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Charge-ordered states in twisted MoTe$_2$
Authors:
Sparsh Mishra,
Tobias M. R. Wolf,
Allan H. MacDonald
Abstract:
We analyze interaction-driven charge-density-wave (CDW) states in the spin-valley polarized first valence miniband of twisted MoTe$_2$ (tMoTe$_2$) using an adiabatic mapping from the continuum model to an effective Landau-level (LL) problem. When projected to the lowest LL, the leading spatial harmonic of the moiré-periodic potential changes sign at a magic twist angle $θ_c$ where the band reaches…
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We analyze interaction-driven charge-density-wave (CDW) states in the spin-valley polarized first valence miniband of twisted MoTe$_2$ (tMoTe$_2$) using an adiabatic mapping from the continuum model to an effective Landau-level (LL) problem. When projected to the lowest LL, the leading spatial harmonic of the moiré-periodic potential changes sign at a magic twist angle $θ_c$ where the band reaches its minimum bandwidth. By solving self-consistent Hartree-Fock equations in a multi-LL Hilbert space, we find that triangular-lattice CDW states with density maxima on MX (or XM) sites or on MM sites are favored on opposite sides of the magic angle at most filling factors and that stripe order appears near $ν_h=1/2$. We show that CDW states at $ν_h >1/2$ can carry a nonzero total Chern number, providing a natural route to reentrant integer quantum Hall effects and discuss the energy competition between fractional Chern insulator and CDW states.
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Submitted 9 March, 2026; v1 submitted 5 March, 2026;
originally announced March 2026.
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Exciton-based sensing of remote electron correlations in 2D heterostructures
Authors:
Tobias M. R. Wolf,
Tian Xie,
Chenhao Jin,
Allan H. MacDonald
Abstract:
Many monolayer transition metal dichalcogenides, including MoS$_2$, MoSe$_2$, WS$_2$, and WSe$_2$, are direct bandgap two-dimensional (2D) semiconductors with sharp optical resonances at excitonic bound state frequencies. Recent experiments have demonstrated that excitonic resonance frequencies in multilayer van der Waals stacks are altered by long-range Coulomb interactions with electrons in near…
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Many monolayer transition metal dichalcogenides, including MoS$_2$, MoSe$_2$, WS$_2$, and WSe$_2$, are direct bandgap two-dimensional (2D) semiconductors with sharp optical resonances at excitonic bound state frequencies. Recent experiments have demonstrated that excitonic resonance frequencies in multilayer van der Waals stacks are altered by long-range Coulomb interactions with electrons in nearby but electrically isolated 2D materials. These modulations have been successfully used to detect transitions between distinct states of remote strongly correlated 2D electron fluids. In this Letter we provide a theory of these frequency shifts, enabling a more quantitative interpretation of excitonic-sensing experiments, and apply it as an example to WSe$_2$ that is proximate to graphene bilayers and multilayers.
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Submitted 24 October, 2025;
originally announced October 2025.
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Theory of magnetoroton bands in moiré materials
Authors:
Bishoy M. Kousa,
Nicolás Morales-Durán,
Tobias M. R. Wolf,
Eslam Khalaf,
Allan H. MacDonald
Abstract:
The recent realization of Hofstadter spectra and fractional Chern insulators in moiré materials has introduced a new ingredient, a periodic lattice potential, to the study of quantum Hall phases. While the fractionalized states in moiré systems are expected to be in the same universality class as their counterparts in Landau levels, the periodic potential can have qualitative and quantitative effe…
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The recent realization of Hofstadter spectra and fractional Chern insulators in moiré materials has introduced a new ingredient, a periodic lattice potential, to the study of quantum Hall phases. While the fractionalized states in moiré systems are expected to be in the same universality class as their counterparts in Landau levels, the periodic potential can have qualitative and quantitative effects on physical observables. Here, we examine how the magnetoroton collective modes of fractional quantum Hall (FQH) states are altered by external periodic potentials. Employing a single-mode-approximation, we derive an effective Hamiltonian for the low-energy neutral excitations expressed in terms of three-point density correlation functions, which are computed using Monte Carlo. Our analysis is applicable to FQH states in graphene with a hexagonal boron nitride (hBN) substrate and also to fractional Chern insulator (FCI) states in twisted MoTe$_2$ bilayers. We predict experimentally testable trends in the THz absorption characteristics of FCI and FQH states and estimate the external potential strength at which a soft-mode phase transition occurs between FQH and charge density wave states.
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Submitted 23 April, 2026; v1 submitted 24 February, 2025;
originally announced February 2025.
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Intraband collective excitations in fractional Chern insulators are dark
Authors:
Tobias M. R. Wolf,
Yung-Chun Chao,
Allan H. MacDonald,
Jung Jung Su
Abstract:
The low-energy collective excitations of semiconductors and insulators often couple strongly to light, allowing them to be probed optically. We argue here that in fractional Chern insulators intra-band collective excitations are dark in the sense that they couple anomalously weakly to light. This conclusion is based on a relationship between ideal quantum geometry and the structure factor of a Che…
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The low-energy collective excitations of semiconductors and insulators often couple strongly to light, allowing them to be probed optically. We argue here that in fractional Chern insulators intra-band collective excitations are dark in the sense that they couple anomalously weakly to light. This conclusion is based on a relationship between ideal quantum geometry and the structure factor of a Chern band, and on a classical plasma analogy motivated by the vortexibility property of ideal Chern bands.
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Submitted 15 June, 2024;
originally announced June 2024.
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Gate-tunable topological phases in superlattice modulated bilayer graphene
Authors:
Yongxin Zeng,
Tobias M. R. Wolf,
Chunli Huang,
Nemin Wei,
Sayed Ali Akbar Ghorashi,
Allan H. MacDonald,
Jennifer Cano
Abstract:
Superlattice potential modulation can produce flat minibands in Bernal-stacked bilayer graphene. In this work we study how band topology and interaction-induced symmetry-broken phases in this system are controlled by tuning the displacement field and the shape and strength of the superlattice potential. We use an analytic perturbative analysis to demonstrate that topological flat bands are favored…
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Superlattice potential modulation can produce flat minibands in Bernal-stacked bilayer graphene. In this work we study how band topology and interaction-induced symmetry-broken phases in this system are controlled by tuning the displacement field and the shape and strength of the superlattice potential. We use an analytic perturbative analysis to demonstrate that topological flat bands are favored by a honeycomb-lattice-shaped potential, and numerics to show that the robustness of topological bands depends on both the displacement field strength and the periodicity of the superlattice potential. At integer fillings of the topological flat bands, the strength of the displacement field and the superlattice potential tune phase transitions between quantum anomalous Hall insulator, trivial insulator, and metallic states. We present mean-field phase diagrams in a gate voltage parameter space at filling factor $ν=1$, and discuss the prospects of realizing quantum anomalous Hall insulators and fractional Chern insulators when the superlattice potential modulation is produced by dielectric patterning or adjacent moiré materials.
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Submitted 8 January, 2024;
originally announced January 2024.
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Quasi-boson approximation yields accurate correlation energy in the 2D electron gas
Authors:
Tobias M. R. Wolf,
Chunli Huang
Abstract:
We report the successful adaptation of the quasi-boson approximation, a technique traditionally employed in nuclear physics, to the analysis of the two-dimensional electron gas. We show that the correlation energy estimated from this approximation agrees closely with the results obtained from quantum Monte Carlo simulations. Our methodology comprehensively incorporates the exchange self-energy, di…
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We report the successful adaptation of the quasi-boson approximation, a technique traditionally employed in nuclear physics, to the analysis of the two-dimensional electron gas. We show that the correlation energy estimated from this approximation agrees closely with the results obtained from quantum Monte Carlo simulations. Our methodology comprehensively incorporates the exchange self-energy, direct scattering, and exchange scattering for a particle-hole pair excited out of the mean-field groundstate within the equation-of-motion framework. The linearization of the equation of motion leads to a generalized-random-phase-approximation (gRPA) eigenvalue equation whose spectrum indicates that the plasmon dispersion remains unaffected by exchange effects, while the particle-hole continuum experiences a marked upward shift due to the exchange self-energy. Notably, the plasmon mode retains its collective nature within the particle-hole continuum, up to moderately short wavelength ($q\sim 0.3 k_F$ at metallic density $r_s=4$). Using the gRPA excitation spectrum, we calculate the zero-point energy of the quasi-boson Hamiltonian, thereby approximating the correlation energy of the original Hamiltonian. This research highlights the potential and effectiveness of applying the quasi-boson approximation to the gRPA spectrum, a fundamental technique in nuclear physics, to extended condensed matter systems.
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Submitted 19 November, 2023;
originally announced November 2023.
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Non-unitary multiorbital superconductivity from competing interactions in Dirac materials
Authors:
Tobias M. R. Wolf,
Maximilian F. Holst,
Manfred Sigrist,
Jose L. Lado
Abstract:
Unconventional superconductors represent one of the most intriguing quantum states of matter. In particular, multiorbital systems have the potential to host exotic non-unitary superconducting states. While the microscopic origin of non-unitarity is not yet fully solved, competing interactions are suggested to play a crucial role in stabilizing such states. The interplay between charge order and su…
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Unconventional superconductors represent one of the most intriguing quantum states of matter. In particular, multiorbital systems have the potential to host exotic non-unitary superconducting states. While the microscopic origin of non-unitarity is not yet fully solved, competing interactions are suggested to play a crucial role in stabilizing such states. The interplay between charge order and superconductivity has been a recurring theme in unconventionally superconducting systems, ranging from cuprate-based superconductors to dichalcogenide systems and even to twisted van der Waals materials. Here, we demonstrate that the existence of competing interactions gives rise to a non-unitary superconducting state. We show that the non-unitarity stems from a competing charge-ordered state whose interplay with superconductivity promotes a non-trivial multiorbital order. We establish this mechanism both from a Ginzburg-Landau perspective, and also from a fully microscopic selfconsistent solution of a multiorbital Dirac material. Our results put forward competing interactions as a powerful mechanism for driving non-unitary multiorbital superconductivity.
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Submitted 3 August, 2021;
originally announced August 2021.
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Spontaneous Valley Spirals in Magnetically Encapsulated Twisted Bilayer Graphene
Authors:
Tobias M. R. Wolf,
Oded Zilberberg,
Gianni Blatter,
Jose L. Lado
Abstract:
Van der Waals heterostructures provide a rich platform for emergent physics due to their tunable hybridization of electronic orbital- and spin-degrees of freedom. Here, we show that a heterostructure formed by twisted bilayer graphene sandwiched between ferromagnetic insulators develops flat bands stemming from the interplay between twist, exchange proximity and spin-orbit coupling. We demonstrate…
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Van der Waals heterostructures provide a rich platform for emergent physics due to their tunable hybridization of electronic orbital- and spin-degrees of freedom. Here, we show that a heterostructure formed by twisted bilayer graphene sandwiched between ferromagnetic insulators develops flat bands stemming from the interplay between twist, exchange proximity and spin-orbit coupling. We demonstrate that in this flat-band regime, the spin degree of freedom is hybridized, giving rise to an effective triangular superlattice with valley as a degenerate pseudospin degree of freedom. Incorporating electronic interactions at half-filling leads to a spontaneous valley-mixed state, i.e., a correlated state in the valley sector with geometric frustration of the valley spinor. We show that an electric interlayer bias generates an artificial valley-orbit coupling in the effective model, controlling both the valley anisotropy and the microscopic details of the correlated state, with both phenomena understood in terms of a valley-Heisenberg model with easy-plane anisotropic exchange. Our results put forward twisted graphene encapsulated between magnetic van der Waals heterostructures as platforms to explore purely valley-correlated states in graphene.
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Submitted 14 August, 2020;
originally announced August 2020.
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Electrically Tunable Flat Bands and Magnetism in Twisted Bilayer Graphene
Authors:
T. M. R. Wolf,
J. L. Lado,
G. Blatter,
O. Zilberberg
Abstract:
Twisted graphene bilayers provide a versatile platform to engineer metamaterials with novel emergent properties by exploiting the resulting geometric moiré superlattice. Such superlattices are known to host bulk valley currents at tiny angles ($α\approx 0.3 ^\circ$) and flat bands at magic angles ($α\approx 1^\circ$). We show that tuning the twist angle to $α^*\approx 0.8^\circ$ generates flat ban…
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Twisted graphene bilayers provide a versatile platform to engineer metamaterials with novel emergent properties by exploiting the resulting geometric moiré superlattice. Such superlattices are known to host bulk valley currents at tiny angles ($α\approx 0.3 ^\circ$) and flat bands at magic angles ($α\approx 1^\circ$). We show that tuning the twist angle to $α^*\approx 0.8^\circ$ generates flat bands away from charge neutrality with a triangular superlattice periodicity. When doped with $\pm 6$ electrons per moiré cell, these bands are half-filled and electronic interactions produce a symmetry-broken ground state (Stoner instability) with spin-polarized regions that order ferromagnetically. Application of an interlayer electric field breaks inversion symmetry and introduces valley-dependent dispersion that quenches the magnetic order. With these results, we propose a solid-state platform that realizes electrically tunable strong correlations.
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Submitted 31 August, 2019; v1 submitted 18 May, 2019;
originally announced May 2019.
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Tunneling into a finite Luttinger liquid coupled to noisy capacitive leads
Authors:
Antonio Štrkalj,
Michael S. Ferguson,
Tobias M. R. Wolf,
Ivan Levkivskyi,
Oded Zilberberg
Abstract:
Tunneling spectroscopy of one-dimensional interacting wires can be profoundly sensitive to the boundary conditions of the wire. Here, we analyze the tunneling spectroscopy of a wire coupled to capacitive metallic leads. Strikingly, with increasing many-body interactions in the wire, the impact of the boundary noise becomes more prominent. This interplay allows for a smooth crossover from standard…
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Tunneling spectroscopy of one-dimensional interacting wires can be profoundly sensitive to the boundary conditions of the wire. Here, we analyze the tunneling spectroscopy of a wire coupled to capacitive metallic leads. Strikingly, with increasing many-body interactions in the wire, the impact of the boundary noise becomes more prominent. This interplay allows for a smooth crossover from standard 1D tunneling signatures into a regime where the tunneling is dominated by the fluctuations at the leads. This regime is characterized by elevated zero-bias tunneling alongside a universal power-law decay at high energies. Furthermore, local tunneling measurements in this regime show a unique spatial-dependence that marks the formation of plasmonic standing waves in the wire. Our result offers a tunable method by which to control the boundary effects and measure the interaction strength (Luttinger parameter) within the wire.
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Submitted 5 September, 2018;
originally announced September 2018.
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Substrate-induced topological minibands in graphene
Authors:
Tobias M. R. Wolf,
Oded Zilberberg,
Ivan Levkivkskyi,
Gianni Blatter
Abstract:
The honeycomb lattice sets the basic arena for numerous ideas to implement electronic, photonic, or phononic topological bands in (meta-)materials. Novel opportunities to manipulate Dirac electrons in graphene through band engineering arise from superlattice potentials as induced by a substrate such as hexagonal boron-nitride. Making use of the general form of a weak substrate potential as dictate…
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The honeycomb lattice sets the basic arena for numerous ideas to implement electronic, photonic, or phononic topological bands in (meta-)materials. Novel opportunities to manipulate Dirac electrons in graphene through band engineering arise from superlattice potentials as induced by a substrate such as hexagonal boron-nitride. Making use of the general form of a weak substrate potential as dictated by symmetry, we analytically derive the low-energy minibands of the superstructure, including a characteristic 1.5 Dirac cone deriving from a three-band crossing at the Brillouin zone edge. Assuming a large supercell, we focus on a single Dirac cone (or valley) and find all possible arrangements of the low-energy electron and hole bands in a complete six-dimensional parameter space. We identify the various symmetry planes in parameter space inducing gap closures and find the sectors hosting topological minibands, including also complex band crossings that generate a valley Chern number atypically larger than one. Our map provides a starting point for the systematic design of topological bands by substrate engineering.
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Submitted 25 October, 2019; v1 submitted 27 May, 2018;
originally announced May 2018.