Showing 1–50 of 194 results for author: Guo, C

Tunable Statistics-Induced Caging in the Anyon-Hubbard Model

Authors: Zenong Zhou, Chaorong Guo, Hongzheng Wu, Qianglin Hu, Xiaobing Luo

Abstract: We study the quantum dynamics of two interacting anyons in the Anyon-Hubbard model on a four-site plaquette, a system that is exactly mappable to a Bose-Hubbard model. We reveal that static Aharonov-Bohm (AB) caging, induced by only specific statistical phases, emerges in the strongly interacting limit but breaks down under weak interparticle interactions. To address this, we demonstrate that stat… ▽ More We study the quantum dynamics of two interacting anyons in the Anyon-Hubbard model on a four-site plaquette, a system that is exactly mappable to a Bose-Hubbard model. We reveal that static Aharonov-Bohm (AB) caging, induced by only specific statistical phases, emerges in the strongly interacting limit but breaks down under weak interparticle interactions. To address this, we demonstrate that statistical-factor-induced AB caging can be dynamically restored via Floquet engineering. This dynamical mechanism, governed by the synthetic Floquet flux and the anyonic statistical phase, extends the caging effect into the weakly interacting regime across the full spectrum of statistical phases. Furthermore, we show that the external drive enables the selective caging of anyons, providing an efficient approach for manipulating anyons and identifying statistical phases. △ Less

Submitted 16 August, 2026; originally announced August 2026.

Comments: 10 pages, 8 figures

Spin lifetime anisotropy in graphene induced by the SiO2 interface

Authors: Aron W. Cummings, Chunhao Guo, Andrew Grieder, Shihao Tu, Mayank Gupta, Junqing Xu, Juan Marmolejo-Tejada, Yuan Ping

Abstract: Understanding how common dielectric substrates influence the spin transport properties of graphene is essential for advancing graphene-based spintronic technologies. Here we use a comprehensive set of numerical simulations to reveal how a SiO$_2$ substrate modifies the spin texture and governs spin relaxation in graphene. Using first-principles density matrix dynamics simulations, as well as tight… ▽ More Understanding how common dielectric substrates influence the spin transport properties of graphene is essential for advancing graphene-based spintronic technologies. Here we use a comprehensive set of numerical simulations to reveal how a SiO$_2$ substrate modifies the spin texture and governs spin relaxation in graphene. Using first-principles density matrix dynamics simulations, as well as tight-binding (TB) transport simulations, we quantify the effects of electron-phonon scattering, impurity scattering, and electrostatic disorder on the spin relaxation process. We find that a 2D SiO$_2$ substrate induces a predominantly Rashba-type helical spin texture in graphene, leading to a spin lifetime anisotropy of 1/2. Meanwhile, bulk SiO$_2$ breaks in-plane symmetry in graphene, leading to anisotropic in-plane and out-of-plane components in the spin texture, which we capture with a newly-developed TB model of graphene. Transport simulations under realistic disorder conditions reveal a spin lifetime anisotropy between 0.5 and 1, similar to what is seen in measurements of graphene spin valves on a SiO$_2$ substrate. Our results reveal a more complex picture of spin relaxation at the ubiquitous graphene/SiO$_2$ interface, beyond the standard Rashba model, providing critical insight for interpreting experiments and guiding substrate engineering for graphene spintronics. △ Less

Submitted 11 August, 2026; originally announced August 2026.

Compound symmetries and double antisymmetry groups in linear time-invariant photonic systems

Authors: Yunrui Wang, Shiyu Li, Cheng Guo

Abstract: Symmetry is fundamental to photonic systems. External (spatial) symmetries and internal symmetries---Lorentz reciprocity, energy conservation, and time-reversal symmetry---constrain the electromagnetic response. Photonic systems can also possess compound symmetries that combine external and internal transformations, exemplified by parity-time (PT) symmetry. However, a unified framework for general… ▽ More Symmetry is fundamental to photonic systems. External (spatial) symmetries and internal symmetries---Lorentz reciprocity, energy conservation, and time-reversal symmetry---constrain the electromagnetic response. Photonic systems can also possess compound symmetries that combine external and internal transformations, exemplified by parity-time (PT) symmetry. However, a unified framework for general compound symmetries involving reciprocity, energy conservation, and time reversal remains lacking, leaving their classification and physical implications unexplored. In this paper, we present such a framework for linear photonic systems. We define compound transformations and symmetries, and derive their constraints on electromagnetic fields and scattering matrices. We show that internal, external, and compound symmetries are naturally described by the theory of double antisymmetry groups. This theory classifies linear time-invariant photonic systems into twelve symmetry categories, each imposing characteristic constraints on the electromagnetic response. We illustrate two representative categories with numerical examples of photonic crystal slabs and apply the theory to examine Kirchhoff's law of thermal radiation for a gyrotropic sphere. Our work provides a systematic foundation for analyzing and engineering symmetry in photonic systems. △ Less

Submitted 3 August, 2026; originally announced August 2026.

Comments: 21 pages, 6 figures, including the appendices

Journal ref: Phys. Rev. A 114, 023501 (2026)

Cryogenic focused-ion-beam microstructuring enabling quantitative $c$-axis transport measurements in Tl$_2$Ba$_2$CuO$_{6+δ}$

Authors: Ayanesh Maiti, Carsten Putzke, Linus Holeschovsky, Roemer D. H. Hinlopen, Chunyu Guo, Dorothee Herrmann, Seunghyun Khim, Berit H. Goodge, Andre W. Tyler, Michele S. Conroy, Andreas W. Rost, Andrew P. Mackenzie, Philip J. W. Moll

Abstract: Absolute transport measurements in correlated quantum materials are often limited by disorder, inhomogeneity, geometric uncertainty, and small crystal size. Focused ion beam (FIB) technology offers a route to overcome many of these limitations by enabling transport devices with precisely defined geometry to be fabricated from lamellae extracted from carefully selected regions of a crystal, but its… ▽ More Absolute transport measurements in correlated quantum materials are often limited by disorder, inhomogeneity, geometric uncertainty, and small crystal size. Focused ion beam (FIB) technology offers a route to overcome many of these limitations by enabling transport devices with precisely defined geometry to be fabricated from lamellae extracted from carefully selected regions of a crystal, but its application to cuprate superconductors has been hindered by ion-beam-induced damage. Here we study the clean overdoped cuprate Tl2201 and show that conventional FIB processing causes thermally driven oxygen loss, while cryogenic FIB microstructuring largely suppresses this degradation and preserves the crystal structure from the bulk to the atomic scale. Microstructured devices quantitatively reproduce established in-plane resistivity and Hall carrier density measurements without rescaling. Applying this approach to $c$-axis transport, we obtain absolute $ρ_c(T)$ values approximately three times larger than previously reported, bringing the transport anisotropy into quantitative agreement with the known Fermi surface geometry within an isotropic relaxation-time approximation. These results resolve a long-standing discrepancy between transport and quantum oscillation measurements in overdoped Tl2201 and establish cryogenic FIB microstructuring as a route to reliable quantitative transport measurements in quantum materials where disorder, inhomogeneity, geometry, or small crystal size have previously limited experimental accuracy. △ Less

Submitted 3 August, 2026; originally announced August 2026.

Spin-orbit coupling induced geometric squeezing in rotating Bose-Einstein condensates

Authors: Fei Zhu, Chunxia Guo, Rui Zhang, Lianghui Huang, Ren Zhang, Li Chen

Abstract: Squeezed states play a key role in diverse frontiers of quantum physics. Geometrically squeezed states, a squeezed state in the orbital phase space of rotating Bose-Einstein condensates (BEC), have been conventionally generated by anisotropic trapping potentials. In this work, we propose a different route to generate geometric squeezing via spin-orbit coupling (SOC) in a pseudospin-1/2 BEC. We sho… ▽ More Squeezed states play a key role in diverse frontiers of quantum physics. Geometrically squeezed states, a squeezed state in the orbital phase space of rotating Bose-Einstein condensates (BEC), have been conventionally generated by anisotropic trapping potentials. In this work, we propose a different route to generate geometric squeezing via spin-orbit coupling (SOC) in a pseudospin-1/2 BEC. We show that the SOC enables effective two-phonon transitions within the lowest Landau level via virtual spin-flip processes, leading to exponential squeezing dynamics in both spin components. Furthermore, by applying a $π/2$ spin rotation, the two spin channels can be coherently coupled to produce two-mode geometric squeezing. We also investigate the influence of interatomic interactions on squeezing performance and identify parameters where robust squeezing can be achieved. Our work provides a viable pathway to realize and manipulate geometric squeezing in spinor quantum gases. △ Less

Submitted 29 June, 2026; originally announced June 2026.

Anomalous Floquet Heating from Sparse Long-Range Interactions

Authors: Chenyue Guo, Andrea Pizzi, Hongzheng Zhao

Abstract: Regular lattices of interacting particles under a periodic drive typically heat with rate $γ\sim e^{-\mathcal{O}(ω)}$ which is exponentially suppressed in drive frequency $ω$. Here, we show that sparse infinite-range interactions, which have recently become accessible in quantum simulators, can lead to anomalous heating with rate $γ\sim e^{-\mathcal{O}(\sqrtω)}$. This anomaly originates from the b… ▽ More Regular lattices of interacting particles under a periodic drive typically heat with rate $γ\sim e^{-\mathcal{O}(ω)}$ which is exponentially suppressed in drive frequency $ω$. Here, we show that sparse infinite-range interactions, which have recently become accessible in quantum simulators, can lead to anomalous heating with rate $γ\sim e^{-\mathcal{O}(\sqrtω)}$. This anomaly originates from the broad distribution of coordination numbers across the network: as the driving frequency increases, heating becomes dominated by sites with larger coordination numbers, making the characteristic local energy scale relevant for heating grow with frequency. For small-world networks, we develop an analytic theory that thoroughly matches our large scale numerics. Finally, we discuss how network topology can serve as a control knob for engineering non-equilibrium phases of matter. Our results uncover a new mechanism for Floquet heating and suggest new routes toward stabilizing nonequilibrium phases in driven systems with programmable interaction networks. △ Less

Submitted 23 June, 2026; originally announced June 2026.

Grassmann time-evolving matrix product operators for fermionic impurities coupled to a superconducting bath

Authors: Chu Guo, Wei Wu, Xiansong Xu, Ping-Xing Chen, Changming Yue, Tian Jiang, Ruofan Chen

Abstract: The Grassmann time-evolving matrix product operator (GTEMPO) method, which represents the Feynman-Vernon influence functional as a temporal matrix product state, has been shown to be a flexible and potentially scalable solution for fermionic quantum impurity problems. In this work, we extend GTEMPO to solve fermionic impurity problems in the Nambu formalism, in which the impurity is coupled to a s… ▽ More The Grassmann time-evolving matrix product operator (GTEMPO) method, which represents the Feynman-Vernon influence functional as a temporal matrix product state, has been shown to be a flexible and potentially scalable solution for fermionic quantum impurity problems. In this work, we extend GTEMPO to solve fermionic impurity problems in the Nambu formalism, in which the impurity is coupled to a superconducting bath. A key insight is that by employing the Bogoliubov transformation for the superconducting bath, one could obtain the analytic expression of the Feynman-Vernon influence functional in a similar form to the case of a normal bath, after which the core algorithms of GTEMPO can be straightforwardly adapted. We demonstrate the accuracy of our method by benchmarking it against exact diagonalization in several exactly solvable cases, and against the continuous-time quantum Monte Carlo method using converged dynamical mean field theory (DMFT) iterations on the imaginary contour in the non-integrable case. In all cases, we perform both imaginary- and real-time calculations to illustrate the flexibility of our method. These results illustrate that our method could be potentially useful as an impurity solver in DMFT as well as its non-equilibrium extension for fermionic impurity problems in the Nambu formalism. △ Less

Submitted 25 April, 2026; originally announced April 2026.

Comments: 15 pages, 8 figures

Decoding Equilibrium and Dynamical Criticality in the 2D Topological Order

Authors: Xiao-Ming Zhao, Cui-Xian Guo, Gaoyong Sun, Su-Peng Kou

Abstract: Analytically connecting equilibrium criticality and dynamical quantum phase transitions (DQPTs) under complex driving fields remains a significant challenge, primarily due to the combinatorial complexity of non-local long-range entanglement. Here, we decode this connection in the 2D strongly interacting Wen-plaquette model. By mapping its anyonic excitations to 1D effective dissipative channels, w… ▽ More Analytically connecting equilibrium criticality and dynamical quantum phase transitions (DQPTs) under complex driving fields remains a significant challenge, primarily due to the combinatorial complexity of non-local long-range entanglement. Here, we decode this connection in the 2D strongly interacting Wen-plaquette model. By mapping its anyonic excitations to 1D effective dissipative channels, we reveal that microscopic single-particle fidelity zeros exactly reconstruct the macroscopic equilibrium topological phase boundaries. Beyond equilibrium, we demonstrate that during non-unitary quench dynamics, these very same static singularities enforce a momentumspace exclusion against dynamical Fisher zeros. Furthermore, a newly identified dissipation-phase racing mechanism prematurely depletes the decaying mode, suppressing DQPTs and generating topologically trivial steady states. Our results establish exact microscopic static singularities as an analytical decoder for macroscopic non-unitary topological dynamics involving discrete symmetry breaking. △ Less

Submitted 25 July, 2026; v1 submitted 6 April, 2026; originally announced April 2026.

Comments: 6 pages, 3 figures

Time-evolving matrix product operators for off-diagonal system-bath coupling

Authors: Chu Guo, Wei Wu, Xiansong Xu, Tian Jiang, Ping-Xing Chen, Ruofan Chen

Abstract: The time-evolving matrix product operator (TEMPO) method has proven to be a powerful method to study the long-time dynamics of bosonic impurity problems where a small system is linearly coupled to a noninteracting bosonic bath. However, current developments of TEMPO have mostly focused on the case of diagonal system-bath coupling, i.e., $\sum_k \Aop(V_k \bdop_k + \hc)$, with $\Aop$ a Hermitian ope… ▽ More The time-evolving matrix product operator (TEMPO) method has proven to be a powerful method to study the long-time dynamics of bosonic impurity problems where a small system is linearly coupled to a noninteracting bosonic bath. However, current developments of TEMPO have mostly focused on the case of diagonal system-bath coupling, i.e., $\sum_k \Aop(V_k \bdop_k + \hc)$, with $\Aop$ a Hermitian operator of the system. Based on the process tensor framework, we extend TEMPO to the more general case of off-diagonal system-bath coupling in the form $\sum_k (V_k\Aop\bdop_k + \hc)$, where $\Aop$ could be non-Hermitian. As applications, we study the real-time dynamics of a spin that is coupled to a sub-ohmic bath via the Jaynes-Cummings-type system-bath coupling and compare it against the standard spin-boson model, where we show that the commonly used rotating-wave approximation could be very poor for this bath. We also study the imaginary-time evolution of a bosonic impurity with nonzero on-site interaction that is coupled to a sub-ohmic bath, to illustrate the flexibility of our method. Our method provides a unified framework to understand different variants of TEMPO, and is a promising building block for an impurity solver in the bosonic dynamical mean field theory for the normal phase with a scalar hybridization function. △ Less

Submitted 10 August, 2026; v1 submitted 1 April, 2026; originally announced April 2026.

Comments: 21 pages, 12 figures

Tailoring Corner States and Exceptional Points in Altermagnets

Authors: Xiao-Ming Zhao, Cui-Xian Guo, Xin-Ran Ma, Xiao-Ran Wang, Su-Peng Kou

Abstract: Altermagnets (AMs) exhibit vanishing net magnetization but strong momentum-dependent spin splitting enforced by crystal symmetry. Here, we explore the non-Hermitian effects in dissipative two-dimensional AMs. We show that symmetry-compliant dissipation naturally induces an imaginary staggered exchange field, driving a NH topological phase transition absent in conventional antiferromagnets. In the… ▽ More Altermagnets (AMs) exhibit vanishing net magnetization but strong momentum-dependent spin splitting enforced by crystal symmetry. Here, we explore the non-Hermitian effects in dissipative two-dimensional AMs. We show that symmetry-compliant dissipation naturally induces an imaginary staggered exchange field, driving a NH topological phase transition absent in conventional antiferromagnets. In the topologically nontrivial phase, hybrid skin-topological modes driven by altermagnetic d-wave anisotropy emerge, as captured by the chiral skin effect framework. In the gapless phase, we elucidate the creation and annihilation dynamics of exceptional points. Crucially, we analytically prove via the transfer matrix method that corner states are deterministically controlled by the boundary sublattice termination. Owing to the symmetry constraints and the robustness of chiral states, these findings hold universally across all topological AMs. A general framework is established for controlling topological corner states, offering a new strategy for designing magnetic materials with tailored non-Hermitian properties. △ Less

Submitted 19 March, 2026; originally announced March 2026.

Comments: 8 pages,5figures

Lee-Yang Zeros and Pseudocritical Drift in J-Q Néel-VBS Transitions

Authors: Chunhao Guo, Zhe Wang, Danhe Wang, Zenan Liu, Haiyuan Zou, Zheng Yan

Abstract: Square-lattice J-Q models provide a sign-problem-free setting for probing the quantum phase transition between Néel antiferromagnet and columnar valence-bond solid. We analyze this transition through the scaling of Lee-Yang zeros, computed within stochastic series expansion quantum Monte Carlo by reweighting configurations sampled near criticality in the presence of complex source fields. Benchmar… ▽ More Square-lattice J-Q models provide a sign-problem-free setting for probing the quantum phase transition between Néel antiferromagnet and columnar valence-bond solid. We analyze this transition through the scaling of Lee-Yang zeros, computed within stochastic series expansion quantum Monte Carlo by reweighting configurations sampled near criticality in the presence of complex source fields. Benchmark studies of the dimerized Heisenberg model and the checkerboard J-Q model validate the method, yielding stable O(3) critical scaling in the former and clear spacetime-volume scaling in the latter, as expected for a first-order transition. Applying the same analysis to the J-Q models, we find a pronounced and systematic drift of the leading-zero scaling with increasing system size, consistent with an extended pseudocritical regime. The Lee-Yang scaling implies an effective scaling dimension of the SO(5) order-parameter field that decreases with size and is consistent with vanishing in the thermodynamic limit. Such behavior lies below the scalar unitarity bound of any unitary relativistic conformal field theory in 2+1 dimensions and enforces inverse spacetime-volume scaling of the zeros, the hallmark of a first-order transition. These results support a weakly first-order interpretation of the Néel-VBS transition and establish finite-size Lee-Yang zeros as a sensitive, symmetry-resolved diagnostic of pseudocriticality and transition order in the J-Q family. △ Less

Submitted 29 March, 2026; v1 submitted 16 March, 2026; originally announced March 2026.

Tunable decoupling of coexisting magnetic orders in Co$_{1/3}$TaS$_2$

Authors: Yining Hu, Zili Feng, Takashi Kurumaji, Linda Ye, Chunyu Mark Guo, Philip J. W. Moll

Abstract: In multiferroics, new physical responses and functionalities emerge when symmetry-distinct order parameters couple. This conventionally occurs when lattice and magnetic degrees of freedom order independently in a material. Here, we report an all-magnetic analogue of multiferroic behavior in the antiferromagnet Co$_{1/3}$TaS$_2$, where topological scalar spin chirality and nematicity coexist on the… ▽ More In multiferroics, new physical responses and functionalities emerge when symmetry-distinct order parameters couple. This conventionally occurs when lattice and magnetic degrees of freedom order independently in a material. Here, we report an all-magnetic analogue of multiferroic behavior in the antiferromagnet Co$_{1/3}$TaS$_2$, where topological scalar spin chirality and nematicity coexist on the same spin lattice. While the chiral spin texture generates an anomalous Hall effect (AHE), the nematic order breaks threefold rotational symmetry and dominates longitudinal transport. Crucially, in zero field these symmetry-distinct orders merely coexist yet magnetic fields induce strong coupling between them, thus realizing a new type of multiferroic bebhavior via tuning of the coupling itself instead of direct manipulation of secondary orders. In sub-domain sized devices with achiral geometry, we demonstrate that nonreciprocal transport serves as a symmetry-based probe of the global spin chirality, co-aligned with the strong topological AHE of the system. In Co$_{1/3}$TaS$_2$ the topological Hall state inherits a large resistance anomaly via chiral-nematic coupling, thus our results showcase how hybrid magnetic orders can achieve advanced functionalities by merging symmetry-forbidden material responses. △ Less

Submitted 12 March, 2026; originally announced March 2026.

Comments: 25 pages, 13 figures

Universal and non-universal contributions of entanglement under different bipartitions

Authors: Zhe Wang, Chunhao Guo, Bin-Bin Mao, Zheng Yan

Abstract: Entanglement entropy (EE) is a fundamental probe of quantum phases and critical phenomena, which was thought to reflect only bulk universality for a long time. Very recently, people realized that the microscopic geometry of the entanglement cut can induce distinct entanglement-edge modes, whose coupling to bulk critical fluctuations may alter the scaling of the EE. However, this perception is very… ▽ More Entanglement entropy (EE) is a fundamental probe of quantum phases and critical phenomena, which was thought to reflect only bulk universality for a long time. Very recently, people realized that the microscopic geometry of the entanglement cut can induce distinct entanglement-edge modes, whose coupling to bulk critical fluctuations may alter the scaling of the EE. However, this perception is very qualitative and lacks quantitative consideration. Here, we investigate this problem through high-precision quantum Monte Carlo simulations combined with the analysis of scaling theory to build a quantitative understanding. By considering three distinct bipartitions corresponding to three surface criticality types, we reveal a striking dependence of the constant term γ on the microscopic cut at the quantum critical point. Notably, cuts that generate extra gapless edge modes yield a sign reversal in γ compared to those producing gapped edges. We explain this behavior via a modified scaling form that incorporates contributions from both bulk and surface critical modes. Furthermore, we demonstrate that the derivative of EE robustly extracts the bulk critical point and exponent ν regardless of the cut geometry, providing a reliable diagnostic of bulk universality in the presence of strong surface effects. Our work for the first time establishes a direct quantitative connection between surface criticality and entanglement scaling, challenging the conventional view that EE solely reflects bulk properties and offering a refined framework for interpreting entanglement in systems with boundary-sensitive criticality. △ Less

Submitted 18 January, 2026; originally announced January 2026.

Comments: 6 pages, 3 figures

Optimal universal bounds for waves with varied coherence based on supremum and infimum coherence spectra

Authors: Shiyu Li, Cheng Guo

Abstract: We establish a majorization-based theory for bounding observables of waves with varied coherence. For any measurement, exact bounds are attained by the maximal and minimal elements in the set of input coherence spectra. The set's supremum and infimum, which may lie outside the set, provide optimal universal bounds: any alternative spectrum yielding universal bounds produces weaker constraints. We… ▽ More We establish a majorization-based theory for bounding observables of waves with varied coherence. For any measurement, exact bounds are attained by the maximal and minimal elements in the set of input coherence spectra. The set's supremum and infimum, which may lie outside the set, provide optimal universal bounds: any alternative spectrum yielding universal bounds produces weaker constraints. We present an algorithm to compute the supremum and infimum, and prove that they lie either at singular boundary points or strictly outside the set of coherence spectra. △ Less

Submitted 15 January, 2026; originally announced January 2026.

Comments: 19 pages, 12 figures, including appendices

Migration of gold atoms into a thiol-bonded molecular self-assembled monolayer, forming a cluster exhibiting a Coulomb staircase

Authors: Bingxin Li, Shanglong Ning, Chunyang Miao, Chenyang Guo, Gyu Don Kong, Xintai Wang, Victor I. Coldea, Yuqiao Li, Sam Harley, Oleg V. Kolosov, James Newson, Sam P. Jarvis, Ben J. Robinson, Mohammed Alzanbaqi, Ali Ismael, Colin J. Lambert, Hyo Jae Yoon, Jeremy J. Baumberg, Christopher J. B. Ford

Abstract: Thiol-based self-assembled monolayers (SAMs) on gold surfaces are one of the fundamental building blocks of molecular electronics. The strong chemical affinity of the gold and sulfur (Au-S) enables the formation of close-packed SAMs, but it also has recently been found to create a dynamic interface where surface reconstruction can occur under illumination, even with ambient light. This reconstruct… ▽ More Thiol-based self-assembled monolayers (SAMs) on gold surfaces are one of the fundamental building blocks of molecular electronics. The strong chemical affinity of the gold and sulfur (Au-S) enables the formation of close-packed SAMs, but it also has recently been found to create a dynamic interface where surface reconstruction can occur under illumination, even with ambient light. This reconstruction may facilitate migration of gold atoms, potentially leading to in-situ formation of gold clusters. However, research on this mechanism often centers on Au(111) crystalline surfaces and flicker-noise measurements. Electron transport in ensembles of molecules in lithographically defined junctions has remained largely unexplored at cryogenic temperatures. In this study, we observe single-electron phenomena characterized by reproducible Coulomb staircases across various long-chain alkanethiol SAMs, which fit the Coulomb-blockade theory of nm-sized metallic nanoparticles. We find no such current steps in samples with amine, rather than thiol, anchors. Additionally, we find that by adding a bipyridyl functional group, these phenomena can be harnessed for memristive switching and negative differential resistance. These findings indicate that the generally observed lack of reliability and reproducibility of molecular devices may be alleviated by using amine anchors instead of thiols to avoid nanoparticle effects. Conversely, the spontaneous formation of the nanoparticles could potentially be controlled and used to achieve useful functionalities, offering new pathways for designing multifunctional nanoelectronic components. △ Less

Submitted 21 December, 2025; originally announced December 2025.

Phase-field simulation of domain switching in ferroelectric trilayer films under bending-induced strain gradient

Authors: Changqing Guo, Letao Yang, Jing Wang, Houbing Huang

Abstract: Flexible ferroelectrics possess significant potential for wearable electronics and bio-inspired devices, yet their electromechanical coupling mechanisms under dynamic bending remain elusive. This study employs phase-field simulations to investigate the effects of bending deformation on domain structures and macroscopic ferroelectric responses in (SrTiO3)10/(PbTiO3)10/(SrTiO3)10 trilayer films. By… ▽ More Flexible ferroelectrics possess significant potential for wearable electronics and bio-inspired devices, yet their electromechanical coupling mechanisms under dynamic bending remain elusive. This study employs phase-field simulations to investigate the effects of bending deformation on domain structures and macroscopic ferroelectric responses in (SrTiO3)10/(PbTiO3)10/(SrTiO3)10 trilayer films. By constructing computational models for upward-concave (U-shaped) and downward-concave (N-shaped) configurations, we analyze the regulation of polarization patterns by strain distributions under varying curvature radii. The results demonstrate that the two bending modes generate opposite through-thickness strain gradients: U-shaped bending produces compressive strain in the upper layer and tensile strain in the lower, while N-shaped bending yields the reverse. These inhomogeneous strains drive distinct polarization reconfigurations within the PTO layer. While stable vortex-antivortex pairs persist at moderate curvatures, reducing the bending radius triggers divergent topological transitions -- U-shaped bending transforms vortex pairs into zigzag-like domains, whereas N-shaped bending promotes out-of-plane c-domain evolution. Crucially, bending-induced strain gradients generate transverse flexoelectric fields that markedly modulate hysteresis loops. U-shaped bending introduces a negative flexoelectric field, shifting loops rightward and suppressing maximum polarization Pmax. In contrast, N-shaped bending generates a positive field, shifting loops leftward and enhancing Pmax. Furthermore, analysis of polarization switching reveals that bending mediates domain-evolution pathways and reversal dynamics. △ Less

Submitted 14 December, 2025; originally announced December 2025.

Comments: 19 pages, 7 figures, published in Acta Physica Sinica

Journal ref: Acta Phys. Sin., 2025, 74(12): 127501

Hierarchical geometric deep learning enables scalable analysis of molecular dynamics

Authors: Zihan Pengmei, Spencer C. Guo, Chatipat Lorpaiboon, Aaron R. Dinner

Abstract: Molecular dynamics simulations can generate atomically detailed trajectories of complex systems, but analyzing these dynamics can be challenging when systems lack well-established quantitative descriptors (features). Graph neural networks (GNNs) in which messages are passed between nodes that represent atoms that are spatial neighbors promise to obviate manual feature engineering, but the use of G… ▽ More Molecular dynamics simulations can generate atomically detailed trajectories of complex systems, but analyzing these dynamics can be challenging when systems lack well-established quantitative descriptors (features). Graph neural networks (GNNs) in which messages are passed between nodes that represent atoms that are spatial neighbors promise to obviate manual feature engineering, but the use of GNNs with biomolecular systems of more than a few hundred residues has been limited in the context of analyzing dynamics by both difficulties in capturing the details of long-range interactions with message passing and the memory and runtime requirements associated with large graphs. Here, we show how local information can be aggregated to reduce memory and runtime requirements without sacrificing atomic detail. We demonstrate that this approach opens the door to analyzing simulations of protein-nucleic acid complexes with thousands of residues on single GPUs within minutes. For systems with hundreds of residues, for which there are sufficient data to make quantitative comparisons, we show that the approach improves performance and interpretability. △ Less

Submitted 6 December, 2025; originally announced December 2025.

Comments: 17 pages, 12 figures

Emergent long-tail dynamics in driven magnets with dynamical frustration

Authors: Chenyue Guo, Hongzheng Zhao, Zi Cai

Abstract: In this study, we show that dynamical frustration can spontaneously emerge in frustration-free magnetic systems under periodic driving. Specifically, we consider a classical spin system and demonstrate the emergence of spin-ice physics when drive-induced heating is well suppressed. In particular, we focus on the dynamics of magnetic monopole excitations, which, in sharp contrast to their equilibri… ▽ More In this study, we show that dynamical frustration can spontaneously emerge in frustration-free magnetic systems under periodic driving. Specifically, we consider a classical spin system and demonstrate the emergence of spin-ice physics when drive-induced heating is well suppressed. In particular, we focus on the dynamics of magnetic monopole excitations, which, in sharp contrast to their equilibrium counterparts, exhibit a non-ergodic stochastic random-walk process with long-tailed, power-law distributed waiting times, where the power-law exponent is tunable by the system's effective temperature. Heating is accelerated at intermediate driving frequencies, and the system eventually heats up to an infinite-temperature state. However, the heating time is extremely sensitive to different initial-state realizations and also follows a long-tailed power-law distribution. We show that a drive-induced short-range attractive interaction between monopoles is responsible for the long-tailed distributions observed in both monopole and heating dynamics. △ Less

Submitted 12 November, 2025; originally announced November 2025.

Joint control of coherent transmission, reflection, and absorption

Authors: Shiyu Li, Dongha Kim, Shanhui Fan, Cheng Guo

Abstract: Controlling multiple wave properties simultaneously poses a key challenge in coherent control of wave transport. We present a theory for joint coherent control of transmission, reflection, and absorption in linear systems. We prove that the numerical range provides the mathematical structure governing achievable responses, and reveal non-abelian effects due to non-commutativity between transmissio… ▽ More Controlling multiple wave properties simultaneously poses a key challenge in coherent control of wave transport. We present a theory for joint coherent control of transmission, reflection, and absorption in linear systems. We prove that the numerical range provides the mathematical structure governing achievable responses, and reveal non-abelian effects due to non-commutativity between transmission, reflection, and absorption matrices. We provide an algorithm to achieve arbitrary target responses. Our results establish a theoretical foundation for joint coherent control of waves. △ Less

Submitted 6 November, 2025; originally announced November 2025.

Comments: 12 pages, 7 figures, including appendices

Journal ref: Physical Review B 112, 245421 (2025)

Probability Distribution for Coherent Transport of Random Waves

Authors: Yunrui Wang, Cheng Guo

Abstract: We establish a comprehensive probability theory for coherent transport of random waves through arbitrary linear media. The transmissivity distribution for random coherent waves is a fundamental B-spline with knots at the transmission eigenvalues. We analyze the distribution's shape, bounds, moments, and asymptotic behaviors. In the large n limit, the distribution converges to a Gaussian whose mean… ▽ More We establish a comprehensive probability theory for coherent transport of random waves through arbitrary linear media. The transmissivity distribution for random coherent waves is a fundamental B-spline with knots at the transmission eigenvalues. We analyze the distribution's shape, bounds, moments, and asymptotic behaviors. In the large n limit, the distribution converges to a Gaussian whose mean and variance depend solely on those of the eigenvalues. This result resolves the apparent paradox between bimodal eigenvalue distribution and unimodal transmissivity distribution. △ Less

Submitted 6 November, 2025; originally announced November 2025.

Comments: 9 pages, 6 figures, including supplementary material

Improved time-translationally invariant tensor network influence functional method for Anderson impurity problems

Authors: Zhijie Sun, Zhenyu Li, Chu Guo

Abstract: The Anderson impurity model (AIM) is of fundamental importance in condensed matter physics for studying strongly correlated phenomena. However, accurately simulating its long-time dynamics still remains a significant numerical challenge. A class of recently developed numerical approaches represents the Feynman-Vernon influence functional (IF), which encodes all the bath effects on the impurity, as… ▽ More The Anderson impurity model (AIM) is of fundamental importance in condensed matter physics for studying strongly correlated phenomena. However, accurately simulating its long-time dynamics still remains a significant numerical challenge. A class of recently developed numerical approaches represents the Feynman-Vernon influence functional (IF), which encodes all the bath effects on the impurity, as a matrix product state (MPS) in the temporal domain. The computational cost of this approach is largely determined by the bond dimension $χ$ of the temporal MPS. In this work, we propose an efficient and accurate method that, when the hybridization function in the IF can be approximated as a sum of $n$ exponential functions, systematically constructs the IF as an MPS by multiplying $O(n)$ small MPSs, each with bond dimension $2$. Our method yields a worst case scaling of $χ$ as $2^{8n}$ and $2^{2n}$ for real- and imaginary-time evolution respectively. We demonstrate the performance of our method for two commonly used bath spectral functions, and show that the required bond dimensions are significantly smaller than the worst case. △ Less

Submitted 30 June, 2026; v1 submitted 13 October, 2025; originally announced October 2025.

Comments: 15 pages, 5 figures

Monitoring Nitric Oxide in Trigeminal Neuralgia Rats with a Cerium Single-Atom Nanozyme Electrochemical Biosensor

Authors: Kangling Tian, Fuhua Li, Ran Chen, Shihong Chen, Wenbin Wei, Yihang Shen, Muzi Xu, Chunxian Guo, Luigi G. Occhipinti, Hong Bin Yang, Fangxin Hu

Abstract: Trigeminal neuralgia (TN) is the most common neuropathic disorder; however, its pathogenesis remains unclear. A prevailing theory suggests that nitric oxide (NO) may induce nerve compression and irritation via vascular dilation, thereby being responsible for the condition, making real-time detection of generated NO critical. However, traditional evaluations of NO rely on indirect colorimetric or c… ▽ More Trigeminal neuralgia (TN) is the most common neuropathic disorder; however, its pathogenesis remains unclear. A prevailing theory suggests that nitric oxide (NO) may induce nerve compression and irritation via vascular dilation, thereby being responsible for the condition, making real-time detection of generated NO critical. However, traditional evaluations of NO rely on indirect colorimetric or chemiluminescence techniques, which offer limited sensitivity and spatial resolution for its real-time assessment in biological environments. Herein, we reported the development of a highly sensitive NO electrochemical biosensor based cerium single-atom nanozyme (Ce1-CN) with ultrawide linear range from 1.08 nM to 143.9 μM, and ultralow detection limit of 0.36 nM, which enables efficient and real-time evaluation of NO in TN rats. In-situ attenuated total reflection surface-enhanced infrared spectroscopy combined with density functional theory calculations revealed the high-performance biosensing mechanism, whereby the Ce centers in Ce1-CN nanoenzymes adsorb NO and subsequently react with OH- to form *HNO2. Results demonstrated that NO concentration was associated with TN onset. Following carbamazepine treatment, NO production from nerves decreased, accompanied by an alleviation of pain. These findings indicate that the biosensor serves as a valuable tool for investigating the pathogenesis of TN and guiding subsequent therapeutic strategies. △ Less

Submitted 22 September, 2025; originally announced September 2025.

Scalable tensor network algorithm for quantum impurity problems

Authors: Zhijie Sun, Ruofan Chen, Zhenyu Li, Chu Guo

Abstract: The Grassmann time-evolving matrix product operator method has shown great potential as a general-purpose quantum impurity solver, as its numerical errors can be well-controlled and it is flexible to be applied on both the imaginary- and real-time axis. However, a major limitation of it is that its computational cost grows exponentially with the number of impurity flavors. In this work, we propose… ▽ More The Grassmann time-evolving matrix product operator method has shown great potential as a general-purpose quantum impurity solver, as its numerical errors can be well-controlled and it is flexible to be applied on both the imaginary- and real-time axis. However, a major limitation of it is that its computational cost grows exponentially with the number of impurity flavors. In this work, we propose a multi-flavor extension of it to overcome this limitation. The key insight is that to calculate multi-time correlation functions on one or a few impurity flavors, one could integrate out the degrees of freedom of the rest flavors before hand, which could greatly simplify the calculation. The idea is particularly effective for quantum impurity problems with diagonal hybridization function, i.e., each impurity flavor is coupled to an independent bath, a setting which is commonly used in the field. We demonstrate the accuracy and scalability of our method for the imaginary time evolution of impurity problems with up to three impurity orbitals, i.e., 6 flavors, and benchmark our results against continuous-time quantum Monte Carlo calculations. Our method paves the way of scaling up tensor network algorithms to solve large-scale quantum impurity problems. △ Less

Submitted 7 October, 2025; v1 submitted 16 July, 2025; originally announced July 2025.

Comments: 12 pages, 6 figures

Journal ref: Phys. Rev. B 112, 155115 (2025)

Hetero-Orbital Two-Component Fractional Quantum Hall States in Bilayer Graphene

Authors: Ke Huang, Ajit C. Balram, Hailong Fu, Chengqi Guo, Kenji Watanabe, Takashi Taniguchi, Jainendra K. Jain, Jun Zhu

Abstract: A two-dimensional electron system exposed to a strong magnetic field produces a plethora of strongly interacting fractional quantum Hall (FQH) states, the complex topological orders of which are revealed through exotic emergent particles, such as composite fermions, fractionally charged Abelian and non-Abelian anyons. Much insight has been gained by the study of multi-component FQH states, where s… ▽ More A two-dimensional electron system exposed to a strong magnetic field produces a plethora of strongly interacting fractional quantum Hall (FQH) states, the complex topological orders of which are revealed through exotic emergent particles, such as composite fermions, fractionally charged Abelian and non-Abelian anyons. Much insight has been gained by the study of multi-component FQH states, where spin and pseudospin indices of the electron contribute additional correlation. Traditional multi-component FQH states develop in situations where the components share the same orbital states and the resulting interactions are pseudospin independent; this homo-orbital nature was also crucial to their theoretical understanding. Here, we study "hetero-orbital" two-component FQH states, in which the orbital index is part of the pseudospin, rendering the multi-component interactions strongly SU(2) anisotropic in the pseudospin space. Such states, obtained in bilayer graphene at the isospin transition between N = 0 and N = 1 electron Landau levels, are markedly different from previous homo-orbital two-component FQH states. In particular, we observe strikingly different behaviors for the parallel-flux and reverse-flux composite fermion states, and an anomalously strong two-component 2/5 state over a wide range of magnetic field before it abruptly disappears at a high field. Our findings, combined with detailed theoretical calculations, reveal the surprising robustness of the hetero-orbital FQH effects, significantly enriching our understanding of FQH physics in this novel regime. △ Less

Submitted 26 July, 2025; v1 submitted 17 June, 2025; originally announced June 2025.

Comments: 21 pages, 12 figures including appendices

Journal ref: Phys. Rev. X 15, 031023 (2025)

Putative excitonic insulating state in narrow-gap semiconductor La$_3$Cd$_2$As$_6$

Authors: Caitlin S. Kengle, Noah Schnitzer, Elizabeth A. Peterson, Chunyu Guo, Ling Zhang, Matthew S. Cook, Jian-Xin Zhu, Sean M. Thomas, Philip J. W. Moll, Filip Ronning, Priscila F. S. Rosa

Abstract: Excitonic insulators are electronically-driven phases of matter characterized by the spontaneous condensation of electron-hole pairs. Here we show that La$_3$Cd$_2$As$_6$ undergoes a transition at $T_{0}=278$ K to a highly insulating state with no accompanying structural transition. We observe quasi-two-dimensional electrical transport and charge fluctuations consistent with an electronic transiti… ▽ More Excitonic insulators are electronically-driven phases of matter characterized by the spontaneous condensation of electron-hole pairs. Here we show that La$_3$Cd$_2$As$_6$ undergoes a transition at $T_{0}=278$ K to a highly insulating state with no accompanying structural transition. We observe quasi-two-dimensional electrical transport and charge fluctuations consistent with an electronic transition enabled by enhanced Coulomb interactions. Density functional theory calculations are unable to replicate the insulating ground state. Our results support the opening of a gap by excitonic effects at $T_{0}$, placing La$_3$Cd$_2$As$_6$ as a rare example of a bulk excitonic insulator. △ Less

Submitted 10 June, 2025; originally announced June 2025.

Comments: LA-UR-25-25525

Symmetry-broken ground state and phonon mediated superconductivity in Kagome CsV$_3$Sb$_5$

Authors: Manex Alkorta, Martin Gutierrez-Amigo, Ðorđe Dangić, Chunyu Guo, Philip J. W. Moll, Maia G. Vergniory, Ion Errea

Abstract: The newly discovered family of non-magnetic Kagome metals AV$_3$Sb$_5$ (A=K,Rb,Cs) provides a unique platform for exploring the interplay between charge density wave (CDW) order, superconductivity, non-trivial topology, and spontaneous time-reversal symmetry breaking. Although characterizing the CDW phase is essential for understanding and modeling these exotic phenomena, its nature remains unreso… ▽ More The newly discovered family of non-magnetic Kagome metals AV$_3$Sb$_5$ (A=K,Rb,Cs) provides a unique platform for exploring the interplay between charge density wave (CDW) order, superconductivity, non-trivial topology, and spontaneous time-reversal symmetry breaking. Although characterizing the CDW phase is essential for understanding and modeling these exotic phenomena, its nature remains unresolved. In this work, we employ first-principles free-energy calculations, accounting for both ionic kinetic energy and anharmonic effects, to resolve the atomistic phase diagram of CsV$_3$Sb$_5$ and its charge ordering structure. Our results uncover that the CDW ground state is formed by reconstructed vanadium Kagome layers in a triangular hexagonal pattern, featuring energetically degenerate different stacking orders. This accounts for the various out-of-plane modulations observed experimentally and supports the coexistence of multiple domains. The discovered symmetry-broken ground state is consistent with the absence of any electronic anisotropy in transport experiments. By combining anharmonic phonons with the calculation of electron-phonon matrix elements, we predict a superconducting critical temperature for the CDW phase in agreement with experiments, showing that superconductivity is phonon mediated. These findings not only resolve a long-standing structural puzzle, but also clarify the impact of the CDW in superconductivity, highlighting its fundamental importance in shaping the low-temperature quantum phase diagram of Kagome metals. △ Less

Submitted 21 August, 2025; v1 submitted 26 May, 2025; originally announced May 2025.

Comments: 8 pages, 5 figures

Journal ref: Phys. Rev. Lett. 136, 206401 (2026)

Tuning Topological States by Dissipation

Authors: Xue-Ping Ren, Yue Hu, Long-Ye Lu, Xin-Ran Ma, Ji-Yao Fan, Cui-Xian Guo, Su-Peng Kou

Abstract: The bulk-boundary correspondence plays a crucial role in topological quantum systems, however,this principle is broken in non-Hermitian systems. The breakdown of the bulk-boundary correspondence indicates that the global phase diagrams under open boundary conditions are significantly different from those under periodic boundary conditions. In this paper, we investigate how the bulk-boundary corres… ▽ More The bulk-boundary correspondence plays a crucial role in topological quantum systems, however,this principle is broken in non-Hermitian systems. The breakdown of the bulk-boundary correspondence indicates that the global phase diagrams under open boundary conditions are significantly different from those under periodic boundary conditions. In this paper, we investigate how the bulk-boundary correspondence breaks down by gradually tearing the system. We find that by tuning the strength of gain and loss domain wall, in the thermodynamic limit, the global phase diagrams of the topological system become the hybrids of those under periodic and open boundary conditions. Moreover, during the breakdown of the bulk-boundary correspondence, several phase transitions occur. This situation is quite different from earlier work, where the breakdown of the bulk-boundary correspondence in the thermodynamic limit occurred suddenly due to infinitesimal boundary hopping amplitudes. To support our conclusions, we provide both analytical and numerical calculations. These results help researchers better understand non-Hermitian topological systems. △ Less

Submitted 22 May, 2025; originally announced May 2025.

Comments: 15 pages, 7 figures, submitted to Physical Review B on May 13, 2025

A Unified Framework for the Non-Hermitian Localization: Boundary-Insensitive Modes and Electric-Magnetic Analogy

Authors: Zheng Wei, Ji-Yao Fan, Kui Cao, Xin-Ran Ma, Cui-Xian Guo, Xue-Ping Ren, Su-Peng Kou

Abstract: The non-Hermitian skin effect is fundamentally characterized by its sensitivity to boundary conditions, reflected in changes to the energy spectrum and boundary-localized eigenstates. Here, we demonstrate that a spatially inhomogeneous imaginary scalar potential field induces a skin effect that is insensitive to boundary conditions. Both the spectrum and eigenstate distribution remain invariant, a… ▽ More The non-Hermitian skin effect is fundamentally characterized by its sensitivity to boundary conditions, reflected in changes to the energy spectrum and boundary-localized eigenstates. Here, we demonstrate that a spatially inhomogeneous imaginary scalar potential field induces a skin effect that is insensitive to boundary conditions. Both the spectrum and eigenstate distribution remain invariant, a behavior not captured by existing theories. We attribute this anomaly to translational symmetry breaking induced by spatially varying imaginary potentials in finite systems. We further formulate a theory that universally predicts localization in single-particle non-Hermitian systems. This framework classifies skin effects into two fundamental types: electric, driven by imaginary scalar potentials, and magnetic, driven by imaginary vector potentials, and reveals a phase transition between them, where eigenstates become fully delocalized. Our work provides a unified theory for non-Hermitian localization, allowing full control over skin modes via potential engineering in various platforms like photonic crystals and cold-atom systems. △ Less

Submitted 15 May, 2026; v1 submitted 15 May, 2025; originally announced May 2025.

Phonon-Assisted Radiative Lifetimes and Exciton Dynamics from First Principles

Authors: Chunhao Guo, Gabriele Riva, Jacopo Simoni, Junqing Xu, Yuan Ping

Abstract: Exciton-phonon interactions play a fundamental role in phonon-assisted radiative recombination and exciton dynamics in solids. In this work, we present a first-principles framework for computing phonon-assisted radiative lifetimes and exciton dynamics at finite temperatures. Starting from the solution of the Bethe-Salpeter equation, we construct an effective excitonic Hamiltonian that incorporates… ▽ More Exciton-phonon interactions play a fundamental role in phonon-assisted radiative recombination and exciton dynamics in solids. In this work, we present a first-principles framework for computing phonon-assisted radiative lifetimes and exciton dynamics at finite temperatures. Starting from the solution of the Bethe-Salpeter equation, we construct an effective excitonic Hamiltonian that incorporates both exciton-photon and exciton-phonon interactions. Phonon-assisted radiative lifetimes in anisotropic media are evaluated using time-dependent second-order perturbation theory. We further analyze the temperature and phonon-mode dependence of phonon-assisted radiative lifetime and compare our results with available experimental data. We explain the nonmonotonic temperature dependence of the phonon-assisted radiative lifetime by different mechanisms at low and high-temperature regimes. Finally, we perform real-time exciton relaxation at the diagonal approximation of Lindbladian dynamics for time-resolved exciton occupation, providing insights into ultrafast thermalization and scattering pathways. Our ab-initio theory offers a detailed microscopic understanding of phonon-mediated exciton relaxation and recombination processes, and provides in-depth perspectives on phonon-assisted many-body interactions and their influence on optical properties for light-emitting and optoelectronic applications. △ Less

Submitted 25 April, 2025; originally announced April 2025.

Electronic dimensionality of UTe2

Authors: L. Zhang, C. Guo, D. Graf, C. Putzke, M. M. Bordelon, E. D. Bauer, S. M. Thomas, F. Ronning, P. F. S. Rosa, P. J. W. Moll

Abstract: Superconductivity in the heavy-fermion metal UTe2 survives the application of very high magnetic fields, presenting both an intriguing puzzle and an experimental challenge. The strong, non-perturbative influence of the magnetic field complicates the determination of superconducting order parameters in the high-field phases. Here, we report electronic transport anisotropy measurements in precisely… ▽ More Superconductivity in the heavy-fermion metal UTe2 survives the application of very high magnetic fields, presenting both an intriguing puzzle and an experimental challenge. The strong, non-perturbative influence of the magnetic field complicates the determination of superconducting order parameters in the high-field phases. Here, we report electronic transport anisotropy measurements in precisely aligned microbars in magnetic fields to 45 T applied along the b-axis. Our results reveal a highly directional vortex pinning force in the field-reinforced phase. The critical current is significantly suppressed for currents along the c direction, whereas the flux-flow voltage is reduced with slight angular misalignments--hallmarks of vortex lock-in transitions typically seen in quasi-2D superconductors like cuprates and pnictides. These findings challenge the assumption of nearly isotropic charge transport in UTe2 and point to enhanced two-dimensionality in the high-field state, consistent with a change in the order parameter. A pair-density-wave-like state at high fields could naturally induce a layered modulation of the superfluid density, forming planar structures that confine vortices and guide their sliding in the flux-flow regime. △ Less

Submitted 21 April, 2025; originally announced April 2025.

Roadmap on Nonlocality in Photonic Materials and Metamaterials

Authors: Francesco Monticone, N. Asger Mortensen, Antonio I. Fernández-Domínguez, Yu Luo, Xuezhi Zheng, Christos Tserkezis, Jacob B. Khurgin, Tigran V. Shahbazyan, André J. Chaves, Nuno M. R. Peres, Gino Wegner, Kurt Busch, Huatian Hu, Fabio Della Sala, Pu Zhang, Cristian Ciracì, Javier Aizpurua, Antton Babaze, Andrei G. Borisov, Xue-Wen Chen, Thomas Christensen, Wei Yan, Yi Yang, Ulrich Hohenester, Lorenz Huber , et al. (41 additional authors not shown)

Abstract: Photonic technologies continue to drive the quest for new optical materials with unprecedented responses. A major frontier in this field is the exploration of nonlocal (spatially dispersive) materials, going beyond the local, wavevector-independent assumption traditionally made in optical material modeling. On one end, the growing interest in plasmonic, polaritonic and quantum materials has reveal… ▽ More Photonic technologies continue to drive the quest for new optical materials with unprecedented responses. A major frontier in this field is the exploration of nonlocal (spatially dispersive) materials, going beyond the local, wavevector-independent assumption traditionally made in optical material modeling. On one end, the growing interest in plasmonic, polaritonic and quantum materials has revealed naturally occurring nonlocalities, emphasizing the need for more accurate models to predict and design their optical responses. This has major implications also for topological, nonreciprocal, and time-varying systems based on these material platforms. Beyond natural materials, artificially structured materials--metamaterials and metasurfaces--can provide even stronger and engineered nonlocal effects, emerging from long-range interactions or multipolar effects. This is a rapidly expanding area in the field of photonic metamaterials, with open frontiers yet to be explored. In the case of metasurfaces, in particular, nonlocality engineering has become a powerful tool for designing strongly wavevector-dependent responses, enabling enhanced wavefront control, spatial compression, multifunctional devices, and wave-based computing. Furthermore, nonlocality and related concepts play a critical role in defining the ultimate limits of what is possible in optics, photonics, and wave physics. This Roadmap aims to survey the most exciting developments in nonlocal photonic materials, highlight new opportunities and open challenges, and chart new pathways that will drive this emerging field forward--toward new scientific discoveries and technological advancements. △ Less

Submitted 28 March, 2025; v1 submitted 1 March, 2025; originally announced March 2025.

Journal ref: Optical Materials Express 15, 1544 (2025)

Cryogen-free low-temperature photoemission electron microscopy for high-resolution nondestructive imaging of electronic phases

Authors: Chen Wang, Shaoshan Wang, Chuan Guo, Chengjian Yu, Qi Fu, Xiaopeng Xie, Changxi Zheng

Abstract: Quantum materials exhibit phases such as superconductivity at low temperatures, yet imaging their phase transition dynamics with high spatial resolution remains challenging due to conventional tools' limitations - scanning tunneling microscopy offers static snapshots, while transmission electron microscopy lacks band sensitivity. Photoemission electron microscopy (PEEM) can resolve band structures… ▽ More Quantum materials exhibit phases such as superconductivity at low temperatures, yet imaging their phase transition dynamics with high spatial resolution remains challenging due to conventional tools' limitations - scanning tunneling microscopy offers static snapshots, while transmission electron microscopy lacks band sensitivity. Photoemission electron microscopy (PEEM) can resolve band structures in real/reciprocal spaces rapidly, but suffering from insufficient resolution for (near)atomic-scale quantum physics due to the unstable cooling designs. Here, we developed cryogen-free low-temperature PEEM (CFLT-PEEM) achieving 21.1 K stably. CFLT-PEEM attains a record-breaking resolution of 4.48 nm without aberration correction, enabling direct visualization of surface-state distribution characteristics along individual atomic steps. The advancement lies in narrowing the segment of band structures for imaging down to 160 meV, which minimizes the chromatic aberration of PEEM. CFLT-PEEM enables rapid, nondestructive high-resolution imaging of cryogenic electronic structures, positioning it as a powerful tool for physics and beyond. △ Less

Submitted 1 March, 2025; originally announced March 2025.

Comments: This submission is a single PDF file containing the main text and Supplementary Information. The document is 23 pages long and includes 12 figures. The Supplementary Information begins on page 15

Infinite Grassmann time-evolving matrix product operators for quantum impurity problems after a quench

Authors: Zhijie Sun, Ruofan Chen, Zhenyu Li, Chu Guo

Abstract: An emergent numerical approach to solve quantum impurity problems is to encode the impurity path integral as a matrix product state. For time-dependent problems, the cost of this approach generally scales with the evolution time. Here we consider a common non-equilibrium scenario where an impurity, initially in equilibrium with a thermal bath, is driven out of equilibrium by a sudden quench of the… ▽ More An emergent numerical approach to solve quantum impurity problems is to encode the impurity path integral as a matrix product state. For time-dependent problems, the cost of this approach generally scales with the evolution time. Here we consider a common non-equilibrium scenario where an impurity, initially in equilibrium with a thermal bath, is driven out of equilibrium by a sudden quench of the impurity Hamiltonian. Despite that there is no time-translational invariance in the problem, we show that we could still make full use of the infinite matrix product state technique, resulting in a method whose cost is essentially independent of the evolution time. We demonstrate the effectiveness of this method in the integrable case against exact diagonalization, and against existing calculations on the L-shaped Kadanoff-Baym contour in the general case. Our method could be a very competitive method for studying long-time non-equilibrium quantum dynamics, and be potentially used as an efficient impurity solver in the non-equilibrium dynamical mean field theory. △ Less

Submitted 25 August, 2025; v1 submitted 5 December, 2024; originally announced December 2024.

Comments: 13 pages, 10 figures

Journal ref: Phys. Rev. B, 112, 125145 (2025)

Emergence of steady quantum transport in a superconducting processor

Authors: Pengfei Zhang, Yu Gao, Xiansong Xu, Ning Wang, Hang Dong, Chu Guo, Jinfeng Deng, Xu Zhang, Jiachen Chen, Shibo Xu, Ke Wang, Yaozu Wu, Chuanyu Zhang, Feitong Jin, Xuhao Zhu, Aosai Zhang, Yiren Zou, Ziqi Tan, Zhengyi Cui, Zitian Zhu, Fanhao Shen, Tingting Li, Jiarun Zhong, Zehang Bao, Liangtian Zhao , et al. (7 additional authors not shown)

Abstract: Non-equilibrium quantum transport is crucial to technological advances ranging from nanoelectronics to thermal management. In essence, it deals with the coherent transfer of energy and (quasi-)particles through quantum channels between thermodynamic baths. A complete understanding of quantum transport thus requires the ability to simulate and probe macroscopic and microscopic physics on equal foot… ▽ More Non-equilibrium quantum transport is crucial to technological advances ranging from nanoelectronics to thermal management. In essence, it deals with the coherent transfer of energy and (quasi-)particles through quantum channels between thermodynamic baths. A complete understanding of quantum transport thus requires the ability to simulate and probe macroscopic and microscopic physics on equal footing. Using a superconducting quantum processor, we demonstrate the emergence of non-equilibrium steady quantum transport by emulating the baths with qubit ladders and realising steady particle currents between the baths. We experimentally show that the currents are independent of the microscopic details of bath initialisation, and their temporal fluctuations decrease rapidly with the size of the baths, emulating those predicted by thermodynamic baths. The above characteristics are experimental evidence of pure-state statistical mechanics and prethermalisation in non-equilibrium many-body quantum systems. Furthermore, by utilising precise controls and measurements with single-site resolution, we demonstrate the capability to tune steady currents by manipulating the macroscopic properties of the baths, including filling and spectral properties. Our investigation paves the way for a new generation of experimental exploration of non-equilibrium quantum transport in strongly correlated quantum matter. △ Less

Submitted 11 November, 2024; originally announced November 2024.

Comments: 7 pages, 4 figures

Journal ref: Nat. Commun. 15, 10115 (2024)

Scale-tailored localization and its observation in non-Hermitian electrical circuits

Authors: Cui-Xian Guo, Luhong Su, Yongliang Wang, Li Li, Jinzhe Wang, Xinhui Ruan, Yanjing Du, Dongning Zheng, Shu Chen, Haiping Hu

Abstract: Anderson localization and non-Hermitian skin effect are two paradigmatic wave localization phenomena, resulting from wave interference and the intrinsic non-Hermitian point gap, respectively. In this study, we unveil a novel localization phenomenon associated with long-range asymmetric coupling, termed scale-tailored localization, where the number of induced localized modes and their localization… ▽ More Anderson localization and non-Hermitian skin effect are two paradigmatic wave localization phenomena, resulting from wave interference and the intrinsic non-Hermitian point gap, respectively. In this study, we unveil a novel localization phenomenon associated with long-range asymmetric coupling, termed scale-tailored localization, where the number of induced localized modes and their localization lengths scale exclusively with the coupling range. We show that the long-range coupling fundamentally reshapes the energy spectra and eigenstates by creating multiple connected paths on the lattice. Furthermore, we present experimental observations of scale-tailored localization in non-Hermitian electrical circuits utilizing adjustable voltage followers and switches. The circuit admittance spectra possess separate point-shaped and loop-shaped components in the complex energy plane, corresponding respectively to skin modes and scale-tailored localized states. Our findings not only expand and deepen the understanding of peculiar effects induced by non-Hermiticity but also offer a feasible experimental platform for exploring and controlling wave localizations. △ Less

Submitted 23 October, 2024; originally announced October 2024.

Comments: 10+16 pages, 5+11 figures

Journal ref: Nature Communications 15, 9120 (2024)

Grassmann time-evolving matrix product operators: An efficient numerical approach for fermionic path integral simulations

Authors: Xiansong Xu, Chu Guo, Ruofan Chen

Abstract: Developing numerical exact solvers for open quantum systems is a challenging task due to the non-perturbative and non-Markovian nature when coupling to structured environments. The Feynman-Vernon influence functional approach is a powerful analytical tool to study the dynamics of open quantum systems. Numerical treatments of the influence functional including the quasi-adiabatic propagator techniq… ▽ More Developing numerical exact solvers for open quantum systems is a challenging task due to the non-perturbative and non-Markovian nature when coupling to structured environments. The Feynman-Vernon influence functional approach is a powerful analytical tool to study the dynamics of open quantum systems. Numerical treatments of the influence functional including the quasi-adiabatic propagator technique and the tensor-network-based time-evolving matrix product operator method, have proven to be efficient in studying open quantum systems with bosonic environments. However, the numerical implementation of the fermionic path integral suffers from the Grassmann algebra involved. In this work, we present a detailed introduction of the Grassmann time-evolving matrix product operator method for fermionic open quantum systems. In particular, we introduce the concepts of Grassmann tensor, signed matrix product operator, and Grassmann matrix product state to handle the Grassmann path integral. Using the single-orbital Anderson impurity model as an example, we review the numerical benchmarks for structured fermionic environments for real-time nonequilibrium dynamics, real-time and imaginary-time equilibration dynamics, and its application as an impurity solver. These benchmarks show that our method is a robust and promising numerical approach to study strong coupling physics and non-Markovian dynamics. It can also serve as an alternative impurity solver to study strongly-correlated quantum matter with dynamical mean-field theory. △ Less

Submitted 15 October, 2024; originally announced October 2024.

Comments: 17 pages, 10 figures

Journal ref: J. Chem. Phys. 161, 151001 (2024)

Optical modeling, solver, and design of wafer-scale single-enantiomer carbon nanotube film and reconfigurable chiral photonic device

Authors: Jichao Fan, Benjamin Hillam, Cheng Guo, Hiroyuki Fujinami, Shiba Koki, Haoyu Xie, Ruiyang Chen, Kazuhiro Yanagi, Weilu Gao

Abstract: The interaction of circularly polarized light with chiral matter and functional devices enables novel phenomena and applications. Recently, wafer-scale solid-state single-enantiomer carbon nanotube (CNT) films have become feasible and are emerging as a chiral photonic material platform thanks to their quantum-confinement-induced optical properties and facile scalable assembly. However, optical mod… ▽ More The interaction of circularly polarized light with chiral matter and functional devices enables novel phenomena and applications. Recently, wafer-scale solid-state single-enantiomer carbon nanotube (CNT) films have become feasible and are emerging as a chiral photonic material platform thanks to their quantum-confinement-induced optical properties and facile scalable assembly. However, optical modeling, solver, and device design tools for such materials are non-existent. Here, we prepare wafer-scale single-enantiomer (6,5) and (11,-5) randomly oriented CNT films and create an optical material model based on measured experimental optical spectra. We also implement a highly-parallel graphic-processing-unit accelerated transfer matrix solver for general bi-anisotropic materials and layered structures. Further, we demonstrate reconfigurable chiral photonic devices in a heterostructure with phase change materials through machine learning-enabled efficient gradient-based inverse design and optimization. Our developed full stack of a chiral photonic material and device hardware platform and a corresponding high-performance differential-programming-enabled solver opens the door for future chiral photonic devices and applications based on single-enantiomer CNT films. △ Less

Submitted 11 October, 2024; originally announced October 2024.

Passivity constraints on the relations between transmission, reflection, and absorption eigenvalues

Authors: Cheng Guo, Shanhui Fan

Abstract: We investigate the passivity constraints on the relations between transmission, reflection, and absorption eigenvalues in linear time-invariant systems. Using techniques from matrix analysis, we derive necessary and sufficient conditions for the permissible combinations of these eigenvalues. Our analysis reveals that the set of allowable eigenvalue combinations forms a convex polyhedron in eigenva… ▽ More We investigate the passivity constraints on the relations between transmission, reflection, and absorption eigenvalues in linear time-invariant systems. Using techniques from matrix analysis, we derive necessary and sufficient conditions for the permissible combinations of these eigenvalues. Our analysis reveals that the set of allowable eigenvalue combinations forms a convex polyhedron in eigenvalue space, characterized by a trace equality and a set of linear inequalities. Surprisingly, we uncover a direct connection between this physical problem and Alfred Horn's inequalities, a fundamental result in matrix theory. We provide explicit examples for systems with varying numbers of input ports, demonstrating the increasing complexity of the constraints as system size grows. We apply our theory to analyze the implications of important phenomena, including open and closed channels, coherent perfect reflection and reflectionless scattering modes, and coherent perfect absorption and coherent zero absorption. Our findings not only offer a complete characterization of passivity constraints on wave transport eigenvalues but also establish an unexpected bridge between fundamental wave physics and advanced matrix theory, opening new avenues for research at their intersection. These results have significant implications for the design and optimization of passive wave devices across a wide range of applications in optics, acoustics, and mesoscopic physics. △ Less

Submitted 6 October, 2024; originally announced October 2024.

Comments: 37 pages, 6 figures

Transverse voltage in anisotropic hydrodynamic conductors

Authors: Kaize Wang, Chunyu Guo, Philip J. W. Moll, Tobias Holder

Abstract: Weak momentum dissipation in ultra-clean metals gives rise to novel non-Ohmic current flow, including ballistic and hydrodynamic regimes. Recently, hydrodynamic flow has attracted intense interest because it presents a valuable window into the electronic correlations and the longest lived collective modes of quantum materials. However, diagnosing viscous flow is difficult as the macroscopic observ… ▽ More Weak momentum dissipation in ultra-clean metals gives rise to novel non-Ohmic current flow, including ballistic and hydrodynamic regimes. Recently, hydrodynamic flow has attracted intense interest because it presents a valuable window into the electronic correlations and the longest lived collective modes of quantum materials. However, diagnosing viscous flow is difficult as the macroscopic observables of ballistic and hydrodynamic transport such as the average current distribution can be deceptively similar, even if their respective microscopics deviate notably. Based on kinetic Boltzmann theory, here we propose to address this issue via the transverse channel voltage at zero magnetic field, which can efficiently detect hydrodynamic flow in a number of materials. To this end, we show that the transverse voltage is sensitive to the interplay between anisotropic fermiology and boundary scattering, resulting in a non-trivial behavior in narrow channels along crystalline low-symmetry directions. We discuss several materials where the channel-size dependent stress of the quantum fluid leads to a characteristic sign change of the transverse voltage as a new hallmark of the cross-over from the ballistic to the hydrodynamic regime. △ Less

Submitted 7 February, 2025; v1 submitted 24 September, 2024; originally announced September 2024.

Journal ref: PhysRevB.111.L081402(2025)

Transport measurements of majorization order for wave coherence

Authors: Cheng Guo, David A. B. Miller, Shanhui Fan

Abstract: We investigate the majorization order for comparing wave coherence and reveal its fundamental consequences in transport measurements, including power distribution, absorption, transmission, and reflection. We prove that all these measurements preserve the majorization order under unitary control, enabling direct experimental characterization of the majorization order. Specifically, waves with lowe… ▽ More We investigate the majorization order for comparing wave coherence and reveal its fundamental consequences in transport measurements, including power distribution, absorption, transmission, and reflection. We prove that all these measurements preserve the majorization order under unitary control, enabling direct experimental characterization of the majorization order. Specifically, waves with lower coherence in the majorization order exhibit more restricted ranges of achievable measurement values. Our results deepen the understanding of coherence in transport phenomena. △ Less

Submitted 10 August, 2024; originally announced August 2024.

Comments: 11 pages, 3 figures

Unitary control of partially coherent waves. II. Transmission or reflection

Authors: Cheng Guo, Shanhui Fan

Abstract: Coherent control of wave transmission and reflection is crucial for applications in communication, imaging, and sensing. However, many practical scenarios involve partially coherent waves rather than fully coherent ones. We present a systematic theory for the unitary control of partially coherent wave transmission and reflection. For a linear time-invariant system with an incident partially cohere… ▽ More Coherent control of wave transmission and reflection is crucial for applications in communication, imaging, and sensing. However, many practical scenarios involve partially coherent waves rather than fully coherent ones. We present a systematic theory for the unitary control of partially coherent wave transmission and reflection. For a linear time-invariant system with an incident partially coherent wave, we derive analytical expressions for the range of attainable total transmittance and reflectance under arbitrary unitary transformations. We also introduce an explicit algorithm to construct a unitary control scheme that achieves any desired transmission or reflection within the attainable range. As applications of our theory, we establish conditions for four novel phenomena: partially coherent perfect transmission, partially coherent perfect reflection, partially coherent zero transmission, and partially coherent zero reflection. We also prove a theorem that relates the degree of coherence of the incident field, quantified by the majorization order, to the resulting transmission and reflection intervals. Furthermore, we demonstrate that reciprocity (or energy conservation) imposes direct symmetry constraints on bilateral transmission (or transmission and reflection) of partially coherent waves under unitary control. Our results provide fundamental insights and practical guidelines for using unitary control to manipulate the transmission and reflection of partially coherent waves. This theory applies to various wave systems, including electromagnetic and acoustic waves. △ Less

Submitted 10 August, 2024; originally announced August 2024.

Comments: 31 pages, 5 figures

Journal ref: Phys. Rev. B 110, 035431 (2024)

Unitary control of partially coherent waves. I. Absorption

Authors: Cheng Guo, Shanhui Fan

Abstract: The coherent control of wave absorption has important applications in areas such as energy harvesting, imaging, and sensing. However, most practical scenarios involve the absorption of partially coherent rather than fully coherent waves. Here we present a systematic theory of unitary control over the absorption of partially coherent waves by linear systems. Given an absorbing system and incident p… ▽ More The coherent control of wave absorption has important applications in areas such as energy harvesting, imaging, and sensing. However, most practical scenarios involve the absorption of partially coherent rather than fully coherent waves. Here we present a systematic theory of unitary control over the absorption of partially coherent waves by linear systems. Given an absorbing system and incident partially coherent wave, we provide analytical expressions for the range of attainable absorptivity under arbitrary unitary transformations of the incident field. We also present an explicit algorithm to construct the unitary control scheme that achieves any desired absorptivity within that attainable range. As applications of our theory, we derive the conditions required for achieving two new phenomena - partially coherent perfect absorption and partially coherent zero absorption. Furthermore, we prove a theorem relating the coherence properties of the incident field, as quantified by majorization, to the resulting absorption intervals. Our results provide both fundamental insights and practical prescriptions for exploiting unitary control to shape the absorption of partially coherent waves. The theory applies across the electromagnetic spectrum as well as to other classical wave systems such as acoustic waves. △ Less

Submitted 10 August, 2024; originally announced August 2024.

Comments: 26 pages, 4 figures

Journal ref: Phys. Rev. B 110, 035430 (2024)

Unitary control of multiport wave transmission

Authors: Cheng Guo, David A. B. Miller, Shanhui Fan

Abstract: Controlling wave transmission is crucial for various applications. In this work, we apply the concept of unitary control to manipulate multiport wave transmission. Unitary control aims to control the behaviors of a set of orthogonal waves simultaneously. The approach fully harnesses the capability of wavefront shaping techniques, with promising applications in communication, imaging, and photonic… ▽ More Controlling wave transmission is crucial for various applications. In this work, we apply the concept of unitary control to manipulate multiport wave transmission. Unitary control aims to control the behaviors of a set of orthogonal waves simultaneously. The approach fully harnesses the capability of wavefront shaping techniques, with promising applications in communication, imaging, and photonic integrated circuits. Here we present a detailed theory of unitary control of wave transmission, focusing on two key characteristics: total (power) transmittance and direct (field) transmission. The total transmittance for an input port represents the fraction of total transmitted power with respect to the input power for wave incident from an input port. The direct transmission for an input port denotes the complex transmission amplitude from that input port to its corresponding output port. We address two main questions: (i) the achievable total transmittance and direct transmission for each port, and (ii) the configuration of unitary control to attain desired transmission values for each port. Our theory illustrates that unitary control enables uniform total transmittance and direct transmission across any medium. Furthermore, we show that reciprocity and energy conservation enforce direct symmetry constraints on wave transmission in both forward and backward directions under unitary control. △ Less

Submitted 10 August, 2024; originally announced August 2024.

Comments: 29 pages, 3 figures

Enantiomer-Selective Magnetoresistance in Chiral Gold Nanocrystals by Magnetic Control of Surface Potentials

Authors: Fengxia Wu, Ying Wang, Yufei Zhao, Zhenyu Yang, Yu Tian, Zuoti Xie, Wenxin Niu, Binghai Yan, Cunlan Guo

Abstract: Chiral nanomaterials offer intriguing possibilities for novel electronic and chemical applications. Here, we report the discovery of an enantiomer-selective magnetoresistance effect in chiral gold nanocrystals. Based on precise control of nanocrystal chiral morphology using amino acid-directed synthesis, we demonstrate that an external magnetic field can dramatically modulate resistance in an enan… ▽ More Chiral nanomaterials offer intriguing possibilities for novel electronic and chemical applications. Here, we report the discovery of an enantiomer-selective magnetoresistance effect in chiral gold nanocrystals. Based on precise control of nanocrystal chiral morphology using amino acid-directed synthesis, we demonstrate that an external magnetic field can dramatically modulate resistance in an enantiomer-specific manner. For a given enantiomer, a magnetic field in one direction alters the resistance by dozens of times, while the opposite field direction leaves it unchanged. This asymmetric response reverses for the opposite enantiomer and are reproduced in both single nanocrystals by conduction atomic force microscopy and nanocrystal thin films in solid state devices. We attribute this phenomenon to a chirality-driven charge pumping effect, where the interplay between the chiral morphology and the magnetic field selectively modifies the surface potential. The magnitude and sign of the magnetoresistance can be further tuned by the surface chemistry of the nanocrystal, as demonstrated through sulfide treatment. Our findings reveal a new form of chirality-dependent magnetoresistance, distinct from previously known effects such as chirality-induced spin selectivity and electric magnetochiral anisotropy. The ability to remotely control surface potentials of chiral nanostructures using magnetic fields could enable novel approaches in catalysis, drug delivery, and nanoelectronics. △ Less

Submitted 27 February, 2025; v1 submitted 6 August, 2024; originally announced August 2024.

Comments: 55 pages including 6 figures, 31 Extended Data Figures and 4 Extended Data Tables

Anomalous diffusion in quantum system driven by heavy-tailed stochastic processes

Authors: Chenyue Guo, Yuchen Bi

Abstract: In this paper, we study a stochastically driven non-equilibrium quantum system where the driving protocols consist of hopping and waiting processes. The waiting times between two hopping processes satisfy a heavy-tailed distribution. By calculating the squared width of the wavepackets, our findings demonstrate the emergence of various anomalous transport phenomena when the system remains unchanged… ▽ More In this paper, we study a stochastically driven non-equilibrium quantum system where the driving protocols consist of hopping and waiting processes. The waiting times between two hopping processes satisfy a heavy-tailed distribution. By calculating the squared width of the wavepackets, our findings demonstrate the emergence of various anomalous transport phenomena when the system remains unchanged within the heavy-tailed regime, including superdiffusive, subdiffusive, and standard diffusive motion. Only subdiffusion occurs when the system has evolved during the waiting process. All these transport behaviors are accompanied by a breakdown of ergodicity, highlighting the complex dynamics induced by the stochastic driving mechanism. △ Less

Submitted 10 January, 2025; v1 submitted 28 July, 2024; originally announced July 2024.

Comments: 10 pages, 9 figures

Topological winding guaranteed coherent orthogonal scattering

Authors: Cheng Guo, Shanhui Fan

Abstract: Coherent control has enabled various novel phenomena in wave scattering. We introduce an effect called coherent orthogonal scattering, where the output wave becomes orthogonal to the reference output state without scatterers. This effect leads to a unity extinction coefficient and complete mode conversion. We examine the conditions for this effect and reveal its topological nature by relating it t… ▽ More Coherent control has enabled various novel phenomena in wave scattering. We introduce an effect called coherent orthogonal scattering, where the output wave becomes orthogonal to the reference output state without scatterers. This effect leads to a unity extinction coefficient and complete mode conversion. We examine the conditions for this effect and reveal its topological nature by relating it to the indivisibility between the dimension and the winding number of scattering submatrices. These findings deepen our understanding of topological scattering phenomena. △ Less

Submitted 26 June, 2024; originally announced June 2024.

Comments: 13 pages, 7 figures. In press

Journal ref: Phys. Rev. A 109, L061503 (2024)

Tensor-Networks-based Learning of Probabilistic Cellular Automata Dynamics

Authors: Heitor P. Casagrande, Bo Xing, William J. Munro, Chu Guo, Dario Poletti

Abstract: Algorithms developed to solve many-body quantum problems, like tensor networks, can turn into powerful quantum-inspired tools to tackle problems in the classical domain. In this work, we focus on matrix product operators, a prominent numerical technique to study many-body quantum systems, especially in one dimension. It has been previously shown that such a tool can be used for classification, lea… ▽ More Algorithms developed to solve many-body quantum problems, like tensor networks, can turn into powerful quantum-inspired tools to tackle problems in the classical domain. In this work, we focus on matrix product operators, a prominent numerical technique to study many-body quantum systems, especially in one dimension. It has been previously shown that such a tool can be used for classification, learning of deterministic sequence-to-sequence processes and of generic quantum processes. We further develop a matrix product operator algorithm to learn probabilistic sequence-to-sequence processes and apply this algorithm to probabilistic cellular automata. This new approach can accurately learn probabilistic cellular automata processes in different conditions, even when the process is a probabilistic mixture of different chaotic rules. In addition, we find that the ability to learn these dynamics is a function of the bit-wise difference between the rules and whether one is much more likely than the other. △ Less

Submitted 17 April, 2024; originally announced April 2024.

Comments: 9 pages, 7 figures

Solving quantum impurity problems on the L-shaped Kadanoff-Baym contour

Authors: Ruofan Chen, Chu Guo

Abstract: The path integral formalism is the building block of many powerful numerical methods for quantum impurity problems. However, existing fermionic path integral based numerical calculations have only been performed in either the imaginary-time or the real-time axis, while the most generic scenario formulated on the L-shaped Kadanoff-Baym contour is left unexplored. In this work, we extended the recen… ▽ More The path integral formalism is the building block of many powerful numerical methods for quantum impurity problems. However, existing fermionic path integral based numerical calculations have only been performed in either the imaginary-time or the real-time axis, while the most generic scenario formulated on the L-shaped Kadanoff-Baym contour is left unexplored. In this work, we extended the recently developed Grassmann time-evolving matrix product operator (GTEMPO) method to solve quantum impurity problems directly on the Kadanoff-Baym contour. The resulting method is numerically exact, with only two sources of numerical errors, e.g., the time discretization error and the matrix product state bond truncation error. The accuracy of this method is numerically demonstrated against exact solutions in the noninteracting case, and against existing calculations on the real- and imaginary-time axes for the single-orbital Anderson impurity model. We also show that the numerical errors of the method can be well suppressed as we refine the hyperparameters. Our method is a perfect benchmarking baseline for its alternatives which often employ less-controlled approximations, and can also be used as a real-time impurity solver in dynamical mean field theory. △ Less

Submitted 7 October, 2024; v1 submitted 8 April, 2024; originally announced April 2024.

Comments: 13 pages, 8 figures

Journal ref: Phys. Rev. B, 110, 165114 (2024)

Infinite Grassmann time-evolving matrix product operator method for zero-temperature equilibrium quantum impurity problems

Authors: Chu Guo, Ruofan Chen

Abstract: The Grassmann time-evolving matrix product operator (GTEMPO) method has proven to be an accurate and efficient numerical method for the real-time dynamics of quantum impurity problems. Whereas its application for imaginary-time calculations is much less competitive compared to well-established methods such as the continuous-time quantum Monte Carlo (CTQMC). In this work, we unleash the full power… ▽ More The Grassmann time-evolving matrix product operator (GTEMPO) method has proven to be an accurate and efficient numerical method for the real-time dynamics of quantum impurity problems. Whereas its application for imaginary-time calculations is much less competitive compared to well-established methods such as the continuous-time quantum Monte Carlo (CTQMC). In this work, we unleash the full power of GTEMPO for zero-temperature imaginary-time calculations: the multi-time impurity state is time-translationally invariant with infinite boundary condition, therefore it can be represented as an infinite Grassmann matrix product state (GMPS) with nontrivial unit cell in a single time step, instead of an open boundary GMPS spanning the whole imaginary-time axis. We devise a very efficient infinite GTEMPO algorithm targeted at zero-temperature equilibrium quantum impurity problems, which is known to be a hard regime for quantum Monte Carlo methods. To demonstrate the performance of our method, we benchmark it against exact solutions in the noninteracting limit, and against CTQMC calculations in the Anderson impurity models with up to two orbitals, where we show that the required bond dimension of the infinite GMPS is much smaller than its finite-temperature counterpart. △ Less

Submitted 8 October, 2024; v1 submitted 6 April, 2024; originally announced April 2024.

Comments: 9 pages, 7 figures

Journal ref: Phys. Rev. B, 110, 165119 (2024)

Infinite Grassmann Time-Evolving Matrix Product Operator Method in the Steady State

Authors: Chu Guo, Ruofan Chen

Abstract: We present an infinite Grassmann time-evolving matrix product operator method for quantum impurity problems, which directly works in the steady state. The method embraces the well-established infinite matrix product state algorithms with the recently developed GTEMPO method, and benefits from both sides: it obtains real-time Green's functions without sampling noises and bath discretization error,… ▽ More We present an infinite Grassmann time-evolving matrix product operator method for quantum impurity problems, which directly works in the steady state. The method embraces the well-established infinite matrix product state algorithms with the recently developed GTEMPO method, and benefits from both sides: it obtains real-time Green's functions without sampling noises and bath discretization error, it is applicable for any temperature without the sign problem, its computational cost is independent of the transient dynamics and does not scale with the number of baths. We benchmark the method on the finite-temperature equilibrium Green's function in the noninteracting limit against exact solutions and in the single-orbital Anderson impurity model against GTEMPO calculations. We also study the zero-temperature non-equilibrium steady state of an impurity coupled to two baths with a voltage bias, obtaining consistent particle currents with existing calculations. The method is ideal for studying steady-state quantum transport, and can be readily used as an efficient real-time impurity solver in the dynamical mean field theory and its non-equilibrium extension. △ Less

Submitted 8 August, 2024; v1 submitted 25 March, 2024; originally announced March 2024.

Comments: 11 pages, 7 figures

Journal ref: Physical Review B 110, 045106(2024)