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Superconductivity-induced Phonon Renormalization on NaFe$_{1-x}$Co$_{x}$As
Authors:
Y. J. Um,
Yunkyu Bang,
B. H. Min,
Y. S. Kwon,
M. Le Tacon
Abstract:
We report a study of the lattice dynamics in superconducting NaFeAs (Tc = 8 K) and doped NaFe0.97Co0.03As (Tc = 20 K) using Raman light scattering. Five of the six phonon modes expected from group theory are observed. In contrast with results obtained on iso-structural and iso-electronic LiFeAs, anomalous broadening of Eg(As) and A1g(Na) modes upon cooling is observed in both samples. In addition,…
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We report a study of the lattice dynamics in superconducting NaFeAs (Tc = 8 K) and doped NaFe0.97Co0.03As (Tc = 20 K) using Raman light scattering. Five of the six phonon modes expected from group theory are observed. In contrast with results obtained on iso-structural and iso-electronic LiFeAs, anomalous broadening of Eg(As) and A1g(Na) modes upon cooling is observed in both samples. In addition, in the Co-doped sample, a superconductivity-induced renormalization of the frequency and linewidth of the B1g(Fe) vibration is observed. This renormalization can not be understood within a single band and simple multi-band approaches. A theoretical model that includes the effects of SDW correlations along with sign-changing s-wave pairing state and interband scattering has been developed to explain the observed behavior of the B1g(Fe) mode.
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Submitted 6 May, 2014;
originally announced May 2014.
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Anomalous dependence of the c-axis polarized Fe B$_{1g}$ phonon mode with Fe and Se concentrations in Fe$_{1+y}$Te$_{1-x}$Se$_x$
Authors:
Y. J. Um,
A. Subedi,
P. Toulemonde,
A. Y. Ganin,
L. Boeri,
M. Rahlenbeck,
Y. Liu,
C. T. Lin,
S. J. E. Carlsson,
A. Sulpice,
M. J. Rosseinsky,
B. Keimer,
M. Le Tacon
Abstract:
We report an investigation of the lattice dynamical properties in a range of Fe$_{1+y}$Te$_{1-x}$Se$_{x}$ compounds, with special emphasis on the c-axis polarized vibration of Fe with B$_{1g}$ symmetry, a Raman active mode common to all families of Fe-based superconductors. We have carried out a systematic study of the temperature dependence of this phonon mode as a function of Se $x$ and excess F…
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We report an investigation of the lattice dynamical properties in a range of Fe$_{1+y}$Te$_{1-x}$Se$_{x}$ compounds, with special emphasis on the c-axis polarized vibration of Fe with B$_{1g}$ symmetry, a Raman active mode common to all families of Fe-based superconductors. We have carried out a systematic study of the temperature dependence of this phonon mode as a function of Se $x$ and excess Fe $y$ concentrations. In parent compound Fe$_{1+y}$Te, we observe an unconventional broadening of the phonon between room temperature and magnetic ordering temperature $T_N$. The situation smoothly evolves towards a regular anharmonic behavior as Te is substituted for Se and long range magnetic order is replaced by superconductivity. Irrespective to Se contents, excess Fe is shown to provide an additional damping channel for the B$_{1g}$ phonon at low temperatures. We performed Density Functional Theory (DFT) ab-initio calculations within the local density approximation (LDA) to calcuate the phonon frequencies including magnetic polarization and Fe non-stoichiometry in the Virtual Crystal Approximation (VCA). We obtained a good agreement with the measured phonon frequencies in the Fe-deficient samples, while the effects of Fe excess are poorly reproduced. This may be due to excess Fe-induced local magnetism and low energy magnetic fluctuations that can not be treated accurately within these approaches. As recently revealed by neutron scattering and $μ$-SR studies, these phenomena occur in the temperature range where anomalous decay of the B$_{1g}$ phonon is observed, and suggests a peculiar coupling of this mode with local moments and spin fluctuations in Fe$_{1+y}$Te$_{1-x}$Se$_{x}$.
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Submitted 23 February, 2012; v1 submitted 2 February, 2012;
originally announced February 2012.
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Raman Scattering Study of the Lattice Dynamics of Superconducting LiFeAs
Authors:
Y. J. Um,
J. T. Park,
B. H. Min,
Y. J. Song,
Y. S. Kwon,
B. Keimer,
M. Le Tacon
Abstract:
We report an investigation of the lattice dynamical properties of LiFeAs using inelastic light scattering. Five out of the six expected phonon modes are observed. The temperature evolution of their frequencies and linewidths is in good agreement with an anharmonic-decay model. We find no evidence for substantial electron-phonon coupling, and no superconductivity-induced phonon anomalies.
We report an investigation of the lattice dynamical properties of LiFeAs using inelastic light scattering. Five out of the six expected phonon modes are observed. The temperature evolution of their frequencies and linewidths is in good agreement with an anharmonic-decay model. We find no evidence for substantial electron-phonon coupling, and no superconductivity-induced phonon anomalies.
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Submitted 12 January, 2012; v1 submitted 27 September, 2011;
originally announced September 2011.