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Probing spatially resolved spin density correlations with trapped excitons
Authors:
Shanshan Ding,
Jose Antonio Valerrama Botia,
Aleksi Julku,
Zhigang Wu,
G. M. Bruun
Abstract:
The rapidly growing class of atomically thin and tunable van der Waals materials is intensely investigated both in the context of fundamental science and for new technologies. There is in this connection a widespread need for new ways to probe the electronic properties of these layered materials, since their two-dimensional (2D) character make conventional probes less efficient. Here, we show how…
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The rapidly growing class of atomically thin and tunable van der Waals materials is intensely investigated both in the context of fundamental science and for new technologies. There is in this connection a widespread need for new ways to probe the electronic properties of these layered materials, since their two-dimensional (2D) character make conventional probes less efficient. Here, we show how excitons trapped in a moiré lattice can be used as an optical probe for spatially resolved electron spin density correlations in such materials. The electrons in the material of interest virtually tunnel to the moiré lattice where they scatter on the excitons after which they tunnel back. This gives rise to an effective spin-dependent and spatially localised potential felt by the electrons, which in turn leads to energy shifts that can be measured spectroscopically in the exciton spectrum. Using second order perturbation theory combined with a solution to the exciton-electron scattering problem, we show that the electrons mediate an interaction between two excitons resulting in an energy shift proportional to their two-point spin density-density correlation function evaluated at the exciton positions. We then discuss two specific applications of our setup. First, we show that quantum phase transitions between different in-plane anti-ferromagnetic orders in a 2D lattice give rise to large and measurable shifts in the exciton spectrum in the critical regions. Second, we analyse how different pairing symmetries of superconducting phases can be probed. This demonstrates that our scheme opens up new ways to probe electron spin density correlations, which is a key property of many quantum phases predicted to exist in the new 2D materials.
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Submitted 16 December, 2025;
originally announced December 2025.
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Exciton interacting with a moiré lattice: Polarons, strings, and optical probing of spin correlations
Authors:
Aleksi Julku,
Shanshan Ding,
Georg M. Bruun
Abstract:
We develop a general theory for how an exciton in an atomically thin transition metal dichacogenide (TMD) monolayer couples to spin and charge correlations in an adjacent moire lattice created by a TMD bi-layer. Virtual tunneling of charge carriers, assumed for concreteness to be holes, between the moire lattice and the monolayer combined with the presence of bound hole-exciton states, i.e. trions…
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We develop a general theory for how an exciton in an atomically thin transition metal dichacogenide (TMD) monolayer couples to spin and charge correlations in an adjacent moire lattice created by a TMD bi-layer. Virtual tunneling of charge carriers, assumed for concreteness to be holes, between the moire lattice and the monolayer combined with the presence of bound hole-exciton states, i.e. trions, give rise to an effective interaction between the moire holes and the exciton. In addition to the Umklapp scattering, we show that this interaction is spin-dependent and therefore couples the exciton to the spin correlations of the moire holes, which may be in- as well as out-of-plane. We then use our theory to examine two specific examples where the moire holes form in-plane ferromagnetic or anti-ferromagnetic order. In both cases, the exciton creates spin waves in the moire lattice, which we analyse by using a self-consistent Born approximation that includes such processes to infinite order. We show that the competition between magnetic order and exciton motion leads to the formation of a well-defined quasiparticle consisting of the exciton surrounded by a cloud of magnetic frustration in the moire lattice sites below. For the anti-ferromagnet, we furthermore demonstrate the presence of the elusive geometric string excitations and discuss how they can be observed via their smoking gun energy dependence on the spin-spin coupling, which can be tuned by varying the twist angle of the moire bi-layer. All these phenomena have clear signatures in the exciton spectrum, and as such our results illustrate that excitons are promising probes providing optical access to the spin correlations of new quantum phases predicted to exist in TMD materials.
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Submitted 2 August, 2024; v1 submitted 6 November, 2023;
originally announced November 2023.
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Polarons and bipolarons in a two-dimensional square lattice
Authors:
Shanshan Ding,
G. A. Domínguez-Castro,
Aleksi Julku,
Arturo Camacho-Guardian,
Georg M. Bruun
Abstract:
Quasiparticles and their interactions are a key part of our understanding of quantum many-body systems. Quantum simulation experiments with cold atoms have in recent years advanced our understanding of isolated quasiparticles, but so far they have provided limited information regarding their interactions and possible bound states. Here, we show how exploring mobile impurities immersed in a Bose-Ei…
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Quasiparticles and their interactions are a key part of our understanding of quantum many-body systems. Quantum simulation experiments with cold atoms have in recent years advanced our understanding of isolated quasiparticles, but so far they have provided limited information regarding their interactions and possible bound states. Here, we show how exploring mobile impurities immersed in a Bose-Einstein condensate (BEC) in a two-dimensional lattice can address this problem. First, the spectral properties of individual impurities are examined, and in addition to the attractive and repulsive polarons known from continuum gases, we identify a new kind of quasiparticle stable for repulsive boson-impurity interactions. The spatial properties of polarons are calculated showing that there is an increased density of bosons at the site of the impurity both for repulsive and attractive interactions. We then derive an effective Schrödinger equation describing two polarons interacting via the exchange of density oscillations in the BEC, which takes into account strong impurity-boson two-body correlations. Using this, we show that the attractive nature of the effective interaction between two polarons combined with the two-dimensionality of the lattice leads to the formation of bound states -- i.e. bipolarons. The wave functions of the bipolarons are examined showing that the ground state is symmetric under particle exchange and therefore relevant for bosonic impurities, whereas the first excited state is doubly degenerate and odd under particle exchange making it relevant for fermionic impurities. Our results show that quantum gas microscopy in optical lattices is a promising platform to explore the spatial properties of polarons as well as to finally observe the elusive bipolarons.
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Submitted 21 January, 2023; v1 submitted 1 December, 2022;
originally announced December 2022.
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Supefluidity of flat band Bose-Einstein condensates revisited
Authors:
Aleksi Julku,
Grazia Salerno,
Päivi Törmä
Abstract:
We consider the superfluid weight, speed of sound and excitation fraction of a flat band Bose-Einstein condensate (BEC) within multiband Bogoliubov theory. The superfluid weight is calculated by introducing a phase winding and minimizing the free energy with respect to it. We find that the superfluid weight has a contribution arising from the change of the condensate density and chemical potential…
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We consider the superfluid weight, speed of sound and excitation fraction of a flat band Bose-Einstein condensate (BEC) within multiband Bogoliubov theory. The superfluid weight is calculated by introducing a phase winding and minimizing the free energy with respect to it. We find that the superfluid weight has a contribution arising from the change of the condensate density and chemical potential upon the phase twist that has been neglected in the previous literature. We also point out that the speed of sound and the excitation fraction are proportional to orbital-position-independent generalizations of the quantum metric and the quantum distance, and reduce to the usual quantum metric (Fubini-Study metric) and the Hilbert-Schmidt quantum distance only in special cases. We derive a second order perturbation correction to the dependence of the speed of sound on the generalized quantum metric, and show that it compares well with numerical calculations. Our results provide a consistent connection between flat band BEC and quantum geometry, with physical observables being independent of the orbital positions as they should, and complete formulas for the evaluation of the superfluid weight within the Bogoliubov theory. We discuss the limitations of the Bogoliubov theory in evaluating the superfluid weight.
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Submitted 10 April, 2023; v1 submitted 21 October, 2022;
originally announced October 2022.
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Non-local interactions and supersolidity of moiré excitons
Authors:
Aleksi Julku
Abstract:
Heterobilayer transition metal dichalcogenide (TMDC) moiré systems provide an ideal framework to investigate strongly correlated physics. Here we theoretically study bosonic many-body phases of excitons in moiré TMDCs. By using two moiré models and cluster mean-field theory, we reveal that, due to non-local Coulomb interactions, moiré excitons can feature exotic supersolid phases, i.e. superfluids…
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Heterobilayer transition metal dichalcogenide (TMDC) moiré systems provide an ideal framework to investigate strongly correlated physics. Here we theoretically study bosonic many-body phases of excitons in moiré TMDCs. By using two moiré models and cluster mean-field theory, we reveal that, due to non-local Coulomb interactions, moiré excitons can feature exotic supersolid phases, i.e. superfluids of broken translational invariance, and correlated insulating states. The correlated phases exist at experimentally accessible temperatures and are tunable via the twist angle and exciton density.
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Submitted 1 July, 2022; v1 submitted 3 May, 2022;
originally announced May 2022.
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Light-induced topological superconductivity in transition metal dichalcogenide monolayers
Authors:
Aleksi Julku,
Jami J. Kinnunen,
Arturo Camacho-Guardian,
Georg M. Bruun
Abstract:
Monolayer transition metal dichalcogenides (TMDs) host deeply bound excitons interacting with itinerant electrons, and as such they represent an exciting new quantum many-body Bose-Fermi mixture. Here, we demonstrate that electrons interacting with a Bose-Einstein condensate (BEC) of exciton-polaritons can realise a two-dimensional topological $p_x+ip_y$ superconductor. Using strong coupling Elias…
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Monolayer transition metal dichalcogenides (TMDs) host deeply bound excitons interacting with itinerant electrons, and as such they represent an exciting new quantum many-body Bose-Fermi mixture. Here, we demonstrate that electrons interacting with a Bose-Einstein condensate (BEC) of exciton-polaritons can realise a two-dimensional topological $p_x+ip_y$ superconductor. Using strong coupling Eliashberg theory, we show that this is caused by an attractive interaction mediated by the BEC, which overcompensates the repulsive Coulomb interaction between the electrons. The hybrid light-matter nature of the BEC is crucial for achieving this, since it can be used to reduce retardation effects and increase the mediated interaction in regimes important for pairing. We finally show how the great flexibility of TMDs allows one to tune the critical temperature of the topological superconducting phase to be within experimental reach.
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Submitted 21 October, 2022; v1 submitted 26 April, 2022;
originally announced April 2022.
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Quantum geometry and flat band Bose-Einstein condensation
Authors:
Aleksi Julku,
Georg M. Bruun,
Päivi Törmä
Abstract:
We study the properties of a weakly interacting Bose-Einstein condensate (BEC) in a flat band lattice system by using multiband Bogoliubov theory, and discover fundamental connections to the underlying quantum geometry. In a flat band, the speed of sound and the quantum depletion of the condensate are dictated by the quantum geometry, and a finite quantum distance between the condensed and other s…
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We study the properties of a weakly interacting Bose-Einstein condensate (BEC) in a flat band lattice system by using multiband Bogoliubov theory, and discover fundamental connections to the underlying quantum geometry. In a flat band, the speed of sound and the quantum depletion of the condensate are dictated by the quantum geometry, and a finite quantum distance between the condensed and other states guarantees stability of the BEC. Our results reveal that a suitable quantum geometry allows one to reach the strong quantum correlation regime even with weak interactions.
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Submitted 1 October, 2021; v1 submitted 29 April, 2021;
originally announced April 2021.
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Nonlinear optical response of resonantly driven polaron-polaritons
Authors:
Aleksi Julku,
Miguel. A. Bastarrachea-Magnani,
Arturo Camacho-Guardian,
Georg M. Bruun
Abstract:
Exciton polaritons in two-dimensional semiconductors inside microcavities are powerful platforms to explore hybrid light-matter quantum systems. Here, we study a macroscopic coherent population of the lowest energy state of polaron-polaritons, which are quasiparticles formed by the dressing of exciton polaritons by particle-hole excitations in a surrounding electron gas. Using a non-perturbative m…
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Exciton polaritons in two-dimensional semiconductors inside microcavities are powerful platforms to explore hybrid light-matter quantum systems. Here, we study a macroscopic coherent population of the lowest energy state of polaron-polaritons, which are quasiparticles formed by the dressing of exciton polaritons by particle-hole excitations in a surrounding electron gas. Using a non-perturbative many-body theory to describe exciton-electron correlations combined with a non-equilibrium theory for the macroscopically populated state, we show that the electrons strongly affect the collective properties of the polaron-polaritons. This stems from the dependence of the polaron-polariton energy and the interaction between them on the electron density, which leads to strong nonlinearities. We identify stable and unstable regimes of the polaron-polaritons by calculating its excitation spectrum, and show that they result in prominent hysteresis effects when the electron density is varied. Our results should be readily observable using present experimental technology.
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Submitted 1 October, 2021; v1 submitted 30 March, 2021;
originally announced March 2021.
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Superfluid weight and Berezinskii-Kosterlitz-Thouless transition temperature of twisted bilayer graphene
Authors:
Aleksi Julku,
Teemu J. Peltonen,
Long Liang,
Tero T. Heikkilä,
Päivi Törmä
Abstract:
We study superconductivity of twisted bilayer graphene with local and non-local attractive interactions. We obtain the superfluid weight and Berezinskii-Kosterlitz-Thouless (BKT) transition temperature for microscopic tight-binding and low-energy continuum models. We predict qualitative differences between local and non-local interaction schemes which could be distinguished experimentally. In the…
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We study superconductivity of twisted bilayer graphene with local and non-local attractive interactions. We obtain the superfluid weight and Berezinskii-Kosterlitz-Thouless (BKT) transition temperature for microscopic tight-binding and low-energy continuum models. We predict qualitative differences between local and non-local interaction schemes which could be distinguished experimentally. In the flat band limit where the pair potential exceeds the band width we show that the superfluid weight and BKT temperature are determined by multiband processes and quantum geometry of the band.
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Submitted 27 August, 2019; v1 submitted 14 June, 2019;
originally announced June 2019.
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Superfluid weight and Berezinskii-Kosterlitz-Thouless temperature of spin-imbalanced and spin-orbit-coupled Fulde-Ferrell phases in lattice systems
Authors:
Aleksi Julku,
Long Liang,
Päivi Törmä
Abstract:
We study the superfluid weight $D^s$ and Berezinskii-Kosterlitz-Thouless (BKT) transition temperatures $T_{BKT}$ in case of exotic Fulde-Ferrell (FF) superfluid states in lattice systems. We consider spin-imbalanced systems with and without spin-orbit coupling (SOC) accompanied with in-plane Zeeman field. By applying mean-field theory, we derive general equations for $D^s$ and $T_{BKT}$ in the pre…
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We study the superfluid weight $D^s$ and Berezinskii-Kosterlitz-Thouless (BKT) transition temperatures $T_{BKT}$ in case of exotic Fulde-Ferrell (FF) superfluid states in lattice systems. We consider spin-imbalanced systems with and without spin-orbit coupling (SOC) accompanied with in-plane Zeeman field. By applying mean-field theory, we derive general equations for $D^s$ and $T_{BKT}$ in the presence of SOC and the Zeeman fields for 2D Fermi-Hubbard lattice models, and apply our results to a 2D square lattice. We show that conventional spin-imbalanced FF states without SOC can be observed at finite temperatures and that FF phases are further stabilized against thermal fluctuations by introducing SOC. We also propose how topologically non-trivial SOC-induced FF phases could be identified experimentally by studying the total density profiles. Furthermore, the relative behavior of transverse and longitudinal superfluid weight components and the role of the geometric superfluid contribution are discussed.
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Submitted 20 August, 2018; v1 submitted 30 April, 2018;
originally announced April 2018.
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Bose-Einstein Condensation in a Plasmonic Lattice
Authors:
Tommi K. Hakala,
Antti J. Moilanen,
Aaro I. Väkeväinen,
Rui Guo,
Jani-Petri Martikainen,
Konstantinos S. Daskalakis,
Heikki T. Rekola,
Aleksi Julku,
Päivi Törmä
Abstract:
Bose-Einstein condensation is a remarkable manifestation of quantum statistics and macroscopic quantum coherence. Superconductivity and superfluidity have their origin in Bose-Einstein condensation. Ultracold quantum gases have provided condensates close to the original ideas of Bose and Einstein, while condensation of polaritons and magnons have introduced novel concepts of non-equilibrium conden…
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Bose-Einstein condensation is a remarkable manifestation of quantum statistics and macroscopic quantum coherence. Superconductivity and superfluidity have their origin in Bose-Einstein condensation. Ultracold quantum gases have provided condensates close to the original ideas of Bose and Einstein, while condensation of polaritons and magnons have introduced novel concepts of non-equilibrium condensation. Here, we demonstrate a Bose-Einstein condensate (BEC) of surface plasmon polaritons in lattice modes of a metal nanoparticle array. Interaction of the nanoscale-confined surface plasmons with a room-temperature bath of dye molecules enables thermalization and condensation in picoseconds. The ultrafast thermalization and condensation dynamics are revealed by an experiment that exploits thermalization under propagation and the open cavity character of the system. A crossover from BEC to usual lasing is realized by tailoring the band structure. This new condensate of surface plasmon lattice excitations has promise for future technologies due to its ultrafast, room-temperature and on-chip nature.
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Submitted 16 November, 2018; v1 submitted 5 June, 2017;
originally announced June 2017.
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Geometric origin of superfluidity in the Lieb lattice flat band
Authors:
Aleksi Julku,
Sebastiano Peotta,
Tuomas Vanhala,
Dong-Hee Kim,
Päivi Törmä
Abstract:
The ground state and transport properties of the Lieb lattice flat band in the presence of an attractive Hubbard interaction are considered. It is shown that the superfluid weight can be large even for an isolated and strictly flat band. Moreover the superfluid weight is proportional to the interaction strength and to the quantum metric, a band structure invariant obtained from the flat-band Bloch…
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The ground state and transport properties of the Lieb lattice flat band in the presence of an attractive Hubbard interaction are considered. It is shown that the superfluid weight can be large even for an isolated and strictly flat band. Moreover the superfluid weight is proportional to the interaction strength and to the quantum metric, a band structure invariant obtained from the flat-band Bloch functions. These predictions are amenable to verification with ultracold gases and may explain the anomalous behaviour of the superfluid weight of high-Tc superconductors.
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Submitted 8 May, 2016; v1 submitted 10 March, 2016;
originally announced March 2016.