Showing 1–50 of 69 results for author: Booth, J

Sapphire Photonic Crystal Fiber Sensor

Authors: Mohan Wang, Tongyu Liu, Zipei Song, Richard Reeves, Frank P. Payne, Igor N. Dyson, Kaihui Zhang, Tao Wang, Jian Zhang, Zhitai Jia, Patrick S. Salter, Martin J. Booth, Julian A. J. Fells

Abstract: Sapphire optical fiber shows great promise for remote sensing in extreme environments approaching 2000 degC, by using laser-processing to form a single-mode waveguide within it. However, for practical application, longer devices with high manufacturability and reliability are required. We report the design, modeling, fabrication, and optimization of an index-guiding sapphire photonic crystal fiber… ▽ More Sapphire optical fiber shows great promise for remote sensing in extreme environments approaching 2000 degC, by using laser-processing to form a single-mode waveguide within it. However, for practical application, longer devices with high manufacturability and reliability are required. We report the design, modeling, fabrication, and optimization of an index-guiding sapphire photonic crystal fiber Bragg grating temperature sensor. The device is fabricated using femtosecond laser direct writing to inscribe both the photonic crystal waveguide and the Bragg grating. A spatial light modulator was used to compensate for the mismatch between the immersion objective and the high-index oil used. This improved the aspect ratio and suppressed cracking during fabrication, for higher reliability. The design results in a 6-fold reduction in fabrication time over an equivalent depressed cladding waveguide, significantly reducing the cost of manufacture. Devices up to 7 cm long were fabricated and spliced to standard single-mode fiber. The propagation loss was estimated to be 0.7 dB/cm and the Bragg gratings had a bandwidth of approximately 0.12 nm. Devices were tested in a furnace showing a temperature sensitivity of between 19.0-32.3 pm/degC over a range 25-1200 degC. These longer devices have the potential to enable practical high precision extreme temperature monitoring in many applications, with lower manufacturing cost and higher reliability. △ Less

Submitted 3 May, 2026; originally announced May 2026.

Comments: This work has been submitted to the IEEE for possible publication. 9 pages + 2 pages Supplementary Information

Straight Directional Couplers via Scan-Engineered Index Control

Authors: Mohan Wang, Martin J. Booth, Patrick S. Salter

Abstract: A novel design for straight directional waveguide couplers and interferometers is demonstrated in glass, fabricated using femtosecond laser direct writing and operating at telecommunication wavelengths (~1550 nm). The devices consisted of parallel waveguides with a spacing of 15 um, where the coupling strength was controlled by scan-engineered refractive index modulation along the length of the wa… ▽ More A novel design for straight directional waveguide couplers and interferometers is demonstrated in glass, fabricated using femtosecond laser direct writing and operating at telecommunication wavelengths (~1550 nm). The devices consisted of parallel waveguides with a spacing of 15 um, where the coupling strength was controlled by scan-engineered refractive index modulation along the length of the waveguide. Using this approach, we realized a 50:50 directional coupler formed by two identical waveguides with a footprint of < 40 um x 15 um x 6 mm, as well as a Mach-Zehnder interferometer with unbalanced arms. A waveguide array with 15 um spacing was also demonstrated, highlighting the potential for compact, high-density, and three-dimensional photonic integration. △ Less

Submitted 13 April, 2026; originally announced April 2026.

Consistent initialization of mixed-dimensional multiphysics models for fractured reservoirs under geomechanical constraints and field measurements

Authors: Jakub Wiktor Both, Inga Berre

Abstract: Modeling coupled processes in fractured porous media -- flow, deformation, fracture mechanics, and thermal/chemical effects -- often relies on mixed dimensional multiphysics formulations. These systems are nonlinear and depend on physical states and state dependent material laws. While in-situ field measurements consistently describe the deformed equilibrium configuration, computational models typ… ▽ More Modeling coupled processes in fractured porous media -- flow, deformation, fracture mechanics, and thermal/chemical effects -- often relies on mixed dimensional multiphysics formulations. These systems are nonlinear and depend on physical states and state dependent material laws. While in-situ field measurements consistently describe the deformed equilibrium configuration, computational models typically start from an idealized reference configuration and require explicit initialization of the in-situ stress state. This mismatch complicates initialization and linearization of constitutive laws. As a consequence, due to the two scale nature of fractured media, this can induce large deviations in fracture aperture directly impacting flow predictions. To address this, a discrete fracture model is introduced whose constitutive laws are expressed with respect to the unknown equilibrium state. This is paired with a fixed point initialization strategy that consistently reconstructs the reference configuration, consistent with both geomechanical constraints and field measurements up to load-path dependence. This data-consistent strategy provides a foundation for extending models to more complex scenarios, including multiphase and multicomponent flow in fractured reservoirs. △ Less

Submitted 2 March, 2026; originally announced March 2026.

Depth-adapted adaptive optics for three-photon microscopy

Authors: Qi Hu, Jingyu Wang, Huriye Atilgan, Armin Lak, Martin J. Booth

Abstract: Three-photon (3-P) fluorescence microscopy enables deep in vivo imaging with subcellular resolution, but its performance is fundamentally constrained by the maximum permissible laser power required to avoid tissue heating and photodamage. Under these power-limited conditions, fluorescence signal generation, image contrast, and achievable imaging depth are strongly affected by the illumination beam… ▽ More Three-photon (3-P) fluorescence microscopy enables deep in vivo imaging with subcellular resolution, but its performance is fundamentally constrained by the maximum permissible laser power required to avoid tissue heating and photodamage. Under these power-limited conditions, fluorescence signal generation, image contrast, and achievable imaging depth are strongly affected by the illumination beam profile and aberration correction strategy. In this paper, we showed that using a fixed illumination beam size was suboptimal across different imaging depths. We further showed that conventional Zernike-based adaptive optics (AO) correction degrades under reduced Gaussian illumination beam sizes due to loss of modal orthogonality. This degradation results in slow convergence, unintended focal and field-of-view shifts, and excessive wavefront deformations. To overcome these limitations, we introduced a depth-adapted AO framework in which both the illumination beam profile and the aberration correction basis were dynamically matched to the imaging conditions. By combining depth-optimised beam underfilling with a bespoke set of illumination-matched aberration modes, we achieved faster and more stable AO convergence, enhanced fluorescence signal and image quality during deep in vivo multi-channel neuroimaging. Together, these results established a practical and robust AO-enabled three-photon microscopy strategy that maximised imaging performance under realistic power constraints. △ Less

Submitted 3 March, 2026; v1 submitted 28 February, 2026; originally announced March 2026.

Tunable Dynamic Speckle Generation for Random Illumination Microscopy

Authors: Lilian Magermans, Assia Benachir, Nathan P. Spiller, Tianxin Wang, Federico Vernuccio, Randy Bartels, Stephen M. Morris, Steve J. Elston, Martin J. Booth, Hervé Rigneault

Abstract: Speckled illumination enhances widefield fluorescence microscopy by enabling optical sectioning and super resolution. In random illumination microscopy, sequences of speckled illumination patterns are used to excite fluorescent samples and images are reconstructed based on a statistical analysis of the intensity fluctuations. Although random illumination microscopy has been shown to give excellent… ▽ More Speckled illumination enhances widefield fluorescence microscopy by enabling optical sectioning and super resolution. In random illumination microscopy, sequences of speckled illumination patterns are used to excite fluorescent samples and images are reconstructed based on a statistical analysis of the intensity fluctuations. Although random illumination microscopy has been shown to give excellent performance, its widespread implementation is hindered by the high cost and complexity of the generation of suitable speckled illumination patterns, which is achieved using digital micro-mirror devices or spatial light modulators. Here, we present a zwitterion-doped liquid crystal (LC) device capable of generating independent, high-contrast speckle patterns with a tunable decorrelation time in the 0.1 s to 0.1 ms range under visible laser illumination. This LC-based dynamic speckle generator is applied to widefield random illumination fluorescence microscopy of tissue and cell samples, where it enables optical sectioning with a 2 micron axial resolution, and a 1.5-fold improvement in lateral spatial resolution. Owing to its low cost and simplicity, this LC speckle generator offers an attractive alternative to digital micro-mirror and spatial light modulator devices for implementing widefield random illumination microscopy. △ Less

Submitted 27 February, 2026; originally announced February 2026.

Comments: 12 pages, 6 figures

Journal ref: Advanced Materials Technologies n/a, e02098 (2026)

Oxygen atom density and kinetics in intermediate-pressure radiofrequency capacitively-coupled plasmas in pure O2

Authors: Shu Zhang, Andrey Volynets, Garrett A. Curley, Jean-Paul Booth

Abstract: We have studied radiofrequency capacitively coupled plasmas in pure O2 using single mode laser cavity ringdown spectroscopy of oxygen atoms at 630 nm. The absolute atom densities and translational temperatures were determined over a range of pressures and RF power . At pressures of 267 Pa and above, the O atom mole fraction increases with RF power and decreases with pressure, reaching a maximum of… ▽ More We have studied radiofrequency capacitively coupled plasmas in pure O2 using single mode laser cavity ringdown spectroscopy of oxygen atoms at 630 nm. The absolute atom densities and translational temperatures were determined over a range of pressures and RF power . At pressures of 267 Pa and above, the O atom mole fraction increases with RF power and decreases with pressure, reaching a maximum of 15 percent. However, at 133 and 67 Pa it passes through a distinct maximum with power before decreasing significantly. The atom recombination processes are probed by time resolved measurements in the afterglow of pulse modulated plasmas. At 133 and 67 Pa the atom loss is dominated by surface recombination, and we see clear evidence that this rate is increased by energetic ion bombardment, in agreement with a study from Bill Graham group. This effect partially explains the observed decrease in dissociation at high RF power. The time-resolved results also allow the O negative ion density to be determined and indicate the creation of ozone in the afterglow. At 133 Pa, the trends with RF power of the O2 dissociation, O negative ion density and gas temperature suggest a transition at high power to a plasma mode with fewer high energy electrons. At higher pressures gas phase recombination mechanisms become dominant, however gas convection driven by gas cooling in the afterglow makes it complex to analyse the time-resolved data. △ Less

Submitted 19 January, 2026; originally announced January 2026.

Enhanced and directional light emission from two-dimensional excitons using Mie voids

Authors: Avishek Sarbajna, Ganesh Ghimire, Ilia Breev, Xavier Zambrana-Puyalto, Cheng Xiang, Alexander Huck, Timothy J. Booth, Søren Raza

Abstract: Controlling light emission at the nanoscale has important applications in solid-state lighting, displays, and quantum light sources. Achieving this control requires both enhanced local electromagnetic fields to boost emission intensity and engineered radiation patterns to direct photons efficiently. Mie voids, consisting of an air cavity surrounded by a high-index semiconductor, are particularly s… ▽ More Controlling light emission at the nanoscale has important applications in solid-state lighting, displays, and quantum light sources. Achieving this control requires both enhanced local electromagnetic fields to boost emission intensity and engineered radiation patterns to direct photons efficiently. Mie voids, consisting of an air cavity surrounded by a high-index semiconductor, are particularly suited for this purpose because they expose their strongest fields in an accessible region for nearby emitters while supporting resonances that shape directional emission through interference. Here, we demonstrate an all-van der Waals nanophotonic platform that couples excitons in atomically thin WS$_2$ to Mie void resonators formed in WSe$_2$. Guided by electromagnetic simulations, we identify void geometries that maximize photoluminescence through synergistic enhancement of excitation and emission processes. We also develop a two-step fabrication strategy that enables independent control of void diameter and depth, providing a route to systematically tune the optical response. Experimentally, we observe up to a 600-fold increase in photoluminescence intensity from monolayer WS$_2$ placed on individual voids compared to on an unstructured WSe$_2$, along with pronounced out-of-plane beaming of light that yields a forward-to-off-axis enhancement of 2.6 dB. Our results establish Mie voids in van der Waals semiconductors as a new platform for controlling light-matter interactions and realizing compact, directional, and efficient nanoscale light sources. △ Less

Submitted 19 December, 2025; originally announced December 2025.

Performance of an open-source image-based history matching framework for CO$_2$ storage

Authors: David Landa-Marbán, Tor Harald Sandve, Jakub Wiktor Both, Jan Martin Nordbotten, Sarah Eileen Gasda

Abstract: We present a history matching (HM) workflow applied to the International FluidFlower benchmark study dataset, which features high-resolution images of CO$_2$ storage in a meter-scale, geologically complex reservoir. The dataset provides dense spatial and temporal observations of fluid displacement, offering a rare opportunity to validate and enhance HM techniques for geological carbon storage (GCS… ▽ More We present a history matching (HM) workflow applied to the International FluidFlower benchmark study dataset, which features high-resolution images of CO$_2$ storage in a meter-scale, geologically complex reservoir. The dataset provides dense spatial and temporal observations of fluid displacement, offering a rare opportunity to validate and enhance HM techniques for geological carbon storage (GCS). The combination of detailed experimental data and direct visual observation of flow behavior at this scale is novel and valuable. This study explores the potential and limitations of using experimental data to calibrate standard models for GCS simulation. By leveraging high-resolution images and resulting interpretations of fluid phase distributions, we adjust uncertain parameters and reduce the mismatch between simulation results and observed data. Simulations are performed using the open-source OPM Flow simulator, while the open-source Everest decision-making tool is employed to conduct the HM. After the HM process, the final simulation results show good agreement with the experimental CO$_2$ storage data. This suggests that the system can be effectively described using standard flow equations, conventional saturation functions, and typical PVT properties for CO$_2$-brine mixtures. Our results demonstrate that the Wasserstein distance is a particularly effective metric for matching multi-phase, multi-component flow data. The entire workflow is implemented in a Python package named pofff (Python OPM Flow FluidFlower), which organizes all functionality through a single input file. This design ensures reproducibility and facilitates future extensions of the study. △ Less

Submitted 25 November, 2025; v1 submitted 23 October, 2025; originally announced October 2025.

Laser written waveguides to the sample edge

Authors: Zhi-Kai Pong, Mohan Wang, Ji Qin, Martin J. Booth, Patrick S. Salter

Abstract: A method is presented for fabrication of femtosecond laser written waveguides in glass to remove the need for polishing of substrates after processing. It is shown that by amplitude masking the fabrication laser beam near the sample edge and increasing the pulse energy it is possible to write waveguides that are not affected by edge aberrations and display mode profiles well matched to single mode… ▽ More A method is presented for fabrication of femtosecond laser written waveguides in glass to remove the need for polishing of substrates after processing. It is shown that by amplitude masking the fabrication laser beam near the sample edge and increasing the pulse energy it is possible to write waveguides that are not affected by edge aberrations and display mode profiles well matched to single mode fiber. Results are presented for different depths in fused silica and borosilicate glass substrates. The transmission from fiber to photonic circuit is significantly improved for situations where it is not possible to polish glass substrates after laser writing, creating new opportunities in photonic packaging. △ Less

Submitted 24 February, 2026; v1 submitted 20 October, 2025; originally announced October 2025.

Raman Microspectroscopy for Real-Time Structure Indicator in Ultrafast Laser Writing

Authors: Xingrui Cheng, Eugenio Picheo, Zhixin Chen, Martin J. Booth, Patrick S. Salter, Álvaro Fernández-Galiana

Abstract: Femtosecond laser fabrication enables the creation of a wide range of devices, but its scalability and yield can be limited by the lack of real-time, in-situ monitoring tools. In particular, there is a strong need for metrics that directly correlate with device performance. Raman microspectroscopy provides a non-destructive route for in-situ characterization. Here, we demonstrate its potential to… ▽ More Femtosecond laser fabrication enables the creation of a wide range of devices, but its scalability and yield can be limited by the lack of real-time, in-situ monitoring tools. In particular, there is a strong need for metrics that directly correlate with device performance. Raman microspectroscopy provides a non-destructive route for in-situ characterization. Here, we demonstrate its potential to assess the electrical performance of laser-written graphitic electrodes in diamond. By combining hyperspectral mapping with electrical testing, we show that depletion of the 1332 cm$^{-1}$ sp3 Raman line serves as a monotonic and robust predictor of resistance, offering clear advantages over commonly used spectral features. We further introduce hyperspectral unmixing as a label-free approach to identify relevant spectral signatures in fabrication processes where Raman markers are less defined. Importantly, the methodology we present is not restricted to diamond but can be adapted to other host materials and functionalities, offering a practical path toward specification-driven fs-laser microfabrication. △ Less

Submitted 8 November, 2025; v1 submitted 13 October, 2025; originally announced October 2025.

Trends in porous media laboratory imaging and open science practices

Authors: Na Liu, Jakub Wiktor Both, Geir Ersland, Jan Martin Nordbotten, Martin Fernø

Abstract: Understanding processes in porous media is fundamental to a broad spectrum of environmental, energy, and geoscience applications. These processes include multiphase fluid transport, interfacial dynamics, reactive transformations, and interactions with solids or microbial components, all governed by wettability, capillarity, and reactive transport at fluid-fluid and fluid-solid interfaces. Laborato… ▽ More Understanding processes in porous media is fundamental to a broad spectrum of environmental, energy, and geoscience applications. These processes include multiphase fluid transport, interfacial dynamics, reactive transformations, and interactions with solids or microbial components, all governed by wettability, capillarity, and reactive transport at fluid-fluid and fluid-solid interfaces. Laboratory-based multiscale imaging provides critical insights into these phenomena, enabling direct visualization and quantitative characterization from the nanometer to meter scale. It is essential for advancing predictive models and optimizing the design of subsurface and engineered porous systems. This review presents an integrated overview of imaging techniques relevant to porous media research, emphasizing the type of information each method can provide, their applicability to porous media systems, and their inherent limitations. We highlight how imaging data are combined with quantitative analyses and modeling to bridge pore-scale mechanisms with continuum-scale behavior, and we critically discuss current challenges such as limited spatio-temporal resolution, sample representativity, and restricted data accessibility. We conduct an in-depth analysis on open-science trends in experimental and computational porous media research and find that, while open-access publishing has become widespread, the availability of imaging data and analysis code remains limited, often restricted to 'upon request'. Finally, we underscore the importance of open sharing of imaging datasets to enable reproducibility, foster cross-disciplinary integration, and support the development of robust predictive frameworks for porous media systems. △ Less

Submitted 6 October, 2025; originally announced October 2025.

Comments: Preprint submitted to Advances in Colloid and Interface Science

Single image sensorless adaptive optics for microscopy

Authors: Biwei Zhang, Qi Hu, Jingyu Wang, Martin J. Booth

Abstract: Images obtained by microscopes are generally degraded by aberrations. Adaptive optics (AO) has been widely used in to compensate for aberrations and improve reduced image quality. Requiring no separate wavefront sensor, sensorless AO methods deduce the aberrations from a sequence of images acquired with different phase modulations. Despite that these methods are versatile and flexible, they involv… ▽ More Images obtained by microscopes are generally degraded by aberrations. Adaptive optics (AO) has been widely used in to compensate for aberrations and improve reduced image quality. Requiring no separate wavefront sensor, sensorless AO methods deduce the aberrations from a sequence of images acquired with different phase modulations. Despite that these methods are versatile and flexible, they involve sequential acquisition of multiple images thus time-consuming to implement. Here, we propose a new sensorless AO method based on only a single image. Experimental results on a two-photon fluorescence microscope showed that our method achieved distinct correction while imaging different types of structures under various noise levels with each correction loop taking less than 1 second. This work has significantly accelerated sensorless AO, which will assist its application in many challenging imaging scenarios of microscopy. △ Less

Submitted 22 September, 2025; originally announced September 2025.

Speckle suppression in digital in-line holographic microscopy through liquid crystal dynamic scattering

Authors: Emilia Wdowiak, Nathan Spiller, Tianxin Wang, Camron Nourshargh, Jolanta Mierzejewska, Piotr Zdańkowski, Stephen M. Morris, Steve J. Elston, Maciej Trusiak, Martin J. Booth

Abstract: We demonstrate speckle noise reduction in an in-line holographic imaging system using a Zwitterion-doped liquid crystal dynamic scatterer (LCDS) cell diffuser. Integrated into a minimally modified bright-field microscope, the LCDS actively modulates system's spatial coherence. The proposed solution suppresses coherent artifacts without introducing bulky moving parts, while enhancing image resoluti… ▽ More We demonstrate speckle noise reduction in an in-line holographic imaging system using a Zwitterion-doped liquid crystal dynamic scatterer (LCDS) cell diffuser. Integrated into a minimally modified bright-field microscope, the LCDS actively modulates system's spatial coherence. The proposed solution suppresses coherent artifacts without introducing bulky moving parts, while enhancing image resolution and preserving overall system simplicity. Quantitative performance tested on a phase and amplitude test targets, as well as phase-amplitude biological sample, shows significant noise reduction and methods versatility. Though validated in a holographic in-line setup, the approach is applicable to other imaging techniques requiring compact, vibration-free speckle suppression. △ Less

Submitted 21 August, 2025; originally announced August 2025.

Comments: 4 pages, 3 figures

Gradient Electronic Landscapes in van der Waals Heterostructures

Authors: Nolan Lassaline, Camilla H. Sørensen, Giulia Meucci, Sander J. Linde, Kian Latifi Yaghin, Tuan K. Chau, Damon J. Carrad, Peter Bøggild, Thomas S. Jespersen, Timothy J. Booth

Abstract: Two-dimensional (2D) materials such as graphene and hexagonal boron nitride (hBN) provide a versatile platform for quantum electronics. Experiments generally require encapsulating graphene within hBN flakes, forming a protective van der Waals (vdW) heterostructure that preserves delicate properties of the embedded crystal. To produce functional devices, heterostructures are typically shaped by ele… ▽ More Two-dimensional (2D) materials such as graphene and hexagonal boron nitride (hBN) provide a versatile platform for quantum electronics. Experiments generally require encapsulating graphene within hBN flakes, forming a protective van der Waals (vdW) heterostructure that preserves delicate properties of the embedded crystal. To produce functional devices, heterostructures are typically shaped by electron beam lithography and etching, which has driven progress in 2D materials research. However, patterns are primarily restricted to in-plane geometries such as boxes, holes, and stripes, limiting opportunities for advanced architectures. Here, we use thermal scanning-probe lithography (tSPL) to produce smooth topographic landscapes in vdW heterostructures, controlling the thickness degree of freedom with nanometer precision. We electrically gate a sinusoidal topography to impose an electric-field gradient on the graphene layer to spatially modulate charge-carrier doping. We observe signatures of the landscape in transport measurements-resistance-peak spreading and commensurability oscillations-establishing tSPL for tailoring high-quality quantum electronics. △ Less

Submitted 11 August, 2025; originally announced August 2025.

Benchmarking CO$_2$ Storage Simulations: Results from the 11th Society of Petroleum Engineers Comparative Solution Project

Authors: Jan M. Nordbotten, Martin A. Fernø, Bernd Flemisch, Anthony R. Kovscek, Knut-Andreas Lie, Jakub W. Both, Olav Møyner, Tor Harald Sandve, Etienne Ahusborde, Sebastian Bauer, Zhangxing Chen, Holger Class, Chaojie Di, Didier Ding, David Element, Abbas Firoozabadi, Eric Flauraud, Jacques Franc, Firdovsi Gasanzade, Yousef Ghomian, Marie Ann Giddins, Christopher Green, Bruno R. B. Fernandes, George Hadjisotiriou, Glenn Hammond , et al. (18 additional authors not shown)

Abstract: The 11th Society of Petroleum Engineers Comparative Solution Project (shortened SPE11 herein) benchmarked simulation tools for geological carbon dioxide (CO$_2$) storage. A total of 45 groups from leading research institutions and industry across the globe signed up to participate, with 18 ultimately contributing valid results that were included in the comparative study reported here. This paper… ▽ More The 11th Society of Petroleum Engineers Comparative Solution Project (shortened SPE11 herein) benchmarked simulation tools for geological carbon dioxide (CO$_2$) storage. A total of 45 groups from leading research institutions and industry across the globe signed up to participate, with 18 ultimately contributing valid results that were included in the comparative study reported here. This paper summarizes the SPE11. A comprehensive introduction and qualitative discussion of the submitted data are provided, together with an overview of online resources for accessing the full depth of data. A global metric for analyzing the relative distance between submissions is proposed and used to conduct a quantitative analysis of the submissions. This analysis attempts to statistically resolve the key aspects influencing the variability between submissions. The study shows that the major qualitative variation between the submitted results is related to thermal effects, dissolution-driven convective mixing, and resolution of facies discontinuities. Moreover, a strong dependence on grid resolution is observed across all three versions of the SPE11. However, our quantitative analysis suggests that the observed variations are predominantly influenced by factors not documented in the technical responses provided by the participants. We therefore identify that unreported variations due to human choices within the process of setting up, conducting, and reporting on the simulations underlying each SPE11 submission are at least as impactful as the computational choices reported. △ Less

Submitted 5 July, 2025; originally announced July 2025.

Invariance of quantum scattering rate coefficients to anisotropy of atom-molecule interactions

Authors: Xuyang Guo, Kirk W. Madison, James L. Booth, Roman V. Krems

Abstract: Quantum scattering calculations for strongly interacting molecular systems are computationally demanding due to the large number of molecular states coupled by the anisotropy of atom - molecule interactions. We demonstrate that thermal rate coefficients for total (elastic + inelastic) atom - molecule scattering are insensitive to the interaction anisotropy of the underlying potential energy surfac… ▽ More Quantum scattering calculations for strongly interacting molecular systems are computationally demanding due to the large number of molecular states coupled by the anisotropy of atom - molecule interactions. We demonstrate that thermal rate coefficients for total (elastic + inelastic) atom - molecule scattering are insensitive to the interaction anisotropy of the underlying potential energy surface. In particular, we show that the rate coefficients for Rb-H$_2$ and Rb-N$_2$ scattering at room temperature can be computed to 1% accuracy with anisotropy set to zero, reducing the complexity of coupled channel quantum scattering calculations to numerical solutions of a single differential equation. Our numerical calculations and statistical analysis based on Gaussian process regression elucidate the origin and limitations of the invariance of the total scattering rate coefficients to changes in atom - molecule interaction anisotropy. △ Less

Submitted 2 January, 2026; v1 submitted 4 July, 2025; originally announced July 2025.

Journal ref: Phys. Rev. A 113 (2026), 012801

Information-guided optimization of image-based sensorless adaptive optics methods

Authors: Biwei Zhang, Martin J. Booth, Qi Hu

Abstract: Adaptive optics (AO) are reconfigurable devices that compensate for wavefront distortions or aberrations in optical systems such as microscopes, telescopes and ophthalmoscopes. Aberrations have detrimental effects that can reduce imaging quality and compromise scientific information. Sensorless AO methods were introduced to correct aberrations without a separate wavefront sensor, inferring wavefro… ▽ More Adaptive optics (AO) are reconfigurable devices that compensate for wavefront distortions or aberrations in optical systems such as microscopes, telescopes and ophthalmoscopes. Aberrations have detrimental effects that can reduce imaging quality and compromise scientific information. Sensorless AO methods were introduced to correct aberrations without a separate wavefront sensor, inferring wavefront-related information directly from phase-diverse sample images. Most sensorless AO control systems, although effective and flexible to use, were operated based on empirical experience with suboptimal performance. In this paper, we introduced a Fisher information-based analysis framework to provide information-guided method optimization. Results suggested that our framework can effectively improve the accuracy and efficiency of different sensorless AO methods. The framework is not specific to any AO method or imaging modality and has the potential to benefit a wide range of applications. △ Less

Submitted 9 June, 2025; originally announced June 2025.

Comments: Submitted to Optics Express

Fourier-Tailored Light-Matter Coupling in van der Waals Heterostructures

Authors: Dorte R. Danielsen, Nolan Lassaline, Sander J. Linde, Magnus V. Nielsen, Xavier Zambrana-Puyalto, Avishek Sarbajna, Duc Hieu Nguyen, Timothy J. Booth, Nicolas Stenger, Søren Raza

Abstract: Dielectric structures can support low-absorption optical modes, which are attractive for engineering light-matter interactions with excitonic resonances in two-dimensional (2D) materials. However, the coupling strength is often limited by the electromagnetic field being confined inside the dielectric, reducing spatial overlap with the active excitonic material. Here, we demonstrate a scheme for en… ▽ More Dielectric structures can support low-absorption optical modes, which are attractive for engineering light-matter interactions with excitonic resonances in two-dimensional (2D) materials. However, the coupling strength is often limited by the electromagnetic field being confined inside the dielectric, reducing spatial overlap with the active excitonic material. Here, we demonstrate a scheme for enhanced light-matter coupling by embedding excitonic tungsten disulfide (WS$_2$) within dielectric hexagonal boron nitride (hBN), forming a van der Waals (vdW) heterostructure that optimizes the field overlap and alignment between excitons and optical waveguide modes. To tailor diffractive coupling between free-space light and the waveguide modes in the vdW heterostructure, we fabricate Fourier surfaces in the top hBN layer using thermal scanning-probe lithography and etching, producing sinusoidal topographic landscapes with nanometer precision. We observe the formation of exciton-polaritons with a Rabi splitting indicating that the system is at the onset of strong coupling. These results demonstrate the potential of Fourier-tailored vdW heterostructures for exploring advanced optoelectronic and quantum devices. △ Less

Submitted 4 February, 2025; originally announced February 2025.

Recommendations and tools to enable reproducibility in 2D materials research

Authors: Peter Bøggild, Timothy John Booth, Bjarke Sørensen Jessen, Abhay Shivayogimath, Nolan Lassaline, Stephan Hofmann, Kim Daasbjerg, Anders Smith, Kasper Nørgaard, Amaia Zurutuza, Terrance Barkan, Andrew J. Pollard

Abstract: Research on 2D materials has achieved significant milestones and fuelled a rapidly growing industrial sector. This progress, however, is accompanied by challenges in reproducibility, arising from the atomic thinness, fragility, and environmental sensitivity of these materials. Subtle variations in methods or materials can lead to drastically different outcomes, undermining reliability and slowing… ▽ More Research on 2D materials has achieved significant milestones and fuelled a rapidly growing industrial sector. This progress, however, is accompanied by challenges in reproducibility, arising from the atomic thinness, fragility, and environmental sensitivity of these materials. Subtle variations in methods or materials can lead to drastically different outcomes, undermining reliability and slowing down both scientific and technological advances. At the same time, academic publishing and funding systems continue to place greater value on novelty than on efforts to improve reproducibility. This Expert Recommendation outlines concrete, actions researchers can take to improve reproducibility in 2D materials science. We introduce two tools - STEP (Standardised Template for Experimental Procedures) and ReChart (Reproducibility Charter) - designed to support rigorous documentation and transparent sharing of protocols, failure modes, and raw data. To illustrate the application of STEP, we provide three detailed examples covering key processes in 2D materials research: graphene growth by chemical vapour deposition (CVD) on copper foil, wet transfer of CVD graphene, and dry assembly of van der Waals heterostructures. We offer practical recommendations that spans the full research process and show how researchers can engage constructively with stakeholders across academia, funding, publishing, and industry to create a stronger basis for reproducibility, transparency and trust in the field. △ Less

Submitted 9 October, 2025; v1 submitted 18 September, 2024; originally announced September 2024.

Comments: 24 pages, 2 tables, 1 figure

Laser-written scalable sapphire integrated photonics platform

Authors: Mohan Wang, Patrick S. Salter, Frank P. Payne, Tongyu Liu, Martin J. Booth, Julian A. J. Fells

Abstract: In this paper, we demonstrate the integration of photonic devices on sapphire substrates using multi-layer depressed cladding waveguides at both 780 nm and 1550 nm. The devices are up to 10-cm long and written at depths down to 400 um. The propagation losses for single-mode guiding are ~ 0.6 dB/cm at 780 nm and ~ 0.7 dB/cm at 1550 nm. A number of structures have been fabricated with simultaneous s… ▽ More In this paper, we demonstrate the integration of photonic devices on sapphire substrates using multi-layer depressed cladding waveguides at both 780 nm and 1550 nm. The devices are up to 10-cm long and written at depths down to 400 um. The propagation losses for single-mode guiding are ~ 0.6 dB/cm at 780 nm and ~ 0.7 dB/cm at 1550 nm. A number of structures have been fabricated with simultaneous single-mode and polarization independent operation: evanescently coupled waveguide arrays, Y-branch splitters, Mach-Zehnder interferometers, and a 2x2 directional-coupler. All the devices were fabricated using adaptive optics-assisted femtosecond laser direct writing with a customized laser writing algorithm. This work enables the integration of single-mode sapphire photonics devices in a scalable manner, enabling many applications in communications, imaging, computing, and sensing. △ Less

Submitted 19 September, 2024; originally announced September 2024.

Boundaries of universality of thermal collisions for atom-atom scattering

Authors: Xuyang Guo, Kirk W. Madison, James L. Booth, Roman V. Krems

Abstract: Thermal rate coefficients for some atomic collisions have been observed to be remarkably independent of the details of interatomic interactions at short range. This makes these rate coefficients universal functions of the long-range interaction parameters and masses, which was previously exploited to develop a self-defining atomic sensor for ambient pressure. Here, we employ rigorous quantum scatt… ▽ More Thermal rate coefficients for some atomic collisions have been observed to be remarkably independent of the details of interatomic interactions at short range. This makes these rate coefficients universal functions of the long-range interaction parameters and masses, which was previously exploited to develop a self-defining atomic sensor for ambient pressure. Here, we employ rigorous quantum scattering calculations to examine the response of thermally averaged rate coefficients for atom-atom collisions to changes in the interaction potentials. We perform a comprehensive analysis of the universality, and the boundaries thereof, by treating the quantum scattering observables as probabilistic predictions determined by a distribution of interaction potentials. We show that there is a characteristic change of the resulting distributions of rate coefficients, separating light, few-electron atoms and heavy, polarizable atoms. We produce diagrams that illustrate the boundaries of the thermal collision universality at different temperatures and provide guidance for future experiments seeking to exploit the universality. △ Less

Submitted 19 December, 2024; v1 submitted 30 August, 2024; originally announced September 2024.

Journal ref: Phys. Rev. A 110, 063317 (2024)

Revising the Universality Hypothesis for Room-temperature Collisions

Authors: James L. Booth, Kirk W. Madison

Abstract: Atoms constitute promising quantum sensors for a variety of scenarios including vacuum metrology. Key to this application is knowledge of the collision rate coefficient of the sensor atom with the particles being detected. Prior work demonstrated that, for room-temperature collisions, the total collision rate coefficient and the trap depth dependence of the sensor atom loss rate from shallow traps… ▽ More Atoms constitute promising quantum sensors for a variety of scenarios including vacuum metrology. Key to this application is knowledge of the collision rate coefficient of the sensor atom with the particles being detected. Prior work demonstrated that, for room-temperature collisions, the total collision rate coefficient and the trap depth dependence of the sensor atom loss rate from shallow traps are both universal, independent of the interaction potential at short range. It was also shown that measurements of the energy transferred to the sensor atom by the collision can be used to estimate the total collision rate coefficient. However, discrepancies found when comparing the results of this and other methods of deducing the rate coefficient call into question its accuracy. Here the universality hypothesis is re-examined and an important correction is presented. We find that measurements of the post-collision recoil energy of sensor atoms held in shallow magnetic traps only provide information about the interaction potential at the very largest inter-atomic distances (e.g.~the value of $C_6$ for a leading order term of $C_6/r^6$). As other non-negligible terms exist at medium and long ranges, the total collision rate coefficient, even if universal, can differ from that computed solely from the value of $C_6$. By incorporating these other long-range terms into a simple semi-classical (SC) calculation, we find the SC prediction matches that of full, multi-channel, quantum mechanical scattering calculations using the complete potential. This work resolves the discrepancies, demonstrates the simplicity of estimating the rate coefficients for universal collision partners, and provides guidance for using atoms as a self-calibrating primary quantum pressure standard. △ Less

Submitted 10 September, 2024; v1 submitted 24 June, 2024; originally announced June 2024.

Comments: 20 pages, 9 figures

Intensity adaptive optics

Authors: Zimo Zhao, Yifei Ma, Zipei Song, Jacopo Antonello, Jiahe Cui, Binguo Chen, Jingyu Wang, Bangshan Sun, Honghui He, Lin Luo, Julian A. J. Fells, Steve J. Elston, Martin J. Booth, Stephen M. Morris, Chao He

Abstract: Adaptive optics (AO) is a powerful tool employed across various research fields, from aerospace to microscopy. Traditionally, AO has focused on correcting optical phase aberrations, with recent advances extending to polarisation compensation. However, intensity errors are also prevalent in optical systems, yet effective correction methods are still in their infancy. Here, we introduce a novel AO a… ▽ More Adaptive optics (AO) is a powerful tool employed across various research fields, from aerospace to microscopy. Traditionally, AO has focused on correcting optical phase aberrations, with recent advances extending to polarisation compensation. However, intensity errors are also prevalent in optical systems, yet effective correction methods are still in their infancy. Here, we introduce a novel AO approach, termed intensity adaptive optics (I-AO), which employs a dual-feedback loop mechanism to first address non-uniform intensity distribution and subsequently compensate for energy loss at the pupil plane. We demonstrate that I-AO can operate in both sensor-based and sensorless formats and validate its feasibility by quantitatively analysing the focus quality of an aberrated system. This technique expands the AO toolkit, paving the way for next-generation AO technology. △ Less

Submitted 17 March, 2025; v1 submitted 25 May, 2024; originally announced May 2024.

Topological Protection of Optical Skyrmions through Complex Media

Authors: An Aloysius Wang, Zimo Zhao, Yifei Ma, Yuxi Cai, Runchen Zhang, Xiaoyi Shang, Yunqi Zhang, Ji Qin, Zhi Kai Pong, Tade Marozsak, Binguo Chen, Honghui He, Lin Luo, Martin J Booth, Steve J Elston, Stephen M Morris, Chao He

Abstract: Optical Skyrmions have many important properties that make them ideal units for high-density data applications, including the ability to carry digital information through a discrete topological number and the independence of spatially varying polarization to other dimensions. More importantly, the topological nature of the optical Skyrmion heuristically suggests a strong degree of robustness to pe… ▽ More Optical Skyrmions have many important properties that make them ideal units for high-density data applications, including the ability to carry digital information through a discrete topological number and the independence of spatially varying polarization to other dimensions. More importantly, the topological nature of the optical Skyrmion heuristically suggests a strong degree of robustness to perturbations, which is crucial for reliably carrying information in noisy environments. However, the study of the topological robustness of optical Skyrmions is still in its infancy. Here, we quantify this robustness precisely by proving that the topological nature of the Skyrmion arises from its structure on the boundary and, by duality, is therefore resilient to complex perturbations provided they respect the relevant boundary conditions of the unperturbed Skyrmion. We then present experimental evidence validating this robustness in the context of paraxial Skyrmion beams against different polarization aberrations. Our work provides a framework for handling various perturbations of Skyrmion fields and offers guarantees of robustness in a general sense. This, in turn, has implications for applications of the optical Skyrmion where their topological nature is exploited explicitly, and, in particular, provides an underpinning for the use of Skyrmions in optical communications and photonic computing. △ Less

Submitted 6 August, 2024; v1 submitted 12 March, 2024; originally announced March 2024.

Cross-calibration of atomic sensors for pressure metrology

Authors: Erik Frieling, Riley A. Stewart, James L. Booth, Kirk W. Madison

Abstract: Atomic sensors have shown great promise for density and pressure metrology in the high, ultra-high, and extremely-high vacuum regimes. Specifically, the density of background gas particles in vacuum can be determined by measuring the collision rate between the particles and an ensemble of sensor atoms. This requires preparing the sensor atoms in a particular quantum state, observing the rate of ch… ▽ More Atomic sensors have shown great promise for density and pressure metrology in the high, ultra-high, and extremely-high vacuum regimes. Specifically, the density of background gas particles in vacuum can be determined by measuring the collision rate between the particles and an ensemble of sensor atoms. This requires preparing the sensor atoms in a particular quantum state, observing the rate of changes of that state, and using the cross section coefficient for state-changing collisions to convert the rate into a corresponding density. The cross section can be known by various methods including by quantum scattering calculations using an ansatz for the interaction potential between the collision pair, by measurements of the post-collision sensor-atom momentum recoil distribution, or by empirical calibration of the sensor atom at a known density. Identifying systematic errors in the results of these methods can be aided by direct comparisons between them. Alternatively, measurements of different sensor atoms exposed to the same background gas offers another point of comparison free of the systematic errors inherent in creating a background gas at a known density. Here, we present such measurements for two sensor atoms, $^{87}$Rb and $^6$Li, and a variety of atomic and molecular background gases including H$_2$, N$_2$, Ar, Ne, Kr, and Xe. We find results consistent with, yet statistically different at the level of 3.5(5)%, from recent theoretical and experiment measurements. This work demonstrates a model-free method for transferring the primacy of one atomic standard to another sensor atom and highlights the utility of sensor-atom cross-calibration experiments to check the validity of direct measurements and theoretical predictions. △ Less

Submitted 2 April, 2024; v1 submitted 24 December, 2023; originally announced December 2023.

Comments: 17 pages, 7 figures

High-fidelity experimental model verification for flow in fractured porous media

Authors: Jakub Wiktor Both, Bergit Brattekås, Martin Fernø, Eirik Keilegavlen, Jan Martin Nordbotten

Abstract: Mixed-dimensional mathematical models for flow in fractured media have been prevalent in the modeling community for almost two decades, utilizing the explicit representation of fractures by lower-dimensional manifolds embedded in the surrounding porous media. In this work, for the first time, direct qualitative and quantitative comparisons of mixed-dimensional models are drawn against laboratory e… ▽ More Mixed-dimensional mathematical models for flow in fractured media have been prevalent in the modeling community for almost two decades, utilizing the explicit representation of fractures by lower-dimensional manifolds embedded in the surrounding porous media. In this work, for the first time, direct qualitative and quantitative comparisons of mixed-dimensional models are drawn against laboratory experiments. Dedicated displacement experiments of steady-state laminar flow in fractured media are investigated using both high-resolution PET images as well as state-of-the-art numerical simulations. △ Less

Submitted 22 December, 2023; originally announced December 2023.

A reconfigurable arbitrary retarder array as complex structured matter

Authors: Chao He, Binguo Chen, Zipei Song, Zimo Zhao, Yifei Ma, Honghui He, Lin Luo, Tade Marozsak, An Wang, Rui Xu, Peixiang Huang, Jiawen Li, Xuke Qiu, Yunqi Zhang, Bangshan Sun, Jiahe Cui, Yuxi Cai, Yun Zhang, Andong Wang, Mohan Wang, Patrick Salter, Julian AJ Fells, Ben Dai, Shaoxiong Liu, Limei Guo , et al. (9 additional authors not shown)

Abstract: Tuneable retarder arrays, such as spatially patterned liquid crystal devices, have given rise to impressive photonic functionality, fuelling diverse applications ranging from microscopy and holography to encryption and communications. Presently these solutions are limited by the controllable degrees of freedom of structured matter, hindering applications that demand photonic systems with high flex… ▽ More Tuneable retarder arrays, such as spatially patterned liquid crystal devices, have given rise to impressive photonic functionality, fuelling diverse applications ranging from microscopy and holography to encryption and communications. Presently these solutions are limited by the controllable degrees of freedom of structured matter, hindering applications that demand photonic systems with high flexibility and reconfigurable topologies. Here we demonstrate a compound modulator that implements a synthetic tuneable arbitrary retarder array as virtual pixels derived by cascading low functionality tuneable devices, realising full dynamic control of its arbitrary elliptical axis geometry, retardance value, and induced phase. Our approach offers unprecedented functionality that is user-defined and possesses high flexibility, allowing our modulator to act as a new beam generator, analyser, and corrector, opening an exciting path to tuneable topologies of light and matter. △ Less

Submitted 19 July, 2025; v1 submitted 29 November, 2023; originally announced November 2023.

Polarization based modulation of splitting ratio in femtosecond laser direct written directional couplers

Authors: Zhi-Kai Pong, Bangshan Sun, Patrick S. Salter, Martin J. Booth

Abstract: This work characterizes a phenomenon in direct laser written directional couplers where the splitting ratio for output light is dependent on the input polarization state. In general, for laser written waveguides, different coupling strengths exist for different polarization states of the input light. If the linear polarization state of the input light is not aligned with one of the symmetry axes o… ▽ More This work characterizes a phenomenon in direct laser written directional couplers where the splitting ratio for output light is dependent on the input polarization state. In general, for laser written waveguides, different coupling strengths exist for different polarization states of the input light. If the linear polarization state of the input light is not aligned with one of the symmetry axes of the system, an additional amplitude beating is imposed on the transfer of light in directional couplers of different interaction length. We present results for in-plane and out of plane directional couplers, which are supported by theoretical analysis. These new results provide insights for understanding and controlling polarization properties of directional couplers and larger photonic circuits. △ Less

Submitted 4 December, 2023; v1 submitted 20 November, 2023; originally announced November 2023.

Journal ref: Optics Communications (2025) Vol. 575 Pages 131303

Low Cross-Talk Optical Addressing of Trapped-Ion Qubits Using a Novel Integrated Photonic Chip

Authors: A. S. Sotirova, B. Sun, J. D. Leppard, A. Wang, M. Wang, A. Vazquez-Brennan, D. P. Nadlinger, S. Moser, A. Jesacher, C. He, F. Pokorny, M. J. Booth, C. J. Ballance

Abstract: Individual optical addressing in chains of trapped atomic ions requires generation of many small, closely spaced beams with low cross-talk. Furthermore, implementing parallel operations necessitates phase, frequency, and amplitude control of each individual beam. Here we present a scalable method for achieving all of these capabilities using a novel integrated photonic chip coupled to a network of… ▽ More Individual optical addressing in chains of trapped atomic ions requires generation of many small, closely spaced beams with low cross-talk. Furthermore, implementing parallel operations necessitates phase, frequency, and amplitude control of each individual beam. Here we present a scalable method for achieving all of these capabilities using a novel integrated photonic chip coupled to a network of optical fibre components. The chip design results in very low cross-talk between neighbouring channels even at the micrometre-scale spacing by implementing a very high refractive index contrast between the channel core and cladding. Furthermore, the photonic chip manufacturing procedure is highly flexible, allowing for the creation of devices with an arbitrary number of channels as well as non-uniform channel spacing at the chip output. We present the system used to integrate the chip within our ion trap apparatus and characterise the performance of the full individual addressing setup using a single trapped ion as a light-field sensor. Our measurements showed intensity cross-talk below $10^{-3}$ across the chip, with minimum observed cross-talk as low as $O\left(10^{-5}\right)$. △ Less

Submitted 20 October, 2023; originally announced October 2023.

Comments: 14 pages, 12 figures

Terahertz s-SNOM reveals nonlocal nanoscale conductivity of graphene

Authors: Henrik B. Lassen, William V. Carstensen, Leonid Iliushyn, Timothy J. Booth, Peter Bøggild, Edmund J. R. Kelleher, Peter U. Jepsen

Abstract: As photonic and electronic technologies approach nanometre length scales and terahertz operating speeds, electrical conductivity can no longer be treated as a purely local material parameter. In this regime, charge transport becomes intrinsically nonlocal, with conductivity depending on both frequency and momentum, $σ(ω,q)$, fundamentally limiting field confinement, dispersion, and loss in nanosca… ▽ More As photonic and electronic technologies approach nanometre length scales and terahertz operating speeds, electrical conductivity can no longer be treated as a purely local material parameter. In this regime, charge transport becomes intrinsically nonlocal, with conductivity depending on both frequency and momentum, $σ(ω,q)$, fundamentally limiting field confinement, dispersion, and loss in nanoscale devices. Here, we directly measure the nonlocal nanoscale conductivity of graphene using terahertz scattering-type near-field optical microscopy. By combining broadband THz near-field spectroscopy with quantitative electrodynamic modelling, we extract the complex conductivity of single- and few-layer graphene with $\sim$50 nm spatial resolution. We find that nonlocal response dominates the terahertz conductivity of monolayer graphene even at length scales comparable to practical device dimensions. These results establish nonlocal conductivity as a measurable and design-relevant material property in the terahertz regime, providing a quantitative foundation for predicting performance limits in ultracompact photonic and electronic systems. △ Less

Submitted 13 February, 2026; v1 submitted 11 October, 2023; originally announced October 2023.

Trapped particle evolution driven by residual gas collisions

Authors: Avinash Deshmukh, Riley A. Stewart, Pinrui Shen, James L. Booth, Kirk W. Madison

Abstract: We present a comprehensive mathematical model and experimental measurements for the evolution of a trapped particle ensemble driven by collisions with a room-temperature background vapor. The model accommodates any trap geometry, confining potential, initial trapped distribution, and other experimental details; it only depends on the the probability distribution function $P_t(E)$ for the collision… ▽ More We present a comprehensive mathematical model and experimental measurements for the evolution of a trapped particle ensemble driven by collisions with a room-temperature background vapor. The model accommodates any trap geometry, confining potential, initial trapped distribution, and other experimental details; it only depends on the the probability distribution function $P_t(E)$ for the collision-induced energy transfer to the trapped ensemble. We describe how to find $P_t(E)$ using quantum scattering calculations and how it can be approximated using quantum diffractive universality. We then compare our model to experimental measurements of a $^{87}$Rb ensemble energy evolution exposed to a room temperature background gas of Ar by means of a single parameter fit for the total collision rate $Γ$. We extracted a collision rate of $Γ= 0.646(1)\ \text{s}^{-1}$. This is compared to a value of $0.664(4)\ \text{s}^{-1}$ found by the commonly used method of zero-trap depth extrapolation, a $2.8\%$ correction that is a result of our model fully taking ensemble loss and heating into account. Finally, we report a five-fold increase in the precision of our collision rate extraction from the experimental data. △ Less

Submitted 28 May, 2024; v1 submitted 6 October, 2023; originally announced October 2023.

Comments: 14 pages, 6 figures

Journal ref: Phys. Rev. A Vol. 109, Iss. 3 March 2024

High-precision optical fiber sensing beyond 1000°C

Authors: Mohan Wang, Patrick S. Salter, Frank P. Payne, Adrian Shipley, Igor N. Dyson, Tongyu Lui, 1tao Wang, Kaihui Zhang, Jian Zhang, Zhitai Jia, Stephen M. Morris, Martin J. Booth, Julian A. J. Fells

Abstract: Sapphire fiber can withstand around 2000°C, but it is multimoded, giving poor precision sensors. We demonstrate a single-mode sapphire fiber Bragg grating temperature sensor operating up to 1200°C. The repeatability above 1000°C is within {\pm}0.08%. Sapphire fiber can withstand around 2000°C, but it is multimoded, giving poor precision sensors. We demonstrate a single-mode sapphire fiber Bragg grating temperature sensor operating up to 1200°C. The repeatability above 1000°C is within {\pm}0.08%. △ Less

Submitted 14 August, 2023; originally announced September 2023.

Comments: 4 Pages, 5 Figures

High Speed Precise Refractive Index Modification for Photonic Chips through Phase Aberrated Pulsed Lasers

Authors: Bangshan Sun, Simon Moser, Alexander Jesacher, Patrick S. Salter, Robert R. Thomson, Martin J. Booth

Abstract: Integrated photonic chips have significant potential in telecommunications, classic computing, quantum systems, and topological photonics. Direct laser writing offers unique capability for creating three-dimensional photonic devices in an optical glass chip with quick prototyping. However, existing laser writing schemes cannot create index-modified structures in glass that precisely match the lase… ▽ More Integrated photonic chips have significant potential in telecommunications, classic computing, quantum systems, and topological photonics. Direct laser writing offers unique capability for creating three-dimensional photonic devices in an optical glass chip with quick prototyping. However, existing laser writing schemes cannot create index-modified structures in glass that precisely match the laser focal shape while also achieving high scanning speed and high refractive index contrast. Here, we introduce the theory of a refractive index modification scheme that combines the advantages of both traditional non-thermal and thermal regime fabrication methods. We also propose a model of waveguide formation that was verified through a thorough study on the effects of phase aberrations on the laser focus. The presented new photonic chip fabrication scheme uses a novel focal intensity distribution, where pulse energy is relocated to the bottom of a laser focus by manipulating primary and higher order spherical aberrations. The technique can produce index modifications with high scanning speed (20 mm/s or higher), high index contrast (16 x 10-3), and high precision to fabricate with arbitrary cross-sections. This method has potential to expand the capabilities of photonic chips in applications that require small-scale, high precision, or high contrast refractive index control. △ Less

Submitted 26 July, 2023; originally announced July 2023.

The LHCb upgrade I

Authors: LHCb collaboration, R. Aaij, A. S. W. Abdelmotteleb, C. Abellan Beteta, F. Abudinén, C. Achard, T. Ackernley, B. Adeva, M. Adinolfi, P. Adlarson, H. Afsharnia, C. Agapopoulou, C. A. Aidala, Z. Ajaltouni, S. Akar, K. Akiba, P. Albicocco, J. Albrecht, F. Alessio, M. Alexander, A. Alfonso Albero, Z. Aliouche, P. Alvarez Cartelle, R. Amalric, S. Amato , et al. (1298 additional authors not shown)

Abstract: The LHCb upgrade represents a major change of the experiment. The detectors have been almost completely renewed to allow running at an instantaneous luminosity five times larger than that of the previous running periods. Readout of all detectors into an all-software trigger is central to the new design, facilitating the reconstruction of events at the maximum LHC interaction rate, and their select… ▽ More The LHCb upgrade represents a major change of the experiment. The detectors have been almost completely renewed to allow running at an instantaneous luminosity five times larger than that of the previous running periods. Readout of all detectors into an all-software trigger is central to the new design, facilitating the reconstruction of events at the maximum LHC interaction rate, and their selection in real time. The experiment's tracking system has been completely upgraded with a new pixel vertex detector, a silicon tracker upstream of the dipole magnet and three scintillating fibre tracking stations downstream of the magnet. The whole photon detection system of the RICH detectors has been renewed and the readout electronics of the calorimeter and muon systems have been fully overhauled. The first stage of the all-software trigger is implemented on a GPU farm. The output of the trigger provides a combination of totally reconstructed physics objects, such as tracks and vertices, ready for final analysis, and of entire events which need further offline reprocessing. This scheme required a complete revision of the computing model and rewriting of the experiment's software. △ Less

Submitted 10 September, 2024; v1 submitted 17 May, 2023; originally announced May 2023.

Comments: All figures and tables, along with any supplementary material and additional information, are available at http://lhcbproject.web.cern.ch/lhcbproject/Publications/LHCbProjectPublic/LHCb-DP-2022-002.html (LHCb public pages)

Report number: LHCb-DP-2022-002

Journal ref: JINST 19 (2024) P05065

Topologically controlled multiskyrmions in photonic gradient-index lenses

Authors: Yijie Shen, Chao He, Zipei Song, Binguo Chen, Honghui He, Yifei Ma, Julian A. J. Fells, Steve J. Elston, Stephen M. Morris, Martin J. Booth, Andrew Forbes

Abstract: Skyrmions are topologically protected quasiparticles, originally studied in condensed-matter systems and recently in photonics, with great potential in ultra-high-capacity information storage. Despite the recent attention, most optical solutions require complex and expensive systems yet produce limited topologies. Here we demonstrate an extended family of quasiparticles beyond normal skyrmions, wh… ▽ More Skyrmions are topologically protected quasiparticles, originally studied in condensed-matter systems and recently in photonics, with great potential in ultra-high-capacity information storage. Despite the recent attention, most optical solutions require complex and expensive systems yet produce limited topologies. Here we demonstrate an extended family of quasiparticles beyond normal skyrmions, which are controlled in confined photonic gradient-index media, extending to higher-order members such as multiskyrmions and multimerons, with increasingly complex topologies. We introduce new topological numbers to describe these complex photonic quasiparticles and propose how this new zoology of particles could be used in future high-capacity information transfer. Our compact creation system lends integrated and programmable solutions of complex particle textures, with potential impacts on both photonic and condensed-matter systems for revolutionizing topological informatics and logic devices. △ Less

Submitted 13 April, 2023; originally announced April 2023.

Physical variability in meter-scale laboratory CO$_2$ injections in faulted geometries

Authors: Malin Haugen, Lluis Salo-Salgado, Kristoffer Eikehaug, Benyamine Benali, Jakub W. Both, Erlend Storvik, Olav Folkvord, Ruben Juanes, Jan Martin Nordbotten, Martin A. Ferno

Abstract: Carbon, capture, and storage (CCS) is an important bridging technology to combat climate change in the transition towards net-zero. The FluidFlower concept has been developed to visualize and study CO$_2$ flow and storage mechanisms in sedimentary systems in a laboratory setting. Meter-scale multiphase flow in two geological geometries, including normal faults with and without smearing, is studied… ▽ More Carbon, capture, and storage (CCS) is an important bridging technology to combat climate change in the transition towards net-zero. The FluidFlower concept has been developed to visualize and study CO$_2$ flow and storage mechanisms in sedimentary systems in a laboratory setting. Meter-scale multiphase flow in two geological geometries, including normal faults with and without smearing, is studied. The experimental protocols developed to provide key input parameters for numerical simulations are detailed, including an evaluation of operational parameters for the FluidFlower benchmark study. Variability in CO$_2$ migration patterns for two different geometries is quantified, both between 16 repeated laboratory runs and between history-matched models and a CO$_2$ injection experiment. The predicative capability of a history-matched model is then evaluated in a different geological setting. △ Less

Submitted 18 January, 2023; originally announced January 2023.

Comments: manuscript + supplementary material

Room-scale CO2 injections in a physical reservoir model with faults

Authors: Martin A. Ferno, Malin Haugen, Kristoffer Eikehaug, Olav Folkvord, Benyamine Benali, Jakub W. Both, Erlend Storvik, Casey W. Nixon, Robert L. Gawthrope, Jan Martin Nordbotten

Abstract: We perform a series of repeated CO2 injections in a room-scale physical model of a faulted geological cross-section. Relevant parameters for subsurface carbon sequestration, including multiphase flows, capillary CO2 trapping, dissolution, and convective mixing, are studied and quantified. As part of a forecasting benchmark study, we address and quantify six predefined metrics for storage capacity… ▽ More We perform a series of repeated CO2 injections in a room-scale physical model of a faulted geological cross-section. Relevant parameters for subsurface carbon sequestration, including multiphase flows, capillary CO2 trapping, dissolution, and convective mixing, are studied and quantified. As part of a forecasting benchmark study, we address and quantify six predefined metrics for storage capacity and security in typical CO2 storage operations. Using the same geometry, we investigate the degree of reproducibility of five repeated experimental runs. Our analysis focuses on physical variations of the spatial distribution of mobile and dissolved CO2, multiphase flow patterns, development in mass of the aqueous and gaseous phases, gravitational fingers, and leakage dynamics. We observe very good reproducibility in homogenous regions with up to 97 % overlap between repeated runs, and that fault-related heterogeneity tends to decrease reproducibility. Notably, we observe an oscillating anticline CO2 leakage behavior from an open anticline with a spill point in the immediate footwall of a normal fault, and discuss the underlying causes for the observed phenomenon within the constraints of the studied system. △ Less

Submitted 16 January, 2023; originally announced January 2023.

Comments: Supplementary materials included

Universal adaptive optics for microscopy through embedded neural network control

Authors: Qi Hu, Martin Hailstone, Jingyu Wang, Matthew Wincott, Danail Stoychev, Huriye Atilgan, Dalia Gala, Tai Chaiamarit, Richard M. Parton, Jacopo Antonello, Adam M. Packer, Ilan Davis, Martin J. Booth

Abstract: The resolution and contrast of microscope imaging is often affected by aberrations introduced by imperfect optical systems and inhomogeneous refractive structures in specimens. Adaptive optics (AO) compensates these aberrations and restores diffraction limited performance. A wide range of AO solutions have been introduced, often tailored to a specific microscope type or application. Until now, a u… ▽ More The resolution and contrast of microscope imaging is often affected by aberrations introduced by imperfect optical systems and inhomogeneous refractive structures in specimens. Adaptive optics (AO) compensates these aberrations and restores diffraction limited performance. A wide range of AO solutions have been introduced, often tailored to a specific microscope type or application. Until now, a universal AO solution -- one that can be readily transferred between microscope modalities -- has not been deployed. We propose versatile and fast aberration correction using a physics-based machine learning (ML) assisted wavefront-sensorless AO control method. Unlike previous ML methods, we used a bespoke neural network (NN) architecture, designed using physical understanding of image formation, that was embedded in the control loop of the microscope. The approach means that not only is the resulting NN orders of magnitude simpler than previous NN methods, but the concept is translatable across microscope modalities. We demonstrated the method on a two-photon, a three-photon and a widefield three-dimensional (3D) structured illumination microscope. Results showed that the method outperformed commonly-used modal-based sensorless AO methods. We also showed that our ML-based method was robust in a range of challenging imaging conditions, such as extended 3D sample structures, specimen motion, low signal to noise ratio and activity-induced fluorescence fluctuations. Moreover, as the bespoke architecture encapsulated physical understanding of the imaging process, the internal NN configuration was no-longer a ``black box'', but provided physical insights on internal workings, which could influence future designs. △ Less

Submitted 25 April, 2023; v1 submitted 6 January, 2023; originally announced January 2023.

Comments: 27 pages, 12 figures

PoroTwin: A digital twin for a FluidFlower rig

Authors: Eirik Keilegavlen, Eivind Fonn, Kjetil Johannessen, Kristoffer Eikehaug, Jakub Both, Martin Fernø, Trond Kvamsdal, Adil Rasheed, Jan M. Nordbotten

Abstract: We present a framework for integrated experiments and simulations of tracer transport in heterogeneous porous media using digital twin technology. The physical asset in our setup is a meter-scale FluidFlower rig. The digital twin consists of a traditional physics-based forward simulation tool and a correction technique which compensates for mismatches between simulation results and observations. T… ▽ More We present a framework for integrated experiments and simulations of tracer transport in heterogeneous porous media using digital twin technology. The physical asset in our setup is a meter-scale FluidFlower rig. The digital twin consists of a traditional physics-based forward simulation tool and a correction technique which compensates for mismatches between simulation results and observations. The latter augments the range of the physics-based simulation and allows us to bridge the gap between simulation and experiments in a quantitative sense. We describe the setup of the physical and digital twin, including data transfer protocols using cloud technology. The accuracy of the digital twin is demonstrated on a case with artificially high diffusion that must be compensated by the correction approach, as well as by simulations in geologically complex media. The digital twin is then applied to control tracer transport by manipulating fluid injection and production in the experimental rig, thereby enabling two-way coupling between the physical and digital twins. △ Less

Submitted 6 January, 2023; v1 submitted 1 December, 2022; originally announced December 2022.

Direct laser written aperiodic photonic volume elements for complex light shaping with high efficiency: inverse design and fabrication

Authors: Nicolas Barré, Ravi Shivaraman, Simon Moser, Patrick Salter, Michael Schmidt, Martin J. Booth, Alexander Jesacher

Abstract: Light plays the central role in many applications. The key to unlocking its versatility lies in shaping it into the most appropriate form for the task at hand. Specifically tailored refractive index modifications, directly manufactured inside glass using a short pulsed laser, enable an almost arbitrary control of the light flow. However, the stringent requirements for quantitative knowledge of the… ▽ More Light plays the central role in many applications. The key to unlocking its versatility lies in shaping it into the most appropriate form for the task at hand. Specifically tailored refractive index modifications, directly manufactured inside glass using a short pulsed laser, enable an almost arbitrary control of the light flow. However, the stringent requirements for quantitative knowledge of these modifications, as well as for fabrication precision, have so far prevented the fabrication of light-efficient aperiodic photonic volume elements (APVEs). Here we present a powerful approach to the design and manufacturing of light-efficient APVEs. We optimize application-specific 3D arrangements of hundred thousands of microscopic voxels and manufacture them using femtosecond direct laser writing inside millimeter-sized glass volumes. We experimentally achieve unprecedented diffraction efficiencies up to 80%, which is enabled by precise voxel characterization and adaptive optics during fabrication. We demonstrate APVEs with various functionalities, including a spatial mode converter and combined intensity shaping and wavelength-multiplexing. Our elements can be freely designed and are efficient, compact and robust. Our approach is not limited to borosilicate glass, but is potentially extendable to other substrates, including birefringent and nonlinear materials, giving a preview of even broader functionalities including polarization modulation and dynamic elements. △ Less

Submitted 22 November, 2022; v1 submitted 28 September, 2022; originally announced September 2022.

Cross-calibration of atomic pressure sensors and deviation from quantum diffractive collision universality for light particles

Authors: Pinrui Shen, Erik Frieling, Katherine R. Herperger, Denis Uhland, Riley A. Stewart, Avinash Deshmukh, Roman V. Krems, James L. Booth, Kirk W. Madison

Abstract: The total room-temperature, velocity-averaged cross section for atom-atom and atom-molecule collisions is well approximated by a universal function depending only on the magnitude of the leading order dispersion coefficient, $C_6$. This feature of the total cross section together with the universal function for the energy distribution transferred by glancing angle collisions ($P_{\rm{QDU}6}$) can… ▽ More The total room-temperature, velocity-averaged cross section for atom-atom and atom-molecule collisions is well approximated by a universal function depending only on the magnitude of the leading order dispersion coefficient, $C_6$. This feature of the total cross section together with the universal function for the energy distribution transferred by glancing angle collisions ($P_{\rm{QDU}6}$) can be used to empirically determine the total collision cross section and realize a self-calibrating, vacuum pressure standard. This was previously validated for Rb+N$_2$ and Rb+Rb collisions. However, the post-collision energy distribution is expected to deviate from $P_{\rm{QDU}6}$ in the limit of small $C_6$ and small reduced mass. Here we observe this deviation experimentally by performing a direct cross-species loss rate comparison between Rb+H$_2$ and Li+H$_2$ and using the \textit{ab initio} value of $\langle σ_{\rm{tot}} \, v \rangle_{\rm{Li+H}_2}$. We find a velocity averaged total collision cross section ratio, $R = \langle σ_{\rm{tot}} \, v \rangle_{\rm{Li+H}_2} : \langle σ_{\rm{tot}} \, v \rangle_{\rm{Rb+H}_2} = 0.83(5)$. Based on an \textit{ab initio} computation of $\langle σ_{\rm{tot}} \, v \rangle_{\rm{Li+H}_2} = 3.13(6)\times 10^{-15}$ m$^3$/s, we deduce $\langle σ_{\rm{tot}} \, v \rangle_{\rm{Rb+H}_2} = 3.8(2) \times 10^{-15}$ m$^3$/s, in agreement with a Rb+H$_2$ \textit{ab initio} value of $\langle σ_{\mathrm{tot}} v \rangle_{\mathrm{Rb+H_2}} = 3.57 \times 10^{-15} \mathrm{m}^3/\mathrm{s}$.By contrast, fitting the Rb+H$_2$ loss rate as a function of trap depth to the universal function we find $\langle σ_{\rm{tot}} \, v \rangle_{\rm{Rb+H}_2} = 5.52(9) \times 10^{-15}$ m$^3$/s. Finally, this work demonstrates how to perform a cross-calibration of sensor atoms to extend and enhance the cold atom based pressure sensor. △ Less

Submitted 12 September, 2022; v1 submitted 6 September, 2022; originally announced September 2022.

Comments: 14 pages, 9 figures

Measurement of Rb-Rb van der Waals coefficient via Quantum Diffractive Universality

Authors: Riley A. Stewart, Pinrui Shen, James L. Booth, Kirk W. Madison

Abstract: Collisions between trapped atoms or trapped molecules with room temperature particles in the surrounding vacuum induce loss of the trapped population at a rate proportional to the density of the background gas particles. The total velocity-averaged loss rate coefficient $\langle σ_\mathrm{tot} v \rangle$ for such collisions and the variation of the loss rate with trap depth has been shown to depen… ▽ More Collisions between trapped atoms or trapped molecules with room temperature particles in the surrounding vacuum induce loss of the trapped population at a rate proportional to the density of the background gas particles. The total velocity-averaged loss rate coefficient $\langle σ_\mathrm{tot} v \rangle$ for such collisions and the variation of the loss rate with trap depth has been shown to depend only on the long range interaction potential between the collision partners. This collision universality was previously used to realize a self-calibrating, atom-based, primary pressure standard and was validated by indirect comparison with an orifice flow standard. Here, we use collision universality to measure $\langle σ_\mathrm{tot} v \rangle = 6.44(11)(5) \times 10^{-15}~\rm{m^3/s}$ for Rb-Rb collisions and deduce the corresponding $C_6 = 4688(198)(95)~E_ha_0^6$, in excellent agreement with predictions based upon $\textit{ab initio}$ calculated and previously measured $C_6$ values. △ Less

Submitted 26 August, 2022; originally announced August 2022.

Comments: 9 pages, 4 figures

Fermi Level Depinning in Two-Dimensional Materials Using a Fluorinated Bilayer Graphene Barrier

Authors: Cunzhi Sun, Cheng Xiang, Rongdun Hong, Feng Zhang, Timothy J. Booth, Peter Bøggild, Manh-Ha Doan

Abstract: Strong Fermi level pinning (FLP) - often attributed to metal-induced gap states at the interfacial contacts - severely reduces the tunability of the Schottky barrier height of the junction and limits applications of the 2D materials in electronics and optoelectronics. Here, we show that fluorinated bilayer graphene (FBLG) can be used as a barrier to effectively prevent FLP at metal/2D materials in… ▽ More Strong Fermi level pinning (FLP) - often attributed to metal-induced gap states at the interfacial contacts - severely reduces the tunability of the Schottky barrier height of the junction and limits applications of the 2D materials in electronics and optoelectronics. Here, we show that fluorinated bilayer graphene (FBLG) can be used as a barrier to effectively prevent FLP at metal/2D materials interfaces. FLBG can be produced via short exposure (1-3 min) to SF6 plasma that fluorinates only the top layer of a bilayer graphene with covalent C-F bonding, while the bottom layer remains intrinsic, resulting in a band gap opening of about 75 meV. Inserting FBLG between the metallic contacts and a layer of MoS2 reduces the Schottky barrier height dramatically for the low-work function metals (313 and 260 meV for Ti and Cr, respectively) while it increases for the high-work function one ( 160 meV for Pd), corresponding to an improved pinning factor. Our results provide a straightforward method to generate atomically thin dielectrics with applications not only for depinning the Fermi level at metal/transition metal dichalcogenide (TMD) interfaces but also for solving many other problems in electronics and optoelectronics △ Less

Submitted 2 August, 2022; originally announced August 2022.

Single-mode sapphire fiber Bragg grating

Authors: Mohan Wang, Patrick S. Salter, Frank P. Payne, Adrian Shipley, Stephen M. Morris, Martin J. Booth, Julian A. J. Fells

Abstract: We present here the inscription of single-mode waveguides with Bragg gratings in sapphire. The waveguide Bragg gratings have a novel multi-layer depressed cladding design in the 1550 nm telecommunications waveband. The Bragg gratings have a narrow bandwidth (<0.5 nm) and have survived annealing at 1000°C. The structures are inscribed with femtosecond laser direct writing, using adaptive beam shapi… ▽ More We present here the inscription of single-mode waveguides with Bragg gratings in sapphire. The waveguide Bragg gratings have a novel multi-layer depressed cladding design in the 1550 nm telecommunications waveband. The Bragg gratings have a narrow bandwidth (<0.5 nm) and have survived annealing at 1000°C. The structures are inscribed with femtosecond laser direct writing, using adaptive beam shaping with a non-immersion objective. A single-mode sapphire fiber Bragg grating is created by writing a waveguide with a Bragg grating within a 425 μm diameter sapphire optical fiber, providing significant potential for accurate remote sensing in ultra-extreme environments. △ Less

Submitted 23 December, 2021; originally announced December 2021.

Comments: Submitted to Optica 12 November 2021

SenAOReFoc: A Closed-Loop Sensorbased Adaptive Optics and Remote Focusing Control Software

Authors: Jiahe Cui, Karen M. Hampson, Matthew Wincott, Martin J. Booth

Abstract: SenAOReFoc is a closed-loop sensorbased adaptive optics (AO) and remote focusing control software that works with a deformable mirror (DM) and a Shack-Hartmann wavefront sensor (SHWS). It is programmed in Python and is open-source on Github https://github.com/jiahecui/SenAOReFoc. A detailed user guide can be found in the Github repository. Here, we give a brief summary of basic software functional… ▽ More SenAOReFoc is a closed-loop sensorbased adaptive optics (AO) and remote focusing control software that works with a deformable mirror (DM) and a Shack-Hartmann wavefront sensor (SHWS). It is programmed in Python and is open-source on Github https://github.com/jiahecui/SenAOReFoc. A detailed user guide can be found in the Github repository. Here, we give a brief summary of basic software functionalities, a statement of need, and some examples for the usage of this software. △ Less

Submitted 17 December, 2021; originally announced December 2021.

On-chip beam rotators, adiabatic mode converters, and waveplates through low-loss waveguides with variable cross-sections

Authors: Bangshan Sun, Fyodor Morozko, Patrick S. Salter, Simon Moser, Zhikai Pong, Raj B. Patel, Ian A. Walmsley, Mohan Wang, Adir Hazan, Nicolas Barre, Alexander Jesacher, Julian Fells, Chao He, Aviad Katiyi, ZhenNan Tian, Alina Karabchevsky, Martin J. Booth

Abstract: Photonics integrated circuitry would benefit considerably from the ability to arbitrarily control waveguide cross-sections with high precision and low loss, in order to provide more degrees of freedom in manipulating propagating light. Here, we report a new method for femtosecond laser writing of optical-fibre-compatible glass waveguides, namely spherical phase induced multi-core waveguide (SPIM-W… ▽ More Photonics integrated circuitry would benefit considerably from the ability to arbitrarily control waveguide cross-sections with high precision and low loss, in order to provide more degrees of freedom in manipulating propagating light. Here, we report a new method for femtosecond laser writing of optical-fibre-compatible glass waveguides, namely spherical phase induced multi-core waveguide (SPIM-WG), which addresses this challenging task with three dimensional on-chip light control. Fabricating in the heating regime with high scanning speed, precise deformation of cross-sections is still achievable along the waveguide, with shapes and sizes finely controllable of high resolution in both horizontal and vertical transversal directions. We observed that these waveguides have high refractive index contrast of 0.017, low propagation loss of 0.14 dB/cm, and very low coupling loss of 0.19 dB coupled from a single mode fibre. SPIM-WG devices were easily fabricated that were able to perform on-chip beam rotation through varying angles, or manipulate polarization state of propagating light for target wavelengths. We also demonstrated SPIM-WG mode converters that provide arbitrary adiabatic mode conversion with high efficiency between symmetric and asymmetric non-uniform modes; examples include circular, elliptical modes and asymmetric modes from ppKTP (periodically-poled potassium titanyl phosphate) waveguides which are generally applied in frequency conversion and quantum light sources. Created inside optical glass, these waveguides and devices have the capability to operate across ultra-broad bands from visible to infrared wavelengths. The compatibility with optical fibre also paves the way toward packaged photonic integrated circuitry, which usually needs input and output fibre connections. △ Less

Submitted 14 July, 2022; v1 submitted 5 December, 2021; originally announced December 2021.

Comments: Published in Nature: Light Science & Applications

Journal ref: Light: Science & Applications (2022) 11:214

Super-Resolution Nanolithography of Two-Dimensional Materials by Anisotropic Etching

Authors: Dorte R. Danielsen, Anton Lyksborg-Andersen, Kirstine E. S. Nielsen, Bjarke S. Jessen, Timothy J. Booth, Manh-Ha Doan, Yingqiu Zhou, Peter Bøggild, Lene Gammelgaard

Abstract: Nanostructuring allows altering of the electronic and photonic properties of two-dimensional (2D) materials. The efficiency, flexibility, and convenience of top-down lithography processes are however compromised by nm-scale edge roughness and resolution variability issues, which especially affects the performance of 2D materials. Here we study how dry anisotropic etching of multilayer 2D materials… ▽ More Nanostructuring allows altering of the electronic and photonic properties of two-dimensional (2D) materials. The efficiency, flexibility, and convenience of top-down lithography processes are however compromised by nm-scale edge roughness and resolution variability issues, which especially affects the performance of 2D materials. Here we study how dry anisotropic etching of multilayer 2D materials with sulfur hexafluoride (SF6) may overcome some of these issues, showing results for hexagonal boron nitride (hBN), tungsten disulfide (WS2), tungsten diselenide (WSe2), molybdenum disulfide (MoS2), molybdenum ditelluride (MoTe2). Scanning and transmission electron microscopy reveal that etching leads to anisotropic hexagonal features in the studied transition metal dichalcogenides, with the relative degree of anisotropy ranked as: WS2 > WSe2 > MoTe2 / MoS2. Etched holes are terminated by zigzag edges while etched dots (protrusions) are terminated by armchair edges. This can be explained by Wulff constructions, taking the relative stabilities of the edges and the AA stacking order into account. Patterns in WS2 are transferred to an underlying graphite layer, demonstrating a possible use for creating sub-10 nm features. In contrast, multilayer hBN exhibits no lateral anisotropy, but shows consistent vertical etch angles, independent of crystal orientation. This is used to create super-resolution lithographic patterns with ultra-sharp corners at the base of the hBN crystal, which are transferred into an underlying graphite crystal. We find that the anisotropic SF6 reactive ion etching process makes it possible to downsize nanostructures to obtain smooth edges, sharp corners, and feature sizes significantly below the resolution limit of electron beam lithography. The nanostructured 2D materials can be used themselves or as etch-masks to pattern other nanomaterials. △ Less

Submitted 7 October, 2021; originally announced October 2021.

Journal ref: ACS Appl. Mater. Interfaces 2021, 13, 35

Vectorial adaptive optics

Authors: Chao He, Jacopo Antonello, Martin J. Booth

Abstract: Adaptive optics normally concerns the feedback correction of phase aberrations. Such correction has been of benefit in various optical systems, with applications ranging in scale from astronomical telescopes to super-resolution microscopes. Here we extend this powerful tool into the vectorial domain, encompassing higher-dimensional feedback correction of both polarisation and phase. This technique… ▽ More Adaptive optics normally concerns the feedback correction of phase aberrations. Such correction has been of benefit in various optical systems, with applications ranging in scale from astronomical telescopes to super-resolution microscopes. Here we extend this powerful tool into the vectorial domain, encompassing higher-dimensional feedback correction of both polarisation and phase. This technique is termed vectorial adaptive optics (V-AO). We show that V-AO can be implemented using sensor feedback, indirectly using sensorless AO, or in hybrid form combining aspects of both. We validate improvements in both vector field state and the focal quality of an optical system, through correction for commonplace vectorial aberration sources, ranging from objective lenses to biological samples. This technique pushes the boundaries of traditional scalar beam shaping by providing feedback control of extra vectorial degrees of freedom. This paves the way for next generation AO functionality by manipulating the complex vectorial field. △ Less

Submitted 6 October, 2021; originally announced October 2021.

Polarisation optics for biomedical and clinical applications: a review

Authors: Chao He, Honghui He, Jintao Chang, Binguo Chen, Hui Ma, Martin J. Booth

Abstract: Many polarisation techniques have been harnessed for decades in biological and clinical research, each based upon measurement of the vectorial properties of light or the vectorial transformations imposed on light by objects. Various advanced vector measurement/sensing techniques, physical interpretation methods, and approaches to analyse biomedically relevant information have been developed and ha… ▽ More Many polarisation techniques have been harnessed for decades in biological and clinical research, each based upon measurement of the vectorial properties of light or the vectorial transformations imposed on light by objects. Various advanced vector measurement/sensing techniques, physical interpretation methods, and approaches to analyse biomedically relevant information have been developed and harnessed. In this review, we focus mainly on summarizing methodologies and applications related to tissue polarimetry, with an emphasis on the adoption of the Stokes-Mueller formalism. Several recent breakthroughs, development trends, and potential multi-modal uses in conjunction with other techniques are also presented. The primary goal of the review is to give the reader a general overview in the use of vectorial information that can be obtained by polarisation optics for applications in biomedical and clinical research. △ Less

Submitted 10 August, 2021; originally announced August 2021.

Revealing complex optical phenomena through vectorial metrics

Authors: Chao He, Jintao Chang, Patrick S. Salter, Yuanxing Shen, Ben Dai, Pengcheng Li, Yihan Jin, Samlan Chandran Thodika, Mengmeng Li, Aziz Tariq, Jingyu Wang, Jacopo Antonello, Yang Dong, Ji Qi, Jianyu Lin, Honghui He, Daniel S. Elson, Min Zhang, Hui Ma, Martin J. Booth

Abstract: Advances in vectorial polarisation-resolved imaging are bringing new capabilities to applications ranging from fundamental physics through to clinical diagnosis. Imaging polarimetry requires determination of the Mueller matrix (MM) at every point, providing a complete description of an object's vectorial properties. Despite forming a comprehensive representation, the MM does not usually provide ea… ▽ More Advances in vectorial polarisation-resolved imaging are bringing new capabilities to applications ranging from fundamental physics through to clinical diagnosis. Imaging polarimetry requires determination of the Mueller matrix (MM) at every point, providing a complete description of an object's vectorial properties. Despite forming a comprehensive representation, the MM does not usually provide easily-interpretable information about the object's internal structure. Certain simpler vectorial metrics are derived from subsets of the MM elements. These metrics permit extraction of signatures that provide direct indicators of hidden optical properties of complex systems, while featuring an intriguing asymmetry about what information can or cannot be inferred via these metrics. We harness such characteristics to reveal the spin-Hall effect of light, infer microscopic structure within laser-written photonic waveguides, and conduct rapid pathological diagnosis through analysis of healthy and cancerous tissue. This provides new insight for the broader usage of such asymmetric inferred vectorial information. △ Less

Submitted 21 July, 2021; v1 submitted 20 July, 2021; originally announced July 2021.