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Probing Local Variations of Superconductivity on the Surface of Ba(Fe1-xCox)2As2 Single Crystals
Authors:
T. -H. Kim,
R. Jin,
L. R. Walker,
J. Y. Howe,
M. H. Pan,
J. F. Wendelken,
J. R. Thompson,
A. S. Sefat,
M. A. McGuire,
B. C. Sales,
D. Mandrus,
A. P. Li
Abstract:
The spatially resolved electrical transport properties have been studied on the surface of optimally-doped superconducting Ba(Fe1-xCox)2As2 single crystal by using a four-probe scanning tunneling microscopy. While some non-uniform contrast appears near the edge of the cleaved crystal, the scanning electron microscopy (SEM) reveals mostly uniform contrast. For the regions that showed uniform SEM…
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The spatially resolved electrical transport properties have been studied on the surface of optimally-doped superconducting Ba(Fe1-xCox)2As2 single crystal by using a four-probe scanning tunneling microscopy. While some non-uniform contrast appears near the edge of the cleaved crystal, the scanning electron microscopy (SEM) reveals mostly uniform contrast. For the regions that showed uniform SEM contrast, a sharp superconducting transition at TC = 22.1 K has been observed with a transition width (delta)Tc = 0.2 K. In the non-uniform contrast region, TC is found to vary between 19.6 and 22.2 K with (delta)Tc from 0.3 to 3.2 K. The wavelength dispersive x-ray spectroscopy reveals that Co concentration remains 7.72% in the uniform region, but changes between 7.38% and 7.62% in the non-uniform region. Thus the variations of superconductivity are associated with local compositional change.
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Submitted 1 March, 2010;
originally announced March 2010.
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Surface Geometric and Electronic Structure of BaFe2As2(001)
Authors:
V. B. Nascimento,
Ang Li,
Dilushan R. Jayasundara,
Yi Xuan,
Jared O'Neal,
Shuheng Pan,
T. Y. Chien,
Biao Hu,
X. B. He,
Guorong Li,
A. S. Sefat,
M. A. McGuire,
B. C. Sales,
D. Mandrus,
M. H. Pan,
Jiandi Zhang,
R. Jin,
E. W. Plummer
Abstract:
BaFe2As2 exhibits properties characteristic of the parent compounds of the newly discovered iron (Fe)-based high-TC superconductors. By combining the real space imaging of scanning tunneling microscopy/spectroscopy (STM/S) with momentum space quantitative Low Energy Electron Diffraction (LEED) we have identified the surface plane of cleaved BaFe2As2 crystals as the As terminated Fe-As layer - th…
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BaFe2As2 exhibits properties characteristic of the parent compounds of the newly discovered iron (Fe)-based high-TC superconductors. By combining the real space imaging of scanning tunneling microscopy/spectroscopy (STM/S) with momentum space quantitative Low Energy Electron Diffraction (LEED) we have identified the surface plane of cleaved BaFe2As2 crystals as the As terminated Fe-As layer - the plane where superconductivity occurs. LEED and STM/S data on the BaFe2As2(001) surface indicate an ordered arsenic (As) - terminated metallic surface without reconstruction or lattice distortion. It is surprising that the STM images the different Fe-As orbitals associated with the orthorhombic structure, not the As atoms in the surface plane.
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Submitted 19 May, 2009;
originally announced May 2009.
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Temperature and Spatial Dependence of the Superconducting and Pseudogap of NdFeAsO0.86F0.14
Authors:
M. H. Pan,
X. B. He,
G. R. Li,
J. F. Wendelken,
R. Jin,
A. S. Sefat,
M. A. McGuire,
B. C. Sales,
D. Mandrus,
E. W. Plummer
Abstract:
The discovery of superconductivity with a critical temperature exceeding 55 K in the iron-oxypnictides and related compounds has quite suddenly given the community a new set of materials - breaking the tyranny of copper. This new class of materials raises fundamental questions related to the origin of the electron pairing in the superconducting state and to the similarity to superconductivity in…
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The discovery of superconductivity with a critical temperature exceeding 55 K in the iron-oxypnictides and related compounds has quite suddenly given the community a new set of materials - breaking the tyranny of copper. This new class of materials raises fundamental questions related to the origin of the electron pairing in the superconducting state and to the similarity to superconductivity in the cuprates. Here, we report spatially resolved measurements using scanning tunneling microscopy/spectroscopy (STM/STS) of the newly discovered iron-based layered superconductor NdFeAsO0.86F0.14 (Tc = 48 K) as a function of temperature. The tunneling spectra at 17 K show a suppression of spectral intensity within +/- 10 meV, indicative of the opening of the superconducting gap (SG). Below Tc, the sample exhibits two characteristic gaps - a large one (18 meV) and a small one (9 meV) - existing in different spatial locations. Both gaps are closed above Tc at the bulk Tc, but only the small gap can be fitted with a superconducting gap function. This gap displays a BCS - like order parameter. Above Tc, at the same location where the small gap was observed, a pseudogap (PG) opens abruptly at a temperature just above Tc and closes at 120 K. In contrast to the cuprates, the SG and PG have competing order parameters.
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Submitted 6 August, 2008;
originally announced August 2008.