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Magnetic Field Dependence of the Spin Fluctuations in CeCu$_{5.8}$Ag$_{0.2}$
Authors:
X. Boraley,
A. D. Christianson,
J. Lass,
C. Balz,
M. Bartkowiak,
Ch. Niedermayer,
J. M. Lawrence,
L. Poudel,
D. G. Mandrus,
F. Ronning,
M. Janoschek,
D. G. Mazzone
Abstract:
Quantum phase transitions are among the most intriguing phenomena that can occur when the electronic ground state of correlated metals are tuned by external parameters such as pressure, magnetic field or chemical substitution. Such transitions between distinct states of matter are driven by quantum fluctuations, and can give rise to macroscopically coherent phases that are at the forefront of cond…
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Quantum phase transitions are among the most intriguing phenomena that can occur when the electronic ground state of correlated metals are tuned by external parameters such as pressure, magnetic field or chemical substitution. Such transitions between distinct states of matter are driven by quantum fluctuations, and can give rise to macroscopically coherent phases that are at the forefront of condensed matter research. However, the nature of the critical fluctuations, and thus the fundamental physics controlling many quantum phase transitions, remain poorly understood in numerous strongly correlated metals. Here we study the model material CeCu$_{5.8}$Ag$_{0.2}$ to gain insight into the implications of critical fluctuations originating from different regions in reciprocal space. By employing an external magnetic field along the crystallographic $a$- and $c$-axis as auxiliary tuning parameter we observe a pronounced anisotropy in the suppression of the quantum critical fluctuations, reflecting the spin anisotropy of the long-range ordered ground state at larger silver concentration. Coupled with the temperature dependence of the quantum critical fluctuations, these results suggest that the quantum phase transition in CeCu$_{5.8}$Ag$_{0.2}$ is driven by three-dimensional spin-density wave fluctuations.
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Submitted 30 January, 2026; v1 submitted 12 September, 2025;
originally announced September 2025.
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Intricacies of Frustrated Magnetism in the Kondo Metal YbAgGe
Authors:
D. G. Mazzone,
C. B. Larsen,
B. Ueland,
X. Boraley,
D. M. Pajerowski,
Y. Skourski,
J. Taylor,
B. Fak,
S. L. Bud'ko,
R. McQueeney,
P. C. Canfield,
O. Zaharko
Abstract:
The combination of localized magnetic moments, their frustration and interaction with itinerant electrons is a key challenge of condensed matter physics. Frustrated magnetic interactions promote degenerate ground states with enhanced fluctuations, a topic that is predominantly studied in magnetic insulators. The coupling between itinerant and localized electrons in metals add complexity to the pro…
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The combination of localized magnetic moments, their frustration and interaction with itinerant electrons is a key challenge of condensed matter physics. Frustrated magnetic interactions promote degenerate ground states with enhanced fluctuations, a topic that is predominantly studied in magnetic insulators. The coupling between itinerant and localized electrons in metals add complexity to the problem, and presently formulated only for extreme cases in which the itinerant electrons mediate exchange between localized spins (RKKY interaction) or suppress the formation of magnetic moments (Kondo screening). Here, we report an in-depth experimental study of the distorted Kagome metal YbAgGe, unravelling the open questions of how frustration, localized magnetism and itinerant electrons are intertwined in frustrated Kondo metals. We find that coupled itinerant and localized electrons give rise to dynamic magnetic correlations below T* ~ 20 K. At lower temperature, frustrated magnetic interactions establish anisotropic magnetic short-range correlations that culminate into antiferromagnetic long-range order below TN = 0.68 K with a significantly reduced modulated magnetic moment. We show that local moment Hamiltonians can yield limited understanding of the microscopic behaviour in frustrated metals, and prompt the extension of more sophisticated model Hamiltonians incorporating itinerant effects.
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Submitted 29 July, 2026; v1 submitted 2 September, 2025;
originally announced September 2025.
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Microscopic Origin of Reduced Magnetic Order in a Frustrated Metal
Authors:
X. Boraley,
O. Stockert,
J. Lass,
R. Sibille,
Ø. S. Fjellvåg,
S. H. Moody,
A. M. Läuchli,
V. Fritsch,
D. G. Mazzone
Abstract:
Although magnetic frustration in metals provides a promising avenue for novel quantum phenomena, their microscopic interpretation is often challenging. Here we use the face-centered cubic intermetallic HoInCu$_4$ as model material to show that Hamiltonians neglecting the charge degree of freedom are appropriate for frustrated metals possessing low density of states at the Fermi surface. Through ne…
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Although magnetic frustration in metals provides a promising avenue for novel quantum phenomena, their microscopic interpretation is often challenging. Here we use the face-centered cubic intermetallic HoInCu$_4$ as model material to show that Hamiltonians neglecting the charge degree of freedom are appropriate for frustrated metals possessing low density of states at the Fermi surface. Through neutron scattering techniques we determine matching magnetic exchange interactions in the paramagnetic and field-polarized states using an effective spin-1 Heisenberg Hamiltonian, for which we identify antiferromagnetic nearest and next-nearest neighbour interactions $J_1$ and $J_2$ that are close to the critical ratio $J_2$/$J_1$ = 1/2. The study further provides evidence that spin-wave theory fails to predict the low-energy spin dynamics in the antiferromagnetic zero-field state, which is dominated by overdamped magnetic excitations. We conclude that the low-energy fluctuations arise from quantum fluctuations, accounting for the missing moment of the strongly renormalized magnetic long-range order.
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Submitted 24 July, 2025; v1 submitted 12 February, 2025;
originally announced February 2025.
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Magnetic ground state and perturbations of the distorted kagome Ising metal TmAgGe
Authors:
C. B. Larsen,
D. G. Mazzone,
N. Gauthier,
H. D. Rosales,
F. A. Gómez Albarracín,
J. Lass,
X. Boraley,
S. L. Bud'ko,
P. C. Canfield,
O. Zaharko
Abstract:
We present the magnetic orders and excitations of the distorted kagome intermetallic magnet TmAgGe. Using neutron single crystal diffraction we identify the propagation vectors $\bf{k}$ = (1/2 0 0) and $\bf{k}$ = (0 0 0) and determine the magnetic structures of the zero-field and magnetic field-induced phases for $H$ along the $a$ and [-1 1 0] crystal directions. We determine the experimental magn…
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We present the magnetic orders and excitations of the distorted kagome intermetallic magnet TmAgGe. Using neutron single crystal diffraction we identify the propagation vectors $\bf{k}$ = (1/2 0 0) and $\bf{k}$ = (0 0 0) and determine the magnetic structures of the zero-field and magnetic field-induced phases for $H$ along the $a$ and [-1 1 0] crystal directions. We determine the experimental magnetic field-temperature ($H$, $T$)-phase diagram and reproduce it by Monte-Carlo simulations of an effective spin exchange Hamiltonian for one distorted kagome layer. Our model includes a strong axial single-ion anisotropy and significantly smaller exchange couplings which span up to the third-nearest neighbours within the layer. Single crystal inelastic neutron scattering (INS) measurements reveal an almost flat, only weakly dispersive mode around 7 meV that we use alongside bulk magnetization data to deduce the crystal-electric field (CEF) scheme for the Tm$^{3+}$ ions. Random phase approximation (RPA) calculations based on the determined CEF wave functions of the two lowest quasi-doublets enable an estimation of the interlayer coupling that is compatible with the experimental INS spectra. No evidence for low-energy spin waves associated to the magnetic order was found, which is consistent with the strongly Ising nature of the ground state.
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Submitted 16 June, 2023;
originally announced June 2023.