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Condensed Matter > Strongly Correlated Electrons

arXiv:2107.01585 (cond-mat)
[Submitted on 4 Jul 2021]

Title:Survival of itinerant excitations and quantum spin state transitions in YbMgGaO$_4$ with chemical disorder

Authors:X. Rao, G. Hussain, Q. Huang, W. J. Chu, N. Li, X. Zhao, Z. Dun, E. S. Choi, T. Asaba, L. Chen, L. Li, X. Y. Yue, N. N. Wang, J.-G. Cheng, Y. H. Gao, Y. Shen, J. Zhao, G. Chen, H. D. Zhou, X. F. Sun
View a PDF of the paper titled Survival of itinerant excitations and quantum spin state transitions in YbMgGaO$_4$ with chemical disorder, by X. Rao and 19 other authors
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Abstract:A recent focus of quantum spin liquid (QSL) studies is how disorder/randomness in a QSL candidate affects its true magnetic ground state. The ultimate question is whether the QSL survives disorder or the disorder leads to a "spin-liquid-like" state, such as the proposed random-singlet (RS) state. Since disorder is a standard feature of most QSL candidates, this question represents a major challenge for QSL candidates. YbMgGaO$_4$, a triangular lattice antiferromagnet with effective spin-1/2 Yb$^{3+}$ ions, is an ideal system to address this question, since it shows no long-range magnetic ordering with Mg/Ga site disorder. Despite the intensive study, it remains unresolved as to whether YbMgGaO$_4$ is a QSL or in the RS state. Here, through ultralow-temperature thermal conductivity and magnetic torque measurements, plus specific heat and DC magnetization data, we observed a residual $\kappa_0/T$ term and series of quantum spin state transitions in the zero temperature limit for YbMgGaO$_4$. These observations strongly suggest that a QSL state with itinerant excitations and quantum spin fluctuations survives disorder in YbMgGaO$_4$.
Comments: 31 pages, 10 figures
Subjects: Strongly Correlated Electrons (cond-mat.str-el)
Cite as: arXiv:2107.01585 [cond-mat.str-el]
  (or arXiv:2107.01585v1 [cond-mat.str-el] for this version)
  https://doi.org/10.48550/arXiv.2107.01585
arXiv-issued DOI via DataCite
Journal reference: Nat. Commun. 12, 4949 (2021)
Related DOI: https://doi.org/10.1038/s41467-021-25247-6
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From: X. F. Sun [view email]
[v1] Sun, 4 Jul 2021 10:22:02 UTC (1,341 KB)
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