronounced ``hump'' near 25 K. These distinct behaviors reveal a disorder-driven transition from band-structure-dominated transp… ▽ More We investigate the Seebeck coefficient ($S$) in infinite-layer nickelate films with different disorder levels. The disordered NdNiO$_{2}$ film exhibits a flat $S/T$ curve, whereas cleaner samples display a logarithmic divergence with decreasing temperature, followed by a pronounced ``hump'' near 25 K. These distinct behaviors reveal a disorder-driven transition from band-structure-dominated transport to quantum-critical-dominated transport. Below the ``hump'' temperature, four-fold symmetry breaking is observed in the in-plane angular magnetoresistance, indicating the presence of short-range antiferromagnetic order in parent infinite-layer nickelate films. Furthermore, the logarithmic divergence in $S/T$ is also observed in a clean superconducting Sm$_{0.73}$Ca$_{0.05}$Eu$_{0.22}$NiO$_{2}$ film, where it coexists with linear-in-temperature resistivity over the same temperature range. These findings demonstrate the existence of quantum criticality over a wide doping range in clean infinite-layer nickelate films, similar to cuprates, which highlights the central role of antiferromagnetic spin correlations in their superconducting pairing mechanisms. △ Less

Submitted 18 August, 2025; originally announced August 2025.

Comments: 8 pages, 4 figures

Observation and Modulation of the Quantum Mpemba Effect on a Superconducting Quantum Processor

Authors: Yueshan Xu, Cai-Ping Fang, Bing-Jie Chen, Ming-Chuan Wang, Zi-Yong Ge, Yun-Hao Shi, Yu Liu, Cheng-Lin Deng, Kui Zhao, Zheng-He Liu, Tian-Ming Li, Hao Li, Ziting Wang, Gui-Han Liang, Da'er Feng, Xueyi Guo, Xu-Yang Gu, Yang He, Hao-Tian Liu, Zheng-Yang Mei, Yongxi Xiao, Yu Yan, Yi-Han Yu, Wei-Ping Yuan, Jia-Chi Zhang , et al. (11 additional authors not shown)

Abstract: In non-equilibrium quantum systems, the quantum Mpemba effect (QME) emerges as a counterintuitive phenomenon: systems exhibiting greater initial symmetry breaking restore symmetry faster. It has been attracting broad interest in studying QME dynamics and potential applications in quantum information science. While theoretical exploration of QME has surged, experimental studies, specifically on its… ▽ More In non-equilibrium quantum systems, the quantum Mpemba effect (QME) emerges as a counterintuitive phenomenon: systems exhibiting greater initial symmetry breaking restore symmetry faster. It has been attracting broad interest in studying QME dynamics and potential applications in quantum information science. While theoretical exploration of QME has surged, experimental studies, specifically on its flexible modulation, remain limited. Here, we report the observation and modulation of QME using a superconducting processor featuring an all-to-all connected, tunable-coupling architecture that enables precise control from short- to long-range interactions. This platform allows independent manipulation of coupling regimes, on-site potentials, and initial states, enabling us to elucidate their roles in QME. To quantify symmetry restoration, we employ entanglement asymmetry (EA), derived from the reconstructed density matrix via quantum state tomography, as a sensitive probe. In strong short-range coupling regimes, EA crossovers during quenches from tilted Néel states confirm the presence of QME. In contrast, in intermediate coupling regimes, synchronized EA and entanglement entropy dynamics reveal the suppression of QME. Remarkably, QME reemerges with the introduction of on-site linear potentials or quenches from tilted ferromagnetic states, the latter proving robust against on-site disorder. Our study demonstrates flexible QME modulation on a superconducting platform with multiple controllable parameters, shedding light on quantum many-body non-equilibrium dynamics and opening avenues for quantum information applications. △ Less

Submitted 29 May, 2026; v1 submitted 11 August, 2025; originally announced August 2025.

Comments: Figures modified and new discussions added. Final version published in PRL

Journal ref: Phys. Rev. Lett. 137, 010402 (2026)

Many-body delocalization with a two-dimensional 70-qubit superconducting quantum simulator

Authors: Tian-Ming Li, Zheng-Hang Sun, Yun-Hao Shi, Zhen-Ting Bao, Yong-Yi Wang, Jia-Chi Zhang, Yu Liu, Cheng-Lin Deng, Yi-Han Yu, Zheng-He Liu, Chi-Tong Chen, Li Li, Hao Li, Hao-Tian Liu, Si-Yun Zhou, Zhen-Yu Peng, Yan-Jun Liu, Ziting Wang, Yue-Shan Xu, Kui Zhao, Yang He, Da'er Feng, Jia-Cheng Song, Cai-Ping Fang, Junrui Deng , et al. (13 additional authors not shown)

Abstract: Quantum many-body systems with sufficiently strong disorder can exhibit a non-equilibrium phenomenon, known as the many-body localization (MBL), which is distinct from conventional thermalization. While the MBL regime has been extensively studied in one dimension, its existence in higher dimensions remains elusive, challenged by the avalanche instability. Here, using a 70-qubit two-dimensional (2D… ▽ More Quantum many-body systems with sufficiently strong disorder can exhibit a non-equilibrium phenomenon, known as the many-body localization (MBL), which is distinct from conventional thermalization. While the MBL regime has been extensively studied in one dimension, its existence in higher dimensions remains elusive, challenged by the avalanche instability. Here, using a 70-qubit two-dimensional (2D) superconducting quantum simulator, we experimentally explore the robustness of the MBL regime in controlled finite-size 2D systems. We observe that the decay of imbalance becomes more pronounced with increasing system sizes, scaling up from 21, 42 to 70 qubits, with a relatively large disorder strength, and for the first time, provide an evidence for the many-body delocalization in 2D disordered systems. Our experimental results are consistent with the avalanche theory that predicts the instability of MBL regime beyond one spatial dimension. This work establishes a scalable platform for probing high-dimensional non-equilibrium phases of matter and their finite-size effects using superconducting quantum circuits. △ Less

Submitted 22 July, 2025; originally announced July 2025.

Comments: main text: 7 pages, 3 figures; supplementary information: 19 pages, 17 figures

Observation of superconductivity-induced leading-edge gap in Sr-doped $\mathrm{La}_{3}\mathrm{Ni}_{2}\mathrm{O}_{7}$ thin films

Authors: Wenjie Sun, Zhicheng Jiang, Bo Hao, Shengjun Yan, Hongyi Zhang, Maosen Wang, Yang Yang, Haoying Sun, Zhengtai Liu, Dianxiang Ji, Zhengbin Gu, Jian Zhou, Dawei Shen, Donglai Feng, Yuefeng Nie

Abstract: The discovery of high-temperature superconductivity in pressurized bulk $\mathrm{La}_{3}\mathrm{Ni}_{2}\mathrm{O}_{7}$ has ignited significant interest in nickelate superconductors. Unlike cuprates, where superconductivity predominantly originates from the $\mathrm{3}d_{x^2-y^2}$ orbital, nickelates exhibit additional complexities involving contributions from the $\mathrm{3}d_{z^2}$ orbital, promp… ▽ More The discovery of high-temperature superconductivity in pressurized bulk $\mathrm{La}_{3}\mathrm{Ni}_{2}\mathrm{O}_{7}$ has ignited significant interest in nickelate superconductors. Unlike cuprates, where superconductivity predominantly originates from the $\mathrm{3}d_{x^2-y^2}$ orbital, nickelates exhibit additional complexities involving contributions from the $\mathrm{3}d_{z^2}$ orbital, prompting fundamental questions about their pairing mechanisms. Despite recent progress in stabilizing superconductivity in $\mathrm{La}_{3}\mathrm{Ni}_{2}\mathrm{O}_{7}$ thin films at ambient pressure, direct spectroscopic evidence of the superconducting gap opening remains elusive. Here, we present an in-situ angle-resolved photoemission spectroscopy study of Sr-doped superconducting $\mathrm{La}_{3}\mathrm{Ni}_{2}\mathrm{O}_{7}$ thin films. Fermi surface mapping reveals Ni-$\mathrm{3}d_{x^2-y^2}$-derived $α$ and $β$ pockets, with orbital fillings of 0.11$\pm$0.02 electrons and 0.66$\pm$0.03 holes per Ni, respectively, resulting in a total of 0.45$\pm$0.04 electrons for each Ni. These bands exhibit moderate electron correlations, characterized by a band renormalization factor of 3-4. Notably, both $α$ and $β$ bands exhibit leading-edge shifts across the superconducting transition, with gap magnitude of ~1-2 meV at Fermi momenta along the Brillouin zone diagonal and slightly away from the zone diagonal, deviating from the conventional $d_{x^2-y^2}$-wave gap structure. Additionally, the Ni-$\mathrm{3}d_{z^2}$-derived $γ$ band lies ~75 meV below the Fermi level, indicating a $\mathrm{3}d_{x^2-y^2}$-dominated fermiology in this compound. △ Less

Submitted 10 July, 2025; originally announced July 2025.

Comments: 18 pages and 5 figures

Observation of Electride-like $s$ States Coexisting with Correlated $d$ Electrons in NdNiO$_2$

Authors: Chihao Li, Yutong Chen, Xiang Ding, Yezhao Zhuang, Nan Guo, Zhihui Chen, Yu Fan, Jiahao Ye, Zhitong An, Suppanut Sangphet, Shenglin Tang, Xiaoxiao Wang, Hai Huang, Haichao Xu, Donglai Feng, Rui Peng

Abstract: Despite exhibiting a similar $d_{x^2-y^2}$ band character to cuprates, infinite-layer nickelates host additional electron pockets that distinguish them from single-band cuprates. The elusive orbital origin of these electron pockets has led to competing theoretical scenarios. Here, using polarization-dependent and resonant angle-resolved photoemission spectroscopy (ARPES), we determine the orbital… ▽ More Despite exhibiting a similar $d_{x^2-y^2}$ band character to cuprates, infinite-layer nickelates host additional electron pockets that distinguish them from single-band cuprates. The elusive orbital origin of these electron pockets has led to competing theoretical scenarios. Here, using polarization-dependent and resonant angle-resolved photoemission spectroscopy (ARPES), we determine the orbital character of the Fermi surfaces in NdNiO$_2$. Our data reveal that the electron-like pocket arises predominantly from interstitial $s$ states, with negligible contributions from rare-earth 5$d$ and 4$f$ orbitals near the Fermi level. The observation of well-defined quantum well states indicates a uniform distribution of these interstitial electrons throughout the film thickness. By comparing with electronic structure of LaNiO$_2$, we find that the rare-earth element modulates the Ni-derived bands and hopping integrals through a chemical pressure effect. These findings clarify the role of rare-earth elements in shaping the low-energy electronic structure and establish the presence of electride-like interstitial $s$ states in a correlated oxide system, where electrons occupy lattice voids rather than atomic orbitals. The electride-like character offer new insight into the self-doping and superconductivity in infinite-layer nickelates. △ Less

Submitted 6 July, 2025; originally announced July 2025.

Comments: 7pages, 4 figures

MSC Class: 82D55

Journal ref: Phys. Rev. Lett. 135, 116501 (2025)

High Temperature Superconductivity Dominated by Inner Underdoped CuO$_2$ Planes in Quadruple-Layer Cuprate (Cu,C)Ba$_2$Ca$_3$Cu$_4$O$_{11+δ}$

Authors: Xingtian Sun, Suppanut Sangphet, Nan Guo, Yu Fan, Yutong Chen, Minyinan Lei, Xue Ming, Xiyu Zhu, Hai-Hu Wen, Haichao Xu, Rui Peng, Donglai Feng

Abstract: The superconducting transition temperature ($T_{\mathrm{c}}$) of trilayer or quadruple-layer cuprates typically surpasses that of single-layer or bilayer systems. This observation is often interpreted within the ``composite picture", where strong proximity effect between inner CuO$_2$ planes (IPs) and outer CuO$_2$ planes (OPs) is crucial. Albeit intriguing, a straightforward scrutinization of thi… ▽ More The superconducting transition temperature ($T_{\mathrm{c}}$) of trilayer or quadruple-layer cuprates typically surpasses that of single-layer or bilayer systems. This observation is often interpreted within the ``composite picture", where strong proximity effect between inner CuO$_2$ planes (IPs) and outer CuO$_2$ planes (OPs) is crucial. Albeit intriguing, a straightforward scrutinization of this composite picture is still lacking. In this study, using angle-resolved photoemission spectroscopy to investigate (Cu,C)Ba$_2$Ca$_3$Cu$_4$O$_{11+δ}$ (CuC-1234) with a high $T_{\mathrm{c}}$ of 110~K, we found that the OPs are not superconducting at the $T_{\mathrm{c}}$ of the material. Instead, the large pairing strength and phase coherence concurrently emerge at the underdoped IPs, suggesting that the high $T_{\mathrm{c}}$ is primarily driven by these underdoped IPs. Given that the $T_{\mathrm{c}}$ of CuC-1234 is comparable to other trilayer or quadruple-layer cuprates, our findings suggest that the conventional ``composite picture" is not universally required for achieving high $T_{\mathrm{c}}$. More importantly, we demonstrate that CuO$_2$ planes free of apical oxygen can support superconductivity up to 110~K even at a doping level of 0.07 holes per Cu, a level that lies deep in the underdoped regime of single- and bilayer cuprates. These findings provide new insights into the origin of high $T_{\mathrm{c}}$ in multilayer cuprates. △ Less

Submitted 5 July, 2025; originally announced July 2025.

Comments: 6 pages, 4 figures

Journal ref: Phys. Rev. Lett. 136, 186401 (2026)

Unconventional band splitting of CeSb in the devil's staircase transition

Authors: Tongrui Li, Zhanfeng Liu, Peng Li, Yuzhe Wang, Zhisheng Zhao, Shiwu Su, Zhicheng Jiang, Yuhao Hong, Hui Tian, Xin Zheng, Yi Liu, Yilin Wang, Zhengtai Liu, Dawei Shen, Zhe Sun, Yang Liu, Juan Jiang, Donglai Feng

Abstract: The interplay between magnetism and electronic band structure is a central theme in condensed matter physics. CeSb, with its complex devil's staircase antiferromagnetic transition, offers a unique opportunity to explore this interplay. Using angle-resolved photoemission spectroscopy (ARPES), we investigate the electronic structure evolution across the devil's staircase transition. Upon entering th… ▽ More The interplay between magnetism and electronic band structure is a central theme in condensed matter physics. CeSb, with its complex devil's staircase antiferromagnetic transition, offers a unique opportunity to explore this interplay. Using angle-resolved photoemission spectroscopy (ARPES), we investigate the electronic structure evolution across the devil's staircase transition. Upon entering the antiferromagnetic phase, we observe an intriguing band splitting of the electron pocket around the X point. The energy separation between the split bands changes abruptly with temperature, consistent with the characteristics of the first-order phase transition. However, their respective spectral weights behave gradually with temperature. Combined with our density functional theory (DFT) calculations, we suggest that this atypical behavior deviates from conventional magnetically induced band splitting and potentially arises from the intricate modulation of paramagnetic and antiferromagnetic layers within the devil's staircase transition. Our results provide insights into the complex relationship between electronic structure and magnetism in correlated electron systems. △ Less

Submitted 18 May, 2025; originally announced May 2025.

Comments: 13 pages, 4 figures

Journal ref: Communications Materials volume 6, Article number: 97 (2025)

Prethermalization by Random Multipolar Driving on a 78-Qubit Superconducting Processor

Authors: Zheng-He Liu, Yu Liu, Gui-Han Liang, Cheng-Lin Deng, Keyang Chen, Yun-Hao Shi, Tian-Ming Li, Lv Zhang, Bing-Jie Chen, Cai-Ping Fang, Da'er Feng, Xu-Yang Gu, Yang He, Kaixuan Huang, Hao Li, Hao-Tian Liu, Li Li, Zheng-Yang Mei, Zhen-Yu Peng, Jia-Cheng Song, Ming-Chuan Wang, Shuai-Li Wang, Ziting Wang, Yongxi Xiao, Minke Xu , et al. (21 additional authors not shown)

Abstract: Time-dependent drives hold the promise of realizing non-equilibrium many-body phenomena that are absent in undriven systems. Yet, drive-induced heating normally destabilizes the systems, which can be parametrically suppressed in the high-frequency regime by using periodic (Floquet) drives. It remains largely unknown to what extent highly controllable quantum simulators can suppress heating in non-… ▽ More Time-dependent drives hold the promise of realizing non-equilibrium many-body phenomena that are absent in undriven systems. Yet, drive-induced heating normally destabilizes the systems, which can be parametrically suppressed in the high-frequency regime by using periodic (Floquet) drives. It remains largely unknown to what extent highly controllable quantum simulators can suppress heating in non-periodically driven systems. Using the 78-qubit superconducting quantum processor, Chuang-tzu 2.0, we report the experimental observation of long-lived prethermal phases in many-body systems with tunable heating rates, driven by structured random protocols, characterized by $n$-multipolar temporal correlations. By measuring both the particle imbalance and subsystem entanglement entropy, we monitor the entire heating process over 1,000 driving cycles and observe the existence of the prethermal plateau. The prethermal lifetime is `doubly tunable': one way by driving frequency, the other by multipolar order; it grows algebraically with the frequency with the universal scaling exponent $2n{+}1$. Using quantum state tomography on different subsystems, we demonstrate a non-uniform spatial entanglement distribution and observe a crossover from area-law to volume-law entanglement scaling. With 78 qubits and 137 couplers in a 2D configuration, the entire far-from-equilibrium heating dynamics are beyond the reach of simulation using tensor-network numerical techniques. Our work highlights superconducting quantum processors as a powerful platform for exploring universal scaling laws and non-equilibrium phases of matter in driven systems in regimes where classical simulation faces formidable challenges. △ Less

Submitted 1 April, 2025; v1 submitted 27 March, 2025; originally announced March 2025.

Journal ref: Nature 650, 79-85 (2026)

Yin-Yang vortex on UTe2 (011) surface

Authors: Ruotong Yin, Yuanji Li, Zengyi Du, Dengpeng Yuan, Shiyuan Wang, Jiashuo Gong, Mingzhe Li, Ziyuan Chen, Jiakang Zhang, Yuguang Wang, Ziwei Xue, Xinchun Lai, Shiyong Tan, Da Wang, Qiang-Hua Wang, Dong-Lai Feng, Ya-Jun Yan

Abstract: UTe2 is a promising candidate for spin-triplet superconductor, yet its exact superconducting order parameter remains highly debated. Here, via scanning tunneling microscopy/spectroscopy, we observe a novel type of magnetic vortex with distinct dark-bright contrast in local density of states on UTe2 (011) surface under a perpendicular magnetic field, resembling the conjugate structure of Yin-Yang d… ▽ More UTe2 is a promising candidate for spin-triplet superconductor, yet its exact superconducting order parameter remains highly debated. Here, via scanning tunneling microscopy/spectroscopy, we observe a novel type of magnetic vortex with distinct dark-bright contrast in local density of states on UTe2 (011) surface under a perpendicular magnetic field, resembling the conjugate structure of Yin-Yang diagram in Taoism. Each Yin-Yang vortex contains a quantized magnetic flux, and the boundary between the Yin and Yang parts aligns with the crystallographic a-axis of UTe2. The vortex states exhibit intriguing behaviors -- a sharp zero-energy conductance peak exists at the Yang part, while a superconducting gap with pronounced coherence peaks exists at the Yin part, which is even sharper than those measured far from the vortex core or in the absence of magnetic field. By theoretical modeling, we show that the Yin-Yang vortices on UTe2 (011) surface can be explained by the asymmetric vortex-derived local distortion of the zero-energy surface states associated with spin-triplet pairing with appropriate d-vectors. Therefore, the observation of Yin-Yang vortex confirms the spin-triplet pairing in UTe2 and imposes constraints on the candidate d-vector for the spin-triplet pairing. △ Less

Submitted 21 May, 2025; v1 submitted 27 March, 2025; originally announced March 2025.

Comments: 13 pages, 4 figures

Revealing the electron-spin fluctuation coupling by photoemission in CaKFe4As4

Authors: Peng Li, Yuzhe Wang, Yabin Liu, Jianghao Yao, Zhisheng Zhao, Zhengtai Liu, Dawei Shen, Huiqian Luo, Guanghan Cao, Juan Jiang, Donglai Feng

Abstract: Electron-boson coupling in unconventional superconductors is one of the key parameters in understanding the superconducting pairing symmetry. Here, we report definitive photoemission evidence of electron-spin exciton coupling in the iron-based superconductor CaKFe4As4, obtained via high-resolution ARPES. Our study identifies a distinct kink structure on the α band, observable only in the supercond… ▽ More Electron-boson coupling in unconventional superconductors is one of the key parameters in understanding the superconducting pairing symmetry. Here, we report definitive photoemission evidence of electron-spin exciton coupling in the iron-based superconductor CaKFe4As4, obtained via high-resolution ARPES. Our study identifies a distinct kink structure on the α band, observable only in the superconducting phase and closely linked with the superconductivity, indicative of strong electron-boson interactions. Notably, this kink structure corresponds to two distinct bosonic modes at 11 meV and 13 meV, aligning with spin resonance modes previously observed in inelastic neutron scattering experiments. This alignment underscores the significant role of antiferromagnetic fluctuations in the pairing mechanism of this superconductor. Furthermore, the unique momentum-dependent and orbital-selective properties of the coupling revealed by ARPES provide profound insights into the pairing symmetry, suggesting predominantly s_+- wave pairing facilitated by spin fluctuations. Our findings not only highlight the pivotal role of spin resonance in the superconductivity of CaKFe4As4 but also enhance understanding of the electron-spin exciton interactions in unconventional superconductors. △ Less

Submitted 5 March, 2025; originally announced March 2025.

Comments: Phys. Rev. X - Accepted 4 March, 2025

Revealing Higher-Order Topological Bulk-boundary Correspondence in Bismuth Crystal with Spin-helical Hinge State Loop and Proximity Superconductivity

Authors: D. M. Zhao, Y. Zhong, T. Yuan, H. T. Wang, T. X. Jiang, Y. Qi, H. J. Xiang, X. G. Gong, D. L. Feng, T. Zhang

Abstract: Topological materials are typically characterized by gapless boundary states originated from nontrivial bulk band topology, known as topological bulk-boundary correspondence. Recently, this fundamental concept has been generalized in higher-order topological insulators (HOTIs). E.g., a second-order three-dimensional (3D) TI hosts one-dimensional (1D) topological hinge states winding around the cry… ▽ More Topological materials are typically characterized by gapless boundary states originated from nontrivial bulk band topology, known as topological bulk-boundary correspondence. Recently, this fundamental concept has been generalized in higher-order topological insulators (HOTIs). E.g., a second-order three-dimensional (3D) TI hosts one-dimensional (1D) topological hinge states winding around the crystal. However, a complete verification of higher-order topology is still lacking as it requires probing all the crystal boundaries. Here we studied a promising candidate of second-order TI, bismuth (Bi), in the form of mesoscopic crystals grown on superconducting V3Si. Using low-temperature scanning tunneling microscopy, we directly observed dispersive 1D states on various hinges of the crystal. Upon introducing magnetic scatterers, new scattering channels emerged selectively on certain hinges, revealing their spin-helical nature. Combining first-principle calculation and global symmetry analysis, we find these hinge states are topological and formed a closed loop encircling the crystal. This provides direct evidence on the higher-order topology in Bi. Moreover, proximity superconductivity is observed in the topological hinge states, enabling HOTI as a promising platform for realizing topological superconductivity and Majorana quasiparticles. △ Less

Submitted 29 January, 2026; v1 submitted 11 February, 2025; originally announced February 2025.

Comments: Complete version,29 pages,16 figures. Supplementary Material included

Journal ref: Science Bulletin 70, 3310 (2025)

Direct Visualization of an Incommensurate Unidirectional Charge Density Wave in La$_4$Ni$_3$O$_{10}$

Authors: Mingzhe Li, Jiashuo Gong, Yinghao Zhu, Ziyuan Chen, Jiakang Zhang, Enkang Zhang, Yuanji Li, Ruotong Yin, Shiyuan Wang, Jun Zhao, Dong-Lai Feng, Zengyi Du, Ya-Jun Yan

Abstract: Superconductivity emerges in both La$_3$Ni$_2$O$_7$ and La$_4$Ni$_3$O$_{10}$ under high pressure by suppressing their density-wave transitions, but critical temperature (Tc) differs significantly between these two compounds. To gain deeper insights into the distinct superconducting states, it is essential to unravel the nature of the density-wave states at ambient pressure, a topic that remains la… ▽ More Superconductivity emerges in both La$_3$Ni$_2$O$_7$ and La$_4$Ni$_3$O$_{10}$ under high pressure by suppressing their density-wave transitions, but critical temperature (Tc) differs significantly between these two compounds. To gain deeper insights into the distinct superconducting states, it is essential to unravel the nature of the density-wave states at ambient pressure, a topic that remains largely unexplored. Here, using scanning tunneling microscopy/spectroscopy (STM/STS), we report the direct visualization of an incommensurate unidirectional charge density wave (CDW) in La$_4$Ni$_3$O$_{10}$ in real space. The density of states (DOS) is strongly depleted near $E_F$, indicating the opening of a CDW gap of $2Δ \approx 71$ meV, which is unfavorable for the formation of superconductivity at ambient pressure. We propose that the CDW arises from Fermi surface nesting, and is likely a subsidiary phase of a spin density wave. Compared to La$_3$Ni$_2$O$_7$, the weaker electronic correlation in La$_4$Ni$_3$O$_{10}$ is likely one reason for the lower $T_c$. △ Less

Submitted 30 January, 2025; originally announced January 2025.

Comments: 11 pages, 4 figures

Exact Decoding of Repetition Code under Circuit Level Noise

Authors: Hanyan Cao, Shoukuan Zhao, Dongyang Feng, Zisong Shen, Haisheng Yan, Tang Su, Weijie Sun, Huikai Xu, Feng Pan, Haifeng Yu, Pan Zhang

Abstract: Repetition code forms a fundamental basis for quantum error correction experiments. To date, it stands as the sole code that has achieved large distances and extremely low error rates. Its applications span the spectrum of evaluating hardware limitations, pinpointing hardware defects, and detecting rare events. However, current methods for decoding repetition codes under circuit level noise are su… ▽ More Repetition code forms a fundamental basis for quantum error correction experiments. To date, it stands as the sole code that has achieved large distances and extremely low error rates. Its applications span the spectrum of evaluating hardware limitations, pinpointing hardware defects, and detecting rare events. However, current methods for decoding repetition codes under circuit level noise are suboptimal, leading to inaccurate error correction thresholds and introducing additional errors in event detection. In this work, we establish that repetition code under circuit level noise has an exact solution, and we propose an optimal maximum likelihood decoding algorithm called planar. The algorithm is based on the exact solution of the spin glass partition function on planar graphs and has polynomial computational complexity. Through extensive numerical experiments, we demonstrate that our algorithm uncovers the exact threshold for depolarizing noise and realistic superconductor SI1000 noise. Furthermore, we apply our method to analyze data from recent quantum memory experiments conducted by Google Quantum AI, revealing that part of the error floor was attributed to the decoding algorithm used by Google. Finally, we implemented the repetition code quantum memory on superconducting systems with a 72-qubit quantum chip lacking reset gates, demonstrating that even with an unknown error model, the proposed algorithm achieves a significantly lower logical error rate than the matching-based algorithm. △ Less

Submitted 7 January, 2025; originally announced January 2025.

All-passive upconversion of incoherent near-infrared light at intensities down to 10$^{-7}$ W/cm$^2$

Authors: Rabeeya Hamid, Demeng Feng, Pournima Narayanan, Justin S. Edwards, Manchen Hu, Emma Belliveau, Minjeong Kim, Sanket Deshpande, Chenghao Wan, Linda Pucurimay, David A. Czaplewski, Daniel N. Congreve, Mikhail A. Kats

Abstract: Frequency upconversion, which converts low-energy photons into higher-energy ones, typically requires intense coherent illumination to drive nonlinear processes or the use of externally driven optoelectronic devices. Here, we demonstrate an upconversion system that converts low-intensity (down to ~10-7 W/cm$^2$) incoherent near-infrared (NIR) light into the visible, reaching intensities perceptibl… ▽ More Frequency upconversion, which converts low-energy photons into higher-energy ones, typically requires intense coherent illumination to drive nonlinear processes or the use of externally driven optoelectronic devices. Here, we demonstrate an upconversion system that converts low-intensity (down to ~10-7 W/cm$^2$) incoherent near-infrared (NIR) light into the visible, reaching intensities perceptible by the human eye, without the use of any external power input. Our upconverting element is enabled by the following ingredients: (1) photon upconversion via triplet-triplet annihilation in a bulk heterojunction of the organic semiconductors Y6 and rubrene; (2) plasmonic enhancement of absorption and field intensity in the heterojunction layer; (3) collection enhancement using a dichroic thin-film assembly. To enable high-resolution imaging, the upconverting element is inserted at an intermediate image plane of a dual-wavelength telescope system, which preserves the relative directionality of rays between the incident NIR light and output visible light. Our all-passive upconversion imaging system will enable NIR imaging and sensing in low-light environments under energy constraints. △ Less

Submitted 23 June, 2025; v1 submitted 27 November, 2024; originally announced November 2024.

Comments: Main text + Supporting Info. Added a new section in the Supporting Info

Observation of Yu-Shiba-Rusinov-like states at the edge of CrBr3/NbSe2 heterostructure

Authors: Yuanji Li, Ruotong Yin, Mingzhe Li, Jiashuo Gong, Ziyuan Chen, Jiakang Zhang, Ya-Jun Yan, Dong-Lai Feng

Abstract: The hybrid ferromagnet-superconductor heterostructures have attracted extensive attention as they potentially host topological superconductivity. Relevant experimental signatures have recently been reported in CrBr3/NbSe2 ferromagnet-superconductor heterostructure, but controversies remain. Here, we reinvestigate CrBr3/NbSe2 by an ultralow temperature scanning tunneling microscope with higher spat… ▽ More The hybrid ferromagnet-superconductor heterostructures have attracted extensive attention as they potentially host topological superconductivity. Relevant experimental signatures have recently been reported in CrBr3/NbSe2 ferromagnet-superconductor heterostructure, but controversies remain. Here, we reinvestigate CrBr3/NbSe2 by an ultralow temperature scanning tunneling microscope with higher spatial and energy resolutions. We find that the single-layer CrBr3 film is insulating and acts likely as a vacuum barrier, the measured superconducting gap and vortex state on it are nearly the same as those of NbSe2 substrate. Meanwhile, in-gap features are observed at the edges of CrBr3 island, which display either a zero-energy conductance peak or a pair of particle-hole symmetric bound states. They are discretely distributed at the edges of CrBr3 film, and their appearance is found closely related to the atomic lattice reconstruction near the edges. By increasing tunneling transmissivity, the zero-energy conductance peak quickly splits, while the pair of nonzero in-gap bound states first approach each other, merge, and then split again. These behaviors are unexpected for Majorana edge modes, but in consistent with the conventional Yu-Shiba-Rusinov states. Our results provide critical information for further understanding the interfacial coupling in CrBr3/NbSe2 heterostructure. △ Less

Submitted 27 November, 2024; originally announced November 2024.

Comments: 13 pages, 5 figures

Journal ref: Nature Communications 15, 10121 (2024)

Exploring structure diversity in atomic resolution microscopy with graph neural networks

Authors: Zheng Luo, Ming Feng, Zijian Gao, Jinyang Yu, Liang Hu, Tao Wang, Shenao Xue, Shen Zhou, Fangping Ouyang, Dawei Feng, Kele Xu, Shanshan Wang

Abstract: The emergence of deep learning (DL) has provided great opportunities for the high-throughput analysis of atomic-resolution micrographs. However, the DL models trained by image patches in fixed size generally lack efficiency and flexibility when processing micrographs containing diversified atomic configurations. Herein, inspired by the similarity between the atomic structures and graphs, we descri… ▽ More The emergence of deep learning (DL) has provided great opportunities for the high-throughput analysis of atomic-resolution micrographs. However, the DL models trained by image patches in fixed size generally lack efficiency and flexibility when processing micrographs containing diversified atomic configurations. Herein, inspired by the similarity between the atomic structures and graphs, we describe a few-shot learning framework based on an equivariant graph neural network (EGNN) to analyze a library of atomic structures (e.g., vacancies, phases, grain boundaries, doping, etc.), showing significantly promoted robustness and three orders of magnitude reduced computing parameters compared to the image-driven DL models, which is especially evident for those aggregated vacancy lines with flexible lattice distortion. Besides, the intuitiveness of graphs enables quantitative and straightforward extraction of the atomic-scale structural features in batches, thus statistically unveiling the self-assembly dynamics of vacancy lines under electron beam irradiation. A versatile model toolkit is established by integrating EGNN sub-models for single structure recognition to process images involving varied configurations in the form of a task chain, leading to the discovery of novel doping configurations with superior electrocatalytic properties for hydrogen evolution reactions. This work provides a powerful tool to explore structure diversity in a fast, accurate, and intelligent manner. △ Less

Submitted 23 October, 2024; originally announced October 2024.

Revealing nanoscale structural phase separation in La$_{3}$Ni$_{2}$O$_{7-δ}$ single crystal via scanning near-field optical microscopy

Authors: Xiaoxiang Zhou, Weihong He, Kaipeng Ni, Mengwu Huo, Deyuan Hu, Yinghao Zhu, Enkang Zhang, Zhicheng Jiang, Shuaikang Zhang, Shiwu Su, Juan Jiang, Yajun Yan, Yilin Wang, Dawei Shen, Xue Liu, Jun Zhao, Meng Wang, Zengyi Du, Donglai Feng

Abstract: The discovery of superconductivity in La3Ni2O7-$δ$ under high pressure,with an onset critical temperature around 80 K, has sparked significant interest in the superconducting phases of Ruddlesden-Popper nickelates, Lan+1NinO3n+1. While La4Ni3O10 exhibits nearly 100% superconductivity with Tc~30 K under high pressure, magnetic susceptibility studies on La3Ni2O7-$δ$, however, reveal a more complex p… ▽ More The discovery of superconductivity in La3Ni2O7-$δ$ under high pressure,with an onset critical temperature around 80 K, has sparked significant interest in the superconducting phases of Ruddlesden-Popper nickelates, Lan+1NinO3n+1. While La4Ni3O10 exhibits nearly 100% superconductivity with Tc~30 K under high pressure, magnetic susceptibility studies on La3Ni2O7-$δ$, however, reveal a more complex picture, indicating either filamentary superconductivity or that approximately 50% of crystal phase becomes superconducting in polycrystalline samples. In this study, we employed scattering-type scanning near-field optical microscopy to visualize nanoscale structural phase separation in La3Ni2O7-$δ$, identifying enhanced optical conductivity with stripes approximately 183 nm wide. These stripes run diagonally with respect to the Ni-O-Ni bond directions in the a-b plane, ruling out the possibility that they arise from impurity phases, like the '1313', '214' or '4310' structures. The dark regions and bright stripes exhibit optical conductivities ~ 22% and 29% of gold's, respectively. Additionally, we find that the bright stripes constitute about 38% of the total field of view, while the remainder consists of dark regions and the transitional region between dark regions and bright stripes. Our results suggest that optical conductivity stripes originate from nanoscale structural phase separation. In contrast, La4Ni3O10 exhibits uniform and higher optical conductivity with no observable evidence of phase separation. Thus, our study represents a pioneering effort to directly image nanoscale phase separation in Lan+1NinO3n+1 nickelates. This observation could provide crucial insights into the factors that limit the superconducting volume fraction of La3Ni2O7-$δ$, highlighting SNOM as a powerful probe for exploring nanoscale low-energy physics in correlated quantum materials. △ Less

Submitted 17 March, 2025; v1 submitted 9 October, 2024; originally announced October 2024.

Comments: 12 pages, 4 figures

Preventing overfitting in infrared ellipsometry using temperature dependence: fused silica as a case study

Authors: Shenwei Yin, Jin-Woo Cho, Demeng Feng, Hongyan Mei, Tanuj Kumar, Chenghao Wan, Yeonghoon Jin, Minjeong Kim, Mikhail A. Kats

Abstract: Fitting oscillator models to variable-angle spectroscopic ellipsometry (VASE) data can lead to non-unique, unphysical results. We demonstrate using temperature-dependent trends to prevent overfitting and ensure model physicality. As a case study, we performed mid-infrared VASE measurements on fused silica (SiO2) of various grades, from room temperature to 600 °C. We fitted oscillator models indepe… ▽ More Fitting oscillator models to variable-angle spectroscopic ellipsometry (VASE) data can lead to non-unique, unphysical results. We demonstrate using temperature-dependent trends to prevent overfitting and ensure model physicality. As a case study, we performed mid-infrared VASE measurements on fused silica (SiO2) of various grades, from room temperature to 600 °C. We fitted oscillator models independently at each temperature, and confirmed the model's physical validity by observing the expected monotonic trends in vibrational oscillator parameters. Using this technique, we generated a highly accurate dataset for the temperature-dependent complex refractive index of fused silica for modeling mid-infrared optical components such as thermal emitters. △ Less

Submitted 16 June, 2025; v1 submitted 9 September, 2024; originally announced September 2024.

Comments: Main text + supplementary (updated June 16, 2025). The data can be found at this Zenodo record: https://zenodo.org/records/15178466

Evidence of electron interaction with an unidentified bosonic mode in superconductor CsCa$_2$Fe$_4$As$_4$F$_2$

Authors: Peng Li, Sen Liao, Zhicheng Wang, Huaxun Li, Shiwu Su, Jiakang Zhang, Ziyuan Chen, Zhicheng Jiang, Zhengtai Liu, Lexian Yang, Linwei Huai, Junfeng He, Shengtao Cui, Zhe Sun, Yajun Yan, Guanghan Cao, Dawei Shen, Juan Jiang, Donglai Feng

Abstract: The kink structure in band dispersion usually refers to a certain electron-boson interaction, which is crucial in understanding the pairing in unconventional superconductors. Here we report the evidence of the observation of a kink structure in Fe-based superconductor CsCa$_2$Fe$_4$As$_4$F$_2$ using angle-resolved photoemission spectroscopy. The kink shows an orbital selective and momentum depende… ▽ More The kink structure in band dispersion usually refers to a certain electron-boson interaction, which is crucial in understanding the pairing in unconventional superconductors. Here we report the evidence of the observation of a kink structure in Fe-based superconductor CsCa$_2$Fe$_4$As$_4$F$_2$ using angle-resolved photoemission spectroscopy. The kink shows an orbital selective and momentum dependent behavior, which is located at 15 meV below Fermi level along the Gamma-M direction at the band with dxz orbital character and vanishes when approaching the Gamma-X direction, correlated with a slight decrease of the superconducting gap. Most importantly, this kink structure disappears when the superconducting gap closes, indicating that the corresponding bosonic mode (9 meV) is closely related to superconductivity. However, the origin of this mode remains unidentified, since it cannot be related to phonons or the spin resonance mode (15 meV) observed by inelastic neutron scattering. The behavior of this mode is rather unique and challenges our present understanding of the superconducting paring mechanism of the bilayer FeAs-based superconductors. △ Less

Submitted 1 August, 2024; originally announced August 2024.

Comments: 14 pages, 4 figures

Journal ref: Nature Communications 15,2024,6433

Interface suppressed nematicity and enhanced superconductivity of FeSe/NdFeO3 in the low doping regime

Authors: Chihao Li, Yuanhe Song, Xiaoxiao Wang, Minyinan Lei, Xiaoyang Chen, Haichao Xu, Rui Peng, Donglai Feng

Abstract: The discovery of interface-enhanced superconductivity in single-layer FeSe/oxides has generated intensive research interests. Beyond the family of FeSe interfaced with various TiO$_2$ terminated oxides, high pairing temperature up to 80~K has been recently observed in FeSe interfaced with FeO$_x$-terminated LaFeO$_3$. Here we successfully extend the FeSe/FeO$_x$ superconducting interface to FeSe/N… ▽ More The discovery of interface-enhanced superconductivity in single-layer FeSe/oxides has generated intensive research interests. Beyond the family of FeSe interfaced with various TiO$_2$ terminated oxides, high pairing temperature up to 80~K has been recently observed in FeSe interfaced with FeO$_x$-terminated LaFeO$_3$. Here we successfully extend the FeSe/FeO$_x$ superconducting interface to FeSe/NdFeO$_3$, by constructing 1uc-FeSe/6uc-NdFeO$_3$/Nb:SrTiO$_3$ heterostructures. Intriguingly, well-annealed FeSe/NdFeO$_3$ exhibits a low doping level of 0.038$\sim$0.046 ~e$^-/$Fe which deviates universally magic doping level (0.10$\sim$0.12 e$^-/\rm{Fe}$) and provides a new playground for studying the FeSe/oxide interface in the low electron-doped regime. Comparing it with thick FeSe films at the comparable electron doping level induced by surface potassium dosing, FeSe/NdFeO$_3$ shows a larger superconducting gap and the absence of a nematic gap, indicating an enhancement of the superconductivity and suppression of nematicity by the FeSe/FeO$_x$ interface. These results not only expand the FeSe/FeO$_x$ superconducting family but also enrich the current understanding on the roles of the oxide interface. △ Less

Submitted 16 July, 2024; originally announced July 2024.

Comments: 8 pages, 4 figures

Journal ref: Nano Lett. 24, 27, 8303-8310 (2024)

Inferior interfacial superconductivity in 1 UC FeSe/SrVO$_3$/SrTiO$_3$ with screened interfacial electron-phonon coupling

Authors: Nan Guo, Xiaoyang Chen, Tianlun Yu, Yu Fan, Qinghua Zhang, Minyinan Lei, Xiaofeng Xu, Xuetao Zhu, Jiandong Guo, Lin Gu, Haichao Xu, Rui Peng, Donglai Feng

Abstract: Monolayer FeSe/TiO$_x$ and FeSe/FeO$_x$ interfaces exhibit significant superconductivity enhancement compared to bulk FeSe, with interfacial electron-phonon coupling (EPC) playing a crucial role. However, the reduced dimensionality in monolayer FeSe, which may drive superconducting fluctuations, complicates the understanding of the enhancement mechanisms. Here we construct a new superconducting in… ▽ More Monolayer FeSe/TiO$_x$ and FeSe/FeO$_x$ interfaces exhibit significant superconductivity enhancement compared to bulk FeSe, with interfacial electron-phonon coupling (EPC) playing a crucial role. However, the reduced dimensionality in monolayer FeSe, which may drive superconducting fluctuations, complicates the understanding of the enhancement mechanisms. Here we construct a new superconducting interface: monolayer FeSe/SrVO$_3$/SrTiO$_3$, in which the itinerant electrons of highly metallic SrVO$_3$ films can screen all the high-energy Fuchs-Kliewer phonons, including those of SrTiO$_3$, making it the first FeSe/oxide system with screened interfacial EPC while maintaining the monolayer FeSe thickness. Despite comparable doping levels, the heavily electron-doped monolayer FeSe/SrVO$_3$ exhibits a lower pairing temperature ($T_\mathrm{g}$ $\sim$ 48 K) than FeSe/SrTiO$_3$ and FeSe/LaFeO$_3$. Our findings disentangle the contributions of interfacial EPC from dimensionality on enhancing $T_\mathrm{g}$ in FeSe/oxide interfaces, underscoring the importance of interfacial EPC in $T_\mathrm{g}$ enhancement. This FeSe/VO$_x$ interface also provides a platform for studying the interfacial superconductivity. △ Less

Submitted 13 July, 2024; originally announced July 2024.

Comments: Published in Nano Letters, 11 pages, 4 figures, 1 table

Large band-splitting in $g$-wave type altermagnet CrSb

Authors: Jianyang Ding, Zhicheng Jiang, Xiuhua Chen, Zicheng Tao, Zhengtai Liu, Tongrui Li, Jishan Liu, Jianping Sun, Jinguang Cheng, Jiayu Liu, Yichen Yang, Runfeng Zhang, Liwei Deng, Wenchuan Jing, Yu Huang, Yuming Shi, Mao Ye, Shan Qiao, Yilin Wang, Yanfeng Guo, Donglai Feng, Dawei Shen

Abstract: Altermagnetism (AM), a newly discovered magnetic state, ingeniously integrates the properties of ferromagnetism and antiferromagnetism, representing a significant breakthrough in the field of magnetic materials. Despite experimental verification of some typical AM materials, such as MnTe and MnTe$_2$, the pursuit of AM materials that feature larger spin splitting and higher transition temperature… ▽ More Altermagnetism (AM), a newly discovered magnetic state, ingeniously integrates the properties of ferromagnetism and antiferromagnetism, representing a significant breakthrough in the field of magnetic materials. Despite experimental verification of some typical AM materials, such as MnTe and MnTe$_2$, the pursuit of AM materials that feature larger spin splitting and higher transition temperature is still essential. Here, our research focuses on CrSb, which possesses N{é}el temperature of up to 700K and giant spin splitting near the Fermi level ($E_F$). Utilizing high-resolution angle-resolved photoemission spectroscopy and density functional theory calculations, we meticulously map the three-dimensional electronic structure of CrSb. Our photoemission spectroscopic results on both (0001) and (10$\overline{1}$0) cleavages of CrSb collaboratively reveal unprecedented details on AM-induced band splitting, and subsequently pin down its unique bulk $g$-wave symmetry through quantitative analysis of the angular and photon-energy dependence of spin splitting. Moreover, the observed spin splitting reaches the magnitude of 0.93~eV near $E_F$, the most substantial among all confirmed AM materials. This study not only validates the nature of CrSb as a prototype $g$-wave like AM material but also underscores its pivotal role in pioneering applications in spintronics. △ Less

Submitted 15 November, 2024; v1 submitted 21 May, 2024; originally announced May 2024.

Comments: 7 pages, 4 figures

Journal ref: Phys.Rev.Lett.133,206401(2024)

Self-referencing photothermal common-path interferometry to measure absorption of Si3N4 membranes for laser-light sails

Authors: Tanuj Kumar, Demeng Feng, Shenwei Yin, Merlin Mah, Phyo Lin, Margaret Fortman, Gabriel R. Jaffe, Chenghao Wan, Hongyan Mei, Yuzhe Xiao, Ron Synowicki, Ronald J. Warzoha, Victor W. Brar, Joseph J. Talghader, Mikhail A. Kats

Abstract: Laser-light sails are a spacecraft concept wherein lightweight "sails" are propelled by high-intensity lasers. We investigated the near-infrared absorption of free-standing membranes of stoichiometric silicon nitride (Si$_3$N$_4$), a candidate sail material. To resolve the small but non-zero optical loss, we used photothermal common-path interferometry (PCI), for which we developed a self-referenc… ▽ More Laser-light sails are a spacecraft concept wherein lightweight "sails" are propelled by high-intensity lasers. We investigated the near-infrared absorption of free-standing membranes of stoichiometric silicon nitride (Si$_3$N$_4$), a candidate sail material. To resolve the small but non-zero optical loss, we used photothermal common-path interferometry (PCI), for which we developed a self-referencing modality where a PCI measurement is performed twice: once on a bare membrane, and a second time with monolayer graphene deposited on the membrane. The graphene increases the absorption of the sample by orders of magnitude, such that it can be measured by ellipsometry, without significantly affecting the thermal properties. We measured the absorption coefficient of Si$_3$N$_4$ to be (1.5-3) $\times$ 10$^{-2}$ cm$^{-1}$ at 1064 nm, making it a suitable sail material for laser intensities as high as ~10 GW/m$^2$. By comparison, silicon-rich "low stress" SiN$_x$ (x~1), with a measured absorption coefficient of approximately 8 cm$^{-1}$, is unlikely to survive such high laser intensities. Our self-referencing technique enables testing of low-loss membranes of various materials for laser sails and other applications. △ Less

Submitted 13 June, 2025; v1 submitted 5 April, 2024; originally announced April 2024.

Comments: Main text + supplementary. Updated with new experiments and analysis

Revealing the Microscopic Mechanism of Elementary Vortex Pinning in Superconductors

Authors: C. Chen, Y. Liu, Y. Chen, Y. N. Hu, T. Z. Zhang, D. Li, X. Wang, C. X. Wang, Z. Y. W. Lu, Y. H. Zhang, Q. L. Zhang, X. L. Dong, R. Wang, D. L. Feng, T. Zhang

Abstract: Vortex pinning is a crucial factor that determines the critical current of practical superconductors and enables their diverse applications. However, the underlying mechanism of vortex pinning has long been elusive, lacking a clear microscopic explanation. Here using high-resolution scanning tunneling microscopy, we studied single vortex pinning induced by point defect in layered FeSe-based superc… ▽ More Vortex pinning is a crucial factor that determines the critical current of practical superconductors and enables their diverse applications. However, the underlying mechanism of vortex pinning has long been elusive, lacking a clear microscopic explanation. Here using high-resolution scanning tunneling microscopy, we studied single vortex pinning induced by point defect in layered FeSe-based superconductors. We found the defect-vortex interaction drives low-energy vortex bound states away from EF, creating a "mini" gap that effectively lowers the system energy and enhances pinning. By measuring the local density-of-states, we directly obtained the elementary pinning energy and estimated the pinning force via the spatial gradient of pinning energy. The results are consistent with bulk critical current measurement. Furthermore, we show that a general microscopic quantum model incorporating defect-vortex interaction can naturally capture our observation. It suggests that the local pairing near pinned vortex core is actually enhanced compared to unpinned vortex, which is beyond the traditional understanding that non-superconducting regions pin vortices. Our study thus unveils a general microscopic mechanism of vortex pinning in superconductors, and provides insights for enhancing the critical current of practical superconductors. △ Less

Submitted 27 September, 2024; v1 submitted 26 March, 2024; originally announced March 2024.

Comments: 32 pages, 18 figures, Supplementary Materials included. Comments are welcome

Journal ref: Phys. Rev. X 14, 041039 (2024)

Cuprate-like Electronic Structures in Infinite-Layer Nickelates with Substantial Hole Dopings

Authors: X. Ding, Y. Fan, X. X. Wang, C. H. Li, Z. T. An, J. H. Ye, S. L. Tang, M. Y. N. Lei, X. T. Sun, N. Guo, Z. H. Chen, S. Sangphet, Y. L. Wang, H. C. Xu, R. Peng, D. L. Feng

Abstract: The superconducting infinite-layer (IL) nickelates offer a new platform for investigating the long-standing problem of high-temperature superconductivity. Many models were proposed to understand its superconducting mechanisms based on the calculated electronic structure, and the multiple Fermi surfaces and multiple orbitals involved create complications and controversial conclusions. Over the past… ▽ More The superconducting infinite-layer (IL) nickelates offer a new platform for investigating the long-standing problem of high-temperature superconductivity. Many models were proposed to understand its superconducting mechanisms based on the calculated electronic structure, and the multiple Fermi surfaces and multiple orbitals involved create complications and controversial conclusions. Over the past 5 years, the lack of direct measurements of the electronic structure has hindered the understanding of nickelate superconductors. Here we fill this gap by directly resolving the electronic structures of the parent compound LaNiO$_2$ and superconducting La$_{0.8}$Ca$_{0.2}$NiO$_2$ using angle-resolved photoemission spectroscopy (ARPES). We find that their Fermi surfaces consist of a quasi-two-dimensional (quasi-2D) hole pocket and a three-dimensional (3D) electron pocket at the Brillouin zone corner, whose volumes change upon Ca doping. The Fermi surface topology and band dispersion of the hole pocket closely resemble those observed in hole-doped cuprates. However, the cuprate-like band exhibits significantly higher hole doping in superconducting La$_{0.8}$Ca$_{0.2}$NiO$_2$ compared to superconducting cuprates, highlighting the disparities in the electronic states of the superconducting phase. Our observations highlight the novel aspects of the IL nickelates, and pave the way toward the microscopic understanding of the IL nickelate family and its superconductivity. △ Less

Submitted 5 June, 2024; v1 submitted 12 March, 2024; originally announced March 2024.

Comments: 12 pages, 4 figures

Journal ref: National Science Review, nwae194 (2024)

Discovery of Itinerant Magnetic Domain Wall and Quasiparticle Boundary State in Spin-Density-Waves

Authors: Yining Hu, Xu Wang, Chen Chen, Qingle Zhang, Dongming Zhao, Tianzhen Zhang, Chenxi Wang, Qiang-Hua Wang, Donglai Feng, Tong Zhang

Abstract: Conventional magnetic domain walls are characterized by reorientation of local spins. However, what occurs at the boundary of itinerant magnets is largely unknown. Here using spin-sensitive scanning tunneling microscopy, we investigated the microscopic domain wall structure of the spin-density-wave (SDW) state in a prototypical itinerant antiferromagnet - chromium (Cr). At the boundary of two inco… ▽ More Conventional magnetic domain walls are characterized by reorientation of local spins. However, what occurs at the boundary of itinerant magnets is largely unknown. Here using spin-sensitive scanning tunneling microscopy, we investigated the microscopic domain wall structure of the spin-density-wave (SDW) state in a prototypical itinerant antiferromagnet - chromium (Cr). At the boundary of two incommensurate SDW domains, we found the spins undergo finite-scale decay rather than reorientation. This generates a double-Q SDW state, which is further evidenced by an accompanying second-order charge modulation. In the commensurate SDW domains, a clear SDW energy gap is observed. Interestingly, the screw dislocations induced half vortex and anti-vortex of SDW, paired by antiphase domain wall. The spin density vanished at such antiphase domain walls. Remarkably, for the first time we observed the SDW quasiparticle states at the boundary, resembling the Andreev bound states in superconductors. These unique SDW boundary structures can be viewed as consequences of local interference of two SDWs, either with different Q or reversed phases. Our findings thus reveal a new type of domain wall distinct to that of local moment magnetism, with a mechanism rooted in the itinerant nature of SDW. △ Less

Submitted 4 August, 2025; v1 submitted 25 February, 2024; originally announced February 2024.

Comments: 25 pages, 15 figures, supplementary materials included

Electronic and magnetic excitations in La$_3$Ni$_2$O$_7$

Authors: Xiaoyang Chen, Jaewon Choi, Zhicheng Jiang, Jiong Mei, Kun Jiang, Jie Li, Stefano Agrestini, Mirian Garcia-Fernandez, Xing Huang, Hualei Sun, Dawei Shen, Meng Wang, Jiangping Hu, Yi Lu, Ke-Jin Zhou, Donglai Feng

Abstract: The striking discovery of high-temperature superconductivity (HTSC) of 80 K in a bilayer nickelate La$_3$Ni$_2$O$_7$ under a moderately high pressure of about 14 GPa ignited a new wave of studying HTSC in nickelates. The properties of the parental phase at ambient pressure may contain key information on basic interactions therein and bosons that may mediate pairing giving birth to superconductivit… ▽ More The striking discovery of high-temperature superconductivity (HTSC) of 80 K in a bilayer nickelate La$_3$Ni$_2$O$_7$ under a moderately high pressure of about 14 GPa ignited a new wave of studying HTSC in nickelates. The properties of the parental phase at ambient pressure may contain key information on basic interactions therein and bosons that may mediate pairing giving birth to superconductivity. Moreover, the bilayer structure of La$_3$Ni$_2$O$_7$ may suggest a distinct minimal model in comparison to cuprate superconductors. Here using X-ray absorption spectroscopy and resonant inelastic X-ray scattering, we studied La$_3$Ni$_2$O$_7$ at ambient pressure, and found that Ni 3$d_{x^2-y^2}$, Ni 3$d_{z^2}$, and ligand oxygen 2$p$ orbitals dominate the low-energy physics with a small charge-transfer energy. Remarkably, well-defined optical-like magnetic excitations were found to soften into a quasi-static spin-density-wave ordering, evidencing the strong electronic correlations and rich magnetic properties. Based on a Heisenberg spin model, we found that the inter-layer effective magnetic superexchange interaction is much larger than the intra-layer ones, and proposed two viable magnetic structures. Our results set the foundation for further exploration of La$_3$Ni$_2$O$_7$ superconductor. △ Less

Submitted 23 January, 2024; originally announced January 2024.

Journal ref: Nature Communications 15, 9597 (2024)

Sampling-accelerated First-principles Prediction of Phonon Scattering Rates for Converged Thermal Conductivity and Radiative Properties

Authors: Ziqi Guo, Zherui Han, Dudong Feng, Guang Lin, Xiulin Ruan

Abstract: First-principles prediction of thermal conductivity and radiative properties is crucial. However, computing phonon scattering, especially for four-phonon scattering, could be prohibitively expensive, and the thermal conductivity even for silicon was still under-predicted and not converged in the literature. Here we propose a method to estimate scattering rates from a small sample of scattering pro… ▽ More First-principles prediction of thermal conductivity and radiative properties is crucial. However, computing phonon scattering, especially for four-phonon scattering, could be prohibitively expensive, and the thermal conductivity even for silicon was still under-predicted and not converged in the literature. Here we propose a method to estimate scattering rates from a small sample of scattering processes using maximum likelihood estimation. The computational cost of estimating scattering rates and associated thermal conductivity and radiative properties is dramatically reduced by over 99%. This allows us to use an unprecedented q-mesh of 32*32*32 for silicon and achieve a converged thermal conductivity value that agrees much better with experiments. The accuracy and efficiency of our approach make it ideal for the high-throughput screening of materials for thermal and optical applications. △ Less

Submitted 21 November, 2023; originally announced November 2023.

Four phonon-dominated near-field radiation in weakly anharmonic polar materials

Authors: Dudong Feng, Xiaolong Yang, Zherui Han, Xiulin Ruan

Abstract: Inelastic scattering processes typically introduce friction among carriers and reduce the transport properties of photons, phonons, and electrons. However, we predict that in contrast to the role in reducing thermal conductivity, four-phonon scattering dominates near-field radiative heat transfer (NFRHT) in both boron arsenide~(BAs) and boron antimonide. Including four-phonon scattering results in… ▽ More Inelastic scattering processes typically introduce friction among carriers and reduce the transport properties of photons, phonons, and electrons. However, we predict that in contrast to the role in reducing thermal conductivity, four-phonon scattering dominates near-field radiative heat transfer (NFRHT) in both boron arsenide~(BAs) and boron antimonide. Including four-phonon scattering results in a nearly 400-fold increase in the total heat flux between two BAs thin-films compared to three-phonon scattering alone. This non-intuitive enhancement arises from the large number of NFRHT channels activated by four-phonon scattering outcompete the effect of decreased coupling strength of surface phonon polaritons at the resonance frequency. Additionally, we point out that four-phonon scattering to decrease NFRHT in certain other systems. △ Less

Submitted 29 September, 2023; originally announced September 2023.

Classification of skyrmionic textures and extraction of Hamiltonian parameters via machine learning

Authors: Dushuo Feng, Zhihao Guan, Xiaoping Wu, Yan Wu, Changsheng Song

Abstract: Classifying skyrmionic textures and extracting magnetic Hamiltonian parameters are fundamental and demanding endeavors within the field of two-dimensional (2D) spintronics. By using micromagnetic simulation and machine learning (ML) methods, we theoretically realize the recognition of nine skyrmionic textures and the mining of magnetic Hamiltonian parameters from massive spin texture images in 2D… ▽ More Classifying skyrmionic textures and extracting magnetic Hamiltonian parameters are fundamental and demanding endeavors within the field of two-dimensional (2D) spintronics. By using micromagnetic simulation and machine learning (ML) methods, we theoretically realize the recognition of nine skyrmionic textures and the mining of magnetic Hamiltonian parameters from massive spin texture images in 2D Heisenberg model. For textures classification, a deep neural network (DNN) trained according to transfer learning is proposed to distinguish nine different skyrmionic textures. For parameters extraction, based on the textures generated by different Heisenberg exchange stiffness (J), Dzyaloshinskii-Moriya strength (D), and anisotropy constant (K), we apply a multi-input single-output (MISO) deep learning model (handling with both images and parameters) and a support vector regression (SVR) model (dealing with Fourier features) to extract the parameters embedded in the spin textures. The models for classification and extraction both achieve great results with the accuracy of 98% (DNN),90% (MISO) and 80% (SVR). Importantly, via our ML methods, the skyrmionic textures with blurred phase boundaries can be effectively distinguished, and the concluded formation conditions of various skyrmionic textures, especially the skyrmion crystal, are consistent with previous reports. Besides, our models demonstrate the mapping relationship between spin texture images and magnetic parameters, which proves the feasibility of extracting microscopic mechanisms from experimental images and has guiding significance for the experiments of spintronics. △ Less

Submitted 27 September, 2023; originally announced September 2023.