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Out-of-equilibrium spin-valley dynamics of ferromagnets in topological Chern bands
Authors:
J. James,
I. Krastilevskiy,
F. Pichler,
L. Wang,
A. Iafarova,
F. Menzel,
K. Watanabe,
T. Taniguchi,
C. Kuhlenkamp,
M. Knap,
T. Smoleński
Abstract:
Understanding quantum matter far from equilibrium is a central goal of modern physics. Twisted MoTe2 bilayers constitute a promising platform for exploring this frontier by combining strong Coulomb interactions, nontrivial band geometry, and optical control. Here, we exploit this setting to investigate the role of topology and many-body correlations in the out-of-equilibrium dynamics of ferromagne…
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Understanding quantum matter far from equilibrium is a central goal of modern physics. Twisted MoTe2 bilayers constitute a promising platform for exploring this frontier by combining strong Coulomb interactions, nontrivial band geometry, and optical control. Here, we exploit this setting to investigate the role of topology and many-body correlations in the out-of-equilibrium dynamics of ferromagnets in Chern bands. Using a focused circularly polarized light pulse, we create a local magnetic domain oriented opposite to an external magnetic field and directly image its subsequent spin-valley relaxation in spatially and time-resolved low-temperature experiments. We demonstrate that in the vicinity of both integer and fractional Chern insulating states, the dynamics is governed by qualitatively different mechanisms than in ferromagnetic metals. Whereas metallic domains collapse by shrinking, Chern domains melt via thermal activation, resulting in drastically different temporal spin evolution and orders-of-magnitude longer relaxation times. These findings demonstrate the influence of topology and strong correlations on far-from-equilibrium collective spin phases, opening new opportunities for dynamical control of ferromagnets in the quantum Hall regime.
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Submitted 7 August, 2026;
originally announced August 2026.
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Ultrafast Formation and Annihilation of Strongly Bound, Anisotropic Excitons
Authors:
Lawson T. Lloyd,
Tommaso Pincelli,
Mohamed Amine Wahada,
Alessandro De Vita,
Ferdinand Menzel,
Kseniia Mosina,
Túlio H. L. G. Castro,
Alexander Neef,
Andreas V. Stier,
Nathan P. Wilson,
Zdeněk Sofer,
Jonathan J. Finley,
Martin Wolf,
Laurenz Rettig,
Ralph Ernstorfer
Abstract:
Van der Waals (vdW) layered materials with long-range magnetic order have the potential to enable novel optoelectronic and spintronic applications. Among these, CrSBr is an air-stable, direct band gap semiconductor that hosts interlayer antiferromagnetic order, a highly anisotropic electronic structure, and strongly bound excitons. In particular, excitons in CrSBr have been shown to inherit the qu…
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Van der Waals (vdW) layered materials with long-range magnetic order have the potential to enable novel optoelectronic and spintronic applications. Among these, CrSBr is an air-stable, direct band gap semiconductor that hosts interlayer antiferromagnetic order, a highly anisotropic electronic structure, and strongly bound excitons. In particular, excitons in CrSBr have been shown to inherit the quasi-one-dimensional nature of the material and also couple to the underlying spinorder. However, mechanisms of exciton formation, dissociation, and interaction with free carriers remain largely unexplored, despite being crucial for spintronic and optoelectronic applications. Here, we employ time- and angle-resolved photoemission spectroscopy to map the electronic structure and excited state dynamics in CrSBr. We directly resolve an exceptionally large exciton binding energy (~800 meV) and a highly anisotropic momentum space distribution of the exciton, revealing its quasi-1D real-space character. We observe an excitation-density-dependent interconversion between bound excitons and quasi-free carriers on sub- to few-picosecond timescales, indicating that many-body effects govern the excited-state dynamics and optical properties during the initial stages of relaxation. Our work highlights the strongly bound, anisotropic character of excitons in CrSBr, as well as the microscopic interactions steering relaxation pathways after photoexcitation in elevated density regimes relevant for future device applications.
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Submitted 27 March, 2026;
originally announced March 2026.
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Spectroscopy of Wigner crystal polarons in an atomically thin semiconductor
Authors:
L. Wang,
F. Menzel,
F. Pichler,
P. Knüppel,
K. Watanabe,
T. Taniguchi,
M. Knap,
T. Smoleński
Abstract:
Strongly interacting electrons in two-dimensional systems can spontaneously break translational symmetry, forming a periodic Wigner crystal. Although these crystals have been realized in several platforms, experimental studies of their collective many-body excitations in the absence of a magnetic field remain an outstanding challenge. Here, we access this regime optically by uncovering Wigner crys…
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Strongly interacting electrons in two-dimensional systems can spontaneously break translational symmetry, forming a periodic Wigner crystal. Although these crystals have been realized in several platforms, experimental studies of their collective many-body excitations in the absence of a magnetic field remain an outstanding challenge. Here, we access this regime optically by uncovering Wigner crystal polarons: novel light-matter excitations arising from the dressing of excitons by collective excitations of the Wigner crystal. These hybrid quasiparticles manifest as new optical resonances in cryogenic reflectance spectra of a charge-tunable WSe$_2$ monolayer, appearing concurrently with previously identified exciton umklapp transitions. In contrast to the latter, the energies of Wigner crystal polarons are governed not only by the electronic lattice constant but also by their hybridization with attractive exciton-polarons, whose strength is controlled by electronic interactions. These novel many-body excitations provide an optical interface to the spin state of the Wigner crystal, which as we demonstrate, can be controlled both magnetically and optically. Our work establishes layered materials as a unique platform for exploring dynamical impurity dressing by strongly correlated electronic orders.
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Submitted 18 December, 2025;
originally announced December 2025.