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Mobile Exceptional Points Generate Momentum-Space Switching Domains
Authors:
Jung-Wan Ryu,
Chang-Hwan Yi
Abstract:
Exceptional points (EPs), non-Hermitian degeneracies where both eigenvalues and eigenvectors coalesce, play a central role in the topology of non-Hermitian spectra. Recent advances have enabled the controlled creation and manipulation of EPs in a wide range of physical systems, raising the question of what new band topology emerges when EPs become mobile under cyclic modulation. Here we show that…
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Exceptional points (EPs), non-Hermitian degeneracies where both eigenvalues and eigenvectors coalesce, play a central role in the topology of non-Hermitian spectra. Recent advances have enabled the controlled creation and manipulation of EPs in a wide range of physical systems, raising the question of what new band topology emerges when EPs become mobile under cyclic modulation. Here we show that mobile EPs generate momentum-space switching domains that partition the Brillouin zone into regions with distinct band-switching behavior. Using a minimal two-band lattice model, we introduce a band-permutation invariant that determines whether eigenmodes exchange after one modulation cycle. The boundaries between switching regions arise from the projection of EP trajectories in an extended parameter space combining crystal momentum and the modulation parameter. As the modulation strength increases, the switching domains expand and eventually cover the entire Brillouin zone, resulting in global band switching. The predicted switching-domain structure is further demonstrated in a photonic crystal with lossy materials. These results open a new avenue within non-Hermitian topology by enabling the engineering of EP-driven phenomena through their controlled motion.
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Submitted 30 April, 2026;
originally announced April 2026.
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When Blinking Helps: Suppressed Biexciton Emission in Lead Halide Perovskite Quantum Dots
Authors:
Adam Olejniczak,
Jehyeok Ryu,
Francesco Di Stasio,
Yury Rakovich,
Victor Krivenkov
Abstract:
Blinking and multiphoton emission in metal halide perovskite quantum dots (PQDs) limit their use as single-photon quantum emitters. Conventional models distinguish between trion-related A-type blinking and defect-assisted BC-type blinking, both expected to degrade single-photon purity in a dark state. Here, time-resolved spectroscopy on individual PQDs reveals a qualitatively different regime in w…
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Blinking and multiphoton emission in metal halide perovskite quantum dots (PQDs) limit their use as single-photon quantum emitters. Conventional models distinguish between trion-related A-type blinking and defect-assisted BC-type blinking, both expected to degrade single-photon purity in a dark state. Here, time-resolved spectroscopy on individual PQDs reveals a qualitatively different regime in which low emitting dark states exhibit higher single-photon purity than bright states. For those PQDs state-resolved $g^{(2)}(τ)$ analysis shows that the exciton photoluminescence quantum yield decreases by a factor of $\sim 8$, while the biexciton one is suppressed by a factor of $\sim 10$. This leads to a moderate improvement of single-photon purity with $g^{(2)}_0$ decreased from 0.155 to 0.120. In contrast, PQDs with fluorescence lifetime--intensity distribution patterns characteristic for A-type blinking, display the expected increase of $g^{(2)}_0$ in charged, trion-dominated states. To explain the observed improvement of single-photon purity of low-emitting dark states, we propose a self-trapped-exciton (STE) mechanism that selectively blocks biexciton formation by diverting hot excitons into long-lived, weakly emissive STE configurations. This STE-mediated blinking channel explains why certain low-emitting states improve, rather than degrade, single-photon purity and suggests a lattice-driven route to perovskite quantum emitters with intrinsically suppressed multiphoton events.
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Submitted 11 February, 2026;
originally announced February 2026.
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Biorthogonal scattering and generalized unitarity in non-Hermitian systems
Authors:
Jung-Wan Ryu,
Henning Schomerus,
Hee Chul Park
Abstract:
We investigate the two-port scattering process in non-Hermitian dimer models via quantum measurements using external leads. We focus on two exemplary dimer models that preserve parity-time symmetry via spatial gain-loss balance and exhibit non-reciprocity due to directional hopping. The scattering matrix is constructed using the biorthogonality of the left and right scattering states of the Hamilt…
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We investigate the two-port scattering process in non-Hermitian dimer models via quantum measurements using external leads. We focus on two exemplary dimer models that preserve parity-time symmetry via spatial gain-loss balance and exhibit non-reciprocity due to directional hopping. The scattering matrix is constructed using the biorthogonality of the left and right scattering states of the Hamiltonian, allowing us to calculate the reflection and transmission probabilities. Our analysis compares the reflection and transmission coefficients derived from the left, right, and combined scattering states, revealing that, unlike in Hermitian systems, the non-Hermitian scattering process does not adhere to unitarity when considering only the right scattering states. Furthermore, non-Hermitian scattering can enhance the reflection and transmission probabilities, with distinct physical contributions arising independently from complex eigenvalues and the non-orthogonality of eigenstates. Our results clarify how biorthogonality restores generalized unitarity and identify distinct physical origins of enhanced transport in PT-symmetric and non-reciprocal dimers, providing new insights into quantum transport in non-Hermitian systems.
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Submitted 5 February, 2026;
originally announced February 2026.
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Size-dependent Dielectric Permittivity of Perovskite Nanocrystals
Authors:
Jehyeok Ryu,
Victor Krivenkov,
Vitaly Goryashko,
Yury Rakovich,
Alexey Y. Nikitin
Abstract:
Perovskite nanocrystals (PNCs) are promising building blocks for quantum photonic devices. Optical properties of PNCs can be enhanced by integration with optical cavities or nanoantennas. Designing such structures requires accurate size dependent dielectric permittivity of PNCs. However, current reports provide primarily ensemble averaged values with limited access to the intrinsic response of ind…
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Perovskite nanocrystals (PNCs) are promising building blocks for quantum photonic devices. Optical properties of PNCs can be enhanced by integration with optical cavities or nanoantennas. Designing such structures requires accurate size dependent dielectric permittivity of PNCs. However, current reports provide primarily ensemble averaged values with limited access to the intrinsic response of individual PNCs. Here we suggest a methodology to reconstruct the size dependent complex dielectric permittivity of CsPbBr3 PNCs from the measured absorbance spectrum of colloidal solution. The permittivity of PNCs is modeled as a sum of Voigt profile oscillators, with the size dependent transition energies governed by the exciton effective mass. Using a transmission electron microscopy derived size distribution of the PNCs, the solution permittivity is obtained via Maxwell Garnett effective medium approximation. This permittivity is used in a transfer matrix method to simulate and fit the absorbance spectrum, from which the permittivity of PNCs is reconstructed. The extracted spectral linewidth from the imaginary part of the permittivity (78.4 meV) is consistent with single nanocrystal emission linewidths at room temperature. Finite element simulations show enhanced absorption cross section of a single PNC coupled to a nanoantenna, demonstrating applicability of the extracted permittivity. More generally, these findings provide a route to extract intrinsic permittivity of individual nanocrystals from absorbance measurements of their ensembles.
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Submitted 22 January, 2026;
originally announced January 2026.
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Perovskite Nanocrystals as Emerging Single-Photon Emitters: Progress, Challenges, and Opportunities
Authors:
Jehyeok Ryu,
Victor Krivenkov,
Adam Olejniczak,
Alexey Y. Nikitin,
Yury Rakovich
Abstract:
Metal-halide perovskite nanocrystals (PNCs) have emerged as leading candidates for next-generation quantum emitters, offering a unique combination of high photoluminescence quantum yield, tunable emission, short radiative lifetimes, and record-high single-photon purity under ambient conditions. These properties, together with low-cost and scalable solution-phase fabrication, position PNCs as attra…
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Metal-halide perovskite nanocrystals (PNCs) have emerged as leading candidates for next-generation quantum emitters, offering a unique combination of high photoluminescence quantum yield, tunable emission, short radiative lifetimes, and record-high single-photon purity under ambient conditions. These properties, together with low-cost and scalable solution-phase fabrication, position PNCs as attractive alternatives to traditional epitaxial and colloidal quantum dots. In this Review, we outline the physical parameters that define quantum emission in PNCs, compare their performance to other established and emerging quantum emitters, and assess the key figures of merit, including photostability, single-photon purity, and photon indistinguishability, required for practical quantum applications. We discuss underlying mechanisms affecting PNC emission behavior and highlight recent advances in improving their quantum emitting properties through synthetic and photonic engineering approaches. While challenges related to environmental stability and photon indistinguishability remain, emerging strategies, such as surface passivation, metal ion doping, and coupling with electromagnetic nano- and micro-cavities, are steadily closing the gap between PNCs and ideal quantum light sources.
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Submitted 14 November, 2025;
originally announced November 2025.
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Amplified Photocurrent in Heterojunctions comprising Nano-rippled Zinc Oxide and Perovskite-inspired Cs3Cu2I5
Authors:
Si Hyeok Yang,
Lim Kyung Oh,
Na Young Lee,
Dong Ho Lee,
Sang Min Choi,
Bowon Oh,
Yun Ji Park,
Yunji Cho,
Jaesel Ryu,
Hongki Kim,
Sang-Hyun Chin,
Yeonjin Yi,
Myungkwan Song,
Han Seul Kim,
Jin Woo Choi
Abstract:
Molecular zero-dimensional (0D) halide perovskite-inspired cesium copper iodide (Cs3Cu2I5) is a highly promising candidate for optoelectronic applications due to their low toxicity, high stability, and intense blue emission. However, their intrinsically poor electrical conductivity, stemming from isolated conductive copper iodide tetrahedra by cesium atoms, severely limits charge transport which p…
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Molecular zero-dimensional (0D) halide perovskite-inspired cesium copper iodide (Cs3Cu2I5) is a highly promising candidate for optoelectronic applications due to their low toxicity, high stability, and intense blue emission. However, their intrinsically poor electrical conductivity, stemming from isolated conductive copper iodide tetrahedra by cesium atoms, severely limits charge transport which poses a critical challenge for optoelectronic applications. In this study, we propose a novel strategy to overcome this limitation by utilizing precisely optimized zinc oxide nanoripple structures within a lateral Cs3Cu2I5 photodetector (PD) architecture featuring interdigitated electrodes (IDEs). The ZnO nanoripple was systematically tuned to improve the percolation paths, providing efficient routes for photogenerated carriers to migrate to the IDEs. Consequently, the optimized heterojunctions comprising Cs3Cu2I5 and ZnO exhibited superior photocurrent compared to the pristine Cs3Cu2I5 counterparts. This nanostructure-mediated charge transport engineering strategy for lateral structured PDs offers a new pathway for utilizing low-conductivity 0D materials for conventional optoelectronics, next-generation Internet of Things sensor networks, and plausibly biosensing applications.
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Submitted 27 October, 2025;
originally announced October 2025.
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Operational Quasiprobability in Quantum Thermodynamics: Work Extraction by Coherence and Non-joint Measurability
Authors:
Jeongwoo Jae,
Junghee Ryu,
Hoon Ryu
Abstract:
We employ the operational quasiprobability (OQ) as a work distribution, which reproduces the Jarzynski equality and yields the average work consistent with the classical definition. The OQ distribution can be experimentally implemented through the end-point measurement and the two-point measurement scheme. Using this framework, we demonstrate the explicit contribution of coherence to the fluctuati…
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We employ the operational quasiprobability (OQ) as a work distribution, which reproduces the Jarzynski equality and yields the average work consistent with the classical definition. The OQ distribution can be experimentally implemented through the end-point measurement and the two-point measurement scheme. Using this framework, we demonstrate the explicit contribution of coherence to the fluctuation, the average, and the second moment of work. In a two-level system, we show that non-joint measurability, a generalized notion of measurement incompatibility, can increase the amount of extractable work beyond the classical bound imposed by jointly measurable measurements. We further prove that the real part of Kirkwood-Dirac quasiprobability (KDQ) and the OQ are equivalent in two-level systems, and they are nonnegative for binary unbiased measurements if and only if the measurements are jointly measurable. In a three-level Nitrogen-vacancy center system, the OQ and the KDQ exhibit different amounts of negativities while enabling the same work extraction, implying that the magnitude of negativity is not a faithful indicator of nonclassical work. These results highlight that coherence and non-joint measurability play fundamental roles in the enhancement of work.
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Submitted 5 October, 2025;
originally announced October 2025.
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Quantum simulation approach to ultra-weak magnetic anisotropy in a frustrated spin-1/2 antiferromagnet
Authors:
Ki Won Jeong,
Jae Yeon Seo,
Sunghyun Lim,
Jae Min Hong,
Hyeon Jun Ryu,
Jongseok Byeon,
Kyungsun Moon,
Nara Lee,
Young Jai Choi
Abstract:
The intrinsic equivalence between electron spin and qubit offers a natural foundation for quantum simulations of magnetic materials. However, incorporating magnetocrystalline anisotropy (MCA), a key feature of real magnets, remains a major challenge. Here, we develop a quantum simulation framework for MCA in CuSb2O6, a spin-1/2 antiferromagnet with alternating ferromagnetic chains arising from fru…
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The intrinsic equivalence between electron spin and qubit offers a natural foundation for quantum simulations of magnetic materials. However, incorporating magnetocrystalline anisotropy (MCA), a key feature of real magnets, remains a major challenge. Here, we develop a quantum simulation framework for MCA in CuSb2O6, a spin-1/2 antiferromagnet with alternating ferromagnetic chains arising from frustrated, anisotropic exchange interactions in a nearly square lattice. The $\mathrm{Cu}^{2+}$ spin network is modeled as a four-qubit square lattice, with four paired ancilla qubits introduced to encode angle-dependent MCA. This two-qubit representation per spin site resolves the limitation that squared Pauli operators yield only the identity, enabling MCA terms to be faithfully embedded into quantum circuits. Using the variational quantum eigensolver, we determine an exceptionally small easy-axis MCA constant, just 0.00022% of the nearest-neighbor exchange interaction, yet sufficient to drive a spin-flop transition with $90^{\circ}$ spin reorientation and strong angular variation in magnetic torque. Beyond this regime, the simulations uncover a half-saturated magnetic phase at ultra-high fields, stabilized by anisotropic next-nearest-neighbor interactions. Our findings demonstrate the feasibility of resource-efficient quantum simulations of complex magnetic phenomena in real materials.
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Submitted 1 October, 2025; v1 submitted 26 September, 2025;
originally announced September 2025.
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Raman spectroscopy of graphite with water as the pressure medium
Authors:
K. Perry,
A. T. Roy,
A. R. Parmenter,
Y. J. Ryu,
V. B. Prakapenka,
J. Lim
Abstract:
We report a high-pressure Raman spectroscopy study of a graphite-water mixture using water as the pressure-transmitting medium up to 9.9 GPa. In the graphite-rich region, three characteristic Raman features-the $E_{2g}^{(1)}$ shear mode, the G band ($E_{2g}^{(2)}$), and the 2D band-were observed and tracked as a function of pressure. The G band exhibits a pronounced blue shift with increasing pres…
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We report a high-pressure Raman spectroscopy study of a graphite-water mixture using water as the pressure-transmitting medium up to 9.9 GPa. In the graphite-rich region, three characteristic Raman features-the $E_{2g}^{(1)}$ shear mode, the G band ($E_{2g}^{(2)}$), and the 2D band-were observed and tracked as a function of pressure. The G band exhibits a pronounced blue shift with increasing pressure, indicating enhanced interlayer coupling between graphite planes. In the water-rich region, the librational band and three distinct O-H stretching modes were identified. Notably, above 8 GPa, the slope of the pressure dependence decreases relative to the earlier report, likely due to the influence of the water pressure medium, emphasizing the need for further investigation at higher pressures.
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Submitted 1 September, 2025;
originally announced September 2025.
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Dark states of electrons in a quantum system with two pairs of sublattices
Authors:
Yoonah Chung,
Minsu Kim,
Yeryn Kim,
Seyeong Cha,
Joon Woo Park,
Jeehong Park,
Yeonjin Yi,
Dongjoon Song,
Jung Hyun Ryu,
Kimoon Lee,
Timur K. Kim,
Cephise Cacho,
Jonathan Denlinger,
Chris Jozwiak,
Eli Rotenberg,
Aaron Bostwick,
Keun Su Kim
Abstract:
A quantum state of matter that is forbidden to interact with photons and is therefore undetectable by spectroscopic means is called a dark state. This basic concept can be applied to condensed matter where it suggests that a whole band of quantum states could be undetectable across a full Brillouin zone. Here we report the discovery of such condensed matter dark states in palladium diselenide as a…
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A quantum state of matter that is forbidden to interact with photons and is therefore undetectable by spectroscopic means is called a dark state. This basic concept can be applied to condensed matter where it suggests that a whole band of quantum states could be undetectable across a full Brillouin zone. Here we report the discovery of such condensed matter dark states in palladium diselenide as a model system that has two pairs of sublattices in the primitive cell. By using angle-resolved photoemission spectroscopy, we find valence bands that are practically unobservable over the whole Brillouin zone at any photon energy, polarisation, and scattering plane. Our model shows that two pairs of sublattices located at half-translation positions and related by multiple glide-mirror symmetries make their relative quantum phases polarised into only four kinds, three of which become dark due to double destructive interference. This mechanism is generic to other systems with two pairs of sublattices, and we show how the phenomena observed in cuprates, lead-halide perovskites, and density wave systems can be resolved by the mechanism of dark states. Our results suggest that the sublattice degree of freedom, which has been overlooked so far, should be considered in the study of correlated phenomena and optoelectronic characteristics.
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Submitted 10 July, 2025;
originally announced July 2025.
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Nickel Doping Unlocks Ambient-condition Photostability in Individual Cesium Lead Bromide Perovskite Quantum Dots
Authors:
Jehyeok Ryu,
Victor Krivenkov,
Adam Olejniczak,
Mikel Arruabarrena,
Jozef Janovec,
Aritz Leonardo,
Virginia Martínez-Martínez,
Andres Ayuela,
Alexey Nikitin,
Yury Rakovich
Abstract:
Developing efficient single-photon sources is fundamental to advancing photonic quantum technologies. In particular, achieving scalable, cost-effective, stable, high-rate, and high-purity single-photon emission at ambient conditions is paramount for free-space quantum communication. However, fulfilling all the requirements simultaneously under ambient conditions has remained a significant challeng…
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Developing efficient single-photon sources is fundamental to advancing photonic quantum technologies. In particular, achieving scalable, cost-effective, stable, high-rate, and high-purity single-photon emission at ambient conditions is paramount for free-space quantum communication. However, fulfilling all the requirements simultaneously under ambient conditions has remained a significant challenge. Here, the scalable, cost-effective ambient condition synthesis of nickel doped (Ni doped) CsPbBr3 perovskite quantum dots (NPQDs) is presented using a modified ligand-assisted reprecipitation (LARP) method. The resulting individual NPQDs demonstrate remarkable photostability, sustaining their performance for over 10 minutes under ambient conditions with environment humidity of ~55%, and exhibit exceptional single-photon purity (>99%) with a narrow emission linewidth (~70 meV). The remarkable photostability could be attributed to the spatial localization of exciton by Ni atoms on the surface of the nanocrystal, reducing its interaction with the environment. Our results demonstrated that NPQDs with outstanding combinations of quantum emitting properties can be both synthesized and operated at ambient conditions. These findings mark a significant step toward scalable, cost-effective quantum light sources for real-world applications, paving the way for robust quantum communication systems and devices.
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Submitted 14 November, 2025; v1 submitted 8 June, 2025;
originally announced June 2025.
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Non-orientable Exceptional Points in Twisted Boundary Systems
Authors:
Jung-Wan Ryu,
Jae-Ho Han,
Moon Jip Park,
Hee Chul Park,
Chang-Hwan Yi
Abstract:
Non-orientable manifolds, such as the Möbius strip and the Klein bottle, defy conventional geometric intuition through their twisted boundary conditions. As a result, topological defects on non-orientable manifolds give rise to novel physical phenomena. We study the adiabatic transport of exceptional points (EPs) along non-orientable closed loops and uncover distinct topological responses arising…
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Non-orientable manifolds, such as the Möbius strip and the Klein bottle, defy conventional geometric intuition through their twisted boundary conditions. As a result, topological defects on non-orientable manifolds give rise to novel physical phenomena. We study the adiabatic transport of exceptional points (EPs) along non-orientable closed loops and uncover distinct topological responses arising from the lack of global orientation. Notably, we demonstrate that the cyclic permutation of eigenstates across an EP depends sensitively on the loop orientation, yielding inequivalent braid representations for clockwise and counterclockwise encirclement; this is a feature unique to non-orientable geometries. Orientation-dependent geometric quantities, such as the winding number, cannot be consistently defined due to the absence of a global orientation. However, when a boundary is introduced, such quantities become well defined within the local interior, even though the global manifold remains non-orientable. We further demonstrate the adiabatic evolution of EPs and the emergence of orientation-sensitive observables in a Klein Brillouin zone, described by an effective non-Hermitian Hamiltonian that preserves momentum-space glide symmetry. Finally, we numerically implement these ideas in a microdisk cavity with embedded scatterers using synthetic momenta.
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Submitted 16 April, 2025;
originally announced April 2025.
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Superconducting dome and structural changes in LaRu$_3$Si$_2$ under pressure
Authors:
Zhuoqi Li,
Shuyuan Huyan,
Elizabeth C. Thompson,
Tyler J. Slade,
Dongzhou Zhang,
Young J. Ryu,
Wenli Bi,
Sergey L. Bud'ko,
Paul C. Canfield
Abstract:
LaRu$_3$Si$_2$ is of current research interest as a kagome metal with a superconducting transition temperature, $T_c\sim$7 K and higher temperature charge density wave (CDW) orders. Here we report electrical transport and X-ray diffraction measurements on LaRu$_3$Si$_2$ under pressure up to 65 GPa and 35 GPa respectively. The superconducting transition temperature $T_c$ first gets slightly enhance…
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LaRu$_3$Si$_2$ is of current research interest as a kagome metal with a superconducting transition temperature, $T_c\sim$7 K and higher temperature charge density wave (CDW) orders. Here we report electrical transport and X-ray diffraction measurements on LaRu$_3$Si$_2$ under pressure up to 65 GPa and 35 GPa respectively. The superconducting transition temperature $T_c$ first gets slightly enhanced and reaches a maximum $\sim$8.7 K at $\sim$8.5 GPa. With further applied pressure, $T_c$ is initially gradually suppressed, then more rapidly suppressed, followed by gradual suppression, revealing a superconducting dome. Two possible pressure-induced structural phase transitions are also observed at room temperature, from original hexagonal phase to another hexagonal structure above $\sim$11.5 GPa, and further to a structure with lower symmetry above $\sim$23.5 GPa. These transition pressures roughly correlate with features found in our pressure dependent transport data.
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Submitted 18 April, 2025; v1 submitted 14 March, 2025;
originally announced March 2025.
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Engineering high Chern number insulators
Authors:
Sungjong Woo,
Seungbum Woo,
Jung-Wan Ryu,
Hee Chul Park
Abstract:
The concept of Chern insulators is one of the most important buliding block of topological physics, enabling the quantum Hall effect without external magnetic fields. The construction of Chern insulators has been typically through an guess-and-confirm approach, which can be inefficient and unpredictable. In this paper, we introduce a systematic method to directly construct two-dimensional Chern in…
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The concept of Chern insulators is one of the most important buliding block of topological physics, enabling the quantum Hall effect without external magnetic fields. The construction of Chern insulators has been typically through an guess-and-confirm approach, which can be inefficient and unpredictable. In this paper, we introduce a systematic method to directly construct two-dimensional Chern insulators that can provide any nontrivial Chern number. Our method is built upon the one-dimensional Rice-Mele model, which is well known for its adjustable polarization properties, providing a reliable framework for manipulation. By extending this model into two dimensions, we are able to engineer lattice structures that demonstrate predetermined topological quantities effectively. This research not only contributes the development of Chern insulators but also paves the way for designing a variety of lattice structures with significant topological implications, potentially impacting quantum computing and materials science. With this approach, we are to shed light on the pathways for designing more complex and functional topological phases in synthetic materials.
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Submitted 23 July, 2024;
originally announced July 2024.
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Pseudo-Hermitian Topology of Multiband Non-Hermitian Systems
Authors:
Jung-Wan Ryu,
Jae-Ho Han,
Chang-Hwan Yi,
Hee Chul Park,
Moon Jip Park
Abstract:
The complex eigenenergies and non-orthogonal eigenstates of non-Hermitian systems exhibit unique topological phenomena that cannot appear in Hermitian systems. Representative examples are the non-Hermitian skin effect and exceptional points. In a two-dimensional parameter space, topological classifications of non-separable bands in multiband non-Hermitian systems can be established by invoking a p…
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The complex eigenenergies and non-orthogonal eigenstates of non-Hermitian systems exhibit unique topological phenomena that cannot appear in Hermitian systems. Representative examples are the non-Hermitian skin effect and exceptional points. In a two-dimensional parameter space, topological classifications of non-separable bands in multiband non-Hermitian systems can be established by invoking a permutation group, where the product of the permutation represents state exchange due to exceptional points in the space. We unveil in this work the role of pseudo-Hermitian lines in non-Hermitian topology for multiple bands. In particular, the non-separability of non-Hermitian multibands can be topologically non-trivial without exceptional points in two-dimensional space. As a physical illustration of the role of pseudo-Hermitian lines, we examine a multiband structure of a photonic crystal system with lossy materials. Our work builds on the fundamental and comprehensive understanding of non-Hermitian multiband systems and also offers versatile applications and realizations of non-Hermitian systems without the need to consider exceptional points.
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Submitted 17 December, 2024; v1 submitted 27 May, 2024;
originally announced May 2024.
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Boundary effect and quantum phases in spin chains
Authors:
Jinhyeok Ryu,
Jaeyoon Cho
Abstract:
Boundary effect is a widespread idea in many-body theories. However, it is more of a conceptual notion than a rigorously defined physical quantity. One can quantify the boundary effect by comparing two ground states of the same physical model, which differ only slightly in system size. Here, we analyze the quantity, which we call a boundary effect function, for an XXZ spin-1/2 model using density…
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Boundary effect is a widespread idea in many-body theories. However, it is more of a conceptual notion than a rigorously defined physical quantity. One can quantify the boundary effect by comparing two ground states of the same physical model, which differ only slightly in system size. Here, we analyze the quantity, which we call a boundary effect function, for an XXZ spin-1/2 model using density matrix renormalization group calculations. We find that three quantum phases of the model manifest as different functional forms of the boundary effect function. As a result, the quantum phase transition of the model is associated with a nonanalytic change of the boundary effect function. This work thus provides and concretizes a novel perspective on the relationship between bulk and boundary properties of ground states.
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Submitted 30 April, 2024;
originally announced April 2024.
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On the feasibility of quantum teleportation protocols implemented with Silicon devices
Authors:
Junghee Ryu,
Hoon Ryu
Abstract:
With recent experimental advancements demonstrating high-fidelity universal logic gates and basic programmability, Silicon-based spin quantum bit (qubit) have emerged as promising candidates for scalable quantum computing. However, implementation of more complex quantum information protocols with many qubits still remains a critical challenge for realization of practical programmability in Silicon…
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With recent experimental advancements demonstrating high-fidelity universal logic gates and basic programmability, Silicon-based spin quantum bit (qubit) have emerged as promising candidates for scalable quantum computing. However, implementation of more complex quantum information protocols with many qubits still remains a critical challenge for realization of practical programmability in Silicon devices. In this study, we present a computational investigation of entanglement-based quantum information applications implemented on an electrically defined quantum dot structure in Silicon. Using in-house multi-scale simulations based on tight-binding calculations augmented with bulk physics, we model a five quantum dot system that can create up to five electron spin qubits, and discuss details of control engineering needed to implement single-qubit rotations and two-qubit logic operations in a programmable manner. Using these elementary operations, then, we design a five-qubit quantum teleportation protocol and computationally verify its end-to-end operation including a simple but clear analysis on how the designed circuit can be affected by charge noise. With engineering details that are not well uncovered by experiments, our results demonstrate the advanced programmability of Silicon quantum dot systems, delivering the practical guidelines for potential designs of quantum information processes based on electrically defined Silicon quantum dot structures.
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Submitted 4 October, 2024; v1 submitted 28 March, 2024;
originally announced March 2024.
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Seamless monolithic three-dimensional integration of single-crystalline films by growth
Authors:
Ki Seok Kim,
Seunghwan Seo,
Junyoung Kwon,
Doyoon Lee,
Changhyun Kim,
Jung-El Ryu,
Jekyung Kim,
Min-Kyu Song,
Jun Min Suh,
Hang-Gyo Jung,
Youhwan Jo,
Hogeun Ahn,
Sangho Lee,
Kyeongjae Cho,
Jongwook Jeon,
Minsu Seol,
Jin-Hong Park,
Sang Won Kim,
Jeehwan Kim
Abstract:
The demand for the three-dimensional (3D) integration of electronic components is on a steady rise. The through-silicon-via (TSV) technique emerges as the only viable method for integrating single-crystalline device components in a 3D format, despite encountering significant processing challenges. While monolithic 3D (M3D) integration schemes show promise, the seamless connection of single-crystal…
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The demand for the three-dimensional (3D) integration of electronic components is on a steady rise. The through-silicon-via (TSV) technique emerges as the only viable method for integrating single-crystalline device components in a 3D format, despite encountering significant processing challenges. While monolithic 3D (M3D) integration schemes show promise, the seamless connection of single-crystalline semiconductors without intervening wafers has yet to be demonstrated. This challenge arises from the inherent difficulty of growing single crystals on amorphous or polycrystalline surfaces post the back-end-of-the-line process at low temperatures to preserve the underlying circuitry. Consequently, a practical growth-based solution for M3D of single crystals remains elusive. Here, we present a method for growing single-crystalline channel materials, specifically composed of transition metal dichalcogenides, on amorphous and polycrystalline surfaces at temperatures lower than 400 °C. Building on this developed technique, we demonstrate the seamless monolithic integration of vertical single-crystalline logic transistor arrays. This accomplishment leads to the development of unprecedented vertical CMOS arrays, thereby constructing vertical inverters. Ultimately, this achievement sets the stage to pave the way for M3D integration of various electronic and optoelectronic hardware in the form of single crystals.
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Submitted 6 December, 2023; v1 submitted 5 December, 2023;
originally announced December 2023.
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Spontaneous Unidirectional Loop Extrusion Emerges from Symmetry Breaking of SMC Extension
Authors:
Andrea Bonato,
Jae-Won Jang,
Kyoung-Wook Moon,
Davide Michieletto,
Je-Kyung Ryu
Abstract:
DNA loop extrusion is arguably one of the most important players in genome organization. The precise mechanism by which loop extruding factors (LEFs) work is still unresolved and much debated. One of the major open questions in this field is how do LEFs establish and maintain unidirectional motion along DNA. In this paper, we use High-Speed AFM data to show that condensin hinge domain displays a s…
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DNA loop extrusion is arguably one of the most important players in genome organization. The precise mechanism by which loop extruding factors (LEFs) work is still unresolved and much debated. One of the major open questions in this field is how do LEFs establish and maintain unidirectional motion along DNA. In this paper, we use High-Speed AFM data to show that condensin hinge domain displays a structural, geometric constraint on the angle within which it can extend with respect to the DNA-bound domains. Using computer simulations, we then show that such a geometrical constraint results in a local symmetry breaking and is enough to rectify the extrusion process, yielding unidirectional loop extrusion along DNA. Our work highlights an overlooked geometric aspect of the loop extrusion process that may have a universal impact on SMC function across organisms.
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Submitted 15 September, 2023;
originally announced September 2023.
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Symmetry-protected flatband condition for Hamiltonians with local symmetry
Authors:
Jung-Wan Ryu,
Alexei Andreanov,
Hee Chul Park,
Jae-Ho Han
Abstract:
We derive symmetry-based conditions for tight-binding Hamiltonians with flatbands to have compact localized eigenstates occupying a single unit cell. The conditions are based on unitary operators commuting with the Hamiltonian and associated with local symmetries that guarantee compact localized states and a flatband. We illustrate the conditions for compact localized states and flatbands with sim…
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We derive symmetry-based conditions for tight-binding Hamiltonians with flatbands to have compact localized eigenstates occupying a single unit cell. The conditions are based on unitary operators commuting with the Hamiltonian and associated with local symmetries that guarantee compact localized states and a flatband. We illustrate the conditions for compact localized states and flatbands with simple Hamiltonians with given symmetries. We also apply these results to general cases such as the Hamiltonian with long-range hoppings and higher-dimensional Hamiltonian.
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Submitted 28 August, 2023;
originally announced August 2023.
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Exceptional Classifications of Non-Hermitian Systems
Authors:
Jung-Wan Ryu,
Jae-Ho Han,
Chang-Hwan Yi,
Moon Jip Park,
Hee Chul Park
Abstract:
Eigenstate coalescence in non-Hermitian systems is widely observed in diverse scientific domains encompassing optics and open quantum systems. Recent investigations have revealed that adiabatic encircling of exceptional points (EPs) leads to a nontrivial Berry phase in addition to an exchange of eigenstates. Based on these phenomena, we propose in this work an exhaustive classification framework f…
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Eigenstate coalescence in non-Hermitian systems is widely observed in diverse scientific domains encompassing optics and open quantum systems. Recent investigations have revealed that adiabatic encircling of exceptional points (EPs) leads to a nontrivial Berry phase in addition to an exchange of eigenstates. Based on these phenomena, we propose in this work an exhaustive classification framework for EPs in non-Hermitian physical systems. In contrast to previous classifications that only incorporate the eigenstate exchange effect, our proposed classification gives rise to finer $\mathbb{Z}_2$ classifications depending on the presence of a $π$ Berry phase after the encircling of the EPs. Moreover, by mapping arbitrary one-dimensional systems to the adiabatic encircling of EPs, we can classify one-dimensional non-Hermitian systems characterized by topological phase transitions involving EPs. Applying our exceptional classification to various one-dimensional models, such as the non-reciprocal Su--Schrieffer--Heeger (SSH) model, we exhibit the potential for enhancing the understanding of topological phases in non-Hermitian systems. Additionally, we address exceptional bulk-boundary correspondence and the emergence of distinct topological boundary modes in non-Hermitian systems.
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Submitted 12 June, 2023;
originally announced June 2023.
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Realization of Non-Hermitian Hopf Bundle Matter
Authors:
Yung Kim,
Hee Chul Park,
Minwook Kyung,
Kyungmin Lee,
Jung-Wan Ryu,
Oubo You,
Shuang Zhang,
Bumki Min,
Moon Jip Park
Abstract:
Line excitations in topological phases are a subject of particular interest because their mutual linking structures encode robust topological information of matter. It has been recently shown that the linking and winding of complex eigenenergy strings can classify one-dimensional non-Hermitian topological matter. However, in higher dimensions, bundles of linked strings can emerge such that every s…
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Line excitations in topological phases are a subject of particular interest because their mutual linking structures encode robust topological information of matter. It has been recently shown that the linking and winding of complex eigenenergy strings can classify one-dimensional non-Hermitian topological matter. However, in higher dimensions, bundles of linked strings can emerge such that every string is mutually linked with all the other strings. Interestingly, despite being an unconventional topological structure, a non-Hermitian Hopf bundle has not been experimentally clarified. Here, we make the first attempt to explore the non-Hermitian Hopf bundle by visualizing the global linking structure of spinor strings in the momentum space of a two-dimensional electric circuit. By exploiting the flexibility of reconfigurable couplings between circuit nodes, we can study the non-Hermitian topological phase transition and gain insight into the intricate structure of the Hopf bundle. Furthermore, we find that the emergence of a higher-order skin effect in real space is accompanied by the linking of spinor strings in momentum space, revealing a bulk-boundary correspondence between the two domains. The proposed non-Hermitian Hopf bundle platform and visualization methodology pave the way to design new topologically robust non-Hermitian phases of matter.
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Submitted 23 March, 2023;
originally announced March 2023.
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Effects of Crystalline Disorder on Interfacial and Magnetic Properties of Sputtered Topological Insulator/Ferromagnet Heterostructures
Authors:
Nirjhar Bhattacharjee,
Krishnamurthy Mahalingam,
Adrian Fedorko,
Alexandria Will-Cole,
Jaehyeon Ryu,
Michael Page,
Michael McConney,
Hui Fang,
Don Heiman,
Nian Xiang Sun
Abstract:
Thin films of Topological insulators (TIs) coupled with ferromagnets (FMs) are excellent candidates for energy-efficient spintronics devices. Here, the effect of crystalline structural disorder of TI on interfacial and magnetic properties of sputter-deposited TI/FM, Bi2Te3/Ni80Fe20, heterostructures is reported. Ni and a smaller amount of Fe from Py was found to diffuse across the interface and re…
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Thin films of Topological insulators (TIs) coupled with ferromagnets (FMs) are excellent candidates for energy-efficient spintronics devices. Here, the effect of crystalline structural disorder of TI on interfacial and magnetic properties of sputter-deposited TI/FM, Bi2Te3/Ni80Fe20, heterostructures is reported. Ni and a smaller amount of Fe from Py was found to diffuse across the interface and react with Bi2Te3. For highly crystalline c-axis oriented Bi2Te3 films, a giant enhancement in Gilbert damping is observed, accompanied by an effective out-of-plane magnetic anisotropy and enhanced damping-like spin-orbit torque (DL-SOT), possibly due to the topological surface states (TSS) of Bi2Te3. Furthermore, a spontaneous exchange bias is observed in hysteresis loop measurements at low temperatures. This is because of an antiferromagnetic topological interfacial layer formed by reaction of the diffused Ni with Bi2Te3 which couples with the FM, Ni80Fe20. For increasing disorder of Bi2Te3, a significant weakening of exchange interaction in the AFM interfacial layer is found. These experimental results Abstract length is one paragraph.
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Submitted 19 May, 2022;
originally announced May 2022.
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Exploring entanglement resource in Si quantum dot systems with operational quasiprobability approach
Authors:
Junghee Ryu,
Hoon Ryu
Abstract:
We characterize the quantum entanglement of the realistic two-qubit signals that are sensitive to charge noises. Our working example is the time response generated from a silicon double quantum dot (DQD) platform, where a single-qubit rotation and a two-qubit controlled-NOT operation are conducted sequentially in time to generate arbitrary entangled states. In order to characterize the entanglemen…
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We characterize the quantum entanglement of the realistic two-qubit signals that are sensitive to charge noises. Our working example is the time response generated from a silicon double quantum dot (DQD) platform, where a single-qubit rotation and a two-qubit controlled-NOT operation are conducted sequentially in time to generate arbitrary entangled states. In order to characterize the entanglement of two-qubit states, we employ the marginal operational quasiprobability (OQ) approach that allows negative values of the probability function if a given state is entangled. While the charge noise, which is omnipresent in semiconductor devices, severely affects logic operations implemented in the DQD platform, causing huge degradation in fidelity of unitary operations as well as resulting two-qubit states, the pattern in the OQ-driven entanglement strength turns out to be quite invariant, indicating that the resource of quantum entanglement is not significantly broken though the physical system is exposed to noise-driven fluctuations in exchange interaction between quantum dots.
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Submitted 27 September, 2022; v1 submitted 30 March, 2022;
originally announced March 2022.
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Direct observation of orbital driven strong interlayer coupling in puckered two-dimensional PdSe2
Authors:
Jung Hyun Ryu,
Jeong-Gyu Kim,
Bongjae Kim,
Kyoo Kim,
Sooran Kim,
Byeong-Gyu Park,
Younghak Kim,
Kyung-Tae Ko,
Kimoon Lee
Abstract:
Interlayer coupling between individual unit layers has played a critical role for layer-dependent properties in two-dimensional (2D) materials. While recent studies have revealed the significant degrees of interlayer interactions, the overall electronic structure of the 2D material has been mostly addressed by the intralayer interactions. Here, we report the direct observation of a highly dispersi…
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Interlayer coupling between individual unit layers has played a critical role for layer-dependent properties in two-dimensional (2D) materials. While recent studies have revealed the significant degrees of interlayer interactions, the overall electronic structure of the 2D material has been mostly addressed by the intralayer interactions. Here, we report the direct observation of a highly dispersive single electronic band along the interlayer direction in puckered 2D PdSe2 as an experimental hallmark of strong interlayer couplings. Remarkably large band dispersion along kz-direction near Fermi level, which is even wider than the in-plane one, is observed by the angle-resolved photoemission spectroscopy measurement. Employing the X-ray absorption spectroscopy and density functional theory calculations, we reveal that the strong interlayer coupling in 2D PdSe2 originates from the unique directional bonding of Pd d orbitals associated with unexpected Pd 4d9 configuration, which consequently gives rise to the strong layer-dependency of the band gap.
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Submitted 19 July, 2021;
originally announced July 2021.
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Stochastic thermodynamics of inertial-like Stuart-Landau dimer
Authors:
Jung-Wan Ryu,
Alexandre Lazarescu,
Rahul Marathe,
Juzar Thingna
Abstract:
Stuart-Landau limit-cycle oscillators are a paradigm in the study of coherent and incoherent limit cycles. In this work, we generalize the standard Stuart-Landau dimer model to include effects due to an inertia-like term and noise and study its dynamics and stochastic thermodynamics. In the absence of noise (zero-temperature limit), the dynamics show the emergence of a new bistable phase where coh…
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Stuart-Landau limit-cycle oscillators are a paradigm in the study of coherent and incoherent limit cycles. In this work, we generalize the standard Stuart-Landau dimer model to include effects due to an inertia-like term and noise and study its dynamics and stochastic thermodynamics. In the absence of noise (zero-temperature limit), the dynamics show the emergence of a new bistable phase where coherent and incoherent limit cycles coexist. At finite temperatures, we develop a stochastic thermodynamic framework based on the dynamics of a charged particle in a magnetic field to identify physically meaningful heat and work. The stochastic system no longer exhibits the bistable phase but the thermodynamic observables, such as work, exhibit bistability in the temporally metastable regime. We demonstrate that the inertial-like Stuart-Landau dimer operates like a machine, reliably outputting the most work when the oscillators coherently synchronize and unreliable with minimum work output when the oscillators are incoherent. Overall, our results show the importance of coherent synchronization within the working substance in the operation of a thermal machine.
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Submitted 5 October, 2021; v1 submitted 1 July, 2021;
originally announced July 2021.
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Topological edge states in bowtie ladders with different cutting edges
Authors:
Jung-Wan Ryu,
Sungjong Woo,
Nojoon Myoung,
Hee Chul Park
Abstract:
We have studied topological edge states in bowtie ladders with various edge truncations. The symmetric bowtie ladder, which comprises two trivial Su-Schrieffer-Heeger (SSH) lattices, exhibits an insulator-metal transition with trivial insulating states. On the other hand, the lattice can be transformed into an extended SSH lattice depending on the edge shapes with non-trivial insulating states in…
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We have studied topological edge states in bowtie ladders with various edge truncations. The symmetric bowtie ladder, which comprises two trivial Su-Schrieffer-Heeger (SSH) lattices, exhibits an insulator-metal transition with trivial insulating states. On the other hand, the lattice can be transformed into an extended SSH lattice depending on the edge shapes with non-trivial insulating states in that the winding number is non-zero. The winding numbers are permutationally designated in the phase diagram depending on the choice of unit cell. The topological edge states are affected by the shape of the edge and the corresponding winding number. We also studied general bowtie ladder models with richer phase diagrams using the characteristics of the localization length of the edge states showing state bifurcation.
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Submitted 1 December, 2020;
originally announced December 2020.
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Nanoscale characterization of the impact of beverages on the enamel surface of human teeth
Authors:
Panpan Li,
Chungik Oh,
Hongjun Kim,
Melodie Chen-Glasser,
Gun Park,
Albina Jetybayeva,
Jiwon Yeom,
Hoon Kim,
Jeongjae Ryu,
Seungbum Hong
Abstract:
Here we quantitatively evaluate the early stages of mechanical and morphological changes of polished human enamel surfaces induced by soft drinks using atomic force microscopy. With an increase of the immersion time in soft drinks, we found a significant increase of surface roughness (Ra) and a considerable decrease of elastic modulus (E) of the enamel. The prismatic structure of enamel was clearl…
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Here we quantitatively evaluate the early stages of mechanical and morphological changes of polished human enamel surfaces induced by soft drinks using atomic force microscopy. With an increase of the immersion time in soft drinks, we found a significant increase of surface roughness (Ra) and a considerable decrease of elastic modulus (E) of the enamel. The prismatic structure of enamel was clearly observed after a one-hour immersion in Coca-Cola, which shows its strong erosion effect. A high surface roughness of enamel results in a high chance of cavities due to easier bacterial adhesion on rougher surface, while a drastic deterioration of the mechanical properties of the enamel weakens its protection property. Our findings show the variation of enamel surface at the very beginning stage of etching process by acidic drinks, which can also be applicable to the etching mechanism of enamel surface by other sources.
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Submitted 2 September, 2019;
originally announced September 2019.
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Emergent localized states at the interface of a twofold $\mathcal{PT}$-symmetric lattice
Authors:
Jung-Wan Ryu,
Nojoon Myoung,
Sungjong Woo,
Ara Go,
Sang-Jun Choi,
Hee Chul Park
Abstract:
We consider the role of non-triviality resulting from a non-Hermitian Hamiltonian that conserves twofold PT-symmetry assembled by interconnections between a PT-symmetric lattice and its time reversal partner. Twofold PT-symmetry in the lattice produces additional surface exceptional points that play the role of new critical points, along with the bulk exceptional point. We show that there are two…
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We consider the role of non-triviality resulting from a non-Hermitian Hamiltonian that conserves twofold PT-symmetry assembled by interconnections between a PT-symmetric lattice and its time reversal partner. Twofold PT-symmetry in the lattice produces additional surface exceptional points that play the role of new critical points, along with the bulk exceptional point. We show that there are two distinct regimes possessing symmetry-protected localized states, of which localization lengths are robust against external gain and loss. The states are demonstrated by numerical calculation of a quasi-1D ladder lattice and a 2D bilayered square lattice.
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Submitted 31 March, 2019;
originally announced April 2019.
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Splitting of conductance resonance through a magnetic quantum dot in graphene
Authors:
Nojoon Myoung,
Jung-Wan Ryu,
Hee Chul Park,
Seung Joo Lee,
Sungjong Woo
Abstract:
We report a dual resonance feature in ballistic conductance through a quantum Hall graphene nanoribbon with a magnetic quantum dot. Such a magnetic quantum dot localizes Dirac fermions exhibiting anisotropic eigenenergy spectra with broken time-reversal symmetry. Interplay between the localized states and quantum Hall edge states is found to be two-fold, showing Breit-Wigner and Fano resonances, w…
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We report a dual resonance feature in ballistic conductance through a quantum Hall graphene nanoribbon with a magnetic quantum dot. Such a magnetic quantum dot localizes Dirac fermions exhibiting anisotropic eigenenergy spectra with broken time-reversal symmetry. Interplay between the localized states and quantum Hall edge states is found to be two-fold, showing Breit-Wigner and Fano resonances, which is reminiscent of a double quantum dot system. By fitting the numerical results with the Fano-Breit-Wigner lineshape from the double quantum dot model, we demonstrate that the two-fold resonance is due to the valley mixing that comes from the coupling of the magnetic quantum dot with quantum Hall edge channels; an effective double quantum dot system emerges from a single magnetic quantum dot in virtue of the valley degree of freedom. It is further confirmed that the coupling is weaker for the Fano resonance and stronger for the Breit-Wigner resonace.
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Submitted 2 November, 2018;
originally announced November 2018.
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Antiresonance induced by symmetry-broken contacts in quasi-one-dimensional lattices
Authors:
Jung-Wan Ryu,
Nojoon Myoung,
Hee Chul Park
Abstract:
We report the effect of symmetry-broken contacts on quantum transport in quasi-one-dimensional lattices. In contrast to 1D chains, transport in quasi-one-dimensional lattices, which are made up of a finite number of 1D chain layers, is strongly influenced by contacts. Contact symmetry depends on whether the contacts maintain or break the parity symmetry between the layers. With balanced on-site po…
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We report the effect of symmetry-broken contacts on quantum transport in quasi-one-dimensional lattices. In contrast to 1D chains, transport in quasi-one-dimensional lattices, which are made up of a finite number of 1D chain layers, is strongly influenced by contacts. Contact symmetry depends on whether the contacts maintain or break the parity symmetry between the layers. With balanced on-site potential, a flat band can be detected by asymmetric contacts, but not by symmetric contacts. In the case of asymmetric contacts with imbalanced on-site potential, transmission is suppressed at certain energies. We elucidate these energies of transmission suppression related to antiresonance using reduced lattice models and Feynman paths. These results provide a nondestructive measurement of flat band energy which it is difficult to detect.
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Submitted 31 August, 2017;
originally announced September 2017.
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P-type polar transition of chemically doped multilayer MoS2 transistor
Authors:
Xiaochi Liu,
Deshun Qu,
Jungjin Ryu,
Faisal Ahmed,
Zheng Yang,
Daeyeong Lee,
Won Jong Yoo
Abstract:
The accessibility of both n-type and p-type MoS2 FET is necessary for complementary device applications involving MoS2. However, MoS2 PFET is rarely achieved due to pinning effect resulting high Rc at metal-MoS2 interface and the inherently strong n-type property of the MoS2 material. In this study, we realized a high-performance multi-layer MoS2 PFET via controllable chemical doping, which has an…
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The accessibility of both n-type and p-type MoS2 FET is necessary for complementary device applications involving MoS2. However, MoS2 PFET is rarely achieved due to pinning effect resulting high Rc at metal-MoS2 interface and the inherently strong n-type property of the MoS2 material. In this study, we realized a high-performance multi-layer MoS2 PFET via controllable chemical doping, which has an excellent on/off ratio of 107 and a maximum hole mobility of 72 cm2/Vs at room temperature, and these values are further exceeding to 109 and 132 cm2/Vs at 133K. In addition, we revealed that large Rc hindered the polar transition of MoS2 FET from n-type to p-type, meanwhile channel Rs limited Ion of PFET. Therefore it is suggested that reducing Rc at high work function metal-MoS2 interface and p-type doping of channel were necessary for achieving high performance MoS2 PFET. Based on the high performance PFET, we successfully demonstrated a MoS2 CMOS inverter by integrating NFET and PFET.
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Submitted 9 December, 2015;
originally announced April 2016.
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Ultimate Thin Vertical p-n Junction Composed of 2D Layered Molybdenum Disulfide
Authors:
Hua-Min Li,
Daeyeong Lee,
Deshun Qu,
Xiaochi Liu,
Jungjin Ryu,
Alan Seabaugh,
Won Jong Yoo
Abstract:
Semiconducting 2D crystals are currently receiving significant attention due to their great potential to be an ultra-thin body for efficient electrostatic modulation which enables to overcome the limitations of silicon technology. Here we report that, as a key building block for 2D semiconductor devices, vertical p-n junctions are fabricated in ultrathin MoS2 by introducing AuCl3 and benzyl violog…
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Semiconducting 2D crystals are currently receiving significant attention due to their great potential to be an ultra-thin body for efficient electrostatic modulation which enables to overcome the limitations of silicon technology. Here we report that, as a key building block for 2D semiconductor devices, vertical p-n junctions are fabricated in ultrathin MoS2 by introducing AuCl3 and benzyl viologen dopants. Unlike usual unipolar MoS2, the MoS2 p-n junctions show (i) ambipolar carrier transport, (ii) current rectification via modulation of potential barrier in films thicker than 8 nm, and (iii) reversed current rectification via tunneling in films thinner than 8 nm. The ultimate thinness of the vertical p-n homogeneous junctions in MoS2 is experimentally found to be 3 nm, and the chemical doping depth is found to be 1.5 nm. The ultrathin MoS2 p-n junctions present a significant potential of the 2D crystals for flexible, transparent, high-efficiency electronic and optoelectronic applications.
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Submitted 12 February, 2015;
originally announced February 2015.
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Spin-Wave Propagation in the Presence of Interfacial Dzyaloshinskii-Moriya Interaction
Authors:
Jung-Hwan Moon,
Soo-Man Seo,
Kyung-Jin Lee,
Kyung-Whan Kim,
Jisu Ryu,
Hyun-Woo Lee,
R. D. McMichael,
M. D. Stiles
Abstract:
In ferromagnetic thin films, broken inversion symmetry and spin-orbit coupling give rise to interfacial Dzyaloshinskii-Moriya interactions. Analytic expressions for spin-wave properties show that the interfacial Dzyaloshinskii-Moriya interaction leads to non-reciprocal spin-wave propagation, i.e. different properties for spin waves propagating in opposite directions. In favorable situations, it ca…
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In ferromagnetic thin films, broken inversion symmetry and spin-orbit coupling give rise to interfacial Dzyaloshinskii-Moriya interactions. Analytic expressions for spin-wave properties show that the interfacial Dzyaloshinskii-Moriya interaction leads to non-reciprocal spin-wave propagation, i.e. different properties for spin waves propagating in opposite directions. In favorable situations, it can increase the spin-wave attenuation length. Comparing measured spin wave properties in ferromagnet$|$normal metal bilayers and other artificial layered structures with these calculations can provide a useful characterization of the interfacial Dzyaloshinskii-Moriya interactions.
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Submitted 15 August, 2013;
originally announced August 2013.
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Current-driven domain wall motion with spin Hall effect: Reduction of threshold current density
Authors:
Jisu Ryu,
Kyung-Jin Lee,
Hyun-Woo Lee
Abstract:
We theoretically study the current-driven domain wall motion in the presence of both the spin Hall effect and an extrinsic pinning potential. The spin Hall effect mainly affects the damping ratio of the domain wall precession in the pinning potential. When the pinning potential is not too strong, this results in a significant reduction of a threshold current density for the depinning of a domain w…
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We theoretically study the current-driven domain wall motion in the presence of both the spin Hall effect and an extrinsic pinning potential. The spin Hall effect mainly affects the damping ratio of the domain wall precession in the pinning potential. When the pinning potential is not too strong, this results in a significant reduction of a threshold current density for the depinning of a domain wall with certain polarity. We also propose one way to distinguish the spin Hall effect induced spin-transfer torque from the one induced by the Rashba spin-orbit coupling experimentally.
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Submitted 26 March, 2013;
originally announced March 2013.
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Theoretical Modeling of ME effect at Low frequency and Resonance Frequency for Magnetoelectric Laminates with Anisotropic Piezoelectric Properties
Authors:
Deepak Rajaram Patil,
Yisheng Chai,
Rahul C. Kambale,
Byung-Gu Jeon,
Jungho Ryu,
Woon-Ha Yoon,
Dong-Soo Park,
Dae-Yong Jeong,
Sang-Goo Lee,
Jeongho Lee,
Joong-Hee Nam,
Jeong-Ho Cho,
Byung-Ik Kim,
Kee Hoon Kim
Abstract:
A new theory is developed for the magnetoelectric (ME) coupling in a symmetric 2-2 ME laminate having a representative piezoelectric crystal (PMN-PT) particularly with anisotropic piezoelectric properties. Considering the average field method, the theoretical expressions for the transverse ME voltage coefficients at low and resonance frequencies were derived. The theory takes into account the anis…
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A new theory is developed for the magnetoelectric (ME) coupling in a symmetric 2-2 ME laminate having a representative piezoelectric crystal (PMN-PT) particularly with anisotropic piezoelectric properties. Considering the average field method, the theoretical expressions for the transverse ME voltage coefficients at low and resonance frequencies were derived. The theory takes into account the anisotropic properties of the piezoelectric materials providing two different expressions of transverse ME voltage coefficients for different in-plane magnetic fields both at low and resonance frequencies. The numerical simulations show multiple resonance frequencies and phase differences between transverse ME voltage coefficients showing good agreement with the experimental results. Our theory should be generally applicable to other ME laminates with any piezoelectric with anisotropic piezoelectric coefficients.
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Submitted 9 December, 2012; v1 submitted 29 November, 2012;
originally announced November 2012.
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Current-induced motion of a transverse magnetic domain wall in the presence of spin Hall effect
Authors:
Soo-Man Seo,
Kyoung-Whan Kim,
Jisu Ryu,
Hyun-Woo Lee,
Kyung-Jin Lee
Abstract:
We theoretically study the current-induced dynamics of a transverse magnetic domain wall in bi-layer nanowires consisting of a ferromagnet on top of a nonmagnet having strong spin-orbit coupling. Domain wall dynamics is characterized by two threshold current densities, $J_{th}^{WB}$ and $J_{th}^{REV}$, where $J_{th}^{WB}$ is a threshold for the chirality switching of the domain wall and…
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We theoretically study the current-induced dynamics of a transverse magnetic domain wall in bi-layer nanowires consisting of a ferromagnet on top of a nonmagnet having strong spin-orbit coupling. Domain wall dynamics is characterized by two threshold current densities, $J_{th}^{WB}$ and $J_{th}^{REV}$, where $J_{th}^{WB}$ is a threshold for the chirality switching of the domain wall and $J_{th}^{REV}$ is another threshold for the reversed domain wall motion caused by spin Hall effect. Domain walls with a certain chirality may move opposite to the electron-flow direction with high speed in the current range $J_{th}^{REV} < J < J_{th}^{WB}$ for the system designed to satisfy the conditions $J_{th}^{WB} > J_{th}^{REV}$ and α> β, where αis the Gilbert damping constant and βis the nonadiabaticity of spin torque. Micromagnetic simulations confirm the validity of analytical results.
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Submitted 15 February, 2012;
originally announced February 2012.
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Magnetization dynamics induced by in-plane currents in ultrathin magnetic nanostructures
Authors:
Kyoung-Whan Kim,
Soo-Man Seo,
Jisu Ryu,
Kyung-Jin Lee,
Hyun-Woo Lee
Abstract:
Ultrathin magnetic systems have properties qualitatively different from their thicker counterparts, implying that different physics governs their properties. We demonstrate that various such properties can be explained naturally by the Rashba spin-orbit coupling in ultrathin magnetic systems. This work will be valuable for the development of next generation spintronic devices based on ultrathin ma…
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Ultrathin magnetic systems have properties qualitatively different from their thicker counterparts, implying that different physics governs their properties. We demonstrate that various such properties can be explained naturally by the Rashba spin-orbit coupling in ultrathin magnetic systems. This work will be valuable for the development of next generation spintronic devices based on ultrathin magnetic systems.
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Submitted 5 January, 2012; v1 submitted 14 November, 2011;
originally announced November 2011.
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Magnetic domain wall motion in a nanowire: depinning and creep
Authors:
Jisu Ryu,
Sug-Bong Choe,
Hyun-Woo Lee
Abstract:
The domain wall motion in a magnetic nanowire is examined theoretically in the regime where the domain wall driving force is weak and its competition against disorders is assisted by thermal agitations. Two types of driving forces are considered; magnetic field and current. While the field induces the domain wall motion through the Zeeman energy, the current induces the domain wall motion by gener…
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The domain wall motion in a magnetic nanowire is examined theoretically in the regime where the domain wall driving force is weak and its competition against disorders is assisted by thermal agitations. Two types of driving forces are considered; magnetic field and current. While the field induces the domain wall motion through the Zeeman energy, the current induces the domain wall motion by generating the spin transfer torque, of which effects in this regime remain controversial. The spin transfer torque has two mutually orthogonal vector components, the adiabatic spin transfer torque and the nonadiabatic spin transfer torque. We investigate separate effects of the two components on the domain wall depinning rate in one-dimensional systems and on the domain wall creep velocity in two-dimensional systems, both below the Walker breakdown threshold. In addition to the leading order contribution coming from the field and/or the nonadiabatic spin transfer torque, we find that the adiabatic spin transfer torque generates corrections, which can be of relevance for an unambiguous analysis of experimental results. For instance, it is demonstrated that the neglect of the corrections in experimental analysis may lead to incorrect evaluation of the nonadiabaticity parameter. Effects of the Rashba spin-orbit coupling on the domain wall motion are also analyzed.
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Submitted 11 April, 2011; v1 submitted 5 April, 2011;
originally announced April 2011.
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Roles of adiabatic and nonadiabatic spin transfer torques on magnetic domain wall motion
Authors:
Jae-Chul Lee,
Kab-Jin Kim,
Jisu Ryu,
Kyoung-Woong Moon,
Sang-Jun Yun,
Gi-Hong Gim,
Kang-Soo Lee,
Kyung-Ho Shin,
Hyun-Woo Lee,
Sug-Bong Choe
Abstract:
Electric current exerts torques-so-called spin transfer torques (STTs)-on magnetic domain walls (DWs), resulting in DW motion. At low current densities, the STTs should compete against disorders in ferromagnetic nanowires but the nature of the competition remains poorly understood. By achieving two-dimensional contour maps of DW speed with respect to current density and magnetic field, here we vis…
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Electric current exerts torques-so-called spin transfer torques (STTs)-on magnetic domain walls (DWs), resulting in DW motion. At low current densities, the STTs should compete against disorders in ferromagnetic nanowires but the nature of the competition remains poorly understood. By achieving two-dimensional contour maps of DW speed with respect to current density and magnetic field, here we visualize unambiguously distinct roles of the two STTs-adiabatic and nonadiabatic-in scaling behaviour of DW dynamics arising from the competition. The contour maps are in excellent agreement with predictions of a generalized scaling theory, and all experimental data collapse onto a single curve. This result indicates that the adiabatic STT becomes dominant for large current densities, whereas the nonadiabatic STT-playing the same role as a magnetic field-subsists at low current densities required to make emerging magnetic nanodevices practical.
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Submitted 7 June, 2010;
originally announced June 2010.
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Universality between current- and field-driven domain wall dynamics in ferromagnetic nanowires
Authors:
Jae-Chul Lee,
Kab-Jin Kim,
Jisu Ryu,
Kyoung-Woong Moon,
Sang-Jun Yun,
Gi-Hong Gim,
Kang-Soo Lee,
Kyung-Ho Shin,
Hyun-Woo Lee,
Sug-Bong Choe
Abstract:
Spin-polarized electric current exerts torque on local magnetic spins, resulting in magnetic domain-wall (DW) motion in ferromagnetic nanowires. Such current-driven DW motion opens great opportunities toward next-generation magnetic devices controlled by current instead of magnetic field. However, the nature of the current-driven DW motion--considered qualitatively different from magnetic-field-…
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Spin-polarized electric current exerts torque on local magnetic spins, resulting in magnetic domain-wall (DW) motion in ferromagnetic nanowires. Such current-driven DW motion opens great opportunities toward next-generation magnetic devices controlled by current instead of magnetic field. However, the nature of the current-driven DW motion--considered qualitatively different from magnetic-field-driven DW motion--remains yet unclear mainly due to the painfully high operation current densities J_OP, which introduce uncontrollable experimental artefacts with serious Joule heating. It is also crucial to reduce J_OP for practical device operation. By use of metallic Pt/Co/Pt nanowires with perpendicular magnetic anisotropy, here we demonstrate DW motion at current densities down to the range of 10^9 A/m^2--two orders smaller than existing reports. Surprisingly the current-driven motion exhibits a scaling behaviour identical to the field-driven motion and thus, belongs to the same universality class despite their qualitative differences. Moreover all DW motions driven by either current or field (or by both) collapse onto a single curve, signalling the unification of the two driving mechanisms. The unified law manifests non-vanishing current efficiency at low current densities down to the practical level, applicable to emerging magnetic nanodevices.
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Submitted 8 June, 2010; v1 submitted 27 December, 2009;
originally announced December 2009.
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Significant Reduction of the Microwave Surface Resistance of MgB2 Films by Surface Ion Milling
Authors:
Sang Young Lee,
J. H. Lee,
Jung Hun Lee,
J. S. Ryu,
J. Lim,
S. H. Moon,
H. N. Lee,
H. G. Kim,
B. Oh
Abstract:
The microwave surface resistance Rs of MgB2 films with the zero-resistance temperature of - 39 K was measured at 8.0 - 8.5 GHz. The MgB2 films were prepared by deposition of boron films on c-cut sapphire, followed by annealing in a vaporized magnesium environment. The Rs appeared significantly reduced by ion milling of the as-grown MgB2 film surface, with the observed Rs of ~ 0.8 mohm at 24 K fo…
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The microwave surface resistance Rs of MgB2 films with the zero-resistance temperature of - 39 K was measured at 8.0 - 8.5 GHz. The MgB2 films were prepared by deposition of boron films on c-cut sapphire, followed by annealing in a vaporized magnesium environment. The Rs appeared significantly reduced by ion milling of the as-grown MgB2 film surface, with the observed Rs of ~ 0.8 mohm at 24 K for an ion-milled MgB2 film as small as 1/15 of the value for the corresponding as-grown MgB2 film. The reduced Rs of the ion-milled MgB2 films is attributed to the effects of the Mg-rich metallic layer existing at the surfaces of the as-grown MgB2 films.
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Submitted 12 November, 2001; v1 submitted 16 May, 2001;
originally announced May 2001.