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Direct demonstration of electric chirality control in a helimagnetic YMn$_6$Sn$_6$ by spin-polarized neutron scattering
Authors:
Hidetoshi Masuda,
Yutaro Yanagisawa,
Kazuki Ohishi,
Yusuke Nambu,
Yoichi Nii,
Yoshinori Onose
Abstract:
The spiral handedness of magnetic moments, referred to as chirality, gives rise to emergent electromagnetic phenomena in helimagnets. In insulating helimagnets, known as multiferroics, the cycloidal spin structure induces electric polarization by utilizing the inverse Dzyaloshinskii-Moriya mechanism. Spin-polarized neutron diffraction experiments, which directly probe circular spin arrangements, c…
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The spiral handedness of magnetic moments, referred to as chirality, gives rise to emergent electromagnetic phenomena in helimagnets. In insulating helimagnets, known as multiferroics, the cycloidal spin structure induces electric polarization by utilizing the inverse Dzyaloshinskii-Moriya mechanism. Spin-polarized neutron diffraction experiments, which directly probe circular spin arrangements, clearly demonstrated that an electric field controlled the chirality in multiferroic helimagnets. On the other hand, it was unclear until recently how the chirality could be controlled in metallic helimagnets where a large electric field cannot be applied, while the chirality control technique in metallic helimagnets should enable the exploration of chirality-dependent spintronic functionalities. Recently, Jiang et al. succeeded in controlling the chirality of a spiral structure by the simultaneous application of a magnetic field and electric current in a metallic helimagnet, utilizing the nonreciprocal electronic transport as an indirect probe of chirality, highlighting the need for a neutron diffraction experiment that directly probes the chirality. Here, we directly demonstrate the chirality control in a metallic helimagnet YMn$_6$Sn$_6$ by means of spin-polarized neutron diffraction, which should give rise to a firm basis for the development of future helimagnetic spintronics.
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Submitted 5 December, 2025;
originally announced December 2025.
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Electric Current Control of Helimagnetic Chirality from a Multidomain State in the Helimagnet MnAu$_2$
Authors:
Yuta Kimoto,
Hidetoshi Masuda,
Jun-ichiro Ohe,
Shoya Sakamoto,
Takeshi Seki,
Yoshinori Onose
Abstract:
In this paper, we study the domain wall dynamics under electric current in the helimagnet MnAu$_2$. We have found that the threshold electric current of the transition from a multidomain state to a single-chiral domain state in a magnetic field is much lower than that of chirality reversal from a single-chiral domain within certain ranges of temperature and magnetic field. The chirality after the…
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In this paper, we study the domain wall dynamics under electric current in the helimagnet MnAu$_2$. We have found that the threshold electric current of the transition from a multidomain state to a single-chiral domain state in a magnetic field is much lower than that of chirality reversal from a single-chiral domain within certain ranges of temperature and magnetic field. The chirality after the transition depends on whether the magnetic field and electric current were parallel or antiparallel. Numerical calculations based on the Landau-Lifshitz-Gilbert equation reproduced the experimental observations. These results indicate that the domain walls are highly mobile in the helimagnet.
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Submitted 9 June, 2026; v1 submitted 26 November, 2025;
originally announced November 2025.
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Magnetic excitations in the noncentrosymmetric magnet Sr2MnSi2O7
Authors:
Masahiro Kawamata,
Xiaoqi Pang,
Hiroshi Murakawa,
Seiko Ohira-Kawamura,
Kenji Nakajima,
Hidetoshi Masuda,
Masaki Fujita,
Noriaki Hanasaki,
Yoshinori Onose,
Yusuke Nambu
Abstract:
Magnetic excitations in the noncentrosymmetric magnet Sr$_2$MnSi$_2$O$_7$ were investigated through inelastic neutron scattering measurements. Major magnetic excitations are limited up to the energy transfer of 0.5 meV, and two magnon branches under zero magnetic field were well explained in the framework of linear spin-wave theory. The magnitudes of the square-lattice in-plane and inter-plane nea…
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Magnetic excitations in the noncentrosymmetric magnet Sr$_2$MnSi$_2$O$_7$ were investigated through inelastic neutron scattering measurements. Major magnetic excitations are limited up to the energy transfer of 0.5 meV, and two magnon branches under zero magnetic field were well explained in the framework of linear spin-wave theory. The magnitudes of the square-lattice in-plane and inter-plane nearest-neighbor interactions, spin anisotropy term, and the Dzyaloshinskii-Moriya interaction are respectively estimated to be $J_1=45.54(5)$ $μ$eV, $J_2=0.52(1)$ $μ$eV, $Λ=4.98(11)$ $μ$eV, $D_{xy}=0.02(9)$ $μ$eV, and $D_z=4.10(1)$ $μ$eV, and calculations using these parameters reproduce experimental data quite well. Sr$_2$MnSi$_2$O$_7$ appears to have the smallest energy scale among the melilite-type compounds, and the small $J_2/J_1=0.0114(2)$ indicates the sufficient two-dimensionality.
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Submitted 30 October, 2024;
originally announced October 2024.
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Magnetic structure of the noncentrosymmetric magnet Sr2MnSi2O7 through irreducible representation and magnetic space group analyses
Authors:
Y. Nambu,
M. Kawamata,
X. Pang,
H. Murakawa,
M. Avdeev,
H. Kimura,
H. Masuda,
N. Hanasaki,
Y. Onose
Abstract:
Magnetic structures of the noncentrosymmetric magnet Sr$_2$MnSi$_2$O$_7$ were examined through neutron diffraction for powder and single-crystalline samples, as well as magnetometry measurements. All allowed magnetic structures under the space group $P\bar{4}2_1 m$ with the magnetic wavevector $\vec{q}_{\rm m}=(0,0,1/2)$~r.l.u., were analysed via irreducible representation and magnetic space group…
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Magnetic structures of the noncentrosymmetric magnet Sr$_2$MnSi$_2$O$_7$ were examined through neutron diffraction for powder and single-crystalline samples, as well as magnetometry measurements. All allowed magnetic structures under the space group $P\bar{4}2_1 m$ with the magnetic wavevector $\vec{q}_{\rm m}=(0,0,1/2)$~r.l.u., were analysed via irreducible representation and magnetic space group approaches. The compound is refined to have in-plane magnetic moments within the magnetic space group $Cmc2_1.1^{\prime}_c$ (\#36.177) under zero field, which can be altered to $P2_1 2_1 2_1.1^{\prime}_c$ (\#19.28) above $μ_0 H=0.067(5)$~T to align induced weak-ferromagnetic components within one layer on the $ab$-plane. All refined parameters are provided following the recent framework based upon the magnetic space group, which better conveys when exchanging crystallographic information for commensurate magnetic structures.
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Submitted 5 October, 2024;
originally announced October 2024.
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Observation of nonreciprocal diffraction of surface acoustic wave
Authors:
Yoichi Nii,
Kei Yamamoto,
Masaki Kanno,
Sadamichi Maekawa,
Yoshinori Onose
Abstract:
Rectification phenomenon caused by the simultaneous breaking of time reversal and spatial inversion symmetries has been extended to a wide range of (quasi)particles and waves; however, the nonreciprocal diffraction, which is the imbalance of upward and downward deflections, was previously observed only for photons and remained to be extended to other (quasi)particles. In this study, we present evi…
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Rectification phenomenon caused by the simultaneous breaking of time reversal and spatial inversion symmetries has been extended to a wide range of (quasi)particles and waves; however, the nonreciprocal diffraction, which is the imbalance of upward and downward deflections, was previously observed only for photons and remained to be extended to other (quasi)particles. In this study, we present evidence of the nonreciprocal diffraction of surface acoustic wave (SAW) utilizing a magnetoelastic grating on a SAW device. Asymmetric diffraction intensities were observed when the ferromagnetic resonance was acoustically excited. Based on a theoretical model, we attribute the microscopic origin of this phenomenon to the resonant scattering involving ferromagnetic resonance excitations. The novel property may pave an avenue to further development of SAW devices for various purposes, including microwave communications and quantum engineering applications.
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Submitted 29 May, 2024;
originally announced May 2024.
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A high-temperature multiferroic Tb$_2$(MoO$_4$)$_3$
Authors:
Shimon Tajima,
Hidetoshi Masuda,
Yoichi Nii,
Shojiro Kimura,
Yoshinori Onose
Abstract:
Magnetoelectric mutual control in multiferroics, which is the electric control of magnetization, or reciprocally the magnetic control of polarization has attracted much attention because of its possible applications to spintronic devices, multi-bit memories, and so on. While the required working temperature for the practical application is much higher than room temperature, which ensures stable fu…
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Magnetoelectric mutual control in multiferroics, which is the electric control of magnetization, or reciprocally the magnetic control of polarization has attracted much attention because of its possible applications to spintronic devices, multi-bit memories, and so on. While the required working temperature for the practical application is much higher than room temperature, which ensures stable functionality at room temperature, the reported working temperatures were at most around room temperature. Here, we demonstrated magnetic control of ferroelectric polarization at 432 K in ferroelectric and ferroelastic Tb$_2$(MoO$_4$)$_3$, in which the polarity of ferroelectric polarization is coupled to the orthorhombic strain below the transition temperature 432 K. The paramagnetic but strongly magnetoelastic Tb$^{3+}$ magnetic moments enable the magnetic control of ferroelectric and ferroelastic domains; the ferroelectric polarization is controlled depending on whether the magnetic field is applied along [110] or [$\bar{1}$10]. This result may pave a new avenue for designing high-temperature multiferroics.
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Submitted 9 May, 2024;
originally announced May 2024.
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Band-asymmetry-driven nonreciprocal electronic transport in a helimagnetic semimetal α-EuP$_3$
Authors:
Alex Hiro Mayo,
Darius-Alexandru Deaconu,
Hidetoshi Masuda,
Yoichi Nii,
Hidefumi Takahashi,
Rodion Vladimirovich Belosludov,
Shintaro Ishiwata,
Mohammad Saeed Bahramy,
Yoshinori Onose
Abstract:
Chiral magnetic textures give rise to unconventional magnetotransport phenomena such as the topological Hall effect and nonreciprocal electronic transport. While the correspondence between real-space magnetic topology/symmetry and such transport phenomena has been well established, a microscopic understanding based on the spin-dependent band structure in momentum space remains elusive. Here we dem…
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Chiral magnetic textures give rise to unconventional magnetotransport phenomena such as the topological Hall effect and nonreciprocal electronic transport. While the correspondence between real-space magnetic topology/symmetry and such transport phenomena has been well established, a microscopic understanding based on the spin-dependent band structure in momentum space remains elusive. Here we demonstrate how a chiral magnetic structure in real space introduces an asymmetry in the electronic band structure and triggers a nonreciprocal electronic transport in a centrosymmetric helimagnet α-EuP$_3$. The magnetic structure of α-EuP$_3$ is highly tunable by a magnetic field and closely coupled to its semi-metallic electronic band structure, enabling a systematic study across chiral and achiral magnetic phases on the correspondence between nonreciprocal transport and electronic band asymmetry. Our findings reveal how a microscopic change in the magnetic configuration of charge carriers can lead to nonreciprocal electronic transport, paving the way for designing chiral magnets with desirable properties.
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Submitted 22 April, 2024;
originally announced April 2024.
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Current-induced sliding motion in a helimagnet MnAu$_2$
Authors:
Yuta Kimoto,
Hidetoshi Masuda,
Takeshi Seki,
Yoichi Nii,
Jun-ichiro Ohe,
Yusuke Nambu,
Yoshinori Onose
Abstract:
We found signatures of current-induced sliding motion in helimagnetic $\mathrm{Mn}\mathrm{Au}_2$ thin films. An abrupt change in differential resistivity occurred at a threshold bias current in the helimagnetic state, whereas it was absent in the induced ferromagnetic state. Broadband voltage noise also emerged above the threshold current in the helimagnetic state. Based on the similarity to canon…
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We found signatures of current-induced sliding motion in helimagnetic $\mathrm{Mn}\mathrm{Au}_2$ thin films. An abrupt change in differential resistivity occurred at a threshold bias current in the helimagnetic state, whereas it was absent in the induced ferromagnetic state. Broadband voltage noise also emerged above the threshold current in the helimagnetic state. Based on the similarity to canonical charge/spin density wave systems, we ascribed the origin of these phenomena to the sliding motion of the helimagnetic structure.
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Submitted 13 November, 2024; v1 submitted 29 February, 2024;
originally announced March 2024.
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Chirality-dependent spin current generation in a helimagnet: zero-field probe of chirality
Authors:
Hidetoshi Masuda,
Takeshi Seki,
Jun-ichiro Ohe,
Yoichi Nii,
Koki Takanashi,
Yoshinori Onose
Abstract:
In a magnetic texture, the spin of a conduction electron is forced to be aligned to the localized moment. As a result, the topology of the magnetic texture affects the electron dynamics in nontrivial ways. A representative example is the topological Hall effect in noncoplanar spin textures with finite spin chirality. While propagating in the noncoplanar spin texture, electrons acquire Berry phase,…
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In a magnetic texture, the spin of a conduction electron is forced to be aligned to the localized moment. As a result, the topology of the magnetic texture affects the electron dynamics in nontrivial ways. A representative example is the topological Hall effect in noncoplanar spin textures with finite spin chirality. While propagating in the noncoplanar spin texture, electrons acquire Berry phase, and their motion is deflected as if they were in a magnetic field. Here, we report a distinct Berry phase effect in a coplanar helimagnet: the spin moment of the conduction electron is polarized under electric currents depending on the chirality of the helimagnet. The accumulated spin polarization works as a source of spin current, and the chirality can be detected by the inverse spin Hall mechanism. The functionality allows us to read out the chirality without magnetic fields, and therefore paves the way to future helimagnet-based spintronics.
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Submitted 21 December, 2022;
originally announced December 2022.
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Microwave impedance microscopy imaging of acoustic topological edge mode on a patterned substrate
Authors:
Yoichi Nii,
Yoshinori Onose
Abstract:
We have studied acoustic topological edge modes in a honeycomb phononic crystal composed of metallic nano-pillars on a LiNbO$_3$ substrate. Acoustic band calculations show that the topological surface acoustic wave (SAW) mode inhabits the edge of the honeycomb phononic crystal in spite of the hybridization with the internal acoustic modes of the substrate. Pulse-type microwave impedance microscopy…
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We have studied acoustic topological edge modes in a honeycomb phononic crystal composed of metallic nano-pillars on a LiNbO$_3$ substrate. Acoustic band calculations show that the topological surface acoustic wave (SAW) mode inhabits the edge of the honeycomb phononic crystal in spite of the hybridization with the internal acoustic modes of the substrate. Pulse-type microwave impedance microscopy realized clear visualization of the gigahertz topological edge mode between two mutually inverted topological phononic crystals. A frequency-dependent image showed that the edge mode evolves as the bulk SAW modes are suppressed owing to the energy gap formation, consistent with the topological nature. The realization of a topological waveguide in a simple pillar structure on a substrate might pave a new path to the development of topological SAW devices.
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Submitted 5 June, 2022;
originally announced June 2022.
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Room-temperature chirality switching in a helimagnetic thin film
Authors:
Hidetoshi Masuda,
Takeshi Seki,
Yoichi Nii,
Hiroto Masuda,
Koki Takanashi,
Yoshinori Onose
Abstract:
Helimagnetic structures, in which the magnetic moments are spirally ordered, host an internal degree of freedom called chirality (or helicity) corresponding to the handedness of the helix. The chirality seems quite robust against disturbances and is therefore promising for next-generation magnetic memory. While the chirality control was recently achieved by the magnetic field sweep with the applic…
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Helimagnetic structures, in which the magnetic moments are spirally ordered, host an internal degree of freedom called chirality (or helicity) corresponding to the handedness of the helix. The chirality seems quite robust against disturbances and is therefore promising for next-generation magnetic memory. While the chirality control was recently achieved by the magnetic field sweep with the application of an electric current at low temperature in a conducting helimagnet, problems such as low working temperature and cumbersome control sequence have to be solved in practical applications. Another issue is the thin film fabrication that enables the development of spintronic devices based on helimagnets. Here we show chirality switching by electric current pulses at room temperature in a thin-film MnAu$_2$ helimagnetic conductor. The result demonstrates the feasibility of helimagnet-based spintronics that can overcome all the above problems.
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Submitted 25 May, 2022;
originally announced May 2022.
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Elastic study of electric quadrupolar correlation in the paramagnetic state of a frustrated quantum magnet $\rm Tb_{2+\it δ}Ti_{2-\it δ}O_7$
Authors:
Y. Nii,
Y. Hirokane,
S. Nakamura,
S. Kimura,
Y. Tomioka,
T. Nojima,
Y. Onose
Abstract:
Electric quadrupolar state in a frustrated quantum magnet $\rm Tb_{2+\it δ}Ti_{2-\it δ}O_7$ has been studied by means of ultrasonic and magnetostriction measurements. A single crystal showed elastic anomaly at about 0.4 K, manifesting a long-range quadrupole ordering. By investigating anisotropy of the magnetoelastic responses, we found a crossover temperature for the strongly correlated quadrupol…
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Electric quadrupolar state in a frustrated quantum magnet $\rm Tb_{2+\it δ}Ti_{2-\it δ}O_7$ has been studied by means of ultrasonic and magnetostriction measurements. A single crystal showed elastic anomaly at about 0.4 K, manifesting a long-range quadrupole ordering. By investigating anisotropy of the magnetoelastic responses, we found a crossover temperature for the strongly correlated quadrupole state, below which the experimental data of elastic constant and magnetostriction become qualitatively different from their calculations based on a single-ion model. We suppose that relatively high onset temperature of the quadrupole correlation compared with the transition temperature is ascribed to the geometrical frustration effect, and this correlated state seems to be responsible for the unusual properties in the paramagentic state of $\rm Tb_2Ti_2O_7$.
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Submitted 24 September, 2021;
originally announced September 2021.
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Chirality memory stored in magnetic domain walls in the ferromagnetic state of MnP
Authors:
N. Jiang,
Y. Nii,
H. Arisawa,
E. Saitoh,
Y. Onose
Abstract:
Chirality in a helimagnetic structure is determined by the sense of magnetic moment rotation. We found that the chiral information did not disappear even after the phase transition to the high-temperature ferromagnetic phase in a helimagnet MnP. The 2nd harmonic resistivity $ρ^{\rm 2f}$, which reflects the breaking down of mirror symmetry, was found to be almost unchanged after heating the sample…
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Chirality in a helimagnetic structure is determined by the sense of magnetic moment rotation. We found that the chiral information did not disappear even after the phase transition to the high-temperature ferromagnetic phase in a helimagnet MnP. The 2nd harmonic resistivity $ρ^{\rm 2f}$, which reflects the breaking down of mirror symmetry, was found to be almost unchanged after heating the sample above the ferromagnetic transition temperature and cooling it back to the helimagnetic state. The application of a magnetic field along the easy axis in the ferromagnetic state quenched the chirality-induced $ρ^{\rm 2f}$. This indicates that the chirality memory effect originated from the ferromagnetic domain walls.
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Submitted 6 October, 2020;
originally announced October 2020.
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Magnetization control by angular momentum transfer from surface acoustic wave to ferromagnetic spin moments
Authors:
R. Sasaki,
Y. Nii,
Y. Onose
Abstract:
The angular momentum interconversion between electron spin and other type of angular momenta is useful to develop new spintronic functionalities. The conversions from the angular momentum of photon and mechanical rotation to ferromagnetic spin moment have been well studied. While the recent studies theoretically suggested circular vibration of atoms works as angular momentum of phonon, the direct…
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The angular momentum interconversion between electron spin and other type of angular momenta is useful to develop new spintronic functionalities. The conversions from the angular momentum of photon and mechanical rotation to ferromagnetic spin moment have been well studied. While the recent studies theoretically suggested circular vibration of atoms works as angular momentum of phonon, the direct experimental demonstration of conversion to spin moments remains to be performed. Here we demonstrate that the phonon angular momentum of surface acoustic wave can control the magnetization of a ferromagnetic Ni film by means of the phononic-to-electronic conversion of angular momentum in Ni/LiNbO$_3$ hybrid device. This result clearly shows the phonon angular momentum is useful to further fictionalize spintronic devices.
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Submitted 7 July, 2020;
originally announced July 2020.
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Nonreciprocal thermal transport in a multiferroic helimagnet
Authors:
Yuji Hirokane,
Yoichi Nii,
Hidetoshi Masuda,
Yoshinori Onose
Abstract:
Breaking of spatial inversion symmetry (SIS) induces unique phenomena in condensed matter. Besides the classic examples such as natural optical activity and piezoelectricity, the spin-orbit interaction further enriches the effect of SIS breaking, as exemplified by the Rashba effect. In particular, by combining this symmetry with magnetic fields or another type of time-reversal symmetry (TRS) break…
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Breaking of spatial inversion symmetry (SIS) induces unique phenomena in condensed matter. Besides the classic examples such as natural optical activity and piezoelectricity, the spin-orbit interaction further enriches the effect of SIS breaking, as exemplified by the Rashba effect. In particular, by combining this symmetry with magnetic fields or another type of time-reversal symmetry (TRS) breaking, noncentrosymmetric materials can be made to exhibit nonreciprocal responses, which are responses that differ for rightward and leftward stimuli. For example, resistivity becomes directionally dependent; that is to say, rectification appears in noncentrosymmetric materials in a magnetic field. However, the effect of SIS breaking on thermal transport remains to be elucidated. Here we show nonreciprocal thermal transport in the multiferroic helimagnet TbMnO3. The longitudinal thermal conductivity depends on whether the thermal current is parallel or antiparallel to the vector product of the electric polarization and magnetization. This phenomenon is thermal rectification that is controllable with external fields in a uniform crystal. This discovery may pave the way to thermal diodes with controllability and scalability.
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Submitted 8 April, 2020;
originally announced April 2020.
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Electric current control of spin helicity in an itinerant helimagnet
Authors:
N. Jiang,
Y. Nii,
H. Arisawa,
E. Saitoh,
Y. Onose
Abstract:
Chirality is breaking of mirror symmetry in matter. In the fields of biology and chemistry, this is particularly important because some of the essential molecules in life such as amino acids and DNA have chirality. It is a long-standing mystery how one of the enantiomers was chosen at the beginning stage of life. The understanding of the emergence of homochirality under some conditions is indispen…
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Chirality is breaking of mirror symmetry in matter. In the fields of biology and chemistry, this is particularly important because some of the essential molecules in life such as amino acids and DNA have chirality. It is a long-standing mystery how one of the enantiomers was chosen at the beginning stage of life. The understanding of the emergence of homochirality under some conditions is indispensable for the study of the origin of life as well as pharmaceutical science. The chirality is also emergent in magnetic structures. The longitudinal helical magnetic structure is the chiral object composed of magnetic moments, in which the ordered direction of the magnetic moment spatially rotates in the plane perpendicular to the propagation vector (Fig. 1a). Since the sense of rotation, which is denoted as helicity, is reversed by any mirror operation, it is corresponding to the chirality. Here we show that the chirality of a longitudinal helical structure can be controlled by the magnetic field and electric current owing to the spin-transfer torque irrelevant to the spin-orbit interaction and probed by electrical magnetochiral effect, which is sensitive to the chiral symmetry breaking, in an itinerant helimagnet MnP. This phenomenon is distinct from the multiferroicity in transverse-type insulating helical magnets, in which the helical plane is parallel to the propagation vector, because the magnetic structure has polar symmetry not chiral one. While the combination of the magnetic field and electric current satisfies the symmetrical rule of external stimulus for the chirality control, the control with them was not reported for any chiral object previously. The present result may pave a new route to the control of chiralities originating from magnetic and atomical arrangements.
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Submitted 3 July, 2019;
originally announced July 2019.
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Surface acoustic wave coupled to magnetic resonance on a multiferroic CuB$_2$O$_4$
Authors:
R. Sasaki,
Y. Nii,
Y. Onose
Abstract:
We observed surface acoustic wave (SAW) propagation on a multiferroic material CuB$_2$O$_4$ with use of two interdigital transducers (IDTs). The period of IDT fingers is as short as 1.6 $μ$m so that the frequency of SAW is 3 GHz, which is comparable with that of magnetic resonance. In antiferromagnetic phase, the SAW excitation intensity varied with the magnitude and direction of the magnetic fiel…
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We observed surface acoustic wave (SAW) propagation on a multiferroic material CuB$_2$O$_4$ with use of two interdigital transducers (IDTs). The period of IDT fingers is as short as 1.6 $μ$m so that the frequency of SAW is 3 GHz, which is comparable with that of magnetic resonance. In antiferromagnetic phase, the SAW excitation intensity varied with the magnitude and direction of the magnetic field, owing to the dynamical coupling between SAWs and antiferromagnetic resonance of CuB$_2$O$_4$. The microscopic mechanism is discussed based on the symmetrically allowed magentoelastic coupling.
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Submitted 5 November, 2018;
originally announced November 2018.
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Designing Rashba-Dresselhaus effect in magnetic insulators
Authors:
Masataka Kawano,
Yoshinori Onose,
Chisa Hotta
Abstract:
One of the major strategies to control magnetism in spintronics is to utilize the coupling between electron spin and its orbital motion. The Rashba and Dresselhaus spin-orbit couplings induce magnetic textures of band electrons called spin momentum locking, which produces a spin torque by the injection of electric current. However, joule heating had been a bottleneck for device applications. Here,…
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One of the major strategies to control magnetism in spintronics is to utilize the coupling between electron spin and its orbital motion. The Rashba and Dresselhaus spin-orbit couplings induce magnetic textures of band electrons called spin momentum locking, which produces a spin torque by the injection of electric current. However, joule heating had been a bottleneck for device applications. Here, we propose a theory to generate further rich spin textures in insulating antiferromagnets with broken spatial inversion symmetry (SIS), which is easily controlled by a small magnetic field. In antiferromagnets, the ordered moments host two species of magnons that serve as internal degrees of freedom in analogy with electron spins. The Dzyaloshinskii-Moriya interaction introduced by the SIS breaking couples the two-magnon-degrees of freedom with the magnon momentum. We present a systematic way to design such texture and to detect it via magnonic spin current for the realization of antiferromagnetic memory.
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Submitted 8 March, 2019; v1 submitted 10 May, 2018;
originally announced May 2018.
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Microwave non-reciprocity of magnon excitations in a non-centrosymmetric antiferromagnet Ba$_2$MnGe$_2$O$_7$
Authors:
Y. Iguchi,
Y. Nii,
M. Kawano,
H. Murakawa,
N. Hanasaki,
Y. Onose
Abstract:
We have investigated the microwave non-reciprocity for a non-centrosymmetric antiferromagnet Ba$_2$MnGe$_2$O$_7$. The magnon modes expected by the conventional spin wave theory for staggered antiferromagnets are certainly observed. The magnitudes of exchange interaction and magnetic anisotropy are obtained by the comparison with the theory. The microwave non-reciprocity is identified for one of th…
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We have investigated the microwave non-reciprocity for a non-centrosymmetric antiferromagnet Ba$_2$MnGe$_2$O$_7$. The magnon modes expected by the conventional spin wave theory for staggered antiferromagnets are certainly observed. The magnitudes of exchange interaction and magnetic anisotropy are obtained by the comparison with the theory. The microwave non-reciprocity is identified for one of these mode. The relative magnitude of microwave non-reciprocity can be explained with use of spin wave theory and Kubo formula.
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Submitted 9 April, 2018;
originally announced April 2018.
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Magnetotransport properties in a noncentrosymmetric itinerant magnet Cr$_{11}$Ge$_{19}$
Authors:
N. Jiang,
Y. Nii,
R. Ishii,
Z. Hiroi,
Y. Onose
Abstract:
We have investigated anomalous Hall effect and magnetoresistance in a noncentrosymmetric itinerant magnet Cr$_{11}$Ge$_{19}$. While the temperature- and magnetic-field-dependent anomalous Hall conductivity is just proportional to the magnetization above 30 K, it is more enhanced in the lower temperature region. The magnitude of negative magnetoresistance begins to increase toward low temperature a…
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We have investigated anomalous Hall effect and magnetoresistance in a noncentrosymmetric itinerant magnet Cr$_{11}$Ge$_{19}$. While the temperature- and magnetic-field-dependent anomalous Hall conductivity is just proportional to the magnetization above 30 K, it is more enhanced in the lower temperature region. The magnitude of negative magnetoresistance begins to increase toward low temperature around 30 K. The anisotropic magnetoresistance emerges at similar temperature. Because there is no anomaly in the temperature dependence of magnetization around 30 K, the origin of these observations in transport properties is ascribed to some electronic structure with the energy scale of 30 K. We speculate this is caused by the spin splitting due to breaking of spatial inversion symmetry.
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Submitted 17 May, 2017;
originally announced May 2017.
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Universality of the helimagnetic transition in cubic chiral magnets: Small angle neutron scattering and neutron spin echo spectroscopy studies of Fe$_{1-x}$Co$_x$Si
Authors:
L. J. Bannenberg,
K. Kakurai,
P. Falus,
E. Lelièvre-Berna,
R. M. Dalgliesh,
C. D. Dewhurst,
F. Qian,
Y. Onose,
Y. Endoh,
Y. Tokura,
C. Pappas
Abstract:
We present a comprehensive Small Angle Neutron Scattering (SANS) and Neutron Spin Echo Spectroscopy (NSE) study of the structural and dynamical aspects of the helimagnetic transition in Fe$_{1-x}$Co$_x$Si with $x$ = 0.30. In contrast to the sharp transition observed in the archetype chiral magnet MnSi, the transition in Fe$_{1-x}$Co$_x$Si is gradual and long-range helimagnetic ordering coexists wi…
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We present a comprehensive Small Angle Neutron Scattering (SANS) and Neutron Spin Echo Spectroscopy (NSE) study of the structural and dynamical aspects of the helimagnetic transition in Fe$_{1-x}$Co$_x$Si with $x$ = 0.30. In contrast to the sharp transition observed in the archetype chiral magnet MnSi, the transition in Fe$_{1-x}$Co$_x$Si is gradual and long-range helimagnetic ordering coexists with short-range correlations over a wide temperature range. The dynamics are more complex than in MnSi and involve long relaxation times with a stretched exponential relaxation which persists even under magnetic field. These results in conjunction with an analysis of the hierarchy of the relevant length scales show that the helimagnetic transition in Fe$_{1-x}$Co$_x$Si differs substantially from the transition in MnSi and question the validity of a universal approach to the helimagnetic transition in chiral magnets.
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Submitted 28 April, 2017; v1 submitted 19 January, 2017;
originally announced January 2017.
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Extended skyrmion lattice scattering and long-time memory in the chiral magnet Fe$_{1-x}$Co$_x$Si
Authors:
L. J. Bannenberg,
K. Kakurai,
F. Qian,
E. Lelièvre-Berna,
C. D. Dewhurst,
Y. Onose,
Y. Endoh,
Y. Tokura,
C. Pappas
Abstract:
Small angle neutron scattering measurements on a bulk single crystal of the doped chiral magnet Fe$_{1-x}$Co$_x$Si with $x$=0.3 reveal a pronounced effect of the magnetic history and cooling rates on the magnetic phase diagram. The extracted phase diagrams are qualitatively different for zero and field cooling and reveal a metastable skyrmion lattice phase outside the A-phase for the latter case.…
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Small angle neutron scattering measurements on a bulk single crystal of the doped chiral magnet Fe$_{1-x}$Co$_x$Si with $x$=0.3 reveal a pronounced effect of the magnetic history and cooling rates on the magnetic phase diagram. The extracted phase diagrams are qualitatively different for zero and field cooling and reveal a metastable skyrmion lattice phase outside the A-phase for the latter case. These thermodynamically metastable skyrmion lattice correlations coexist with the conical phase and can be enhanced by increasing the cooling rate. They appear in a wide region of the phase diagram at temperatures below the $A$-phase but also at fields considerably smaller or higher than the fields required to stabilize the A-phase.
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Submitted 22 October, 2016;
originally announced October 2016.
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Magnetic relaxation phenomena in the Chiral Magnet Fe$_{1-x}$Co$_x$Si: An ac susceptibility study
Authors:
L. J. Bannenberg,
A. L. E. Lefering,
K. Kakurai,
Y. Onose,
Y. Endoh,
Y. Tokura,
C. Pappas
Abstract:
We present a systematic study of the ac susceptibility of the chiral magnet Fe$_{1-x}$Co$_x$Si with $x$ = 0.30 covering four orders of magnitude in frequencies from 0.1 Hz to 1 kHz, with particular emphasis to the pronounced history dependence. Characteristic relaxation times ranging from a few milliseconds to tens of seconds are observed around the skyrmion lattice A-phase, the helical-to-conical…
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We present a systematic study of the ac susceptibility of the chiral magnet Fe$_{1-x}$Co$_x$Si with $x$ = 0.30 covering four orders of magnitude in frequencies from 0.1 Hz to 1 kHz, with particular emphasis to the pronounced history dependence. Characteristic relaxation times ranging from a few milliseconds to tens of seconds are observed around the skyrmion lattice A-phase, the helical-to-conical transition and in a region above $T_C$. The distribution of relaxation frequencies around the A-phase is broad, asymmetric and originates from multiple coexisting relaxation processes. The pronounced dependence of the magnetic phase diagram on the magnetic history and cooling rates as well as the asymmetric frequency dependence and slow dynamics suggest more complicated physical phenomena in Fe$_{0.7}$Co$_{0.3}$Si than in other chiral magnets.
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Submitted 31 October, 2016; v1 submitted 1 August, 2016;
originally announced August 2016.
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Magnetoelectrical control of nonreciprocal microwave response in a multiferroic helimagnet
Authors:
Y. Iguchi,
Y. Nii,
Y. Onose
Abstract:
Control of physical property in terms of external fields is essential for contemporary technologies. The conductance can be controlled by a gate electric field in a field effect transistor, which is a main component of the integrated circuit. Optical phenomena induced by an electric field such as electroluminescence and electrochromism are useful for display and other technologies. Control of micr…
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Control of physical property in terms of external fields is essential for contemporary technologies. The conductance can be controlled by a gate electric field in a field effect transistor, which is a main component of the integrated circuit. Optical phenomena induced by an electric field such as electroluminescence and electrochromism are useful for display and other technologies. Control of microwave propagation seems also imperative for future wireless communication technology. Microwave properties in solids are dominated mostly by magnetic excitations, which cannot be easily controlled by an electric field. One of the solutions for this problem is utilizing magnetically induced ferroelectrics (multiferroics). Here we show that microwave nonreciprocity, which is difference between oppositely propagating microwaves, can be reversed by the external electric field in a multiferroic helimagnet Ba$_2$Mg$_2$Fe$_{12}$O$_{22}$. This result offers a new avenue for the electrical control of microwave properties.
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Submitted 23 July, 2016;
originally announced July 2016.
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Microwave Magneto-Chiral Effect in a Noncentro-symmetric Magnet CuB2O4
Authors:
Y. Nii,
R. Sasaki,
Y. Iguchi,
Y. Onose
Abstract:
We have investigated microwave nonreciprocity in a noncentro-symmetric magnet CuB2O4. We simultaneously observed differently originated nonreciprocities; the classical magnetic dipolar effect and the magneto-chiral (MCh) effect. By rotating magnetic field in a tetragonal plane, we clearly unveil qualitative difference between them. The MCh effect signal reveals chiral transitions from one enantiom…
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We have investigated microwave nonreciprocity in a noncentro-symmetric magnet CuB2O4. We simultaneously observed differently originated nonreciprocities; the classical magnetic dipolar effect and the magneto-chiral (MCh) effect. By rotating magnetic field in a tetragonal plane, we clearly unveil qualitative difference between them. The MCh effect signal reveals chiral transitions from one enantiomer to the other via intermediate achiral state. We show magnetoelectric effect plays an essential role for the emergence of microwave MCh effect.
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Submitted 24 May, 2016;
originally announced May 2016.
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Nonreciprocal propagation of surface acoustic wave in Ni/LiNbO3
Authors:
R. Sasaki,
Y. Nii,
Y. Iguchi,
Y. Onose
Abstract:
We have investigated surface acoustic wave propagation in Ni/LiNbO$_3$ hybrid devices. We have found the absorption and phase velocity are dependent on the sign of wave vector in a device, which indicates the nonreciprocal propagation characteristic of systems with time reversal and spatial inversion simultaneously broken symmetries. The nonreciprocity is reversed by the 180$^\circ$ rotation of ma…
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We have investigated surface acoustic wave propagation in Ni/LiNbO$_3$ hybrid devices. We have found the absorption and phase velocity are dependent on the sign of wave vector in a device, which indicates the nonreciprocal propagation characteristic of systems with time reversal and spatial inversion simultaneously broken symmetries. The nonreciprocity is reversed by the 180$^\circ$ rotation of magnetic field. Nonreciprocity seems largely dependent on the shape of ferromagnetic Ni film. The origin of these observations is ascribed to film shape dependent magnetoelastic coupling.
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Submitted 13 May, 2016;
originally announced May 2016.
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Nonreciprocal magnon propagation in a noncentrosymmetric ferromagnet
Authors:
Y. Iguchi,
S. Uemura,
K. Ueno,
Y. Onose
Abstract:
Relativistic spin-orbit interaction drastically modifies electronic band and endows emergent functionalities. One of the example is the Rashba effect. In noncentrosymmetric systems such as interface and polar materials, the electronic band is spin-splitted depending on the momentum direction owing to the spin-orbit interaction, which is useful for the electric manipulation of spin current. Similar…
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Relativistic spin-orbit interaction drastically modifies electronic band and endows emergent functionalities. One of the example is the Rashba effect. In noncentrosymmetric systems such as interface and polar materials, the electronic band is spin-splitted depending on the momentum direction owing to the spin-orbit interaction, which is useful for the electric manipulation of spin current. Similar relativistic band-modification is also emergent for spin wave (magnon) in magnetic materials. The asymmetric magnon band dispersion induced by the Dzyaloshinskii-Moriya interaction, which is antisymmetric exchange interaction originating from the spin-orbit interaction, is theoretically expected, and experimentally observed recently in noncentrosymmetric ferromagnets. Here, we demonstrate that the nonreciprocal microwave response can be induced by the asymmetric magnon band in a noncentrosymmetric ferrimagnet LiFe$_5$O$_8$. This result may pave a new path to designing magnonic device based on the relativistic band engineering.
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Submitted 8 May, 2015;
originally announced May 2015.
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Real-space observation of short-period cubic lattice of skyrmions in MnGe
Authors:
Toshiaki Tanigaki,
Kiyou Shibata,
Naoya Kanazawa,
Xiuzhen Yu,
Sinji Aizawa,
Yoshinori Onose,
Hyun Soon Park,
Daisuke Shindo,
Yoshinori Tokura
Abstract:
Emergent phenomena and functions arising from topological electron-spin textures in real space or momentum space are attracting growing interest for new concept of states of matter as well as for possible applications to spintronics. One such example is a magnetic skyrmion, a topologically stable nanoscale spin vortex structure characterized by a topological index. Real-space regular arrays of sky…
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Emergent phenomena and functions arising from topological electron-spin textures in real space or momentum space are attracting growing interest for new concept of states of matter as well as for possible applications to spintronics. One such example is a magnetic skyrmion, a topologically stable nanoscale spin vortex structure characterized by a topological index. Real-space regular arrays of skyrmions are described by combination of multi-directional spin helixes. Nanoscale configurations and characteristics of the two-dimensional skyrmion hexagonal-lattice have been revealed extensively by real-space observations. Other three-dimensional forms of skyrmion lattices, such as a cubic-lattice of skyrmions, are also anticipated to exist, yet their direct observations remain elusive. Here we report real-space observations of spin configurations of the skyrmion cubic-lattice in MnGe with a very short period (~3 nm) and hence endowed with the largest skyrmion number density. The skyrmion lattices parallel to the {100} atomic lattices are directly observed using Lorentz transmission electron microscopes (Lorentz TEMs). It enables the first simultaneous observation of magnetic skyrmions and underlying atomic-lattice fringes. These results indicate the emergence of skyrmion-antiskyrmion lattice in MnGe, which is a source of emergent electromagnetic responses and will open a possibility of controlling few-nanometer scale skyrmion lattices through atomic lattice modulations.
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Submitted 12 March, 2015;
originally announced March 2015.
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Observation of magnetic excitations of skyrmion crystal in a helimagnetic insulator
Authors:
Y. Onose,
Y. Okamura,
S. Seki,
S. Ishiwata,
Y. Tokura
Abstract:
The skyrmion is a topologically stable spin texture, in which the spin direction wraps a sphere. The topological nature gives rise to emergent electromagnetic phenomena such as topological Hall effect. Recently, the crystallization of nanoscale skyrmions was observed in chiral helimagnets with use of the neutron diffraction and Lorentz transmission electron microscopy. The skyrmions are quite mobi…
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The skyrmion is a topologically stable spin texture, in which the spin direction wraps a sphere. The topological nature gives rise to emergent electromagnetic phenomena such as topological Hall effect. Recently, the crystallization of nanoscale skyrmions was observed in chiral helimagnets with use of the neutron diffraction and Lorentz transmission electron microscopy. The skyrmions are quite mobile under electric current density as low as $\sim$ 10$^6$ A/m$^2$, and, in some cases, stable up to near room temperature. These features suggest that the skyrmions may work as a magnetic stable-variable similar to the bubble memory but equipped with topological functionalities. Here, we investigate the low-energy excitations of the skyrmion crystal in a helimagnetic insulator Cu$_2$OSeO$_3$ in terms of microwave response. We have observed two distinct excitations of the skyrmion with different polarization characteristics; the counter-clockwise circulating mode at 1 GHz and the breathing mode at 1.5 GHz. These modes may play a crucial role in the low energy dynamics of skyrmions and hence in their manipulation via external stimuli.
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Submitted 23 April, 2012;
originally announced April 2012.
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Effect of lattice geometry on magnon Hall effect in ferromagnetic insulators
Authors:
T. Ideue,
Y. Onose,
H. Katsura,
Y. Shiomi,
S. Ishiwata,
N. Nagaosa,
Y. Tokura
Abstract:
We have investigated the thermal Hall effect of magnons for various ferromagnetic insulators. For pyrochlore ferromagnetic insulators Lu$_2$V$_2$O$_7$, Ho$_2$V$_2$O$_7$, and In$_2$Mn$_2$O$_7$, finite thermal Hall conductivities have been observed below the Curie temperature $T_C$ . From the temperature and magnetic field dependences, it is concluded that magnons are responsible for the thermal Hal…
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We have investigated the thermal Hall effect of magnons for various ferromagnetic insulators. For pyrochlore ferromagnetic insulators Lu$_2$V$_2$O$_7$, Ho$_2$V$_2$O$_7$, and In$_2$Mn$_2$O$_7$, finite thermal Hall conductivities have been observed below the Curie temperature $T_C$ . From the temperature and magnetic field dependences, it is concluded that magnons are responsible for the thermal Hall effect. The Hall effect of magnons can be well explained by the theory based on the Berry curvature in momentum space induced by the Dzyaloshinskii-Moriya (DM) interaction. The analysis has been extended to the transition metal (TM) oxides with perovskite structure. The thermal Hall signal was absent or far smaller in La$_2$NiMnO$_6$ and YTiO$_3$, which have the distorted perovskite structure with four TM ions in the unit cell. On the other hand, a finite thermal Hall response is discernible below $T_C$ in another ferromagentic perovskite oxide BiMnO$_3$, which shows orbital ordering with a larger unit cell. The presence or absence of the thermal Hall effect in insulating pyrochlore and perovskite systems reflect the geometric and topological aspect of DM-induced magnon Hall effect.
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Submitted 3 April, 2012; v1 submitted 14 January, 2012;
originally announced January 2012.
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Chirality of Matter Shows Up via Spin Excitations
Authors:
Sandor Bordacs,
Istvan Kezsmarki,
David Szaller,
Laszlo Demko,
Noriaki Kida,
Hiroshi Murakawa,
Yoshinori Onose,
Ryo Shimano,
Toomas Room,
Urmas Nagel,
Shin Miyahara,
Nobuo Furukawa,
Yoshinori Tokura
Abstract:
Right- and left-handed circularly polarized light interact differently with electronic charges in chiral materials. This asymmetry generates the natural circular dichroism and gyrotropy, also known as the optical activity. Here we demonstrate that optical activity is not a privilege of the electronic charge excitations but it can also emerge for the spin excitations in magnetic matter. The square-…
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Right- and left-handed circularly polarized light interact differently with electronic charges in chiral materials. This asymmetry generates the natural circular dichroism and gyrotropy, also known as the optical activity. Here we demonstrate that optical activity is not a privilege of the electronic charge excitations but it can also emerge for the spin excitations in magnetic matter. The square-lattice antiferromagnet Ba$_2$CoGe$_2$O$_7$ offers an ideal arena to test this idea, since it can be transformed to a chiral form by application of external magnetic fields. As a direct proof of the field-induced chiral state, we observed large optical activity when the light is in resonance with spin excitations at sub-terahertz frequencies. In addition, we found that the magnetochiral effect, the absorption difference for the light beams propagating parallel and anti-parallel to the applied magnetic field, has an exceptionally large amplitude close to 100%. All these features are ascribed to the magnetoelectric nature of spin excitations as they interact both with the electric and magnetic components of light.
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Submitted 7 September, 2011;
originally announced September 2011.
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Thermoelectric response in the incoherent transport region near Mott transition: the case study of La1-xSrxVO3
Authors:
M. Uchida,
K. Oishi,
M. Matsuo,
W. Koshibae,
Y. Onose,
M. Mori,
J. Fujioka,
S. Miyasaka,
S. Maekawa,
Y. Tokura
Abstract:
We report a systematic investigation on the high-temperature thermoelectric response in a typical filling-control Mott transition system La1-xSrxVO3. In the vicinity of the Mott transition, incoherent charge transport appears with increasing temperature and the thermopower undergoes two essential crossovers, asymptotically approaching the limit values expected from the entropy consideration, as kn…
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We report a systematic investigation on the high-temperature thermoelectric response in a typical filling-control Mott transition system La1-xSrxVO3. In the vicinity of the Mott transition, incoherent charge transport appears with increasing temperature and the thermopower undergoes two essential crossovers, asymptotically approaching the limit values expected from the entropy consideration, as known as Heikes formula. By comparison with the results of the dynamical mean field theory, we show that the thermopower in the Mott critical state mainly measures the entropy per charge carrier that depends on electronic degrees of freedom available at the measurement temperature. Our findings verify that the Heikes formula is indeed applicable to the real correlated electron systems at practical temperatures (T>200K).
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Submitted 14 March, 2011; v1 submitted 6 March, 2011;
originally announced March 2011.
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Large Magnetoresistance and Spin-Polarized Heavy-Mass Electron State in a Doped Valence Bond Solid (Ti1-xVx)2O3
Authors:
M. Uchida,
Y. Onose,
Y. Tokura
Abstract:
A heavy-mass electron state is realized in a doped valence bond solid (Ti1-xVx)2O3. In this system, itinerant holes mediate the mainly ferromagnetic RKKY interaction between the localized magnetic moments and become readily spin-polarized under a magnetic field, while showing large negative magnetoresistance. In spite of the ferromagnetic interaction among the carriers, their effective mass is fou…
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A heavy-mass electron state is realized in a doped valence bond solid (Ti1-xVx)2O3. In this system, itinerant holes mediate the mainly ferromagnetic RKKY interaction between the localized magnetic moments and become readily spin-polarized under a magnetic field, while showing large negative magnetoresistance. In spite of the ferromagnetic interaction among the carriers, their effective mass is found to be 1 or 2 orders of magnitude larger than that of usual doped semiconductors. Such strong mass renormalization is ascribable to the polaron formation on the Ti-dimer, where the spin-singlet state is originally formed. Doping dependence of the electronic specific-heat coefficient implies that the dimeric lattice fluctuation or softening is responsible for the enhanced electron-phonon interaction.
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Submitted 21 February, 2011;
originally announced February 2011.
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Pseudogap of metallic layered nickelate R2-xSrxNiO4 (R=Nd, Eu) crystals measured using angle-resolved photoemission spectroscopy
Authors:
M. Uchida,
K. Ishizaka,
P. Hansmann,
Y. Kaneko,
Y. Ishida,
X. Yang,
R. Kumai,
A. Toschi,
Y. Onose,
R. Arita,
K. Held,
O. K. Andersen,
S. Shin,
Y. Tokura
Abstract:
We have investigated charge dynamics and electronic structures for single crystals of metallic layered nickelates, R2-xSrxNiO4 (R=Nd, Eu), isostructural to La2-xSrxCuO4. Angle-resolved photoemission spectroscopy on the barely-metallic Eu0.9Sr1.1NiO4 (R=Eu, x=1.1) has revealed a large hole surface of x2-y2 character with a high-energy pseudogap of the same symmetry and comparable magnitude with tho…
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We have investigated charge dynamics and electronic structures for single crystals of metallic layered nickelates, R2-xSrxNiO4 (R=Nd, Eu), isostructural to La2-xSrxCuO4. Angle-resolved photoemission spectroscopy on the barely-metallic Eu0.9Sr1.1NiO4 (R=Eu, x=1.1) has revealed a large hole surface of x2-y2 character with a high-energy pseudogap of the same symmetry and comparable magnitude with those of underdoped (x<0.1) cuprates, although the antiferromagnetic interactions are one order of magnitude smaller. This finding strongly indicates that the momentum-dependent pseudogap feature in the layered nickelate arises from the real-space charge correlation.
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Submitted 28 February, 2011; v1 submitted 26 December, 2010;
originally announced December 2010.
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Giant directional dichroism of terahertz light in resonance with magnetic excitations of the multiferroic oxide BaCo$_2$Ge$_2$O$_7$
Authors:
I. Kezsmarki,
N. Kida,
H. Murakawa,
S. Bordacs,
Y. Onose,
Y. Tokura
Abstract:
We propose that concurrently magnetic and ferroelectric, i.e. multiferroic, compounds endowed with electrically-active magnetic excitations (electromagnons) provide a key to produce large directional dichroism for long wavelengths of light. By exploiting the control of ferroelectric polarization and magnetization in a multiferroic oxide Ba$_2$CoGe$_2$O$_7$, we demonstrate the realization of such a…
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We propose that concurrently magnetic and ferroelectric, i.e. multiferroic, compounds endowed with electrically-active magnetic excitations (electromagnons) provide a key to produce large directional dichroism for long wavelengths of light. By exploiting the control of ferroelectric polarization and magnetization in a multiferroic oxide Ba$_2$CoGe$_2$O$_7$, we demonstrate the realization of such a directional light-switch function at terahertz frequecies in resonance with the electromagnon absorption. Our results imply that this hidden potential is present in a broad variety of multiferroics.
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Submitted 26 October, 2010;
originally announced October 2010.
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Observation of the Magnon Hall Effect
Authors:
Y. Onose,
T. Ideue,
H. Katsura,
Y. Shiomi,
N. Nagaosa,
Y. Tokura
Abstract:
The Hall effect usually occurs when the Lorentz force acts on a charge current in a conductor in the presence of perpendicular magnetic field. On the other hand, neutral quasi-particles such as phonons and spins can carry heat current and potentially show the Hall effect without resorting to the Lorentz force. We report experimental evidence for the anomalous thermal Hall effect caused by spin exc…
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The Hall effect usually occurs when the Lorentz force acts on a charge current in a conductor in the presence of perpendicular magnetic field. On the other hand, neutral quasi-particles such as phonons and spins can carry heat current and potentially show the Hall effect without resorting to the Lorentz force. We report experimental evidence for the anomalous thermal Hall effect caused by spin excitations (magnons) in an insulating ferromagnet with a pyrochlore lattice structure. Our theoretical analysis indicates that the propagation of the spin wave is influenced by the Dzyaloshinskii-Moriya spin-orbit interaction, which plays the role of the vector potential as in the intrinsic anomalous Hall effect in metallic ferromagnets.
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Submitted 9 August, 2010;
originally announced August 2010.
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Ferroelectricity induced by spin-dependent metal-ligand hybridization in Ba$_2$CoGe$_2$O$_7$
Authors:
H. Murakawa,
Y. Onose,
S. Miyahara,
N. Furukawa,
Y. Tokura
Abstract:
We have investigated the variation of induced ferroelectric polarization under magnetic field with various directions and magnitudes in a staggered antiferromagnet Ba$_2$CoGe$_2$O$_7$. While the ferroelectric polarization cannot be explained by the well-accepted spin current model nor exchange striction mechanism, we have shown that it is induced by the spin-dependent $p$-$d$ hybridization between…
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We have investigated the variation of induced ferroelectric polarization under magnetic field with various directions and magnitudes in a staggered antiferromagnet Ba$_2$CoGe$_2$O$_7$. While the ferroelectric polarization cannot be explained by the well-accepted spin current model nor exchange striction mechanism, we have shown that it is induced by the spin-dependent $p$-$d$ hybridization between the transition-metal (Co) and ligand (O) via the spin-orbit interaction. On the basis of the correspondence between the direction of electric polarization and the magnetic state, we have also demonstrated the electrical control of the magnetization direction.
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Submitted 27 May, 2010;
originally announced May 2010.
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Magnetic digital flop of ferroelectric domain with fixed spin chirality in a triangular lattice helimagnet
Authors:
S. Seki,
H. Murakawa,
Y. Onose,
Y. Tokura
Abstract:
Ferroelectric properties in magnetic fields of varying magnitude and direction have been investigated for a triangular-lattice helimagnet CuFe1-xGaxO2 (x=0.035). The magnetoelectric phase diagrams were deduced for magnetic fields along [001], [110], and [1-10] direction, and the in-plane magnetic field was found to induce the rearrangement of six possible multiferroic domains. Upon every 60-degr…
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Ferroelectric properties in magnetic fields of varying magnitude and direction have been investigated for a triangular-lattice helimagnet CuFe1-xGaxO2 (x=0.035). The magnetoelectric phase diagrams were deduced for magnetic fields along [001], [110], and [1-10] direction, and the in-plane magnetic field was found to induce the rearrangement of six possible multiferroic domains. Upon every 60-degree rotation of in-plane magnetic field around the c-axis, unique 120-degree flop of electric polarization occurs as a result of the switch of helical magnetic q-vector. The chirality of spin helix is always conserved upon the q-flop. The possible origin is discussed in the light of the stable structure of multiferroic domain wall.
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Submitted 12 November, 2009; v1 submitted 1 June, 2009;
originally announced June 2009.
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Dynamics of Multiferroic Domain Wall in Spin-Cycloidal Ferroelectric DyMnO$_{3}$
Authors:
F. Kagawa,
M. Mochizuki,
Y. Onose,
H. Murakawa,
Y. Kaneko,
N. Furukawa,
Y. Tokura
Abstract:
We report the dielectric dispersion of the giant magnetocapacitance (GMC) in multiferroic DyMnO$_{3}$ over a wide frequency range. The GMC is found to be attributable not to the softened electromagnon but to the electric-field-driven motion of multiferroic domain wall (DW). In contrast to conventional ferroelectric DWs, the present multiferroic DW motion holds extremely high relaxation rate of…
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We report the dielectric dispersion of the giant magnetocapacitance (GMC) in multiferroic DyMnO$_{3}$ over a wide frequency range. The GMC is found to be attributable not to the softened electromagnon but to the electric-field-driven motion of multiferroic domain wall (DW). In contrast to conventional ferroelectric DWs, the present multiferroic DW motion holds extremely high relaxation rate of $\sim$$10^{7}$ s$^{-1}$ even at low temperatures. This mobile nature as well as the model simulation suggests that the multiferroic DW is not atomically thin as in ferroelectrics but thick, reflecting its magnetic origin.
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Submitted 9 February, 2009;
originally announced February 2009.
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Smectic to nematic transition of magnetic texture in conical state
Authors:
Masayasu Takeda,
Yasuo Endoh,
Kazuhisa Kakurai,
Yoshinori Onose,
Junichi Suzuki,
Yoshinori Tokura
Abstract:
Small-angle neutron scattering (SANS) profiles revealed the existence of magnetic textures like liquid crystals in the low-temperature helical phase of Fe0.7Co0.3Si, isomorphous of MnSi.
Small-angle neutron scattering (SANS) profiles revealed the existence of magnetic textures like liquid crystals in the low-temperature helical phase of Fe0.7Co0.3Si, isomorphous of MnSi.
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Submitted 5 January, 2009;
originally announced January 2009.
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Unusual Hall Effect Anomaly in MnSi Under Pressure
Authors:
Minhyea Lee,
W. Kang,
Y. Onose,
Y. Tokura,
N. P. Ong
Abstract:
We report the observation of a highly unusual Hall current in the MnSi in an applied pressure P = 6-12 kbar. The Hall conductivity displays a distinctive step-wise field profile quite unlike any other Hall response observed in solids. We identify the origin of this Hall current with the effective real-space magnetic field due to chiral spin textures, which may be a precursor of the partial-order…
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We report the observation of a highly unusual Hall current in the MnSi in an applied pressure P = 6-12 kbar. The Hall conductivity displays a distinctive step-wise field profile quite unlike any other Hall response observed in solids. We identify the origin of this Hall current with the effective real-space magnetic field due to chiral spin textures, which may be a precursor of the partial-order state at P>14.6 kbar. We discuss evidence favoring the chiral spin mechanism for the origin of the observed Hall anomaly.
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Submitted 5 May, 2009; v1 submitted 19 November, 2008;
originally announced November 2008.
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Charge dynamics in thermally and doping induced insulator-metal transitions of (Ti1-xVx)2O3
Authors:
M. Uchida,
J. Fujioka,
Y. Onose,
Y. Tokura
Abstract:
Charge dynamics of (Ti1-xVx)2O3 with x=0-0.06 has been investigated by measurements of charge transport and optical conductivity spectra in a wide temperature range of 2-600K with the focus on the thermally and doping induced insulator-metal transitions (IMTs). The optical conductivity peaks for the interband transitions in the 3d t2g manifold are observed in the both insulating and metallic sta…
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Charge dynamics of (Ti1-xVx)2O3 with x=0-0.06 has been investigated by measurements of charge transport and optical conductivity spectra in a wide temperature range of 2-600K with the focus on the thermally and doping induced insulator-metal transitions (IMTs). The optical conductivity peaks for the interband transitions in the 3d t2g manifold are observed in the both insulating and metallic states, while their large variation (by ~0.4 eV) with change of temperature and doping level scales with that of the Ti-Ti dimer bond length, indicating the weakened singlet bond in the course of IMTs. The thermally and V-doping induced IMTs are driven with the increase in carrier density by band-crossing and hole-doping, respectively, in contrast to the canonical IMT of correlated oxides accompanied by the whole collapse of the Mott gap.
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Submitted 12 May, 2008;
originally announced May 2008.
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Spin-driven ferroelectricity and possible antiferroelectricity in triangular lattice antiferromagnets ACrO2 (A = Cu, Ag, Li, or Na)
Authors:
S. Seki,
Y. Onose,
Y. Tokura
Abstract:
Correlation between dielectric and magnetic properties was investigated on the triangular lattice antiferromagnets ACrO2 (A= Cu, Ag, Li, or Na) showing 120-degree spiral spin structure with easy-axis anisotropy. For the A= Cu and Ag compounds with delafossite structure, ferroelectric polarization emerges upon the spiral spin order, implying the strong coupling between the ferroelectricity and sp…
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Correlation between dielectric and magnetic properties was investigated on the triangular lattice antiferromagnets ACrO2 (A= Cu, Ag, Li, or Na) showing 120-degree spiral spin structure with easy-axis anisotropy. For the A= Cu and Ag compounds with delafossite structure, ferroelectric polarization emerges upon the spiral spin order, implying the strong coupling between the ferroelectricity and spiral spin structure. On the other hand, for the A = Li and Na compounds with ordered rock salt structure, no polarization but only clear anomalies in dielectric constant can be observed upon the spiral spin order. The absence of polarization can be interpreted as the antiferroelectric state induced by the alternate stacking of Cr3+ layer with opposite spin vector chirality. These results imply that a vast range of trigonally stacked triangular-lattice systems with 120-degree spin structure can be multiferroic, irrespective of their magnetic anisotropy.
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Submitted 24 January, 2008;
originally announced January 2008.
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The Lorenz number in CeCoIn$_5$ inferred from the thermal and charge Hall currents
Authors:
Y. Onose,
N. P. Ong,
C. Petrovic
Abstract:
The thermal Hall conductivity $κ_{xy}$ and Hall conductivity $σ_{xy}$ in CeCoIn$_5$ are used to determine the Lorenz number ${\cal L}_H$ at low temperature $T$. This enables the separation of the observed thermal conductivity into its electronic and non-electronic parts. We uncover evidence for a charge-neutral, field-dependent thermal conductivity, which we identify with spin excitations. At lo…
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The thermal Hall conductivity $κ_{xy}$ and Hall conductivity $σ_{xy}$ in CeCoIn$_5$ are used to determine the Lorenz number ${\cal L}_H$ at low temperature $T$. This enables the separation of the observed thermal conductivity into its electronic and non-electronic parts. We uncover evidence for a charge-neutral, field-dependent thermal conductivity, which we identify with spin excitations. At low $T$, these excitations dominate the scattering of charge carriers. We show that suppression of the spin excitations in high fields leads to a steep enhancement of the electron mean-free-path, which leads to an interesting scaling relation between the magnetoresistance, thermal conductivity and $σ_{xy}$.
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Submitted 7 September, 2007; v1 submitted 18 June, 2007;
originally announced June 2007.
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Anomalous thermopower and Nernst effect in $\rm CeCoIn_5$: entropy-current loss in precursor state
Authors:
Y. Onose,
Lu Li,
C. Petrovic,
N. P. Ong
Abstract:
The heavy-electron superconductor CeCoIn$_5$ exhibits a puzzling precursor state above its superconducting critical temperature at $T_c$ = 2.3 K. The thermopower and Nernst signal are anomalous. Below 15 K, the entropy current of the electrons undergoes a steep decrease reaching $\sim$0 at $T_c$. Concurrently, the off-diagonal thermoelectric current $α_{xy}$ is enhanced. The delicate sensitivity…
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The heavy-electron superconductor CeCoIn$_5$ exhibits a puzzling precursor state above its superconducting critical temperature at $T_c$ = 2.3 K. The thermopower and Nernst signal are anomalous. Below 15 K, the entropy current of the electrons undergoes a steep decrease reaching $\sim$0 at $T_c$. Concurrently, the off-diagonal thermoelectric current $α_{xy}$ is enhanced. The delicate sensitivity of the zero-entropy state to field implies phase coherence over large distances. The prominent anomalies in the thermoelectric current contrast with the relatively weak effects in the resistivity and magnetization.
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Submitted 7 May, 2007;
originally announced May 2007.
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Resonance in Optimally Electron-Doped Superconductor Nd$_{1.85}$Ce$_{0.15}$CuO$_{4-δ}$
Authors:
Jun Zhao,
Pengcheng Dai,
Shiliang Li,
Paul G. Freeman,
Y. Onose,
Y. Tokura
Abstract:
We use inelastic neutron scattering to probe magnetic excitations of an optimally electron-doped superconductor Nd$_{1.85}$Ce$_{0.15}$CuO$_{4-δ}$ above and below its superconducting transition temperature $T_c=25$ K. In addition to gradually opening a spin pseudo gap at the antiferromagnetic ordering wavevector ${\bf Q}=(1/2,1/2,0)$, the effect of superconductivity is to form a resonance centere…
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We use inelastic neutron scattering to probe magnetic excitations of an optimally electron-doped superconductor Nd$_{1.85}$Ce$_{0.15}$CuO$_{4-δ}$ above and below its superconducting transition temperature $T_c=25$ K. In addition to gradually opening a spin pseudo gap at the antiferromagnetic ordering wavevector ${\bf Q}=(1/2,1/2,0)$, the effect of superconductivity is to form a resonance centered also at ${\bf Q}=(1/2,1/2,0)$ but at energies above the spin pseudo gap. The intensity of the resonance develops like a superconducting order parameter, similar to those for hole-doped superconductors and electron-doped Pr$_{0.88}$LaCe$_{0.12}$CuO$_4$. The resonance is therefore a general phenomenon of cuprate superconductors, and must be fundamental to the mechanism of high-$T_c$ superconductivity.
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Submitted 29 March, 2007; v1 submitted 27 March, 2007;
originally announced March 2007.
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Impurity-doping induced ferroelectricity in frustrated antiferromagnet CuFeO2
Authors:
S. Seki,
Y. Yamasaki,
Y. Shiomi,
S. Iguchi,
Y. Onose,
Y. Tokura
Abstract:
Dielectric responses have been investigated on the triangular-lattice antiferromagnet CuFeO2 and its site-diluted analogs CuFe1-xAlxO2 (x=0.01 and 0.02) with and without application of magnetic field. We have found a ferroelectric behavior at zero magnetic field for x=0.02. At any doping level, the onset field of the ferroelectricity always coincides with that of the noncollinear magnetic struct…
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Dielectric responses have been investigated on the triangular-lattice antiferromagnet CuFeO2 and its site-diluted analogs CuFe1-xAlxO2 (x=0.01 and 0.02) with and without application of magnetic field. We have found a ferroelectric behavior at zero magnetic field for x=0.02. At any doping level, the onset field of the ferroelectricity always coincides with that of the noncollinear magnetic structure while the transition field dramatically decreases to zero field with Al doping. The results imply the further possibility of producing the ferroelectricity by modifying the frustrated spin structure in terms of site-doping and external magnetic field.
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Submitted 9 November, 2006;
originally announced November 2006.
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A hidden constant in the anomalous Hall effect of a high-purity magnet MnSi
Authors:
Minhyea Lee,
Y. Onose,
Y. Tokura,
N. P. Ong
Abstract:
Measurements of the Hall conductivity in MnSi can provide incisive tests of theories of the anomalous Hall (AH) effect, because both the mean-free-path and magnetoresistance (MR) are unusually large for a ferromagnet. The large MR provides an accurate way to separate the AH conductivity $σ_{xy}^A$ from the ordinary Hall conductivity $σ_{xy}^N$. Below the Curie temperature $T_C$, $σ_{xy}^A$ is li…
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Measurements of the Hall conductivity in MnSi can provide incisive tests of theories of the anomalous Hall (AH) effect, because both the mean-free-path and magnetoresistance (MR) are unusually large for a ferromagnet. The large MR provides an accurate way to separate the AH conductivity $σ_{xy}^A$ from the ordinary Hall conductivity $σ_{xy}^N$. Below the Curie temperature $T_C$, $σ_{xy}^A$ is linearly proportional to $ M$ (magnetization) with a proportionality constant $S_H$ that is independent of both $T$ and $H$. In particular, $S_H$ remains a constant while $σ_{xy}^N$ changes by a factor of 100 between 5 K and $T_C$. We discuss implications of the hidden constancy in $S_H$.
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Submitted 5 February, 2007; v1 submitted 27 October, 2006;
originally announced October 2006.
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Thermal-Hall conductivity and long-lived quasiparticles in CeCoIn$_5$
Authors:
Y. Onose,
N. P. Ong,
C. Petrovic
Abstract:
In CeCoIn$_5$, the thermal conductivity $κ_{xx}$ and Hall conductivity $κ_{xy}$ below $T_c$ display large anomalies below $T_c$. The strong suppression of the anomalies in weak fields implies the existence of long-lived quasiparticles. We also discuss briefly the Wiedemann-Franz ratio and the existence of a strongly field-dependent spin-fluctuation heat current.
In CeCoIn$_5$, the thermal conductivity $κ_{xx}$ and Hall conductivity $κ_{xy}$ below $T_c$ display large anomalies below $T_c$. The strong suppression of the anomalies in weak fields implies the existence of long-lived quasiparticles. We also discuss briefly the Wiedemann-Franz ratio and the existence of a strongly field-dependent spin-fluctuation heat current.
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Submitted 25 October, 2006;
originally announced October 2006.
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Universal Scaling Behavior of Anomalous Hall Effect and Anomalous Nernst Effect in Itinerant Ferromagnets
Authors:
T. Miyasato,
N. Abe,
T. Fujii,
A. Asamitsu,
S. Onoda,
Y. Onose,
N. Nagaosa,
Y. Tokura
Abstract:
Anomalous Hall effect (AHE) and anomalous Nernst effect (ANE) in a variety of ferromagnetic metals including pure metals, oxides, and chalcogenides, are studied to obtain unified understandings of their origins. We show a universal scaling behavior of anomalous Hall conductivity $σ_{xy}$ as a function of longitudinal conductivity $σ_{xx}$ over five orders of magnitude, which is well explained by…
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Anomalous Hall effect (AHE) and anomalous Nernst effect (ANE) in a variety of ferromagnetic metals including pure metals, oxides, and chalcogenides, are studied to obtain unified understandings of their origins. We show a universal scaling behavior of anomalous Hall conductivity $σ_{xy}$ as a function of longitudinal conductivity $σ_{xx}$ over five orders of magnitude, which is well explained by a recent theory of the AHE taking into account both the intrinsic and extrinsic contributions. ANE is closely related with AHE and provides us with further information about the low-temperature electronic state of itinerant ferromagnets. Temperature dependence of transverse Peltier coefficient $α_{xy}$ shows an almost similar behavior among various ferromagnets, and this behavior is in good agreement quantitatively with that expected from the Mott rule.
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Submitted 11 October, 2006;
originally announced October 2006.