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The MARTINI Platform (I): Se I-X atomic calculation and expansion opacity for early-stage kilonova spectral analysis
Authors:
Matteo Bezmalinovich,
Mattia Bulla,
Gediminas Gaigalas,
Diego Vescovi,
Matteo Canzari,
Sergio Cristallo
Abstract:
Kilonovae represent key sites of r-process nucleosynthesis, making opacity estimation and spectral analysis crucial for constraining their composition. Since light r-process elements shape the early ($\sim$0.5-1.5$\mathrm{d}$) ejecta opacity, a detailed study of the selenium element with a focus on atomic data calculation, expansion opacity estimation and spectral analysis is presented. Se atomic…
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Kilonovae represent key sites of r-process nucleosynthesis, making opacity estimation and spectral analysis crucial for constraining their composition. Since light r-process elements shape the early ($\sim$0.5-1.5$\mathrm{d}$) ejecta opacity, a detailed study of the selenium element with a focus on atomic data calculation, expansion opacity estimation and spectral analysis is presented. Se atomic data are calculated from Se I to Se X using the GRASP2018 code. A systematic analysis and evaluation of their precision is performed through detailed comparison with the NIST ASD, and other works available in the literature. These atomic data are then used to estimate expansion opacity at different temperatures (e.g., T=5000 K, 10000 K, 20000 K, 100000 K) and densities (e.g., $ρ= 10^{-13}\,\mathrm{g\,cm^{-3}},\,3\times10^{-12}\,\mathrm{g\,cm^{-3}}$). Spectral analysis has been performed with radiative transfer code POSSIS with a pre-computed opacity grid calculated with new densities and temperatures, ranging from -19.5 to -4.5 $\mathrm{g\,cm^{-3}}$ in log-scale and from 1 000 to 51 000 K, respectively. Two scenarios are considered: one in which the opacity contribution comes from 100\% Se ejecta, and another in which Se contributes only partially to the total opacity ($\sim$ 10\% of the total mass). Se atomic calculations show a good agreement with NIST ASD, with accurate energy levels and transitions determined alongside atomic data for higher ionisation stages not fully covered by NIST. The expansion opacities calculated with these new Se data exhibit differences in comparison to existing literature works. Se spectral features can only be observed in the KN scenario consisting of 100\% Se. When Se accounts for about 10\% of the total KN mass, these features become undetectable. All Se results are now available in the new open-source MARTINI platform dedicated to element nucleosynthesis.
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Submitted 26 February, 2026;
originally announced February 2026.
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Towards a new generation of solid total-energy detectors for neutron-capture time-of-flight experiments with intense neutron beams
Authors:
J. Balibrea-Correa,
V. Babiano-Suarez,
J. Lerendegui-Marco,
C. Domingo-Pardo,
I. Ladarescu,
A. Tarifeño-Saldivia,
G. de la Fuente-Rosales,
B. Gameiro,
N. Zaitseva,
V. Alcayne,
D. Cano-Ott,
E. González-Romero,
T. Martínez,
E. Mendoza,
A. Pérez de Rada,
J. Plaza del Olmo,
A. Sánchez-Caballero,
A. Casanovas,
F. Calviño,
S. Valenta,
O. Aberle,
S. Altieri,
S. Amaducci,
J. Andrzejewski,
M. Bacak
, et al. (112 additional authors not shown)
Abstract:
Challenging neutron-capture cross-section measurements of small cross sections and samples with a very limited number of atoms require high-flux time-of-flight facilities. In turn, such facilities need innovative detection setups that are fast, have low sensitivity to neutrons, can quickly recover from the so-called $γ$-flash, and offer the highest possible detection sensitivity. In this paper, we…
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Challenging neutron-capture cross-section measurements of small cross sections and samples with a very limited number of atoms require high-flux time-of-flight facilities. In turn, such facilities need innovative detection setups that are fast, have low sensitivity to neutrons, can quickly recover from the so-called $γ$-flash, and offer the highest possible detection sensitivity. In this paper, we present several steps toward such advanced systems. Specifically, we describe the performance of a high-sensitivity experimental setup at CERN n\_TOF EAR2. It consists of nine sTED detector modules in a compact cylindrical configuration, two conventional used large-volume C$_{6}$D$_{6}$ detectors, and one LaCl$_{3}$(Ce) detector. The performance of these detection systems is compared using $^{93}$Nb($n$,$γ$) data. We also developed a detailed \textsc{Geant4} Monte Carlo model of the experimental EAR2 setup, which allows for a better understanding of the detector features, including their efficiency determination. This Monte Carlo model has been used for further optimization, thus leading to a new conceptual design of a $γ$ detector array, STAR, based on a deuterated-stilbene crystal array. Finally, the suitability of deuterated-stilbene crystals for the future STAR array is investigaged experimentally utilizing a small stilbene-d12 prototype. The results suggest a similar or superior performance of STAR with respect to other setups based on liquid-scintillators, and allow for additional features such as neutron-gamma discrimination and a higher level of customization capability.
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Submitted 28 November, 2024;
originally announced November 2024.
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Pushing the high count rate limits of scintillation detectors for challenging neutron-capture experiments
Authors:
J. Balibrea Correa,
J. Lerendegui-Marco,
V. Babiano-Suarez,
C. Domingo-Pardo,
I. Ladarescu,
A. Tarifeño-Saldivia,
V. Alcayne,
D. Cano-Ott,
E. González-Romero,
T. Martínez,
E. Mendoza,
A. Pérez de Rada,
J. Plaza del Olmo,
A. Sánchez-Caballero,
A. Casanovas,
F. Calviño,
S. Valenta,
O. Aberle,
S. Altieri,
S. Amaducci,
J. Andrzejewski,
M. Bacak,
C. Beltrami,
S. Bennett,
A. P. Bernardes
, et al. (109 additional authors not shown)
Abstract:
One of the critical aspects for the accurate determination of neutron capture cross sections when combining time-of-flight and total energy detector techniques is the characterization and control of systematic uncertainties associated to the measuring devices. In this work we explore the most conspicuous effects associated to harsh count rate conditions: dead-time and pile-up effects. Both effects…
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One of the critical aspects for the accurate determination of neutron capture cross sections when combining time-of-flight and total energy detector techniques is the characterization and control of systematic uncertainties associated to the measuring devices. In this work we explore the most conspicuous effects associated to harsh count rate conditions: dead-time and pile-up effects. Both effects, when not properly treated, can lead to large systematic uncertainties and bias in the determination of neutron cross sections. In the majority of neutron capture measurements carried out at the CERN n\_TOF facility, the detectors of choice are the C$_{6}$D$_{6}$ liquid-based either in form of large-volume cells or recently commissioned sTED detector array, consisting of much smaller-volume modules. To account for the aforementioned effects, we introduce a Monte Carlo model for these detectors mimicking harsh count rate conditions similar to those happening at the CERN n\_TOF 20~m fligth path vertical measuring station. The model parameters are extracted by comparison with the experimental data taken at the same facility during 2022 experimental campaign. We propose a novel methodology to consider both, dead-time and pile-up effects simultaneously for these fast detectors and check the applicability to experimental data from $^{197}$Au($n$,$γ$), including the saturated 4.9~eV resonance which is an important component of normalization for neutron cross section measurements.
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Submitted 2 November, 2023;
originally announced November 2023.
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Storage, Accumulation and Deceleration of Secondary Beams for Nuclear Astrophysics
Authors:
J. Glorius,
Yu. A. Litvinov,
M. Aliotta,
F. Amjad,
B. Brückner,
C. G. Bruno,
R. Chen,
T. Davinson,
S. F. Dellmann,
T. Dickel,
I. Dillmann,
P. Erbacher,
O. Forstner,
H. Geissel,
C. J. Griffin,
R. Grisenti,
A. Gumberidze,
E. Haettner,
R. Hess,
P. -M. Hillenbrand,
C. Hornung,
R. Joseph,
B. Jurado,
E. Kazanseva,
R. Knöbel
, et al. (39 additional authors not shown)
Abstract:
Low-energy investigations on rare ion beams are often limited by the available intensity and purity of the ion species in focus. Here, we present the first application of a technique that combines in-flight production at relativistic energies with subsequent secondary beam storage, accumulation and finally deceleration to the energy of interest. Using the FRS and ESR facilities at GSI, this scheme…
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Low-energy investigations on rare ion beams are often limited by the available intensity and purity of the ion species in focus. Here, we present the first application of a technique that combines in-flight production at relativistic energies with subsequent secondary beam storage, accumulation and finally deceleration to the energy of interest. Using the FRS and ESR facilities at GSI, this scheme was pioneered to provide a secondary beam of $^{118}$Te$^{52+}$ for the measurement of nuclear proton-capture at energies of 6 and 7 MeV/u. The technique provided stored beam intensities of about $10^6$ ions at high purity and brilliance, representing a major step towards low-energy nuclear physics studies using rare ion beams.
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Submitted 30 May, 2023; v1 submitted 25 May, 2023;
originally announced May 2023.
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The CERN n TOF NEAR station for astrophysics- and application-related neutron activation measurements
Authors:
N. Patronis,
A. Mengoni,
N. Colonna,
M. Cecchetto,
C. Domingo-Pardo,
O. Aberle,
J. Lerendegui-Marco,
G. Gervino,
M. E. Stamati,
S. Goula,
A. P. Bernardes,
M. Mastromarco,
A. Manna,
R. Vlastou,
C. Massimi,
M. Calviani,
V. Alcayne,
S. Altieri,
S. Amaducci,
J. Andrzejewski,
V. Babiano-Suarez,
M. Bacak,
J. Balibrea,
C. Beltrami,
S. Bennett
, et al. (108 additional authors not shown)
Abstract:
A new experimental area, the NEAR station, has recently been built at the CERN n TOF facility, at a short distance from the spallation target (1.5 m). The new area, characterized by a neutron beam of very high flux, has been designed with the purpose of performing activation measurements of interest for astrophysics and various applications. The beam is transported from the spallation target to th…
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A new experimental area, the NEAR station, has recently been built at the CERN n TOF facility, at a short distance from the spallation target (1.5 m). The new area, characterized by a neutron beam of very high flux, has been designed with the purpose of performing activation measurements of interest for astrophysics and various applications. The beam is transported from the spallation target to the NEAR station through a hole in the shielding wall of the target, inside which a collimator is inserted. The new area is complemented with a γ-ray spectroscopy laboratory, the GEAR station, equipped with a high efficiency HPGe detector, for the measurement of the activity resulting from irradiation of a sample in the NEAR station. The use of a moderator/filter assembly is envisaged, in order to produce a neutron beam of Maxwellian shape at different thermal energies, necessary for the measurement of Maxwellian Averaged Cross Sections of astrophysical interest. A new fast-cycling activation technique is also being investigated, for measurements of reactions leading to isotopes of very short half life.
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Submitted 5 September, 2022;
originally announced September 2022.
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Imaging neutron capture cross sections: i-TED proof-of-concept and future prospects based on Machine-Learning techniques
Authors:
V. Babiano-Suárez,
J. Lerendegui-Marco,
J. Balibrea-Correa,
L. Caballero,
D. Calvo,
I. Ladarescu,
C. Domingo-Pardo,
F. Calviño,
A. Casanovas,
A. Tarifeño-Saldivia,
V. Alcayne,
C. Guerrero,
M. A. Millán-Callado,
M. T. Rodríguez González,
M. Barbagallo,
O. Aberle,
S. Amaducci,
J. Andrzejewski,
L. Audouin,
M. Bacak,
S. Bennett,
E. Berthoumieux,
J. Billowes,
D. Bosnar,
A. Brown
, et al. (110 additional authors not shown)
Abstract:
i-TED is an innovative detection system which exploits Compton imaging techniques to achieve a superior signal-to-background ratio in ($n,γ$) cross-section measurements using time-of-flight technique. This work presents the first experimental validation of the i-TED apparatus for high-resolution time-of-flight experiments and demonstrates for the first time the concept proposed for background reje…
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i-TED is an innovative detection system which exploits Compton imaging techniques to achieve a superior signal-to-background ratio in ($n,γ$) cross-section measurements using time-of-flight technique. This work presents the first experimental validation of the i-TED apparatus for high-resolution time-of-flight experiments and demonstrates for the first time the concept proposed for background rejection. To this aim both $^{197}$Au($n,γ$) and $^{56}$Fe($n, γ$) reactions were measured at CERN n\_TOF using an i-TED demonstrator based on only three position-sensitive detectors. Two \cds detectors were also used to benchmark the performance of i-TED. The i-TED prototype built for this study shows a factor of $\sim$3 higher detection sensitivity than state-of-the-art \cds detectors in the $\sim$10~keV neutron energy range of astrophysical interest. This paper explores also the perspectives of further enhancement in performance attainable with the final i-TED array consisting of twenty position-sensitive detectors and new analysis methodologies based on Machine-Learning techniques.
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Submitted 18 December, 2020;
originally announced December 2020.
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s-Processing in AGB Stars Revisited. III. Neutron captures from MHD mixing at different metallicities and observational constraints
Authors:
Maurizio Busso,
Diego Vescovi,
Sara Palmerini,
Sergio Cristallo,
Vincenzo Antonuccio Delogu
Abstract:
We present post process neutron capture computations for Asymptotic Giant Branch stars of 1.5 to 3 Mo and metallicities -1.3 to 0.1. The reference stellar models are computed with the FRANEC code, using the Schwarzschild's criterion for convection. Motivations for this choice are outlined. We assume that MHD processes induce the penetration of protons below the convective boundary, when the third…
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We present post process neutron capture computations for Asymptotic Giant Branch stars of 1.5 to 3 Mo and metallicities -1.3 to 0.1. The reference stellar models are computed with the FRANEC code, using the Schwarzschild's criterion for convection. Motivations for this choice are outlined. We assume that MHD processes induce the penetration of protons below the convective boundary, when the third dredge up occurs. There, the 13C(alpha,n)16O neutron source can subsequently operate, merging its effects with those of the 22Ne(alpha,n)25Mg reaction, activated at the temperature peaks characterizing AGB stages. This work has three main scopes. i) We provide a grid of abundance yields, as produced through our MHD mixing scheme, uniformly sampled in mass and metallicity. From it, we deduce that the solar s process distribution, as well as the abundances in recent stellar populations, can be accounted for, without the need of the extra primary like contributions suggested in the past. ii) We formulate analytical expressions for the mass of the 13C pockets generated, in order to allow easy verification of our findings. iii) We compare our results with observations of evolved stars and with isotopic ratios in presolar SiC grains, also noticing how some flux tubes should survive turbulent disruption, carrying C rich materials into the winds even when the envelope is O rich. This wind phase is approximated through the G component of AGB s processing. We conclude that MHD induced mixing is adequate to drive slow neutron capture phenomena accounting for observations. Our prescriptions should permit its inclusion into current stellar evolutionary codes.
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Submitted 15 November, 2020;
originally announced November 2020.
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Review and new concepts for neutron-capture measurements of astrophysical interest
Authors:
C. Domingo-Pardo,
V. Babiano-Suarez,
J. Balibrea-Correa,
L. Caballero,
I. Ladarescu,
J. Lerendegui-Marco,
J. L. Tain,
F. Calviño,
A. Casanovas,
A. Segarra,
A. E. Tarifeño-Saldivia,
C. Guerrero,
M. A. Millán-Callado,
J. M. Quesada,
M. T. Rodríguez-González,
O. Aberle,
V. Alcayne,
S. Amaducci,
J. Andrzejewski,
L. Audouin,
M. Bacak,
M. Barbagallo,
S. Bennett,
E. Berthoumieux,
D. Bosnar
, et al. (106 additional authors not shown)
Abstract:
The idea of slow-neutron capture nucleosynthesis formulated in 1957 triggered a tremendous experimental effort in different laboratories worldwide to measure the relevant nuclear physics input quantities, namely ($n,γ$) cross sections over the stellar temperature range (from few eV up to several hundred keV) for most of the isotopes involved from Fe up to Bi. A brief historical review focused on t…
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The idea of slow-neutron capture nucleosynthesis formulated in 1957 triggered a tremendous experimental effort in different laboratories worldwide to measure the relevant nuclear physics input quantities, namely ($n,γ$) cross sections over the stellar temperature range (from few eV up to several hundred keV) for most of the isotopes involved from Fe up to Bi. A brief historical review focused on total energy detectors will be presented to illustrate how, advances in instrumentation have led, over the years, to the assessment and discovery of many new aspects of $s$-process nucleosynthesis and to the progressive refinement of theoretical models of stellar evolution. A summary will be presented on current efforts to develop new detection concepts, such as the Total-Energy Detector with $γ$-ray imaging capability (i-TED). The latter is based on the simultaneous combination of Compton imaging with neutron time-of-flight (TOF) techniques, in order to achieve a superior level of sensitivity and selectivity in the measurement of stellar neutron capture rates.
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Submitted 16 November, 2019;
originally announced November 2019.
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Plane shear flows of frictionless spheres: Kinetic theory and 3D soft-sphere discrete element method simulations
Authors:
Dalila Vescovi,
Diego Berzi,
Patrick Richard,
Nicolas Brodu
Abstract:
We use existing 3D Discrete Element simulations of simple shear flows of spheres to evaluate the radial distribution function at contact that enables kinetic theory to correctly predict the pressure and the shear stress, for different values of the collisional coefficient of restitution. Then, we perform 3D Discrete Element simulations of plane flows of frictionless, inelastic spheres, sheared bet…
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We use existing 3D Discrete Element simulations of simple shear flows of spheres to evaluate the radial distribution function at contact that enables kinetic theory to correctly predict the pressure and the shear stress, for different values of the collisional coefficient of restitution. Then, we perform 3D Discrete Element simulations of plane flows of frictionless, inelastic spheres, sheared between walls made bumpy by gluing particles in a regular array, at fixed average volume fraction and distance between the walls. The results of the numerical simulations are used to derive boundary conditions appropriated in the cases of large and small bumpiness. Those boundary conditions are, then, employed to numerically integrate the differential equations of Extended Kinetic Theory, where the breaking of the molecular chaos assumption at volume fraction larger than 0.49 is taken into account in the expression of the dissipation rate. We show that the Extended Kinetic Theory is in very good agreement with the numerical simulations, even for coefficients of restitution as low as 0.50. When the bumpiness is increased, we observe that some of the flowing particles are stuck in the gaps between the wall spheres. As a consequence, the walls are more dissipative than expected, and the flows resemble simple shear flows, i.e., flows of rather constant volume fraction and granular temperature.
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Submitted 2 June, 2014;
originally announced June 2014.