Showing 1–30 of 30 results for author: McMahon, I

Search for planetary-mass ultra-compact binaries using data from the first part of the LIGO--Virgo--KAGRA fourth observing run

Authors: The LIGO Scientific Collaboration, the Virgo Collaboration, the KAGRA Collaboration, A. G. Abac, I. Abouelfettouh, F. Acernese, K. Ackley, C. Adamcewicz, S. Adhicary, D. Adhikari, N. Adhikari, R. X. Adhikari, V. K. Adkins, S. Afroz, A. Agapito, D. Agarwal, M. Agathos, N. Aggarwal, S. Aggarwal, O. D. Aguiar, I. -L. Ahrend, L. Aiello, A. Ain, P. Ajith, T. Akutsu , et al. (1743 additional authors not shown)

Abstract: We present a search for gravitational waves from inspiraling, planetary-mass ultra-compact binaries using data from the first part of the fourth observing run of LIGO, Virgo and KAGRA. Finding no evidence of such systems, we determine the maximum distance reach for such objects and their merger rate densities, independently of how they could have formed. Then, we identify classes of primordial bla… ▽ More We present a search for gravitational waves from inspiraling, planetary-mass ultra-compact binaries using data from the first part of the fourth observing run of LIGO, Virgo and KAGRA. Finding no evidence of such systems, we determine the maximum distance reach for such objects and their merger rate densities, independently of how they could have formed. Then, we identify classes of primordial black-hole mass distributions for which these rate limits can be translated into relevant constraints on the mass distribution of primordial black holes, assuming that they compose all of dark matter, in the mass range $[10^{-6},10^{-3}]M_\odot$. Our constraints are consistent with existing microlensing results in the planetary-mass range, and provide a complementary probe to sub-solar mass objects. △ Less

Submitted 5 December, 2025; v1 submitted 24 November, 2025; originally announced November 2025.

Comments: 6 pages (main) + 7 pages (appendix) + refs; 8 figures

Report number: P2500248

All-sky search for continuous gravitational-wave signals from unknown neutron stars in binary systems in the first part of the fourth LIGO-Virgo-KAGRA observing run

Authors: The LIGO Scientific Collaboration, the Virgo Collaboration, the KAGRA Collaboration, A. G. Abac, I. Abouelfettouh, F. Acernese, K. Ackley, C. Adamcewicz, S. Adhicary, D. Adhikari, N. Adhikari, R. X. Adhikari, V. K. Adkins, S. Afroz, A. Agapito, D. Agarwal, M. Agathos, N. Aggarwal, S. Aggarwal, O. D. Aguiar, I. -L. Ahrend, L. Aiello, A. Ain, P. Ajith, T. Akutsu , et al. (1743 additional authors not shown)

Abstract: We present the results of a blind all-sky search for continuous gravitational-wave signals from neutron stars in binary systems using data from the first part of the fourth observing run (O4a) using LIGO detectors data. Rapidly rotating, non-axisymmetric neutron stars are expected to emit continuous gravitational waves, whose detection would significantly improve our understanding of the galactic… ▽ More We present the results of a blind all-sky search for continuous gravitational-wave signals from neutron stars in binary systems using data from the first part of the fourth observing run (O4a) using LIGO detectors data. Rapidly rotating, non-axisymmetric neutron stars are expected to emit continuous gravitational waves, whose detection would significantly improve our understanding of the galactic neutron star population and matter under extreme conditions, while also providing valuable tests of general relativity. Neutron stars in binary systems likely constitute a substantial fraction of the unobserved galactic population and, due to potential mass accretion, may emit stronger gravitational-wave signals than their isolated counterparts. This search targets signals from neutron stars with frequencies in the 100-350 Hz range, with orbital periods between 7 and 15 days and projected semi-major axes between 5 and 15 light-seconds. The analysis employs the GPU-accelerated fasttracks pipeline. No credible astrophysical signals were identified, and, in the absence of a detection, we report search sensitivity estimates on the population of neutron stars in binary systems in the Milky Way. △ Less

Submitted 4 December, 2025; v1 submitted 20 November, 2025; originally announced November 2025.

Comments: 24 pages, 18 figures, 6 tables

Report number: LIGO-P2500437

Direct multi-model dark-matter search with gravitational-wave interferometers using data from the first part of the fourth LIGO-Virgo-KAGRA observing run

Authors: The LIGO Scientific Collaboration, the Virgo Collaboration, the KAGRA Collaboration, A. G. Abac, I. Abouelfettouh, F. Acernese, K. Ackley, C. Adamcewicz, S. Adhicary, D. Adhikari, N. Adhikari, R. X. Adhikari, V. K. Adkins, S. Afroz, A. Agapito, D. Agarwal, M. Agathos, N. Aggarwal, S. Aggarwal, O. D. Aguiar, I. -L. Ahrend, L. Aiello, A. Ain, P. Ajith, T. Akutsu , et al. (1745 additional authors not shown)

Abstract: Gravitational-wave detectors can probe the existence of dark matter with exquisite sensitivity. Here, we perform a search for three kinds of dark matter -- dilatons (spin-0), dark photons (spin-1) and tensor bosons (spin-2) -- using three independent methods on the first part of the most recent data from the fourth observing run of LIGO--Virgo--KAGRA. Each form of dark matter could have interacted… ▽ More Gravitational-wave detectors can probe the existence of dark matter with exquisite sensitivity. Here, we perform a search for three kinds of dark matter -- dilatons (spin-0), dark photons (spin-1) and tensor bosons (spin-2) -- using three independent methods on the first part of the most recent data from the fourth observing run of LIGO--Virgo--KAGRA. Each form of dark matter could have interacted with different standard-model particles in the instruments, causing unique differential strains on the interferometers. While we do not find any evidence for a signal, we place the most stringent upper limits to-date on each of these models. For scalars with masses between $[4\times 10^{-14},1.5\times 10^{-13}]$ eV that couple to photons or electrons, our constraints improve upon those from the third observing run by one order of magnitude, with the tightest limit of $\sim 10^{-20}\,\text{GeV}^{-1}$ at a mass of $\sim2\times 10^{-13}\text{ eV}$. For vectors with masses between $[7\times 10^{-13},8.47\times 10^{-12}]$ eV that couple to baryons, our constraints supersede those from MICROSCOPE and Eöt-Wash by one to two orders of magnitude, reaching a minimum of $\sim 5\times 10^{-24}$ at a mass of $\sim 10^{-12}$ eV. For tensors with masses of $[4\times 10^{-14},8.47\times 10^{-12}]$ eV (the full mass range analyzed) that couple via a Yukawa interaction, our constraints surpass those from fifth-force experiments by four to five orders of magnitude, achieving a limit as low as $\sim 8\times 10^{-9}$ at $\sim2\times 10^{-13}$ eV. Our results show that gravitational-wave interferometers have become frontiers for new physics and laboratories for direct multi-model dark-matter detection. △ Less

Submitted 11 December, 2025; v1 submitted 30 October, 2025; originally announced October 2025.

Comments: 9 pages, 1 figure (+1 figure in appendix)

Report number: P2500252

GW241011 and GW241110: Exploring Binary Formation and Fundamental Physics with Asymmetric, High-Spin Black Hole Coalescence

Authors: The LIGO Scientific Collaboration, the Virgo Collaboration, the KAGRA Collaboration, A. G. Abac, I. Abouelfettouh, F. Acernese, K. Ackley, C. Adamcewicz, S. Adhicary, D. Adhikari, N. Adhikari, R. X. Adhikari, V. K. Adkins, S. Afroz, A. Agapito, D. Agarwal, M. Agathos, N. Aggarwal, S. Aggarwal, O. D. Aguiar, I. -L. Ahrend, L. Aiello, A. Ain, P. Ajith, T. Akutsu , et al. (1761 additional authors not shown)

Abstract: We report the observation of gravitational waves from two binary black hole coalescences during the fourth observing run of the LIGO--Virgo--KAGRA detector network, GW241011 and GW241110. The sources of these two signals are characterized by rapid and precisely measured primary spins, non-negligible spin--orbit misalignment, and unequal mass ratios between their constituent black holes. These prop… ▽ More We report the observation of gravitational waves from two binary black hole coalescences during the fourth observing run of the LIGO--Virgo--KAGRA detector network, GW241011 and GW241110. The sources of these two signals are characterized by rapid and precisely measured primary spins, non-negligible spin--orbit misalignment, and unequal mass ratios between their constituent black holes. These properties are characteristic of binaries in which the more massive object was itself formed from a previous binary black hole merger, and suggest that the sources of GW241011 and GW241110 may have formed in dense stellar environments in which repeated mergers can take place. As the third loudest gravitational-wave event published to date, with a median network signal-to-noise ratio of $36.0$, GW241011 furthermore yields stringent constraints on the Kerr nature of black holes, the multipolar structure of gravitational-wave generation, and the existence of ultralight bosons within the mass range $10^{-13}$--$10^{-12}$ eV. △ Less

Submitted 30 October, 2025; originally announced October 2025.

Comments: Data available from Zenodo (https://zenodo.org/records/17343574) or the Gravitational-Wave Open Science Center (https://gwosc.org)

Report number: LIGO-P2500402

Journal ref: Astrophys. J. Letters, 993, L21 (2025)

Cosmological and High Energy Physics implications from gravitational-wave background searches in LIGO-Virgo-KAGRA's O1-O4a runs

Authors: The LIGO Scientific Collaboration, the Virgo Collaboration, the KAGRA Collaboration, A. G. Abac, I. Abouelfettouh, F. Acernese, K. Ackley, C. Adamcewicz, S. Adhicary, D. Adhikari, N. Adhikari, R. X. Adhikari, V. K. Adkins, S. Afroz, A. Agapito, D. Agarwal, M. Agathos, N. Aggarwal, S. Aggarwal, O. D. Aguiar, I. -L. Ahrend, L. Aiello, A. Ain, P. Ajith, T. Akutsu , et al. (1747 additional authors not shown)

Abstract: We search for gravitational-wave background signals produced by various early Universe processes in the Advanced LIGO O4a dataset, combined with the data from the earlier O1, O2, and O3 (LIGO-Virgo) runs. The absence of detectable signals enables powerful constraints on fundamental physics. We derive gravitational-wave background energy density upper limits from the O1-O4a data to constrain parame… ▽ More We search for gravitational-wave background signals produced by various early Universe processes in the Advanced LIGO O4a dataset, combined with the data from the earlier O1, O2, and O3 (LIGO-Virgo) runs. The absence of detectable signals enables powerful constraints on fundamental physics. We derive gravitational-wave background energy density upper limits from the O1-O4a data to constrain parameters associated with various possible processes in the early Universe: first-order phase transitions, cosmic strings, domain walls, stiff equation of state, axion inflation, second-order scalar perturbations, primordial black hole binaries, and parity violation. In our analyses, the presence of an astrophysical background produced by compact (black hole and neutron star) binary coalescences throughout the Universe is also considered. We address the implications for various cosmological and high energy physics models based on the obtained parameter constraints. We conclude that LIGO-Virgo data already yield significant constraints on numerous early Universe scenarios. △ Less

Submitted 7 November, 2025; v1 submitted 30 October, 2025; originally announced October 2025.

Comments: Main paper: 45 pages, 20 figures

Report number: LIGO-PP2500150

Directional Search for Persistent Gravitational Waves: Results from the First Part of LIGO-Virgo-KAGRA's Fourth Observing Run

Authors: The LIGO Scientific Collaboration, the Virgo Collaboration, the KAGRA Collaboration, A. G. Abac, I. Abouelfettouh, F. Acernese, K. Ackley, C. Adamcewicz, S. Adhicary, D. Adhikari, N. Adhikari, R. X. Adhikari, V. K. Adkins, S. Afroz, A. Agapito, D. Agarwal, M. Agathos, N. Aggarwal, S. Aggarwal, O. D. Aguiar, I. -L. Ahrend, L. Aiello, A. Ain, P. Ajith, T. Akutsu , et al. (1743 additional authors not shown)

Abstract: The angular distribution of gravitational-wave power from persistent sources may exhibit anisotropies arising from the large-scale structure of the Universe. This motivates directional searches for astrophysical and cosmological gravitational-wave backgrounds, as well as continuous-wave emitters. We present results of such a search using data from the first observing run through the first portion… ▽ More The angular distribution of gravitational-wave power from persistent sources may exhibit anisotropies arising from the large-scale structure of the Universe. This motivates directional searches for astrophysical and cosmological gravitational-wave backgrounds, as well as continuous-wave emitters. We present results of such a search using data from the first observing run through the first portion of the fourth observing run of the LIGO-Virgo-KAGRA Collaborations. We apply gravitational-wave radiometer techniques to generate skymaps and search for both narrowband and broadband persistent gravitational-wave sources. Additionally, we use spherical harmonic decomposition to probe spatially extended sources. No evidence of persistent gravitational-wave signals is found, and we set the most stringent constraints to date on such emissions. For narrowband point sources, our sensitivity estimate to effective strain amplitude lies in the range $(0.03 - 8.4) \times 10^{-24}$ across all sky and frequency range $(20 - 160)$ Hz. For targeted sources -- Scorpius X-1, SN 1987A, the Galactic Center, Terzan 5, and NGC 6397 -- we constrain the strain amplitude with best limits ranging from $\sim 1.1 \times 10^{-25}$ to $6.5 \times 10^{-24}$. For persistent broadband sources, we constrain the gravitational-wave flux $F_{α, \hat{n}}^{95\%, \mathrm{UL}}(25\, \mathrm{Hz}) < (0.008 - 5.5) \times 10^{-8}\, \mathrm{erg\, cm^{-2}\, s^{-1}\, Hz^{-1}}$, depending on the sky direction $\hat{n}$ and spectral index $α=0,\,2/3,\,3$. Finally, for extended sources, we place upper limits on the strain angular power spectrum $C_\ell^{1/2} < (0.63 - 17) \times 10^{-10} \,\mathrm{sr}^{-1}$. △ Less

Submitted 20 October, 2025; originally announced October 2025.

Comments: Main paper: 11 pages and 4 figures; Total with appendices: 39 pages and 12 figures

Report number: LIGO-P250038

GW250114: testing Hawking's area law and the Kerr nature of black holes

Authors: The LIGO Scientific Collaboration, the Virgo Collaboration, the KAGRA Collaboration, A. G. Abac, I. Abouelfettouh, F. Acernese, K. Ackley, C. Adamcewicz, S. Adhicary, D. Adhikari, N. Adhikari, R. X. Adhikari, V. K. Adkins, S. Afroz, A. Agapito, D. Agarwal, M. Agathos, N. Aggarwal, S. Aggarwal, O. D. Aguiar, I. -L. Ahrend, L. Aiello, A. Ain, P. Ajith, T. Akutsu , et al. (1763 additional authors not shown)

Abstract: The gravitational-wave signal GW250114 was observed by the two LIGO detectors with a network matched-filter signal-to-noise ratio of 80. The signal was emitted by the coalescence of two black holes with near-equal masses $m_1 = 33.6^{+1.2}_{-0.8}\,M_\odot$ and $m_2 = 32.2^{+0.8}_{-1.3}\,M_\odot$, and small spins $χ_{1,2} \leq 0.26$ (90% credibility) and negligible eccentricity $e \leq 0.03$. Post-… ▽ More The gravitational-wave signal GW250114 was observed by the two LIGO detectors with a network matched-filter signal-to-noise ratio of 80. The signal was emitted by the coalescence of two black holes with near-equal masses $m_1 = 33.6^{+1.2}_{-0.8}\,M_\odot$ and $m_2 = 32.2^{+0.8}_{-1.3}\,M_\odot$, and small spins $χ_{1,2} \leq 0.26$ (90% credibility) and negligible eccentricity $e \leq 0.03$. Post-merger data excluding the peak region are consistent with the dominant quadrupolar $(\ell = |m| = 2)$ mode of a Kerr black hole and its first overtone. We constrain the modes' frequencies to $\pm 30\%$ of the Kerr spectrum, providing a test of the remnant's Kerr nature. We also examine Hawking's area law, also known as the second law of black hole mechanics, which states that the total area of the black hole event horizons cannot decrease with time. A range of analyses that exclude up to 5 of the strongest merger cycles confirm that the remnant area is larger than the sum of the initial areas to high credibility. △ Less

Submitted 9 September, 2025; originally announced September 2025.

Comments: 6 pages, 5 figures (plus supplement)

Report number: LIGO-P2500421

Directed searches for gravitational waves from ultralight vector boson clouds around merger remnant and galactic black holes during the first part of the fourth LIGO-Virgo-KAGRA observing run

Authors: The LIGO Scientific Collaboration, the Virgo Collaboration, the KAGRA Collaboration, A. G. Abac, I. Abouelfettouh, F. Acernese, K. Ackley, C. Adamcewicz, S. Adhicary, D. Adhikari, N. Adhikari, R. X. Adhikari, V. K. Adkins, S. Afroz, A. Agapito, D. Agarwal, M. Agathos, N. Aggarwal, S. Aggarwal, O. D. Aguiar, I. -L. Ahrend, L. Aiello, A. Ain, P. Ajith, T. Akutsu , et al. (1747 additional authors not shown)

Abstract: We present the first directed searches for long-transient and continuous gravitational waves from ultralight vector boson clouds around known black holes (BHs). We use LIGO data from the first part of the fourth LIGO-Virgo-KAGRA observing run. The searches target two distinct types of BHs and use two new semicoherent methods: hidden Markov model (HMM) tracking for the remnant BHs of the mergers GW… ▽ More We present the first directed searches for long-transient and continuous gravitational waves from ultralight vector boson clouds around known black holes (BHs). We use LIGO data from the first part of the fourth LIGO-Virgo-KAGRA observing run. The searches target two distinct types of BHs and use two new semicoherent methods: hidden Markov model (HMM) tracking for the remnant BHs of the mergers GW230814_230901 and GW231123_135430 (referred to as GW230814 and GW231123 in this study), and a dedicated method using the Band Sampled Data (BSD) framework for the galactic BH in the Cygnus X-1 binary system. Without finding evidence of a signal from vector bosons in the data, we estimate the mass range that can be constrained. For the HMM searches targeting the remnants from GW231123 and GW230814, we disfavor vector boson masses in the ranges $[0.94, 1.08]$ and $[2.75, 3.28] \times 10^{-13}$ eV, respectively, at 30% confidence, assuming a 1% false alarm probability. Although these searches are only marginally sensitive to signals from merger remnants at relatively large distances, future observations are expected to yield more stringent constraints with high confidence. For the BSD search targeting the BH in Cygnus X-1, we exclude vector boson masses in the range $[0.85, 1.59] \times 10^{-13}$ eV at 95% confidence, assuming an initial BH spin larger than 0.5. △ Less

Submitted 14 September, 2025; v1 submitted 8 September, 2025; originally announced September 2025.

Comments: 33 pages, 4 figures

Report number: LIGO-P2500256

GWTC-4.0: Constraints on the Cosmic Expansion Rate and Modified Gravitational-wave Propagation

Authors: The LIGO Scientific Collaboration, the Virgo Collaboration, the KAGRA Collaboration, A. G. Abac, I. Abouelfettouh, F. Acernese, K. Ackley, C. Adamcewicz, S. Adhicary, D. Adhikari, N. Adhikari, R. X. Adhikari, V. K. Adkins, S. Afroz, A. Agapito, D. Agarwal, M. Agathos, N. Aggarwal, S. Aggarwal, O. D. Aguiar, I. -L. Ahrend, L. Aiello, A. Ain, P. Ajith, T. Akutsu , et al. (1750 additional authors not shown)

Abstract: We analyze data from 142 of the 218 gravitational-wave (GW) sources in the fourth LIGO-Virgo-KAGRA Collaboration (LVK) Gravitational-Wave Transient Catalog (GWTC-4.0) to estimate the Hubble constant $H_0$ jointly with the population properties of merging compact binaries. We measure the luminosity distance and redshifted masses of GW sources directly; in contrast, we infer GW source redshifts stat… ▽ More We analyze data from 142 of the 218 gravitational-wave (GW) sources in the fourth LIGO-Virgo-KAGRA Collaboration (LVK) Gravitational-Wave Transient Catalog (GWTC-4.0) to estimate the Hubble constant $H_0$ jointly with the population properties of merging compact binaries. We measure the luminosity distance and redshifted masses of GW sources directly; in contrast, we infer GW source redshifts statistically through i) location of features in the compact object mass spectrum and merger rate evolution, and ii) identifying potential host galaxies in the GW localization volume. Probing the relationship between source luminosity distances and redshifts obtained in this way yields constraints on cosmological parameters. We also constrain parameterized deviations from general relativity which affect GW propagation, specifically those modifying the dependence of a GW signal on the source luminosity distance. Assuming our fiducial model for the source-frame mass distribution and using GW candidates detected up to the end of the fourth observing run (O4a), together with the GLADE+ all-sky galaxy catalog, we estimate $H_0 = 76.6^{+13.0}_{-9.5} (76.6^{+25.2}_{-14.0})$ km s$^{-1}$ Mpc$^{-1}$. This value is reported as a median with 68.3% (90%) symmetric credible interval, and includes combination with the $H_0$ measurement from GW170817 and its electromagnetic counterpart. Using a parametrization of modified GW propagation in terms of the magnitude parameter $Ξ_0$, we estimate $Ξ_0 = 1.2^{+0.8}_{-0.4} (1.2^{+2.4}_{-0.5})$, where $Ξ_0 = 1$ recovers the behavior of general relativity. △ Less

Submitted 7 October, 2025; v1 submitted 4 September, 2025; originally announced September 2025.

Comments: As part of the Astrophysical Journal Letters Focus Issue on the Gravitational Wave Transient Catalog

Report number: LIGO-P2400152

Upper Limits on the Isotropic Gravitational-Wave Background from the first part of LIGO, Virgo, and KAGRA's fourth Observing Run

Authors: The LIGO Scientific Collaboration, the Virgo Collaboration, the KAGRA Collaboration, A. G. Abac, I. Abouelfettouh, F. Acernese, K. Ackley, C. Adamcewicz, S. Adhicary, D. Adhikari, N. Adhikari, R. X. Adhikari, V. K. Adkins, S. Afroz, A. Agapito, D. Agarwal, M. Agathos, N. Aggarwal, S. Aggarwal, O. D. Aguiar, I. -L. Ahrend, L. Aiello, A. Ain, P. Ajith, T. Akutsu , et al. (1751 additional authors not shown)

Abstract: We present results from the search for an isotropic gravitational-wave background using Advanced LIGO and Advanced Virgo data from O1 through O4a, the first part of the fourth observing run. This background is the accumulated signal from unresolved sources throughout cosmic history and encodes information about the merger history of compact binaries throughout the Universe, as well as exotic physi… ▽ More We present results from the search for an isotropic gravitational-wave background using Advanced LIGO and Advanced Virgo data from O1 through O4a, the first part of the fourth observing run. This background is the accumulated signal from unresolved sources throughout cosmic history and encodes information about the merger history of compact binaries throughout the Universe, as well as exotic physics and potentially primordial processes from the early cosmos. Our cross-correlation analysis reveals no statistically significant background signal, enabling us to constrain several theoretical scenarios. For compact binary coalescences which approximately follow a 2/3 power-law spectrum, we constrain the fractional energy density to $Ω_{\rm GW}(25{\rm Hz})\leq 2.0\times 10^{-9}$ (95% cred.), a factor of 1.7 improvement over previous results. Scale-invariant backgrounds are constrained to $Ω_{\rm GW}(25{\rm Hz})\leq 2.8\times 10^{-9}$, representing a 2.1x sensitivity gain. We also place new limits on gravity theories predicting non-standard polarization modes and confirm that terrestrial magnetic noise sources remain below detection threshold. Combining these spectral limits with population models for GWTC-4, the latest gravitational-wave event catalog, we find our constraints remain above predicted merger backgrounds but are approaching detectability. The joint analysis combining the background limits shown here with the GWTC-4 catalog enables improved inference of the binary black hole merger rate evolution across cosmic time. Employing GWTC-4 inference results and standard modeling choices, we estimate that the total background arising from compact binary coalescences is $Ω_{\rm CBC}(25{\rm Hz})={0.9^{+1.1}_{-0.5}\times 10^{-9}}$ at 90% confidence, where the largest contribution is due to binary black holes only, $Ω_{\rm BBH}(25{\rm Hz})=0.8^{+1.1}_{-0.5}\times 10^{-9}$. △ Less

Submitted 28 August, 2025; originally announced August 2025.

Comments: 31 pages, 7 figures

Report number: LIGO-P2500349

GWTC-4.0: Updating the Gravitational-Wave Transient Catalog with Observations from the First Part of the Fourth LIGO-Virgo-KAGRA Observing Run

Authors: The LIGO Scientific Collaboration, the Virgo Collaboration, the KAGRA Collaboration, A. G. Abac, I. Abouelfettouh, F. Acernese, K. Ackley, C. Adamcewicz, S. Adhicary, D. Adhikari, N. Adhikari, R. X. Adhikari, V. K. Adkins, S. Afroz, A. Agapito, D. Agarwal, M. Agathos, N. Aggarwal, S. Aggarwal, O. D. Aguiar, I. -L. Ahrend, L. Aiello, A. Ain, P. Ajith, T. Akutsu , et al. (1748 additional authors not shown)

Abstract: Version 4.0 of the Gravitational-Wave Transient Catalog (GWTC-4.0) adds new candidates detected by the LIGO, Virgo, and KAGRA observatories through the first part of the fourth observing run (O4a: 2023 May 24 15:00:00 to 2024 January 16 16:00:00 UTC) and a preceding engineering run. In this new data, we find 128 new compact binary coalescence candidates that are identified by at least one of our s… ▽ More Version 4.0 of the Gravitational-Wave Transient Catalog (GWTC-4.0) adds new candidates detected by the LIGO, Virgo, and KAGRA observatories through the first part of the fourth observing run (O4a: 2023 May 24 15:00:00 to 2024 January 16 16:00:00 UTC) and a preceding engineering run. In this new data, we find 128 new compact binary coalescence candidates that are identified by at least one of our search algorithms with a probability of astrophysical origin $p_{\rm astro} \geq 0.5$ and that are not vetoed during event validation. We also provide detailed source property measurements for 86 of these that have a false alarm rate $< 1 \rm{yr}^{-1}$. Based on the inferred component masses, these new candidates are consistent with signals from binary black holes and neutron star-black hole binaries (GW230518_125908 and GW230529_181500). Median inferred component masses of binary black holes in the catalog now range from $5.79\,M_\odot$ (GW230627_015337) to $137\,M_\odot$ (GW231123_135430), while GW231123_135430 was probably produced by the most massive binary observed in the catalog. For the first time we have discovered binary black hole signals with network signal-to-noise ratio exceeding 30, GW230814_230901 and GW231226_01520, enabling high-fidelity studies of the waveforms and astrophysical properties of these systems. Combined with the 90 candidates included in GWTC-3.0, the catalog now contains 218 candidates with $p_{\rm astro} \geq 0.5$ and not otherwise vetoed, doubling the size of the catalog and further opening our view of the gravitational-wave Universe. △ Less

Submitted 8 September, 2025; v1 submitted 25 August, 2025; originally announced August 2025.

Comments: As part of the Astrophysical Journal Letters Focus Issue on the Gravitational Wave Transient Catalog

Report number: LIGO-P2400386

Open Data from LIGO, Virgo, and KAGRA through the First Part of the Fourth Observing Run

Authors: The LIGO Scientific Collaboration, the Virgo Collaboration, the KAGRA Collaboration, A. G. Abac, I. Abouelfettouh, F. Acernese, K. Ackley, C. Adamcewicz, S. Adhicary, D. Adhikari, N. Adhikari, R. X. Adhikari, V. K. Adkins, S. Afroz, A. Agapito, D. Agarwal, M. Agathos, N. Aggarwal, S. Aggarwal, O. D. Aguiar, I. -L. Ahrend, L. Aiello, A. Ain, P. Ajith, T. Akutsu , et al. (1746 additional authors not shown)

Abstract: LIGO, Virgo, and KAGRA form a network of gravitational-wave observatories. Data and analysis results from this network are made publicly available through the Gravitational Wave Open Science Center. This paper describes open data from this network, including the addition of data from the first part of the fourth observing run (O4a) and selected periods from the preceding engineering run, collected… ▽ More LIGO, Virgo, and KAGRA form a network of gravitational-wave observatories. Data and analysis results from this network are made publicly available through the Gravitational Wave Open Science Center. This paper describes open data from this network, including the addition of data from the first part of the fourth observing run (O4a) and selected periods from the preceding engineering run, collected from May 2023 to January 2024. The public data set includes calibrated strain time series for each instrument, data from additional channels used for noise subtraction and detector characterization, and analysis data products from version 4.0 of the Gravitational-Wave Transient Catalog. △ Less

Submitted 4 November, 2025; v1 submitted 25 August, 2025; originally announced August 2025.

Comments: 26 pages. The version updates Table 3, updates the author list, removes one figure, and updates some text for clarity and grammar

Report number: LIGO-P2500167

X-ray thermal diffuse scattering as a texture-robust temperature diagnostic for dynamically compressed solids

Authors: P. G. Heighway, D. J. Peake, T. Stevens, J. S. Wark, B. Albertazzi, S. J. Ali, L. Antonelli, M. R. Armstrong, C. Baehtz, O. B. Ball, S. Banerjee, A. B. Belonoshko, C. A. Bolme, V. Bouffetier, R. Briggs, K. Buakor, T. Butcher, S. Di Dio Cafiso, V. Cerantola, J. Chantel, A. Di Cicco, A. L. Coleman, J. Collier, G. Collins, A. J. Comley , et al. (97 additional authors not shown)

Abstract: We present a model of x-ray thermal diffuse scattering (TDS) from a cubic polycrystal with an arbitrary crystallographic texture, based on the classic approach of Warren. We compare the predictions of our model with femtosecond x-ray diffraction patterns obtained from ambient and dynamically compressed rolled copper foils obtained at the High Energy Density (HED) instrument of the European X-Ray F… ▽ More We present a model of x-ray thermal diffuse scattering (TDS) from a cubic polycrystal with an arbitrary crystallographic texture, based on the classic approach of Warren. We compare the predictions of our model with femtosecond x-ray diffraction patterns obtained from ambient and dynamically compressed rolled copper foils obtained at the High Energy Density (HED) instrument of the European X-Ray Free-Electron Laser (EuXFEL), and find that the texture-aware TDS model yields more accurate results than does the conventional powder model owed to Warren. Nevertheless, we further show that: with sufficient angular detector coverage, the TDS signal is largely unchanged by sample orientation and in all cases strongly resembles the signal from a perfectly random powder; shot-to-shot fluctuations in the TDS signal resulting from grain-sampling statistics are at the percent level, in stark contrast to the fluctuations in the Bragg-peak intensities (which are over an order of magnitude greater); and TDS is largely unchanged even following texture evolution caused by compression-induced plastic deformation. We conclude that TDS is robust against texture variation, making it a flexible temperature diagnostic applicable just as well to off-the-shelf commercial foils as to ideal powders. △ Less

Submitted 6 August, 2025; originally announced August 2025.

Comments: 22 pages, 13 figures in main article; 5 pages, 1 figure in supplementary material

A Joint Search for the Electromagnetic Counterpart to the Gravitational-Wave Binary Black-Hole Merger Candidate S250328ae with the Dark Energy Camera and the Prime Focus Spectrograph

Authors: Haibin Zhang, Mitsuru Kokubo, Sean MacBride, Isaac McMahon, Nozomu Tominaga, Yousuke Utsumi, Michitoshi Yoshida, Tomoki Morokuma, Masaomi Tanaka, Akira Arai, Wanqiu He, Yuki Moritani, Masato Onodera, Vera Maria Passegger, Ichi Tanaka, Kiyoto Yabe, Lillian Joseph, Simran Kaur, Hemanth Bommireddy, Nora Sherman, Kenneth Herner, H. Thomas Diehl, Marcelle Soares-Santos

Abstract: The first detection of an optical counterpart to a gravitational wave signal revealed that collaborative efforts between instruments with different specializations provide a unique opportunity to acquire impactful multi-messenger data. We present results of such a joint search with the Dark Energy Camera (DECam) and Prime Focus Spectrograph (PFS) for the optical counterpart of the LIGO-Virgo-KAGRA… ▽ More The first detection of an optical counterpart to a gravitational wave signal revealed that collaborative efforts between instruments with different specializations provide a unique opportunity to acquire impactful multi-messenger data. We present results of such a joint search with the Dark Energy Camera (DECam) and Prime Focus Spectrograph (PFS) for the optical counterpart of the LIGO-Virgo-KAGRA event S250328ae, a binary black hole merger candidate of high significance detected at a distance of 511$\pm$82 Mpc and localized within an area of 3 (15) square degrees at 50% (90%) confidence. We observed the 90% confidence area with DECam and identified 36 high-confidence transient candidates after image processing, candidate selection, and candidate vetting. We observed with PFS to obtain optical spectra of DECam candidates, Swift-XRT candidates, and potential host galaxies of S250328ae. In total, 3897 targets were observed by seven pointings covering ~50% of the 90% confidence area. After template fitting and visual inspection, we identified 12 SNe, 159 QSOs, 2975 galaxies, and 131 stars. With the joint observations of DECam and PFS, we found variability in 12 SNe, 139 QSOs, 37 galaxies, and 2 stars. We do not identify any confident optical counterparts, though the association is not ruled out for three variable candidates that are not observed by PFS and 6 QSO candidates without clear variability if the optical counterpart of S250328ae is faint. Despite the lack of confident optical counterparts, this paper serves as a framework for future collaborations between wide-field imagers and multi-object spectrographs to maximize multi-messenger analyses. △ Less

Submitted 31 July, 2025; originally announced August 2025.

Comments: 15 pages and 8 figures. Submitted to ApJ

All-sky search for long-duration gravitational-wave transients in the first part of the fourth LIGO-Virgo-KAGRA Observing run

Authors: The LIGO Scientific Collaboration, the Virgo Collaboration, the KAGRA Collaboration, A. G. Abac, I. Abouelfettouh, F. Acernese, K. Ackley, C. Adamcewicz, S. Adhicary, D. Adhikari, N. Adhikari, R. X. Adhikari, V. K. Adkins, S. Afroz, A. Agapito, D. Agarwal, M. Agathos, N. Aggarwal, S. Aggarwal, O. D. Aguiar, I. -L. Ahrend, L. Aiello, A. Ain, P. Ajith, T. Akutsu , et al. (1750 additional authors not shown)

Abstract: We present an all-sky search for long-duration gravitational waves (GWs) from the first part of the LIGO-Virgo-KAGRA fourth observing run (O4), called O4a and comprising data taken between 24 May 2023 and 16 January 2024. The GW signals targeted by this search are the so-called "long-duration" (> 1 s) transients expected from a variety of astrophysical processes, including non-axisymmetric deforma… ▽ More We present an all-sky search for long-duration gravitational waves (GWs) from the first part of the LIGO-Virgo-KAGRA fourth observing run (O4), called O4a and comprising data taken between 24 May 2023 and 16 January 2024. The GW signals targeted by this search are the so-called "long-duration" (> 1 s) transients expected from a variety of astrophysical processes, including non-axisymmetric deformations in magnetars or eccentric binary coalescences. We make minimal assumptions on the emitted GW waveforms in terms of morphologies and durations. Overall, our search targets signals with durations ~1-1000 s and frequency content in the range 16-2048 Hz. In the absence of significant detections, we report the sensitivity limits of our search in terms of root-sum-square signal amplitude (hrss) of reference waveforms. These limits improve upon the results from the third LIGO-Virgo-KAGRA observing run (O3) by about 30% on average. Moreover, this analysis demonstrates substantial progress in our ability to search for long-duration GW signals owing to enhancements in pipeline detection efficiencies. As detector sensitivities continue to advance and observational runs grow longer, unmodeled long-duration searches will increasingly be able to explore a range of compelling astrophysical scenarios involving neutron stars and black holes. △ Less

Submitted 23 July, 2025; v1 submitted 16 July, 2025; originally announced July 2025.

Report number: LIGO-P2500090-v6

GW231123: a Binary Black Hole Merger with Total Mass 190-265 $M_{\odot}$

Authors: The LIGO Scientific Collaboration, the Virgo Collaboration, the KAGRA Collaboration, A. G. Abac, I. Abouelfettouh, F. Acernese, K. Ackley, C. Adamcewicz, S. Adhicary, D. Adhikari, N. Adhikari, R. X. Adhikari, V. K. Adkins, S. Afroz, A. Agapito, D. Agarwal, M. Agathos, N. Aggarwal, S. Aggarwal, O. D. Aguiar, I. -L. Ahrend, L. Aiello, A. Ain, P. Ajith, T. Akutsu , et al. (1749 additional authors not shown)

Abstract: On 2023 November 23 the two LIGO observatories both detected GW231123, a gravitational-wave signal consistent with the merger of two black holes with masses $137^{+23}_{-18}\, M_\odot$ and $101^{+22}_{-50}\, M_\odot$ (90\% credible intervals), at luminosity distance 0.7-4.1 Gpc and redshift of $0.40^{+0.27}_{-0.25}$, and a network signal-to-noise ratio of $\sim$20.7. Both black holes exhibit high… ▽ More On 2023 November 23 the two LIGO observatories both detected GW231123, a gravitational-wave signal consistent with the merger of two black holes with masses $137^{+23}_{-18}\, M_\odot$ and $101^{+22}_{-50}\, M_\odot$ (90\% credible intervals), at luminosity distance 0.7-4.1 Gpc and redshift of $0.40^{+0.27}_{-0.25}$, and a network signal-to-noise ratio of $\sim$20.7. Both black holes exhibit high spins, $0.9^{+0.10}_{-0.19}$ and $0.80^{+0.20}_{-0.52}$ respectively. A massive black hole remnant is supported by an independent ringdown analysis. Some properties of GW231123 are subject to large systematic uncertainties, as indicated by differences in inferred parameters between signal models. The primary black hole lies within or above the theorized mass gap where black holes between 60-130 $M_\odot$ should be rare due to pair instability mechanisms, while the secondary spans the gap. The observation of GW231123 therefore suggests the formation of black holes from channels beyond standard stellar collapse, and that intermediate-mass black holes of mass $\sim$200 $M_\odot$ form through gravitational-wave driven mergers. △ Less

Submitted 10 November, 2025; v1 submitted 10 July, 2025; originally announced July 2025.

Comments: 27 pages, 10 figures

Report number: DCC: P2500026-v8

Journal ref: ApJL 993 L25 (2025)

A Careful Examination of Large Behavior Models for Multitask Dexterous Manipulation

Authors: TRI LBM Team, Jose Barreiros, Andrew Beaulieu, Aditya Bhat, Rick Cory, Eric Cousineau, Hongkai Dai, Ching-Hsin Fang, Kunimatsu Hashimoto, Muhammad Zubair Irshad, Masha Itkina, Naveen Kuppuswamy, Kuan-Hui Lee, Katherine Liu, Dale McConachie, Ian McMahon, Haruki Nishimura, Calder Phillips-Grafflin, Charles Richter, Paarth Shah, Krishnan Srinivasan, Blake Wulfe, Chen Xu, Mengchao Zhang, Alex Alspach , et al. (57 additional authors not shown)

Abstract: Robot manipulation has seen tremendous progress in recent years, with imitation learning policies enabling successful performance of dexterous and hard-to-model tasks. Concurrently, scaling data and model size has led to the development of capable language and vision foundation models, motivating large-scale efforts to create general-purpose robot foundation models. While these models have garnere… ▽ More Robot manipulation has seen tremendous progress in recent years, with imitation learning policies enabling successful performance of dexterous and hard-to-model tasks. Concurrently, scaling data and model size has led to the development of capable language and vision foundation models, motivating large-scale efforts to create general-purpose robot foundation models. While these models have garnered significant enthusiasm and investment, meaningful evaluation of real-world performance remains a challenge, limiting both the pace of development and inhibiting a nuanced understanding of current capabilities. In this paper, we rigorously evaluate multitask robot manipulation policies, referred to as Large Behavior Models (LBMs), by extending the Diffusion Policy paradigm across a corpus of simulated and real-world robot data. We propose and validate an evaluation pipeline to rigorously analyze the capabilities of these models with statistical confidence. We compare against single-task baselines through blind, randomized trials in a controlled setting, using both simulation and real-world experiments. We find that multi-task pretraining makes the policies more successful and robust, and enables teaching complex new tasks more quickly, using a fraction of the data when compared to single-task baselines. Moreover, performance predictably increases as pretraining scale and diversity grows. Project page: https://toyotaresearchinstitute.github.io/lbm1/ △ Less

Submitted 7 July, 2025; originally announced July 2025.

Observation of Body-Centered Cubic Iron above 200 Gigapascals

Authors: Zuzana Konopkova, Eric Edmund, Orianna B Ball, Agnes Dewaele, Helene Ginestet, Rachel J Husband, Nicolas Jaisle, Cornelius Strohm, Madden S Anae, Daniele Antonangeli, Karen Appel, Marzena Baron, Silvia Boccato, Khachiwan Buakor, Julien Chantel, Hyunchae Cynn, Anand P Dwivedi, Lars Ehm, Konstantin Glazyrin, Heinz Graafsma, Egor Koemets, Torsten Laurus, Hauke Marquardt, Bernhard Massani, James D McHardy , et al. (12 additional authors not shown)

Abstract: The crystallographic structure of iron under extreme conditions is a key benchmark for cutting-edge experimental and numerical methods. Moreover, it plays a crucial role in understanding planetary cores, as it significantly influences the interpretation of observational data and, consequently, insights into their internal structure and dynamics. However, even the structure of pure solid iron under… ▽ More The crystallographic structure of iron under extreme conditions is a key benchmark for cutting-edge experimental and numerical methods. Moreover, it plays a crucial role in understanding planetary cores, as it significantly influences the interpretation of observational data and, consequently, insights into their internal structure and dynamics. However, even the structure of pure solid iron under the Earth's core conditions remains uncertain, with the commonly expected hexagonal close-packed structure energetically competitive with various cubic lattices. In this study, iron was compressed in a diamond anvil cell to above 200 GPa, and dynamically probed near the melting point using MHz frequency X-ray pulses from the European X-ray Free Electron Laser. The emergence of an additional diffraction line at high temperatures suggests the formation of an entropically stabilized bcc structure. Rapid heating and cooling cycles captured intermediate phases, offering new insights into iron's phase transformation paths. The appearance of the bcc phase near melting at extreme pressures challenges current understanding of the iron phase diagram under Earth's core conditions. △ Less

Submitted 21 May, 2025; originally announced May 2025.

Femtosecond temperature measurements of laser-shocked copper deduced from the intensity of the x-ray thermal diffuse scattering

Authors: J. S. Wark, D. J. Peake, T. Stevens, P. G. Heighway, Y. Ping, P. Sterne, B. Albertazzi, S. J. Ali, L. Antonelli, M. R. Armstrong, C. Baehtz, O. B. Ball, S. Banerjee, A. B. Belonoshko, C. A. Bolme, V. Bouffetier, R. Briggs, K. Buakor, T. Butcher, S. Di Dio Cafiso, V. Cerantola, J. Chantel, A. Di Cicco, A. L. Coleman, J. Collier , et al. (100 additional authors not shown)

Abstract: We present 50-fs, single-shot measurements of the x-ray thermal diffuse scattering (TDS) from copper foils that have been shocked via nanosecond laser-ablation up to pressures above 135~GPa. We hence deduce the x-ray Debye-Waller (DW) factor, providing a temperature measurement. The targets were laser-shocked with the DiPOLE 100-X laser at the High Energy Density (HED) endstation of the European X… ▽ More We present 50-fs, single-shot measurements of the x-ray thermal diffuse scattering (TDS) from copper foils that have been shocked via nanosecond laser-ablation up to pressures above 135~GPa. We hence deduce the x-ray Debye-Waller (DW) factor, providing a temperature measurement. The targets were laser-shocked with the DiPOLE 100-X laser at the High Energy Density (HED) endstation of the European X-ray Free-Electron Laser (EuXFEL). Single x-ray pulses, with a photon energy of 18 keV, were scattered from the samples and recorded on Varex detectors. Despite the targets being highly textured (as evinced by large variations in the elastic scattering), and with such texture changing upon compression, the absolute intensity of the azimuthally averaged inelastic TDS between the Bragg peaks is largely insensitive to these changes, and, allowing for both Compton scattering and the low-level scattering from a sacrificial ablator layer, provides a reliable measurement of $T/Θ_D^2$, where $Θ_D$ is the Debye temperature. We compare our results with the predictions of the SESAME 3336 and LEOS 290 equations of state for copper, and find good agreement within experimental errors. We thus demonstrate that single-shot temperature measurements of dynamically compressed materials can be made via thermal diffuse scattering of XFEL radation. △ Less

Submitted 6 January, 2025; originally announced January 2025.

Comments: 17 pages, 9 figures in main article; 10 pages, 5 figures in supplementary material

Experimental and theoretical confirmation of an orthorhombic phase transition in niobium at high pressure and temperature

Authors: Daniel Errandonea, Leonid Burakovsky, Dean L. Preston, Simon G. MacLeod, David Santamaria-Perez, Shaoping Chen, Hyunchae Cynn, Sergey I. Simak, Malcolm I. McMahon, John E. Proctor, Mohamed Mezouar

Abstract: Compared to other body-centered cubic (bcc) transition metals Nb has been the subject of fewer compression studies and there are still aspects of its phase diagram which are unclear. Here, we report a combined theoretical and experimental study of Nb under high pressure and temperature. We present the results of static laser-heated diamond anvil cell experiments up to 120 GPa using synchrotron-bas… ▽ More Compared to other body-centered cubic (bcc) transition metals Nb has been the subject of fewer compression studies and there are still aspects of its phase diagram which are unclear. Here, we report a combined theoretical and experimental study of Nb under high pressure and temperature. We present the results of static laser-heated diamond anvil cell experiments up to 120 GPa using synchrotron-based fast x-ray diffraction combined with ab initio quantum molecular dynamics simulations. The melting curve of Nb is determined, and evidence for a solid-solid phase transformation in Nb with increasing temperature is found. The high-temperature phase of Nb is orthorhombic Pnma. The bcc-Pnma transition is clearly seen in the experimental data on the Nb principal Hugoniot. The bcc-Pnma coexistence observed in our experiments is explained. Agreement between the measured and calculated melting curves is very good except at 40-60 GPa where three experimental points lie below the theoretical melting curve by 250 K (or 7%); a possible explanation is given. △ Less

Submitted 24 January, 2024; originally announced January 2024.

Comments: 33 pages, 10 figures

Report number: LA-UR-20-27197

Journal ref: COMMUNICATIONS MATERIALS (2020) 1:60

On the Electride Nature of Na-hP4

Authors: Stefano Racioppi, Christian V. Storm, Malcolm I. McMahon, Eva Zurek

Abstract: Early quantum mechanical models suggested that pressure drives solids towards free-electron metal behavior where the ions are locked into simple close-packed structures. The prediction and subsequent discovery of high-pressure electrides (HPEs), compounds assuming open structures where the valence electrons are localized in interstitial voids, required a paradigm shift. Our quantum chemical calcul… ▽ More Early quantum mechanical models suggested that pressure drives solids towards free-electron metal behavior where the ions are locked into simple close-packed structures. The prediction and subsequent discovery of high-pressure electrides (HPEs), compounds assuming open structures where the valence electrons are localized in interstitial voids, required a paradigm shift. Our quantum chemical calculations on the iconic insulating Na-hP4 HPE show that increasing density causes a 3s -> 3pd electronic transition due to Coulomb repulsion between the 1s2s and 3s states, and orthogonality of the 3pd states to the core. The large lobes of the resulting Na-pd hybrid orbitals point towards the center of an 11-membered penta-capped trigonal prism and overlap constructively, forming multi-centered bonds, which are responsible for the emergence of the interstitial charge localization in Na-hP4. These multi-centered bonds facilitate the increased density of this phase, which is key for its stabilization under pressure. △ Less

Submitted 2 November, 2023; originally announced November 2023.

Journal ref: Angew. Chem. Int. Ed. 2023, e202310802

Galaxy Distribution Incompleteness Testing Using Self-Organizing Maps

Authors: Isaac McMahon, Markus Michael Rau, Rachel Mandelbaum

Abstract: The calibration of redshift distributions for photometric samples using spectroscopic surveys is plagued by the difficulty in modelling the selection functions of spectroscopic surveys. In this work, we analyse how these selection functions impact redshift inference and quantify the induced biases using local calibration tests in photometry space. The study is carried out using simulations that mi… ▽ More The calibration of redshift distributions for photometric samples using spectroscopic surveys is plagued by the difficulty in modelling the selection functions of spectroscopic surveys. In this work, we analyse how these selection functions impact redshift inference and quantify the induced biases using local calibration tests in photometry space. The study is carried out using simulations that mimic the radial selection function of a spectroscopic survey and an accompanying mock catalog of a photometric galaxy survey catalog. We use a self-organizing map to partition the photometry space and perform a local $χ^2$ test to study the probability calibration of redshift inferences that use the spectroscopic data for calibration. The goal of this work is to investigate the effect of uncorrected selection functions in the calibration data on redshift prediction accuracy and critically discuss mitigation methods. In particular we test culling-based bias correction techniques, that aim to remove redshift calibration biases by identifying regions in photometry with few spectroscopic calibration data, and propose avenues for future research. We found that removing regions in color-magnitude space that are underpopulated with spectroscopic calibration data does not remove all biases in redshift inference induced by the selection function. △ Less

Submitted 18 July, 2022; originally announced July 2022.

Femtosecond Diffraction and Dynamic High Pressure Science

Authors: Justin S. Wark, Malcolm I. McMahon, Jon H. Eggert

Abstract: Solid state material at high pressure is prevalent throughout the Universe, and an understanding of the structure of matter under such extreme conditions, gleaned from x-ray diffraction, has been pursued for the best part of a century. The highest pressures that can be reached to date (2 TPa) in combination with x-ray diffraction diagnosis have been achieved by dynamic compression via laser ablati… ▽ More Solid state material at high pressure is prevalent throughout the Universe, and an understanding of the structure of matter under such extreme conditions, gleaned from x-ray diffraction, has been pursued for the best part of a century. The highest pressures that can be reached to date (2 TPa) in combination with x-ray diffraction diagnosis have been achieved by dynamic compression via laser ablation . The past decade has witnessed remarkable advances in x-ray technologies, with novel x-ray Free-Electron-Lasers (FELs) affording the capacity to produce high quality single-shot diffraction data on time scales below 100 fsec. We provide a brief history of the field of dynamic compression, spanning from when the x-ray sources were almost always laser-plasma based, to the current state-of-the art diffraction capabilities provided by FELs. We give an overview of the physics of dynamic compression, diagnostic techniques, and the importance of understanding how the rate of compression influences the final temperatures reached. We provide illustrative examples of experiments performed on FEL facilities that are starting to give insight into how materials deform at ultra-high strain rates, their phase diagrams, and the types of states that can be reached. We emphasize that there often appear to be differences in the crystalline phases observed between use of static and dynamic compression techniques. We give our perspective on both the current state of this rapidly evolving field, and some glimpses of how we see it developing in the near-to-medium term. △ Less

Submitted 4 March, 2022; originally announced March 2022.

Comments: 40 pages, 18 figures. This article has been submitted to the Journal of Applied Physics

Non-existence of the s-f transition in structures of solid gadolinium at pressure

Authors: Qingchen Li, Hossein Ehteshami, Keith Munro, Malcolm I McMahon, Graeme J. Ackland

Abstract: Gadolinium has long been believed to undergo a high pressure phase transition with a volume collapse around 5%. Theoretical explanations have focused on the idea of electrons transferring from the extended s-orbital to the compact f-orbital. However, experimental measurement has been unable to detect any associated change in the magnetic properties of the f-electrons. Here we resolve this discrepa… ▽ More Gadolinium has long been believed to undergo a high pressure phase transition with a volume collapse around 5%. Theoretical explanations have focused on the idea of electrons transferring from the extended s-orbital to the compact f-orbital. However, experimental measurement has been unable to detect any associated change in the magnetic properties of the f-electrons. Here we resolve this discrepancy by showing that there is no significant volume collapse, beyond what is typical in high pressure phase transformations. We present density functional theory calculations of solid gadolinium under high pressure using a range of methods, and revisit the experimental situation using X-ray diffraction (XRD). The standard lanthanide pressure-transformation sequence involving different stackings of close-packed planes: hcp to 9R to dhcp to fcc to d-fcc is reproduced. The so-called "volume collapsed" high-pressure phase is shown to be an unusual stacking of close-packed planes, with Fddd symmetry and a density change less than 2%. The distorted fcc (d-fcc) structure is revealed to arise as a consequence of antiferromagnetism. The theoretical results are shown to be remarkably robust to various treatments of the f-electrons. The key result is that there is no XRD evidence for volume collapse in Gadolinium. The sequence of phase transitions is well described by standard DFT. There is no need for special treatment of the f-electrons or evidence of f-electron bonding. Noting previous spectroscopic evidence is that there is no change in the f-electrons we conclude that high pressure Gadolinium has no complicated f-electron physics such as Mott-Hubbard, Kondo or valence transition. △ Less

Submitted 9 September, 2021; v1 submitted 21 July, 2020; originally announced July 2020.

Thermomechanical response of thickly tamped targets and diamond anvil cells under pulsed hard x-ray irradiation

Authors: J. Meza-Galvez, N. Gomez-Perez, A. Marshall, A. L. Coleman, K. Appel, H. P. Liermann, M. I. McMahon, Z. Konopkova, R. S. McWilliams

Abstract: In the laboratory study of extreme conditions of temperature and density, the exposure of matter to high intensity radiation sources has been of central importance. Here we interrogate the performance of multi-layered targets in experiments involving high intensity, hard x-ray irradiation, motivated by the advent of extremely high brightness hard x-ray sources, such as free electron lasers and 4th… ▽ More In the laboratory study of extreme conditions of temperature and density, the exposure of matter to high intensity radiation sources has been of central importance. Here we interrogate the performance of multi-layered targets in experiments involving high intensity, hard x-ray irradiation, motivated by the advent of extremely high brightness hard x-ray sources, such as free electron lasers and 4th-generation synchrotron facilities. Intense hard x-ray beams can deliver significant energy in targets having thick x-ray transparent layers (tampers) around samples of interest, for the study of novel states of matter and materials' dynamics. Heated-state lifetimes in such targets can approach the microsecond level, regardless of radiation pulse duration, enabling the exploration of conditions of local thermal and thermodynamic equilibrium at extreme temperature in solid density matter. The thermal and mechanical response of such thick layered targets following x-ray heating, including hydrodynamic relaxation and heat flow on picosecond to millisecond timescales, is modelled using radiation hydrocode simulation, finite element analysis, and thermodynamic calculations. Assessing the potential for target survival over one or more exposures, and resistance to damage arising from heating and resulting mechanical stresses, this study doubles as an investigation into the performance of diamond-anvil high pressure cells under high x-ray fluences. Long used in conjunction with synchrotron x-ray radiation and high power optical lasers, the strong confinement afforded by such cells suggests novel applications at emerging high intensity x-ray facilities and new routes to studying thermodynamic equilibrium states of warm, very dense matter. △ Less

Submitted 4 December, 2019; v1 submitted 28 June, 2018; originally announced June 2018.

High-pressure high-temperature phase diagram of zinc

Authors: D. Errandonea, S. G. MacLeod, J. Ruiz-Fuertes, L. Burakovsky, M. I. McMahon, C. W. Wilson, J. Ibanez, D. Daisenberger, C. Popescu

Abstract: The phase diagram of Zn has been explored up to 140 GPa and 6000 K, by combining optical observations, x-ray diffraction, and ab-initio calculations. In the pressure range covered by this study, Zn is found to retain a hexagonal close-packed crystal symmetry up to the melting temperature. The known decrease of the axial ratio of the hcp phase of Zn under compression is observed in x-ray diffractio… ▽ More The phase diagram of Zn has been explored up to 140 GPa and 6000 K, by combining optical observations, x-ray diffraction, and ab-initio calculations. In the pressure range covered by this study, Zn is found to retain a hexagonal close-packed crystal symmetry up to the melting temperature. The known decrease of the axial ratio of the hcp phase of Zn under compression is observed in x-ray diffraction experiments from 300 K up to the melting temperature. The pressure at which the axial ratio reaches the square root of 3 value, around 10 GPa, is slightly affected by temperature. When this axial ratio is reached, we observed that single crystals of Zn, formed at high temperature, break into multiple polycrystals. In addition, a noticeable change in the pressure dependence of the axial ratio takes place at the same pressure. Both phenomena could be caused by an isomorphic second-order phase transition induced by pressure in Zn. The reported melt curve extends previous results from 24 to 135 GPa. The pressure dependence obtained for the melting temperature is accurately described up to 135 GPa by using a Simon-Glatzel equation. The determined melt curve agrees with previous low-pressure studies and with shock-wave experiments, with a melting temperature of 5060 K at 135 GPa. Finally, a thermal equation of state is reported, which at room-temperature agrees with the literature. △ Less

Submitted 25 June, 2018; originally announced June 2018.

Comments: 26 pages, 7 figures

Journal ref: J. Phys.: Condens. Matter 30, 295402 (2018)

Thallium under extreme compression

Authors: C. Cazorla, S. G. MacLeod, D. Errandonea, K. A. Munro, M. I. McMahon, C. Popescu

Abstract: We present a combined theoretical and experimental study of the high-pressure behavior of thallium. X-ray diffraction experiments have been carried out at room temperature up to 125 GPa using diamond-anvil cells, nearly doubling the pressure range of previous experiments. We have confirmed the hcp-fcc transition at 3.5 GPa and determined that the fcc structure remains stable up to the highest pres… ▽ More We present a combined theoretical and experimental study of the high-pressure behavior of thallium. X-ray diffraction experiments have been carried out at room temperature up to 125 GPa using diamond-anvil cells, nearly doubling the pressure range of previous experiments. We have confirmed the hcp-fcc transition at 3.5 GPa and determined that the fcc structure remains stable up to the highest pressure attained in the experiments. In addition, HP-HT experiments have been performed up to 8 GPa and 700 K by using a combination of x-ray diffraction and a resistively heated diamond-anvil cell. Information on the phase boundaries is obtained, as well as crystallographic information on the HT bcc phase. The equation of state for different phases is reported. Ab initio calculations have also been carried out considering several potential high-pressure structures. They are consistent with the experimental results and predict that, among the structures considered in the calculations, the fcc structure of thallium is stable up to 4.3 TPa. Calculations also predict the post-fcc phase to have a close-packed orthorhombic structure above 4.3 TPa. △ Less

Submitted 3 October, 2016; originally announced October 2016.

Comments: 29 pages, 14 figures

Journal ref: J. Phys.: Condens. Matter 28 (2016) 445401

Pressure dependence of the structure and electronic properties of Sr3Ir2O7

Authors: C. Donnerer, Z. Feng, J. G. Vale, S. N. Andreev, I. V. Solovyev, E. C. Hunter, M. Hanfland, R. S. Perry, H. M. Rønnow, M. I. McMahon, V. V. Mazurenko, D. F. McMorrow

Abstract: We study the structural evolution of Sr$_3$Ir$_2$O$_7$ as a function of pressure using x-ray diffraction. At a pressure of 54 GPa at room temperature, we observe a first-order structural phase transition, associated with a change from tetragonal to monoclinic symmetry, and accompanied by a 4% volume collapse. Rietveld refinement of the high-pressure phase reveals a novel modification of the Ruddle… ▽ More We study the structural evolution of Sr$_3$Ir$_2$O$_7$ as a function of pressure using x-ray diffraction. At a pressure of 54 GPa at room temperature, we observe a first-order structural phase transition, associated with a change from tetragonal to monoclinic symmetry, and accompanied by a 4% volume collapse. Rietveld refinement of the high-pressure phase reveals a novel modification of the Ruddlesden-Popper structure, which adopts an altered stacking sequence of the perovskite bilayers. As the positions of the oxygen atoms could not be reliably refined from the data, we use density functional theory (local-density approximation+$U$+spin orbit) to optimize the crystal structure, and to elucidate the electronic and magnetic properties of Sr$_3$Ir$_2$O$_7$ at high pressure. In the low-pressure tetragonal phase, we find that the in-plane rotation of the IrO$_6$ octahedra increases with pressure. The calculations further indicate that a bandwidth-driven insulator-metal transition occurs at $\sim$20 GPa, along with a quenching of the magnetic moment. In the high-pressure monoclinic phase, structural optimization resulted in complex tilting and rotation of the oxygen octahedra, and strongly overlapping $t_{2g}$ and $e_g$ bands. The $t_{2g}$ bandwidth renders both the spin-orbit coupling and electronic correlations ineffectual in opening an electronic gap, resulting in a robust metallic state for the high-pressure phase of Sr$_3$Ir$_2$O$_7$. △ Less

Submitted 16 May, 2016; v1 submitted 18 August, 2015; originally announced August 2015.

Comments: 9 pages, 12 figures, accepted in PRB

Journal ref: Phys. Rev. B 93, 174118 (2016)

One-dimensional chain "melting" in incommensurate potassium

Authors: Emma E. McBride, Keith A. Munro, Graham W. Stinton, Rachel J. Husband, Richard Briggs, Hanns-Peter Liermann, Malcolm I. McMahon

Abstract: Between 19 and 54 GPa, potassium has a complex composite incommensurate host-guest structure which undergoes two intraphase transitions over this pressure range. The temperature dependence of these host-guest phases is further complicated by the onset of an order-disorder transition in their guest chains. Here, we report single crystal, quasi-single crystal, and powder synchrotron X-ray diffractio… ▽ More Between 19 and 54 GPa, potassium has a complex composite incommensurate host-guest structure which undergoes two intraphase transitions over this pressure range. The temperature dependence of these host-guest phases is further complicated by the onset of an order-disorder transition in their guest chains. Here, we report single crystal, quasi-single crystal, and powder synchrotron X-ray diffraction measurements of this order-disorder phenomenon in incommensurate potassium to 47 GPa and 750 K. The so-called chain "melting" transition is clearly visible over a 22 GPa pressure range, and there are significant changes in the slope of the phase boundary which divides the ordered and disordered phases, one of which results from the intraphase transitions in the guest structure. △ Less

Submitted 11 April, 2015; originally announced April 2015.

The Structure of Eu-III

Authors: R. J. Husband, I. Loa, G. W. Stinton, S. R. Evans, G. J. Ackland, M. I. McMahon

Abstract: Previous x-ray diffraction studies have reported Eu to transform from the hcp structure to a new phase, Eu-III, at 18 GPa. Using x-ray powder diffraction we have determined that Eu remains hcp up to 33 GPa, and that the extra peaks that appear at 18 GPa are from an impurity phase with space group R-3c . Above 33 GPa the diffraction pattern becomes very much more complex, signalling a transition to… ▽ More Previous x-ray diffraction studies have reported Eu to transform from the hcp structure to a new phase, Eu-III, at 18 GPa. Using x-ray powder diffraction we have determined that Eu remains hcp up to 33 GPa, and that the extra peaks that appear at 18 GPa are from an impurity phase with space group R-3c . Above 33 GPa the diffraction pattern becomes very much more complex, signalling a transition to a phase with a distorted hcp structure. △ Less

Submitted 18 April, 2012; originally announced April 2012.

Comments: 4 pages, 4 figures, AIRAPT-23 Conference, Mumbai, 2011

Journal ref: Journal of Physics: Conference Series 377 (2012) 012030