Trapping Surface Electrons on Graphene Layers and Islands
Authors:
D. Niesner,
Th. Fauster,
J. I. Dadap,
N. Zaki,
K. R. Knox,
P. -C. Yeh,
R. Bhandari,
R. M. Osgood,
M. Petrović,
M. Kralj
Abstract:
We report the use of time- and angle-resolved two-photon photoemission to map the bound, unoccupied electronic structure of the weakly coupled graphene/Ir(111) system. The energy, dispersion, and lifetime of the lowest three image-potential states are measured. In addition, the weak interaction between Ir and graphene permits observation of resonant transitions from an unquenched Shockley-type sur…
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We report the use of time- and angle-resolved two-photon photoemission to map the bound, unoccupied electronic structure of the weakly coupled graphene/Ir(111) system. The energy, dispersion, and lifetime of the lowest three image-potential states are measured. In addition, the weak interaction between Ir and graphene permits observation of resonant transitions from an unquenched Shockley-type surface state of the Ir substrate to graphene/Ir image-potential states. The image-potential-state lifetimes are comparable to those of mid-gap clean metal surfaces. Evidence of localization of the excited electrons on single-atom-layer graphene islands is provided by coverage-dependent measurements.
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Submitted 29 December, 2011; v1 submitted 9 September, 2011;
originally announced September 2011.