-
Linear and nonlinear optical responses in the chiral multifold semimetal BeAu: A quantum-geometric perspective
Authors:
Babu Baijnath Prasad,
Taisuke Ozaki
Abstract:
Chiral topological semimetals provide a natural platform for exploring how multifold band topology and quantum geometry manifest in optical and photovoltaic responses. BeAu is a chiral multifold semimetal hosting band crossings at $Γ$, $M$, and $R$ with Chern numbers $C_Γ=-4$, $C_M=-2$, and $C_R=+4$, respectively. In this work, we study the linear optical conductivity and second-order dc photocurr…
▽ More
Chiral topological semimetals provide a natural platform for exploring how multifold band topology and quantum geometry manifest in optical and photovoltaic responses. BeAu is a chiral multifold semimetal hosting band crossings at $Γ$, $M$, and $R$ with Chern numbers $C_Γ=-4$, $C_M=-2$, and $C_R=+4$, respectively. In this work, we study the linear optical conductivity and second-order dc photocurrent responses of BeAu using fully relativistic first-principles calculations. The calculated interband linear optical conductivity, Re $σ_{xx}(ω)$, is quantitatively reproduced by $(e^2/\hbar)ωg_{xx}(ω)$, showing that its spectral features are governed by the photon energy factor and the variation of the photon energy-resolved quantum-metric spectral weight. The linear shift current conductivity is closely related to the symplectic connection, whereas the circular injection current susceptibility is governed by the transition-resolved product of Berry curvature and the interband group velocity difference. At the Fermi level, the linear shift current conductivity reaches approximately -810 $μ$A/V$^2$ at a photon energy of 0.05 eV. Aligning the chemical potential with the multifold crossings strongly reshapes both responses, producing the largest linear shift current conductivity peak for $μ=μ_R$ and pronounced changes in the magnitude and sign of the circular injection current susceptibility. The circular photogalvanic trace is strongly photon-energy and chemical-potential dependent and does not exhibit a broad quantized plateau, indicating competing multiband transitions. Our results establish a unified quantum-geometric description of the linear and nonlinear optical responses of BeAu and identify it as a promising platform for optoelectronic phenomena governed by multifold band topology and quantum geometry.
△ Less
Submitted 19 August, 2026;
originally announced August 2026.
-
Anion Doping Driven Non-Ferroelectric-to-Ferroelectric Phase Transition in Epitaxial Y:HfO2
Authors:
Soumyajyoti Mondal,
Binoy Krishna De,
Asraful Haque,
Shubham Kumar Parate,
Arup Basak,
Naushad Ahemad,
Pramod Kumar Yadav,
Kaushal Tiwari,
Bhagwati Prasad,
Matthew K. Sharpe,
Catia Costa,
Satheesh Krishnamurthy,
Pavan Nukala
Abstract:
Oxygen vacancies are often essential for stabilizing the orthorhombic ferroelectric phase in HfO2, with cationic doping widely employed to introduce such defects. In contrast, systematic studies on anionic doping to induce ferroelectricity remains largely in nascent stages. Here, using epitaxial Y:HfO2 films grown on ITO-buffered YSZ substrates that initially crystallize predominantly in the monoc…
▽ More
Oxygen vacancies are often essential for stabilizing the orthorhombic ferroelectric phase in HfO2, with cationic doping widely employed to introduce such defects. In contrast, systematic studies on anionic doping to induce ferroelectricity remains largely in nascent stages. Here, using epitaxial Y:HfO2 films grown on ITO-buffered YSZ substrates that initially crystallize predominantly in the monoclinic non-polar phase, we demonstrate that post-deposition rapid thermal annealing in N2 atmosphere at 900 °C enables nitrogen incorporation without disrupting epitaxy. As the annealing duration increases from 10 s to 2 min, the monoclinic phase diminishes, accompanied by the emergence of robust ferroelectric hysteresis and a corresponding increase in the orthorhombic phase fraction. Combining independent spectroscopic and compositional analyses, we experimentally establish that nitrogen preferentially incorporates into pre-existing neutral oxygen-vacancy sites, converting them into charged oxygen vacancies that drive the transformation from the non-polar monoclinic phase to the ferroelectric orthorhombic phase. Our epitaxial model platform therefore reveals an anion-mediated defect-engineering pathway for controlling ferroelectricity in Y:HfO2, establishing nitrogen incorporation not merely as a chemical dopant, but as a route to fundamentally reconfigure the defect thermodynamics governing phase stability in fluorite ferroelectrics.
△ Less
Submitted 25 June, 2026; v1 submitted 2 September, 2025;
originally announced September 2025.
-
Axially confined binary quantum droplets: ground states and central vortices
Authors:
Srivatsa B. Prasad,
Thomas P. Billam,
Nick G. Parker
Abstract:
Ultracold miscible mixtures of bosonic gases have been observed to form quantum droplet states stabilized by beyond-mean-field quantum fluctuations. Here we study the properties of the droplets when subjected to harmonic trapping in one dimension, using a combination of numerical, variational and analytical approaches. We map out the phase diagram between bound droplets and the unbound gas state a…
▽ More
Ultracold miscible mixtures of bosonic gases have been observed to form quantum droplet states stabilized by beyond-mean-field quantum fluctuations. Here we study the properties of the droplets when subjected to harmonic trapping in one dimension, using a combination of numerical, variational and analytical approaches. We map out the phase diagram between bound droplets and the unbound gas state and the form of the ground states. We additionally consider how the droplet solutions are modified by the presence of a central vortex and use these results to estimate the critical rotation frequency for vortices to be energetically favored. Our work helps to understand the physics of self-bound droplets and vortex droplets in flattened geometries.
△ Less
Submitted 14 August, 2025; v1 submitted 29 July, 2025;
originally announced July 2025.
-
Crow instability of vortex lines in dipolar superfluids
Authors:
Srivatsa B. Prasad,
Nick G. Parker,
Andrew W. Baggaley
Abstract:
In classical inviscid fluids, antiparallel vortices perturbed by Kelvin waves exhibit the Crow instability, where the mutual interaction of the Kelvin modes renders them dynamically unstable. This results in the approach and reconnection of the vortices, leading to a cascaded decay into ever-smaller vortex loops. Through mean-field simulations we study the Crow instability of quantum vortex lines…
▽ More
In classical inviscid fluids, antiparallel vortices perturbed by Kelvin waves exhibit the Crow instability, where the mutual interaction of the Kelvin modes renders them dynamically unstable. This results in the approach and reconnection of the vortices, leading to a cascaded decay into ever-smaller vortex loops. Through mean-field simulations we study the Crow instability of quantum vortex lines in a superfluid whose atoms are subject to the anisotropic, long-ranged dipole-dipole interaction. We observe that the direction of dipole polarization plays a crucial role in determining the dynamically favored Kelvin modes. The subsequent rate of the instability is linked to the mediation of the vortex curvature by the effective dipole-dipole interaction between the vortices themselves. The vortex curvature is strongly suppressed and modes of lower wavenumber are preferred when the dipole polarization is parallel to the vortices, whereas the curvature is maximized for polarizations along the vortices' separation axis. For polarizations along the binormal axis, modes of higher wavenumber are favorable but the instability rate is considerably inhibited. This paves the way to a deeper understanding of vortex reconnections, vortex loop cascades and turbulence in dipolar superfluids.
△ Less
Submitted 29 September, 2025; v1 submitted 4 July, 2024;
originally announced July 2024.
-
Magnetism-induced second-order nonlinear optical responses in multiferroic BiFeO$_3$
Authors:
Babu Baijnath Prasad,
Guan-Fu Liu,
Guang-Yu Guo
Abstract:
Nonlinear optical (NLO) responses of noncentrosymmetric nonmagnets have drawn a lot of attention in the past decades because of their significance in materials characterization, green energy and device applications. However, the magnetism-induced NLO responses have rarely been studied so far. In this paper, we first extend the numerical calculation friendly formula by Rashkeev $\textit{et al.}$ [P…
▽ More
Nonlinear optical (NLO) responses of noncentrosymmetric nonmagnets have drawn a lot of attention in the past decades because of their significance in materials characterization, green energy and device applications. However, the magnetism-induced NLO responses have rarely been studied so far. In this paper, we first extend the numerical calculation friendly formula by Rashkeev $\textit{et al.}$ [Phys. Rev. B $\textbf{57}$, 3905 (1998)] for second harmonic generation (SHG) in nonmagnetic materials to include magnetic systems and then calculate the magnetism-induced NLO responses of BiFeO$_3$, a multiferroic that exhibits both ferroelectricity and antiferromagnetic (AFM) ordering at room temperature and has a band gap that falls in the visible frequency region. First, we find that the calculated magnetism-induced SHG susceptibilities are large and the SHG intensity is tunable with the reversal of magnetization. In particular, we find a strong magnetic contrast of the SHG signal of approximately 440% at SHG photon energy of 4.82 eV, thus enabling a magnetic control of the SHG in BiFeO$_3$. Also, because of the sensitivity of the SHG signal to the direction of the Néel vector, the SHG can be utilized to detect the reversal of the Néel vector in the AFM materials, which is an important issue for AFM spintronics. Second, the calculated BPVE in BiFeO$_3$ are also strong, being larger than some well-known NLO compounds such as BaTiO$_3$, GaAs, CdS and CdSe. Finally, we analyse the origins of the prominent features in the NLO response spectra in terms of the calculated quantum geometric quantities. Our interesting findings suggest that the magnetism-driven NLO responses in BiFeO$_3$ are significant, anisotropic and tunable, and that understanding the magnetism-driven components of both SHG and BPVE is essential for their applications in, e.g., multiferroic-based photovoltaic devices.
△ Less
Submitted 19 June, 2024;
originally announced June 2024.
-
Vortex pair dynamics in three-dimensional homogeneous dipolar superfluids
Authors:
Srivatsa B. Prasad,
Nick G. Parker,
Andrew W. Baggaley
Abstract:
The static and dynamic properties of vortices in dipolar Bose-Einstein condensates (dBECs) can be considerably modified relative to their nondipolar counterparts by the anisotropic and long-ranged nature of the dipole-dipole interaction. Working in a uniform dBEC, we analyze the structure of single vortices and the dynamics of vortex pairs, investigating the deviations from the nondipolar paradigm…
▽ More
The static and dynamic properties of vortices in dipolar Bose-Einstein condensates (dBECs) can be considerably modified relative to their nondipolar counterparts by the anisotropic and long-ranged nature of the dipole-dipole interaction. Working in a uniform dBEC, we analyze the structure of single vortices and the dynamics of vortex pairs, investigating the deviations from the nondipolar paradigm. For a straight vortex line, we find that the induced dipolar interaction potential is axially anisotropic when the dipole moments have a nonzero projection orthogonal to the vortex line. This results in a corresponding elongation of the vortex core along this projection as well as an anisotropic superfluid phase and enhanced compressibility in the vicinity of the vortex core. Consequently, the trajectories of like-signed vortex pairs are described by a family of elliptical and oval-like curves rather than the familiar circular orbits. Similarly for opposite-signed vortex pairs their translation speeds along the binormal are found to be dipole interaction-dependent. We expect that these findings will shed light on the underlying mechanisms of many-vortex phenomena in dBECs such as quantum turbulence, vortex reconnections, and vortex lattices.
△ Less
Submitted 4 December, 2023; v1 submitted 28 November, 2023;
originally announced November 2023.
-
Vortex depinning in a two-dimensional superfluid
Authors:
I-Kang Liu,
Srivatsa B. Prasad,
Andrew W. Baggaley,
Carlo F. Barenghi,
Toby S. Wood
Abstract:
We employ the Gross--Pitaevskii theory to model a quantized vortex depinning from a small obstacle in a two-dimensional superfluid due to an imposed background superfluid flow. We find that, when the flow's velocity exceeds a critical value, the vortex drifts orthogonally to the flow before subsequently moving parallel to it away from the pinning site. The motion of the vortex around the pinning s…
▽ More
We employ the Gross--Pitaevskii theory to model a quantized vortex depinning from a small obstacle in a two-dimensional superfluid due to an imposed background superfluid flow. We find that, when the flow's velocity exceeds a critical value, the vortex drifts orthogonally to the flow before subsequently moving parallel to it away from the pinning site. The motion of the vortex around the pinning site is also accompanied by an emission of a spiral-shaped sound pulse. Through simulations, we present a phase diagram of the critical flow velocity for vortex depinning together with an empirical formula that illustrates how the critical velocity increases with the height and width of the pinning site. By employing a variety of choices of initial and boundary conditions, we are able to obtain lower and upper bounds on the critical velocity and demonstrate the robustness of these results.
△ Less
Submitted 21 November, 2023; v1 submitted 11 November, 2023;
originally announced November 2023.
-
Voltage-based magnetization switching and reading in magnetoelectric spin-orbit nanodevices
Authors:
Diogo C. Vaz,
Chia-Ching Lin,
John J. Plombon,
Won Young Choi,
Inge Groen,
Isabel C. Arango,
Andrey Chuvilin,
Luis E. Hueso,
Dmitri E. Nikonov,
Hai Li,
Punyashloka Debashis,
Scott B. Clendenning,
Tanay A. Gosavi,
Yen-Lin Huang,
Bhagwati Prasad,
Ramamoorthy Ramesh,
Aymeric Vecchiola,
Manuel Bibes,
Karim Bouzehouane,
Stephane Fusil,
Vincent Garcia,
Ian A. Young,
Fèlix Casanova
Abstract:
As CMOS technologies face challenges in dimensional and voltage scaling, the demand for novel logic devices has never been greater, with spin-based devices offering scaling potential, at the cost of significantly high switching energies. Alternatively, magnetoelectric materials are predicted to enable low-power magnetization control, a solution with limited device-level results. Here, we demonstra…
▽ More
As CMOS technologies face challenges in dimensional and voltage scaling, the demand for novel logic devices has never been greater, with spin-based devices offering scaling potential, at the cost of significantly high switching energies. Alternatively, magnetoelectric materials are predicted to enable low-power magnetization control, a solution with limited device-level results. Here, we demonstrate voltage-based magnetization switching and reading in nanodevices at room temperature, enabled by exchange coupling between multiferroic BiFeO$_3$ and ferromagnetic CoFe, for writing, and spin-to-charge current conversion between CoFe and Pt, for reading. We show that upon the electrical switching of the BiFeO$_3$, the magnetization of the CoFe can be reversed, giving rise to different voltage outputs. Through additional microscopy techniques, magnetization reversal is linked with the polarization state and antiferromagnetic cycloid propagation direction in the BiFeO$_3$. This study constitutes the building block for magnetoelectric spin-orbit logic, opening a new avenue for low-power beyond-CMOS technologies.
△ Less
Submitted 30 October, 2024; v1 submitted 23 February, 2023;
originally announced February 2023.
-
Helicity-tunable spin Hall and spin Nernst effects in unconventional chiral fermion semimetals XY (X=Co, Rh; Y=Si, Ge)
Authors:
Ting-Yun Hsieh,
Babu Baijnath Prasad,
Guang-Yu Guo
Abstract:
Transition metal monosilicides CoSi, CoGe, RhSi and RhGe in the chiral cubic B20 structure have recently been found to host unconventional chiral fermions beyond spin-1/2 WFs, and also exhibit exotic physical phenomena such as long Fermi arc surface states, GME and quantized CPGE. Thus, exploring novel spin-related transports in these unconventional chiral fermion semimetals may open a new door fo…
▽ More
Transition metal monosilicides CoSi, CoGe, RhSi and RhGe in the chiral cubic B20 structure have recently been found to host unconventional chiral fermions beyond spin-1/2 WFs, and also exhibit exotic physical phenomena such as long Fermi arc surface states, GME and quantized CPGE. Thus, exploring novel spin-related transports in these unconventional chiral fermion semimetals may open a new door for spintronics and spin caloritronics. In this paper, we study the intrinsic SHE and SNE in the CoSi family based on ab initio relativistic band structure calculations. First, we find that unlike nonchiral cubic metals, the CoSi family have two independent nonzero SHC (SNC) tensor elements, namely, $σ_{xy}^z$ and $σ_{xz}^y$ ($α_{xy}^z$ and $α_{xz}^y$) instead of one element. Furthermore, the SHC ($σ_{xy}^z$ and $σ_{xz}^y$) and helicity of the chiral structure are found to be correlated, thus enabling SHE detection of structural helicity and also chiral fermion chirality. Second, the intrinsic SHE and SNE in some of the CoSi family are large. In particular, the calculated SHC of RhGe is as large as -140 ($\hbar$/e)(S/cm). The calculated SNC of CoGe is also large, being -1.3 ($\hbar$/e)(A/m K) at room temperature. Due to their semimetallic nature with low electrical conductivity, these topological semimetals may have large spin Hall and spin Nernst angles, being comparable to that of Pt metal. The SHC and SNC of these compounds can also be increased by raising or lowering $μ$ to, e.g., the topological nodes, via either chemical doping or electrical gating. Our findings thus indicate that the CoSi family not only would provide a material platform for exploring novel spin-transports and exotic phenomena in unconventional chiral fermion semimetals but also could be promising materials for developing better spintronic and spin caloritronic devices.
△ Less
Submitted 23 September, 2022; v1 submitted 20 May, 2022;
originally announced May 2022.
-
Magnetic and electronic ordering phenomena in the [Ru$_2$O$_6$] honeycomb lattice compound AgRuO$_3$
Authors:
Walter Schnelle,
Beluvalli E. Prasad,
Claudia Felser,
Martin Jansen,
Evgenia V. Komleva,
Sergey V. Streltsov,
Igor I. Mazin,
Dmitry Khalyavin,
Pascal Manuel,
Sukanya Pal,
D. V. S. Muthu,
A. K. Sood,
Ekaterina S. Klyushina,
Bella Lake,
Jean-Christophe Orain,
Hubertus Luetkens
Abstract:
The silver ruthenium oxide AgRuO$_3$ consists of honeycomb [Ru$_2^{5+}$O$_6^{2-}$] layers, and can be considered an analogue of SrRu$_2$O$_6$ with a different intercalation stage. We present measurements of magnetic susceptibility and specific heat on AgRuO$_3$ single crystals which reveal a sharp antiferromagnetic transition at 342(3)K. The electrical transport in single crystals of AgRuO$_3$ is…
▽ More
The silver ruthenium oxide AgRuO$_3$ consists of honeycomb [Ru$_2^{5+}$O$_6^{2-}$] layers, and can be considered an analogue of SrRu$_2$O$_6$ with a different intercalation stage. We present measurements of magnetic susceptibility and specific heat on AgRuO$_3$ single crystals which reveal a sharp antiferromagnetic transition at 342(3)K. The electrical transport in single crystals of AgRuO$_3$ is determined by a combination of activated conduction over an intrinsic semiconducting gap of $\approx$ 100 meV and carriers trapped and thermally released from defects. From powder neutron diffraction data a Néel-type antiferromagnetic structure with the Ru moments along the $c$ axis is derived. Raman and muon spin rotation spectroscopy measurements on AgRuO$_3$ powder samples indicate a further weak phase transition or a crossover in the temperature range 125-200 K. The transition does not show up in magnetic susceptibility and its origin is argued to be related to defects but cannot be fully clarified. The experimental findings are complemented by DFT-based electronic structure calculations. It is found that the magnetism in AgRuO$_3$ is similar to that of SrRu$_2$O$_6$, however with stronger intralayer and weaker interlayer magnetic exchange interactions.
△ Less
Submitted 8 March, 2021;
originally announced March 2021.
-
Arbitrary-angle rotation of the polarization of a dipolar Bose-Einstein condensate
Authors:
S. B. Prasad,
B. C. Mulkerin,
A. M. Martin
Abstract:
We have employed the theory of harmonically trapped dipolar Bose-Einstein condensates to examine the influence of a uniform magnetic field that rotates at an arbitrary angle to its own orientation. This is achieved by semi-analytically solving the dipolar superfluid hydrodynamics of this system within the Thomas-Fermi approximation and by allowing the body frame of the condensate's density profile…
▽ More
We have employed the theory of harmonically trapped dipolar Bose-Einstein condensates to examine the influence of a uniform magnetic field that rotates at an arbitrary angle to its own orientation. This is achieved by semi-analytically solving the dipolar superfluid hydrodynamics of this system within the Thomas-Fermi approximation and by allowing the body frame of the condensate's density profile to be tilted with respect to the symmetry axes of the nonrotating harmonic trap. This additional degree of freedom manifests itself in the presence of previously unknown stationary solution branches for any given dipole tilt angle. We also find that the tilt angle of the stationary state's body frame with respect to the rotation axis is a nontrivial function of the trapping geometry, rotation frequency and dipole tilt angle. For rotation frequencies of at least an order of magnitude higher than the in-plane trapping frequency, the stationary state density profile is almost perfectly equivalent to the profile expected in a time-averaged dipolar potential that effectively vanishes when the dipoles are tilted along the `magic angle', $54.7 °$. However, by linearizing the fully time-dependent superfluid hydrodynamics about these stationary states, we find that they are dynamically unstable against the formation of collective modes, which we expect would result in turbulent decay.
△ Less
Submitted 23 March, 2021; v1 submitted 20 October, 2020;
originally announced October 2020.
-
Tunable spin Hall and spin Nernst effects in Dirac line-node semimetals XCuYAs (X=Zr, Hf; Y=Si, Ge)
Authors:
Babu Baijnath Prasad,
Guang-Yu Guo
Abstract:
The quaternary arsenide compounds XCuYAs (X=Zr, Hf; Y= Si, Ge) belong to the vast family of the 1111-type quaternary compounds, which possess outstanding physical properties ranging from $p$-type transparent semiconductors to high-temperature Fe-based superconductors. In this paper, we study the electronic structure topology, spin Hall effect (SHE) and spin Nernst effect (SNE) in these compounds b…
▽ More
The quaternary arsenide compounds XCuYAs (X=Zr, Hf; Y= Si, Ge) belong to the vast family of the 1111-type quaternary compounds, which possess outstanding physical properties ranging from $p$-type transparent semiconductors to high-temperature Fe-based superconductors. In this paper, we study the electronic structure topology, spin Hall effect (SHE) and spin Nernst effect (SNE) in these compounds based on density functional theory calculations. First we find that the four considered compounds are Dirac semimetals with the nonsymmorphic symmetry-protected Dirac line nodes along the Brillouin zone boundary $A$-$M$ and $X$-$R$ and low density of states (DOS) near the Fermi level ($E_F$). Second, the intrinsic SHE and SNE in some of these considered compounds are found to be large. In particular, the calculated spin Hall conductivity (SHC) of HfCuGeAs is as large as -514 ($\hbar$/e)(S/cm). The spin Nernst conductivity (SNC) of HfCuGeAs at room temperature is also large, being -0.73 ($\hbar$/e)(A/m-K). Moreover, both the magnitude and sign of the SHC and SNC in these compounds can be manipulated by varying either the applied electric field direction or spin current direction. The SHE and SNE in these compounds can also be enhanced by tuning the Fermi level via chemical doping or electric gating. Finally, a detailed analysis of the band-decomposed and $k$-resolved spin Berry curvatures reveals that these large SHC and SNC as well as their notable tunabilities originate largely from the presence of a large number of spin-orbit coupling-gapped Dirac points near the Fermi level as well as the gapless Dirac line-nodes, which give rise to large spin Berry curvatures. Our findings thus suggest that the four XCuYAs compounds not only provide a valuable platform for exploring the interplay between SHE, SNE and band topology but also have promising applications in spintronics and spin caloritronics.
△ Less
Submitted 30 July, 2020;
originally announced July 2020.
-
Charge transfer energy in iridates: a hard x-ray photoelectron spectroscopy study
Authors:
D. Takegami,
D. Kasinathan,
K. K. Wolff,
S. G. Altendorf,
C. F. Chang,
K. Hoefer,
A. Melendez-Sans,
Y. Utsumi,
F. Meneghin,
T. D. Ha,
C. H. Yen,
K. Chen,
C. Y. Kuo,
Y. F. Liao,
K. D. Tsuei,
R. Morrow,
S. Wurmehl,
B. Büchner,
B. E. Prasad,
M. Jansen,
A. C. Komarek,
P. Hansmann,
L. H. Tjeng
Abstract:
We have investigated the electronic structure of iridates in the double perovskite crystal structure containing either Ir$^{4+}$ or Ir$^{5+}$ using hard x-ray photoelectron spectroscopy. The experimental valence band spectra can be well reproduced using tight binding calculations including only the Ir $5d$, O $2p$ and O $2s$ orbitals with parameters based on the downfolding of the density-function…
▽ More
We have investigated the electronic structure of iridates in the double perovskite crystal structure containing either Ir$^{4+}$ or Ir$^{5+}$ using hard x-ray photoelectron spectroscopy. The experimental valence band spectra can be well reproduced using tight binding calculations including only the Ir $5d$, O $2p$ and O $2s$ orbitals with parameters based on the downfolding of the density-functional band structure results. We found that regardless of the A and B cations, the A$_2$BIrO$_6$ iridates have essentially zero O $2p$ to Ir $5d$ charge transfer energies. Hence, double perovskite iridates turn out to be extremely covalent systems with the consequence being that the magnetic exchange interactions become very long-ranged, thereby hampering the materialization of the long-sought Kitaev physics. Nevertheless, it still would be possible to realize a spin-liquid system using the iridates with a proper tuning of the various competing exchange interactions.
△ Less
Submitted 25 May, 2020;
originally announced May 2020.
-
Stationary states, dynamical stability, and vorticity of Bose-Einstein condensates in tilted rotating harmonic traps
Authors:
Srivatsa B. Prasad,
Brendan C. Mulkerin,
Andrew M. Martin
Abstract:
We theoretically investigate a Bose-Einstein condensate confined by a rotating harmonic trap whose rotation axis is not aligned with any of its principal axes. The principal axes of the Thomas-Fermi density profiles of the resulting stationary solutions are found to be tilted with respect to those of the rotating trap, representing an extra degree of freedom that is associated with the existence o…
▽ More
We theoretically investigate a Bose-Einstein condensate confined by a rotating harmonic trap whose rotation axis is not aligned with any of its principal axes. The principal axes of the Thomas-Fermi density profiles of the resulting stationary solutions are found to be tilted with respect to those of the rotating trap, representing an extra degree of freedom that is associated with the existence of additional branches of stationary solutions for any given rotation axis alignment. By linearizing the time-dependent theory about the stationary states, we obtain a semi-analytical prediction of their dynamical instability at high rotation frequencies against collective modes arising from environmental perturbations. Comparing the stationary states to direct simulations of the Gross-Pitaevskii equation, we predict the nucleation of quantum vortices in the dynamically unstable rotational regime. These vortex lines are aligned along the rotation axis despite the tilting of the rotating trap although the background density profile is tilted with respect to the trapping and rotation axes.
△ Less
Submitted 11 May, 2020; v1 submitted 6 April, 2020;
originally announced April 2020.
-
Vortex Lattice Formation in Dipolar Bose-Einstein Condensates via Rotation of the Polarization
Authors:
Srivatsa B. Prasad,
Thomas Bland,
Brendan C. Mulkerin,
Nick G. Parker,
Andrew M. Martin
Abstract:
The behaviour of a harmonically trapped dipolar Bose-Einstein condensate with its dipole moments rotating at angular frequencies lower than the transverse harmonic trapping frequency is explored in the co-rotating frame. We obtain semi-analytical solutions for the stationary states in the Thomas-Fermi limit of the corresponding dipolar Gross-Pitaevskii equation and utilise linear stability analysi…
▽ More
The behaviour of a harmonically trapped dipolar Bose-Einstein condensate with its dipole moments rotating at angular frequencies lower than the transverse harmonic trapping frequency is explored in the co-rotating frame. We obtain semi-analytical solutions for the stationary states in the Thomas-Fermi limit of the corresponding dipolar Gross-Pitaevskii equation and utilise linear stability analysis to elucidate a phase diagram for the dynamical stability of these stationary solutions with respect to collective modes. These results are verified via direct numerical simulations of the dipolar Gross-Pitaevskii equation, which demonstrate that dynamical instabilities of the co-rotating stationary solutions lead to the seeding of vortices that eventually relax into a triangular lattice configuration. Our results illustrate that rotation of the dipole polarization represents a new route to vortex formation in dipolar Bose-Einstein condensates.
△ Less
Submitted 7 August, 2019; v1 submitted 20 June, 2019;
originally announced June 2019.
-
A high-energy density antiferroelectric made by interfacial electrostatic engineering
Authors:
Julia A. Mundy,
Colin A. Heikes,
Bastien F. Grosso,
Dan Ferenc Segedin,
Zhe Wang,
Berit H. Goodge,
Quintin N. Meier,
Christopher T. Nelson,
Bhagwati Prasad,
Lena F. Kourkoutis,
William D. Ratcliff,
Nicola A. Spaldin,
Ramamoorthy Ramesh,
Darrell G. Schlom
Abstract:
Dielectric capacitors hold a tremendous advantage for energy storage due to their fast charge/discharge times and stability in comparison to batteries and supercapacitors. A key limitation to today's dielectric capacitors, however, is the low storage capacity of conventional dielectric materials. To mitigate this issue, antiferroelectric materials have been proposed, but relatively few families of…
▽ More
Dielectric capacitors hold a tremendous advantage for energy storage due to their fast charge/discharge times and stability in comparison to batteries and supercapacitors. A key limitation to today's dielectric capacitors, however, is the low storage capacity of conventional dielectric materials. To mitigate this issue, antiferroelectric materials have been proposed, but relatively few families of antiferroelectric materials have been identified to date. Here, we propose a new design strategy for the construction of lead-free antiferroelectric materials using interfacial electrostatic engineering. We begin with a ferroelectric material with one of the highest known bulk polarizations, BiFeO3. We show that by confining atomically-precise thin layers of BiFeO3 in a dielectric matrix that we can induce a metastable antiferroelectric structure. Application of an electric field reversibly switches between this new phase and a ferroelectric state, in addition, tuning of the dielectric layer causes coexistence of the ferroelectric and antiferroelectric states. Precise engineering of the structure generates an antiferroelectric phase with energy storage comparable to that of the best lead-based materials. The use of electrostatic confinement provides a new pathway for the design of engineered antiferroelectric materials with large and potentially coupled responses.
△ Less
Submitted 22 December, 2018;
originally announced December 2018.
-
Instability of Rotationally Tuned Dipolar Bose-Einstein Condensates
Authors:
S. B. Prasad,
T. Bland,
B. C. Mulkerin,
N. G. Parker,
A. M. Martin
Abstract:
The possibility of effectively inverting the sign of the dipole-dipole interaction, by fast rotation of the dipole polarization, is examined within a harmonically trapped dipolar Bose-Einstein condensate. Our analysis is based on the stationary states in the Thomas-Fermi limit, in the corotating frame, as well as direct numerical simulations in the Thomas-Fermi regime, explicitly accounting for th…
▽ More
The possibility of effectively inverting the sign of the dipole-dipole interaction, by fast rotation of the dipole polarization, is examined within a harmonically trapped dipolar Bose-Einstein condensate. Our analysis is based on the stationary states in the Thomas-Fermi limit, in the corotating frame, as well as direct numerical simulations in the Thomas-Fermi regime, explicitly accounting for the rotating polarization. The condensate is found to be inherently unstable due to the dynamical instability of collective modes. This ultimately prevents the realization of robust and long-lived rotationally tuned states. Our findings have major implications for experimentally accessing this regime.
△ Less
Submitted 12 February, 2019; v1 submitted 21 October, 2018;
originally announced October 2018.
-
Effective Three-Body Interactions in Jaynes-Cummings-Hubbard Systems
Authors:
Srivatsa B. Prasad,
Andrew M. Martin
Abstract:
A generalisation of the Jaynes-Cummings-Hubbard model for coupled-cavity arrays is introduced, where the embedded two-level system in each cavity is replaced by a $Ξ$-type three-level system. We demonstrate that the resulting effective polariton-polariton interactions at each site are both two-body and three-body. By tuning the ratio of the two transition dipole matrix elements, we show that the s…
▽ More
A generalisation of the Jaynes-Cummings-Hubbard model for coupled-cavity arrays is introduced, where the embedded two-level system in each cavity is replaced by a $Ξ$-type three-level system. We demonstrate that the resulting effective polariton-polariton interactions at each site are both two-body and three-body. By tuning the ratio of the two transition dipole matrix elements, we show that the strength and sign of the two-body interaction can be controlled whilst maintaining a three-body repulsion. We then proceed to demonstrate how different two-body and three-body interactions alter the mean field superfluid-Mott insulator phase diagram, with the possible emergence of a pair superfluid phase in the two-body attractive regime.
△ Less
Submitted 21 October, 2018; v1 submitted 6 October, 2017;
originally announced October 2017.
-
Superconductivity at 4K in Pd deficient layered Ta_2Pd_xS_6
Authors:
Brajesh Tiwari,
Babu Baijnath Prasad,
Rajveer Jha,
Dharmendra Kumar Singh,
V. P. S. Awana
Abstract:
Here in this short note, we report on the low dimensional 4d and 5d transition metals-chalcogenide based compounds i.e., Ta2PdxS6, showing semiconducting to superconducting transition around 4K with upper critical field outside Pauli paramagnetic limit. It seems couple of different superconducting phases do exist in these new set of compounds. Our short note in this regards is thought provoking, a…
▽ More
Here in this short note, we report on the low dimensional 4d and 5d transition metals-chalcogenide based compounds i.e., Ta2PdxS6, showing semiconducting to superconducting transition around 4K with upper critical field outside Pauli paramagnetic limit. It seems couple of different superconducting phases do exist in these new set of compounds. Our short note in this regards is thought provoking, asking to explore various unearthed possible superconducting phases in (Nb/Ta)2Pdx(S/Se/Te)y systems.
△ Less
Submitted 20 August, 2014; v1 submitted 7 July, 2014;
originally announced July 2014.