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Design of 2D Skyrmionic Metamaterial Through Controlled Assembly
Authors:
Qichen Xu,
Zhuanglin Shen,
Alexander Edström,
I. P. Miranda,
Zhiwei Lu,
Anders Bergman,
Danny Thonig,
Wanjian Yin,
Olle Eriksson,
Anna Delin
Abstract:
Despite extensive research on magnetic skyrmions and antiskyrmions, a significant challenge remains in crafting nontrivial high-order skyrmionic textures with varying, or even tailor-made, topologies. We address this challenge, by focusing on a construction pathway of skyrmionic metamaterials within a monolayer thin film and suggest several skyrmionic metamaterials that are surprisingly stable, i.…
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Despite extensive research on magnetic skyrmions and antiskyrmions, a significant challenge remains in crafting nontrivial high-order skyrmionic textures with varying, or even tailor-made, topologies. We address this challenge, by focusing on a construction pathway of skyrmionic metamaterials within a monolayer thin film and suggest several skyrmionic metamaterials that are surprisingly stable, i.e., long-lived, due to a self-stabilization mechanism. This makes these new textures promising for applications. Central to our approach is the concept of 'simulated controlled assembly', in short, a protocol inspired by 'click chemistry' that allows for positioning topological magnetic structures where one likes, and then allowing for energy minimization to elucidate the stability. Utilizing high-throughput atomistic-spin-dynamic simulations alongside state-of-the-art AI-driven tools, we have isolated skyrmions (topological charge Q=1), antiskyrmions (Q=-1), and skyrmionium (Q=0). These entities serve as foundational 'skyrmionic building blocks' to form the here reported intricate textures. In this work, two key contributions are introduced to the field of skyrmionic systems. First, we present a a novel combination of atomistic spin dynamics simulations and controlled assembly protocols for the stabilization and investigation of new topological magnets. Second, using the aforementioned methods we report on the discovery of skyrmionic metamaterials.
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Submitted 13 January, 2025; v1 submitted 16 February, 2024;
originally announced February 2024.
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Terahertz emission from $α$-W/CoFe epitaxial spintronic emitters
Authors:
Venkatesh Mottamchetty,
Rimantas Brucas,
Anna L. Ravensburg,
Renan Maciel,
Danny Thonig,
Jurgen Henk,
Rahul Gupta,
Arne Roos,
Cheuk Wai Tai,
Vassilios Kapaklis,
Peter Svedlindh
Abstract:
We report efficient terahertz (THz) generation in epitaxial $α$-W/Co$_{60}$Fe$_{40}$ spintronic emitters. Two types of emitters have been investigated; epitaxial $α$-W$(110)$/Co$_{60}$Fe$_{40}(110)$ and $α$-W$(001)$/Co$_{60}$Fe$_{40}(001)$ deposited on single crystalline Al$_{2}$O$_{3}$($11\bar{2}0$) and MgO($001$) substrates, respectively. First principle calculations of the electronic band struc…
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We report efficient terahertz (THz) generation in epitaxial $α$-W/Co$_{60}$Fe$_{40}$ spintronic emitters. Two types of emitters have been investigated; epitaxial $α$-W$(110)$/Co$_{60}$Fe$_{40}(110)$ and $α$-W$(001)$/Co$_{60}$Fe$_{40}(001)$ deposited on single crystalline Al$_{2}$O$_{3}$($11\bar{2}0$) and MgO($001$) substrates, respectively. First principle calculations of the electronic band structure at the W$(001)$ surface reveal Dirac-type surface states, similar to that reported previously for the W$(110)$ surface. The generated THz radiation is about $10\%$ larger for $α$-W$(110)$/Co$_{60}$Fe$_{40}(110)$ grown on single crystalline Al$_{2}$O$_{3}$($11\bar{2}0$), which is explained by the fact that the $α$-W$(110)$/Co$_{60}$Fe$_{40}(110)$ interface for this emitter is more transparent to the spin current due to the presence of Ångstr\" om-scale interface intermixing at the W/CoFe interface. Our results also reveal that the generation of THz radiation is larger when pumping with the laser light from the substrate side, which is explained by a larger part of the laser light due to interference effects in the film stack being absorbed in the ferromagnetic Co$_{60}$Fe$_{40}$ layer in this measurement configuration.
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Submitted 10 October, 2024; v1 submitted 18 January, 2024;
originally announced January 2024.
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Metaheuristic conditional neural network for harvesting skyrmionic metastable states
Authors:
Qichen Xu,
I. P. Miranda,
Manuel Pereiro,
Filipp N. Rybakov,
Danny Thonig,
Erik Sjöqvist,
Pavel Bessarab,
Anders Bergman,
Olle Eriksson,
Pawel Herman,
Anna Delin
Abstract:
We present a metaheuristic conditional neural-network-based method aimed at identifying physically interesting metastable states in a potential energy surface of high rugosity. To demonstrate how this method works, we identify and analyze spin textures with topological charge $Q$ ranging from 1 to $-13$ (where antiskyrmions have $Q<0$) in the Pd/Fe/Ir(111) system, which we model using a classical…
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We present a metaheuristic conditional neural-network-based method aimed at identifying physically interesting metastable states in a potential energy surface of high rugosity. To demonstrate how this method works, we identify and analyze spin textures with topological charge $Q$ ranging from 1 to $-13$ (where antiskyrmions have $Q<0$) in the Pd/Fe/Ir(111) system, which we model using a classical atomistic spin Hamiltonian based on parameters computed from density functional theory. To facilitate the harvest of relevant spin textures, we make use of the newly developed Segment Anything Model (SAM). Spin textures with $Q$ ranging from $-3$ to $-6$ are further analyzed using finite-temperature spin-dynamics simulations. We observe that for temperatures up to around 20\,K, lifetimes longer than 200\,ps are predicted, and that when these textures decay, new topological spin textures are formed. We also find that the relative stability of the spin textures depend linearly on the topological charge, but only when comparing the most stable antiskyrmions for each topological charge. In general, the number of holes (i.e., non-self-intersecting curves that define closed domain walls in the structure) in the spin texture is an important predictor of stability -- the more holes, the less stable is the texture. Methods for systematic identification and characterization of complex metastable skyrmionic textures -- such as the one demonstrated here -- are highly relevant for advancements in the field of topological spintronics.
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Submitted 29 May, 2023; v1 submitted 5 March, 2023;
originally announced March 2023.