Showing 1–50 of 90 results for author: Zang, J

Large Language Models for Superconductor Discovery

Authors: Suman Itani, Yibo Zhang, Ranjit Itani, Jiadong Zang

Abstract: Large language models (LLMs) offer new opportunities for automated data extraction and property prediction across materials science, yet their use in superconductivity research remains limited. Here we construct a large experimental database of 78,203 records, covering 19,058 unique compositions, extracted from scientific literature using an LLM-driven workflow. Each entry includes chemical compos… ▽ More Large language models (LLMs) offer new opportunities for automated data extraction and property prediction across materials science, yet their use in superconductivity research remains limited. Here we construct a large experimental database of 78,203 records, covering 19,058 unique compositions, extracted from scientific literature using an LLM-driven workflow. Each entry includes chemical composition, critical temperature, measurement pressure, structural descriptors, and critical fields. We fine-tune several open-source LLMs for three tasks: (i) classifying superconductors vs. non-superconductors, (ii) predicting the superconducting transition temperature directly from composition or structure-informed inputs, and (iii) inverse design of candidate compositions conditioned on target Tc. The fine-tuned LLMs achieve performance comparable to traditional feature-based models and in some cases exceed them, while substantially outperforming their base versions and capturing meaningful chemical and structural trends. The inverse-design model generates chemically plausible compositions, including 28% novel candidates not seen in training. Finally, applying the trained predictors to the GNoME database identifies unreported materials with predicted Tc > 10 K. Although unverified, these candidates illustrate how integrating an LLM-driven workflow can enable scalable hypothesis generation for superconductivity discovery. △ Less

Submitted 11 December, 2025; originally announced December 2025.

Comments: 15 pages, 6 figures

Charge disproportionation driven polar magnetic metallic double-layered perovskite Sr$_3$Co$_2$O$_7$

Authors: Hong-Fei Huang, Houssam Sabri, Jiadong Zang, Jie-Xiang Yu

Abstract: Strong coupling among spontaneous structural symmetric breaking, magnetism and metallicity in an intrinsic polar magnetic metal can give rise to novel physical phenomena and holds great promise for applications in spintronics. Here, we elucidate the mechanism of metallic ferroelectricity in the recently discovered polar metal Sr$_3$Co$_2$O$_7$. Our first-principles calculations reveal that both th… ▽ More Strong coupling among spontaneous structural symmetric breaking, magnetism and metallicity in an intrinsic polar magnetic metal can give rise to novel physical phenomena and holds great promise for applications in spintronics. Here, we elucidate the mechanism of metallic ferroelectricity in the recently discovered polar metal Sr$_3$Co$_2$O$_7$. Our first-principles calculations reveal that both the spontaneous ferroelectric displacements and the metallicity originate from charge disproportionation of Co ions. This is characterized by an inverted ligand-field splitting of the Co $t_2g$ orbitals at one site, while the metallic behavior is preserved by the t$_2g$ orbitals at both sites. The charge disproportionation stabilizes the asymmetric phase Within the framework of the on-site Hubbard U interaction. We thus propose that in related transition metal oxides, charge disproportionation within specific orbitals can concurrently drive metallicity and ferroelectricity, enabling strong coupling between these properties. More remarkably, this mechanism allows for the coexistence of magnetism, as evidenced in Sr$_3$Co$_2$O$_7$. Our findings highlight a promising avenue for realizing polar magnetic metals and provide a new design principle for exploring multifunctional materials. △ Less

Submitted 3 November, 2025; originally announced November 2025.

Comments: 4 figures

Construction of Hopfion Crystals

Authors: Wen-Tao Hou, Zhuoxian Xiang, Yizhou Liu, Jiadong Zang

Abstract: Hopfions, three-dimensional topological solitons characterized by nontrivial Hopf indices, represent a fundamental class of field configurations that emerge across diverse areas of physics. Despite extensive studies of isolated hopfions, a framework for constructing spatially ordered arrays of hopfions, i.e., hopfion crystals, has been lacking. Here, we present a systematic approach for generating… ▽ More Hopfions, three-dimensional topological solitons characterized by nontrivial Hopf indices, represent a fundamental class of field configurations that emerge across diverse areas of physics. Despite extensive studies of isolated hopfions, a framework for constructing spatially ordered arrays of hopfions, i.e., hopfion crystals, has been lacking. Here, we present a systematic approach for generating hopfion crystals with cubic symmetry by combining the Hopf map with rational mapping techniques. By superposing helical waves in $\mathbb{R}^4$, we construct hopfion crystals with tunable Hopf indices and controllable topology. We demonstrate simple cubic, facecentered cubic, and body-centered cubic hopfion crystals, and extend our framework to create crystals of more complex topological structures, including axially symmetric tori, torus links, and torus knots with higher Hopf indices. Our results provide a foundation for searching hopfions in real materials and studying their collective phenomena. △ Less

Submitted 4 April, 2025; originally announced April 2025.

Comments: 10 pages,7 figures

Renormalization group analysis of noisy neural field

Authors: Jie Zang, Pascal Helson, Shenquan Liu, Arvind Kumar, Dhrubaditya Mitra

Abstract: Neurons in the brain show great diversity in their individual properties and their connections to other neurons. To develop an understanding of how neuronal diversity contributes to brain dynamics and function at large scales we start with a linearized version of the Wilson-Kowan model and introduce a random anisotropy to inter-neuron connection. The resultant model is Edwards-Wilkinson model with… ▽ More Neurons in the brain show great diversity in their individual properties and their connections to other neurons. To develop an understanding of how neuronal diversity contributes to brain dynamics and function at large scales we start with a linearized version of the Wilson-Kowan model and introduce a random anisotropy to inter-neuron connection. The resultant model is Edwards-Wilkinson model with a random anisotropic term. Averaging over the quenched randomness with the replica method we obtain a bi-quadratic nonlinearity. We use Wilsonian dynamic renormalization group to analyze this model. We find that, up to one loop order, for dimensions higher than two, the effect of the noise is to change dynamic exponent from two to one. △ Less

Submitted 18 July, 2025; v1 submitted 27 March, 2025; originally announced March 2025.

Comments: major changes from previous version

Symmetry and Minimal Hamiltonian of Nonsymmorphic Collinear Antiferromagnet MnTe

Authors: Koichiro Takahashi, Hong-Fei Huang, Jie-Xiang Yu, Jiadong Zang

Abstract: $α$-MnTe, an $A$-type collinear antiferromagnet, has recently attracted significant attention due to its pronounced spin splitting despite having net zero magnetization, a phenomenon unique for a new class of magnetism dubbed altermagnetism. In this work, we develop a minimal effective Hamiltonian for $α$-MnTe based on realistic orbitals near the Fermi level at both the $Γ$ and $A… ▽ More $α$-MnTe, an $A$-type collinear antiferromagnet, has recently attracted significant attention due to its pronounced spin splitting despite having net zero magnetization, a phenomenon unique for a new class of magnetism dubbed altermagnetism. In this work, we develop a minimal effective Hamiltonian for $α$-MnTe based on realistic orbitals near the Fermi level at both the $Γ$ and $A$ points. Our model is derived using group representation theory, first-principles calculations, and tight-binding modeling. The resulting effective Hamiltonian exhibits qualitatively distinct electron transport characteristics between these high-symmetry points and for different in-plane Néel vector orientations along the $[11\bar{2}0]$ and $[1\bar{1}00]$ directions. Although relativistic correction of the spin-orbit coupling (SOC) is believed to be not important in altermagnets, we show the dominant role of SOC in the spin splitting and valence electrons of MnTe. These findings provide critical insights into altermagnetic electron transport in MnTe and establish a model playground for future theoretical and experimental studies. △ Less

Submitted 10 March, 2025; originally announced March 2025.

Comments: 6 figures. Supplementary Materials is included in the TeX source

Large Language Model-Driven Database for Thermoelectric Materials

Authors: Suman Itani, Yibo Zhang, Jiadong Zang

Abstract: Thermoelectric materials provide a sustainable way to convert waste heat into electricity. However, data-driven discovery and optimization of these materials are challenging because of a lack of a reliable database. Here we developed a comprehensive database of 7,123 thermoelectric compounds, containing key information such as chemical composition, structural detail, seebeck coefficient, electrica… ▽ More Thermoelectric materials provide a sustainable way to convert waste heat into electricity. However, data-driven discovery and optimization of these materials are challenging because of a lack of a reliable database. Here we developed a comprehensive database of 7,123 thermoelectric compounds, containing key information such as chemical composition, structural detail, seebeck coefficient, electrical and thermal conductivity, power factor, and figure of merit (ZT). We used the GPTArticleExtractor workflow, powered by large language models (LLM), to extract and curate data automatically from the scientific literature published in Elsevier journals. This process enabled the creation of a structured database that addresses the challenges of manual data collection. The open access database could stimulate data-driven research and advance thermoelectric material analysis and discovery. △ Less

Submitted 31 December, 2024; originally announced January 2025.

Neural Vector Tomography for Reconstructing a Magnetization Vector Field

Authors: Giorgi Butbaia, Jiadong Zang

Abstract: Discretized techniques for vector tomographic reconstructions are prone to producing artifacts in the reconstructions. The quality of these reconstructions may further deteriorate as the amount of noise increases. In this work, we instead model the underlying vector fields using smooth neural fields. Owing to the fact that the activation functions in the neural network may be chosen to be smooth a… ▽ More Discretized techniques for vector tomographic reconstructions are prone to producing artifacts in the reconstructions. The quality of these reconstructions may further deteriorate as the amount of noise increases. In this work, we instead model the underlying vector fields using smooth neural fields. Owing to the fact that the activation functions in the neural network may be chosen to be smooth and the domain is no longer pixelated, the model results in high-quality reconstructions, even under presence of noise. In the case where we have underlying global continuous symmetry, we find that the neural network substantially improves the accuracy of the reconstruction over the existing techniques. △ Less

Submitted 13 December, 2024; originally announced December 2024.

Comments: 6 pages, 5 figures

Topological Hall-like behavior of multidomain ferromagnets

Authors: Houssam Sabri, Benjamin E. Carlson, Sergey S. Pershoguba, Jiadong Zang

Abstract: We investigate the emergence of topological Hall-like (THE-like) signals in disordered multidomain ferromagnets. Non-monotonic behavior in Hall resistivity, commonly attributed to topological spin textures such as skyrmions, is produced in a random resistor network model without any chirality. It arises from simple mechanisms of the anomalous Hall effect (AHE) in combination with the domain wall s… ▽ More We investigate the emergence of topological Hall-like (THE-like) signals in disordered multidomain ferromagnets. Non-monotonic behavior in Hall resistivity, commonly attributed to topological spin textures such as skyrmions, is produced in a random resistor network model without any chirality. It arises from simple mechanisms of the anomalous Hall effect (AHE) in combination with the domain wall scattering. By varying domain configurations and domain wall resistances, we explore the conditions under which the non-monotonic resistivity can be enhanced. Our results emphasize the need for careful analysis in distinguishing between true topological Hall effects and artifacts caused by domain disorders. △ Less

Submitted 27 February, 2025; v1 submitted 11 November, 2024; originally announced November 2024.

Anomalous Tunneling Magnetoresistance Oscillation and Electrically Tunable Tunneling Anisotropic Magnetoresistance in Few-layer CrPS4

Authors: ZhuangEn Fu, Hong-Fei Huang, Piumi Samarawickrama, Kenji Watanabe, Takashi Taniguchi, Wenyong Wang, John Ackerman, Jiadong Zang, Jie-Xiang Yu, Jifa Tian

Abstract: Two-dimensional (2D) van der Waals (vdW) magnets with layer-dependent magnetic states and/or diverse magnetic interactions and anisotropies have attracted extensive research interest. Despite the advances, a notable challenge persists in effectively manipulating the tunneling anisotropic magnetoresistance (TAMR) of 2D vdW magnet-based magnetic tunnel junctions (MTJs). Here, we report the novel and… ▽ More Two-dimensional (2D) van der Waals (vdW) magnets with layer-dependent magnetic states and/or diverse magnetic interactions and anisotropies have attracted extensive research interest. Despite the advances, a notable challenge persists in effectively manipulating the tunneling anisotropic magnetoresistance (TAMR) of 2D vdW magnet-based magnetic tunnel junctions (MTJs). Here, we report the novel and anomalous tunneling magnetoresistance (TMR) oscillations and pioneering demonstration of bias and gate voltage controllable TAMR in 2D vdw MTJs, utilizing few-layer CrPS4. This material, inherently an antiferromagnet, transitions to a canted magnetic order upon application of external magnetic fields. Through TMR measurements, we unveil the novel, layer-dependent oscillations in the tunneling resistance for few-layer CrPS4 devices under both out-of-plane and in-plane magnetic fields, with a pronounced controllability via gate voltage. Intriguingly, we demonstrate that both the polarity and magnitude of TAMR in CrPS4 can be effectively tuned through either a bias or gate voltage. We further elucidate the mechanism behind this electrically tunable TAMR through first-principles calculations. The implications of our findings are far-reaching, providing new insights into 2D magnetism and opening avenues for the development of innovative spintronic devices based on 2D vdW magnets. △ Less

Submitted 24 October, 2024; originally announced October 2024.

Comments: 22 pages, 4 figures

Journal ref: Adv. Physics Res. 2024, 3, 2400052

Inertia in skyrmions confined to one-dimensional geometries

Authors: Koichiro Takahashi, Sergey S. Pershoguba, Jiadong Zang

Abstract: Magnetic skyrmions are conventionally attributed to having zero mass. In contrast, we show that skyrmions confined to one-dimensional geometries generically acquire mass (inertia) due to the combined effects of the skyrmion Hall effect and the elasticity of the system. We investigate the massive behavior of the skyrmion for a simplified periodic model of the disorder. We show that skyrmion mass lo… ▽ More Magnetic skyrmions are conventionally attributed to having zero mass. In contrast, we show that skyrmions confined to one-dimensional geometries generically acquire mass (inertia) due to the combined effects of the skyrmion Hall effect and the elasticity of the system. We investigate the massive behavior of the skyrmion for a simplified periodic model of the disorder. We show that skyrmion mass lowers the critical depinning force and leads to a step-like behavior in the skyrmion velocity-vs-current curves, which were recently observed in experiments. Finite mass could also lead to hysteresis in the velocity-vs-current curves. △ Less

Submitted 25 September, 2024; originally announced September 2024.

Comments: 6 pages, 4 figures

The Northeast Materials Database for Magnetic Materials

Authors: Suman Itani, Yibo Zhang, Jiadong Zang

Abstract: The discovery of magnetic materials with high operating temperature ranges and optimized performance is essential for advanced applications. Current data-driven approaches are limited by the lack of accurate, comprehensive, and feature-rich databases. This study aims to address this challenge by using Large Language Models (LLMs) to create a comprehensive, experiment-based, magnetic materials data… ▽ More The discovery of magnetic materials with high operating temperature ranges and optimized performance is essential for advanced applications. Current data-driven approaches are limited by the lack of accurate, comprehensive, and feature-rich databases. This study aims to address this challenge by using Large Language Models (LLMs) to create a comprehensive, experiment-based, magnetic materials database named the Northeast Materials Database (NEMAD), which consists of 67,573 magnetic materials entries(www.nemad.org). The database incorporates chemical composition, magnetic phase transition temperatures, structural details, and magnetic properties. Enabled by NEMAD, we trained machine learning models to classify materials and predict transition temperatures. Our classification model achieved an accuracy of 90% in categorizing materials as ferromagnetic (FM), antiferromagnetic (AFM), and non-magnetic (NM). The regression models predict Curie (Néel) temperature with a coefficient of determination (R2) of 0.87 (0.83) and a mean absolute error (MAE) of 56K (38K). These models identified 25 (13) FM (AFM) candidates with a predicted Curie (Néel) temperature above 500K (100K) from the Materials Project. This work shows the feasibility of combining LLMs for automated data extraction and machine learning models to accelerate the discovery of magnetic materials. △ Less

Submitted 24 September, 2025; v1 submitted 23 September, 2024; originally announced September 2024.

Journal ref: Nat. Commun. 16, 9415 (2025)

Microscopic Theory of Nonlinear Hall Effect in Three-dimensional Magnetic Systems

Authors: Wen-Tao Hou, Jiadong Zang

Abstract: The nonlinear Hall effect (NLHE) has been detected in various of condensed matter systems. Unlike linear Hall effect, NLHE may exist in physical systems with broken inversion symmetry in the crystal. On the other hand, real space spin texture may also break inversion symmetry and result in NLHE. In this letter, we employ the Feynman diagramatic technique to calculate nonlinear Hall conductivity (N… ▽ More The nonlinear Hall effect (NLHE) has been detected in various of condensed matter systems. Unlike linear Hall effect, NLHE may exist in physical systems with broken inversion symmetry in the crystal. On the other hand, real space spin texture may also break inversion symmetry and result in NLHE. In this letter, we employ the Feynman diagramatic technique to calculate nonlinear Hall conductivity (NLHC) in three-dimensional magnetic systems. The results connect NLHE with the physical quantity of emergent electrodynamics which oringates from the magnetic texture. The leading order contribution of NLHC $χ_{abb}$ is proportional to the emergent toroidal moment $\mathcal{T}_{a}^{e}$ which reflects how the spin textures wind in three dimension. △ Less

Submitted 7 October, 2024; v1 submitted 6 September, 2024; originally announced September 2024.

Stoner instabilities and Ising excitonic states in twisted transition metal dichalcogenides

Authors: Augusto Ghiotto, LingNan Wei, Larry Song, Jiawei Zang, Aya Batoul Tazi, Daniel Ostrom, Kenji Watanabe, Takashi Taniguchi, James C. Hone, Daniel A. Rhodes, Andrew J. Millis, Cory R. Dean, Lei Wang, Abhay N. Pasupathy

Abstract: Moiré transition metal dichalcogenide (TMD) systems provide a tunable platform for studying electron-correlation driven quantum phases. Such phases have so far been found at rational fillings of the moiré superlattice, and it is believed that lattice commensurability plays a key role in their stability. In this work, we show via magnetotransport measurements on twisted WSe2 that new correlated ele… ▽ More Moiré transition metal dichalcogenide (TMD) systems provide a tunable platform for studying electron-correlation driven quantum phases. Such phases have so far been found at rational fillings of the moiré superlattice, and it is believed that lattice commensurability plays a key role in their stability. In this work, we show via magnetotransport measurements on twisted WSe2 that new correlated electronic phases can exist away from commensurability. The first phase is an antiferromagnetic metal that is driven by proximity to the van Hove singularity. The second is a re-entrant magnetic field-driven insulator. This insulator is formed from a small and equal density of electrons and holes with opposite spin projections - an Ising excitonic insulator. △ Less

Submitted 27 May, 2024; originally announced May 2024.

Machine learning-based compression of quantum many body physics: PCA and autoencoder representation of the vertex function

Authors: Jiawei Zang, Matija Medvidović, Dominik Kiese, Domenico Di Sante, Anirvan M. Sengupta, Andrew J. Millis

Abstract: Characterizing complex many-body phases of matter has been a central question in quantum physics for decades. Numerical methods built around approximations of the renormalization group (RG) flow equations have offered reliable and systematically improvable answers to the initial question -- what simple physics drives quantum order and disorder? The flow equations are a very high dimensional set of… ▽ More Characterizing complex many-body phases of matter has been a central question in quantum physics for decades. Numerical methods built around approximations of the renormalization group (RG) flow equations have offered reliable and systematically improvable answers to the initial question -- what simple physics drives quantum order and disorder? The flow equations are a very high dimensional set of coupled nonlinear equations whose solution is the two particle vertex function, a function of three continuous momenta that describes particle-particle scattering and encodes much of the low energy physics including whether the system exhibits various forms of long ranged order. In this work, we take a simple and interpretable data-driven approach to the open question of compressing the two-particle vertex. We use PCA and an autoencoder neural network to derive compact, low-dimensional representations of underlying physics for the case of interacting fermions on a lattice. We quantify errors in the representations by multiple metrics and show that a simple linear PCA offers more physical insight and better out-of-distribution (zero-shot) generalization than the nominally more expressive nonlinear models. Even with a modest number of principal components (10 - 20), we find excellent reconstruction of vertex functions across the phase diagram. This result suggests that many other many-body functions may be similarly compressible, potentially allowing for efficient computation of observables. Finally, we identify principal component subspaces that are shared between known phases, offering new physical insight. △ Less

Submitted 22 March, 2024; originally announced March 2024.

Comments: 4 figures

Fast Lithium Ion Diffusion in Brownmillerite $\mathrm{Li}_{x}\mathrm{{Sr}_{2}{Co}_{2}{O}_{5}}$

Authors: Xin Chen, Xixiang Zhang, Jie-Xiang Yu, Jiadong Zang

Abstract: Ionic conductors have great potential for interesting tunable physical properties via ionic liquid gating and novel energy storage applications such as all-solid-state lithium batteries. In particular, low migration barriers and high hopping attempt frequency are the keys to achieve fast ion diffusion in solids. Taking advantage of the oxygen-vacancy channel in… ▽ More Ionic conductors have great potential for interesting tunable physical properties via ionic liquid gating and novel energy storage applications such as all-solid-state lithium batteries. In particular, low migration barriers and high hopping attempt frequency are the keys to achieve fast ion diffusion in solids. Taking advantage of the oxygen-vacancy channel in $\mathrm{Li}_{x}\mathrm{{Sr}_{2}{Co}_{2}{O}_{5}}$, we show that migration barriers of lithium ion are as small as 0.28~0.17eV depending on the lithium concentration rates. Our first-principles calculation also investigated hopping attempt frequency and concluded the room temperature ionic diffusivity and ion conductivity is high as ${10}^{-7}\sim{10}^{-6}~\mathrm{{cm}^{2}~s^{-1}}$ and ${10}^{-3}\sim{10}^{-2}~\mathrm{S\cdot{cm}^{-1}}$ respectively, which outperform most of perovskite-type, garnet-type and sulfide Li-ion solid-state electrolytes. This work proves $\mathrm{Li}_{x}\mathrm{{Sr}_{2}{Co}_{2}{O}_{5}}$ as a promising super-ionic conductor. △ Less

Submitted 10 December, 2024; v1 submitted 27 February, 2024; originally announced February 2024.

Comments: 8 pages, 7 figures

Compressing the two-particle Green's function using wavelets: Theory and application to the Hubbard atom

Authors: Emin Moghadas, Nikolaus Dräger, Alessandro Toschi, Jiawei Zang, Matija Medvidović, Dominik Kiese, Andrew J. Millis, Anirvan M. Sengupta, Sabine Andergassen, Domenico Di Sante

Abstract: Precise algorithms capable of providing controlled solutions in the presence of strong interactions are transforming the landscape of quantum many-body physics. Particularly exciting breakthroughs are enabling the computation of non-zero temperature correlation functions. However, computational challenges arise due to constraints in resources and memory limitations, especially in scenarios involvi… ▽ More Precise algorithms capable of providing controlled solutions in the presence of strong interactions are transforming the landscape of quantum many-body physics. Particularly exciting breakthroughs are enabling the computation of non-zero temperature correlation functions. However, computational challenges arise due to constraints in resources and memory limitations, especially in scenarios involving complex Green's functions and lattice effects. Leveraging the principles of signal processing and data compression, this paper explores the wavelet decomposition as a versatile and efficient method for obtaining compact and resource-efficient representations of the many-body theory of interacting systems. The effectiveness of the wavelet decomposition is illustrated through its application to the representation of generalized susceptibilities and self-energies in a prototypical interacting fermionic system, namely the Hubbard model at half-filling in its atomic limit. These results are the first proof-of-principle application of the wavelet compression within the realm of many-body physics and demonstrate the potential of this wavelet-based compression scheme for understanding the physics of correlated electron systems. △ Less

Submitted 4 September, 2024; v1 submitted 20 February, 2024; originally announced February 2024.

Comments: 25 pages, 16 figures, 2 tables

Journal ref: Eur. Phys. J. Plus 139, 700 (2024)

GPTArticleExtractor: An Automated Workflow for Magnetic Material Database Construction

Authors: Yibo Zhang, Suman Itani, Kamal Khanal, Emmanuel Okyere, Gavin Smith, Koichiro Takahashi, Jiadong Zang

Abstract: A comprehensive database of magnetic materials is valuable for researching the properties of magnetic materials and discovering new ones. This article introduces a novel workflow that leverages large language models for extracting key information from scientific literature. From 22,120 articles in the Journal of Magnetism and Magnetic Materials, a database containing 2,035 magnetic materials was a… ▽ More A comprehensive database of magnetic materials is valuable for researching the properties of magnetic materials and discovering new ones. This article introduces a novel workflow that leverages large language models for extracting key information from scientific literature. From 22,120 articles in the Journal of Magnetism and Magnetic Materials, a database containing 2,035 magnetic materials was automatically generated, with ferromagnetic materials constituting 76% of the total. Each entry in the database includes the material's chemical compounds, as well as related structures (space group, crystal structure) and magnetic temperatures (Curie, N'eel, and other transitional temperatures). To ensure data accuracy, we meticulously compared each entry in the database against the original literature, verifying the precision and reliability of each entry. △ Less

Submitted 11 January, 2024; originally announced January 2024.

Spin scattering and Hall effects in monolayer Fe3GeTe2

Authors: Luyan Yu, Jie-Xiang Yu, Jiadong Zang, Roger K. Lake, Houlong Zhuang, Gen Yin

Abstract: We theoretically show that the carrier transport in monolayer Fe3GeTe2 experiences a transition between anomalous Hall effect and spin Hall effect when the spin polarization of disorders switches between out-of-plane and in-plane. These Hall effects are allowed when the magnetization is polarized in-plane, breaking the C3 rotation symmetry. The transition originates from the selection rule of spin… ▽ More We theoretically show that the carrier transport in monolayer Fe3GeTe2 experiences a transition between anomalous Hall effect and spin Hall effect when the spin polarization of disorders switches between out-of-plane and in-plane. These Hall effects are allowed when the magnetization is polarized in-plane, breaking the C3 rotation symmetry. The transition originates from the selection rule of spin scattering, the strong spin-orbit coupling, and the van Hove singularities near the Fermi surface. The scattering selection rule tolerates the sign change of the disorder spin, which provides a convenient method to detect the switching of antiferromagnetic insulators regardless of the interfacial roughness in a heterostructure. This provides a convenient platform for the study of 2D spintronics through various van-der-Waals heterostructures. △ Less

Submitted 16 May, 2023; originally announced May 2023.

Magnetism and Metallicity in Moiré Transition Metal Dichalcogenides

Authors: Patrick Tscheppe, Jiawei Zang, Marcel Klett, Seher Karakuzu, Armelle Celarier, Zhengqian Cheng, Chris A. Marianetti, Thomas A. Maier, Michel Ferrero, Andrew J. Millis, Thomas Schäfer

Abstract: The ability to control the properties of twisted bilayer transition metal dichalcogenides in situ makes them an ideal platform for investigating the interplay of strong correlations and geometric frustration. Of particular interest are the low energy scales, which make it possible to experimentally access both temperature and magnetic fields that are of the order of the bandwidth or the correlatio… ▽ More The ability to control the properties of twisted bilayer transition metal dichalcogenides in situ makes them an ideal platform for investigating the interplay of strong correlations and geometric frustration. Of particular interest are the low energy scales, which make it possible to experimentally access both temperature and magnetic fields that are of the order of the bandwidth or the correlation scale. In this manuscript we analyze the moiré Hubbard model, believed to describe the low energy physics of an important subclass of the twisted bilayer compounds. We establish its magnetic and the metal-insulator phase diagram for the full range of magnetic fields up to the fully spin polarized state. We find a rich phase diagram including fully and partially polarized insulating and metallic phases of which we determine the interplay of magnetic order, Zeeman-field, and metallicity, and make connection to recent experiments. △ Less

Submitted 27 April, 2023; v1 submitted 23 March, 2023; originally announced March 2023.

Comments: 7+10 pages, 4+9 figures

Journal ref: Proceedings of the National Academy of Sciences 121, 3 (2024)

Experimental observation of one-dimensional motion of interstitial skyrmion in FeGe

Authors: Dongsheng Song, Weiwei Wang, Jie-Xiang Yu, Peng Zhang, Sergey S. Pershoguba, Gen Yin, Wensen Wei, Jialiang Jiang, Binghui Ge, Xiaolong Fan, Mingliang Tian, Achim Rosch, Jiadong Zang, Haifeng Du

Abstract: The interplay between dimensionality and topology manifests in magnetism via both exotic texture morphology and novel dynamics. A free magnetic skyrmion exhibits the skyrmion Hall effect under electric currents. Once it is confined in one-dimensional (1D) channels, the skyrmion Hall effect would be suppressed, and the current-driven skyrmion speed should be boosted by the non-adiabatic spin transf… ▽ More The interplay between dimensionality and topology manifests in magnetism via both exotic texture morphology and novel dynamics. A free magnetic skyrmion exhibits the skyrmion Hall effect under electric currents. Once it is confined in one-dimensional (1D) channels, the skyrmion Hall effect would be suppressed, and the current-driven skyrmion speed should be boosted by the non-adiabatic spin transfer torque \b{eta}. Here, we experimentally demonstrate that stripes of a spatially modulated spin helix serve as natural 1D channels to restrict skyrmion. Using FeGe as a benchmark, an interstitial skyrmion is created by geometry notch and further moves steadily without the skyrmion Hall effect. The slope of the current-velocity curve for 1D skyrmion is enhanced almost by an order of magnitude owing to a large \b{eta} in FeGe. This feature is also observed in other topological defects. Utilizing the 1D skyrmion dynamics would be a highly promising route to implement topological spintronic devices. △ Less

Submitted 17 December, 2022; originally announced December 2022.

Real space representation of topological system: twisted bilayer graphene as an example

Authors: Jiawei Zang, Jie Wang, Antoine Georges, Jennifer Cano, Andrew J. Millis

Abstract: We construct a Wannier basis for twisted bilayer graphene that is projected only from the Bloch functions of the twisted bilayer flat bands. The $C_3$ and $C_{2} \mathcal{T}$ symmetries act locally on the Wannier functions while the Wannier function charge density is strongly peaked at the triangular sites and becomes fully sublattice-polarized in the chiral limit. The Wannier functions have a pow… ▽ More We construct a Wannier basis for twisted bilayer graphene that is projected only from the Bloch functions of the twisted bilayer flat bands. The $C_3$ and $C_{2} \mathcal{T}$ symmetries act locally on the Wannier functions while the Wannier function charge density is strongly peaked at the triangular sites and becomes fully sublattice-polarized in the chiral limit. The Wannier functions have a power-law tail, due to the topological obstruction, but most of the charge density is concentrated within one unit cell so that the on-site local Coulomb interaction is much larger than the further neighbor interactions and in general the Hamiltonian parameters may be accurately estimated from a modest number of Wannier functions. One exception is the momentum space components of the single-particle Hamiltonian, where because of the topological obstruction convergence is non-uniform across the Brillouin zone. We observe, however, that mixed position and momentum space representations may be used to avoid this difficulty in the context of quantum embedding methods. Our work provides a new route to study systems with topological obstructions and paves the way for the future investigation of correlated states in twisted bilayer graphene, including studies of non-integer fillings and temperature dependence. △ Less

Submitted 23 October, 2022; v1 submitted 20 October, 2022; originally announced October 2022.

Comments: 10 pages

Hall Effect Induced by Topologically Trivial Target Skyrmions

Authors: Tan Dao, Sergey S. Pershoguba, Jiadong Zang

Abstract: Electrons moving through a noncoplanar magnetic texture acquire a Berry phase, which can be described as an effective magnetic field. This effect is known as the topological Hall effect and has been observed in topological spin textures. Motivated by recent experimental realizations, here we study the Hall effect in a nontopological magnetic texture known as a target skyrmion. We start from a simp… ▽ More Electrons moving through a noncoplanar magnetic texture acquire a Berry phase, which can be described as an effective magnetic field. This effect is known as the topological Hall effect and has been observed in topological spin textures. Motivated by recent experimental realizations, here we study the Hall effect in a nontopological magnetic texture known as a target skyrmion. We start from a simplified semiclassical picture and show that the Hall signal is a nonmonotonic function of both the electronic energy and target skyrmion radius. That observation carries over to the fully quantum mechanical treatment in a Landauer-Büttiker formalism in a mesoscopic setting. Our conclusion challenges the popular opinion in the community that the Hall effect in such structures necessarily requires a nonzero skyrmion number. △ Less

Submitted 20 October, 2022; originally announced October 2022.

Comments: 7 pages, 6 figures

MagNet: machine learning enhanced three-dimensional magnetic reconstruction

Authors: Boyao Lyu, Shihua Zhao, Yibo Zhang, Weiwei Wang, Haifeng Du, Jiadong Zang

Abstract: Three-dimensional (3D) magnetic reconstruction is vital to the study of novel magnetic materials for 3D spintronics. Vector field electron tomography (VFET) is a major in house tool to achieve that. However, conventional VFET reconstruction exhibits significant artefacts due to the unavoidable presence of missing wedges. In this article, we propose a deep-learning enhanced VFET method to address t… ▽ More Three-dimensional (3D) magnetic reconstruction is vital to the study of novel magnetic materials for 3D spintronics. Vector field electron tomography (VFET) is a major in house tool to achieve that. However, conventional VFET reconstruction exhibits significant artefacts due to the unavoidable presence of missing wedges. In this article, we propose a deep-learning enhanced VFET method to address this issue. A magnetic textures library is built by micromagnetic simulations. MagNet, an U-shaped convolutional neural network, is trained and tested with dataset generated from the library. We demonstrate that MagNet outperforms conventional VFET under missing wedge. Quality of reconstructed magnetic induction fields is significantly improved. △ Less

Submitted 6 October, 2022; originally announced October 2022.

Chiral Kondo Lattice in Doped MoTe$_2$/WSe$_2$ Bilayers

Authors: Daniele Guerci, Jie Wang, Jiawei Zang, Jennifer Cano, J. H. Pixley, Andrew Millis

Abstract: We theoretically study the interplay between magnetism and a heavy Fermi liquid in the AB stacked transition metal dichalcogenide bilayer system MoTe$_2$/WSe$_2$ in the regime in which the Mo layer supports localized magnetic moments coupled by interlayer electron tunnelling to a weakly correlated band of itinerant electrons in the W layer. We show that the interlayer electron transfer leads to a… ▽ More We theoretically study the interplay between magnetism and a heavy Fermi liquid in the AB stacked transition metal dichalcogenide bilayer system MoTe$_2$/WSe$_2$ in the regime in which the Mo layer supports localized magnetic moments coupled by interlayer electron tunnelling to a weakly correlated band of itinerant electrons in the W layer. We show that the interlayer electron transfer leads to a chiral Kondo exchange, with consequences including a strong dependence of the Kondo temperature on carrier concentration, a topological hybridization gap and an anomalous Hall effect. The theoretical model exhibits two phases, a small Fermi surface magnet and a large Fermi surface heavy Fermi liquid; the transition between them is first order. A low-energy theory is developed for the the transport properties of the two states. Implications of our results for present and future experiments on MoTe$_2$/WSe$_2$ bilayer heterostructures are discussed. △ Less

Submitted 1 May, 2023; v1 submitted 13 July, 2022; originally announced July 2022.

Comments: (7+9) pages, (4+6) figures

Journal ref: Science Advances 9, eade7701 (2023)

Tunable Stripe Order and Weak Superconductivity in the Moiré Hubbard Model

Authors: Alexander Wietek, Jie Wang, Jiawei Zang, Jennifer Cano, Antoine Georges, Andrew Millis

Abstract: The moiré Hubbard model describes correlations in certain homobilayer twisted transition metal dichalcogenides. Using exact diagonalization and density matrix renormalization group methods, we find magnetic Mott insulating and metallic phases, which, upon doping exhibit intertwined charge and spin ordering and, in some regimes, pair binding of holes. The phases are highly tunable via an interlayer… ▽ More The moiré Hubbard model describes correlations in certain homobilayer twisted transition metal dichalcogenides. Using exact diagonalization and density matrix renormalization group methods, we find magnetic Mott insulating and metallic phases, which, upon doping exhibit intertwined charge and spin ordering and, in some regimes, pair binding of holes. The phases are highly tunable via an interlayer potential difference. Remarkably, the hole binding energy is found to be highly tunable revealing an experimentally accessible regime where holes become attractive. In this attractive regime, we study the superconducting correlation function and point out the possibility of weak superconductivity. △ Less

Submitted 14 November, 2022; v1 submitted 8 April, 2022; originally announced April 2022.

Comments: 9 pages, 9 figures

Journal ref: Phys. Rev. Research 4, 043048 (2022)

Widely Tunable Berry curvature in the Magnetic Semimetal Cr1+dTe2

Authors: Y. Fujisawa, M. Pardo-Almanza, C. H. Hsu, A. Mohamed, K. Yamagami, A. Krishnadas, F. C. Chuang, K. H. Khoo, J. Zang, A. Soumyanarayanan, Y. Okada

Abstract: Magnetic semimetals have increasingly emerged as lucrative platforms hosting spin-based topological phenomena in real and momentum spaces. Of particular interest is the emergence of Berry curvature, whose geometric origin, accessibility from Hall transport experiments, and material tunability, bodes well for new physics and practical devices. Cr1+dTe2, a self-intercalated magnetic transition metal… ▽ More Magnetic semimetals have increasingly emerged as lucrative platforms hosting spin-based topological phenomena in real and momentum spaces. Of particular interest is the emergence of Berry curvature, whose geometric origin, accessibility from Hall transport experiments, and material tunability, bodes well for new physics and practical devices. Cr1+dTe2, a self-intercalated magnetic transition metal dichalcogenide, TMD, exhibits attractive natural attributes relevant to such applications, including topological magnetism, tunable electron filling, magnetic frustration etc. While recent studies have explored real-space Berry curvature effects in this material, similar considerations of momentum-space Berry curvature are lacking. Here, we systematically investigate the electronic structure and transport properties of epitaxial Cr1+dTe2 thin films over a wide range of doping, d between 0.33 and 0.71. Spectroscopic experiments reveal the presence of a characteristic semi-metallic band region near the Brillouin Zone edge, which shows a rigid band like energy shift as a function of d. Transport experiments show that the intrinsic component of the anomalous Hall effect, AHE, is sizable, and undergoes a sign flip across d. Finally, density functional theory calculations establish a causal link between the observed doping evolution of the band structure and AHE: the AHE sign flip is shown to emerge from the sign change of the Berry curvature, as the semi-metallic band region crosses the Fermi energy. Our findings underscore the increasing relevance of momentum-space Berry curvature in magnetic TMDs and provide a unique platform for intertwining topological physics in real and momentum spaces. △ Less

Submitted 4 July, 2022; v1 submitted 5 April, 2022; originally announced April 2022.

Dynamical Mean Field Theory of Moiré Bilayer Transition Metal Dichalcogenides: Phase Diagram, Resistivity, and Quantum Criticality

Authors: Jiawei Zang, Jie Wang, Jennifer Cano, Antoine Georges, Andrew J. Millis

Abstract: We present a comprehensive dynamical mean field study of the triangular lattice moiré Hubbard model, which is believed to represent the physics of moiré bilayer transition metal dichalcogenides. In these materials, important aspects of the band structure including the bandwidth and the order and location of van Hove singularities can be tuned by varying the interlayer potential. We present a magne… ▽ More We present a comprehensive dynamical mean field study of the triangular lattice moiré Hubbard model, which is believed to represent the physics of moiré bilayer transition metal dichalcogenides. In these materials, important aspects of the band structure including the bandwidth and the order and location of van Hove singularities can be tuned by varying the interlayer potential. We present a magnetic and metal-insulator phase diagram and a detailed study of the dependence of the resistivity on temperature, band filling and interlayer potential. We find that transport displays Fermi liquid, strange metal and quantum critical behaviors in distinct regions of the phase diagram. Specifically, we find that the cube-root van Hove singularity ($ρ(ε) \sim|ε|^{-1 / 3}$) gives a strange metal behavior with a $T$-linear scattering rate and $ω/T$ scaling. We show how magnetic order affects the resistivity. Our results elucidate the physics of the correlated states and the metal-insulator continuous transition recently observed in twisted homobilayer WSe$_2$ and heterobilayer MoTe$_2$/WSe$_2$ experiments. △ Less

Submitted 25 June, 2022; v1 submitted 6 December, 2021; originally announced December 2021.

Comments: 12 pages, 11 figures

Journal ref: Phys. Rev. X 12, 021064 (2022)

Staggered Pseudo Magnetic Field in Twisted Transition Metal Dichalcogenides: Physical Origin and Experimental Consequences

Authors: Jie Wang, Jiawei Zang, Jennifer Cano, Andrew J. Millis

Abstract: Strong magnetic fields profoundly affect the quantum physics of charged particles, as seen for example by the integer and fractionally quantized Hall effects, and the fractal `Hofstadter butterfly' spectrum of electrons in the presence of a periodic potential and a magnetic field. Intrinsic physics can lead to effects equivalent to those produced by an externally applied magnetic field. Examples i… ▽ More Strong magnetic fields profoundly affect the quantum physics of charged particles, as seen for example by the integer and fractionally quantized Hall effects, and the fractal `Hofstadter butterfly' spectrum of electrons in the presence of a periodic potential and a magnetic field. Intrinsic physics can lead to effects equivalent to those produced by an externally applied magnetic field. Examples include the `staggered flux' phases emerging in some theories of quantum spin liquids and the Chern insulator behavior of twisted bilayer graphene when valley symmetry is broken. In this paper we show that when two layers of the transition metal dichalcogenide material WSe2 are stacked at a small relative twist angle to form a Moire bilayer, the resulting low energy physics can be understood in terms of electrons moving in a strong and tunable staggered flux. We predict experimental consequences including sign reversals of the Hall coefficient on application of an interlayer potential and spin currents appearing at sample edges and interfaces. △ Less

Submitted 27 October, 2021; originally announced October 2021.

Journal ref: Phys. Rev. Research 5, L012005 (2022)

Imaging the ultrafast coherent control of a skyrmion crystal

Authors: Phoebe Tengdin, Benoit Truc, Alexey Sapozhnik, Lingyao Kong, Nina del Ser, Simone Gargiulo, Ivan Madan, Thomas Schoenenberger, Priya R. Baral, Ping Che, Arnaud Magrez, Dirk Grundler, Henrik M. Rønnow, Thomas Lagrange, Jiadong Zang, Achim Rosch, Fabrizio Carbone

Abstract: Exotic magnetic textures emerging from the subtle interplay between thermodynamic and topological fluctuation have attracted intense interest due to their potential applications in spintronic devices. Recent advances in electron microscopy have enabled the imaging of random photo-generated individual skyrmions. However, their deterministic and dynamical manipulation is hampered by the chaotic natu… ▽ More Exotic magnetic textures emerging from the subtle interplay between thermodynamic and topological fluctuation have attracted intense interest due to their potential applications in spintronic devices. Recent advances in electron microscopy have enabled the imaging of random photo-generated individual skyrmions. However, their deterministic and dynamical manipulation is hampered by the chaotic nature of such fluctuations and the intrinsically irreversible switching between different minima in the magnetic energy landscape. Here, we demonstrate a method to coherently control the rotation of a skyrmion crystal by discrete amounts at speeds which are much faster than previously observed. By employing circularly polarized femtosecond laser pulses with an energy below the bandgap of the Mott insulator Cu2OSeO3, we excite a collective magnon mode via the inverse Faraday effect. This triggers coherent magnetic oscillations that directly control the rotation of a skyrmion crystal imaged by cryo-Lorentz Transmission Electron Microscopy. The manipulation of topological order via ultrafast laser pulses shown here can be used to engineer fast spin-based logical devices. △ Less

Submitted 22 July, 2022; v1 submitted 9 October, 2021; originally announced October 2021.

Gate-tunable Intrinsic Anomalous Hall Effect in Epitaxial MnBi2Te4 Films

Authors: Shanshan Liu, Jiexiang Yu, Enze Zhang, Zihan Li, Qiang Sun, Yong Zhang, Lun Li, Minhao Zhao, Pengliang Leng, Xiangyu Cao, Jin Zou, Xufeng Kou, Jiadong Zang, Faxian Xiu

Abstract: Anomalous Hall effect (AHE) is an important transport signature revealing topological properties of magnetic materials and their spin textures. Recently, antiferromagnetic MnBi2Te4 has been demonstrated to be an intrinsic magnetic topological insulator that exhibits quantum AHE in exfoliated nanoflakes. However, its complicated AHE behaviors may offer an opportunity for the unexplored correlation… ▽ More Anomalous Hall effect (AHE) is an important transport signature revealing topological properties of magnetic materials and their spin textures. Recently, antiferromagnetic MnBi2Te4 has been demonstrated to be an intrinsic magnetic topological insulator that exhibits quantum AHE in exfoliated nanoflakes. However, its complicated AHE behaviors may offer an opportunity for the unexplored correlation between magnetism and band structure. Here, we show the Berry curvature dominated intrinsic AHE in wafer-scale MnBi2Te4 thin films. By utilizing a high-dielectric SrTiO3 as the back-gate, we unveil an ambipolar conduction and electron-hole carrier (n-p) transition in ~7 septuple layer MnBi2Te4. A quadratic relation between the saturated AHE resistance and longitudinal resistance suggests its intrinsic AHE mechanism. For ~3 septuple layer MnBi2Te4, however, the AHE reverses its sign from pristine negative to positive under the electric-gating. The first-principles calculations demonstrate that such behavior is due to the competing Berry curvature between polarized spin-minority-dominated surface states and spin-majority-dominated inner-bands. Our results shed light on the physical mechanism of the gate-tunable intrinsic AHE in MnBi2Te4 thin films and provide a feasible approach to engineering its AHE. △ Less

Submitted 1 October, 2021; originally announced October 2021.

Comments: 16 pages, 5 figures

Electrical manipulation of skyrmions in a chiral magnet

Authors: Weiwei Wang, Dongsheng Song, Wensen Wei, Pengfei Nan, Shilei Zhang, Binghui Ge, Mingliang Tian, Jiadong Zang, Haifeng Du

Abstract: Writing, erasing and computing are three fundamental operations required by any working electronic devices. Magnetic skyrmions could be basic bits in promising in emerging topological spintronic devices. In particular, skyrmions in chiral magnets have outstanding properties like compact texture, uniform size and high mobility. However, creating, deleting and driving isolated skyrmions, as prototyp… ▽ More Writing, erasing and computing are three fundamental operations required by any working electronic devices. Magnetic skyrmions could be basic bits in promising in emerging topological spintronic devices. In particular, skyrmions in chiral magnets have outstanding properties like compact texture, uniform size and high mobility. However, creating, deleting and driving isolated skyrmions, as prototypes of aforementioned basic operations, have been grand challenge in chiral magnets ever since the discovery of skyrmions, and achieving all these three operations in a single device is highly desirable. Here, by engineering chiral magnet Co$_8$Zn$_{10}$Mn$_2$ into the customized micro-devices for in-situ Lorentz transmission electron microscopy observations, we implement these three operations of skyrmions using nanosecond current pulses with a low a current density about $10^{10}$ A/m$^2$ at room temperature. A notched structure can create or delete magnetic skyrmions depending on the direction and magnitude of current pulses. We further show that the magnetic skyrmions can be deterministically shifted step-by-step by current pulses, allowing the establishment of the universal current-velocity relationship. These experimental results have immediate significance towards the skyrmion-based memory or logic devices. △ Less

Submitted 15 August, 2021; originally announced August 2021.

Comments: 16 pages

Magnetic Skyrmion Bundles and Their Current-Driven Dynamics

Authors: Jin Tang, Yaodong Wu, Weiwei Wang, Lingyao Kong, Boyao Lv, Wensen Wei, Jiadong Zang, Mingliang Tian, Haifeng Du

Abstract: Quantization of topological charges determines the various topological spin textures that are expected to play a key role in future spintronic devices. While the magnetic skyrmion with a unit topological charge Q has been extensively studied, spin textures with other integer valued have not been verified well so far. Here, we report the real-space image, creation, and manipulation of a type of mul… ▽ More Quantization of topological charges determines the various topological spin textures that are expected to play a key role in future spintronic devices. While the magnetic skyrmion with a unit topological charge Q has been extensively studied, spin textures with other integer valued have not been verified well so far. Here, we report the real-space image, creation, and manipulation of a type of multi Q three-dimensional skyrmionic texture, where a circular spin spiral ties a bunch of skyrmion tubes. We define these objects as skyrmion bundles, and show they have arbitrarily integer values Q from negative up to at least 55 in our experiment. These textures behave as quasiparticles in dynamics for the collective motions driven by electric pulses. Similar to the skyrmion, skyrmion bundles with non zero Q exhibit the skyrmion Hall effects with a Hall angle of 62 degree. Of particular interest, the skyrmion bundle with Q = 0 propagates collinearly with respect to the current flow without the skyrmion Hall effect. Our results open a new perspective for possible applications of multi Q magnetic objects in future spintronic devices. △ Less

Submitted 5 August, 2021; originally announced August 2021.

Journal ref: Nature Nanotechnology (2021)

Discrete Quantum Geometry and Intrinsic Spin Hall Effect

Authors: Jie-Xiang Yu, Jiadong Zang, Roger K. Lake, Yi Zhang, Gen Yin

Abstract: We show that the quantum geometry of the Fermi surface can be numerically described by a 3-dimensional discrete quantum manifold. This approach not only avoids singularities in the Fermi sea, but it also enables the precise computation of the intrinsic Hall conductivity resolved in spin, as well as any other local properties of the Fermi surface. The method assures numerical accuracy when the Ferm… ▽ More We show that the quantum geometry of the Fermi surface can be numerically described by a 3-dimensional discrete quantum manifold. This approach not only avoids singularities in the Fermi sea, but it also enables the precise computation of the intrinsic Hall conductivity resolved in spin, as well as any other local properties of the Fermi surface. The method assures numerical accuracy when the Fermi level is arbitrarily close to singularities, and it remains robust when Kramers degeneracy is protected by symmetry. The approach is demonstrated by calculating the anomalous Hall and spin Hall conductivities of a 2-band lattice model of a Weyl semimetal and a full-band ab-initio model of zincblende GaAs. △ Less

Submitted 11 November, 2021; v1 submitted 16 June, 2021; originally announced June 2021.

Hartree-Fock study of the moiré Hubbard model for twisted bilayer transition metal dichalcogenides

Authors: Jiawei Zang, Jie Wang, Jennifer Cano, Andrew J. Millis

Abstract: Twisted bilayer transition metal dichalcogenides have emerged as important model systems for the investigation of correlated electron physics because their interaction strength, carrier concentration, band structure, and inversion symmetry breaking are controllable by device fabrication, twist angle, and most importantly, gate voltage, which can be varied in situ. The low energy physics of some of… ▽ More Twisted bilayer transition metal dichalcogenides have emerged as important model systems for the investigation of correlated electron physics because their interaction strength, carrier concentration, band structure, and inversion symmetry breaking are controllable by device fabrication, twist angle, and most importantly, gate voltage, which can be varied in situ. The low energy physics of some of these materials has been shown to be described by a "moiré Hubbard model" generalized from the usual Hubbard model by the addition of strong, tunable spin orbit coupling and inversion symmetry breaking. In this work, we use a Hartree-Fock approximation to reach a comprehensive understanding of the moiré Hubbard model on the mean field level. We determine the magnetic and metal-insulator phase diagrams, and assess the effects of spin orbit coupling, inversion symmetry breaking, and the tunable van Hove singularity. We also consider the spin and orbital effects of applied magnetic fields. This work provides guidance for experiments and sets the stage for beyond mean-field calculations. △ Less

Submitted 30 August, 2021; v1 submitted 25 May, 2021; originally announced May 2021.

Comments: 11 pages, 11 figures

Journal ref: Phys. Rev. B 104, 075150 (2021)

Electronic scattering off a magnetic hopfion

Authors: Sergey S. Pershoguba, Domenico Andreoli, Jiadong Zang

Abstract: We study scattering of itinerant electrons off a magnetic hopfion in a three-dimensional metallic magnet described by a magnetization vector $\mathbf S(\mathbf r)$. A hopfion is a confined topological soliton of $\mathbf S(\mathbf r)$ characterized by an {\it emergent} magnetic field $B_γ(\mathbf r) \equiv ε_{αβγ} \,\mathbf S\cdot(\nabla_α\mathbf S\times \nabla_β\mathbf S)/4 \neq 0$ with vanishing… ▽ More We study scattering of itinerant electrons off a magnetic hopfion in a three-dimensional metallic magnet described by a magnetization vector $\mathbf S(\mathbf r)$. A hopfion is a confined topological soliton of $\mathbf S(\mathbf r)$ characterized by an {\it emergent} magnetic field $B_γ(\mathbf r) \equiv ε_{αβγ} \,\mathbf S\cdot(\nabla_α\mathbf S\times \nabla_β\mathbf S)/4 \neq 0$ with vanishing average value $\langle \mathbf B(\mathbf r)\rangle = 0$. We evaluate the scattering amplitude in the opposite limits of large and small hopfion radius $R$ using the eikonal and Born approximations, respectively. In both limits, we find that the scattering cross-section contains a skew-scattering component giving rise to the Hall effect within a hopfion plane. That conclusion contests the popular notion that the topological Hall effect in non-collinear magnetic structures necessarily implies $\langle \mathbf B(\mathbf r)\rangle \neq 0$. In the limit of small hopfion radius $pR \ll 1$, we expand the Born series in powers of momentum $p$ and identify different expansion terms corresponding to the hopfion anisotropy, toroidal moment, and skew-scattering. △ Less

Submitted 19 April, 2021; originally announced April 2021.

Comments: 8+4 pages, 3+1 figures

Journal ref: Phys. Rev. B 104, 075102 (2021)

Quantum Criticality in Twisted Transition Metal Dichalcogenides

Authors: Augusto Ghiotto, En-Min Shih, Giancarlo S. S. G. Pereira, Daniel A. Rhodes, Bumho Kim, Jiawei Zang, Andrew J. Millis, Kenji Watanabe, Takashi Taniguchi, James C. Hone, Lei Wang, Cory R. Dean, Abhay N. Pasupathy

Abstract: In moiré heterostructures, gate-tunable insulating phases driven by electronic correlations have been recently discovered. Here, we use transport measurements to characterize the gate-driven metal-insulator transitions and the metallic phase in twisted WSe$_2$ near half filling of the first moiré subband. We find that the metal-insulator transition as a function of both density and displacement fi… ▽ More In moiré heterostructures, gate-tunable insulating phases driven by electronic correlations have been recently discovered. Here, we use transport measurements to characterize the gate-driven metal-insulator transitions and the metallic phase in twisted WSe$_2$ near half filling of the first moiré subband. We find that the metal-insulator transition as a function of both density and displacement field is continuous. At the metal-insulator boundary, the resistivity displays strange metal behaviour at low temperature with dissipation comparable to the Planckian limit. Further into the metallic phase, Fermi-liquid behaviour is recovered at low temperature which evolves into a quantum critical fan at intermediate temperatures before eventually reaching an anomalous saturated regime near room temperature. An analysis of the residual resistivity indicates the presence of strong quantum fluctuations in the insulating phase. These results establish twisted WSe$_2$ as a new platform to study doping and bandwidth controlled metal-insulator quantum phase transitions on the triangular lattice. △ Less

Submitted 23 March, 2021; v1 submitted 17 March, 2021; originally announced March 2021.

Journal ref: Nature 597 (2021) 345-349

Giant nonlinear anomalous Hall effect induced by spin-dependent band structure evolution

Authors: Xiangyu Cao, Jie-Xiang Yu, Pengliang Leng, Changjiang Yi, Yunkun Yang, Shanshan Liu, Lingyao Kong, Zihan Li, Xiang Dong, Youguo Shi, Jiadong Zang, Faxian Xiu

Abstract: Anomalous Hall effect (AHE) is the key transport signature unlocking topological properties of magnetic materials. While AHE is usually proportional to the magnetization, the nonlinearity suggests the existence of complex magnetic and electron orders. Nonlinear AHE includes the topological Hall effect (THE) that has been widely used to identify the presence of spin chirality in real space. But it… ▽ More Anomalous Hall effect (AHE) is the key transport signature unlocking topological properties of magnetic materials. While AHE is usually proportional to the magnetization, the nonlinearity suggests the existence of complex magnetic and electron orders. Nonlinear AHE includes the topological Hall effect (THE) that has been widely used to identify the presence of spin chirality in real space. But it can in principle be induced by band structure evolution via Berry curvatures in the reciprocal space. This effect has been largely overlooked due to the intertwined mechanisms in both real and reciprocal spaces. Here, we observed a giant nonlinear AHE with the resistivity up to 383.5 uohm cm, contributing unprecedentedly 97% of the total Hall response in EuCd2As2. Moreover, it can be further enhanced by tilting the magnetic field 30° away from [001] direction, reaching a large anomalous Hall angle up to 21%. Although it shows exactly the same double-peak feature as THE, our scaling analysis and first-principles calculations reveal that the Berry phase is extremely sensitive to the spin canting, and nonlinear AHE is a consequence of band structure evolution under the external magnetic fields. When the spins gradually tilt from the in-plane antiferromagnetic ground state to out-of-plane direction, band crossing and band inversion occur, introducing a bandgap at Γ point at a canting angle of 45°. That contributes to the enhancement of Berry curvature and consequently a large intrinsic Hall conductivity. Our results unequivocally reveal the sensitive dependence of band structures on spin tilting process under external magnetic fields and its pronounced influence on the transport properties, which also need to be taken into consideration in other magnetic materials. △ Less

Submitted 16 March, 2021; originally announced March 2021.

Nature of the ferromagnetic-antiferromagnetic transition in Y$_{1-x}$La$_{x}$TiO$_{3}$

Authors: S. Hameed, S. El-Khatib, K. P. Olson, B. Yu, T. J. Williams, T. Hong, Q. Sheng, K. Yamakawa, J. Zang, Y. J. Uemura, G. Q. Zhao, C. Q. Jin, L. Fu, Y. Gu, F. Ning, Y. Cai, K. M. Kojima, J. W. Freeland, M. Matsuda, C. Leighton, M. Greven

Abstract: We explore the magnetically-ordered ground state of the isovalently-substituted Mott-insulator Y$_{1-x}$La$_{x}$TiO$_{3}$ for $x$ $\leq$ 0.3 via single crystal growth, magnetometry, neutron diffraction, x-ray magnetic circular dichroism (XMCD), muon spin rotation ($μ$SR) and small-angle neutron scattering (SANS). We find that the decrease in the magnetic transition temperature on approaching the f… ▽ More We explore the magnetically-ordered ground state of the isovalently-substituted Mott-insulator Y$_{1-x}$La$_{x}$TiO$_{3}$ for $x$ $\leq$ 0.3 via single crystal growth, magnetometry, neutron diffraction, x-ray magnetic circular dichroism (XMCD), muon spin rotation ($μ$SR) and small-angle neutron scattering (SANS). We find that the decrease in the magnetic transition temperature on approaching the ferromagnetic (FM) - antiferromagnetic (AFM) phase boundary at the La concentration $x_c$ $\approx$ 0.3 is accompanied by a strong suppression of both bulk and local ordered magnetic moments, along with a volume-wise separation into magnetically-ordered and paramagnetic regions. The thermal phase transition does not show conventional second-order behavior, since neither a clear signature of dynamic critical behavior nor a power-law divergence of the magnetic correlation length is found for the studied substitution range; this finding becomes increasingly obvious with substitution. Finally, from SANS and magnetometry measurements, we discern a crossover from easy-axis to easy-plane magneto-crystalline anisotropy with increasing La substitution. These results indicate complex changes in magnetic structure upon approaching the phase boundary. △ Less

Submitted 15 March, 2021; originally announced March 2021.

Comments: 16 pages, 16 figures

Journal ref: Phys. Rev. B 104, 024410 (2021)

Kondo physics in antiferromagnetic Weyl semimetal Mn3+xSn1-x films

Authors: Durga Khadka, T. R. Thapaliya, Sebastian Hurtado Parra, Xingyue Han, Jiajia Wen, Ryan F. Need, Pravin Khanal, Weigang Wang, Jiadong Zang, James M. Kikkawa, Liang Wu, S. X. Huang

Abstract: Topology and strong electron correlations are crucial ingredients in emerging quantum materials, yet their intersection in experimental systems has been relatively limited to date. Strongly correlated Weyl semimetals, particularly when magnetism is incorporated, offer a unique and fertile platform to explore emergent phenomena in novel topological matter and topological spintronics. The antiferrom… ▽ More Topology and strong electron correlations are crucial ingredients in emerging quantum materials, yet their intersection in experimental systems has been relatively limited to date. Strongly correlated Weyl semimetals, particularly when magnetism is incorporated, offer a unique and fertile platform to explore emergent phenomena in novel topological matter and topological spintronics. The antiferromagnetic Weyl semimetal Mn3Sn exhibits many exotic physical properties such as a large spontaneous Hall effect and has recently attracted intense interest. In this work, we report synthesis of epitaxial Mn3+xSn1-x films with greatly extended compositional range in comparison with that of bulk samples. As Sn atoms are replaced by magnetic Mn atoms, the Kondo effect, which is a celebrated example of strong correlations, emerges, develops coherence, and induces a hybridization energy gap. The magnetic doping and gap opening lead to rich extraordinary properties as exemplified by the prominent DC Hall effects and resonance-enhanced terahertz Faraday rotation. △ Less

Submitted 4 July, 2020; originally announced July 2020.

Journal ref: Science Advances 6, eabc1977 (2020)

Three-dimensional dynamics of magnetic hopfion driven by spin transfer torque

Authors: Yizhou Liu, Wentao Hou, Xiufeng Han, Jiadong Zang

Abstract: Magnetic hopfion is three-dimensional (3D) topological soliton with novel spin structure that would enable exotic dynamics. Here we study the current driven 3D dynamics of a magnetic hopfion with unit Hopf index in a frustrated magnet. Attributed to spin Berry phase and symmetry of the hopfion, the phase space entangles multiple collective coordinates, thus the hopfion exhibits rich dynamics inclu… ▽ More Magnetic hopfion is three-dimensional (3D) topological soliton with novel spin structure that would enable exotic dynamics. Here we study the current driven 3D dynamics of a magnetic hopfion with unit Hopf index in a frustrated magnet. Attributed to spin Berry phase and symmetry of the hopfion, the phase space entangles multiple collective coordinates, thus the hopfion exhibits rich dynamics including longitudinal motion along the current direction, transverse motion perpendicular to the current direction, rotational motion and dilation. Furthermore, the characteristics of hopfion dynamics is determined by the ratio between the non-adiabatic spin transfer torque parameter and the damping parameter. Such peculiar 3D dynamics of magnetic hopfion could shed light on understanding the universal physics of hopfions in different systems and boost the prosperous development of 3D spintronics. △ Less

Submitted 2 January, 2020; originally announced January 2020.

Journal ref: Phys. Rev. Lett. 124, 127204 (2020)

The 2020 Skyrmionics Roadmap

Authors: C. Back, V. Cros, H. Ebert, K. Everschor-Sitte, A. Fert, M. Garst, Tianping Ma, S. Mankovsky, T. L. Monchesky, M. Mostovoy, N. Nagaosa, S. S. P. Parkin, C. Pfleiderer, N. Reyren, A. Rosch, Y. Taguchi, Y. Tokura, K. von Bergmann, Jiadong Zang

Abstract: The notion of non-trivial topological winding in condensed matter systems represents a major area of present-day theoretical and experimental research. Magnetic materials offer a versatile platform that is particularly amenable for the exploration of topological spin solitons in real space such as skyrmions. First identified in non-centrosymmetric bulk materials, the rapidly growing zoology of mat… ▽ More The notion of non-trivial topological winding in condensed matter systems represents a major area of present-day theoretical and experimental research. Magnetic materials offer a versatile platform that is particularly amenable for the exploration of topological spin solitons in real space such as skyrmions. First identified in non-centrosymmetric bulk materials, the rapidly growing zoology of materials systems hosting skyrmions and related topological spin solitons includes bulk compounds, surfaces, thin films, heterostructures, nano-wires and nano-dots. This underscores an exceptional potential for major breakthroughs ranging from fundamental questions to applications as driven by an interdisciplinary exchange of ideas between areas in magnetism which traditionally have been pursued rather independently. The skyrmionics roadmap provides a review of the present state of the art and the wide range of research directions and strategies currently under way. These are, for instance, motivated by the identification of the fundamental structural properties of skyrmions and related textures, processes of nucleation and annihilation in the presence of non-trivial topological winding, an exceptionally efficient coupling to spin currents generating spin transfer torques at tiny current densities, as well as the capability to purpose-design broad-band spin dynamic and logic devices. △ Less

Submitted 5 March, 2020; v1 submitted 31 December, 2019; originally announced January 2020.

Comments: J. Phys. D, accepted for publication

Néel-type skyrmion in WTe2/Fe3GeTe2 van der Waals heterostructure

Authors: Yingying Wu, Senfu Zhang, Gen Yin, Junwei Zhang, Wei Wang, Yang Lin Zhu, Jin Hu, Kin Wong, Chi Fang, Caihua Wan, Xiufeng Han, Qiming Shao, Takashi Taniguchi, Kenji Watanabe, Jiadong Zang, Zhiqiang Mao, Xixiang Zhang, Kang L. Wang

Abstract: The promise of high-density and low-energy-consumption devices motivates the search for layered structures that stabilize chiral spin textures such as topologically protected skyrmions. At the same time, layered structures provide a new platform for the discovery of new physics and effects. Recently discovered long-range intrinsic magnetic orders in the two-dimensional van der Waals materials offe… ▽ More The promise of high-density and low-energy-consumption devices motivates the search for layered structures that stabilize chiral spin textures such as topologically protected skyrmions. At the same time, layered structures provide a new platform for the discovery of new physics and effects. Recently discovered long-range intrinsic magnetic orders in the two-dimensional van der Waals materials offer new opportunities. Here we demonstrate the Dzyaloshinskii-Moriya interaction and Néel-type skyrmions are induced at the WTe2/Fe3GeTe2 interface. Fe3GeTe2 is a ferromagnetic material with strong perpendicular magnetic anisotropy. We demonstrate that the strong spin orbit interaction in 1T'-WTe2 does induce a large interfacial Dzyaloshinskii-Moriya interaction at the interface with Fe3GeTe2 due to the inversion symmetry breaking to stabilize skyrmions. Transport measurements show the topological Hall effect in this heterostructure for temperatures below 100 K. Furthermore, Lorentz transmission electron microscopy is used to directly image Néel-type skyrmions along with aligned and stripe-like domain structure. This interfacial coupling induced Dzyaloshinskii-Moriya interaction is estimated to have a large energy of 1.0 mJ/m^2, which can stabilize the Néel-type skyrmions in this heterostructure. This work paves a path towards the skyrmionic devices based on van der Waals heterostructures. △ Less

Submitted 8 January, 2020; v1 submitted 25 July, 2019; originally announced July 2019.

Comments: 32 pages, 4 figures in the main text

Journal ref: Nature Communications 11, Article number: 3860 (2020)

Valley Anisotropy in Elastic Metamaterials

Authors: Shuaifeng Li, Ingi Kim, Satoshi Iwamoto, Jianfeng Zang, Jinkyu Yang

Abstract: Valley, as a new degree of freedom, raises the valleytronics in fundamental and applied science. The elastic analogs of valley states have been proposed by mimicking the symmetrical structure of either two-dimensional materials or photonic valley crystals. However, the asymmetrical valley construction remains unfulfilled. Here, we present the valley anisotropy by introducing asymmetrical design in… ▽ More Valley, as a new degree of freedom, raises the valleytronics in fundamental and applied science. The elastic analogs of valley states have been proposed by mimicking the symmetrical structure of either two-dimensional materials or photonic valley crystals. However, the asymmetrical valley construction remains unfulfilled. Here, we present the valley anisotropy by introducing asymmetrical design into elastic metamaterials. The elastic valley metamaterials are composed of bio-inspired hard spirals and soft materials. The anisotropic topological nature of valley is verified by asymmetrical distribution of the Berry curvature. We show the high tunability of the Berry curvature both in magnitude and sign enabled by our anisotropic valley metamaterials. Finally, we demonstrate the creation of valley topological insulators and show topologically protected propagation of transverse elastic waves relying on operating frequency. The proposed topological properties of elastic valley metamaterials pave the way to better understanding the valley topology and to creating a new type of topological insulators enabled by an additional valley degree of freedom. △ Less

Submitted 24 April, 2019; originally announced April 2019.

Comments: 22 pages, 7 figures

Journal ref: Phys. Rev. B 100, 195102 (2019)

Magnetic-Resonance-Induced Pseudo-electric Field and Giant Current Response in Axion Insulators

Authors: Jiabin Yu, Jiadong Zang, Chao-Xing Liu

Abstract: A quantized version of the magnetoelectric effect, known as the topological magnetoelectric effect, can exist in a time-reversal invariant topological insulator with all its surface states gapped out by magnetism. This topological phase, called the axion insulator phase, has been theoretically proposed but is still lack of conclusive experimental evidence due to the small signal of topological mag… ▽ More A quantized version of the magnetoelectric effect, known as the topological magnetoelectric effect, can exist in a time-reversal invariant topological insulator with all its surface states gapped out by magnetism. This topological phase, called the axion insulator phase, has been theoretically proposed but is still lack of conclusive experimental evidence due to the small signal of topological magnetoelectric effect. In this work, we propose that the dynamical in-plane magnetization in an axion insulator can generate a "pseudo-electric field", which acts on the surface state of topological insulator films and leads to the non-zero response current. Strikingly, we find that the current at magnetic resonance (either ferromagnetic or anti-ferromagnetic) is larger than that of topological magnetoelectric effect by several orders of magnitude, and thereby serves as a feasible smoking gun to confirm the axion insulator phase in the candidate materials. △ Less

Submitted 16 August, 2019; v1 submitted 28 March, 2019; originally announced March 2019.

Comments: 9 pages and 2 figures

Journal ref: Phys. Rev. B 100, 075303 (2019)

Concurrence of Quantum Anomalous Hall and Topological Hall Effects in Magnetic Topological Insulator Sandwich Heterostructures

Authors: Jue Jiang, Di Xiao, Fei Wang, Jae-Ho Shin, Domenico Andreoli, Jianxiao Zhang, Run Xiao, Yi-Fan Zhao, Morteza Kayyalha, Ling Zhang, Ke Wang, Jiadong Zang, Chaoxing Liu, Nitin Samarth, Moses H. W. Chan, Cui-Zu Chang

Abstract: The quantum anomalous Hall (QAH) effect is a quintessential consequence of non-zero Berry curvature in momentum-space. The QAH insulator harbors dissipation-free chiral edge states in the absence of an external magnetic field. On the other hand, the topological Hall (TH) effect, a transport hallmark of the chiral spin textures, is a consequence of real-space Berry curvature. While both the QAH and… ▽ More The quantum anomalous Hall (QAH) effect is a quintessential consequence of non-zero Berry curvature in momentum-space. The QAH insulator harbors dissipation-free chiral edge states in the absence of an external magnetic field. On the other hand, the topological Hall (TH) effect, a transport hallmark of the chiral spin textures, is a consequence of real-space Berry curvature. While both the QAH and TH effects have been reported separately, their coexistence, a manifestation of entangled chiral edge states and chiral spin textures, has not been reported. Here, by inserting a TI layer between two magnetic TI layers to form a sandwich heterostructure, we realized a concurrence of the TH effect and the QAH effect through electric field gating. The TH effect is probed by bulk carriers, while the QAH effect is characterized by chiral edge states. The appearance of TH effect in the QAH insulating regime is the consequence of chiral magnetic domain walls that result from the gate-induced Dzyaloshinskii-Moriya interaction and occur during the magnetization reversal process in the magnetic TI sandwich samples. The coexistence of chiral edge states and chiral spin textures potentially provides a unique platform for proof-of-concept dissipationless spin-textured spintronic applications. △ Less

Submitted 31 December, 2019; v1 submitted 22 January, 2019; originally announced January 2019.

Comments: 22 pages, 4 figures, the accepted version for Nature Materials

Journal ref: Nature Mater.19,732-737(2020)

Thermally Driven Topology in Frustrated Systems

Authors: Jie-Xiang Yu, Morgan Daly, Jiadong Zang

Abstract: Non-trivial topology in a two-dimensional frustrated spin system with the Dzyaloshinskii-Moriya (DM) interaction was investigated by Monto Carlo simulations. At finite temperatures, thermally driven topology was discovered and was found to be dominant at low magnetic field. This topological charge has a quadratic relation with the DM interaction and linear realtions with the external magnetic fiel… ▽ More Non-trivial topology in a two-dimensional frustrated spin system with the Dzyaloshinskii-Moriya (DM) interaction was investigated by Monto Carlo simulations. At finite temperatures, thermally driven topology was discovered and was found to be dominant at low magnetic field. This topological charge has a quadratic relation with the DM interaction and linear realtions with the external magnetic field or the uniaxial magnetic anisotropy. We also proposed a real frustrated system, the Mn-Bi mono-layer film with exceedingly large DM interaction, to enable thermally driven topology. Other topological non-trivial phases in high magnetic field region were also discussed in this real system. △ Less

Submitted 14 September, 2018; originally announced September 2018.

Journal ref: Phys. Rev. B 99, 104431 (2019)

Topological Hall Effect in Magnetic Topological Insulator Films

Authors: Jian-Xiao Zhang, Domenico Andreoli, Jiadong Zang, Chao-Xing Liu

Abstract: Geometric Berry phase can be induced either by spin-orbit coupling, giving rise to the anomalous Hall effect in ferromagnetic materials, or by chiral spin texture, such as skyrmions, leading to the topological Hall effect. Recent experiments have revealed that both phenomena can occur in topological insulator films with magnetic doping, thus providing us with an intriguing platform to study the in… ▽ More Geometric Berry phase can be induced either by spin-orbit coupling, giving rise to the anomalous Hall effect in ferromagnetic materials, or by chiral spin texture, such as skyrmions, leading to the topological Hall effect. Recent experiments have revealed that both phenomena can occur in topological insulator films with magnetic doping, thus providing us with an intriguing platform to study the interplay between these two phenomena. In this work, we numerically study the anomalous Hall and topological Hall effects in a four-band model that can properly describe the quantum well states in the magnetic topological insulator films by combining Landauer-Buttiker formula and the iterative Green's function method. Our numerical results suggest that spin-orbit coupling in this model plays a different role in the quantum transport in the clean and disordered limits. In the clean limit, spin-orbit coupling mainly influences the longitudinal transport but does not have much effect on topological Hall conductance. Such behavior is further studied through the analytical calculation of scattering cross-section due to skyrmion within the four-band model. In the disordered limit, the longitudinal transport is determined by disorder scattering and spin-orbit coupling is found to affect strongly the topological Hall conductance. This sharp contrast unveils a dramatic interplay between spin-orbit coupling and disorder effect in topological Hall effect in magnetic topological insulator systems. △ Less

Submitted 6 September, 2018; originally announced September 2018.

Comments: 8 pages, 9 figures, 1 supplemental material

Giant perpendicular magnetic anisotropy in Fe/III-V nitride thin films

Authors: Jie-Xiang Yu, Jiadong Zang

Abstract: Large perpendicular magnetic anisotropy (PMA) in transition metal thin films provides a pathway for enabling the intriguing physics of nanomagnetism and developing broad spintronics applications. After decades of searches for promising materials, the energy scale of PMA of transition metal thin films, unfortunately, remains only about 1 meV. This limitation has become a major bottleneck in the dev… ▽ More Large perpendicular magnetic anisotropy (PMA) in transition metal thin films provides a pathway for enabling the intriguing physics of nanomagnetism and developing broad spintronics applications. After decades of searches for promising materials, the energy scale of PMA of transition metal thin films, unfortunately, remains only about 1 meV. This limitation has become a major bottleneck in the development of ultradense storage and memory devices. We discovered unprecedented PMA in Fe thin-film growth on the $(000\bar{1})$ N-terminated surface of III-V nitrides from first-principles calculations. PMA ranges from 24.1 meV/u.c. in Fe/BN to 53.7 meV/u.c. in Fe/InN. Symmetry-protected degeneracy between $x^2-y^2$ and $xy$ orbitals and its lift by the spin-orbit coupling play a dominant role. As a consequence, PMA in Fe/III-V nitride thin films is dominated by first-order perturbation of the spin-orbit coupling, instead of second-order in conventional transition metal/oxide thin films. This game-changing scenario would also open a new field of magnetism on transition metal/nitride interfaces. △ Less

Submitted 11 June, 2018; originally announced June 2018.

Journal ref: Science advances 4(3) eaar7814 (2018)

Binding a Hopfion in Chiral Magnet Nanodisk

Authors: Yizhou Liu, Roger Lake, Jiadong Zang

Abstract: Hopfions are three-dimensional (3D) topological textures characterized by the integer Hopf invariant $Q_H$. Here, we present the realization of a zero--field, stable hopfion spin texture in a magnetic system consisting of a chiral magnet nanodisk sandwiched by two films with perpendicular magnetic anisotropy. The preimages of the spin texture and numerical calculations of $Q_H$ show that the hopfi… ▽ More Hopfions are three-dimensional (3D) topological textures characterized by the integer Hopf invariant $Q_H$. Here, we present the realization of a zero--field, stable hopfion spin texture in a magnetic system consisting of a chiral magnet nanodisk sandwiched by two films with perpendicular magnetic anisotropy. The preimages of the spin texture and numerical calculations of $Q_H$ show that the hopfion has $Q_H=1$. Furthermore, another non-trivial state that includes a monopole--antimonopole pair (MAP) is also stabilized in this system. By applying an external magnetic field, hopfion and MAP states with the same polarization can be switched between each other. The topological transition between the hopfion and the MAP state involves a creation (annihilation) of the MAP and twist of the preimages. Our work paves the way to study non-trivial 3D topological spin textures and stimulates more investigations in the field of 3D spintronics. △ Less

Submitted 26 July, 2018; v1 submitted 5 June, 2018; originally announced June 2018.

Journal ref: Phys. Rev. B 98, 174437 (2018)

Planar Hall effect in antiferromagnetic MnTe thin films

Authors: Gen Yin, Jie-Xiang Yu, Yizhou Liu, Roger K. Lake, Jiadong Zang, Kang L. Wang

Abstract: We show that the spin-orbit coupling (SOC) in alpha-MnTe impacts the transport behavior by generating an anisotropic valence-band splitting, resulting in four spin-polarized pockets near Gamma. A minimal k-dot-p model is constructed to capture this splitting by group theory analysis, a tight-binding model and ab initio calculations. The model is shown to describe the rotation symmetry of the zero-… ▽ More We show that the spin-orbit coupling (SOC) in alpha-MnTe impacts the transport behavior by generating an anisotropic valence-band splitting, resulting in four spin-polarized pockets near Gamma. A minimal k-dot-p model is constructed to capture this splitting by group theory analysis, a tight-binding model and ab initio calculations. The model is shown to describe the rotation symmetry of the zero-field planer Hall effect (PHE). The upper limit of the PHE percentage is shown to be fundamentally determined by the band shape, and is quantitatively estimated to be roughly 31% by first principles. △ Less

Submitted 5 April, 2019; v1 submitted 30 May, 2018; originally announced May 2018.

Journal ref: Phys. Rev. Lett. 122, 106602 (2019)