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Condensed Matter > Other Condensed Matter

arXiv:0704.3041 (cond-mat)
[Submitted on 23 Apr 2007]

Title:Magnetization and specific heat of TbFe3(BO3)4: Experiment and crystal field calculations

Authors:E.A. Popova, D.V. Volkov, A.N. Vasiliev, A.A. Demidov, N.P. Kolmakova, I.A. Gudim, L.N. Bezmaternykh, N. Tristan, Yu. Skourski, B. Büchner, C. Hess, R. Klingeler
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Abstract: We have studied the thermodynamic properties of single-crystalline TbFe3(BO3)4. Magnetization measurements have been carried out as a function of magnetic field (up to 50 T) and temperature up to 350K with the magnetic field both parallel and perpendicular to the trigonal c-axis of the crystal. The specific heat has been measured in the temperature range 2-300K with a magnetic field up to 9 T applied parallel to the c-axis. The data indicate a structural phase transition at 192 K and antiferromagnetic spin ordering at 40 K. A Schottky anomaly is present in the specific heat data around 20 K, arising due to two low-lying energy levels of the Tb3+ ions being split by f-d coupling. Below TN magnetic fields parallel to the c-axis drive a spin-flop phase transition, which is associated with a large magnetization jump. The highly anisotropic character of the magnetic susceptibility is ascribed mainly to the Ising-like behavior of the Tb3+ ions in the trigonal crystal field. We describe our results in the framework of an unified approach which is based on mean-field approximation and crystal-field calculations.
Comments: 10 pages, 10 figures, 20 references, accepted by Phys. Rev. B
Subjects: Other Condensed Matter (cond-mat.other)
Cite as: arXiv:0704.3041 [cond-mat.other]
  (or arXiv:0704.3041v1 [cond-mat.other] for this version)
  https://doi.org/10.48550/arXiv.0704.3041
arXiv-issued DOI via DataCite
Related DOI: https://doi.org/10.1103/PhysRevB.75.224413
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Submission history

From: Natalia Tristan [view email]
[v1] Mon, 23 Apr 2007 16:05:27 UTC (300 KB)
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