Emulating quantum entangled biphoton spectroscopy using classical light pulses
We show that for a class of quantum light spectroscopy (QLS) experiments using n= 0, 1, 2,···
classical light pulses and an entangled photon pair (a biphoton state) where one photon
acts as a reference without interacting with the matter sample, identical signals can be
obtained by replacing the biphotons with classical-like coherent states of light, where these
are defined explicitly in terms of the parameters of the biphoton states. An input-output
formulation of quantum nonlinear spectroscopy is used to prove this equivalence. We …
classical light pulses and an entangled photon pair (a biphoton state) where one photon
acts as a reference without interacting with the matter sample, identical signals can be
obtained by replacing the biphotons with classical-like coherent states of light, where these
are defined explicitly in terms of the parameters of the biphoton states. An input-output
formulation of quantum nonlinear spectroscopy is used to prove this equivalence. We …
We show that for a class of quantum light spectroscopy (QLS) experiments using n = 0, 1, 2, ··· classical light pulses and an entangled photon pair (a biphoton state) where one photon acts as a reference without interacting with the matter sample, identical signals can be obtained by replacing the biphotons with classical-like coherent states of light, where these are defined explicitly in terms of the parameters of the biphoton states. An input-output formulation of quantum nonlinear spectroscopy is used to prove this equivalence. We demonstrate the equivalence numerically by comparing a classical pump–quantum probe experiment with the corresponding classical pump–classical probe experiment. This analysis shows that understanding the equivalence between entangled biphoton probes and carefully designed classical-like coherent state probes leads to quantum-inspired classical experiments that yield equivalent signals and provides insights for the future design of QLS experiments that could provide a true quantum advantage.
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