Showing 1–50 of 66 results for author: Aarts, J

Long range proximity effects in planar structures involving the halfmetal ferromagnet La0.7Sr0.3MnO3 and Pt interlayers

Authors: Junxiang Yao, Julian van Doorn, Mariona Cabero, Jan Aarts

Abstract: Over the last decade, there has been steady research on superconducting junctions with a ferromagnet as the weak link, and where triplet correlations can transport supercurrents over a substantial distances. Of particular interest are halfmetallic ferromagnets, in which only one spin band is present, so that, presumably, the induced supercurrent is fully spin-polarized. We have earlier reported on… ▽ More Over the last decade, there has been steady research on superconducting junctions with a ferromagnet as the weak link, and where triplet correlations can transport supercurrents over a substantial distances. Of particular interest are halfmetallic ferromagnets, in which only one spin band is present, so that, presumably, the induced supercurrent is fully spin-polarized. We have earlier reported on a study of triplet transport in planar La0.7Sr0.3MnO3(LSMO) nanostrip Josephson junctions with NbTi superconducting contacts, where we found high values for the supercurrents, and large junction lengths (up to 1.3 μm). Here, we extend that work by studying the dependence of the critical current Ic on the length of the nanostrip between the contacts and the width of the strip. All junctions show strong supercurrents, but we do not observe simple systematics. Apparently, the fabrication process does not allow sufficient control over some of its parameters. To gain more insight in the mechanism for triplet generation at the LSMO/NbTi interface, we also studied the effect of Pt as an interlayer between the LSMO and the NbTi. For this, we etched a NbTi/Pt electrode structure on a full film of LSMO. The results are highly promising, showing sharp superconducting transitions and zero-resistance states being reached at an electrode distance of 2 μm, with indications that larger distances should be feasible. △ Less

Submitted 1 May, 2026; originally announced May 2026.

Comments: 8 pages, 6 figures

Emergent Zeeman-Resilient Superconductivity Beyond the Spin-Paramagnetic Limit in Ultrathin NiBi3

Authors: Gabriel Sant'Ana, Leonardo Pessoa da Silva, Pedro Schio, David Möckli, Jan Aarts, Kaveh Lahabi, Milton A. Tumelero

Abstract: The spin-paramagnetic limit sets a fundamental magnetic-field bound for conventional superconductors. Here we show that ultrathin NiBi$_3$ films develop a highly field-resilient superconducting state, with in-plane critical fields surpassing the spin-paramagnetic limit even above 0.9T$_C$. This enhancement is activated by dimensional confinement and depends sensitively on film thickness and morpho… ▽ More The spin-paramagnetic limit sets a fundamental magnetic-field bound for conventional superconductors. Here we show that ultrathin NiBi$_3$ films develop a highly field-resilient superconducting state, with in-plane critical fields surpassing the spin-paramagnetic limit even above 0.9T$_C$. This enhancement is activated by dimensional confinement and depends sensitively on film thickness and morphology. Standard mechanisms, including strong spin-orbit coupling and multiband superconductivity, fail to quantitatively explain the observed robustness. These findings uncover an unconventional pathway for Zeeman-resistant superconductivity in low-dimensional materials beyond known Ising and Rashba scenarios, and further support earlier theoretical predictions of triplet pairing in low-dimensional NiBi$_3$. △ Less

Submitted 4 May, 2026; v1 submitted 17 September, 2025; originally announced September 2025.

Time-reversal symmetry breaking in microscopic single-crystal Sr$_2$RuO$_4$ devices

Authors: Remko Fermin, Matthijs Rog, Guido Stam, Daan Wielens, Joost Ridderbos, Chuan Li, Yoshi Maeno, Jan Aarts, Kaveh Lahabi

Abstract: Time-reversal symmetry breaking superconductivity is a quintessential unconventional quantum state. In Josephson junctions, time-reversal symmetry breaking manifests itself in the supercurrent interference pattern as the invariance of the critical current under the reversal of both transport and magnetic field directions, i.e., $I_\text{c+}(H) = I_\text{c-}(-H)$. So far, such systems have been rea… ▽ More Time-reversal symmetry breaking superconductivity is a quintessential unconventional quantum state. In Josephson junctions, time-reversal symmetry breaking manifests itself in the supercurrent interference pattern as the invariance of the critical current under the reversal of both transport and magnetic field directions, i.e., $I_\text{c+}(H) = I_\text{c-}(-H)$. So far, such systems have been realized in devices where superconductivity is injected into a deliberately constructed weak link medium, usually carefully tuned by external magnetic fields and electrostatic gating. In this work, we report time-reversal symmetry breaking in spontaneously emerging Josephson junctions without intentionally constructed weak links. This is realized in ultra-pure single-crystal microstructures of Sr$_2$RuO$_4$, an unconventional superconductor with a multi-component order parameter. Here, the Josephson effect emerges intrinsically at the superconducting domain wall, where the degenerate states partially overlap. In addition to violating $I_\text{c+}(H) = I_\text{c-}(-H)$, we find a rich variety of exotic transport phenomena, including a supercurrent diode effect present in the entire interference pattern, two-channel critical current oscillations with a period that deviates from $Φ_0$, fractional Shapiro steps, and current-switchable bistable states with highly asymmetric critical currents. Our findings provide direct evidence of TRSB in unstrained Sr$_2$RuO$_4$ and reveal the potential of domain wall Josephson junctions, which can emerge in any superconductor where the pairing symmetry is described by a multi-component order parameter. △ Less

Submitted 27 April, 2025; originally announced April 2025.

Recombination of localized quasiparticles in disordered superconductors

Authors: Steven A. H. de Rooij, Remko Fermin, Kevin Kouwenhoven, Tonny Coppens, Vignesh Murugesan, David J. Thoen, Jan Aarts, Jochem J. A. Baselmans, Pieter J. de Visser

Abstract: Disordered superconductors offer new impedance regimes for quantum circuits, enable a pathway to protected qubits, and can improve superconducting detectors due to their high kinetic inductance and sheet resistance. The performance of these devices can be limited, however, by quasiparticles - the fundamental excitations of a superconductor. While experiments have shown that disorder affects the re… ▽ More Disordered superconductors offer new impedance regimes for quantum circuits, enable a pathway to protected qubits, and can improve superconducting detectors due to their high kinetic inductance and sheet resistance. The performance of these devices can be limited, however, by quasiparticles - the fundamental excitations of a superconductor. While experiments have shown that disorder affects the relaxation of quasiparticles drastically, the microscopic mechanisms are still not understood. We address this issue by measuring quasiparticle relaxation in a disordered $β$-Ta film, which we pattern as the inductor of a microwave resonator. We observe that quasiparticle recombination is governed by the phonon scattering time, which is faster than conventional recombination in ordered superconductors. We interpret the results as recombination of localized quasiparticles, induced by disorder, which first delocalize via phonon absorption. We analyze quasiparticle relaxation measurements on superconductors with different degrees of disorder and conclude that this phenomenon is inherent to disordered superconductors. △ Less

Submitted 7 August, 2025; v1 submitted 24 October, 2024; originally announced October 2024.

Comments: 11 pages main text, including 6 figures and 1 table

Journal ref: Nat Commun 16, 8465 (2025)

Fabrication of planar halfmetallic ferromagnetic Josephson junctions with long range coupling

Authors: Junxiang Yao, Jan Aarts

Abstract: Superconducting junctions with a ferromagnet as the weak link, where triplet correlations can transport supercurrents over a substantial distance, have been of long-standing interest. In this work, we study the triplet transport in planar La$_{0.7}$Sr$_{0.3}$MnO$_3$ (LSMO) nanowire Josephson junctions with NbTi superconducting contacts. By meticulous ion etching with an artificial Pt hard mask, th… ▽ More Superconducting junctions with a ferromagnet as the weak link, where triplet correlations can transport supercurrents over a substantial distance, have been of long-standing interest. In this work, we study the triplet transport in planar La$_{0.7}$Sr$_{0.3}$MnO$_3$ (LSMO) nanowire Josephson junctions with NbTi superconducting contacts. By meticulous ion etching with an artificial Pt hard mask, the NbTi/LSMO bilayer is structured to form an LSMO bridge without damaging its top layer. We observe superconducting (critical) currents of the order of 10$^{9}$ A/m$^2$ in a junction with a length of 1.3 $μ$m, and distinguishing superconducting quantum interference (SQI) patterns when sweeping a magnetic field perpendicular ($B_\perp$) to the plane of the wire or parallel ($B_\parallel$) to the plane and along the wire. The observed Gaussian-shaped SQI pattern is attributed to the diffusive transport of triplet pairs in the LSMO. Our work demonstrates that combinations of oxide magnets with conventional ($s$-wave) alloy superconductors can be a promising new route to realizing superconducting spintronics. △ Less

Submitted 24 April, 2024; originally announced April 2024.

Comments: 7 pages, 4 figures

Triplet supercurrents in lateral Josephson junctions with a half-metallic ferromagnet

Authors: Yao Junxiang, Remko Fermin, Mariona Cabero, Kaveh Lahabi, Jan Aarts

Abstract: In the area of superconducting spintronics, spin triplet supercurrents in half-metallic ferromagnets (HMFs) could yield dissipationless spin transport over large distances, and high current density. Promising among the HMFs is the perovskite oxide La0.7Sr0.3MnO3 (LSMO), and recent studies in combination with the high-Tc superconductor YBa2Cu3O7, or the conventional superconductor NbTi, showed long… ▽ More In the area of superconducting spintronics, spin triplet supercurrents in half-metallic ferromagnets (HMFs) could yield dissipationless spin transport over large distances, and high current density. Promising among the HMFs is the perovskite oxide La0.7Sr0.3MnO3 (LSMO), and recent studies in combination with the high-Tc superconductor YBa2Cu3O7, or the conventional superconductor NbTi, showed long range effects. Here we focus on two issues that as yet received less attention: the value of the critical current in the HMF in the limit of a very small electrode distance (20 nm), and the nature of the spin triplet generator. We use lateral junctions shaped as bar, square, and disk, and find high supercurrent densities, of order 10^11 A/m2, pointing to an efficient triplet generation mechanism. This is surprising in the sense that no magnetic inhomogeneity is purposely built in, as is done in conventional metal triplet junctions. Furthermore, from the magnetic field dependence of the critical current interference patterns we find a uniform supercurrent distribution in bar-shaped devices, but one more constricted to the rim in disk devices, which is an expected consequence of the geometry. We also analyze the temperature dependence of the critical current and find the quadratic dependence that was predicted in the limit of small junction lengths. From studying the NbTi/LSMO interface with scanning electron transmission microscopy, we conclude that the magnetic inhomogeneity required for triplet generation resides in the LSMO layer adjacent to the interface. △ Less

Submitted 9 October, 2024; v1 submitted 24 March, 2023; originally announced March 2023.

Comments: 9 pages, 6 figures

The unusual distribution of spin-triplet supercurrents in disk-shaped Josephson junctions

Authors: Remko Fermin, Junxiang Yao, Kaveh Lahabi, Jan Aarts

Abstract: The phenomenon of s-wave spin triplet Cooper pairs induced in ferromagnetic metals has been researched now for more than a decade, and its main aspects are well understood. Crucial in converting s-wave singlet pairs in the superconductor to s-wave triplets in the ferromagnet is the engineering of well-defined magnetic inhomogeneity (the 'generator') at the interface with the superconductor. Vertic… ▽ More The phenomenon of s-wave spin triplet Cooper pairs induced in ferromagnetic metals has been researched now for more than a decade, and its main aspects are well understood. Crucial in converting s-wave singlet pairs in the superconductor to s-wave triplets in the ferromagnet is the engineering of well-defined magnetic inhomogeneity (the 'generator') at the interface with the superconductor. Vertical layer stacks are typically used as such, where two separate thin ferromagnetic layers with homogeneous but non-collinear magnetizations, provide the inhomogeneity. Alternatively, magnetic textures, like ferromagnetic domain walls and vortices, are possible triplet generators, although they are far less studied. In this paper we review our experiments on lateral disk-shaped Josephson junctions where a ferromagnetic bottom layer provides a weak link with a vortex magnetization imposed by the shape of the disk. We present three different junction configurations, exhibiting their own generator mechanism. In the first, we utilize the non-collinearity with a second ferromagnetic layer to produce the triplet correlations. The second configuration consists of only the bottom ferromagnet and the superconducting contacts; it relies on the vortex magnetization itself to generate the spin-polarized supercurrents. In the third case we exploit an intrinsic generator by combining a conventional superconductor (NbTi) and a half-metallic ferromagnetic oxide (La$_{0.7}$Sr$_{0.3}$MnO$_3$). We find strong supercurrents in all cases. A particularly interesting finding is that the supercurrents are strongly confined at the rims of the device, independent of the generating mechanism, but directly related to their triplet nature. What causes these rim currents remains an open question. △ Less

Submitted 14 March, 2023; originally announced March 2023.

Beyond the effective length: How to analyze magnetic interference patterns of thin-film planar Josephson junctions with finite lateral dimensions

Authors: Remko Fermin, Bob de Wit and, Jan Aarts

Abstract: The magnetic field dependent critical current $I_{\text{c}}(B)$ of a Josephson junction is determined by the screening currents in its electrodes. In macroscopic junctions, a local vector potential drives the currents, however, in thin film planar junctions, with electrodes of finite size and various shapes, they are governed by non-local electrodynamics. This complicates the extraction of paramet… ▽ More The magnetic field dependent critical current $I_{\text{c}}(B)$ of a Josephson junction is determined by the screening currents in its electrodes. In macroscopic junctions, a local vector potential drives the currents, however, in thin film planar junctions, with electrodes of finite size and various shapes, they are governed by non-local electrodynamics. This complicates the extraction of parameters such as the geometry of the effective junction area, the effective junction length and, the critical current density distribution from the $I_{\text{c}}(B)$ interference patterns. Here we provide a method to tackle this problem by simulating the phase differences that drive the shielding currents and use those to find $I_{\text{c}}(B)$. To this end, we extend the technique proposed by John Clem [Phys. Rev. B, \textbf{81}, 144515 (2010)] to find $I_{\text{c}}(B)$ for Josephson junctions separating a superconducting strip of length $L$ and width $W$ with rectangular, ellipsoid and rhomboid geometries. We find the periodicity of the interference pattern ($ΔB$) to have geometry independent limits for $L \gg W$ and $L \ll W$. By fabricating elliptically shaped S$-$N$-$S junctions with various aspect ratios, we experimentally verify the $L/W$ dependence of $ΔB$. Finally, we incorporate these results to correctly extract the distribution of critical currents in the junction by the Fourier analysis of $I_{\text{c}}(B)$, which makes these results essential for the correct analysis of topological channels in thin film planar Josephson junctions. △ Less

Submitted 10 February, 2023; v1 submitted 11 October, 2022; originally announced October 2022.

Journal ref: Phys. Rev. B 107, 064502 (2023)

Mesoscopic superconducting memory based on bistable magnetic textures

Authors: Remko Fermin, Naor Scheinowitz, Jan Aarts, Kaveh Lahabi

Abstract: With the ever-increasing energy need to process big data, the realization of low-power computing technologies, such as superconducting logic and memories, has become a pressing issue. Developing fast and non-volatile superconducting memory elements, however, remains a challenge. Superconductor-ferromagnet hybrid devices offer a promising solution, as they combine ultra-fast manipulation of spins w… ▽ More With the ever-increasing energy need to process big data, the realization of low-power computing technologies, such as superconducting logic and memories, has become a pressing issue. Developing fast and non-volatile superconducting memory elements, however, remains a challenge. Superconductor-ferromagnet hybrid devices offer a promising solution, as they combine ultra-fast manipulation of spins with dissipationless readout. Here, we present a new type of non-volatile Josephson junction memory that utilizes the bistable magnetic texture of a single mesoscopic ferromagnet. We use micromagnetic simulations to design an ellipse-shaped planar junction structured from a Nb/Co bilayer. The ellipse can be prepared as uniformly magnetized or as a pair of vortices at zero applied field. The two states yield considerably different critical currents, enabling reliable electrical readout of the element. We describe the mechanism used to control the critical current by applying numerical calculations to quantify the local stray field from the ferromagnet, which shifts the superconducting interference pattern. By combining micromagnetic modeling with bistable spin-textured junctions, our approach presents a novel route towards realizing superconducting memory applications. △ Less

Submitted 14 June, 2022; originally announced June 2022.

Superconducting triplet rim currents in a spin-textured ferromagnetic disk

Authors: Remko Fermin, Dyon van Dinter, Michel Hubert, Bart Woltjes, Mikhail Silaev, Jan Aarts, Kaveh Lahabi

Abstract: Since the discovery of the long-range superconducting proximity effect, the interaction between spin-triplet Cooper pairs and magnetic structures such as domain walls and vortices has been the subject of intense theoretical discussions, while the relevant experiments remain scarce. We have developed nanostructured Josephson junctions with highly controllable spin texture, based on a disk-shaped Nb… ▽ More Since the discovery of the long-range superconducting proximity effect, the interaction between spin-triplet Cooper pairs and magnetic structures such as domain walls and vortices has been the subject of intense theoretical discussions, while the relevant experiments remain scarce. We have developed nanostructured Josephson junctions with highly controllable spin texture, based on a disk-shaped Nb/Co bilayer. Here, the vortex magnetization of Co and the Cooper pairs of Nb conspire to induce long-range triplet (LRT) superconductivity in the ferromagnet. Surprisingly, the LRT correlations emerge in highly localized (sub-80 nm) channels at the rim of the ferromagnet, despite its trivial band structure. We show that these robust rim currents arise from the magnetization texture acting as an effective spin-orbit coupling, which results in spin accumulation at the bilayer-vacuum boundary. Lastly, we demonstrate that by altering the spin texture of a single ferromagnet, both $0$ and $π$-channels can be realized in the same device. △ Less

Submitted 2 May, 2022; v1 submitted 25 October, 2021; originally announced October 2021.

Journal ref: Nano Letters 22 (2022) 2209-2216

On the resistance minimum in LaAlO$_3$/Eu$_{1-x}$La$_x$TiO$_3$/SrTiO$_3$ heterostructures

Authors: N. Lebedev, Y. Huang, A. Rana, D. Jannis, N. Gauquelin, J. Verbeeck, J. Aarts

Abstract: In this paper we study LaAlO$_3$/Eu$_{1-x}$La$_x$TiO$_3$/SrTiO$_3$ structures with nominally x = 0, 0.1 and different thicknesses of the Eu$_{1-x}$La$_x$TiO$_3$ layer. We observe that both systems have many properties similar to previously studied LaAlO$_3$/EuTiO$_3$/SrTiO$_3$ and other oxide interfaces, such as the formation of a 2D electron liquid for 1 or 2 unit cells of Eu$_{1-x}$La$_x$TiO… ▽ More In this paper we study LaAlO$_3$/Eu$_{1-x}$La$_x$TiO$_3$/SrTiO$_3$ structures with nominally x = 0, 0.1 and different thicknesses of the Eu$_{1-x}$La$_x$TiO$_3$ layer. We observe that both systems have many properties similar to previously studied LaAlO$_3$/EuTiO$_3$/SrTiO$_3$ and other oxide interfaces, such as the formation of a 2D electron liquid for 1 or 2 unit cells of Eu$_{1-x}$La$_x$TiO$_3$; a metal-insulator transition driven by the thickness increase of Eu$_{1-x}$La$_x$TiO$_3$ layer; the presence of an Anomalous Hall effect (AHE) when driving the systems above the Lifshitz point with a backgate voltage; and a minimum in the temperature dependence of the sheet resistance below the Lifshitz point in the one-band regime, which becomes more pronounced with increasing gate voltage. However, and notwithstanding the likely presence of magnetism in the system, we do not attribute that minimum to the Kondo effect, but rather to the properties of SrTiO$_3$ crystal and the inevitable effects of charge trapping when using back gates. △ Less

Submitted 1 September, 2021; originally announced September 2021.

Comments: 9 pages, 6 figures

Imaging spin-wave damping underneath metals using electron spins in diamond

Authors: Iacopo Bertelli, Brecht G. Simon, Tao Yu, Jan Aarts, Gerrit E. W. Bauer, Yaroslav M. Blanter, Toeno van der Sar

Abstract: Spin waves in magnetic insulators are low-damping signal carriers that could enable a new generation of spintronic devices. The excitation, control, and detection of spin waves by metal electrodes is crucial for interfacing these devices to electrical circuits. It is therefore important to understand metal-induced damping of spin-wave transport, but characterizing this process requires access to t… ▽ More Spin waves in magnetic insulators are low-damping signal carriers that could enable a new generation of spintronic devices. The excitation, control, and detection of spin waves by metal electrodes is crucial for interfacing these devices to electrical circuits. It is therefore important to understand metal-induced damping of spin-wave transport, but characterizing this process requires access to the underlying magnetic films. Here we show that spins in diamond enable imaging of spin waves that propagate underneath metals in magnetic insulators, and then use this capability to reveal a 100-fold increase in spin-wave damping. By analyzing spin-wave-induced currents in the metal, we derive an effective damping parameter that matches these observations well. We furthermore detect buried scattering centers, highlighting the technique's power for assessing spintronic device quality. Our results open new avenues for studying metal - spin-wave interaction and provide access to interfacial processes such as spin-wave injection via the spin-Hall effect. △ Less

Submitted 16 June, 2021; v1 submitted 4 June, 2021; originally announced June 2021.

Universal size-dependent nonlinear charge transport in single crystals of the Mott insulator Ca$_2$RuO$_4$

Authors: Guerino Avallone, Remko Fermin, Kaveh Lahabi, Veronica Granata, Rosalba Fittipaldi, Carla Cirillo, Carmine Attanasio, Antonio Vecchione, Jan Aarts

Abstract: The surprisingly low current density required for inducing the insulator to metal transition has made Ca$_2$RuO$_4$ an attractive candidate material for developing Mott-based electronics devices. The mechanism driving the resistive switching, however, remains a controversial topic in the field of strongly correlated electron systems. Here we probe an uncovered region of phase space by studying hig… ▽ More The surprisingly low current density required for inducing the insulator to metal transition has made Ca$_2$RuO$_4$ an attractive candidate material for developing Mott-based electronics devices. The mechanism driving the resistive switching, however, remains a controversial topic in the field of strongly correlated electron systems. Here we probe an uncovered region of phase space by studying high-purity Ca$_2$RuO$_4$ single crystals, using the sample size as principal tuning parameter. Upon reducing the crystal size, we find a four orders of magnitude increase in the current density required for driving Ca$_2$RuO$_4$ out of the insulating state into a non-equilibrium (also called metastable) phase which is the precursor to the fully metallic phase. By integrating a microscopic platinum thermometer and performing thermal simulations, we gain insight into the local temperature during simultaneous application of current and establish that the size dependence is not a result of Joule heating. The findings suggest an inhomogeneous current distribution in the nominally homogeneous crystal. Our study calls for a reexamination of the interplay between sample size, charge current, and temperature in driving Ca$_2$RuO$_4$ towards the Mott insulator to metal transition. △ Less

Submitted 12 November, 2021; v1 submitted 12 February, 2021; originally announced February 2021.

Journal ref: npj Quantum Materials 6 (2021) 91

Inhomogeneous superconductivity and quasilinear magnetoresistance at amorphous LaTiO3/SrTiO3 interfaces

Authors: N. Lebedev, M. Stehno, A. Rana, N. Gauquelin, J. Verbeeck, A. Brinkman, J. Aarts

Abstract: We have studied the transport properties of LaTiO3/SrTiO3 (LTO/STO) heterostructures. In spite of 2D growth observed in reflection high energy electron diffraction, Transmission Electron Microscopy images revealed that the samples tend to amorphize. Still, we observe that the structures are conducting, and some of them exhibit high conductance and/or superconductivity. We established that conducti… ▽ More We have studied the transport properties of LaTiO3/SrTiO3 (LTO/STO) heterostructures. In spite of 2D growth observed in reflection high energy electron diffraction, Transmission Electron Microscopy images revealed that the samples tend to amorphize. Still, we observe that the structures are conducting, and some of them exhibit high conductance and/or superconductivity. We established that conductivity arises mainly on the STO side of the interface, and shows all the signs of the 2-dimensional electron gas usually observed at interfaces between SrTiO3 and LaTiO3 or LaAlO3, including the presence of two electron bands and tunability with a gate voltage. Analysis of magnetoresistance (MR) and superconductivity indicates presence of a spatial fluctuations of the electronic properties in our samples. That can explain the observed quasilinear out-of-plane MR, as well as various features of the in-plane MR and the observed superconductivity. △ Less

Submitted 7 August, 2020; originally announced August 2020.

Comments: 10 pages, 6 figures, plus Supplementary Information

Magnetic resonance imaging of spin-wave transport and interference in a magnetic insulator

Authors: Iacopo Bertelli, Joris J. Carmiggelt, Tao Yu, Brecht G. Simon, Coosje C. Pothoven, Gerrit E. W. Bauer, Yaroslav M. Blanter, Jan Aarts, Toeno van der Sar

Abstract: Spin waves - the elementary excitations of magnetic materials - are prime candidate signal carriers for low dissipation information processing. Being able to image coherent spin-wave transport is crucial for developing interference-based spin-wave devices. We introduce a platform for probing coherent spin waves based on magnetic resonance imaging with electron spins in diamond. Focusing on a thin-… ▽ More Spin waves - the elementary excitations of magnetic materials - are prime candidate signal carriers for low dissipation information processing. Being able to image coherent spin-wave transport is crucial for developing interference-based spin-wave devices. We introduce a platform for probing coherent spin waves based on magnetic resonance imaging with electron spins in diamond. Focusing on a thin-film magnetic insulator, we quantify spin-wave amplitudes, visualize the dispersion, and demonstrate time-domain measurements of spin-wave packets. We use our platform to study spin-wave interference, revealing uni-directional, autofocused spin-wave patterns with frequency-controlled numerical apertures. A theoretical analysis explains the patterns in terms of chiral spin-wave excitation and stray-field coupling to the sensor spins. These results pave the way for probing spin waves in atomically thin magnets, even when embedded between opaque materials. △ Less

Submitted 16 April, 2020; originally announced April 2020.

Comments: 12 pages, 4 figures

Gate-tuned Anomalous Hall Effect Driven by Rashba Splitting in Intermixed LaAlO3/GdTiO3/SrTiO3

Authors: N. Lebedev, M. Stehno, A. Rana, P. Reith, N. Gauquelin, J. Verbeeck, H. Hilgenkamp, A. Brinkman, J. Aarts

Abstract: The Anomalous Hall Effect (AHE) is an important quantity in determining the properties and understanding the behavior of the two-dimensional electron system forming at the interface of SrTiO3-based oxide heterostructures. The occurrence of AHE is often interpreted as a signature of ferromagnetism, but it is becoming more and more clear that also paramagnets may contribute to AHE. We studied the in… ▽ More The Anomalous Hall Effect (AHE) is an important quantity in determining the properties and understanding the behavior of the two-dimensional electron system forming at the interface of SrTiO3-based oxide heterostructures. The occurrence of AHE is often interpreted as a signature of ferromagnetism, but it is becoming more and more clear that also paramagnets may contribute to AHE. We studied the influence of magnetic ions by measuring intermixed LaAlO3/GdTiO3/SrTiO3 at temperatures below 10 K. We find that, as function of gate voltage, the system undergoes a Lifshitz transition, while at the same time an onset of AHE is observed. However, we do not observe clear signs of ferromagnetism. We argue the AHE to be due to the change in Rashba spin-orbit coupling at the Lifshitz transition and conclude that also paramagnetic moments which are easily polarizable at low temperatures and high magnetic filds lead to the presence of AHE, which needs to be taken into account when extracting carrier densities and mobilities. △ Less

Submitted 26 February, 2020; originally announced February 2020.

Comments: 11 pages, 8 figures; and supplement

Spontaneous emergence of Josephson junctions in homogeneous rings of single-crystal Sr2RuO4

Authors: Yuuki Yasui, Kaveh Lahabi, Victor Fernández Becerra, Remko Fermin, Muhammad Shahbaz Anwar, Shingo Yonezawa, Takahito Terashima, Milorad V. Milošević, Jan Aarts, Yoshiteru Maeno

Abstract: The chiral p-wave order parameter in Sr$_\mathsf{2}$RuO$_\mathsf{4}$ would make it a special case amongst the unconventional superconductors. A consequence of this symmetry is the possible existence of superconducting domains of opposite chirality. At the boundary of such domains, the locally supressed condensate can produce an intrinsic Josephson junction. Here, we provide evidence of such juncti… ▽ More The chiral p-wave order parameter in Sr$_\mathsf{2}$RuO$_\mathsf{4}$ would make it a special case amongst the unconventional superconductors. A consequence of this symmetry is the possible existence of superconducting domains of opposite chirality. At the boundary of such domains, the locally supressed condensate can produce an intrinsic Josephson junction. Here, we provide evidence of such junctions using mesoscopic rings, structured from Sr$_\mathsf{2}$RuO$_\mathsf{4}$ single crystals. Our order parameter simulations predict such rings to host stable domain walls across their arms. Thisis verified with transport experiments on loops, with a sharp transition at 1.5 K, which show distinct critical current oscillations with periodicity corresponding to the flux quantum. In contrast, loops with broadened transitions at around 3 K are void of such junctions and show standard Little-Parks oscillations. Our analysis demonstrates the junctions are of intrinsic origin and makes a compelling case for the existence of superconducting domains. △ Less

Submitted 16 February, 2020; originally announced February 2020.

Comments: 27+11 pages, 6+4 figures

Journal ref: npj Quantum Mater. 5, 21 (2020)

Growing a LaAlO3/SrTiO3 heterostructure on Ca2Nb3O10 nanosheets

Authors: Alexander J. H. van der Torren, Huiyu Yuan, Zhaoliang Liao, Johan E. ten Elshof, Gertjan Koster, Mark Huijben, Guus J. H. M. Rijnders, Marcel B. S. Hesselberth, Johannes Jobst, Sense van der Molen, Jan Aarts

Abstract: The two-dimensional electron liquid which forms between the band insulators LaAlO3 (LAO) and SrTiO3 (STO) is a promising component for oxide electronics, but the requirement of using single crystal SrTiO3 substrates for the growth limits its applications in terms of device fabrication. It is therefore important to find ways to deposit these materials on other substrates, preferably Si, or Si-based… ▽ More The two-dimensional electron liquid which forms between the band insulators LaAlO3 (LAO) and SrTiO3 (STO) is a promising component for oxide electronics, but the requirement of using single crystal SrTiO3 substrates for the growth limits its applications in terms of device fabrication. It is therefore important to find ways to deposit these materials on other substrates, preferably Si, or Si-based, in order to facilitate integration with existing technology. Interesting candidates are micron-sized nanosheets of Ca2Nb3O10 which can be used as seed layers for perovskite materials on any substrate. We have used low-energy electron microscopy (LEEM) with in-situ pulsed laser deposition to study the subsequent growth of STO and LAO on such flakes which were deposited on Si. We can follow the morphology and crystallinity of the layers during growth, as well as fingerprint their electronic properties with angle resolved reflected electron spectroscopy. We find that STO layers, deposited on the nanosheets, can be made crystalline and flat; that LAO can be grown in a layer-by-layer fashion; and that the full heterostructure shows the signature of the formation of a conducting interface. △ Less

Submitted 13 October, 2019; originally announced October 2019.

Comments: 11 pages, 7 figures

Tunable magnetic interactions in LaAlO3/SrTiO3 heterostructures by ionic liquid gating

Authors: Chunhai Yin, Kumar Prateek, Wouter Gelling, Jan Aarts

Abstract: The gating effect achieved by an ionic liquid and its electric double layer allows for charge transfer which can be an order of magnitude larger than with conventional dielectrics. However, the large charged ions also causes inevitable Coulomb scattering in the conducting channel formed at the interface, which can limit the carrier mobility enhancement. In this work, we study the effect of the LaA… ▽ More The gating effect achieved by an ionic liquid and its electric double layer allows for charge transfer which can be an order of magnitude larger than with conventional dielectrics. However, the large charged ions also causes inevitable Coulomb scattering in the conducting channel formed at the interface, which can limit the carrier mobility enhancement. In this work, we study the effect of the LaAlO3 thickness on the transport properties in LaAlO3/SrTiO3 heterostructures by ionic liquid gating. We find that the transport properties of the LaAlO3/SrTiO3 interface are dominated by the intrinsic interactions rather than the LaAlO3 thickness and possible effects from the ions in the liquid. We observe a Kondo effect, which is enhanced while increasing the gate voltage. We also observe a gate-tunable and temperature-dependent anomalous Hall effect, which always emerges near the Kondo temperature. Our experiments pave the way to manipulate the various magnetic interactions in LaAlO3/SrTiO3 heterostructures. △ Less

Submitted 25 April, 2019; originally announced April 2019.

Tuning Rashba spin-orbit coupling at LaAlO3/SrTiO3 interfaces by band filling

Authors: Chunhai Yin, Patrick Seiler, Lucas M. K. Tang, Inge Leermakers, Nikita Lebedev, Uli Zeitler, Jan Aarts

Abstract: The electric-field tunable Rashba spin-orbit coupling at the LaAlO3/SrTiO3 interface shows potential applications in spintronic devices. However, different gate dependence of the coupling strength has been reported in experiments. On the theoretical side, it has been predicted that the largest Rashba effect appears at the crossing point of the $d_{xy}$ and $d_{xz,yz}$ bands. In this work, we study… ▽ More The electric-field tunable Rashba spin-orbit coupling at the LaAlO3/SrTiO3 interface shows potential applications in spintronic devices. However, different gate dependence of the coupling strength has been reported in experiments. On the theoretical side, it has been predicted that the largest Rashba effect appears at the crossing point of the $d_{xy}$ and $d_{xz,yz}$ bands. In this work, we study the tuneability of the Rashba effect in LaAlO3/SrTiO3 by means of back-gating. The Lifshitz transition was crossed multiple times by tuning the gate voltage so that the Fermi energy is tuned to approach or depart from the band crossing. By analyzing the weak antilocalization behavior in the magnetoresistance, we find that the maximum spin-orbit coupling effect occurs when the Fermi energy is near the Lifshitz point. Moreover, we find strong evidence for a single spin winding at the Fermi surface. △ Less

Submitted 7 April, 2019; originally announced April 2019.

Comments: 5 pages, 4 figures

Journal ref: Phys. Rev. B 101, 245114 (2020)

New insights into the electron trapping mechanism in LaAlO_3 / SrTiO3 heterostructures

Authors: Chunhai Yin, Alexander E. M. Smink, Inge Leermakers, Lucas M. K. Tang, Nikita Lebedev, Uli Zeitler, Wilfred G. van der Wiel, Hans Hilgenkamp, Jan Aarts

Abstract: In LaAlO3/SrTiO3 heterostructures, a commonly observed but poorly understood phenomenon is that of electron trapping in back-gating experiments. In this work, by combining magnetotransport measurements and self-consistent Schroedinger-Poisson calculations, we obtain an empirical relation between the amount of trapped electrons and the gate voltage. We find that the trapped electrons follow an expo… ▽ More In LaAlO3/SrTiO3 heterostructures, a commonly observed but poorly understood phenomenon is that of electron trapping in back-gating experiments. In this work, by combining magnetotransport measurements and self-consistent Schroedinger-Poisson calculations, we obtain an empirical relation between the amount of trapped electrons and the gate voltage. We find that the trapped electrons follow an exponentially decaying spatial distribution away from the interface. However, contrary to earlier observations, we find that the Fermi level remains well within the quantum well. The enhanced trapping of electrons induced by the gate voltage can therefore not be explained by a thermal escape mechanism. Further gate sweeping experiments strengthen our conclusion that the thermal escape mechanism is not valid. We propose a new mechanism which involves the electromigration and clustering of oxygen vacancies in SrTiO3. Our work indicates that electron trapping is a universal phenomenon in SrTiO3-based two-dimensional electron systems. △ Less

Submitted 20 February, 2019; originally announced February 2019.

Comments: manuscript + supplementary information, 8 pages

Journal ref: Phys. Rev. Lett. 124, 017702 (2020)

Quantifying work function differences using low-energy electron microscopy: the case of mixed-terminated strontium titanate

Authors: Johannes Jobst, Laurens M. Boers, Chunhai Yin, Jan Aarts, Rudolf M. Tromp, Sense Jan van der Molen

Abstract: For many applications, it is important to measure the local work function of a surface with high lateral resolution. Low-energy electron microscopy is regularly employed to this end since it is, in principle, very well suited as it combines high-resolution imaging with high sensitivity to local electrostatic potentials. For surfaces with areas of different work function, however, lateral electrost… ▽ More For many applications, it is important to measure the local work function of a surface with high lateral resolution. Low-energy electron microscopy is regularly employed to this end since it is, in principle, very well suited as it combines high-resolution imaging with high sensitivity to local electrostatic potentials. For surfaces with areas of different work function, however, lateral electrostatic fields inevitably associated with work function discontinuities deflect the low-energy electrons and thereby cause artifacts near these discontinuities. We use ray-tracing simulations to show that these artifacts extend over hundreds of nanometers and cause an overestimation of the true work function difference near the discontinuity by a factor of 1.6 if the standard image analysis methods are used. We demonstrate on a mixed-terminated strontium titanate surface that comparing LEEM data with detailed ray-tracing simulations leads to much a more robust estimate of the work function difference. △ Less

Submitted 14 December, 2018; originally announced December 2018.

Journal ref: Ultramicroscopy 200, 43 (2019)

Influence of stoichiometry on interfacial conductance in LaAlO$_3$/SrTiO$_3$ grown by 90$^o$ off-axis sputtering

Authors: Chunhai Yin, Dileep Krishnan, Nicolas Gauquelin, Jo Verbeeck, Jan Aarts

Abstract: We report on the fabrication of conducting interfaces between LaAlO$_3$ and SrTiO$_3$ by 90$^o$ off-axis sputtering in an Ar atmosphere. At a growth pressure of 0.04 mbar the interface is metallic, with a carrier density of the order of $10^{13}$ cm$^{-2}$ at 3 K. By increasing the growth pressure, we observe an increase of the out-of-plane lattice constants of the LaAlO$_3$ films while the in-pla… ▽ More We report on the fabrication of conducting interfaces between LaAlO$_3$ and SrTiO$_3$ by 90$^o$ off-axis sputtering in an Ar atmosphere. At a growth pressure of 0.04 mbar the interface is metallic, with a carrier density of the order of $10^{13}$ cm$^{-2}$ at 3 K. By increasing the growth pressure, we observe an increase of the out-of-plane lattice constants of the LaAlO$_3$ films while the in-plane lattice constants do not change. Also, the low-temperature sheet resistance increases with increasing growth pressure, leading to an insulating interface when the growth pressure reaches 0.10 mbar. We attribute the structural variations to an increase of the La/Al ratio, which also explains the transition from metallic behavior to insulating behavior of the interfaces. Our research emphasizes the key role of the cation stoichiometry of LaAlO$_3$ in the formation of the conducting interface, and also the control which is furnished by the Ar pressure in the growth process. △ Less

Submitted 2 November, 2018; originally announced November 2018.

Comments: 4 pages, 4 figures; manuscript under review

Little-Parks oscillations with half-quantum fluxoid features in Sr2RuO4 micro rings

Authors: Yuuki Yasui, Kaveh Lahabi, Muhammad Shahbaz Anwar, Yuji Nakamura, Shingo Yonezawa, Takahito Terashima, Jan Aarts, Yoshiteru Maeno

Abstract: In a micro ring of a superconductor with a spin-triplet equal-spin pairing state, a fluxoid, a combined object of magnetic flux and circulating supercurrent, can penetrate as half-integer multiples of the flux quantum. A candidate material to investigate such half-quantum fluxoids is Sr$_\mathsf{2}$RuO$_\mathsf{4}$. We fabricated Sr$_\mathsf{2}$RuO$_\mathsf{4}$ micro rings using single crystals an… ▽ More In a micro ring of a superconductor with a spin-triplet equal-spin pairing state, a fluxoid, a combined object of magnetic flux and circulating supercurrent, can penetrate as half-integer multiples of the flux quantum. A candidate material to investigate such half-quantum fluxoids is Sr$_\mathsf{2}$RuO$_\mathsf{4}$. We fabricated Sr$_\mathsf{2}$RuO$_\mathsf{4}$ micro rings using single crystals and measured their resistance behavior under magnetic fields controlled with a three-axes vector magnet. Proper Little-Parks oscillations in the magnetovoltage as a function of an axially applied field, associated with fluxoid quantization are clearly observed, for the first time using bulk single crystalline superconductors. We then performed magnetovoltage measurements with additional in-plane magnetic fields. By carefully analyzing both the voltages $V_+$ ($V_-$) measured at positive (negative) current, we find that, above an in-plane threshold field of about 10 mT, the magnetovoltage maxima convert to minima. We interpret this behavior as the peak splitting expected for the half-quantum fluxoid states. △ Less

Submitted 31 October, 2017; originally announced October 2017.

Comments: 16 pages, 15 figures

Journal ref: Phys. Rev. B 96 (2017) 180507(R)

Formation of a conducting LaAlO$_3$ / SrTiO$_3$ interface studied by low energy electron reflection during growth

Authors: A. J. H. van der Torren, Z. Liao, C. Xu, N. Gauquelin, C. Yin, J. Aarts, S. J. van der Molen

Abstract: The two-dimensional electron gas occurring between the band insulators SrTiO$_3$ and LaAlO$_3$ continues to attract considerable interest, due to the possibility of dynamic control over the carrier density, and the ensuing phenomena such as magnetism and superconductivity. The formation of this conducting interface is sensitive to the growth conditions, but despite numerous investigations, there a… ▽ More The two-dimensional electron gas occurring between the band insulators SrTiO$_3$ and LaAlO$_3$ continues to attract considerable interest, due to the possibility of dynamic control over the carrier density, and the ensuing phenomena such as magnetism and superconductivity. The formation of this conducting interface is sensitive to the growth conditions, but despite numerous investigations, there are still questions about the details of the physics involved. In particular, not much is known about the electronic structure of the growing LaAlO$_3$ layer at the growth temperature (around 800 $^o$C) in oxygen (pressure around $5\times 10^{-5}$ mbar), since analysis techniques at these conditions are not readily available. We developed a pulsed laser deposition system inside a low-energy electron microscope in order to study this issue. The setup allows for layer-by-layer growth control and in-situ measurements of the angle-dependent electron reflection intensity, which can be used as a fingerprint of the electronic structure of the surface layers during growth. By using different substrate terminations and growth conditions we observe two families of reflectivity maps, which we can connect either to samples with an AlO$_2$-rich surface and a conducting interface; or to samples with a LaO-rich surface and an insulating interface. Our observations emphasize that substrate termination and stoichiometry determine the electronic structure of the growing layer, and thereby the conductance of the interface. △ Less

Submitted 8 September, 2017; originally announced September 2017.

Comments: 8 pages, 5 figures

Journal ref: Phys. Rev. Materials 1, 075001 (2017)

Controlling supercurrents and their spatial distribution in ferromagnets

Authors: Kaveh Lahabi, Morten Amundsen, Jabir Ali Ouassou, Ewout Beukers, Menno Pleijster, Jacob Linder, Paul Alkemade, Jan Aarts

Abstract: Spin-triplet Cooper pairs induced in ferromagnets form the centrepiece of the emerging field of superconducting spintronics [1,2]. Usually the focus of research is on the spin polarization of the triplets, potentially enabling low-dissipation magnetization switching and domain wall motion. However, the fundamental mechanism for generating triplet pairs [3,4] also permits control over a parameter w… ▽ More Spin-triplet Cooper pairs induced in ferromagnets form the centrepiece of the emerging field of superconducting spintronics [1,2]. Usually the focus of research is on the spin polarization of the triplets, potentially enabling low-dissipation magnetization switching and domain wall motion. However, the fundamental mechanism for generating triplet pairs [3,4] also permits control over a parameter which has not been addressed before, namely the spatial distribution of the supercurrent. Here we demonstrate this control by tailoring distinct supercurrent pathways in the ferromagnetic weak link of a Josephson junction. Combining micromagnetic simulations with three-dimensional critical current calculations, based on the Usadel description of mesoscopic superconductivity [5], we designed a disk-shaped structure with a magnetic vortex, which induces two distinct supercurrent channels across the junction. The design was successfully tested with superconducting quantum interferometry (SQI). Moreover, we show how the position of the pathways can be controlled by moving the vortex with a magnetic field. This novel approach allows adaptable supercurrent paths to be dynamically reconfigured to switch between different functionalities in the same device. △ Less

Submitted 19 May, 2017; originally announced May 2017.

Comments: 27 pages, 10 figures

Long-range proximity effect in Nb-based heterostructures induced by a magnetically inhomogeneous permalloy layer

Authors: Carla Cirillo, Stefano Voltan, Katsiaryna Ilyina, Joan Manel Hernandez, Antoni Garcia-Santiago, Jan Aarts, Carmine Attanasio

Abstract: Odd-frequency triplet Cooper pairs are believed to be the carriers of long-range superconducting correlations in ferromagnets. Such triplet pairs are generated by inhomogeneous magnetism at the interface between a superconductor (S) and a ferromagnet (F). So far, reproducible long-range effects were reported only in complex layered structures designed to provide the magnetic inhomogeneity. Here we… ▽ More Odd-frequency triplet Cooper pairs are believed to be the carriers of long-range superconducting correlations in ferromagnets. Such triplet pairs are generated by inhomogeneous magnetism at the interface between a superconductor (S) and a ferromagnet (F). So far, reproducible long-range effects were reported only in complex layered structures designed to provide the magnetic inhomogeneity. Here we show that spin triplet pair formation can be found in simple unstructured Nb/Permalloy (Py = Ni_0.8Fe_0.2)/Nb trilayers and Nb/Py bilayers, but only when the thickness of the ferromagnetic layer ranges between 140 and 250 nm. The effect is related to the emergence of an intrinsically inhomogeneous magnetic state, which is a precursor of the well-known stripe regime in Py that in our samples sets in at thickness larger than 300 nm. △ Less

Submitted 9 February, 2017; originally announced February 2017.

Comments: accepted for publication on New Journal of Physics, available online http://iopscience.iop.org/article/10.1088/1367-2630/aa5de8

Hybrid cold and hot-wall chamber for fast synthesis of uniform graphene

Authors: Hadi Arjmandi-Tash, Nikita Lebedev, Pauline van Deursen, Jan Aarts, Grégory F. Schneider

Abstract: We introduce a novel modality in the CVD growth of graphene which combines the cold-wall and hot-wall reaction chambers. This hybrid mode preserves the advantages of a cold-wall chamber as the fast growth and low fuel consumption, but boosts the quality of the growth towards conventional CVD with hot-wall chambers. The synthesized graphene is uniform and monolayer. The electronic transport measure… ▽ More We introduce a novel modality in the CVD growth of graphene which combines the cold-wall and hot-wall reaction chambers. This hybrid mode preserves the advantages of a cold-wall chamber as the fast growth and low fuel consumption, but boosts the quality of the growth towards conventional CVD with hot-wall chambers. The synthesized graphene is uniform and monolayer. The electronic transport measurements shows great improvements in charge carrier mobility compared to graphene synthesized in a normal cold-wall reaction chamber. Our results promise the development of a fast and cost-efficient growth of high quality graphene, suitable for scalable industrial applications. △ Less

Submitted 9 January, 2017; originally announced January 2017.

Emergence of the stripe-domain phase in patterned Permalloy films

Authors: S. Voltan, C. Cirillo, H. J. Snijders, K. Lahabi, A. Garcia-Santiago, J. M. Hernandez, C. Attanasio, J. Aarts

Abstract: The occurrence of stripe domains in ferromagnetic Permalloy (Py=Fe$_{20}$Ni$_{80}$) is a well known phenomenon which has been extensively observed and characterized. This peculiar magnetic configuration appears only in films with a thickness above a critical value ($d_{cr}$), which is strongly determined by the sputtering conditions (i.e. deposition rate, temperature, magnetic field). So far,… ▽ More The occurrence of stripe domains in ferromagnetic Permalloy (Py=Fe$_{20}$Ni$_{80}$) is a well known phenomenon which has been extensively observed and characterized. This peculiar magnetic configuration appears only in films with a thickness above a critical value ($d_{cr}$), which is strongly determined by the sputtering conditions (i.e. deposition rate, temperature, magnetic field). So far, $d_{cr}$ has usually been presented as the boundary between the homogeneous (H) and stripe-domains (SD) regime, respectively below and above $d_{cr}$. In this work we study the transition from the H to the SD regime in thin films and microstructured bridges of Py with different thicknesses. We find there is an intermediate regime, over a quite significant thickness range below d$_{cr}$, which is signaled in confined structures by a quickly changing domain-wall configuration and by a broadening of the magnetoresistance dip at the coercive field. We call this the emerging stripe-domains (ESD) regime. The transition from the ESD to the SD regime is accompanied by a sharp increase of the magnetoresistance ratio at the thickness where stripes appear in MFM. △ Less

Submitted 4 August, 2016; originally announced August 2016.

Comments: 9 pages, 9 figures

Journal ref: Phys. Rev. B 94, 094406 (2016)

Growth of half-metallic CrO2 nanostructures for superconducting spintronic applications

Authors: A. Singh, C. Jansen, K. Lahabi, J. Aarts

Abstract: Superconductor-ferromagnet (S-F) hybrids based on half-metallic ferromagnets, such as CrO2, are excellent candidates for superconducting spintronic applications. This is primarily due to their fully spin polarized nature, which produces significantly enhanced long-range triplet proximity effects.. However, reliable production of CrO2-based Josephson junctions (JJs) is challenging, mainly because o… ▽ More Superconductor-ferromagnet (S-F) hybrids based on half-metallic ferromagnets, such as CrO2, are excellent candidates for superconducting spintronic applications. This is primarily due to their fully spin polarized nature, which produces significantly enhanced long-range triplet proximity effects.. However, reliable production of CrO2-based Josephson junctions (JJs) is challenging, mainly because of the difficulty to control the transparency of the S/F interface. We have grown CrO2 nanowires by chemical vapor deposition on TiO2 substrates combined with selective area growth in trenches defined with amorphous SiOx. This allows us to create lateral JJs, with the nanowire as the weak link. We show that the nature of the growth is highly anisotropic, and that the morphology of the CrO2 nanostructructures changes systematically during the growth process, depending on the width of the trench. The detailed growth study enables us to synthesise multifaceted and highly homogeneous CrO2 wires. These are utilized to fabricate JJs with high S/F interface transparency, leading to large supercurrents. The well-defined geometry of the device allows us to reliably estimate an exceptionally high critical current density Jc = 10^9~Am^{-2} over a distance of 600~nm. △ Less

Submitted 8 March, 2016; originally announced March 2016.

Comments: 5 figures

Striped nanoscale phase separation at the metal-insulator transition of heteroepitaxial nickelates

Authors: Giordano Mattoni, Pavlo Zubko, Francesco Maccherozzi, Alexander J. H. van der Torren, Daan B. Boltje, Marios Hadjimichael, Nicola Manca, Sara Catalano, Marta Gibert, Yanwei Liu, Jan Aarts, Jean-Marc Triscone, Sarnjeet S. Dhesi, Andrea D. Caviglia

Abstract: Nucleation processes of mixed-phase states are an intrinsic characteristic of first-order phase transitions, typically related to local symmetry breaking. Direct observation of emerging mixed-phase regions in materials showing a first-order metal-insulator transition (MIT) offers unique opportunities to uncover their driving mechanism. Using photoemission electron microscopy, we image the nanoscal… ▽ More Nucleation processes of mixed-phase states are an intrinsic characteristic of first-order phase transitions, typically related to local symmetry breaking. Direct observation of emerging mixed-phase regions in materials showing a first-order metal-insulator transition (MIT) offers unique opportunities to uncover their driving mechanism. Using photoemission electron microscopy, we image the nanoscale formation and growth of insulating domains across the temperature-driven MIT in NdNiO3 epitaxial thin films. Heteroepitaxy is found to strongly determine the nanoscale nature of the phase transition, inducing preferential formation of striped domains along the terraces of atomically flat stepped surfaces. We show that the distribution of transition temperatures is an intrinsic local property, set by surface morphology and stable across multiple temperature cycles. Our data provides new insights into the MIT of heteroepitaxial nickelates and points to a rich, nanoscale phenomenology in this strongly correlated material. △ Less

Submitted 16 November, 2016; v1 submitted 14 February, 2016; originally announced February 2016.

Journal ref: Nat. Commun. 7 (2016)

The effect of magnetic field on the intrinsic detection efficiency of superconducting single-photon detectors

Authors: J. J. Renema, R. J. Rengelink, I. Komen, Q. Wang, R. Gaudio, K. P. M. op 't Hoog, Z. Zhou, D. Sahin, A. Fiore, P. Kes, J. Aarts, M. P. van Exter, M. J. A. de Dood, E. F. C. Driessen

Abstract: We experimentally investigate the effect of a magnetic field on photon detection in superconducting single-photon detectors. At low fields, the effect of a magnetic field is through the direct modification of the quasiparticle density of states of the superconductor, and magnetic field and bias current are interchangable, as is expected for homogeneous dirty-limit superconductors. At the field whe… ▽ More We experimentally investigate the effect of a magnetic field on photon detection in superconducting single-photon detectors. At low fields, the effect of a magnetic field is through the direct modification of the quasiparticle density of states of the superconductor, and magnetic field and bias current are interchangable, as is expected for homogeneous dirty-limit superconductors. At the field where a first vortex enters the detector, the effect of the magnetic field is reduced, up until the point where the critical current of the detector starts to be determined by flux flow. From this field on, increasing the magnetic field does not alter the detection of photons anymore, whereas it does still change the rate of dark counts. This result points at an intrinsic difference in dark and light counts, and also shows that no enhancement of the intrinsic detection efficiency of a straight SSPD wire is achievable in a magnetic field. △ Less

Submitted 31 October, 2014; originally announced October 2014.

Colossal proximity effect in a superconducting triplet spin valve based on halfmetallic ferromagnetic CrO2

Authors: A. Singh, S. Voltan, K. Lahabi, J. Aarts

Abstract: Ferromagnets can sustain supercurrents through the formation of equal spin triplet Cooper pairs and the mechanism of odd-frequency pairing. Since such pairs are not broken by the exchange energy of the ferromagnet, superconducting triplet correlations are long-ranged and spin-polarized, with promises for superconducting spintronics devices. The main challenge is to understand how triplets are gene… ▽ More Ferromagnets can sustain supercurrents through the formation of equal spin triplet Cooper pairs and the mechanism of odd-frequency pairing. Since such pairs are not broken by the exchange energy of the ferromagnet, superconducting triplet correlations are long-ranged and spin-polarized, with promises for superconducting spintronics devices. The main challenge is to understand how triplets are generated at the superconductor (S)/ ferromagnet (F) interface. Here we use the concept of a so-called triplet spin valve (TSV) to investigate the conversion of singlets in a conventional superconductor to triplets in the halfmetallic ferromagnet CrO_2. TSV's are composed of two ferromagnetic layers (separated by a thin normal metal (N) layer) and a superconductor (F_1/N/F_2/S). The package F_1/N/F_2 generates triplets in F_1 when the magnetization directions of the F_{1,2}-layers are not collinear. This drains singlet pairs from the S-layer, and triplet generation is therefore signalled by a decrease of the critical temperature $T_c$. Recently, experiments with TSV's were reported with Co draining layers, using in-plane fields, and finding T_c-shifts up to 100~mK. Using CrO_2 instead of Co and rotating a magnetic field from in-plane to out-of-plane, we find strong T_c variations of almost a Kelvin up to fields of the order of a Tesla. Such strong drainage is consistent with the large lengths over which supercurrents can flow in CrO_2, which are significantly larger than in conventional ferromagnets. Our results point to the special interest of halfmetals for superconducting spintronics. △ Less

Submitted 18 October, 2014; originally announced October 2014.

Comments: 6 pages, 5 figures; supplementary information separate

Andreev spectroscopy of CrO$_{2}$ thin films on TiO$_{2}$ and Al$_{2}$O$_{3}$

Authors: KA Yates, MS Anwar, J Aarts, O Conde, M Eschrig, T Löfwander, LF Cohen

Abstract: Here we analyse the spectroscopic information gathered at a number of single CrO$_{2}$ / Pb interfaces. We examine thin films requiring additional interfacial layers to generate long range spin triplet proximity effect superconductivity (CrO$_{2}$/TiO$_{2}$) or not (CrO$_{2}$/Al$_{2}$O$_{3}$). We analyse the data using two theoretical models and explore the use of a parameter free method to determ… ▽ More Here we analyse the spectroscopic information gathered at a number of single CrO$_{2}$ / Pb interfaces. We examine thin films requiring additional interfacial layers to generate long range spin triplet proximity effect superconductivity (CrO$_{2}$/TiO$_{2}$) or not (CrO$_{2}$/Al$_{2}$O$_{3}$). We analyse the data using two theoretical models and explore the use of a parameter free method to determine the agreement between the models and experimental observations, showing the necessary temperature range that would be required to make a definitive statement. The use of the excess current as a further tool to distinguish between models is also examined. Analysis of the spectra demonstrates that the temperature dependence of the normalised zero bias conductance is independent of the substrate onto which the films are grown. This result has important implications for the engineering of interfaces required for the long range spin triplet proximity effect. △ Less

Submitted 1 November, 2013; originally announced November 2013.

Comments: 5 pages, 4 figures

Journal ref: EPL, 103, 67005 (2013)

Interface induced room-temperature ferromagnetism in hydrogenated epitaxial graphene

Authors: A. J. M. Giesbers, K. Uhlířová, M. Konečný, E. C. Peters, M. Burghard, J. Aarts, C. F. J. Flipse

Abstract: Due to the predominantly surface character of graphene, it is highly suitable for functionalization with external atoms and/or molecules leading to a plethora of new and interesting phenomena. Here we show ferromagnetic properties of hydrogen-functionalized epitaxial graphene on SiC. Ferromagnetism in such a material is not directly evident as it is inherently composed of only non-magnetic constit… ▽ More Due to the predominantly surface character of graphene, it is highly suitable for functionalization with external atoms and/or molecules leading to a plethora of new and interesting phenomena. Here we show ferromagnetic properties of hydrogen-functionalized epitaxial graphene on SiC. Ferromagnetism in such a material is not directly evident as it is inherently composed of only non-magnetic constituents. Our results nevertheless show strong ferromagnetism, which cannot be explained by simple magnetic impurities. The ferromagnetism is unique to hydrogenated epitaxial graphene on SiC, where interactions with the interfacial buffer layer play a crucial role. We argue that the origin of the observed ferromagnetism is governed by electron correlation effects of the narrow Si-dangling-bond (Si-DB) states in the buffer layer exchange-coupled to localized states in the hydrogenated graphene layer. This forms a quasi-three-dimensional ferromagnet with a Curie temperature higher than 300 K. △ Less

Submitted 14 May, 2013; originally announced May 2013.

Comments: 23 pages, 7 figures, including supplementary information

Anomalous transport in half-metallic ferromagnetic CrO2

Authors: M. S. Anwar, J. Aarts

Abstract: We have investigated transport properties of CrO2 thin films deposited on TiO2 and sapphire substrates. The films are good metals down to low temperatures. The residual resistivity is of the order of 6 micro-ohhmcm for films deposited on TiO2 and two times higher for films on sapphire substrates. The sign of the magnetoresistance (MR) changes from negative to positive at a temperature around 100 K… ▽ More We have investigated transport properties of CrO2 thin films deposited on TiO2 and sapphire substrates. The films are good metals down to low temperatures. The residual resistivity is of the order of 6 micro-ohhmcm for films deposited on TiO2 and two times higher for films on sapphire substrates. The sign of the magnetoresistance (MR) changes from negative to positive at a temperature around 100 K. This fact, as well as a rapid change in the ordinary and anomalous Hall coefficients suggest a change in the electronic state. At lower temperatures the MR is a linear function of the applied field. This linear dependence might be explained as intergrain tunneling MR. This interpretation is also suggested by the angular MR. The planar Hall effect measurements reveal that the CrO2 thin films are not in a single magnetic domain state even for films deposited on an isostructural TiO2 substrate. △ Less

Submitted 15 March, 2013; originally announced March 2013.

Sputter gas pressure effects on the properties of Sm-Co thin films deposited from a single target

Authors: T. G. A. Verhagen, D. B. Boltje, J. M. van Ruitenbeek, J. Aarts

Abstract: We grow epitaxial Sm-Co thin films by sputter deposition from an alloy target with a nominal SmCo5 composition on Cr(100)-buffered MgO(100) single-crystal substrates. By varying the Ar gas pressure, we can change the composition of the film from a SmCo5-like to a Sm2Co7-like phase. The composition, crystal structure, morphology and magnetic properties of these films have been determined using Ruth… ▽ More We grow epitaxial Sm-Co thin films by sputter deposition from an alloy target with a nominal SmCo5 composition on Cr(100)-buffered MgO(100) single-crystal substrates. By varying the Ar gas pressure, we can change the composition of the film from a SmCo5-like to a Sm2Co7-like phase. The composition, crystal structure, morphology and magnetic properties of these films have been determined using Rutherford Backscattering, X-ray diffraction and magnetization measurements. We find that the various properties are sensitive to the sputter background pressure in different ways. In particular, the lattice parameter changes in a continuous way, the coercive fields vary continuously with a maximum value of 3.3 T, but the saturation magnetization peaks when the lattice parameter is close to that of Sm2Co7. Moreover, we find that the Sm content of the films is higher than expected from the expected stoichiometry. △ Less

Submitted 8 October, 2012; originally announced October 2012.

Comments: 6 pages, 8 figures

Journal ref: J. Appl. Phys. 116, 053903 (2014)

Anisotropic magnetothermoelectric power of ferromagnetic thin films

Authors: M. S. Anwar, B. Lacoste, J. Aarts

Abstract: We compare the behavior of the magnetothermoelectric power (MTEP)in metallic ferromagnetic thin films of Ni80Fe20 (Permalloy; Py), Co and CrO2 at temperatures in the range of 100 K to 400 K. In 25 nm thick Py films and 50 nm thick Co films both the anisotropic magnetoresistance (AMR) and MTEP show a relative change in resistance and thermoelectric power (TEP) of the order of 0.2% when the magnetic… ▽ More We compare the behavior of the magnetothermoelectric power (MTEP)in metallic ferromagnetic thin films of Ni80Fe20 (Permalloy; Py), Co and CrO2 at temperatures in the range of 100 K to 400 K. In 25 nm thick Py films and 50 nm thick Co films both the anisotropic magnetoresistance (AMR) and MTEP show a relative change in resistance and thermoelectric power (TEP) of the order of 0.2% when the magnetic field is reversed, and in both cases there is no significant change in AMR or MTEP any more after the saturation field has been reached. Surprisingly, both Py and Co films have opposite MTEP behavior although both have the same sign for AMR and TEP. The data on 100 nm films of fully spin-polarized CrO2, grown both on TiO2 and on sapphire, show a different picture. The MTEP behavior at low fields shows peaks similar to the AMR in these films, with variations up to 1%. With increasing field both the MR and the MTEP variations keeps growing, with MTEP showing relative changes of 1.5% with the thermal gradient along the b-axis and even 20% with the gradient along the c-axis, with an intermediate value of 3% for the film on sapphire. It appears that the low-field effects are due to magnetic domain switching, while the high-field effects are intrinsic to the electronic structure of CrO2. △ Less

Submitted 15 June, 2017; v1 submitted 7 June, 2012; originally announced June 2012.

Comments: 6 pages, 7 figures

The role of stepped surfaces on the magnetotransport in strained thin films of La0.67Ca0.33MnO3

Authors: C. Beekman, J. Aarts

Abstract: We report a comparative study of the properties of very thin films of La0.67Ca0.33MnO3 grown epitaxially under strain on flat SrTiO3 (STO) and on 1 deg miscut STO. For the films on flat STO the transport properties show well-known behavior, namely values of the metal-insulator transition temperature which are strongly reduced with respect to the bulk value. The reduction in films on miscut STO is… ▽ More We report a comparative study of the properties of very thin films of La0.67Ca0.33MnO3 grown epitaxially under strain on flat SrTiO3 (STO) and on 1 deg miscut STO. For the films on flat STO the transport properties show well-known behavior, namely values of the metal-insulator transition temperature which are strongly reduced with respect to the bulk value. The reduction in films on miscut STO is significantly less strong than in films on flat STO, even though they appear similar as to strain state. Moreover, the residual resistance at low temperatures is lower than for the case of flat films. Magnetically, we find reduced values of the saturation magnetization with respect to the bulk value, indicating the presence of a dead layer in both cases. We argue that the higher density of the step edges on the miscut substrates lead to strain relaxation in the form of point defects and an increased electronic bandwidth, which actually make the electronic properties more robust. △ Less

Submitted 4 June, 2012; originally announced June 2012.

Comments: 12 pages,7 figures, 1 table. arXiv admin note: substantial text overlap with arXiv:1102.4004

Long range spin supercurrents in ferromagnetic CrO$_2$ using a multilayer contact structure

Authors: M. S. Anwar, M. Veldhorst, A. Brinkman, J. Aarts

Abstract: e report measurements of long ranged supercurrents through ferromagnetic and fully spin-polarized CrO$_2$ deposited on TiO$_2$ substrates. In earlier work, we found supercurrents in films grown on sapphire but not on TiO$_2$. Here we employed a special contact arrangement, consisting of a Ni/Cu sandwich between the film and the superconducting amorphous Mo$_{70}$Ge$_{30}$ electrodes. The distance… ▽ More e report measurements of long ranged supercurrents through ferromagnetic and fully spin-polarized CrO$_2$ deposited on TiO$_2$ substrates. In earlier work, we found supercurrents in films grown on sapphire but not on TiO$_2$. Here we employed a special contact arrangement, consisting of a Ni/Cu sandwich between the film and the superconducting amorphous Mo$_{70}$Ge$_{30}$ electrodes. The distance between the contacts was almost a micrometer, and we find the critical current density to be significantly higher than found in the films deposited on sapphire. We argue this is due to spin mixing in the Ni/Cu/CrO$_2$ layer structure, which is helpful in the generation of the odd-frequency spin triplet correlations needed to carry the supercurrent. △ Less

Submitted 24 November, 2011; originally announced November 2011.

Comments: 3 pages, 4 figures

Conductivity of LaAlO/SrTiO3 Interfaces made by Sputter Deposition

Authors: I. M. Dildar, D. B. Boltje, M. H. S. Hesselberth, Q. Xu, H. W. Zandbergen, S. Harkema

Abstract: We have investigated the properties of interfaces between LaAlO3 films grown on SrTiO3 substrates singly terminated by TiO2. We used RF sputtering in a high-pressure oxygen atmosphere. The films are smooth, with flat surfaces. Transmission Electron Microscopy shows atomically sharp and continuous interfaces while EELS measurements show some slight intermixing. The elemental ratio of La to Al measu… ▽ More We have investigated the properties of interfaces between LaAlO3 films grown on SrTiO3 substrates singly terminated by TiO2. We used RF sputtering in a high-pressure oxygen atmosphere. The films are smooth, with flat surfaces. Transmission Electron Microscopy shows atomically sharp and continuous interfaces while EELS measurements show some slight intermixing. The elemental ratio of La to Al measured by EDX is found to be 1.07. Importantly, we find these interfaces to be non-conducting, indicating that the sputtered interface is not electronically reconstructed in the way reported for films grown by Pulsed Laser Deposition because of the different interplay between stoichiometry, mixing and oxygen vacancies. △ Less

Submitted 21 November, 2011; originally announced November 2011.

Comments: 3 pages, 5 figures

Large electric field effects on the resistance of La$_{0.67}$Ca$_{0.33}$MnO$_3$ microstructures

Authors: C. Beekman, I. Komissarov, J. Aarts

Abstract: We investigate electric field effects in thin film microbridges of La$_{0.7}$Ca$_{0.3}$MnO$_3$ with the focus on the regime of metal-insulator transition. A mechanically milled SrTiO$_3$ substrate is used as a backgate dielectric. Inside the metal-insulator transition we find a strong unipolar field-induced reduction in resistance, as well as a suppression of the nonlinear features in the I-V curv… ▽ More We investigate electric field effects in thin film microbridges of La$_{0.7}$Ca$_{0.3}$MnO$_3$ with the focus on the regime of metal-insulator transition. A mechanically milled SrTiO$_3$ substrate is used as a backgate dielectric. Inside the metal-insulator transition we find a strong unipolar field-induced reduction in resistance, as well as a suppression of the nonlinear features in the I-V curves we observed earlier. We associate the observed effects with a phase separated state in which metallic regions coexist with short range correlated polaron regions. When the glassy polaron phase has fully developed, and closes off the microbridge, the field effects disappear leaving the strongly nonlinear behavior of the transport current unaltered. △ Less

Submitted 2 June, 2011; originally announced June 2011.

Comments: 3 pages, 5 figures

Manganese valence and magnetotransport in ultrathin films of La$_{0.67}$Ca$_{0.33}$MnO$_3$

Authors: C. Beekman, J. Aarts, M. Porcu, H. Zandbergen

Abstract: We report a comparative study of the properties of very thin films of La$_{0.67}$Ca$_{0.33}$MnO$_3$ grown epitaxially under strain on flat SrTiO$_3$ (STO), lattice matched on NdGaO$_3$ (NGO), and strained on $1^{\circ}$-miscut STO. We use transmission electron microscopy and electron energy loss spectroscopy to study the microstructure, composition, and Mn valence state. Near the interface we find… ▽ More We report a comparative study of the properties of very thin films of La$_{0.67}$Ca$_{0.33}$MnO$_3$ grown epitaxially under strain on flat SrTiO$_3$ (STO), lattice matched on NdGaO$_3$ (NGO), and strained on $1^{\circ}$-miscut STO. We use transmission electron microscopy and electron energy loss spectroscopy to study the microstructure, composition, and Mn valence state. Near the interface we find no significant segregation, but a charge compensation layer where the valence is enhanced over the nominal value of 3.3+, and a relaxation to this value over several nanometer. The transport properties show well-known behavior for the films on flat STO and NGO, namely values of the metal-insulator transition temperature which are strongly (STO) or only little (NGO) reduced with respect to the bulk value. The reduction in films on miscut STO however is less strong than in films on flat STO, even though they appear similar as to strain state and interface layer. Magnetically, we find reduced values of the saturation magnetization for the strained films with respect to the bulk value, which cannot only be ascribed to the interface layer. △ Less

Submitted 19 February, 2011; originally announced February 2011.

Comments: 8 pages, 11 figures

Mesoscopic transport in ultrathin films of La$_{0.67}$Ca$_{0.33}$MnO$_3$

Authors: C. Beekman, J. Zaanen, J. Aarts

Abstract: We investigate the electrical transport in mesoscopic structures of La$_{0.67}$Ca$_{0.33}$MnO$_3$ in the regime of the metal-insulator transition by fabricating microbridges from strained and unstrained thin films. We measure current-voltage characteristics as function of temperature and in high magnetic fields and with varying film thickness. For strained films, in warming from the metallic to th… ▽ More We investigate the electrical transport in mesoscopic structures of La$_{0.67}$Ca$_{0.33}$MnO$_3$ in the regime of the metal-insulator transition by fabricating microbridges from strained and unstrained thin films. We measure current-voltage characteristics as function of temperature and in high magnetic fields and with varying film thickness. For strained films, in warming from the metallic to the insulating state, we find non-linear effects in the steep part of the transition characterized by a differential resistance with a strong peak around zero applied current, and saturating at higher currents after resistance drops up to 60 %. We propose that this nonlinear behavior is associated with melting of the insulating state by injecting charge carriers, signalling the occurrence of an intervening phase which involves the formation of short range polaron correlations. △ Less

Submitted 7 September, 2010; originally announced September 2010.

Comments: 4 pages, 5 figures

Journal ref: Phys. Rev. B, 83, 235128 (2011)

Supercurrents through half-metallic ferromagnetic CrO$_2$ revisited

Authors: M. S. Anwar, M. Hesselberth, M. Porcu, J. Aarts

Abstract: We report on the observation of a supercurrent through the half metallic ferromagnet CrO$_2$ grown on hexagonal Al$_2$O$_3$ (sapphire). The current was observed to flow over a distance of 700 nm between two superconducting amorphous Mo$_{70}$Ge$_{30}$ electrodes which were deposited on the CrO$_2$ film. The critical current $I_c$ increases as function of decreasing temperature. Upon applying an in… ▽ More We report on the observation of a supercurrent through the half metallic ferromagnet CrO$_2$ grown on hexagonal Al$_2$O$_3$ (sapphire). The current was observed to flow over a distance of 700 nm between two superconducting amorphous Mo$_{70}$Ge$_{30}$ electrodes which were deposited on the CrO$_2$ film. The critical current $I_c$ increases as function of decreasing temperature. Upon applying an in-plane magnetic field, $I_c$ goes through a maximum at the rather high field of 80 mT. We believe this to be a long range proximity effect in the ferromagnet, carried by odd-frequency pairing correlations. △ Less

Submitted 23 March, 2010; originally announced March 2010.

Comments: 4 pages, 5 figures

In search for the superconducting spin-switch: Magnetization induced resistance switching effects in La$_{0.67}$Sr$_{0.33}$MnO$_3$/YBa$_2$Cu$_3$O$_{7-δ}$ bi- and trilayers

Authors: M. van Zalk, M. Veldhorst, A. Brinkman, J. Aarts, H. Hilgenkamp

Abstract: We have studied the influence of the magnetization on the superconducting transition temperature ($T_c$) in bi- and trilayers consisting of the half-metallic ferromagnet La$_{0.67}$Sr$_{0.33}$MnO$_3$ (LSMO) and the high-temperature superconductor YBa$_2$Cu$_3$O$_{7-δ}$ (YBCO). We have made use of tilted epitaxial growth in order to achieve contacts between the two materials that are partly in th… ▽ More We have studied the influence of the magnetization on the superconducting transition temperature ($T_c$) in bi- and trilayers consisting of the half-metallic ferromagnet La$_{0.67}$Sr$_{0.33}$MnO$_3$ (LSMO) and the high-temperature superconductor YBa$_2$Cu$_3$O$_{7-δ}$ (YBCO). We have made use of tilted epitaxial growth in order to achieve contacts between the two materials that are partly in the crystallographic $ab$-plane of the YBCO. As a result of uniaxial magnetic anisotropy in the tilted structures, we observe sharp magnetization switching behavior. At temperatures close to $T_c$, the magnetization switching induces resistance jumps in trilayers, resulting in a magnetization dependence of $T_c$. In bilayers, this switching effect can be observed as well, provided that the interface to the ferromagnetic layer is considerably rough. Our results indicate that the switching behavior arises from magnetic stray fields from the ferromagnetic layers that penetrate into the superconductor. A simple model describes the observed behavior well. We find no evidence that the switching behavior is caused by a so-called superconducting spin-switch, nor by accumulation of spin-polarized electrons. Observation of magnetic coupling of the ferromagnetic layers, through the superconductor, supports the idea of field induced resistance switching. △ Less

Submitted 17 March, 2009; originally announced March 2009.

Comments: 11 pages, 12 figures

Journal ref: Phys. Rev. B, 79, 134509 (2009)

Correlations between the morphology and the electronic structure at the surface of thin film manganites, investigated with STM

Authors: S. Kelly, F. Galli, I. Komissarov, J. Aarts

Abstract: Thin-film colossal magnetoresistance manganites such as La$_{0.67}$Ca$_{0.33}$MnO$_{3}$ (LCMO) have now been intensely studied for more than a decade, but the issue of possible nanoscale electronic phase separation is not fully solved. Scanning Tunneling Microscopy / Spectroscopy (STS) has been pivotal in studying phase separation, but is hindered by being surface- rather than bulk-sensitive. Fo… ▽ More Thin-film colossal magnetoresistance manganites such as La$_{0.67}$Ca$_{0.33}$MnO$_{3}$ (LCMO) have now been intensely studied for more than a decade, but the issue of possible nanoscale electronic phase separation is not fully solved. Scanning Tunneling Microscopy / Spectroscopy (STS) has been pivotal in studying phase separation, but is hindered by being surface- rather than bulk-sensitive. For our sputtered LCMO films the data indicates a strong correlation between surface morphology and signatures of phase separation; rough films show phase separation while atomically flat films are electronically homogeneous but have a more or less inactive surface layer. Regardless of surface morphology, the film bulk is electronically and magnetically active. Many of the reported conclusions about electronic inhomogeneities measured by STS have been confused by this issue. We study both strained and unstrained films and find no correlation between substrate-induced strain and either electronic phase separation or dead layers. △ Less

Submitted 4 February, 2009; originally announced February 2009.

Transport properties of microstructured ultrathin films of La0.67Ca0.33MnO3 on SrTiO3

Authors: C. Beekman, I. Komissarov, M. Hesselberth, J. Aarts

Abstract: We have investigated the electrical transport properties of 8 nm thick La0.67Ca0.33MnO3 films, sputter-deposited on SrTiO3 (STO), and etched into 5 micrometer-wide bridges by Ar-ion etching. We find that even slight overetching of the film leads to conductance of the STO substrate, and asymmetric and non-linear current-voltage (I-V) characteristics. However, a brief oxygen plasma etch allows ful… ▽ More We have investigated the electrical transport properties of 8 nm thick La0.67Ca0.33MnO3 films, sputter-deposited on SrTiO3 (STO), and etched into 5 micrometer-wide bridges by Ar-ion etching. We find that even slight overetching of the film leads to conductance of the STO substrate, and asymmetric and non-linear current-voltage (I-V) characteristics. However, a brief oxygen plasma etch allows full recovery of the insulating character of the substrate. The I-V characteristics of the bridges are then fully linear over a large range of current densities. We find colossal magnetoresistance properties typical for strained LCMO on STO but no signature of non-linear effects (so-called electroresistance) connected to electronic inhomogeneites. In the metallic state below 150 K, the highest current densities lead to heating effects and non-linear I-V characteristics. △ Less

Submitted 14 May, 2007; originally announced May 2007.

Comments: 3 pages, 5 figures

Spin dynamics in a superconductor / ferromagnet proximity system

Authors: C. Bell, S. Milikisyants, M. Huber, J. Aarts

Abstract: The ferromagnetic resonance of thin sputtered Ni80Fe20 films grown on Nb is measured. By varying the temperature and thickness of the Nb the role of the superconductivity on the whole ferromagnetic layer in these heterostructures is explored. The change in the spin transport properties below the superconducting transition of the Nb is found to manifest itself in the Ni80Fe20 layer by a sharpenin… ▽ More The ferromagnetic resonance of thin sputtered Ni80Fe20 films grown on Nb is measured. By varying the temperature and thickness of the Nb the role of the superconductivity on the whole ferromagnetic layer in these heterostructures is explored. The change in the spin transport properties below the superconducting transition of the Nb is found to manifest itself in the Ni80Fe20 layer by a sharpening in the resonance of the ferromagnet, or a decrease in the effective Gilbert damping co-efficient. This dynamic proximity effect is in contrast to low frequency studies in these systems, where the effect of the superconductor is confined to a small region in the ferromagnet. We interpret this in terms of the spin pumping model. △ Less

Submitted 20 February, 2007; originally announced February 2007.

Comments: 4 pages, 4 figures, to be submitted for publication

Vortex relaxation and coupling in superconducting heterostructures studied by STM

Authors: G. J. C. van Baarle, F. Galli, P. H. Kes, J. Aarts

Abstract: In a sandwich consisting of two superconducting films, one weakly pinning and one strongly pinning, the vortex positions in both films are determined by the strongly pinning material and the vortex lattice is disordered in both films. We used (strongly pinning) NbN and (weakly pinning) MoGe and studied, by directly imaging the vortex core positions with a scanning tunnelling microscope, how this… ▽ More In a sandwich consisting of two superconducting films, one weakly pinning and one strongly pinning, the vortex positions in both films are determined by the strongly pinning material and the vortex lattice is disordered in both films. We used (strongly pinning) NbN and (weakly pinning) MoGe and studied, by directly imaging the vortex core positions with a scanning tunnelling microscope, how this disorder is restored with increasing thickness of MoGe layer or when the interface is made insulating. For clean interfaces we find that the first reordering of the vortex lattice is found at a layer thickness wich is compatible with the first bending mode of the vortex lines. Making the interface insulating we find that order is restored quickly. We argue that this is can be understood from the competition between the Josephson force working on the vortex segments on the one hand, and the elastic restoring forces inside the weakly pinning layer on the other hand. △ Less

Submitted 5 February, 2007; originally announced February 2007.

Comments: 7 pages, 9 figures