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Discovery of a Highly Anisotropic Type-II Ferromagnetic Weyl State Exhibiting a 3D Quantum Hall Effect
Authors:
Yingdong Guan,
Abhinava Chatterjee,
Trace Bivens,
Seng Huat Lee,
Asuka Honma,
Hirofumi Oka,
Jorge D Vega Bazantes,
Ruiqi Zhang,
David Graf,
Jianwei Sun,
Seigo Souma,
Takafumi Sato,
Yong P. Chen,
Yuanxi Wang,
Chaoxing Liu,
Zhiqiang Mao
Abstract:
Topological semimetals, particularly Weyl semimetals (WSMs), are crucial platforms for exploring emergent quantum phenomena due to their unique electronic structures and potential to transition into various topological phases. In this study, we report the discovery of a ferromagnetic (FM) type-II WSM in Mn(Bi1-xSbx)4Te7, which exhibits a remarkable three-dimensional (3D) quantum Hall effect (QHE).…
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Topological semimetals, particularly Weyl semimetals (WSMs), are crucial platforms for exploring emergent quantum phenomena due to their unique electronic structures and potential to transition into various topological phases. In this study, we report the discovery of a ferromagnetic (FM) type-II WSM in Mn(Bi1-xSbx)4Te7, which exhibits a remarkable three-dimensional (3D) quantum Hall effect (QHE). By precisely tuning the chemical potential through Sb doping, we obtained samples with the Fermi level near the charge neutrality point for x = ~ 0.27. This was confirmed by spectroscopy measurements (ARPES and STS), and these samples showed strong quantum oscillations along with a key transport signature of a Weyl state - chiral anomaly, and Fermi surface reconstruction driven by FM ordering. Our theoretical analysis indicates that this Weyl state evolves from a parent nodal ring state, where higher-order k-terms split the nodal line into type-II Weyl nodes. The Weyl state exhibits significant anisotropy, characterized by a pronounced reduction in Fermi velocity along the kz-axis, likely accounting for the observed 3D QHE. These results not only highlight the exceptional tunability of the Mn(Bi1-xSbx)4Te7 system, where precise control of the chemical potential and magnetic properties opens access to novel quantum phases, but also advance the understanding of FM WSMs.
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Submitted 10 March, 2025;
originally announced March 2025.
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Pauli spin blockade at room temperature in double-quantum-dot tunneling through individual deep dopants in silicon
Authors:
Yoshisuke Ban,
Kimihiko Kato,
Shota Iizuka,
Hiroshi Oka,
Shigenori Murakami,
Koji Ishibashi,
Satoshi Moriyama,
Takahiro Mori,
Keiji Ono
Abstract:
Pauli spin blockade (PSB) is a spin-dependent charge transport process that typically appears in double quantum dot (QD) devices and is employed in fundamental research on single spins in nanostructures to read out semiconductor qubits. The operating temperature of PSB is limited by that of the QDs and remains below 10 K, limiting wide application development. Herein, we confirm that a single deep…
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Pauli spin blockade (PSB) is a spin-dependent charge transport process that typically appears in double quantum dot (QD) devices and is employed in fundamental research on single spins in nanostructures to read out semiconductor qubits. The operating temperature of PSB is limited by that of the QDs and remains below 10 K, limiting wide application development. Herein, we confirm that a single deep dopant in the channel of a silicon field effect transistor functions as a room-temperature QD; consequently, transport through two different deep dopants exhibits PSB up to room temperature. The characteristic magnetoconductance provides a means to identify PSB and enables the PSB device to function as a magnetic sensor with a sensitivity below geomagnetic field. Lifting in PSB caused by magnetic resonance (50 K) and Rabi oscillations (10 K) are also observed. Further development of this unique system may lead to room-temperature quantum technologies based on silicon technology.
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Submitted 24 July, 2025; v1 submitted 17 September, 2024;
originally announced September 2024.
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Charge order with unusual star-of-David lattice in monolayer NbTe2
Authors:
Taiki Taguchi,
Katsuaki Sugawara,
Hirofumi Oka,
Tappei Kawakami,
Yasuaki Saruta,
Takemi Kato,
Kosuke Nakayama,
Seigo Souma,
Takashi Takahashi,
Tomoteru Fukumura,
Takafumi Sato
Abstract:
Interplay between fermiology and electron correlation is crucial for realizing exotic quantum phases. Transition-metal dichalcogenide (TMD) 1T-TaS2 has sparked a tremendous attention owing to its unique Mott-insulating phase coexisting with the charge-density wave (CDW). However, how the fermiology and electron correlation are associated with such properties has yet to be claried. Here we demonstr…
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Interplay between fermiology and electron correlation is crucial for realizing exotic quantum phases. Transition-metal dichalcogenide (TMD) 1T-TaS2 has sparked a tremendous attention owing to its unique Mott-insulating phase coexisting with the charge-density wave (CDW). However, how the fermiology and electron correlation are associated with such properties has yet to be claried. Here we demonstrate that monolayer 1T-NbTe2 is a new class of two-dimensional TMD which has the star-of-David lattice similarly to bulk TaS2 and isostructural monolayer NbSe2, but exhibits a metallic ground state with an unusual lattice periodicity root19xroot19 characterized by the sparsely occupied star-of-David lattice. By using angle-resolved photoemission and scanning-tunneling spectroscopies in combination with first-principles band-structure calculations, we found that the hidden Fermi-surface nesting and associated CDW formation are a primary cause to realize this unique correlated metallic state with no signature of Mott gap. The present result points to a vital role of underlying fermiology to characterize the Mott phase of TMDs.
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Submitted 24 December, 2022;
originally announced December 2022.
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Robust charge-density wave strengthened by electron correlations in monolayer 1T-TaSe2 and 1T-NbSe2
Authors:
Yuki Nakata,
Katsuaki Sugawara,
Ashish Chainani,
Hirofumi Oka,
Changhua Bao,
Shaohua Zhou,
Pei-Yu Chuang,
Cheng-Maw Cheng,
Tappei Kawakami,
Yasuaki Saruta,
Tomoteru Fukumura,
Shuyun Zhou,
Takashi Takahashi,
Takafumi Sato
Abstract:
Combination of low-dimensionality and electron correlation is vital for exotic quantum phenomena such as the Mott-insulating phase and high-temperature superconductivity. Transition-metal dichalcogenide (TMD) 1T-TaS2 has evoked great interest owing to its unique nonmagnetic Mott-insulator nature coupled with a charge-density-wave (CDW). To functionalize such a complex phase, it is essential to enh…
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Combination of low-dimensionality and electron correlation is vital for exotic quantum phenomena such as the Mott-insulating phase and high-temperature superconductivity. Transition-metal dichalcogenide (TMD) 1T-TaS2 has evoked great interest owing to its unique nonmagnetic Mott-insulator nature coupled with a charge-density-wave (CDW). To functionalize such a complex phase, it is essential to enhance the CDW-Mott transition temperature TCDW-Mott, whereas this was difficult for bulk TMDs with TCDW-Mott < 200 K. Here we report a strong-coupling 2D CDW-Mott phase with a transition temperature onset of ~530 K in monolayer 1T-TaSe2. Furthermore, the electron correlation derived lower Hubbard band survives under external perturbations such as carrier doping and photoexcitation, in contrast to the bulk counterpart. The enhanced Mott-Hubbard and CDW gaps for monolayer TaSe2 compared to NbSe2, originating in the lattice distortion assisted by strengthened correlations and disappearance of interlayer hopping, suggest stabilization of a likely nonmagnetic CDW-Mott insulator phase well above the room temperature. The present result lays the foundation for realizing monolayer CDW-Mott insulator based devices operating at room temperature.
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Submitted 8 October, 2021;
originally announced October 2021.
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Topological invariants in two-dimensional quasicrystals
Authors:
Mikito Koshino,
Hiroki Oka
Abstract:
We study the topological characterization of the energy gaps in general two-dimensional quasiperiodic systems consisting of multiple periodicities, represented by twisted two-dimensional materials. We show that every single gap is uniquely characterized by a set of integers, which quantize the area of the momentum space in units of multiple Brillouin zones defined in the redundant periodicities. T…
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We study the topological characterization of the energy gaps in general two-dimensional quasiperiodic systems consisting of multiple periodicities, represented by twisted two-dimensional materials. We show that every single gap is uniquely characterized by a set of integers, which quantize the area of the momentum space in units of multiple Brillouin zones defined in the redundant periodicities. These integers can be expressed as the second Chern numbers, by considering an adiabatic charge pumping under a relative slide of different periodicities, and using a formal relationship to the four-dimensional quantum Hall effect. The integers are independent of commensurability of the multiple periods, and invariant under arbitrary continuous deformations such as a relative rotation of twisted periodicities.
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Submitted 27 September, 2021;
originally announced September 2021.
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Fractal energy gaps and topological invariants in hBN/Graphene/hBN double moiré systems
Authors:
Hiroki Oka,
Mikito Koshino
Abstract:
We calculate the electronic structure in quasiperiodic double-moiré systems of graphene sandwiched by hexagonal boron nitride, and identify the topological invariants of energy gaps. We find that the electronic spectrum contains a number of minigaps, and they exhibit a recursive fractal structure similar to the Hofstadter butterfly when plotted against the twist angle. Each of the energy gaps can…
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We calculate the electronic structure in quasiperiodic double-moiré systems of graphene sandwiched by hexagonal boron nitride, and identify the topological invariants of energy gaps. We find that the electronic spectrum contains a number of minigaps, and they exhibit a recursive fractal structure similar to the Hofstadter butterfly when plotted against the twist angle. Each of the energy gaps can be characterized by a set of integers, which are associated with an area in the momentum space. The corresponding area is geometrically interpreted as a quasi Brillouin zone, which is a polygon enclosed by multiple Bragg planes of the composite periods and can be uniquely specified by the plain wave projection in the weak potential limit.
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Submitted 11 May, 2021;
originally announced May 2021.