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Observation of vortex stripes in UTe$_2$
Authors:
Y. F. Wang,
H. X. Yao,
T. Winyard,
Christopher Broyles,
Shannon Gould,
Q. S. He,
P. H. Zhang,
K. Z. Yao,
J. J. Zhu,
B. K. Xiang,
K. Y. Liang,
Z. J. Li,
B. R. Chen,
Q. Z. Zhou,
D. F. Agterberg,
E. Babaev,
S. Ran,
Y. H. Wang
Abstract:
Quantum vortices are fundamentally important for properties of superconductors. In conventional type-II superconductor they determine the magnetic response of the system and tend to form regular lattices. UTe$_2$ is a recently discovered heavy fermion superconductor exhibiting many anomalous macroscopic behaviors. However, the question whether it has a multicomponent order parameter remains open.…
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Quantum vortices are fundamentally important for properties of superconductors. In conventional type-II superconductor they determine the magnetic response of the system and tend to form regular lattices. UTe$_2$ is a recently discovered heavy fermion superconductor exhibiting many anomalous macroscopic behaviors. However, the question whether it has a multicomponent order parameter remains open. Here, we study magnetic properties of UTe$_2$ by employing scanning superconducting quantum interference device microscopy. We find vortex behavior which is very different from that in ordinary superconductors. We imaged vortices generated by cooling in magnetic field applied along different crystalline directions. While a small out-of-plane magnetic field produces typical isolated vortices, higher field generates vortex stripe patterns which evolve with vortex density. The stripes form at different locations and along different directions in the surface plane when the vortices are crystalized along the crystalline b or c axes. The behavior is reproduced by our simulation based on an anisotropic two-component order parameter. This study shows that UTe$_2$ has a nontrivial disparity of multiple length scales, placing constraints on multicomponent superconductivity. The tendency of vortex stripe formation and their control by external field may be useful in fluxonics applications.
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Submitted 1 September, 2024; v1 submitted 12 August, 2024;
originally announced August 2024.
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Observation of long-range ferromagnetism via anomalous supercurrents in a spin-orbit coupled superconductor
Authors:
B. K. Xiang,
Y. S. Lin,
Q. S. He,
J. J. Zhu,
B. R. Chen,
Y. F. Wang,
K. Y. Liang,
Z. J. Li,
H. X. Yao,
C. X. Wu,
T. Y. Zhou,
M. H. Fang,
Y. Lu,
I. V. Tokatly,
F. S. Bergeret,
Y. H. Wang
Abstract:
Conventional superconductors naturally disfavor ferromagnetism because the supercurrent-carrying electrons are paired into anti-parallel spin singlets. In superconductors with strong Rashba spin-orbit coupling, impurity magnetic moments induce supercurrents through the spin-galvanic effect. As a result, long-range ferromagnetic interaction among the impurity moments may be mediated through such an…
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Conventional superconductors naturally disfavor ferromagnetism because the supercurrent-carrying electrons are paired into anti-parallel spin singlets. In superconductors with strong Rashba spin-orbit coupling, impurity magnetic moments induce supercurrents through the spin-galvanic effect. As a result, long-range ferromagnetic interaction among the impurity moments may be mediated through such anomalous supercurrents in a similar fashion as in itinerant ferromagnets. Fe(Se,Te) is such a superconductor with topological surface bands, previously shown to exhibit quantum anomalous vortices around impurity spins. Here, we take advantage of the flux sensitivity of scanning superconducting quantum interference devices to investigate superconducting Fe(Se,Te) in the regime where supercurrents around impurities overlap. We find homogeneous remanent flux patterns after applying a supercurrent through the sample. The patterns are consistent with anomalous edge and bulk supercurrents generated by in-plane magnetization, which occur above a current threshold and follow hysteresis loops reminiscent of those of a ferromagnet. Similar long-range magnetic orders can be generated by Meissner current under a small out-of-plane magnetic field. The magnetization weakens with increasing temperature and disappears after thermal cycling to above superconducting critical temperature; further suggesting superconductivity is central to establishing and maintaining the magnetic order. These observations demonstrate surface anomalous supercurrents as a mediator for ferromagnetism in a spin-orbit coupled superconductor, which may potentially be utilized for low-power cryogenic memory.
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Submitted 20 July, 2023; v1 submitted 20 July, 2023;
originally announced July 2023.
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Flux focusing with a superconducting nano-needle for scanning SQUID susceptometry
Authors:
B. K. Xiang,
S. Y. Wang,
Y. F. Wang,
J. J. Zhu,
H. T. Xu,
Y. H. Wang
Abstract:
Nano-fabricated superconducting quantum interference device (nano-SQUID) is a direct and sensitive flux probe useful for magnetic imaging of quantum materials and mesoscopic devices. Enabled by functionalities of superconductive integrated circuits, nano-SQUID fabricated on a chip is particularly versatile but spatial resolution has been limited by its planar geometry. Here, we use femtosecond-las…
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Nano-fabricated superconducting quantum interference device (nano-SQUID) is a direct and sensitive flux probe useful for magnetic imaging of quantum materials and mesoscopic devices. Enabled by functionalities of superconductive integrated circuits, nano-SQUID fabricated on a chip is particularly versatile but spatial resolution has been limited by its planar geometry. Here, we use femtosecond-laser 3-dimensional (3D) lithography and print a needle onto a nano-SQUID susceptometer to overcome the limit of a plane-structure. The nano-needle coated with a superconducting shell focuses the flux both from the field coil and the sample. We perform scanning imaging using such a needle-on-SQUID (NoS) device on superconducting test patterns with topographic feedback. The NoS shows improved spatial resolution in both magnetometry and susceptometry over its planarized counterpart. This work serves as a proof-of-principle for the integration and inductive coupling between superconducting 3D nano-structures and on-chip Josephson nano-devices.
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Submitted 21 September, 2022;
originally announced September 2022.
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Direct observation of quantum anomalous vortex in Fe(Se,Te)
Authors:
Y. S. Lin,
S. Y. Wang,
X. Zhang,
Y. Feng,
Y. P. Pan,
H. Ru,
J. J. Zhu,
B. K. Xiang,
K. Liu,
C. L. Zheng,
L. Y. Wei,
M. X. Wang,
Z. K. Liu,
L. Chen,
K. Jiang,
Y. F. Guo,
Ziqiang Wang,
Y. H. Wang
Abstract:
Vortices are topological defects of type-II superconductors in an external magnetic field. In a similar fashion to a quantum anomalous Hall insulator, quantum anomalous vortex (QAV) spontaneously nucleates due to orbital-and-spin exchange interaction between vortex core states and magnetic impurity moment, breaking time-reversal symmetry (TRS) of the vortex without an external field. Here, we used…
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Vortices are topological defects of type-II superconductors in an external magnetic field. In a similar fashion to a quantum anomalous Hall insulator, quantum anomalous vortex (QAV) spontaneously nucleates due to orbital-and-spin exchange interaction between vortex core states and magnetic impurity moment, breaking time-reversal symmetry (TRS) of the vortex without an external field. Here, we used scanning superconducting quantum interference device microscopy (sSQUID) to search for its signatures in iron-chalcogenide superconductor Fe(Se,Te). Under zero magnetic field, we found a stochastic distribution of isolated anomalous vortices and antivortices with flux quanta $Φ_0$. By applying a small local magnetic field under the coil of the nano-SQUID device, we observed hysteretic flipping of the vortices reminiscent of the switching of ferromagnetic domains, suggesting locally broken-TRS. We further showed vectorial rotation of a flux line linking a paired vortex-antivortex with the local field. These unique properties of the anomalous vortices satisfied the defining criteria of QAV. Our observation suggests a quantum vortex phase with spontaneous broken-TRS in a high-temperature superconductor.
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Submitted 1 August, 2022;
originally announced August 2022.
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Oscillating paramagnetic Meissner effect and Berezinskii-Kosterlitz-Thouless transition in $Bi_2Sr_2CaCu_2O_{8+δ}$ monolayer
Authors:
S. Y. Wang,
Y. Yu,
J. X. Hao,
Y. Feng,
J. J. Zhu,
Y. S. Lin,
B. K. Xiang,
H. Ru,
Y. P. Pan,
G. D. Gu,
K. Watanabe,
T. Taniguchi,
Y. Qi,
Y. Zhang,
Y. H. Wang
Abstract:
Monolayers of a prototypical cuprate high transition-temperature ($T_C$) superconductor $Bi_2Sr_2CaCu_2O_{8+δ}$ (Bi2212) was recently found to show $T_C$ and other electronic properties similar to those of the bulk. The robustness of superconductivity in an ideal two-dimensional (2D) system was an intriguing fact that defied the Mermin-Wagner theorem. Here, we took advantage of the high sensitivit…
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Monolayers of a prototypical cuprate high transition-temperature ($T_C$) superconductor $Bi_2Sr_2CaCu_2O_{8+δ}$ (Bi2212) was recently found to show $T_C$ and other electronic properties similar to those of the bulk. The robustness of superconductivity in an ideal two-dimensional (2D) system was an intriguing fact that defied the Mermin-Wagner theorem. Here, we took advantage of the high sensitivity of scanning SQUID susceptometry to image the phase stiffness throughout the phase transition of Bi2212 in the 2D limit. We found susceptibility oscillated with flux between diamagnetism and paramagnetism in a Fraunhofer-like pattern up till $T_C$. The temperature and sample size-dependence of the modulation period agreed well with our Coulomb gas analogy of a finite 2D system based on Berezinskii-Kosterlitz-Thouless (BKT) transition. In the multilayers, the susceptibility oscillation differed in a small temperature regime below $T_C$ in consistent with a dimensional-crossover led by interlayer coupling. Serving as strong evidence of BKT transition in the bulk, there appeared a sharp superfluid density jump at zero-field and paramagnetism at small fields just below $T_C$. These results unified the phase transitions from the monolayer Bi2212 to the bulk as BKT transition with finite interlayer coupling. This elucidating picture favored the pre-formed pairs scenario for the underdoped cuprates regardless of lattice dimensionality.
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Submitted 9 December, 2021;
originally announced December 2021.
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Improving spatial resolution of scanning SQUID microscopy with an on-chip design
Authors:
Y. P. Pan,
J. J. Zhu,
Y. Feng,
Y. S. Lin,
H. B. Wang,
X. Y. Liu,
H. Jin,
Z. Wang,
L. Chen,
Y. H. Wang
Abstract:
Scanning superconducting quantum interference device microscopy (sSQUID) is currently one of the most effective methods for direct and sensitive magnetic flux imaging on the mesoscopic scale. A SQUID-on-chip design allows integration of field coils for susceptometry in a gradiometer setup which is very desirable for measuring magnetic responses of quantum matter. However, the spatial resolution of…
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Scanning superconducting quantum interference device microscopy (sSQUID) is currently one of the most effective methods for direct and sensitive magnetic flux imaging on the mesoscopic scale. A SQUID-on-chip design allows integration of field coils for susceptometry in a gradiometer setup which is very desirable for measuring magnetic responses of quantum matter. However, the spatial resolution of such a design has largely been limited to micrometers due to the difficulty in approaching the sample. Here, we used electron beam lithography technology in the fabrication of the 3D nano-bridge-based SQUID devices to prepare pick-up coils with diameters down to 150 nm. Furthermore, we integrated the deep silicon etching process in order to minimize the distance between the pick-up coil and the wafer edge. Combined with a tuning-fork-based scanning head, the sharpness of the etched chip edge enables a precision of 5 nm in height control. By scanning measurements on niobium chessboard samples using these improved SQUID devices, we demonstrate sub-micron spatial resolutions in both magnetometry and susceptometry, significantly better than our previous generations of nano-SQUIDs. Such improvement in spatial resolution of SQUID-on-chip is a valuable progress for magnetic imaging of quantum materials and devices in various modes.
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Submitted 17 June, 2021;
originally announced June 2021.